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                  ORGANIZATION OF THIS DOCUMENT

This development document for the nonferrous metals manufacturing
category  consists  of  a  general  development  document   which
considers  the general and overall aspects of the regulation  and
31  subcategory specific supplements. These parts  are  organized
into 10 volumes as listed below.

The information in the general document and in the supplements is
organized  by sections with the same type of information reported
in  the same section of each part.  Hence to find information  on
any  specific aspect of the category one would need only look  in
the  same  section  of  the general  document  and  the  specific
supplements of interest.

The ten volumes contain contain the following subjects:

   Volume I    General Development Document
               Bauxite Refining
               Primary Aluminum Smelting
               Secondary Aluminum Smelting

               Primary Copper Smelting
               Primary Electrolytic Copper Refining
               Secondary Copper Refining
               Metallurgical Acid Plants

               Primary Zinc
               Primary Lead
               Secondary Lead
               Primary Antimony

               Primary Precious Metals and Mercury
               Secondary Precious Metals
               Secondary Silver
               Secondary Mercury

               Primary Tungsten
               Secondary Tungsten and Cobalt
               Primary Molybdenum and Rhenium
               Secondary Molybdenum and Vanadium

               Primary Beryllium
               Primary Nickel and Cobalt
               Secondary Nickel
               Secondary Tin

   Volume VIII  Primary Columbium and Tantalum
               Secondary Tantalum
               Secondary Uranium

   Volume IX   Primary and Secondary Titanium
               Primary Zirconium and Hafnium

   Volume X    Primary and Secondary Germanium and Gallium
               Primary Rare Earth Metals
               Secondary Indium
Volume II
Volume III
Volume IV
Volume V
Volume VI
Volume VII

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                DEVELOPMENT DOCUMENT

                         for

    EFFLUENT LIMITATIONS GUIDELINES AND STANDARDS

                       for the

NONFERROUS METALS MANUFACTURING POINT SOURCE  CATEGORY

                      Volume I

            General Development Document

                  William K. Reilly
                    Administrator
                   Rebecca Hanmer
      Acting Assistant Administrator  for Water
             Martha G.  Prothro,  Director
      Office of Water  Regulations  and  Standards
                        m:
            Thomas  M.  O'Farrell,  Director
           Industrial  Technology  Division
             Ernst  P.  Hall,  P.E., Chief
               Metals  Industry  Branch
                         and
              Technical  Project Officer
                      May  1989
        U.S.  Environmental  Protection Agency
                   Office of Water
      Office  of  Water  Regulations and Standards
           Industrial  Technology Division
              Washington,  D.C.  20460

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                  GENERAL DEVELOPMENT DOCUMENT
                            FOREWORD

 This  foreword briefly describes  the recent  history  of  regulations
 promulgated  for  this category and the litigation and   subsequent
 settlement    agreements    resulting  from  promulgation  of    the
 rulemakings.

 Revised   and  expanded effluent limitations  and  standards  for   the
 Nonferrous  Metals   Manufacturing   Point  Source  Category    were
 promulgated in two  separate rulemakings,  sometimes  referred to as
 Phase I  and  Phase  II.   The category was  divided into  two phases
 for    regulatory    convenience;    this division  was   generally
 consistent  with  Agency,  priorities of   regulating  first  those
 segments    which  generate  the  largest  quantities    of  toxic
 pollutants.    The   two finalized rulemakings and the three  minor
 amendments  derived from settlement agreements  are  integral parts
 of  one regulation  (40 CFR Part  421).

 The   Agency used the same overall  approach  in the development   of
 each  rulemaki.ng,  however,  certain assumptions  were made  specific
 to  each  of   the   two   phases.    These   assumptions,   which   are
 described in  this document,  were based on the best data available
 to EPA at the  time  each  phase  was  developed.

 EPA promulgated amendments  to  the  nonferrous metals manufacturing
 category  (Phase  I)  on March 8,   1984   (49  FR  8742).   Twelve
 subcategories  were  addressed at  that  time:

      1.   Primary Aluminum  Smelting
      2.   Secondary Aluminum Smelting
      3.   Primary Copper  Smelting
      4.   Primary Copper  Electrolytic  Refining
      5.   Secondary Copper
      6.   Primary Lead
      7.   Primary Zinc
      8.   Metallurgical  Acid Plants
      9.   Primary Tungsten
   ,10.   Primary Columbium-Tantalum
    11.   Secondary  Silver
    12.   Secondary  Lead

On September 20,  1985, EPA promulgated additional amendments for
the  nonferrous  metals manufacturing  category  (Phase II)  (50  FR
38276).    Twenty-five  subcategories  were  addressed  in   thTs~
amendment.

     1.   Bauxite Refining
     2.   Metallurgical Acid Plants (Molybdenum)
     3.   Primary Antimony
     4.   Primary Beryllium
     5.   Primary Boron
     6.   Primary Cesium and .Rubidium
     7.   Primary and Secondary Germanium and Gallium
     8.   Secondary  Indium
     9.   Primary Lithium
                               11

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                 GENERAL DEVELOPMENT DOCUMENT,
    10.   Primary Magnesium
    11.   Secondary Mercury
    12.   Primary Molybdenum and Rhenium
    13.   Secondary Molybdenum and Vanadium
    14.   Primary Nickel and Cobalt
    15.   Secondary Nickel
    16.   Primary Precious Metals and Mercury
    17.   Secondary Precious Metals
    18.   Primary Rare Earth Metals
    19.   Secondary Tantalum
    20.   Secondary Tin
    21.   Primary and Secondary Titanium
    22.   Secondary Tungsten and Cobalt
    23.   Secondary Uranium
    24.   Secondary Zinc
    25.   Primary Zirconium and Hafnium

After   publication   of  the  March  1984   amendments,   twelve
petitioners   filed   petitions  for  judicial  review   of   the
regulation.   These challenges were consolidated into one lawsuit
by  the  United States Court of Appeals for  the  Fourth  Circuit
(Kennecott v.  EPA, 4th Cir. No. 84-1288 and Consolidated Cases).
On December 26, 1985 the court denied the petitions for review of
the  primary lead,  primary zinc,  primary copper,  metallurgical
acid   plants,   secondary   lead  and   the   columbium-tantalum
subcategories (780 F.  2d 445).   The United States Supreme Court
denied two petitions for a writ of certiorari on October 7, 1986.

In  November,  1985  four  aluminum parties in  the  consolidated
lawsuits  entered into two settlement agreements  which  resolved
issues  raised  by  the petitioners related to  the  primary  and
secondary   aluminum  subcategories.   In  accordance  with   the
Settlement  Agreements,   EPA  published  a  notice  of  proposed
rulemaking on May 20, 1986 and solicited public comments on these
proposed  amendments  to  40 CFR Part 421  (50  FR  18530).   EPA
promulgated  these  amendments (primary  and  secondary  aluminum
subcategories) on July 7, 1987 (52 FR 25552).

On  June 26,  1986 EPA entered into a Settlement  Agreement  with
AMAX,  Inc.  and  intervenor GTE Products Corp.,  two petitioners
affected by the regulations for the Primary Tungsten Subcategory.
As a result of the settlement agreement,  EPA proposed amendments
to  the  Primary Tungsten Subcategory regulation on  January  20,
1987   (52 FR 2480).   After considering public comments  on  this
proposal, ~~EPA promulgated these amendments on January  21,  1988
(53 FR 1704).

Ten   petitioners  challenged  the  September  1985  (Phase   II)
amendments.  The  Agency  has  developed  settlement   agreements
resolving  the complaints of six petitioners;  three  petitioners
have  withdrawn their complaints and one complaint was made  moot
when  the  Agency withdrew the BPT and BAT  limitations  for  one
Subcategory    (primary  rare  :earth  metals).  These   settlement
agreements  are the basis for amendments proposed April 28,  1989
(54FR18412).
                                111

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                 GENERAL DEVELOPMENT DOCUMENT
The five amendments of greatest significance to this document are:
          Proposal

February 17, 1983 (48FR7032)
June 27, 1984 (49FR26352)
May 20, 1986 (50FR18530)
January 20, 1987 (52FR2480)
April 28, 1989 (54FR18412)
      Promulgation

March 8, 1984 (49FR 8742)
September 20, 1985 (50FR38276)
July 7, 1987 (52FR25552)
January 21, 1988 (53FR1704)
In  the preparation of this document, including the  supplements,
the administrative records or court dockets have been used as the
primary source of data and information. Obvious errors have  been
corrected and some substantial editing has been performed in some
areas,  especially where it was necessary to protect  information
claimed  to be confidential by the firm that originally made  the
information  available.  Additionally,  supplements  which   were
originally  prepared to support the March 8, 1984  and  September
20,  1985  promulgations  have been edited to  reflect  the  most
recent  amendments to the regulation. The supplements  have  also
been updated to reflect amendments to the regulations that  would
be   effective  if  the  April  1989  proposed   amendments   are
promulgated without change.

The  Agency has not substantially updated the  information  about
specific  plants or processes. It is recognized that much of  the
information  was  collected in the 1979 to 1983 period  and  that
time  may  have allowed changes to creep into the data.  This  is
unavoidable  and .should be taken into account when the  data  and
information are being used for some purposes. For most uses,  the
data should be completely useful as it defines and clarifies  the
technical basis for the nonferrous metals manufacturing  effluent
limitations and standards.

In providing this technical basis for the regulation,'the  Agency
believes  that it will be useful to industry and  permit  writing
authorities  alike  as  it provides  the  best  technical  advice
relative to the effluent standards and limitations. In an  effort
to  provide  this advice, the Agency has included  a  substantial
amount of technical data about the processes and raw  wastewaters
within the processes. Where this data was available to the Agency
but  is not provided, it has been withheld because of  claims  of
confidentiality. Additionally, where there were' pollutants  found
but  not specifically regulated, the levels at which  they  would
have  been  regulated  are  shown to  permit  a  ready  technical
evaluation in situations where wastewater streams from  different
categories  or  subcategories  are  combined  for  treatment  and
discharge.

Questions,  comments,  and corrections for this document  may  be
addressed  to  The Environmental  Protection  Agency,  Industrial
Technology Division (WH552), Washington, DC  20460.
                               IV

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                 GENERAL DEVELOPMENT DOCUMENT
                            CONTENTS

Section       Title                                      Page

I       Summary and Conclusions                              1

II      Recommendations                                     19

III     Introduction                                        21

IV      Industry Subcategorization                          33

V       Water Use and Wastewater Characteristics            39

VI      Selection of Pollutant Parameters                   49

VII     Control and Treatment Technology                   141

VIII    Cost of Wastewater Treatment and Control           285

IX      Effluent Quality Attainable Through Application    365
        of the Best Practicable Control Technology
        Currently Available

X       Effluent Quality Attainable Through Application    391
        of the Best Available Technology Economically
        Achievable

XI      New Source Performance Standards                   425

XII     Pretreatment Standards                             441

XIII    Best Conventional Pollutant Control Technology     465

XIV     Acknowledgments                                    467

XV      References                                         469

XVI     Glossary
                                v

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Table
1-1
1-2

1-3
II-l
III-l
V-l
VI-1
VI-2

VI-3
VII-1
VII-2
VII-3
VII-4
VII-5
VII-6
VII-7
VII-8
VII-9
VII-10
VII-11
VII-12
GENERAL DEVELOPMENT DOCUMENT
LIST OF TABLES


Title Page
List of Subcategories Considered
Process Wastewater Streams Identified in
Nonferrous Metals Manufacturing
Treatment Options Considered and Selected
Promulgated Effluent Limitations and Standards
Summary of DCP Respondents by Type of Metal
Processed
Distribution of Sampled Plants in the Nonferrous
Metals Manufacturing Category by Subcategories
List of 129 Priority Pollutants
Pollutants Selected for Further Consideration
by Subcategory
Polyneculear Aromatic Hydrocarbons
pH Control Effect on Metals Removal
Effectiveness of Sodium Hydroxide for
Metals Removal
Effectiveness of Lime and Sodium Hydroxide
for Metals Removal
Theoretical Solubilities of Hydroxides and
Sulfides of Selected Metals in Pure Water
Sampling Data from Sulf ide Precipitation —
Sedimentation Systems
Sulfide Precipitation — Sedimentation
Performance
Ferrite Co-Precipitation Performance
Concentration of Total Cyanide
Multimedia Filter Performance
Performance of Selected Settling Systems
Skimming Performance
Selected Partition Coefficients
7
8

16
20
32
48
126
131

143
235
235
236
236
237
238
239
239
240
240
241
241
VI

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Table
VI 1-13
VII-14
VII-15
VII-16
VII-17
VII-18
VII-19
VII-20
VII-21
VII-22
VII-23
VII-24
VII-25
VII-26
VII-27
VII-28
VIII-1
VIII-2
VIII-3
VIII-4
GENERAL DEVELOPMENT DOCUMENT
LIST OP TABLES (Continued)
Title
Trace Organic Removal by Skimming --
API Plus Belt Skimmers
Combined Metals Data Effluent Values
L&S Performance — Additional Pollutants
Combined Metals Data Set-Untreated Wastewaters
Pollutant Content of Untreated Wastewater
Precipitation-Settling-Filtration (LS&F)
Performance — Plant A
Precipitation-Settling-Filtration (LS&F)
Performance — Plant A
Precipitation-Settling-Filtration (LS&F)
Performance — Plant A
Summary of Treatment Effectiveness
Treatability Rating of Priority Pollutants
Utilizing Carbon Adsorption
Classes of Organic Compounds Asdorbed
on Carbon
Activated Carbon Performance (MERCURY)
Ion Exchange Performance
Membrane Filtration System Effluent
Peat Absorption Performance
Ultraf iltrationn Performance
BPT Cost of Compliance for the Nonferrous
Metals Manufacturing Category
BAT Cost of Compliance for the Nonferrous
Metals Manufacturing Category
PSES Costs of Compliance for the Nonferrous
Metals Manufacturing Category
Nonferrous Metals Manufacturing Phase II


Page
242
242
243
243
244
245
246
247
248
249
250
251
251
252
252
253
327
328
329
330
Category Cost Equations for Recommended
Treatment and Control Technologies
                     Vll

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                 GENERAL DEVELOPMENT DOCUMENT

                   LIST OF TABLES  (Continued)

Table                  Title                             Page

VIII-5    Components of Total Capital Investment           341

VIII-6    Components of Total Annualized Costs             342

VIII-7    Wastewater Sampling Frequency                    343

VIII-8    Cost Program Pollutant Parameters                344

VIII-9    Flow Reduction Recycle Ratio and Associated      345
          Cost Assumptions

VIII-10   Nonferrous Metals Manufacturing (Phase I)        347
          Compliance Costs —  Secondary Silver
          Subcategory

VIII-11   Nonferrous Metals Manufacturing Waste Generation 348

VIII-12   Nonferrous Metals Manufacturing Energy           349
          Consumption

IX-1      Summary of Current Treatment Practices           383

IX-2      BPT Regulated Pollutant Parameters               386

X-l       Options Considered for Each of the Nonferrous    415
          Metals Manufacturing Subcategories

X-3       Priority Pollutants Effectively Controlled by    419
          Technologies Upon Which are Based Other Effluent
          Limitations and Guidelines

X-4       Toxic Pollutants Detected but only in Trace      424
          Amounts and are neither causing nor likely to
          cause Toxic Effects

XI-1      Regulated Pollutant Parameters                   436

XII-1     Pollutants Selected for Regulation for           461
          Pretreatment Standards by Subcategory
                               VI11

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                 GENERAL DEVELOPMENT DOCUMENT

                         LIST OF FIGURES
Number               Title                                Page
                           • ' -'K; vV -       '""-.'-"''"
VII-1     Comparative Solubilities of Metal Hydroxides     254
          and Sulfide as a Function of pH

VII-2     Effluent Zinc Concentration vs. Minimum          255
          Effluent pH

VII-3     Lead Solubility in Three Alkalis                 256

VII-4     Hydroxide Precipitation Sedimentation            257
          Effectiveness — Cadmium

VII-5     Hydroxide Precipitation Sedimentation            258
          Effectiveness — Chromium

VII-6     Hydroxide Precipitation Sedimentation            259
          Effectiveness — Copper

VII-7     Hydroxide Precipitation Sedimentation            260
          Effectiveness — Lead

VII-8     Hydroxide Precipitation Sedimentation            261
          Effectiveness — Nickel and Alumimum

VII-9     Hydroxide Precipitation Sedimentation            262
          Effectiveness — Zinc

VII-10    Hydroxide Precipitation Sedimentation            263
          Effectiveness — Iron

VII-11    Hydroxide Precipitation Sedimentation            264
          Effectiveness — Manganese

VII-12    Hydroxide Precipitation Sedimentation            265
          Effectiveness — TSS

VII-13    Hexaualent Chromium Reduction with               266
          Sulfur Dioxide

VII-14    Granular Bed Filtration                          267

VII-15    Pressure Filtration                              268

VII-16    Representative Types of Sedimentation            269

VII-17    Activated Carbon Adsorption Column               270

VII-18    Centrifugation                                   271

VII-19    Treatment of Cyanide Waste by Alkaline           272
          Chlorination
                               IX

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Number
VII-20
VII-21
VII-22
VII-23
VII-24
VII-25
VII-26
VII-27
VII-28
VII-29
VII-30
VII-31
VIII-1
VIII-2
VIII-3
VIII-4
VIII-5
VIII-6
VIII-7
VIII-8
VIII-9
GENERAL DEVELOPMENT DOCUMENT
LIST OF FIGURES (Continued)
Title
Typical Ozone Plant for Waste Treatment
UV/Ozonation
Types of Evaporation Equipment
Dissolved Air Flotation
Gravity Thickening
Ion Exchange with Regeneration
Simplified Reverse Osmosis Schematic
Reverse Osmosis Membrane Configurations
Sludge Drying Bed
Simplified Ultraf iltration Flow Schematic
Vacuum Filtration
Flow Diagram for Recycling with a
Cooling Tower
General Logic Diagram of Computer Cost Model
Logic Diagram of Module Design Procedure
Logic Diagram of the Cost Estimation Routing
Capital and Annual Costs for —
Cooling Tower, Holding Tank
Capital and Annual Costs for —
Flow Equalization
Capital and Annual Costs for —
Cyanide Precipitation
Capital and Annual Costs for —
Ammonia Steam Stripping
Capital and Annual Costs for —
Oil Water Separation
Capital and Annual Costs for —


Page
273
274
275
276
277
278
279
280
281
282
283
284
350
351
352
353
354
355
356
357
358
Chemical Precipitation
                     x

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                 GENERAL DEVELOPMENT  DOCUMENT

                   LIST OF FIGURES  (Continued)


Number               Title

VIII-10   Capital and Annual Costs  for  —
          Sulfide Precipitation

VIII-11   Capital and Annueal, Cos.ts for —-
          Vacuum Filtration

VIII-12   Capital and Annual Qosts  for  —
          Holing Tanks, Recycle
   "  '                      ->i
VIII-13   Capital and Annual tC.osts  for  —
          Multimedia Filtrat^n
                           :-\&   • :
VIII-14   Capital .and Annual. Costs  for  —
          Activated Carbon Adsorption
                            ;"~v~
VIII-15   Costs for Contract "Hauling
Page

  359


  360


  361


  362


  '363


  364
                                XI

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GENERAL DEVELOPMENT DOCUMENT
              XII

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                     RE-
                            SECTION I

                             SUMMARY
The  United  States  Environmental Protection  Agency   (EPA)  has
promulgated effluent limitations and standards for the  nonferrous
metals manufacturing category pursuant to Sections 301, 304, 306,
307,  and 501 of the Clean Water Act.  The promulgated  regulation
contains   effluent  limitations  for  best  practicable  control
technology   currently  available  (BPT),   and  best   available
technology economically achievable (BAT), as well as pretreatment
standards for new and existing sources (PSNS and PSES),  and  new
source performance standards (NSPS).  ;

This development document presents the technical summary of EPA's
study  of  the nonferrous metals  manufacturing  category.   This
volume summarizes the general finding§jof the  study,   while  the
remaining   volumes  contain  supplerl||its  that  detail  specific
results for each subcategory.        Bj
                                     If^;
The Agency's economic analysis of the regulation is set forth  in
two  documents  entitled  Economic Impact  Analysis  of  Effluent
Limitations,  Guidelines  and Standards for the Nonferrous Metals
Manufacturing Point Source Category Phase I, and Phase  II.  These
documents   are  available  from  the'l Office  of  Analysis   and
Evaluation,  Economic Analysis Staff ,\,WH-586, U.S.  Environmental
Protection Agency, Washington, D.C., 20460.
                                     i '
EXISTING REGULATIONS

Since  1974,  implementation  of  the; technology-based  effluent
limitations  and  standards  has  bee,n- guided  by  a   series  of
settlement  agreements  into  which  EPA  entered  with   several
environmental groups, the latest of which occurred in 1979.  NRDC
v. Costle, 12 ERG 1833 (D.D.C. 1979), affirmed and remanded,  EOF
v. Costle, 14 ERG 2161 (1980).  Under^the settlement  agreements,
EPA was required to develop BAT limitations and pretreatment  and
new  source  performance standards for, 65 classes  of  pollutants
discharged from specific industrial point source categories.  The
list  of 65 classes was substantially expanded to a list  of  126
specific  priority  pollutants three of which  subsequently  have
been removed.                          :
                                      'V.'
METHODOLOGY                           ~~:

To  develop  the effluent limitations and standards presented  in
this   document,  the  Agency  characterized  the   category   by
subdividing  it, collecting raw and treated  wastewater  samples,
and  examining  water usage and dischargee rates,  and  production
processes.  To  gather data about the category, EPA  developed  a

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
questionnaire   (data  collection  portfolio  -  dcp)  to  collect
information  regarding  plant  size,  age  and  production,   the
production  processes  used, the quantity of  process  wastewater
used and discharged, wastewater treatment in-place, and  disposal
practices.  The dcp were sent to 540 firms (693 plants) known  or
believed to perform nonferrous smelting and refining  operations.
These  responses were reviewed, and it was determined that  there
were 450 plants among the 693 plants queried that were within the
nonferrous metals manufacturing point source category.

As  a next step,  EPA conducted a sampling and chemical  analysis
program  to characterize the raw (untreated) and treated  process
wastewater.   This program was carried out in three  stages.   In
the  first stage,  30 plants were sampled to characterize all the
significant  waste  streams  and production  processes  in  these
industries.   In  the second stage,  54 plants were  sampled,  to
expand  the data base,  and to confirm data acquired  during  the
first  phase of sampling.   The third stage consisted of a  plant
self-sampling  effort  in  which eight plants submitted  data  on
specific waste streams for which EPA had not previously  acquired
analytical  data.   These  data were used to confirm  assumptions
made  in  developing the  limitations.   Samples  were  generally
analyzed  for  124  of  the 126  priority  pollutants  and  other
pollutants  deemed appropriate.   Because no analytical .standard
was  available  for TCDD,  samples were never analyzed  for  this
pollutant,  although  there is no reason to believe that it would
be present in nonferrous metals manufacturing wastewater.    Also,
few samples were analyzed for asbestos because there is no reason
to  believe that asbestos would be present in  nonferrous  metals
manufacturing  wastewaters.   A discussion of  the  sampling  and
analytical methods and procedures is presented in Section V.

EPA   then  reviewed  the  rate  of  production  and   wastewater
generation   reported  in  the  dcp's  for   each   manufacturing
operation,  as well as the wastewater characteristics  determined
during  sampling, as the principal basis for subcategorizing  the
industry.  The  data  demonstrated that the  industry  should  be
subcategorized   by   major  metal  manufacturing   process.    A
discussion  of  the  subcategorization  scheme  is  presented  in
Section   IV.   For  this  rulemaking,  the   nonferrous   metals
manufacturing     point    source    category     includes     36
subcategories(Table 1-1, page 7).  These subcategories addressed a
total  of  63 metals and metal types including both  primary  and
secondary production.

The  nonferrous  metals manufacturing point  source  category  is
divided  into subcategories based on differences in the  quantity
and  quality  of  wastewater  generated  which  are  related   to
differences in manufacturing processes.   This has resulted in the
designation   of   31    subcategories   for   regulation.     Five
subcategories  were  excluded  from  regulation.  Primary  boron,
primary  cesium and rubidium,  primary lithium and secondary zinc
were excluded because  no plants in these subcategories  discharge
wastewater  and primary magnesium was excluded because no  plants
in   this  subcategory  discharge  treatable  concentrations   of

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
pollutants.   Each  regulated  subcategory  is further  subdivided
into  major sources of wastewater  for .specific  limitation.   The
process  wastewater streams  identified  in the  nonferrous  metals
manufacturing  category  are listed by  subcategory in  Table  1-2
(page 8).

There  are  more  than 450 plants  identified  "in  the  nonferrous
metals   manufacturing  point  source   category  discharging   an
estimated  136.2 billion liters per year of  process  wastewater.
Untreated,   this   process  wastewater  contains   approximately
3,650,000 kilograms of toxic pollutants.

The   pollutants   generated   within   the   "'nonferrous   metals
manufacturing subcategories are diverse in nature due to  varying
raw  materials  and  production  processes.   Thus,  the   Agency
examined  various  end-of-pipe and pretreatment  technologies  to
treat   the   pollutants  present  in   the   identified   process
wastewaters.  The Pollutants selected for consideration for  each
subcategory   are  presented  in  Section  VI.    The   treatment
technologies  considered for each subcategory are shown in  Table
1-3 (Page 16).

Engineering costs were prepared for each of the treatment options
considered for each subcategory.   These costs were then used  by
the  Agency  to  estimate the impact  of  implementation  of  the
various  options by the industry   For each subcategory for  each
control  and treatment option, the number of potential  closures,
number of employees affected, and impact on price were estimated.
These  results  are  reported in  the  economic  impact  analysis
document.

The  Agency then reviewed each of the treatment options for  each
subcategory to determine the estimated mass of pollutant  removed
by  the application of each treatment technology.  The  pollutant
removal  after  the application of the  treatment  technology  is
referred  to as the benefit.  The methodology used  to  calculate
the pollutant removal estimates is presented in Section X.

TECHNOLOGY BASIS FOR LIMITATIONS AND STANDARDS

In  general,  the  BPT level represents the average of  the  best
existing performances of plants of various ages, sizes, processes
or  other common characteristics.   Where existing performance is
uniformly  inadequate,  BPT may be transferred from  a  different
subcategory or category.

In  balancing  costs in relation to effluent reduction  benefits,
EPA.considers the volume and nature of existing  discharges,  the
volume  and  nature of discharges expected after  application  of
BPT,   the  general environmental effects of the  pollutants,  and
cost  and  economic  impacts of the  required  pollution  control
level.

After  examining the various treatment technologies,   the  Agency
has identified BPT to represent the average of the best  existing

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
plants.  Metals  removal  based  on  chemical  precipitation  and
sedimentation technology is the basis for the BPT limitations for
25 subcategories.  Two subcategories, primary copper smelting and
secondary  copper,  are already subject to zero discharge of  all
process wastewater pollutants.  The Agency did not promulgate BPT
requirements for three subcategories, secondary indium, secondary
mercury, and secondary nickel because these subcategories contain
no  existing  direct dischargers.   EPA  promulgated  only  minor
technical  amendments  to  the existing BPT limitations  for  the
bauxite refining subcategory.  Steam stripping is selected as the
basis  for  ammonia  limitations  in  nine  subcategories.    Air
stripping  is  selected  as  the  technology  basis  for  ammonia
limitations in one subcategory,  namely, secondary molybdenum and
vanadium.   Oil  skimming  is selected as the basis for  oil  and
grease  limitations  in three  subcategories:   primary  precious
metals and mercury, primary and secondary titanium, and secondary
tungsten  and cobalt.   Cyanide precipitation is selected as  the
technology   basis  for  cyanide  limitations  for  the   primary
beryllium,  secondary precious metals, secondary tin, and primary
zirconium and hafnium subcategories.  Ion exchange is selected as
the technology basis for gold, platinum and palladium limitations
in  the  primary  precious  metals  and  mercury,  and  secondary
precious   metals  subcategories.    Iron  co-precipitation   was
selected  as the technology basis for molybdenum  limitations  in
the  primary molybdenum and rhenium,  metallurgical acid  plants,
and secondary molybdenum and vanadium subcategories.  To meet the
promulgated BPT effluent limitations based on these technologies,
it  is estimated that the nonferrous metals manufacturing   point
source  category will incur a capital cost of $7.28 million (1982
dollars) and an annual cost of $9.3 million (1982 dollars).

The  BAT  technology  level  represents  the  best   economically
achievable   performance  of  plants  of  various  ages,   sizes,
processes    or  other  shared  characteristics.   BAT   may   be
transferred  from a different subcategory or category.   BAT  may
include feasible process changes or internal controls, even  when
not common industry practice.

In  developing  BAT,  EPA  has given substantial  weight  to  the
reasonableness  of costs.   The Agency considered the volume  and
nature  of  discharges,  the  volume  and  nature  of  discharges
expected  after  application of BAT,  the  general  environmental
effects of the pollutants,  and the costs and economic impacts of
the required pollution control levels.

Despite  this consideration of costs, the primary determinant  of
BAT  is effluent reduction capability.  For BAT, the  Agency  has
built upon the BPT technology basis by adding in-process  control
technologies  which  include recycle of process  water  from  air
pollution  control  and metal contact cooling waste  streams,  as
well  as other flow reductions, where achievable.  Filtration  is
added as an effluent polishing step to the end-of-pipe  treatment
scheme.    Implementation  of  this  technology   increases   the
reliability of the treatment system by making it less susceptible
to  operator  error  and to surges in  raw  wastewater  flow  and

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
concentrations.   Sulfide precipitation technology is  added  for
primary copper electrolytic refining, primary lead, primary zinc,
and metallurgical acid plants facilities.

To  meet  the BAT effluent limitations based on this  technology,
the  nonferrous  metals manufacturing  point source  category  is
estimated to incur a capital cost of $28.4 million (1982 dollars)
and an annual cost of $22.7 million  (1982 dollars).

New  Source Performance Standards (NSPS)  are based on  the  best
demonstrated   available  technology  (BDT),  including   process
changes,    in-plant   controls,   and   end-of-pipe    treatment
technologies  which  reduce  pollution  to  the  maximum   extent
feasible.  NSPS are equivalent to BAT for 25  subcategories.   For
three  subcategories which currently have no direct  dischargers,
BAT  was not promulgated.  For one of these,  secondary  mercury,
metals  removal based on chemical  precipitation,  sedimentation,
and filtration (the selected BAT for most of the 25 subcategories
with  direct dischargers) is the basis for NSPS limitations.  For
the secondary indium and secondary nickel subcategories  chemical
precipitation  and  sedimentation is selected as  the  basis  for
metals  removal.    In selecting NSPS, EPA  recognizes  that  new
plants  have  the  opportunity to implement  the  best  and  most
efficient  manufacturing processes and treatment  technology.  As
such,  new  source  performance standards  for  the  primary  and
secondary  titanium subcategory are equivalent to BAT  plus  zero
discharge for chip crushing, sponge crushing and screening, scrap
milling,  and chlorine liquefaction air pollution  control.   New
source performance standards for the primary aluminum subcategory
are  based on dry alumina air pollution scrubbing systems or  100
percent  recycle.  Implementation of this technology  at  primary
aluminum plants eliminates the discharge of toxic organics due to
air emission scrubbing associated.with anode paste plants,  anode
bake  plants,  potlines  and potrooms.   New  source  performance
standards for the primary lead subcategory require zero discharge
of  all  process  wastewaters  except  for  employee  hand  wash,
employee  respirator  wash,  and laundering  of  uniforms.   Zero
discharge for all other process wastewater is achievable  through
dry  slag conditioning instead of using high pressure water  jets
to granulate smelter slag.

PSES  (pretreatment standards for existing sources) are  designed
to  prevent  the  discharge of  pollutants  which  pass  through,
interfere with, or are otherwise incompatible with the operations
of  POTW.  For PSES, the Agency selected the same  technology  as
BAT,  which is BPT end-of-pipe treatment in conjunction with  in-
process  flow reduction control techniques followed  by  effluent
polishing  filtration,  for  the  secondary  aluminum,  secondary
copper,  primary lead, primary zinc, metallurgical  acid  plants,
primary  tungsten, primary columbium-tantalum,  secondary  silver,
secondary  lead,   secondary precious metals, primary  rare  earth
metals,  secondary  tin,  primary  and  secondary  titanium,  and
secondary    tungsten   and   cobalt   subcategories.     Chemical
precipitation  and  sedimentation is selected as  the  technology
basis  for  PSES  limitations  for   the, primary  and   secondary

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
germanium  and  gallium, secondary indium, and  secondary  nickel
subcategories.  The  Agency  did  not  promulgate  PSES  for  the
remaining 15 subcategories because there are no existing indirect
dischargers  in  these subcategories.  To meet  the  pretreatment
standards   for   existing   sources,   the   nonferrous   metals
manufacturing  point  source  category is estimated  to  incur  a
capital  cost of $12.2 million (1982 dollars) and an annual  cost
of $7.3 million (1982 dollars).

Pretreatment  Standards  for New Sources (PSNS) are  designed  to
prevent the discharge of pollutants which pass through, interfere
with,  or  are otherwise incompatible with the operation  of  the
POTW.   New  indirect dischargers, like new  direct  dischargers,
have   the   opportunity  to  incorporate  the   best   available
demonstrated  technologies  including process  changes,  in-plant
controls,  and  end-of-pipe treatment technologies,  and  to  use
plant   site  selection  to  ensure  adequate  treatment   system
installation.

This  regulation establishes mass-based PSNS for all 31 regulated
subcategories.    For  PSNS,  the  Agency  selected   end-of-pipe
treatment  and  in-process  flow  reduction  control   techniques
equivalent to NSPS for 28 of the subcategories and equivalent  to
PSES for the remaining three subcategories.

Non-Water Quality Environmental Impacts

Eliminating  or  reducing one form of pollution may  cause  other
environmental  problems.   Sections  304(b) and 306  of  the  Act
require  EPA  to  consider the  non-water  quality  environmental
impacts  (including energy requirements) of certain  regulations.
In compliance with these provisions, EPA considered the effect of
this  regulation on air pollution, solid waste generation,  water
scarcity, and energy consumption.

This  regulation  was reviewed by EPA personnel  responsible  for
non-water  quality  programs.   While it is difficult to  balance
pollution problems against each other and against energy use,  we
believe  that  this regulation will best  serve  often  competing
national goals.

Wastewater  treatment sludges from this category are expected  to
be  non-hazardous  by  the  E.P.Toxicity  test  under  RCRA  when
generated  using  the  model technology.   Treatment  of  similar
wastewaters  from  other  categories using  this  technology  has
resulted  in non-hazardous sludges.  Costs for disposal  of  non-
hazardous  wastes  are  included in the annual  costs.  The  only
sludges  expected  to  be hazardous under RCRA,  generated  as  a
result of wastewater treatment, are those from sulfide or cyanide
precipitation  steps. The Agency has included costs for  disposal
of those hazardous sludges in its estimates of compliance costs.

To achieve the BPT and BAT effluent limitations, a typical direct
discharger  will increase total energy consumption by  less  than
one percent of the energy consumed for production purposes.

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                            TABLE 1-1

                LIST OP SUBCATEGORIES CONSIDERED
 1.  Bauxite Refining
 2.  Primary Aluminum Smelting
 3.  Secondary Aluminum Smelting
 4.  Primary Copper Smelting
 5.  Primary Electrolytic Copper Refining
 6.  Secondary Copper
 7.  Primary Lead
 8.  Primary Zinc
 9.  Metallurgical Acid Plants
10.  Primary Tungsten
11.  Primary Columbium-Tantalum
12.  Secondary Silver
13.  Secondary Lead
14.  Primary Antimony
15.  Primary Beryllium
16.  Primary Boron
17.  Primary Cesium and Rubidium
18.  Primary and Secondary Germanium and Gallium
19.  Secondary Indium
20.  Primary Lithium
21.  Primary Magnesium
22.  Secondary Mercury
23.  Primary Molybdenum and Rhenium
24.  Secondary Molybdenum and Vanadium
25.  Primary Nickel and Cobalt
26.  Secondary Nickel
27.  Primary Precious Metals and Mercury
28.  Secondary Precious Metals
29.  Primary Rare Earth Metals
30.  Secondary Tantalum
31.  Secondary Tin
32.  -Primary and Secondary Titanium
33.  Secondary Tungsten and Cobalt
34.  Secondary Uranium
35.  Secondary Zinc
36.  Primary Zirconium and Hafnium

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                            TABLE 1-2

            PROCESS WASTEWATER STREAMS IDENTIFIED IN
                 NONFERROUS METALS MANUFACTURING

Bauxite Refining

Mud Impoundment Effluent  (Net Precipitation Discharge)

Primary Aluminum Smelting

Anode and Cathode Paste Plant Wet Air Pollution Control
Anode Bake Plant Wet Air Pollution Control
Anode Contact Cooling and Briquette Quenching
Cathode Reprocessing
Potline Wet Air Pollution Control
Potroom Wet Air Pollution Control
Direct Chill Casting
Continuous Rod Casting
Stationary Casting or Shot Casting
Degassing Wet Air Pollution Control
Pot Repair and Soaking
Spent Potliner Leachate

Secondary Aluminum Smelting

Scrap Drying Wet Air Pollution Control
Scrap Screening and Milling
Dross Washing
Demagging Wet Air Pollution Control
Delacquering Wet Air Pollution Control
Direct Chill Casting
Ingot Conveyer Casting
Stationary Casting
Shot Casting

Primary 'Copper Smelting

Slag Granulation
Casting Contact Cooling
Casting Wet Air Pollution Control

Primary Electrolytic Copper Refining

Anode and Cathode Rinsing
Spent Electrolyte
Casting Contact Cooling
Casting Wet Air Pollution Control
By-Product Recovery
                                8

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-2 (Continued)

            PROCESS WASTEWATER STREAMS IDENTIFIED IN
                 NONFERROUS METALS MANUFACTURING

Secondary Copper

Slag Milling and Classification
Smelting Wet Air Pollution Control
Casting Contact Cooling
Spent Electrolyte
Slag Granulation

Primary Lead

Sinter Plant Materials Handling Wet Air Pollution Control
Blast Furnace Slag Granulation
Blast Furnace Wet Air Pollution Control
Zinc Fuming Wet Air Pollution Control
Dross Reverberatory Slag Granulation
Dross Reverberatory Furnace Wet Air Pollution Control
Hard Lead Refining Slag Granulation
Hard Lead Refining Wet Air Pollution Control
Facility Washdown
Employee Hand Wash
Employee Respirator Wash
Laundering of Uniforms

Primary Zinc

Zinc Reduction Furnace Wet Air Pollution Control
Preleach of Zinc Concentrates
Leaching Wet Air Pollution Control
Electrolyte Bleed Wastewater
Cathode and Anode Washing
Casting Wet Air Pollution Control
Casting Contact Cooling
Cadmium Plant Wastewater

Metallurgical Acid. Plants

Acid Plant Slowdown

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            GENERAL DEVELOPMENT DOCUMENT
SECT - I
                       TABLE 1-2 (Continued)

             PROCESS WASTEWATER STREAMS IDENTIFIED IN
                  NONPERROUS METALS  MANUFACTURING

 Primary Tungsten

 Tungstic Acid Rinse
 Acid  Leach Wet Air  Pollution Control
 Alkali  Leach Wash
 Ion-Exchange Raffinate
 Calcium Tungstate Precipitate Wash
 Crystallization and Drying  of Ammonium Paratungstate
 Ammonium Paratungstate Conversion to Oxide Wet Air
   Pollution Control
 Ammonium Paratungstate Conversion to Oxides Water of
   Formation
 Reduction to Tungsten  Wet Air Pollution Control
 Reduction to Tungsten  Water of Formation
 Tungsten Powder Acid Leach  and Wash
 Molybdenum Sulfide  Precipitation Wet Air Pollution Control
 Alkali  Leach Condensate

 Primary Columbium-Tantalum

 Concentrate Digestion  Wet Air Pollution Control
 Solvent Extraction  Raffinate
 Solvent Extraction  Wet Air  Pollution Control
 Precipitation  and Filtration  of Metal  Salts
 Precipitation  and Filtration  Wet Air Pollution Control
 Tantalum Salt  Drying
 Reduction of Tantalum  Salt  to Metal
 Reduction of Tantalum  Salt  to Metal Wet Air Pollution
   Control
 Oxides  Calcining  Wet Air Pollution  Control
 Tantalum Powder Wash
 Consolidation  and Casting Contact Cooling

 Secondary Silver
 Film Stripping
 Film Stripping Wet Air Pollution Control
 Precipitation  and Filtration  of Film Stripping Solutions Wet
  Air Pollution Control
 Precipitation  and Filtration  of Film Stripping Solutions
 Precipitation  and Filtration  of Photographic Solutions
 Precipitation  and Filtration  of Photographic Solutions Wet
  Air Pollution Control
 Electrolytic Refining
 Furnace Wet Air Pollution Control
 Leaching
 Leaching Wet Air Pollution Control
 Precipitation of Nonphotographic Solutions Wet Air Pollution
  Control
Precipitation and Filtration of Nonphotographic Solutions
Floor and Equipment  Washdown
                               10

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           GENERAL DEVELOPMENT  DOCUMENT
SECT - I
                       TABLE  1-2  (Continued)

            PROCESS WASTEWATER STREAMS  IDENTIFIED IN
                 NONFERROUS  METALS MANUFACTURING

 Secondary Lead

 Battery Cracking
 Blast, Reverberatory,  and Rotary Furnace Wet Air  Pollution
  Control
 Kettle Wet Air Pollution Control
 Casting Contact Cooling
 Lead Paste Desulfurization
 Truck Wash
 Facility Washdown
 Battery Case Classification
 Employee Hand Wash
 Employee Respirator Wash
 Laundering of Uniforms

 Primary Antimony

 Sodium Antimonate Autoclave  Wastewater
 Fouled Anolyte
 Cathode Antimony Washwater

 Primary Beryllium

 Solvent Extraction Raffinate from Bertrandite Ore
 Solvent Extraction Raffinate from Beryl Ore
 Beryllium Carbonate Filtrate
 Beryllium Hydroxide Filtrate
 Beryllium Oxide Calcining Furnace Wet Air Pollution  Control
 Beryllium Hydroxide Supernatant
 Process Water
 Fluoride Furnace Scrubber
 Chip Treatment Wastewater
 Beryllium Pebble Plant Area-Vent .Wet Air Pollution Control
 Beryl Ore Gangue Dewatering
 Bertrandite Ore Gangue Dewatering
 Beryl Ore Processing
 AIS Area Wastewater
 Bertrandite Ore Leaching Scrubber
 Bertrandite Ore Counter Current
  Decantation Scrubber

 Primary and Secondary Germanium and Gallium

 Still Liquor
 Chlorinator Wet Air Pollution Control
Germanium Hydrolysis Filtrate
Acid Wash and Rinse Water
Gallium Hydrolysis Filtrate
 Solvent Extraction Raffinate
                               11

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-2 (Continued)

            PROCESS WASTEWATER STREAMS IDENTIFIED IN
                 NONFERROUS METALS MANUFACTURING '
Secondary Indium

Displacement Tank Supernatant
Spent Electrolyte

Secondary Mercury

Spent Battery Electrolyte
Acid Wash and Rinse Water
Furnace Wet Air Pollution Control
Primary Molybdenum and Rhenium

Molybdenum Sulfide Leaching
Roaster S02 Scrubber
Molybdic Oxide Leachate
Hydrogen Reduction Furnace Scrubber
Depleted Rhenium Scrubbing Solution

Secondary Molybdenum and Vanadium

Leach Tailings
Molybdenum Filtrate Solvent Extraction Raffinate
Vanadium Decomposition Wet Air Pollution Control
Molybdenum Drying Wet Air Pollution Control
Pure Grade Molybdenum

Primary Nickel and Cobalt

Raw Material Dust Control
Nickel Wash Water
Nickel Reduction Decant
Cobalt Reduction Decant

Secondary Nickel

Slag Reclaim Tailings
Acid Reclaim Leaching Filtrate
Acid Reclaim Leaching Belt Filter Backwash
                               12

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-2 (Continued)

            PROCESS WASTEWATER STREAMS IDENTIFIED IN
                 NONFERROUS METALS MANUFACTURING

Primary Precious Metals and Mercury

Smelter Wet Air Pollution Control
Silver Chloride Reduction Spent Solution
Electrolytic Cells Wet Air Pollution Control
Electrolyte Preparation Wet Air Pollution Control
Calciner Wet Air Pollution Control
Calciner Quench Water
Calciner Stack Gas Contact Cooling Water
Mercury Calcining Condensate
Mercury Cleaning Bath Water

Secondary Precious Metals

Furnace Wet Air Pollution Control
Raw Material Granulation
Spent Plating Solutions
Spent Cyanide Stripping Solutions
Retinery Wet Air Pollution Control
Gold Solvent Extraction Raffinate and Wash Water
Gold Spent Electrolyte
Gold Precipitation and Filtration
Platinum Precipitation and Filtration Palladium Precipitation and
Filtration   Other  Platinum  Group  Metals   Precipitation   and
Filtration Spent Solution from PGC Salt Production Equipment  and
Floor Wash
Preliminary Treatment

Primary Rare Earth Metals

Dryer Vent Water Quench and Scrubber
Dryer Vent Caustic Wet Air Pollution Control
Electrolytic Cell Water Quench and Scrubber
Electrolytic Cell Caustic Wet Air Pollution Control
Sodium Hypochlorite Filter Backwash

Secondary Tantalum

Tantalum Alloy Leach and Rinse
Capacitor Leach and Rinse
Tantalum Sludge Leach and Rinse
Tantalum Powder Acid Wash and Rinse
Leaching Wet Air Pollution Control
                               13

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-2  (Continued)

            PROCESS WASTEWATER STREAMS  IDENTIFIED  IN
                 NONPERROUS METALS MANUFACTURING

Secondary Tin

Tin Smelter SO2 Scrubber
Dealuminizing Rinse
Tin Hydroxide Wash
Tin Mud Acid Neutralization Filtrate
Spent Electrowinning Solution from New  Scrap
Spent Electrowinning Solution from Municipal Solid Waste
Tin Hydroxide Supernatant from Scrap
Tin Hydroxide Supernatant from Spent Flating Solutions and
  Sludges
Tin Hydroxide Filtrate

Primary and Secondary Titanium

Chlorination Off-Gas Wet Air Pollution  Control
Chlorination Area-Vent Wet Air Pollution Control
TiCl4 Handling Wet Air Pollution Control
Reduction Area Wet Air Pollution Control
Melt Cell Wet Air Pollution Control
Chlorine Liquefaction Wet Air Pollution Control
Sodium Reduction Container Reconditioning Wash Water
Chip Crushing Wet Air Pollution Control
Acid Leachate and Rinse Water
Sponge Crushing and Screening Wet Air Pollution Control
Acid Pickle and Wash Water
Scrap Milling Wet Air Pollution Control
Scrap Detergent Wash Water
Casting Crucible Wash Water
Casting Contact Cooling Water

Secondary Tungsten and Cobalt                           ,

Tungsten Detergent Wash and Rinse
Tungsten Leaching Acid
Tungsten Post-Leaching Wash and Rinse
Synthetic Scheelite Filtrate
Tungsten Carbide Leaching Wet Air Pollution Control
Tungsten Carbide Wash Water
Cobalt Sludge Leaching Wet Air Pollution Control
Crystallization Decant         ;
Acid Wash Decant
Cobalt Hydroxide Filtrate
Cobalt Hydroxide Filter Cake Wash
                               14

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-2 (Continued)

            PROCESS WASTEWATER STREAMS IDENTIFIED IN
                 NONFERROUS METALS MANUFACTURING

Secondary Uranium

Refinery Sump Filtrate
Slag leach Reslurry
Solvent Extraction Raffinate Filtrate
Digestion Wet Air Pollution Control
Evaporation and Denitration Wet Air Pollution Control
Hydrofluorination Alkaline Scrubber
Hydrofluorination Water Scrubber
Magnesium Reduction and Casting Floor Wash Water
Laundry Wastewater

Primary Zirconium and Hafnium

Sand Drying Wet Air Pollution Control
Sand Chlorination Off-Gas Wet Air Pollution Control
Sand Chlorination Area-Vent Wet Air Pollution Control
SiCl4 Purification Wet Air Pollution Control
Feed Make-up Wet Air Pollution Control
Iron Extraction (MIBK) Steam Stripper Bottoms
Zirconium Filtrate
Hafnium Filtrate
Calcining Caustic Wet Air Pollution Control
Pure Chlorination Wet Air Pollution Control
Reduction Area-Vent Wet Air Pollution Control
Magnesium Recovery Off Gas We.t Air Pollution Control
Magnesium Recovery Area-Vent Wet Air Pollution Control
Zirconium Chip Crushing Wet Air Pollution Control
Acid Leachate from Zirconium Metal Production
Acid Leachate from Zirconium Alloy Production
Leaching Rinse Water from Zirconium Metal Production
Leaching Rinse Water from Zirconium Alloy Production
                               15

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                            TABLE 1-3

            TREATMENT OPTIONS CONSIDERED AND SELECTED
                                 Treatment Technology Options
  Subcategory
Bauxite Refining
Primary Aluminum Smelting
Secondary Aluminum Smelting

Primary Copper Smelting
Primary Copper Electrolytic
  Refining
Secondary Copper

Primary Lead
Primary Zinc
Metallurgical Acid Plants

Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver

Secondary Lead
Primary Antimony
Primary Beryllium

Primary Boron
Primary Cesium and Rubidium
Primary and Secondary
  Germanium and Gallium

Secondary Indium
Secondary Mercury
Primary Molybdenum and
  Rhenium

Secondary Molybdenum and
  Vanadium
Primary Nickel and Cobalt
Secondary Nickel

Primary Precious Metals
  and Mercury
Secondary Precious Metals
Primary Rare Earth Metals
Considered
A

X
g X
X
C X
X
X
X
X
X
X
X
X
X
X
X
m X
X
X
X
X
X
X
X
X
X
X
B

X
X

X

X
X
X
X
X
X
X







X



X
X
X
C E
X
X
X
X
X
X
X
X
X
X X
X X
X X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X X
Selected
BPT
ZD
-
—
—
—
-
A
-
A
A
A
A
A
A
A
—
_
A
__
-
A
A
A
—
A
A
-
BAT
ZD
C
C
ZD
C
ZD
C
C
C
C
C
C
C
C
C
_
_
A
—
-
C
C
C
—
C
C
-
NSPS
ZD
C
C
ZD
C
ZD
C
C
C
C
C
C
C
C
C
_
-
A
A
C
C
C
C
A
C
C
C
                               16 '

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           GENERAL DEVELOPMENT DOCUMENT
SECT - I
                      TABLE 1-3 (Continued)

            TREATMENT OPTIONS CONSIDERED AND SELECTED
                                 Treatment Technology Options
  Subcategory
Considered
A B
X
X
nium X X
X X
X
X
C E
X
X
X
X
X
X
Selected
BPT
A
A
A
A
A
A
BAT
C
C
C
C
C
C
NSPS
C
C
C
C
C
C
Secondary Tantalum
Secondary Tin
Primary and Secondary Titanium  X

Secondary Tungsten and
  Cobalt
Secondary Uranium
Primary Zirconium and
  Hafnium

Notes: Option  A - Chemical precipitation and  sedimentation  and
       sulfide   precipitation,   iron   co-precipitation,    ion
       exchange,  cyanide  precipitation, ammonia  steam  or  air
       stripping,  activated  carbon adsorption or  oil  skimming
       where appropriate.

       Option B - Option A preceded by flow reduction by
       recycling variable quantities of process wastewater.

       Option C - Option B plus filtration.

       Option E - Option C plus activated carbon adsorption.

       ZD  -  No discharge allowance for  pollutants  in  process
       wastewater discharged.
                               17

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GENERAL DEVELOPMENT DOCUMENT
SECT - I
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                    18

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           GENERAL DEVELOPMENT DOCUMENT
SECT - II
                           SECTION II

                           CONCLUSIONS
The  nonferrous  metals manufacturing point source  category  has
been  divided into thirty six subcategories, thirty one of  which
are regulated by this regulation. The Agency concluded that  five
of  the  subcategories should not be regulated at this  time  and
that  the  remaining  thirty one should be  subject  to  effluent
limitations and standards published in the Federal Register.  For
some  of  the subcategories, limitations or  standards  were  not
developed  for  existing  sources because there  were  either  no
direct discharging or no indirect discharging sources. Table II-l
(Page  20)  lists  all of the  regulated  subcategories  and  the
limitations  and standards promulgated within  each  subcategory.
BCT limitations are not promulgated for any subcategory.

Section  II  of  the  development document  supplement  for  each
specific  subcategory  contains  a  tabulation  of  the  specific
numerical limitations and standards for that subcategory.
                               19

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GENERAL DEVELOPMENT
DOCUMENT

SECT - II


TABLE II-l
PROMULGATED EFFLUENT
Subcategory
Bauxite Refining
Primary Aluminum Smelting
Secondary Aluminum Smelting
Primary Copper Smelting
Primary Electrolytic
Copper Refining
Secondary Copper
Primary Lead
Primary Zinc
Primary Tungsten
Primary Columbium & Tantalum
Secondary Silver
Secondary Lead
Primary Antimony
Primary Beryllium
Primary and Secondary
Germanium and Gallium
Secondary Indium
Secondary Mercury
Primary Molybdenum and Rhenium
Metallurgical Acid Plants
Secondary Molybdenum and
Vanadium
Primary Nickel and Cobalt
Secondary Nickel
Primary Precious Metals
Mercury
Secondary Precious Metals
Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin
Primary and Secondary
Titanium
Secondary Tungsten and Cobalt
Secondary Uranium
Primary Zirconium and Hafnium
LIMITATIONS AND STANDARDS
BPT
X
X
X
X
X

X
.X
X
. X
X
X
X
X
X
X



X
X
X

X

X

X

X
X
X

X
X
X
BAT
X
X
X
X
X

X
X
X
X
X
X
X
X
X
X



X
X
X

X

X

X

X
X
X

X
. X
X
NSPS
X
X
X
X
X

X
X
X
X
X
X
X
X
X
X

X
X
X
X
X

X
X
X

X
X
X
X
X

X
X
X
PSES

X
X
X


X
X
X
X
X
X
X
X



X


X



X


X
X

X
X

X


PSNS

X
X
X
X

X
X
X
X
X
X
X
X
X
X

X
X
X
X
X

X
X
X

X
X
X
X
X

X
X
X
20

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
                           SECTION III

                          INTRODUCTION
PURPOSE AND AUTHORITY

The  Federal  Water  Pollution Control  Act  Amendments  of  1972
established a comprehensive program to "restore and maintain  the
chemical,  physical,  and biological integrity  of  the  Nation's
waters,"  Section 101(a).  By July 1, 1977,  existing  industrial
dischargers  were  required  to  achieve  "effluent   limitations
requiring  the  application  of  the  best  practicable   control
technology currently available" (BPT), Section 301(b)(1)(A).   By
July     1,  1984,  these dischargers were  required  to  achieve
"effluent  limitations  requiring  the application  of  the  best
available technology economically achievable — which will result
in  reasonable  further  progress toward  the  national  goal  of
eliminating  the  discharge  of all  pollutants"  (BAT),  Section
301(b)(2)(A).  New industrial direct dischargers were required to
comply with Section 306 new source performance standards  (NSPS),
based  on  best available demonstrated technology;  and  new  and
existing  dischargers  to publicly owned treatment  works  (POTW)
were subject to pretreatment standards under Sections 307(b)  and
(c)  of the Act. The requirements for direct dischargers were  to
be  incorporated  into National Pollutant  Discharge  Elimination
System  (NPDES)  permits  issued under Section 402  of  the  Act.
Pretreatment  standards  were made enforceable  directly  against
dischargers to POTW (indirect dischargers).

Although Section 402(a)(l) of the 1972 Act authorized the setting
of  requirements for direct dischargers on a case-by-case  basis,
Congress intended that,  for the most part,  control requirements
would be based on regulations promulgated by the Administrator of
EPA.   Section  304(b)  of the Act required the Administrator  to
promulgate regulations providing guidelines for effluent  limita-
tions  setting forth the degree of effluent reduction  attainable
through  the  application of BPT  and  BAT.   Moreover,  Sections
304(c)  and  306 of the Act required promulgation of  regulations
for  NSPS,  and  Sections 304(f),  307(b),  and  307(c)  required
promulgation  of  regulations  for  pretreatment  standards.   In
addition to these regulations for designated industry categories,
Section   307(a)  of  the  Act  required  the  Administrator   to
promulgate  effluent standards applicable to all  dischargers  of
toxic pollutants.   Finally, Section 501(a) of the Act authorized
the   Administrator  to  prescribe  any  additional   regulations
"necessary to carry out his functions" under the Act.

EPA  was  unable to promulgate many of -these regulations  by  the
dates  contained  in the Act.  In 1976, EPA was sued  by  several
environmental groups, and in settlement of this lawsuit, EPA  and
the  plaintiffs  executed  a  "Settlement  Agreement"  which  was
approved  by the District Court.  This Agreement required EPA  to
develop a program and adhere to a schedule for promulgating,  for
                               21

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
 21   major   industries,  BAT  effluent   limitations    guidelines,
 pretreatment standards, and new  source performance standards  for
 65  "priority" pollutants and classes of  pollutants.   See  Natural
 Resources  Defense  Council, Inc..v. Train,  8  ERG   2120  (D.D.C.
 1976),   modified,  12  ERG  1833   (D.D.C.   1979),   modified   by
 additional orders of August 25,  1982, October  26, 1982, August 2,
 1983 and January 6, 1984.

 On  December  27,  1977,  the President signed into law the Federal
 Water Pollution Control Act (P.L.   95-217),  commonly referred to
 as  the  Clean     Water Act of  1977.    Although this law  makes
 several  important     changes   in  the   federal  water  pollution
 control   program,   its  most      significant  feature   is   it
 incorporates into the Act several    of  the  basic elements of the
 Settlement  Agreement  program   for    toxic pollutant  control.
 Sections 301(b)(2)(A) and 301(b)(2)(C)    of the Act  now  require
 the achievement of effluent limitations  requiring BAT for "toxic"
 pollutants,  including  the  65     "pollutants  and   classes   of
 pollutants  which Congress declared "toxic"  under Section  307(a)
 of  the Act.  Likewise, EPA's programs for new source  performance
 standards and pretreatment standards are now aimed principally at
 toxic  pollutant  controls.  Moreover, to strengthen   the  toxics
 control  program,  Section  304(e)  of   the  Act  authorizes  the
 Administrator  to prescribe "best management practices" (BMP)  to
 prevent the release of toxic and hazardous pollutants  from  plant
 site  runoff,  spillage or leaks, sludge or  waste  disposal,  and
 drainage from raw material storage associated with, or  ancillary
 to, the manufacturing or treatment process.

 The  1977  Amendments  added  Section 301(b)(2)(E)  to  the  Act,
 establishing  "best  conventional pollutant  control  technology"
 (BCT)    for discharges of conventional pollutants from  existing
 industrial  point  sources.   Conventional pollutants  are  those
mentioned      specifically  in  Section  304(a)(4)   (biochemical
 oxygen  demanding     pollutants (BOD )  total  suspended  solids
 (TSS)   fecal coliform,  and pH),  and any additional  pollutants
defined  by the Administrator as "conventional."  (To  date,  the
Agency has added one such pollutant, oil and grease,   44 FR 44501,
July  30,  1979.)   before establishing them as BCT.    In no case
may BCT be less stringent than BPT.

BCT  is  not  an additional limitation but replaces BAT  for  the
control of conventional pollutants.  In addition to other factors
 specified  in  Section 304(b)(4)(B),  the Act requires  that  BCT
 limitations   be   assessed  in  light  of  a   two-part   "cost-
 reasonableness" test,   American Paper Institute v.  EPA, 660 F.2d
954  (4th  Cir.  1981).   The first test compares  the  cost  for
private  industry to reduce its conventional pollutants with  the
costs  to  publicly owned treatment works for similar  levels  of
reduction  in  their discharge of these pollutants.    The  second
test  examines  the cost-effectiveness of  additional  industrial
treatment  beyond  BPT.   EPA  must  find  that  limitations  are
 "reasonable" under both tests.
                               22

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - III
EPA  published its methodology for carrying out the BCT  analysis
on August 29,  1979 (44 FR 50372).   In the case mentioned above,
the  Court of Appeals ordered EPA to correct data errors underly-
ing EPA's calculation of the first test, and to apply the  second
cost  test.   (EPA  had argued that a second cost  test  was  not
required.)

A revised methodology for the general development of BCT  limita-
tions was proposed on October 29, 1982 (47 FR 49176), but had not
been  promulgated  as  a  final rule  when  this  regulation  was
promulgated.   We  accordingly  have not proposed BCT limits  for
plants in the nonferrous metals manufacturing category.  We  will
await  establishing  nationally applicable BCT  limits  for  this
industry until promulgation of the final methodology for BCT.

For   nonconventional  pollutants,  Sections   301(b)(2)(A)   and
(b)(2)(F) require achievement of BAT effluent limitations  within
three years after their establishment or July 1, 1984,  whichever
is later, but not later than July 1, 1987.

The purpose of these promulgated regulations is to provide efflu-
ent  limitations  guidelines for BPT and BAT,  and  to  establish
NSPS,  pretreatment  standards for existing sources  (PSES),  and
pretreatment  standards  for new sources (PSNS),  under  Sections
301, 304, 306, 307, and 501 of the Clean Water Act.

PRIOR EPA REGULATIONS
EPA previously promulgated effluent limitations and  pretreatment
standards    for   certain   nonferrous   metals    manufacturing
                 The nonferrous metals manufacturing  regulations
                 to the present rulemaking effort  (Phase  I  and
                 the technological basis  for  them  are  briefly
subcategories.
existing  prior
Phase  II)  and
discussed below.
Bauxite  Refining Subcategory.  EPA promulgated BPT,  BAT,  NSPS,
and PSNS in this subcategory (39 FR 12822, March 26, 1974).  BPT,
BAT,  NSPS  and  PSNS were based on  zero  discharge  of  process
wastewater,  but allow for a monthly net precipitation  discharge
from the red mud impoundment.

Primary  Aluminum Subcategory.  EPA promulgated BPT,  BAT,  NSPS,
and PSNS in this subcategory (39 FR 12822, March 26, -1974).   BPT
was  based  on lime precipitation and  sedimentation  technology.
BAT  was  based on this technology and flow reduction;  NSPS  and
PSNS were based on BPT plus additional flow reduction.

Secondary  Aluminum  Subcategory.   Existing regulations in  this
subcategory cover BPT,  BAT,  NSPS,  PSES and PSNS   (39 FR 12822
(March   26,   1974)  and  41  FR  54854  (December   15,   1976)
(establishing  pretreatment standards)).   BPT was based on  lime
precipitation  and  sedimentation with pH adjustment  to  control
ammonia.   BAT  required no discharge of  wastewater  pollutants,
PSES  was  based on oil skimming,  pH adjustment and ammonia  air
stripping,  while NSPS and PSNS were based on lime  precipitation
                               23

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            GENERAL DEVELOPMENT DOCUMENT
SECT - III
 and sedimentation and flow reduction.   (Promulgated NSPS and PSNS
 were  less   stringent  than BAT and PSES  because   the   processes
 believed to be necessary to achieve zero discharge were not  yet
 demonstrated in 1974  or 1976,  but  it was believed  that  they  would
 be  demonstrated  at   the  time of the  BAT  and  PSES   compliance
 dates.)

 Primary  Copper  Smelting.   The  existing  regulation  covered BPT and
 BAT.  The amended BPT  required  no discharge of  process   wastewater
 pollutants  subject to an  exception for  unlimited discharge of the
 volume of water falling within impoundments in excess of the  10-
 year,  24-hour storm (known as  a catastrophic precipitation event)
 when  a   storm  of at  least that magnitude occurred.   See 45  FR
 44926  (July 2,  1980).  Existing BAT, promulgated  earlier (40  FR
 8523 (February  27,  1975)),  was less stringent  than BPT,   allowing
 as exemptions to zero discharge a  similar unlimited discharge for
 stormwater  (except the  allowance is for  a volume of wastewater  in
 excess   of   a 25-year,  10-hour storm),  and  a  further   discharge
 during   any  calendar  month equal in volume  to   the   difference
 between   precipitation  on and evaporation from  the impoundment
 during    that   month.   This  latter  discharge  is subject   to
 concentration-based limitations.

 Primary  Electrolytic  Copper  Refining.  Existing regulations  cover
 BPT and BAT.    The BPT regulation for  this subcategory  allowed a
 mass-based   continuous  discharge based on lime precipitation and
 sedimentation.    45 FR  44926 (July 2, 1980).  The  BAT regulation,
 promulgated earlier   (40   FR   8524  (February  27,   1975))  was
 impoundment rather  than hardware-based,   and established  a   mass-
 based  continuous  discharge  limitation,   based on  flow  reduction,
 lime precipitation,   sedimentation,  and  the same  allowances  for
 catastrophic stormwater discharge  and net  precipitation discharge
 described   for primary  copper   smelting,   previously.    (Refiners
 located   in areas  of  net evaporation,  however,  cannot discharge
 process  wastewaters,  based  on the  use of  solar evaporation.  The
 monthly  net  precipitation  and  catastrophic  discharges  may  be
 discharged.)

 Secondary   Copper.    EPA  established BPT,   BAT and  PSES^  in   this
 subcategory.   BPT  and BAT,  based on the presence  of impoundments
 (or  cooling tower  circuits),   required no  discharge  of  process
 wastewater pollutants with allowances for  catastrophic stormwater
 discharge and net precipitation  discharge  as described above when
 impoundments are used instead  of cooling tower circuits.   See 40
 FR  8526  (February  27,  1975).   PSES,  promulgated  later  (41  FR
 54854  (December 15,  1976)) was based on  lime precipitation  and
 sedimentation.

 Primary  Lead.   The  existing  BPT and BAT  limitations  in  this
 subcategory  were based on impoundments.    See 40' FR  (February 27,,
 1975).   These  limitations  required ,no  discharge  of  process
wastewater pollutants, with exemptions for catastophic stormwater
and  net  precipitation discharge of acid plant blowdown   (subject
 to   mass   limitations)  and  monthly   net   precipitation   on
 impoundments.   The existing limitations did not  apply to primary
                               24

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - III
lead refineries not oh-site with a smelter.

Primary  Zinc.   EPA promulgated BPT and BAT in this subcategory.
See 40 FR 8528 (February 21, 1975).  This limitation was based on
lime  precipitation  and sedimentation technology for  BPT,  with
flow reduction added for BAT.
                                                          i
Metallurgical Acid Plants.   This subcategory was established  in
1980,  and  at that time included only acid plants (i.e.,  plants
recovering  by-product sulfuric acid from sulfur dioxide  smelter
air  emissions)  associated with primary copper  smelting  opera-
tions.   (See  45 FR 44926.)  Primary lead and zinc  plants  also
have   associated   acid  plants;  the   applicability   of   the
metallurgical  acid  plants subcategory was expanded  to  include
these  sources and was finalized on March 8, 1984 (49  FR  8742).
EPA  further  expanded the existing regulation for  metallurgical
acid  plants by modifying the applicability of the  metallurgical
acid plants subcategory to include molybdenum acid plants.

METHODOLOGY

Approach of_ Study

The  nonferrous  metals manufacturing category  comprises  plants
that  process  ore concentrates and scrap metals to  recover  and
increase  the  metal  purity contained in  these  materials.  The
promulgated  effluent  limitations and standards  for  nonferrous
metals  manufacturing addresses 31 subcategories (See Table  1-3,
page 15).

The  31 subcategories in nonferrous metals manufacturing  contain
38 primary metals and metal groups, 24 secondary metals and metal
groups,  and bauxite refining.  A group of metals— including six
primary  metals  and five secondary  metals—were  excluded  from
regulation  either because the manufacturing processes do not use
           because they are regulated by toxics  limitations  and
           in other categories (e.g.,  ferroalloys and  inorganic
              Four  of  these  metals which  were  excluded  from
            on May 10,  1979 — primary  antimony,  primary  tin,
           molybdenum,  and secondary tantalum — have since been
reconsidered  based  on information received during  more  recent
data  collection efforts.   EPA also studied the segments of  the
nonferrous  metals . industry associated with forming  or  casting
nonferrous  metals.   EPA  promulgated regulations  for  aluminum
forming (48 FR 49126) in October, 1983; for copper forming (48 FR
36942)  in August,  1983;  for metal molding and casting   (50  FR
45212) October, 1985; and  for forming of nonferrous metals other
than aluminum and copper  (50 FR 34242) in August, 1985.

In  the course of developing these,guidelines,  EPA gathered  and
evaluated technical data  in order:to perform the following tasks:

 1.   To  profile  the category with regard  to  the  production,
manufacturing  processes,  geographical  distribution,  potential
wastewater  streams,  and  discharge  mode of . nonferrous  metals
water  or
standards
chemicals) .
regulation
secondary
                               25

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
manufacturing plants.

  2.    To  subcategorize,    if  necessary,   in  order  to  permit
regulation of the nonferrous metals manufacturing category in  an
equitable and manageable way.

  3.  To characterize wastewater, detailing water use, wastewater
discharge,  and  the  occurrence  of  toxic,  conventional,  and
nonconventional  pollutants,  in  waste streams  from  nonferrous
metals manufacturing processes.

  4.     To    select   pollutant   parameters   — those   toxic,
nonconventional,    or   conventional   pollutants   present   at
significant  concentrations  in wastewater streams — that  should
be considered for regulation.

  5.   To  consider control and treatment technologies and  select
alternative  methods  for reducing pollutant  discharge  in  this
category.

  6.   To  evaluate  the costs  of  implementing  the  alternative
control and treatment technologies.

  7.  To present regulatory alternatives.

Data Collection and Methods of Evaluation

Data  on the nonferrous metals manufacturing category were  gath-
ered from previous EPA studies,  literature studies, inquiries to
federal and state environmental agencies,  trade association con-
tacts and the manufacturers themselves.   Meetings were also held
with  industry representatives and the EPA.   All known companies
within  the  nonferrous metals manufacturing category . were,  sent
data  collection portfolios to solicit specific information  con-
cerning each facility.   Finally,  a sampling program was carried
out  at 84 plants.   Wastewater samples were collected  in  three
phases.  In the first phase, 30 plants were sampled in an attempt
to,_ characterize all the significant waste streams and.  production
processes in these segments. In the second phase, 46 plants  were
sampled  to expand the data base, and to confirm  data   acquired
during the first phase of sampling.  The third stage consisted of
a  plant  self-sampling effort, in which eight  plants  submitted
data  on specific waste streams for which EPA had not  previously
acquired  analytical  data.   These data  were  used  to  confirm
assumptions  made  in developing the limitations.   Samples  were
generally analyzed for 124 of the 126 toxic pollutants and  other
pollutants  deemed appropriate.  Because no  analytical  standard
was  available  for TCDD, samples were never  analyzed  for  this
pollutant,  although there is no reason that it would be  present
in  nonferrous metals manufacturing wastewafcer. Asbestos was  not
analyzed for in any of the samples because there was no reason to
believe  it  would be present in wastewater  resulting  from  the
manufacture  of nonferrous metals.  At least one plant  in  every
major subcategory was sampled during the data collection  effort,
with some subcategories sampled at more than one plant, when  the
                               26

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           GENERAL DEVELOPMENT DOCUMENT
                                SECT - III
production processes were different.

Specific details of the sampling program and information from the
above data sources are presented in Section V.  Details on selec-
tion  of plants for sampling,  and analytical results,  are  con-
tained in Section V of each of the subcategory supplements.

Literature  Review.
 	    EPA reviewed and evaluated existing litera-
background information to clarify and  define  various
                                               and  to
ture  for
aspects  of the nonferrous metals manufacturing category
determine  general characteristics and trends in production  pro-
cesses  and wastewater treatment technology.  Review  of  current
literature continued throughout the development of these  limita-
tions  and  standards.  Information gathered in this  review  was
used,  along  with information from other  sources  as  discussed
below, in the following specific areas:

   Subcategory Profile (Section III of each of the subcategory
   supplements) - Description of production processes and the
   associated raw materials and wastewater streams.

   Subcategorization (Section IV of each of the subcategory
   supplements) - Identification of differences in manufac-
   turing process technology and their potential effect on
   associated wastewater streams.

   Selection of Pollutant Parameters (Section VI) - Infor-
   mation regarding the toxicity and potential sources of
   the pollutants identified in wastewater from nonferrous
   metals manufacturing processes.

   Control and Treatment Technology (Section VII) - Infor-
   mation on alternative controls and treatment and
   corresponding effects on pollutant removal.

   Costs (Section VIII) - Formulation of the methodology
   for determining the current capital and annual costs to
   apply the selected treatment alternatives.

Existing Data.   Previous EPA studies of the following nonferrous
metals manufacturing subcategories were reviewed:

Primary Aluminum
Secondary Aluminum
Primary Copper
Secondary Copper
Primary Lead
Primary Zinc
Secondary Lead
Primary Columbium-Tantalum                             .
Primary Beryllium
Primary and Secondary Germanium
Primary Magnesium
Secondary Zinc                                                  ;
Primary Zirconium and Hafnium
                               27

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
The  available  information  included a summary of  the  category
describing    the    production   processes,    the    wastewater
characteristics  associated  with  the   processes,   recommended
pollutant  parameters requiring control;  applicable  end-of-pipe
treatment technologies for wastewaters;  effluent characteristics
resulting  from  this treatment",  and a background  bibliography.
Also  included  in  these studies were  detailed  production  and
sampling information for many plants.

The  concentration  or  mass loading of pollutant  parameters  in
wastewater  effluent  discharges are monitored  and  reported  as
required  by individual state agencies.   Where available,  these
historical  data were obtained from NPDES monitoring reports  and
reviewed.

Other  useful  data  sources were industry  personnel  and  trade
associations.  Contributions from these sources were particularly
useful  for  clarifying  differences  in  production   processes.
Finally, general information was derived from publications of the
U.S.  Bureau  of  Mines,  including  the  Minerals  Yearbook  and
supplements,  and  through discussions with commodity experts  at
the U.S. Bureau of Mines.

Data Collection Portfolios.  EPA conducted a survey of the non-
ferrous   metals  manufacturing  plants  to  gather   information
regarding plant size, age and production, the production  proces-
ses  used, economic parameters, and the quantity, treatment,  and
disposal of wastewater generated at these plants.  This  informa-
tion was requested in data collection portfolios (dcp) mailed  to
all  companies  known  or believed to belong  to  the  nonferrous
metals  manufacturing  category.   A  listing  of
comprising  the  nonferrous  metals industry  .(as
standard  industrial  code numbers) was  compiled
trade associations and the U.S. Bureau of Mines.
        the  companies
        classified  by
        by  consulting
In all,  dcp were sent to 540 firms (693 plants).  In some cases,
companies  contacted were not actually members of the  nonferrous
metals  manufacturing  category as it is defined by  the  Agency.
Where  firms  had nonferrous metals manufacturing  operations  at
more than one location, a dcp was returned for each plant.

If the dcp was not returned, information on production processes,
sources  of  wastewater and treatment technology at these  plants
was  collected  by  telephone  interview.    The  information  so
gathered  was  validated  by sending a copy  of  the  information
recorded to the party consulted.   The information was assumed to
be correct as recorded if no reply was received in 30  days.   In
total,  more than 99 percent of the category was contacted either
by mail or by telephone.

A  total of 450 dcp applicable to the nonferrous metals  manufac-
turing  category were returned.   A breakdown of these facilities
by type of metal processed is presented in Table III-l (page 32).
                               28

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
The dcp responses were interpreted individually, and the follow-
ing data were documented for future reference and evaluation:

   Company name, plant address, and name of the contact
   listed in the dcp.

   Plant discharge status as direct (to surface water),
   indirect (to POTW), or zero discharge.

   Production process and waste streams present at the
   plant, as well as associated flow rates; production
   rates; operating hours; wastewater treatment, reuse,
   or disposal methods; and the quantity and nature of
   process chemicals.

   Capital and annual wastewater treatment costs.

   Availability of pollutant monitoring data provided by the
   plant.

The  summary listing of this information provided  a  consistent,
systematic   method  of  evaluating  and  summarizing   the   dcp
responses.   In addition, procedures were developed  to  simplify
subsequent analyses, which had the following capabilities:

   Selection and listing of plants containing specific pro-
   duction process streams or treatment technologies.

   Summation of the number of plants containing specific
   process waste streams and treatment combinations.

   Calculation of the percent recycle present for specific
   waste streams and summation of the number of plants
   recycling these waste streams within various percent
   recycle ranges.

   Calculation of annual production values associated with
   each process stream and summation of the number of plants
   with these process streams having production values
   within various ranges.

   Calculation of water use and discharge from individual
   process streams.

The  calculated information and summaries were used in developing
these effluent limitations and standards.  Summaries were used in
the category profile, evaluation of subcategorization, and analy-
sis  of in-place treatment- and control technologies.   Calculated
information  was used in the .determination of water use and  dis-
charge  values for the conversion of pollutant concentrations  to
mass loadings.

GENERAL PROFILE OF THE NONFERROUS METALS MANUFACTURING CATEGORY

The  nonferrous metals manufacturing point source category encom-
                               29

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
passes  the  primary smelting and refining of  nonferrous  metals
(Standard Industrial Classification  (SIC) 333) and the  secondary
smelting and refining of nonferrous metals (SIC 334).   The cate-
gory does not include the mining and concentration of ores, roll-
ing/  drawing,  or extruding of metals, or scrap metal collection
and preliminary grading.

Nonferrous  metal manufacturers include processors of ore concen-
trates  or  other virgin materials (primary)  and  processors  of
scrap (secondary).  Metals produced as by- or co-products of pri-
mary metals are themselves considered primary metals.   For exam-
ple, rhenium recovered from primary molybdenum roaster flue gases
is considered to be primary rhenium, rather than secondary. Table
III-l  (page 32) summarizes the nonferrous  metals  manufacturers
studied by the type of metal processed.

The nonferrous metals manufacturing category is quite complex and
the  production  process for a specific metal is dictated by  the
characteristics  of raw materials,  the economics  of  by-product
recovery, and the process chemistry and metallurgy of the metals.

Employment  data are given in the dcp responses for  456  plants.
These plants report a total of 74,500 workers involved in nonfer-
rous  metals manufacturing plants.   Industry production  figures
show  that  bauxite refining and primary aluminum  dominates  the
industry  in  terms of tonnage.   Other subcategories with  large
production figures are primary copper, lead, zinc and molybdenum.

Two  hundred  thirteen  plants  (47 percent)  indicated  that  no
wastewater  from  nonferrous metals manufacturing  operations  is
discharged to either surface waters or a POTW.   Of the remaining
243  plants,   112  (25  percent)  discharge  an  effluent   from
nonferrous  metals manufacturing directly to surface waters,  and
131 (28 percent) discharge indirectly,  sending nonferrous metals
manufacturing effluent through a POTW.

EPA  recognizes  that plants sometimes combine process  and  non-
process  wastewater prior to treatment and discharge.   Pollutant
discharge  allowances will be established under  this  regulation
only for nonferrous metals manufacturing process wastewater,  not
the nonprocess wastewaters.  The nonprocess flows and  wastewater
characteristics  are  a function of the plant  layout  and  water
handling  practices.   As  a  result,  the  pollutant   discharge
effluent  limitation  for nonprocess wastewater streams  will  be
prepared  by  the permitting authority.  A discussion  of  how  a
permit  writer  would  construct a permit  for  a  facility  that
combines wastewater is presented in Section IX.

Section  III  of each of the subcategory supplements  presents  a
detailed  profile of the plants in each subcategory and describes
the production processes involved.   In addition,  the  following
specific information is presented:

1.  Raw materials,
2.  Manufacturing process,
                               30

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
3.  Geographic locations of manufacturing plants,
4.  Age of plants by discharge status,
5.  Production ranges by discharge status, and
6.  Summary of waste streams for each process.
                               31

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           GENERAL DEVELOPMENT DOCUMENT
SECT - III
                           Table III-l

      SUMMARY OP DCP RESPONDENTS BY TYPE OF METAL PROCESSED
Subcategory
         Number
        of Plants
Bauxite Refining
Primary Aluminum Smelting
Secondary Aluminum Smelting
Primary Copper Smelting
Primary Electrolytic Copper Refining
Secondary Copper
Primary Lead
Secondary Lead
Primary Zinc
Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Metallurgical Acid Plants
Primary Antimony
Primary Beryllium
Primary and Secondary Germanium and Gallium
Secondary Indium
Secondary Mercury
Primary Molybdenum and Rhenium
Secondary Molybdenum and Vanadium
Primary Nickel and Cobalt
Secondary Nickel
Primary Precious Metals and Mercury
Secondary Precious Metals
Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin
Primary-and Secondary Titanium
Secondary Tungsten and Cobalt
Secondary Uranium
Primary Zirconium and Hafnium
           8
          33
          59
          21
          17
          31
           9
          73
           8
          18
           5
          81
          29
           8
           2
           5
           1
           4
           9
           1
           1
           2
           8
          49
           4
           3
          12
           8
           6
           3
           3
TOTAL
         521
                               32

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IV
                           SECTION IV

                   INDUSTRY SUBCATEGORIZATION
Subcategorization  should  take into account  pertinent  industry
characteristics,  manufacturing  process  variations,  wastewater
characteristics,  and  other factors.  Effluent  limitations  and
standards  establish mass limitations on the discharge of  pollu-
tants which are applied, through the permit issuance process,  to
specific  dischargers.   To  allow the national  standard  to  be
applied to a wide range of sizes of production units, the mass of
pollutant  discharge must be referenced to a unit of  production.
This factor is referred to as a production normalizing  parameter
and is developed in conjunction with Subcategorization.

Division of the category into subcategories provides a  mechanism
for  addressing  process and product variations which  result  in
distinct wastewater characteristics.  The selection of production
normalizing  parameters  provides the means for compensating  for
differences  in production rates among plants with similar  prod-
ucts  and processes within a uniform set of  mass-based  effluent
limitations and standards.

This  Subcategorization analysis is actually an ongoing  process.
The  first  subcategories  (bauxite  refining,  primary  aluminum
smelting,  and secondary aluminum smelting) were established in a
1973 Agency rulemaking.  Since that time, some subcategories have
been  modified.   New  subcategories were added in 1975 and  then
again in 1980.

A comprehensive analysis of each factor that might warrant  sepa-
rate  limitations for different segments of the industry has  led
the  Agency to promulgate the following Subcategorization  scheme
for  BPT and BAT effluent limitations guidelines and PSNS,   PSES,
and  NSPS in the nonferrous metals manufacturing  category.  (See
listing in Table V-l, page 48)

Most   of   these  subcategories  are  further   segmented   into
subdivisions  for the development of effluent limitations;   these
subdivisions  are  enumerated and discussed  in  the  subcategory
supplements to this document.

SUBCATEGORIZATION BASIS

Technology-based  effluent  limitations are based primarily  upon
the  treatability of pollutants in wastewaters generated  by  the
category under review.    The treatability of these pollutants is,
of  course,   directly related to the flow and characteristics  of
the  untreated wastewater,   which in turn can be affected by fac-
tors inherent to a processing plant in the category.    Therefore,
these factors and the degree to which each influences  wastewater
flow  and characteristics form the basis  for Subcategorization of
the category,   i.e.,   those factors which have a strong influence
                               33

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IV
on  untreated wastewater flow and characteristics are applied
the category to subcategorize it in an appropriate manner.

The  list of potential subcategorization factors  considered
the nonferrous metals manufacturing category include:

    Metal products, co-products, and by-products;
    Raw materials:
    Manufacturing processes;
    Product form;
    Plant location;
    Plant age;
    Plant size;
    Air pollution control methods;
    Meteorological conditions;
    Treatment costs;
    Solid waste generation and disposal;
    Number of employees;
    Total   energy   requirements  (manufacturing
      wastewater treatment and control); and
    Unique plant characteristics.
                    to
                   for
         process   and
For the reasons discussed below, the metal or other products, the
raw materials,  and the manufacturing process were discovered  to
have  the greatest influence on wastewater  flow  characteristics
and  treatability, and thus ultimately on the appropriateness  of
effluent   limitations.   These  three  factors  were   used   to
subcategorize  the  category.  As mentioned  previously,  further
division of some subcategories is warranted based on the  sources
of waste waters (manufacturing processes) within the plant.  Each
manufacturing  process generates differing amounts of  wastewater
and  in some instances specific waste streams contain  pollutants
requiring  preliminary treatment to reduce concentrations of  oil
and  grease,  ammonia,  cyanide,  and  toxic  organics  prior  to
combined treatment.  Thus, each subcategory is further subdivided
based  on the manufacturing processes used.   These  subdivisions
are discussed in the appropriate supplement.

Metal Products, Co-Products, and By-Products

The  metal  products,  co-products,  and by-products is the  most
important factor in identifying subcategories for this  category.
Subcategorizing  on  this basis is consistent with  the  existing
division of plants,  i.e., plants are identified as (and identify
themselves as) nickel plants,  tin plants,  titanium plants, etc.
The  production  of each metal is based on its own raw  materials
and production processes, which directly affect wastewater volume
and characteristics.

In  nonferrous metals manufacturing,  production and refining  of
metal  by-products and co-products generally will be  covered  by
means  of subcategorization with the major metal product.   There
are several examples of this.   EPA found that production of  the
co-product  metals  primary zirconium and hafnium are  inherently
allied,  so  both were considered in a single  subcategory.   The
                               34

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IV
same  is true for primary molybdenum and  rhenium,  primary  nickel
and cobalt, primary precious metals and  mercury, and primary rare
earth metals.   Secondary cobalt  is a by-product of the secondary
tungsten manufacturing process, thus, the two are placed together
in one subcategory.

Raw Materials

The   raw materials used (ore concentrates or scrap) in nonferrous
metals manufacturing determine the reagents used, and to a  large
extent the wastewater characteristics.   Raw materials are  signi-
ficant  in differentiating between primary and secondary  produc-
ers.  It is therefore selected as a basis for  subcategorization.
In  some cases  (e.g., primary  and secondary titanium),  the  raw
material  differences did not warrant separate  subcategorization
due to common processing steps or other  factors.

Manufacturing Processes

The   production  processes  for each metal  are  unique  and  are
affected  by the raw materials used and  the type of end  product.
The processes used will,  in turn,  affect the volume and charac-
teristics of the resulting wastewater.

The   processes  performed (or the air pollution controls used  on
the   process  emissions) in the production of  nonferrous  metals
determine the amount and characteristics of. wastewater  generated
and   thus  are a logical basis for the establishment of  subcate-
gories.   In  this category,  however,   similar processes may  be
applied to differing raw materials in the production of different
metals yielding different wastewater characteristics.    For exam-
ple,  molybdenum, precious metals, and tin may all be produced by
roasting.   As a result of these considerations, specific process
operation  was  not generally found to be suitable as  a  primary
basis for subcategorization.   However,  process variations which
result  in significant differences in wastewater  generation  are
reflected  in the allowances for discrete unit operations  within
each  subcategory  (see  the  discussion of  building  blocks  in
Section IX).

In  the  case of primary  copper  manufacturing,  the  production
processes   used  are  deemed  to  be  a  reasonable  basis   for
subcategorization,  even  though  these processes  are  sometimes
practiced  at a single site.   This resulted in the establishment
of the primary copper smelting subcategory and the primary copper
electrolytic  refining subcategory (see Section IV of the  Primary
Copper Supplement).  This is consistent with the structure of the
category  since  smelting  and refining are  often  conducted  at
different sites.

Product Form

This factor becomes important when the final product from a plant
is actually an intermediate that another plant purchases and pro-
cesses  to render the metal in a different form.    An  example  of
                               35

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           GENERAL DEVELOPMENT, DOCUMENT    SECT - IV


this is the production of  molybdenum,  which some plants produce
by reducing molybdenum trioxide (Mo03),  an intermediate that may
have been produced by another plant.   This practice, however, is
not  found  to  be  common in the  category  and  its  effect  on
wastewater  volume and total subcategory raw waste generation  is
not as significant as the factors chosen.

Plant Location

Most  plants  in  the category are  located  near  raw  materials
sources,  transportation centers, markets, or sources of inexpen-
sive energy.  While larger primary copper, lead, zinc, molybdenum
and  titanium  producers  are mainly found near  Mid-western  and
Western ores and are remote from population centers, proximity to
shipping  lanes in the lower Mississippi region is important  for
bauxite refiners.   Secondary producers,  on the other hand,  are
generally   located   in  or  near  large   metropolitan   areas.
Therefore,  primary  producers often have more land available for
treatment systems than secondary producers.   Plant location also
may  be  significant because evaporation ponds can be  used  only
where  solar evaporation is feasible and where sufficient land is
available.   However,  location  does  not  significantly  affect
wastewater  characteristics or! treatability, and  thus  different
effluent limitations are not warranted based on this factor.

Plant Age

Plants   within  a  given  subcategory  may  have   significantly
different  ages  in terms of initial operating year.   To  remain
competitive, however, plants must be constantly modernized.

Plants may be updated by modernizing a particular  component,  or
by installing new components.   For example, an old furnace might
be  equipped  with oxygen lances to increase the  throughput,  or
replaced entirely by a new,  more efficient furnace.   Moderniza-
tion of production processes and air pollution control  equipment
produces  analogous  wastes  among all plants producing  a  given
metal, despite the^. original plant start-up date.  While the rela-
tive age of a plan't may be important in considering the  economic
impact of a guideline, as a subcategorization factor it does  not
account  for differences in the raw  wastewater  characteristics.
For  these  reasons,  plant age is not selected as  a  basis  for
subcategorization.

Plant Size

The  size of a plant generally does not affect either the produc-
tion methods or the wastewater characteristics.   Generally, more
water  is used at larger plants.   However,  when water  use  and
discharge are normalized on a production basis,  no major differ-
ences  based on plant size are found within the same subcategory.
Thus,  plant  size is not selected as a basis for  subcategoriza-
tion.
                               36

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IV
Air Pollution Control Methods

Many  facilities  use wet scrubbers to  control  emissions  which
influence wastewater characteristics.  In some cases, the type of
air pollution control equipment used provides a basis for regula-
tion,  because if wet air pollution control is used, an allowance
may be necessary for that waste stream,  while a plant using only
dry  systems does not need an allowance for a non-existent  waste
stream.   Therefore, this factor is often selected as a basis for
subdivision within some subcategories (i.e., developing an allow-
ance  for this unit operation as part of the limitation or  stan-
dard for the subcategory), but not as a means for subcategorizing
the category.

Meteorological Conditions

Climate  and precipitation may affect the feasibility of  certain
treatment  methods,  e.g.,  solar evaporation through the use  of
impoundments is a feasible method of wastewater treatment only in
areas of net evaporation.   This factor was not selected for sub-
categorization,  however,  because  the differences in wastewater
characteristics  and treatability are better explained  by  other
factors  such  as  metal products  and  manufacturing  processes.
Therefore,  different  effluent limitations based on this  factor
are not warranted.

Solid Waste Generation and Disposal

Physical and chemical characteristics of solid waste generated by
the  nonferrous  metals  category  are  determined  by  the   raw
material,  process,  and  type  of air pollution control in  use.
Therefore,  this  factor  does not provide a  primary  basis  for
subcategorization.

Number of Employees

The  number of employees in-a plant does not directly  provide  a
basis  for subcategorization because the number of employees does
not directly affect the production or process water usage rate at
any plant.  Because the amount of process wastewater generated is
related to the production rates rather than employee number,  the
number of employees does.not provide a definitive relationship to
wastewater generation.

Total Energy Requirements

Total  energy requirements was not selected as a basis  for  sub-
categorization primarily because energy requirements are found to
vary widely within this category and are not meaningfully related
to wastewater generation and pollutant discharge.   Additionally,
it  is  often difficult to obtain reliable energy estimates  spe-
cifically  for production and waste treatment.   When  available,
estimates are likely to include other energy requirements such as
lighting, air conditioning, and heating or cooling energy.
                               37

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IV
Unique Plant Characteristics

Unique plant characteristics such as land availability and  water
availability  do not provide a proper basis for subcategorization
because they do not materially affect the raw wastewater  charac-
teristics of the plant.  Process water availability may indeed be
a function of the geography of a plant.   However,  the impact of
limited  water  supplies is to encourage conservation by  recycle
and  efficient  use  of  water.   Therefore,  insufficient  water
availability  only tends to encourage the early  installation  of
practices  that are advisable for the entire category in order to
reduce treatment costs and improve pollutant removals.

Limited  land  availability for constructing  a  waste  treatment
facility  may  affect the economic impact of an effluent  limita-
tion.   The availability of land for treatment,  however, is gen-
erally  not a major issue in the nonferrous metals  manufacturing
category.   Most  primary plants are located on very large  sites
and  land availability would not be a  factor.   While  secondary
producers  tend to be located in more urban settings,  the amount
of  land  available to them for treatment is sufficient  for  the
types of treatment and control technologies considered.

PRODUCTION NORMALIZING PARAMETERS

To ensure equitable regulation of the category,  effluent  guide-
lines limitations and standards of performance are established on
a production-related basis (i.e., a mass of pollutant per unit of
production).   In addition, by using these mass-based limitations
the total mass of pollutants discharged is minimized.  The under-
lying  premise for mass-based limitations is that pollutant load-
ings and water discharged from each process are correlated to the
amount of material produced by that process.  This correlation is
calculated as the mass of pollutant or wastewater discharged  per
unit of production.  The units of production are known as produc-
tion  normalizing parameters (PNPs).   The type and value of  the
PNPs  vary according to the subcategory or subdivision.   In  one
case . it  may be the total mass of metal produced from that  line
while  in others it may be some other  characteristic  parameter.
Two  criteria  are  used in selecting the appropriate PNP  for  a
given  subcategory or subdivision:  (1) maximizing the degree  of
correlation between the production of metal reflected by the  PNP
and  the corresponding discharge of pollutants, and (2)  ensuring
that  the  PNP  is  easily  measured  and  feasible  for  use  in
establishing regulations.

The   production  normalizing  parameter  identified   for   each
subcategory  or subdivision,   and the rationale used in selection
are  discussed  in  detail  in  Section  IV  of  the  appropriate
supplements.
                               38

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GENERAL DEVELOPMENT DOCUMENT
                                           SECT - V
              SECTION V

 WATER USE AND WASTEWATER CHARACTERISTICS
                                             category.
                                            production
                                             presented
This  section  presents  the data collection  and  data  analysis
methods   used  for  characterizing  water  use  and   wastewater
associated  with  the nonferrous metals  manufacturing
Raw  waste  and  treated effluent  sample  data,  and
normalized water use and wastewater discharge data are
in Section V of each of the subcategory supplements.

DATA SOURCES

Historical Data

A  useful  source of long-term or historical data  available  for
nonferrous   metals   manufacturing  plants  are  the   Discharge
Monitoring  Reports (DMR's) completed as a part of  the  National
Pollutant  Discharge Elimination System (NPDES).   All applicable
DMR's  were obtained through the EPA regional offices  and  state
regulatory  agencies  for the year 1982, the last  complete  year
prior  to  the proposal of the first segment (Phase  I)  of  this
regulation for which information was available.  These data  were
available  from 14 nonferrous metals manufacturing  plants.   The
DMR's  present a summary of the analytical results from a  series
of  samples  taken  during  a  given  month  for  the  pollutants
designated in the plant's permit.  In general, minimum,  maximum,
and  average values, in mg/1 or Ibs/day, are presented  for  such
pollutants  as total suspended solids, aluminum, oil and  grease,
pH,  copper, and zinc. The samples are collected from  the  plant
outfall(s),  which  represents the discharge(s) from  the  plant.
For  facilities  with wastewater treatment, the DMR's  provide  a
measure  of the performance of the treatment system.  In  theory,
these data could then serve as a basis for characterizing treated
wastewater from nonferrous metals manufacturing plants;  however,
there  is  no  influent to treatment  information  (i.e.,  paired
influent-effluent  data)  and  too  little  information  on   the
performance  of the plant at the time the samples were  collected
to  be  the preferred source of data  in  formulating  achievable
performance  for various types of treatment.  They do serve as  a
set   of  data  that  can  be  used  to  verify  the   technology
performances  presented  in Section VII,  Control  and  Treatment
Technology  (Table  VII-21, page 248).  DMR data from  12  plants
with lime precipitation and sedimentation treatment were used  as
a  check  on  the achievability of  the  treatment  effectiveness
concentrations  used to establish the limitations and  standards.
These  DMR  data  and  a comparison  of  them  to  the  treatment
effectiveness  concentrations  are found in the  record  of  this
rulemaking.

Data Collection Portfolios

Information on plant location and size, number of employees, dis-
                    39

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
charge status,  production processes and  quantities,  wastewater
sources  and flows,  treatment system processes,  operations  and
costs,  economic information, and pollutant characterization data
was solicited in the data collection portfolio  (dcp).

Two  of the most important items are the production processes and
quantities and the associated flows.   These data were evaluated,
and two flow-to-production ratios were calculated for each stream
in each subcategory.   The two ratios,  water use and  wastewater
discharge flow, are differentiated by the flow  value used in cal-
culation.   Water  use is defined as the volume of water or other
fluid required for a given process per mass of metal product  and
is  therefore based on the sum of recycle and make-up flows to  a
given  process.   Wastewater  flow discharged  after  preliminary
treatment  or  recycle   (if these are present)  is the  volume  of
wastewater discharged from a given process to further  treatment,
disposal, or discharge per mass of metal produced. The production
values  used  in this calculation correspond  to  the  production
normalizing parameter, PNP, assigned to each stream, as  outlined
in Section IV of each of the subcategory supplements.  This value
is  most  often the amount of metal processed by  each  operation
that generates a wastewater.

The production normalized water use and discharge flows were com-
piled and summarized for each stream.  The flows are presented in
Section V of each of  the subcategory supplements.   Where appro-
priate,  an  attempt  was  made to identify  factors  that  could
account  for variations in water use.   The flows for each stream
were evaluated to establish BPT, BAT, NSPS, and pretreatment dis-
charge flows.  These are used in calculating the effluent limita-
tions and standards in Sections IX, X, XI, and XII of each of the
subcategory supplements.

The  regulatory  production normalized discharge flows were  also
used to estimate flows at nonferrous metals manufacturing  plants
that supplied EPA with only production data in their dcp.  Actual
discharge flows,  or estimated flows, when an actual flow was not
reported  in ,_the dcp,  were then used to determine the  cost  of
various wastewater treatment options at these facilities.

Sampling and Analysis Program

The  sampling and analysis program discussed in this section  was
undertaken to collect specific data to implement the requirements
of  the 1977 amendments to the Act and to identify pollutants  of
concern  in  the  nonferrous metals  manufacturing  point  source
category,    with  emphasis  on  toxic  pollutants.  EPA  and  its
contractors  collected  and analyzed samples from  84  nonferrous
metals manufacturing facilities.

This  section  summarizes the purpose of the sampling  trips  and
identifies the parameters analyzed.   It also presents an overview
of   sample   collection,    preservation,   and   transportation
techniques.    Finally,   it  describes  the  pollutant  parameters
quantified,   the  methods of analyses and laboratories used,   the
                               40

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
detectable  concentration  of each  pollutant,  and  the  general
approach  used  to ensure the reliability of the analytical  data
produced.

Site  Selection.   Information gathered in  the  data  collection
portfolios  was used to select sites for wastewater sampling  for
each  subcategory.   The  plants  sampled  were  selected  to  be
representative of each subcategory.  Considerations included  how
well  each facility represented the subcategory as  indicated  by
available  data, potential problems in  meeting  technology-based
standards,  differences in production processes used, number  and
variety of unit operations generating wastewater, and  wastewater
treatment  in  place.  Additional details on site  selection  are
presented in Section V of each of the subcategory supplements.

Field Sampling.   After plants to be sampled were selected,  each
plant   was  contacted  by  telephone,   and  sent  a  letter  of
notification  as  to  when  a  visit  would  be  expected.  These
telephone inquiries disclosed facility information necessary  for
efficient  on-site  sampling.   Based on  this  information,  the
sources  of wastewater to be sampled at each plant were selected.
The sample points included,  but were not limited  to,  untreated
and treated discharges, process wastewater, and partially treated
wastewater.

During this program,  84 nonferrous metals manufacturing  plants
were sampled.  The distribution of these plants^by subcategory is
presented in Table V-l (page 48).

Wastewater samples were collected in three stages.   In the first
stage,  30  plants were sampled in an attempt to characterize all
the  significant waste streams and production processes in  these
industries.   In the second stage,  46 plants were sampled  in an
attempt  to fill any gaps in the data base,  and to confirm  data
.acquired during the first phase of sampling.  In the third stage,
EPA  conducted a small plant self-sampling effort  under  Section
308 of the Clean Water-Act. In this effort eight plants submitted
data  on specific waste streams for which EPA had not  previously
acquired  analytical  data.   These  data were  used  to  confirm
assumptions  made by EPA in developing the limitations.   Samples
were generally analyzed for 124 (excluding TCDD and asbestos)  of
the 126 toxic pollutants and other pollutants deemed appropriate.
Because  no analytical standard was available for  TCDD,  samples
were  never  analyzed for this pollutant,  although there  is  no
reason   that   it   would  be  present  in   nonferrous   metals
manufacturing  wastewater.  Also,  no samples were  analyzed  for
asbestos  because  there  is no reason to believe  that  asbestos
would be present in wastewater resulting from the manufacture  of
nonferrous metals.  At least one plant in every major subcategory
was  sampled  during  the  data  collection  effort,   with  some
subcategories  sampled at more than one plant,  when the  produc-
tion processes were different.

To reduce the volume of data handled,  avoid unnecessary expense,
and direct the scope of the sampling program,  analyses were only
                               41

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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - V
 performed   for  pollutants   expected  to  be present  in  a  plant's
 wastewater.   Two  sources of information were  used  for  selecting
 the  analyzed pollutants:   the pollutants that industry   believes
 or knows are present  in  their wastewater, and  the pollutants   the
 Agency believes could be present after studying  the processes  and.
 materials   used by the industry.   If  industry  and the Agency   did
 not  believe  a  pollutant  or class of pollutants   likely  to  be
 present  in the   wastewater after  studying   the   processes   and
 materials   used/ analyses for that pollutant were not  completed.

 The 126 toxic pollutants were listed  in  each dcp and each  facil-
 ity  was asked to  indicate  for each particular pollutant  whether
 it  was  known to  be  present or believed to be present.   If   the
 pollutant had been analyzed for and detected,  the facility  was to
 indicate that it was  known  to be present.   If the  pollutant   had
 not  been analyzed,   but might be present in the wastewater,   the
 facility was to indicate that it was  believed  to be present.   The
 reported  results   are tabulated in Section V  of the  subcategory
 supplements.

 Sample Collection,  Preservation,  and   Transportation.   Samples
 were  collected,   preserved,  and transported  in accordance  with
 procedures  outlined  in Appendix III of "Sampling  and   Analysis
 Procedures  for  Screening  of Industrial Effluents  for   Priority
 Pollutants"   (published by the  Environmental  Monitoring   and
 Support Laboratory,   Cincinnati, Ohio, March 1977,  revised, April
 1977),  "Sampling   Screening Procedure  for  the  Measurement  of
 Priority  Pollutants" (published by the  EPA  Effluent  Guidelines
 Division, Washington, D.C.,  October 1976), Handbook for   Sampling
 and Sample  Preservation  of  Water and Wastewater  (published  by  the
 Environmental  Monitoring   and  Support  Laboratory,  Cincinnati,
 Ohio,  September 1982) and  in "Methods for Chemical  Analysis  of
 Water  and  Wastes",  USEPA,  EMSL, Cincinnati,  Ohio  45268,  EPA-
 600/4-79-020   (March    1983);  "Guidelines    Establishing   Test
 Procedures  for the Analysis of Pollutants Under the Clean  Water
 Act",'  49   PR  43234  (October  26,  1984).   The  procedures  are
 summarized  below.

 Whenever practical,   all samples collected at  each  sampling point
 were  taken from mid-channel at mid-depth in a   turbulent,  well-
 mixed portion of the waste  stream.   Periodically, the temperature
 and pH of each waste  stream  sampled were measured onsite.

 Before  collection  of  automatic composite  samples,  new  Tygon
 tubing was cut to minimum lengths and installed on  the inlet  and
 outlet (suction and discharge) fittings  of the automatic  sampler.
 Two  liters  (2.1  quarts)  of blank water, known to  be   free  of
 organic  compounds  and  brought to the  sampling  site  from  the
 analytical  laboratory,  were pumped through the sampler   and  its
 attached tubing into a 3.8 liter (1 gallon)  glass jug;  the  water
 was  then  distributed  to   cover the interior  of  the   jug  and
 subsequently discarded.

A field blank sample was produced by pumping an additional  three
 liters  (0.8  gal)   of blank water  through the sampler  into  the
                               42

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - V
glass jug.   The blank sample was sealed with a Teflon-lined cap,
labeled,  and  packed  in ice in a plastic foam-insulated  chest.
This sample subsequently was analyzed to determine any contamina-
tion contributed by the automatic sampler.

Each  large composite (Type 1) sample was collected in a 10-liter
(2.6  gallon)  wide-mouth  glass jar that had  been  washed  with
detergent and water, rinsed with tap water, rinsed with distilled
water  and  then  methylene  chloride,  and  air  dried  at  room
temperature in a dust-free environment.

During  collection of each Type 1  sample, the  wide-mouth  glass
jar  was  packed  in ice in  a  separate  plastic  foam-insulated
container.   After  the  complete  composite  sample   had   been
collected,  it was mixed to provide a homogenous mixture, and  1-
liter aliquots were removed for metals analysis and placed in two
new  ^labeled plastic 1-liter bottles which had been  rinsed  with
distilled  water. Both of the 1-liter aliquots were preserved  by
the  addition of 5 ml of concentrated nitric acid.   The  bottles
were  then sealed, placed in an insulated chest and  shipped  for
metals  analyses.   These  analyses  include  atomic   absorption
spectrophotometry  and inductively coupled argon plasma  emission
spectroscopy (ICAP).
                                                              and
                                                              was
                                                                a
                                                              the
After removal of the two 1-liter metals aliquots from the compos-
ite sample,  the balance of the sample in the glass jar was  sub-
divided for analysis of nonvolatile organics,  conventional,
nonconventional  parameters.   If  a portion of this  sample
requested  by a plant representative for independent analysis,
1-liter aliquot was placed in a sample container supplied by
representative.          .

Sample Types 2 (cyanide) and 3 (total phenols) were stored in new
bottles  which had been iced and labeled;  1-liter clear  plastic
bottles  for Type 2,  and 1-liter amber glass for  Type  3.   The
bottles had been cleaned by rinsing with distilled water, and the
samples were preserved as described below.

To  each Type 2 (cyanide) sample,  sodium hydroxide was added  as
necessary  to elevate the pH to 12 or more (as measured using  pH
paper).   Where  the presence of chlorine (which would  decompose
most  of the cyanide) was suspected,  the sample was  tested  for
chlorine  by using potassium iodide-starch paper.   If the  paper
turned  blue,  ascorbic  acid  crystals  were  slowly  added  and
dissolved  until a drop of the sample produced no change  in  the
color of the test paper.  An additional 0.6 gram (0.021 ounce) of
ascorbic acid was added,  and each sample bottle was sealed (by a
Teflon-lined cap), labeled, iced, and shipped for analysis.

To  each Type 3 (total phenols) sample,  sulfuric acid was  added
as necessary to reduce the pH to 2 or less (as measured using  pH
paper).   Each  sample bottle was sealed with a Teflon-lined cap,
labeled, iced, and shipped for analysis.

Each  Type 4 (volatile organics) sample was stored in a new 40-ml
                                43

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           GENERAL DEVELOPMENT DOCUMENT
             SECT  - V
glass  vial  that had been rinsed with tap  water  and  distilled
water,  heated to 105°C  (221°F) for one hour, and cooled.
The  septum  and lid for each bottle were also prepared  by  this
method.   Each  bottle,  when used,  was filled  to  overflowing,
sealed  with  a Teflon-faced silicone septum  (Teflon side  down),
capped;  labeled,  and   iced.   Proper  sealing was  verified  by
inverting and tapping the container to confirm the absence of air
bubbles.   (If bubbles were found,  the bottle was opened,  a few
additional  drops  of sample were added, and proper  sealing  was
verified.)  Samples  were  labeled, iced  to 4°C,  and  sent  for
analysis.

A  1-quart wide-mouth glass bottle was used to collect each  grab
sample for oil and grease analysis.  Because oil tends to form  a
film  on top of water in quiescent streams, the sample  was  col-
lected in an area of complete mixing.  Sulfuric acid was added as
necessary to reduce the pH to less than 2.  The sample bottle was
sealed with a Teflon-lined cap, labeled, iced to 4°C and shipped
for analysis.

Sample  Analysis.   Samples were shipped by air  to  laboratories
where  inductively  coupled argon  plasma  emission  spectroscopy
(ICAP) and atomic absorption spectrophotometry (AA) analyses were
performed. The samples were analyzed only for metals shown to  be
significant  in the nonferrous metals manufacturing  category  or
those  expected to consume large amounts of  lime.   Twenty-three
metals were analyzed by ICAP, and six metals were analyzed by AA,
as shown below.  Total metals analysis was used for all samples.

Two nonconventional metal pollutants (tantalum and tungsten)  were
analyzed   by  X-ray  fluorescence.  Uranium  was   analyzed   by
fluorometry.
 Metals Analyzed by ICAP

  Aluminum
  Barium
 *Beryllium
  Boron
 *Cadmium
  Calcium
 *Chromium
  Cobalt
 *Copper
  Gold
  Iron
 *Lead
  Magnesium
  Manganese
  Molybdenum
 *Nickel
  Sodium
  Tin
  Titanium
  Vanadium
  Yttrium
 *Zinc
  Zirconium
  Metals Analyzed by AA

   *Antimony
   *Arsenic
   *Mercury
*Selenium
*Silver
*Thall'ium
                               44

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
    Metals Analyzed by X-Ray Fluorescence

    Tantalum
    Tungsten

   Metals Analyzed by Fluorometry

    Uranium

*Priority pollutant metals.

Mercury was analyzed by cold vapor flameless atomic absorption
spectrophotometry.

Radium-226 was analyzed by the precipitation method.   The refer-
ence for this method is the Interim Radiochemical Methodology.

Samples also went to laboratories for organics analysis.   Due to
their  very  similar  physical and  chemical  properties,  it  is
extremely   difficult  to  separate  the  seven   polychlorinated
biphenyls  (pollutants 106 to 112) for analytical  identification
and  quantification.  For that reason, the concentrations of  the
polychlorinated biphenyls are reported by the analytical  labora-
tory  in two groups:  one group consists of  PCB-1222,  PCB-1252,
and PCB-1221; the other group consists of PCB-1232 PCB-1248, PC8-
1260,  and  PCB-1016.  For convenience, the first group  has been
referred to as PCB-1254 and the second as PCB-1228.

The samples were not analyzed for Pollutant  129,  2,3,7,8-tetra-
chlorodibenzo-p-dioxin  (TCDD)  because no reference  sample  was
available to the analytical laboratory.

Three of the five conventional pollutant parameters were selected
for  analysis for evaluating treatment system performance.   They
are total suspended solids (TSS),  oil and grease,  and pH.   The
other  two conventionals,  fecal coliform and biochemical  oxygen
demand  (BOD),  were not measured because there is no  reason  to
believe  that  fecal matter or oxygen demanding biological  mate-
rials would be present in these wastewaters.  Ammonia,  fluoride,
and  total phenols (4-AAP) were analyzed for in selected  samples
if there was reason to believe they would be present based on the
processes  used. While not classified as toxic  pollutants,  they
affect the water quality.  Chemical oxygen demand (COD) and total
organic carbon (TOC) were also selected for analysis for selected
samples  for  subsequent  use  in  evaluating,  treatment   system
performance.   Total  dissolved  solids  (TDS)  was  measured  to
evaluate the potential for accumulation of dissolved salts.

In addition,  chloride,  alkalinity-acidity,  total solids, total
phosphorus (as PO4), and sulfate were measured to provide data to
evaluate the performance and cost of lime and settle treatment of
certain wastewater streams.

Samples were also analyzed for asbestos by transmission  electron
microscopy.    Total  fiber  and  chrysotile  fiber  counts  were
                               45

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
 reported by the testing laboratory.  Chrysotile was chosen by  the
 Agency as the screening parameter for asbestos for mining related
 activities because:   (1) of its known toxicity when particles  are
 inhaled,  (2) its industrial prevalence/  (3)  its  distinguishing
 selected  area electron diffraction  (SAED) pattern, and  (4)   the
 cumbersome nature of  the transmission electron microscopic   (TEM)
 analysis technique limits the identification to one mineral  form
 at the present time due to economics and  time constraints.

 While  the asbestos data vary,  the testing  laboratory's  report
 indicates  that  when  the  total fiber   count  is  performed  in
 conjunction  with a count of chrysotile fibers,  a  good  initial
 screening  parameter  is  produced.   The report  recommends   re-
 examining any facility with chrysotile fiber counts greater  than
 100  million  fibers  per liter (MFL) because this  represents  a
 significant  departure from ambient counts of 3 MFL in the  Great
 Lakes Basin.   The technique used had a threshold of detection of
 0.22 MFL.

 The  analytical quantification limits used in evaluation  of   the
 sampling  data  reflect  the accuracy of  the  analytical  methods
 used.   Below  these  concentration,  the identification  of   the
 individual   compounds  is  possible,   but   quantification   is
 difficult.  Pesticides and PCBs can be analytically quantified at
 concentrations  above  0.005  mg/1,  and other  organic  priority
 pollutants  at  concentrations  above  0.010  mg/1.    Analytical
 quantification   limits   associated  with   priority   inorganic
 pollutants  are as follows:  0.100 mg/1 for antimony;  0.10  mg/1
 for arsenic; 10 MFL for asbestos; 0.010 mg/1 for beryllium; 0.002
 mg/1 for cadmium; 0.005 mg/1 for chromium; 0.009 mg/1 for copper;
 0.02  mg/1  for  cyanide; 0.02 mg/1 for  lead;  0.0001  mg/1  for
 mercury;  0.005 mg/1 for nickel; 0.010 mg/1 for  selenium;   0.020
 mg/1  for  silver; 0.100 mg/1 for thallium; and  0.050  mg/1  for
 zinc.

 These  detection limits are not the same as  published  detection
 limit's  for  these pollutants by the same analytical methods   (40
 CFR  Part  136 - Guidelines Establishing Test Procedures for  the
Analysis of Pollutants;  40 CFR Part 136 - Proposed, 44 FR 69464,
 December 3,   1979;  1982 Annual Book of ASTM Standards,  Part 31,
Water,  ASTM, Philadelphia, PA:  "Methods for Chemical Analysis of
Water   and   Wastes,"  Environmental  Monitoring   and   Support
Laboratory,    Office  of  Research  and  Development,   U.S.  EPA
Cincinnati,   OH,  March,  1979,   EPA-600  4-79-020;  Handbook for
Monitoring  Industrial Wastewater, U.S.  EPA Technology  Transfer,
August, 1973).  The detection limits used were reported with  the
analytical data and hence are the appropriate limits to apply  to
 the  data.  Detection limit variation can occur as a result of  a
number  of  laboratory  equipment  and  daily   operator-specific
factors,  such as day-to-day differences in machine  calibration,
variation in stock solutions,  and variation in operators.

Quality Control.  Quality control measures used in performing all
analyses  conducted for this program complied with the guidelines
given  in "Handbook for Analytical Quality Control in  Water  and
                               46

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
Wastewater Laboratories" (published by EPA Environmental Monitor-
ing and Support Laboratory,  Cincinnati, Ohio, 1976).  As part of
the daily quality control program,  blanks (including sealed sam-
ples  of  blank water carried to each sampling site and  returned
unopened,  as well as samples of blank water used in the  field),
standards, and spiked samples were routinely analyzed with actual
samples.   As part of the overall program, all analytical instru-
ments (such as balances,  spectrophotometers, and recorders) were
routinely maintained and calibrated.

The  atomic-absorption spectrophotometer used for metal  analysis
was checked to see that it was operating correctly and performing
within  expected  limits.   Appropriate standards  were  included
after  at least every 10 samples.   Reagent blanks were also ana-
lyzed for each metal.

WATER USE AND WASTEWATER CHARACTERISTICS

In each of the subcategory supplements,  wastewater  characteris-
tics  corresponding to the subcategories in the nonferrous metals
manufacturing category are presented and discussed.   Tables  are
presented  in  Section V of each of the  subcategory  supplements
which present the sampling program data for raw waste and treated
effluent  sampled streams.   For those pollutants detected  above
analytically quantifiable concentrations in any sample of a given
wastewater  stream,  the  actual analytical data  are  presented.
Where  no  data  are listed for a specific day  of  sampling,  it
indicates  that  the wastewater samples for the stream  were  not
collected.

The  statistical analysis of data includes some samples  measured
at  concentrations  considered not quantifiable.   The base  neu-
trals,  acid fraction,  and volatile organics are considered  not
quantifiable  at concentrations equal to or less than 0.010 mg/1.
Below  this level,  organic analytical results are not  quantita-
tively accurate; however, the analyses are useful to indicate the
presence of a particular pollutant.   Nonquantifiable results are
designated  in the tables with an asterisk (double  asterisk  for
pesticides).

When  calculating  averages from the organic  sample  data,  non-
quantifiable  results and data reported as not detected (ND) were
assumed  to  be  zero.   When calculating  averages  from  metal,
cyanide,  conventional and nonconventional sampling data,  values
reported  as  less than a certain value were  considered  as  not
quantifiable, and consequently were assigned a value of zero.
                               47

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           GENERAL DEVELOPMENT DOCUMENT
SECT - V
                            Table V-l

     DISTRIBUTION OF SAMPLED PLANTS IN THE NONFERROUS METALS
              MANUFACTURING CATEGORY BY SUBCATEGORY
Subcategory
     Number
    of Plants
Bauxite Refining
Primary Aluminum Smelting
Secondary Aluminum Smelting
Primary Copper Smelting
Secondary Copper
Primary Lead
Secondary Lead
Primary Zinc
Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Metallurgical Acid Plants*
Primary Antimony
Primary Beryllium
Primary and Secondary Germanium and Gallium
Secondary Indium
Primary Magnesium**
Secondary Mercury
Primary Molybdenum and Rhenium (includes
  Molybdenum Acid Plants
Secondary Molybdenum and Vanadium
Primary Nickel and Cobalt
Secondary Nickel
Primary Precious Metals and Mercury
Secondary Precious Metals
Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin
Primary and Secondary Titanium
Secondary Tungsten and Cobalt  ,
Secondary Uranium
Primary Zirconium and Hafnium
TOTAL (!)
           2
           7
           5
           4
           5
           3
           8
           6
           6
           4
           4
           1
           2
           1
           1
           3
           1
           1
           1
           2
           5
           1
           2
           5
           3
           2
           1
           2
          84
**The primary magnesium subcategory has been recommended for
  exclusion under Paragraph 8 of the Settlement Agreement.
 *Acid plant wastewater samples were collected at the primary
  copper, lead, and zinc plants listed above.
 IBecause several plants were sampled for more than one
  subcategory, the actual number of plants sampled is less  than
  the total number of plants sampled for all subcategories.
                               48

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                           SECTION VI

                SELECTION OF POLLUTANT PARAMETERS
The  Agency  has studied nonferrous metals  manufacturing  waste-
waters  to  determine the presence or absence of  toxic,  conven-
tional,  and  selected  nonconventional  pollutants.   The  toxic
pollutants  and  nonconventional pollutants are  subject  to  BAT
effluent limitations and guidelines.  Conventional pollutants are
considered in establishing BPT, BCT, and NSPS limitations.

Sixty  five pollutants and classes of pollutants were  classified
as  toxic  by the CWA amendments of 1977.  The  Agency  clarified
this  into  the list of 129 specific toxic pollutants  listed  in
Table VI-1 (page 126) for which specific analysis procedures  and
standards  were  available.   These  129  toxic  pollutants   are
sometimes  referred to as priority pollutants.  Three  pollutants
have    been   deleted   from   the   toxic    pollutant    list.
Dichlorodifluoromethane  and trichlorofluoromethane were  deleted
(46  FR 2266, January 8, 1981) followed by the deletion  of  bis-
(chloromethyl)  ether (46 FR 10723, February 4. 1981) The  Agency
has  concluded that deleting these compounds will not  compromise
adequate   control   over  their  discharge  into   the   aquatic
environment   and  that  no  adverse  effects  on   the   aquatic
environment or on human health will occur as a result of deleting
them from the list of toxic pollutants.

Past  studies  by EPA and others have identified  many  pollutant
parameters   in  addition  to  the  toxic  pollutants  useful  in
characterizing industrial wastewaters and in evaluating treatment
process removal efficiencies.  For this reason, a number of other
pollutants  and  pollutant parameters were also studied  for  the
nonferrous metals manufacturing category.

The conventional pollutants considered in this rulemaking  (total
suspended solids, oil and grease, and pH) traditionally have .been
studied to characterize industrial wastewaters.  These parameters
impact  water quality and are especially useful in evaluating the
effectiveness  of some wastewater treatment processes.   EPA  has
defined the criteria for the selection of conventional pollutants
(43 FR 32857 January 11, 1980).

Several nonconventional pollutants were also considered in devel-
oping these regulations.   These include aluminum, barium, boron,
cesium,  cobalt,  gallium, germanium, hafnium, manganese, radium-
226,  rhenium,  rubidium,  uranium, vanadium, zirconium, chemical
oxygen  demand (COD),  and total organic carbon (TOC).   In addi-
tion,  calcium,  chloride,  magnesium,  alkalinity-acidity, total
dissolved  solids,   total phosphorus (as PO4),  and sulfate  were
measured  to provide data to evaluate the cost of  chemical  pre-
cipitation  and  sedimentation treatment  of  certain  wastewater
streams.
                               49

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Fluoride,  ammonia  (NH3),  and total phenols (4-AAP)  were  also
identified as pollutants for some of; the subcategories.  Fluoride
compounds  are  used  in  the  production  of  primary  aluminum,
columbium-tantalum,  and beryllium and secondary uranium and  are
present in the raw wastewater of these industries. NH3 is used in
the  process  or  formed during a process step   in  the  primary
aluminum,    columbium-tantalum,    tungsten,    and    zirconium
subcategories  and  in  the secondary  molybdenum  and  vanadium,
precious  metals,  tungsten  and cobalt,  uranium,  aluminum  and
silver subcategories.   In other subcategories,  it has been used
for neutralization of the wastewater.

RATIONALE FOR SELECTION OF POLLUTANT PARAMETERS

In determining which pollutants to regulate, a pollutant that was
never  detected,  or  that was never found above  its  analytical
quantification level,  usually was eliminated from consideration.
The  analytical  quantification  level for  a  pollutant  is  the
minimum  concentration  at which that pollutant can  be  reliably
measured.  Below  that concentration, the identification  of  the
individual   compounds   is  possible,  but   quantification   is
difficult.   For  the  priority pollutants  in  this  study,  the
analytical quantification levels are:  0.005 mg/1 for pesticides,
PCB's, chromium, and nickel: 0.010 mg/1 for the remaining organic
priority   pollutants  and  cyanide,  arsenic,   beryllium,   and
selenium:  10  million fibers per liter (10  MFL)  for  asbestos:
0.020 mg/1 for lead and silver; 0.009 mg/1 for copper; 0.002 mg/1
for cadmium; and 0.0001 mg/1 for mercury.

These  detection  limits are not the same as published  detection
limits for these pollutants by the same analytical methods.   The
detection limits used were reported with the analytical data  and
hence are the appropriate limits to apply to the data.  Detection
limit  variation can occur as a result of a number of laboratory-
specific,   equipment-specific,   and   daily   operator-specific
factors.   These  factors can include day-to-day  differences  in
machine calibration,  variation in stock solutions, and variation
in operators.

Because  the  analytical standard for TCDD was judged to  be  too
hazardous  to  be made generally available,  samples  were  never
analyzed  for this pollutant.   There is no reason to expect that
TCDD   would  be  present  in  nonferrous  metals   manufacturing
wastewaters.

Pollutants  which were detected below  concentrations  considered
achievable by available treatment technology were also eliminated
from further consideration.   ;For the toxic metals,  the chemical
precipitation,  sedimentation,  and filtration technology values,
which  are presented in Section VII (Table VII-21 page 248)  were
used.   For  the  toxic organic pollutants detected  above  their
analytical  quantification limit,  achievable concentrations  for
activated  carbon  technology were  used.   These  concentrations
represent  the  most stringent treatment options  considered  for
pollutant removal.
                               50


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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
The  pollutant  exclusion procedure was applied to the  raw  waste
data  for each subcategory.   Detailed specific results are  pre-
sented  in  Section VI of each of  the  subcategory  supplements.
Summary  results of selected pollutants for each subcategory  are
presented later in this section.

Toxic pollutants remaining after the application of the exclusion
process  were  then selected for further consideration  in  estab-
lishing specific regulations.

DESCRIPTION OP POLLUTANT PARAMETERS

The  following  discussion  addresses  the  pollutant  parameters
detected  above  their  analytical quantification  limit  in  any
sample  of  nonferrous  metals  manufacturing  wastewater.    The
description of each pollutant provides the following information:
the source of the pollutant;  whether it is a naturally occurring
element,  processed material,  or manufactured compound;  general
physical properties and the form of the pollutant; toxic  effects
of the pollutant in humans and other animals; and behavior of the
pollutant in a POTW at concentrations that might be expected from
industrial discharges.

Acenaphthene  (1) .   Acenaphthene (1,2-dihydroacenaphthylene,  of
1,8-ethylene-naphthalene)  is a polynuclear aromatic  hydrocarbon
(PAH) with molecular weight of 154 and a formula of
Acenaphthene occurs in coal tar produced during high  temperature
coking  of  coal.   It has been detected in cigarette  smoke  and
gasoline exhaust condensates.

The  pure compound is a white crystalline solid at room  tempera-
ture  with a melting range of 95°C to 97°C and a boiling range of
278°C  to 280°C.  Its vapor pressure at room temperature is  less
than 0.02 mm Hg.  Acenaphthene is slightly soluble in water  (100
mg/1), but even more soluble in organic solvents such as ethanol,
toluene, and chloroform.  Acenaphthene can, be oxidized by  oxygen
or  ozone  in the presence of certain catalysts.   It  is  stable
under laboratory conditions.

Acenaphthene is used as a dye intermediate,  in the manufacture of
some plastics, and as an insecticide and fungicide.

So  little  research has been performed on acenaphthene that  its
mammalian and human health effects are virtually  unknown.    The
water  quality  criterion of 0.02 mg/1 is recommended to  prevent
the adverse effects on humans due to the organoleptic  properties
of acenaphthene in water .

No  de-tailed  .study of acenaphthene behavior in a POTW is  avail-
able.  However, it has been demonstrated that none of the organic
toxic pollutants studied so far can be broken down by  biological
treatment processes as readily as fatty acids,  carbohydrates,  or
proteins.   Many  of the toxic pollutants have been investigated,
                               51

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VI
at  least in laboratory-scale studies,  at concentrations  higher
than  those  expected to be contained by  most  municipal  waste-
waters.   General  observations  relating molecular structure  to
ease  of  degradation have been developed for all  of  the  toxic
organic pollutants.

The  conclusion reached by study of the limited data is that bio-
logical  treatment produces little or no degradation of  acenaph-
thene.   No  evidence is available for drawing conclusions  about
its possible toxic or inhibitory effect on POTW operation.

Its  water  solubility would allow acenaphthene  present  in  the
influent to pass through a POTW into the effluent.  The hydrocar-
bon  character of this compound makes it sufficiently hydrophobic
that adsorption onto suspended solids and retention in the sludge
may also be a significant route for removal of acenaphthene  from
the POTW.

Acenaphthene has been demonstrated to affect the growth of plants
through  improper  nuclear  division and  polyploidal  chromosome
number.   However,  it  is not expected that land application  of
sewage  sludge containing acenaphthene at the low  concentrations
which  are  to be expected in a POTW sludge would result  in  any
adverse effects on animals ingesting plants grown in such soil.

Benzene  (4).   Benzene  (C^K^)  is  a  clear,  colorless  liquid
obtained  mainly  from petroleum feedstocks by several  different
processes.   Some is recovered from light oil obtained from  coal
carbonization  gases.  It boils at 80°C and has a vapor  pressure
of  100 mm Hg at 26°C.  It is slightly soluble in water (1.8  g/1
at  25°C) and it dissolves in hydrocarbon solvents.  Annual  U.S.
               gases.
    100 mm Hg at 26°C.
    25°C) and it dissolves in hydrocarbon solvents.
production is three to four million tons.
Most  of  the  benzene  used  in  the  U.S.  goes  into  chemical
manufacture.   About  half of that is converted  to  ethylbenzene
which is    used to make styrene.   Some benzene is used in motor
fuels.

Benzene  is  narmful to human health according to  numerous  pub-
lished  studies.   Most studies relate effects of inhaled benzene
vapors.   These effects include nausea,  loss of muscle coordina-
tion,  and excitement, followed by depression and coma.  Death is
usually the result of respiratory or cardiac failure.   Two  spe-
cific  blood disorders are related to benzene exposure.   One  of
these,  acute  myelogenous leukemia,  represents  a  carcinogenic
effect  of benzene.  However, most human exposure data are  based
on  exposure in occupational settings and benzene  carcinogenisis
is not considered to be firmly established.

Oral  administration  of benzene to laboratory  animals  produced
leukopenia,  a  reduction in number of leukocytes in  the  blood.
Subcutaneous injection of benzene-oil solutions has produced sug-
gestive, but not conclusive, evidence of benzene carcinogenisis.

Benzene  demonstrated teratogenic effects in laboratory  animals,
                               52

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           GENERAL DEVELOPMENT DOCUMENT
                                    SECT - VI
and mutagenic effects in humans and other animals.

For  maximum  protection  of  human  health  from  the  potential
carcinogenic  effects of exposure to benzene through ingestion of
water     and contaminated aquatic organisms,  the ambient  water
concentration  is zero.  Concentrations of benzene  estimated  to
                                                              \~7
result  in
10
  -o
and
  additional lifetime cancer risk at levels of  10"
10~5 are 0.00015 mg/1, 0.0015 mg/1, and  0.015  mg/1,
respectively.

Some studies have been reported regarding the behavior of benzene
in  a POTW.   Biochemical oxidation of benzene  under  laboratory
conditions,  at concentrations of 3 to 10 mg/1,  produced 24, 27,
24,  and  20  percent degradation in 5,  10,  15,  and  20  days,
respectively,  using  unacclimated seed cultures in fresh  water.
Degradation  of 58,  67,  76,  and 80 percent was produced in the
same     time  periods using  acclimated  seed  cultures.   Other
studies  produced  similar  results.   Based on  these  data  and
general  conclusions relating molecular structure to  biochemical
oxidation,  it    is expected that biological treatment in a POTW
will  remove  benzene  readily from  the  water.   Other  reports
indicate  that most    benzene entering a POTW is removed to  the
sludge  and that influent concentrations of lm/1 inhibit  sludge
digestion.   There is    no information about possible effects of
benzene on crops grown    in soils amended with sludge containing
benzene.

Carbon  Tetrachloride  (6).   Carbon tetrachloride  (CC14),  also
called tetrachloromethane, is a colorless liquid produced primar-
ily  by the•chlorination of hydrocarbons,  particularly  methane.
Carbon tetrachloride boils at 77°C and has a vapor pressure of 90
mm  Hg  at 20°C.  It is slightly soluble in water  (0.8  gm/1  at
25°C)  and soluble in many organic solvents.  Approximately  one-
third of a million tons is produced annually in the U.S.

Carbon tetrachloride, which was displaced by perchloroethylene as
a  dry cleaning agent in the 1930's,  is used principally  as  an
intermediate for production of chlorofluoromethanes for refriger-
ants,  aerosols, and blowing agents.  It is also used as a  grain
fumigant.

Carbon  tetrachloride  produces  a variety of  toxic  effects  in
humans.   Ingestion of relatively large quantities - greater than
5  grams  - has frequently proved fatal.   Symptoms  are  burning
sensation  in  the mouth,  esophagus,  and stomach,  followed  by
abdominal pains, nausea, diarrhea, dizziness, abnormal pulse, and
coma.   When death does not occur immediately,  liver and  kidney
damage are usually found.   Symptoms of chronic poisoning are not
as  well defined.   General fatigue,  headache,  and anxiety have
been observed,  accompanied by digestive tract and kidney discom-
fort or pain.

Data concerning teratogenicity and mutagenicity of carbon  tetra-
chloride are scarce and inconclusive.  However, carbon tetrachlo-
ride  has  been  demonstrated to be  carcinogenic  in  laboratory
                               53

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           GENERAL DEVELOPMENT DOCUMENT
                                            SECT  -  VI
animals.  The liver was the target organ.

For maximum protection of human health from the potential carcin-
ogenic effects of exposure to carbon tetrachloride through inges-
tion  of  water and contaminated aquatic organisms,  the  ambient
water concentration is zero.  Concentrations of carbon tetrachlo-
ride  estimated toresult in additional lifetime cancer  risk  at
risk  levels of 10 ', 10 6, and 10~5 are 0.000026  mg/1,  0.00026
mg/1, and 0.0026 mg/1, respectively.
Data  on  the behavior of carbon tetrachloride in a POTW are  not
available.  Many of the toxic organic pollutants have been inves-
tigated, at least in laboratory-scale studies, at  concentrations
higher  than those expected to be found in most municipal  waste-
waters.   General  observations  have  been  developed   relating
molecular  structure to ease of degradation for all of the  toxic
organic  pollutants.   The  conclusion reached by  study  of  the
limited  data  is that biological treatment produces  a  moderate
degree of removal of carbon tetrachloride in a POTW.  No informa-
tion  was  found regarding the possible  interference  of  carbon
tetrachloride  with  treatment  processes.  Based  on  the  water
solubility  of  carbon tetrachloride, and the vapor  pressure  of
this compound, it is expected that some of the undegraded  carbon
tetrachloride  will  pass through to the POTW effluent  and  some
will be volatilized in aerobic processes.

Chlorobenzene
	   (7).   Chlorobenzene  (CsHsCl),  also called  mono-
chlorobenzene   is a clear, colorless, liquid manufactured by  the
liquid  phase chlorination of benzene over a catalyst.  It  boils
at 132°C and has a vapor pressure of 12.5 mm Hg at  25°C.
It  is  almost  insoluble in water (0.5  g/1  at  30°C),  but
dissolves  in   hydrocarbon solvents.  U.S. annual  production  is
near 150,000 tons.

Principal uses  of Chlorobenzene are as a solvent and as an inter-
mediate  for  dyes and pesticides.   Formerly it was used  as  an
intermediate for DDT production, but elimination of production of
that  compound  reduced annual U.S.  production  requirements  for
Chlorobenzene by half.

Data  on  the threat to human health posed by  Chlorobenzene  are
limited.   Laboratory   animals,   administered  large  doses  of
Chlorobenzene subcutaneously, died as a result of central nervous
system depression.  At slightly lower dose rates, animals died of
liver  or kidney damage.  Metabolic disturbances  occurred  also,.
At  even  lower dose rates of orally  administered  Chlorobenzene
similar  effects were observed, but some animals survived  longer
than  at  higher  dose  rates.  No  studies  have  been  reported
regarding   evaluation   of  the   teratogenic,   mutagenic,   or
carcinogenic potential of Chlorobenzene.

For  the  prevention of adverse effects due to  the  organoleptic
properties of Chlorobenzene in water the recommended criterion is
0.020 mg/1.
                               54

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Only  limited  data are available on which  to  base  conclusions
about  the  behavior  of chlorobenzene  in  a  POTW.   Laboratory
studies  of the biochemical oxidation of chlorobenzene have  been
carried  out  at  concentrations greater than those  expected  to
normally be present in POTW influent.   Results showed the extent
of degradation to be 25,  28,  and 44 percent after 5, 10, and 20
days,  respectively.   In another, similar study using a  phenol-
adapted culture, 4 percent degradation was observed after 3 hours
with  a  solution  containing 80 mg/1.   On the  basis  of  these
results  and general conclusions about the relationship of molec-
ular  structure to biochemical oxidation,  it is  concluded  that
chlorobenzene remaining intact is expected to volatilize from the
POTW  in aeration processes.   The estimated half-life of chloro-
benzene  in water based on water solubility,  vapor pressure  and
molecular weight is 5.8 hours.

1,2,4-Trichloroben2ene (8) .     1,2,4-Trichlorobenzene (05113^3),
1,2,4-TCB)  is  a liquid at room temperature,  solidifying  to  a
crystalline  solid at 17°C and boiling at 214°C.  It is  produced
by  liquid  phase chlorination of benzene in the  presence  of  a
catalyst.   Its vapor pressure is 4 mm Hg at 25°C.  1,2,4-TCB  is
insoluble in water and soluble in organic solvents.  Annual  U.S.
production is in the range of 15,000 tons.  1,2,4-TCB is used  in
limited  quantities  as  a solvent and as a dye  carrier  in  the
textile industry.  It is also used as a heat transfer medium  and
as a transfer fluid.  The compound can be selectively chlorinated
to   1,2,4,5-tetrachlorobenzene   using  iodine   plus   antimony
trichloride as catalyst.

No reports were available regarding the toxic effects of  1,2,4-
TCB  on  humans.    Limited  data  from  studies  of  effects  in
laboratory  animals fed 1,2,4-TCB indicate depression of activity
at low doses and predeath extension convulsions at lethal  doses.
Metabolic  disturbances  and  liver changes were  also  observed.
Studies  for the purpose of determining teratogenic or  mutagenic
properties of 1,2,4-TCB have not been conducted.  No studies have
been  made  of carcinogenic behavior  of  1,2,4-TCB  administered
orally.

For  the  prevention of adverse effects due to  the  organoleptic
properties of 1,2,4-trichlorobenzene in water, the water  quality
criterion is 0.013 mg/1.

Data  on  the behavior of 1,2,4-TCB in POTW  are  not  available.
However,  this  compound  has been investigated in  a  laboratory
scale  study  of biochemical oxidation at  concentrations  higher
than  those  expected  to be contained by most  municipal  waste-
waters.   Degradations  of 0, 87, and 100 percent  were  observed
after  5, 10, and 20 days, respectively.  Using this  observation
and general observations relating molecular structure to ease  of
degradation  for  all  of the organic  priority  pollutants,  the
conclusion was reached that biological treatment produces a  high
degree of removal in POTW.
Hexachlorobenzene  (9).
Hexachlorobenzene
            s
                  non-
                               55

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
flammable  crystalline  substance which  is virtually  insoluble  in
water.  However,  it  is  soluble  in benzene, chloroform, and ether.
Hexachlorobenzene (HCB) has a density of 2.044 g/ml.   It melts at
231°C and boils at 323  to  326°C.  Commercial production of HCB in
the  U.S. was discontinued in 1976, though it is still  generated
as  a  by-product of other chemical  operations.    In  1972,  an
estimated 2,425 tons of HCB were produced in this way.

Hexachlorobenzene is   used  as a  fungicide  to  control  fungal
diseases  in cereal  grains.  The main agricultural use of HCB  is
on  wheat seed intended solely  for planting.  HCB  has been  used
as an impurity in other pesticides.  It is used in industry as  a
plasticizer for polyvinyl  chloride as well as a flame  retardant.
HCB  is  also  used as a starting material for the production
pentachlorophenol which is marketed as a wood preservative.
                    of
Hexachlorobenzene  can be harmful to human health as was seen  in
Turkey  from 1955 to 1959.   Wheat that had been treated with HCB
in preparation for planting was consumed as food.   Those  people
affected  by HCB developed cutanea tarda porphyria,  the symptoms
of  which  included blistering and epidermolysis of  the  exposed
parts of the body,  particularly the face and the  hands.   These
symptoms  disappeared after consumption of HCB contaminated bread
was discontinued.   However, the HCB which was stored in body fat
contaminated  maternal milk. ;  As a result of this,  at least  95
percent of the infants feeding on this milk died.   The fact that
HCB remains stored in body fat after exposure has ended  presents
an  additional  problem.   Weight loss may result in  a  dramatic
redistribution  of HCB contained in fatty tissue.   If the stored
levels of HCB are high, adverse effects might ensue.

Limited  testing suggests that hexachlorobenzene is  not  terato-
genic or mutagenic.   However,  two animal studies have been con-
ducted  which indicate that HCB is a carcinogen.   HCB appears to
have multipotential carcinogenic activity; the incidence of hepa-
tomas,  haemangioendotheliomas and thyroid adenomas was  signifi-
cantly increased in animals exposed to.HCB by comparison to  con-
trol animals.

For maximum protection of human health from the potential carcin-
ogenic effects of exposure to hexachlorobenzene through ingestion
of  water and contaminated aquatic organisms,  the ambient  water
concentration is zero.  Concentrations of HCB estimated to result
in  additional lifetime cancer risk at levels of 10~', 10~6,  and
10 5 are 7.2 x 10 8 mg/1, 7.2 x 10~7  mg/1, and 7.2 x 10~6  mg/1,
respectively.   If  contaminated  aquatic  organisms  alone   are
consumed,   excluding  the  consumption  of _water,   the   water
concentration  should  be less than 7.4 x 10~6  mg/1 to  keep  the
increased  lifetime cancer risk below 10~5.  Available data  show
that  adverse  effects on aquatic life  occur  at  concentrations
higher than those cited for human health risks.

No  detailed  study  of hexachlorobenzene  behavior  in  POTW  is
available.    However,  general  observations  relating  molecular
                               56

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           GENERAL DEVELOPMENT DOCUMENT
                    SECT - VI
structure  to ease of degradation have been developed for all  of
the organic priority pollutants.  The conclusion reached by study
of  the limited data is that biological treatment produces little
or no degradation of hexachlorobenzene.  No evidence is available
for   drawing  conclusions  regarding  its  possible   toxic   or
inhibitory effect on POTW operations.

1,2-Dichloroethane  (10).   1,2-Dichloroethane  is a  halogenated
aliphatic  used  in the production of tetraethyl lead  and  vinyl
chloride, as an industrial solvent, and as an intermediate in the
production of other organochlorine compounds.   Some  chlorinated
ethanes  have  been  found in drinking  waters,  natural  waters,
aquatic organisms, and foodstuffs.  Research indicates that  they
may have mutagenic and carcinogenic properties.

1,1,1-Trichloroethane (11).   1,1,1-Trichloroethane is one of the
two possible trichlorethanes.  It is manufactured by hydrochlori-
nating vinyl chloride to 1,1-dichloroethane which is then chlori-
nated to the desired product.  1,1,1-Trichloroethane is a  liquid
at room temperature with a vapor pressure of 96 mm Hg at 20 C and
a boiling point of 74°C.  Its formula is 0:13013   It is slightly
soluble  in  water  (0.48 g/1) and is  very  soluble  in  organic
solvents.  U.S. annual production is greater than one-third of  a
million tons.
1,1,1-Tr ichloroethane
degreasing agent.
is  used  as  an  industrial  solvent  and
Most  human  toxicity data for 1,1,1-trichloroethane  relates  to
inhalation and dermal exposure routes.   Limited data are  avail-
able  for determining toxicity of ingested 1,1,1-trichloroethane,
and those data are all for the compound itself,  not solutions in
water.   No data are available regarding its toxicity to fish and
aquatic organisms.   For the protection of human health from  the
toxic  properties  of 1,1,1-trichloroethane ingested through  the
consumption  of water and fish,  the ambient water  criterion  is
15.7  mg/1.   The  criterion is based on bioassays  for  possible
carcinogenicity.

No  detailed study of 1,1,1-trichloroethane behavior in a POTW is
available.   However,  it has been demonstrated that none of  the
toxic  organic pollutants of this type can be broken down by bio-
logical treatment processes as readily as fatty  acids,  carbohy-
drates, or proteins.

Biochemical oxidation of many of the toxic organic pollutants has
been investigated,  at least in laboratory-scale studies, at con-
centrations  higher  than commonly expected in  municipal  waste-
water.  General observations relating molecular structure to ease
of  degradation have been developed for all of these  pollutants.
The  conclusion  reached  by study of the limited  data  is  that
biological treatment produces a moderate degree of degradation of
1,1,1-trichloroethane.  No evidence is available for drawing con-
clusions  about  its possible toxic or inhibitory effect on  POTW
operation.   However, for degradation to occur, a fairly constant
                                57

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 input of the compound would be necessary.

 Its water solubility would allow  1,1,1-trichloroethane,   present
 in  the  influent  and not  biodegradable,   to pass  through a   POTW
 into the effluent.   One  factor which  has  received  some attention,
 but no detailed study, is  the  volatilization of  the  lower molecu-
 lar weight organics  from a POTW.   If  1,1,1-trichloroethane is not
 biodegraded,   it will volatilize during aeration processes in the
 POTW.

 Hexachloroethane (12).   Hexachloroethane  (CC13CC13),  also called
 perchloroethane is a white crystalline  solid with  a  camphor-like
 odor.    It  is manufactured from tetrachloroethylene,   and  is  a
 minor  product  in many industrial  chlorination processes  designed
 to  produce  lower   chlorinated  hydrocarbons.   Hexachloroethane
 sublimes at 185°C and has  a vapor pressure of about  0.2 mm Hg at
 20°C.   It is  insoluble in  water (50 mg/1 at  22°C)  and  soluble in
 some organic  solvents

 Hexachloroethane can be  used in lubricants designed  to withstand.
 extreme  pressure.    It  is used  as a plasticizer  for cellulose
 esters,  and as a pesticide.  It is also used as  a  retarding  agent
 in fermentation, as  an accelerator in the rubber industry, and in
 pyrotechnic and smoke devices.

 Hexachloroethane is  considered to be toxic to humans by ingestion
 and inhalation.   In laboratory  animals liver and kidney  damage
 have   been   observed.      Symptoms   in    humans   exposed   to
 hexachloroethane vapor  include severe eye irritation  and  vision
 impairment.     Based    on   studies   on    laboratory  animals,
 hexachloroethane is  considered to be carcinogenic.

 For  the   maximum protection to human health  from  the potential
 carcinogenic   effects  of  exposure  to  hexachloroethane   through
 ingestion   of   water  and   contaminated  aquatic  organisms,  the
 ambient  water   concentration  is  zero.  Concentrations  of  hexa-
 chloroethane   estimated  to  result  in additional  lifetime  cancer
 risks  at   levels  of 10 7,  10  b, and  10~5   are  0.000059  mg/1,
 0.00059 mg/1,  and 0.0059 mg/1.  respectively.

 Data  on   the   behavior  of  hexachloroethane  in  POTW  are  not
 available.   Many  of the organic priority pollutants  have   been
 investigated     at    least   in  laboratory  scale   studies,    at
 concentrations  higher than  those  expected to be contained by most
municipal wastewaters.  General observations have been  developed
 relating  molecular  structure  to  ease of degradation for  all  of
 the organic priority pollutants.  The conclusion reached by study
of the limited data  is that biological treatment produces  little
or  no  removal of hexachloroethane in POTW.   The lack  of  water
solubility  and  the expected affinity  of  hexachloroethane  for
solid  particles lead to the expectation that this compound  will
be  removed  to  the sludge in POTW.   No  information  was  found
regarding possible uptake of hexachloroethane by plants grown  on
soils amended with hexachloroethane-bearing sludge.
                               58

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
1,1-Dichloroethane  (13) .     1,1-Dichloroethane,   Q.-^.^.^'  also
called  ethylidene  dichloride  and  ethylidene  chlorrde,  is  a
colorless liquid manufactured by reacting hydrogen chloride  with
vinyl chloride in 1,1-dichloroethane solution in the presence  of
a   catalyst.   However,   it  is  reportedly   not   manufactured
commercially  in the U.S.   1,1-Dichloroethane boils at  57°C  and
has  a  vapor  pressure of 182 mm Hg at  20°C.   It  is  slightly
soluble  in water (5.5 g/1 at 20°C) and very soluble  in  organic
solvents.

1,1-Dichloroethane  is used as an extractant  for  heat-sensitive
substances and as a solvent for rubber and silicone grease.

1,1-Dichloroethane  is less toxic than its isomer  (1,2-dichloro-
ethane),  but  i'ts  use as an anaesthetic has  been  discontinued
because  of  marked excitation of the heart.  It  causes  central
nervous system depression in humans.  There are insufficient data
to derive water quality criteria for 1,1-dichloroethane.

Data  oh  the behavior of 1,1-dichloroethane in a  POTW  are  not
available.   Many  of  the  toxic organic  pollutants  have  been
investigated,  at  least in laboratory-scale studies,  at concen-
trations  higher  than  those expected to be  contained  by  most
municipal wastewaters.   General observations have been developed
relating  molecular structure to ease of degradation for  all  of
the toxic organic pollutants.  The conclusion reached by study of
the  limited  data is that biological treatment produces  only  a
moderate removal of 1,1-dichloroethane in a POTW by degradation.

The  high  vapor  pressure of 1,1-dichloroethane is  expected  to
result  in  volatilization of some of the compound  from  aerobic
processes in a POTW.  Its water solubility will result in some of
the  1,1-dichloroethane  which  enters the POTW  leaving  in  the
effluent from the POTW.                               .   •    '   .

1,1,2-Trichloroethane (14).   1,1,2-Trichloroethane is one of the
two possible trichloroethanes and is sometimes called ethane tri-
chloride or vinyl trichloride.  .It is used as a solvent for fats,
oils,  waxes,  and  resins,  in the manufacture of  1,1-dichloro-
ethylene, and as an intermediate in organic synthesis.

1,1,2-Trichloroethane is a clear,  colorless liquid at room  tem-
perature with a vapor pressure of 16.7 mm Hg at 20°C, and a boil-
ing point of 113°C.  it is insoluble in water and very soluble in
organic solvents.  The formula is CHC12CH2C1.

Human  toxicity  data for 1,1,2-trichloroethane do not appear  in
the literature.   The compound does produce liver and kidney dam-
age  in laboratory animals after intraperitoneal  administration.
No literature data were found concerning teratogenicity or  muta-
genicity  of 1,1,2-trichloroethane.   However,  mice treated with
1,1,2-trichloroethane showed increased incidence of  hepatocellu-
lar carcinoma.   Although bioconcentration factors are not avail-
able  for  1,1,2-trichloroethane 'in fish  and  other  freshwater
aquatic organisms,  it is concluded on the basis of octanol-water
                               59

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            GENERAL DEVELOPMENT  DOCUMENT
SECT - VI
 partition coefficients  that  bioconcentration  does  occur.

 For   the   maximum protection of  human  health  from   the  potential
 carcinogenic  effects  of exposure to  1,1,2-trichloroethane  through
 ingestion  of  water  and  contaminated   aquatic   organisms,   the
 ambient   water   concentration is zero.    Concentrations  of   this
 compound  estimated toresult in  additional  lifetime cancer   risks
 at   risk  levels of 10 ', 10  6, and 10  5  are 0.00006 mg/1,  0.0006
 mg/1,  and 0.006 mg/1, respectively.    If  contaminated   aquatic
 organisms alone are consumed,  excluding  the consumption of water,
 the   water concentration should  be less  than_Q.418  mg/1  to   keep
 the   increased  lifetime cancer risk  below 10   .   Available   data
 show that adverse effects on aquatic life occur at  concentrations
 higher than those cited for  human health  risks.

 No detailed study of  1,1,2-trichloroethane  behavior in a POTW  is
 available.  However,  it is reported  that  small amounts are formed
 by chlorination processes and  that this  compound persists  in   the
 environment  (greater than two years)  and it  is not biologically
 degraded.   This information  is not completely consistent with the
 conclusions  based on   laboratory-scale  biochemical   oxidation
 studies   and  relating  molecular  structure  to ease degradation.
 That study  concluded  that  biological treatment in a  POTW   will
 produce moderate removal of  1,1,2-trichloroethane.

 The   lack   of  water  solubility  and  the  relatively  high  vapor
 pressure   may  lead  to removal  of this compound from a  POTW  by
 volatilization.

 2,4,6-Trichlorophenol  (21).     2,4,6-Trichlorophenol  (6H2C13OH,
 abbreviated here to 2,4,6-TCP) is a  colorless,  crystalline solid
 at   room  temperature.   It is prepared by  the  direct  chlorination
 of   phenol.   2,4,6-TCP  melts at  68°C and  is slightly  soluble   in
 water  (0.8 gm/1 at 25°C).  This phenol does  not produce a  color
 with 4-aminoantipyrene, and therefore does  not contribute to   the
 nonconventional   pollutant  parameter  "Total  Phenols."   No   data
 were'found  on production volumes.

 2,4,6-TCP   is  used as  a fungicide, bactericide,  glue  and  wood
 preservative, and for antimildew treatment.    It is  also used   for
 the     manufacture     of     2,3,4,6-tetrachlorophenol       and
 pentachlorophenol.

 No   data  were   found on human  toxicity  effects   of  2,4,6-TCP.
 Reports  of studies with laboratory animals indicate that  2,4,6-
 TCP  produced convulsions when injected   interperitoneally.  Body
 temperature   was   elevated  also.   The   compound  also  produced
 inhibition  of ATP production 'in isolated rat liver mitochondria,
 increased mutation  rates in one strain of bacteria,  and produced
 a  genetic  change  in rats.    No studies on   teratogenicity  were
 found.  Results  of a  test for ;carcinogenicity were  inconclusive.

For  the  prevention of  adverse effects due  to  the  organoleptic
properties of 2,4,6-trichlorophenol in water,   the water  quality
criterion is  0.100 mg/1.
                               60

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           GENERAL DEVELOPMENT DOCUMENT
              SECT - VI
Although  no data were found regarding the behavior of  2,4f6-TCP
in  a POTW,  studies of the biochemical oxidation of the compound
have been made at laboratory scale at concentrations higher  than
those  normally expected in municipal  wastewaters.   Biochemical
oxidation   to  2,4,6-TCP  at  100  mg/1  produced   23   percent
degradation  using  a  phenol-adapted  acclimated  seed  culture.
Based  on  these  results,  biological treatment  in  a  POTW  is
expected  to produce a moderate degree of  degradation.   Another
study  indicates  that  2,4,6-TCP may be produced in  a  POTW  by
chlorination of phenol during normal chlorination treatment.
Para-chloro-meta-cresol
(22).
be  a
         Para-chloro-meta-cresol
a  4-chloro-3-methyl-phenol  (4-
(C1C7H60H))  is  thought  to
chloro-meta-cresol,  or 2-chloro-5-hydroxy-toluene),  but is also
used by some authorities to refer to 6-chloro-3-methyl-phenol (6-
chloro-meta-cresol,  or 4-chloro-3-hydroxy-toluene), depending on
whether the chlorine is considered to be para to the methyl or to
the  hydroxy  group.   it is assumed for  the  purposes  of  this
document that the subject compound is 2-chloro-5-hydroxy-toluene.
This  compound is a colorless crystalline solid melting at 66  to
68°C.  It is slightly soluble in water (3.8 gm/1) and soluble  in
organic  solvents.  This phenol reacts with p-aminoantipyrene  to
give   a  colored  product  and  therefore  contributes  to   the
nonconventional  pollutant parameter designated "Total  Phenols."
No  information on manufacturing methods or volumes produced  was
found.

Para-chloro-meta cresol (abbreviated here as PCMC) is marketed as
a   microbiocide,   and  was  proposed  as  an   antiseptic   and
disinfectant more than 40 years ago.   It is used in glues, gums,
paints,   inks,  textiles,  and leather goods.  PCMC was found in
raw  wastewaters from the die casting quench operation  from  one
subcategory of foundry operations.

Although no human toxicity data are available for  PCMC,  studies
on  laboratory  animals have demonstrated that this  compound  is
toxic when administered subcutaneously and intravenously.   Death
was preceded by severe muscle tremors.   At high dosages,  kidney
damage  occurred.   On the other hand,  an unspecified isomer  of
chlorocresol,  presumed to be PCMC, is used at a concentration of
0.15  percent  to  preserve mucous  heparin,  a  natural  product
administered intravenously as an anticoagulant.  The report  does
not  indicate  the total amount of PCMC typically  received.   No
information  was  found  regarding  possible  teratogenicity,  or
carcinogenicity of PCMC.

Two   reports   indicate  that  PCMC  undergoes  degradation   in
biochemical  oxidation treatments carried out  at  concentrations
higher  than  are expected to be encountered in  POTW  influents.
One  study  showed  50 percent degradation in 3.5  hours  when  a
phenol-adapted  acclimated seed culture was used with a  solution
of  60 mg/1 PCMC.  The other study showed 100 percent degradation
of  a  20  mg/1  solution of PCMC in  two  weeks  in  an  aerobic
activated  sludge test system.   No degradation of PCMC  occurred
                               61

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            GENERAL DEVELOPMENT DOCUMENT
                            SECT - VI
 under  anaerobic  conditions.
 Chloroform
(23).
Chloroform,
CHC13,
also
called
 trichloromethane,  is  a  colorless  liquid  manufactured  commercially
 by   chlorination   of  methane.    Careful  control   of  conditions
 maximizes   chloroform  production,   but  other   products must   be
 separated.   Chloroform  boils  at 61°C and has a  vapor  pressure   of
 200  mm Hg at 25°C.  It  is  slightly  soluble in water (8.22 g/1   at
 20°C and readily soluble in organic solvents.

 Chloroform   is used as  a solvent  and to  manufacture refrigerants,
 Pharmaceuticals, plastics, and anesthetics.  It is  seldom used  as
 an anesthetic.

 Toxic  effects  of chloroform on  humans  include central  nervous
 system depression,  gastrointestinal irritation, liver  and kidney
 damage, and  possible  cardiac  sensitization to adrenalin.  Carcin-
 ogenicity  has  been  demonstrated for  chloroform   on  laboratory
 animals.

 For  the  maximum protection  of human health from   the  potential
 carcinogenic effects of exposure to chloroform through ingestion
 of   water and contaminated aquatic  organisms,   the  ambient  water
 concentration is zero.  Concentrations of  chloroform  estimated  to
 result in additional  lifetime cancer risks at the levels of 10"',
 10 6, and 10 5 were 0.000021 mg/1,  0.00021 mg/1, and  0.0021 mg/1,
 respectively.

 No   data are available  regarding  the behavior of chloroform in  a
 POTW.   However,  the biochemical oxidation of  this compound  was
 studied  in  one laboratory-scale study  at concentrations  higher
 than  those  expected to be contained by  most  municipal  waste-
 waters.   After 5,  10,  and  20 days no  degradation of  chloroform
 was  observed.   The conclusion reached  is that biological treat-
 ment  produces little or no removal  by degradation  of   chloroform
 in a POTW.

 The  high vapor pressure of chloroform is  expected  to   result   in
 volatilization  of the  compound from aerobic treatment  steps in a
 POTW.   Remaining chloroform is expected to pass through into the
 POTW effluent.
2-Chlorophenol  (24) .   2-Chlorophenol  (ClCs^OH),  also  called
ortho-chlorophenol,  is  a colorless liquid at room  temperature,
manufactured by direct chlorination of phenol followed by distil-
lation to separate it from the other principal product, 4-chloro-
phenol.  2-Chlorophenol solidifies below 7°C and boils at  176°C.
It is soluble in water (28.5 gm/1 at 20°C) and soluble in several
types of organic solvents.  This phenol gives a strong color with
4-aminoantipyrene    and    therefore    contributes    to    the
nonconventional pollutant parameter "Total Phenols."   Production
statistics  could  not be found.  2-Chlorophenol is  used  almost
exclusively  as  a  chemical intermediate in  the  production  of
pes'ticides and dyes.  Production of some phenolic resins uses  2-
chlorophenol.          ,              .....
                               62

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Very  few  data  are available on which to  determine  the  toxic
effects of 2-chlorophenol on humans.   The compound is more toxic
to   laboratory  mammals  when  administered  orally  than   when
administered  subcutaneously  or intravenously.  This  effect  is
attributed to the fact that the compound is almost completely  in
the  unionized  state at the low pH of the stomach and  hence  is
more  readily  absorbed  into the  body.   Initial  symptoms  are
restlessness  and increased respiration rate, followed  by  motor
weakness  and  convulsions  induced  by  noise  or  touch.   Coma
follows.   Following lethal doses, kidney, liver, and  intestinal
damage were observed.  No studies were found which addressed  the
teratogenicity or mutagenicity of 2-chlorophenol.  Studies of  2--
chlorophenol  as  a promoter of carcinogenic  activity  of  other
carcinogens were conducted by dermal application.  Results do not
bear   a   determinable   relationship   to   results   of   oral
administration studies.

For  the  prevention of adverse effects due to  the  organoleptic
properties  of 2-chlorophenol in water,  the criterion is  0.0003
mg/1.

Data  on  the  behavior  of 2-chlorophenol  in  a  POTW  are  not
available.  However, laboratory-scale studies have been conducted
at  concentrations  higher  than those expected to  be  found  in
municipal   wastewaters.   At  1  mg/1  of   2-chlorophenol,   an
acclimated   culture   produced  100   percent   degradation   by
biochemical  oxidation after 15 days.  Another study  showed  45,
70, and 79 percent degradation by biochemical oxidation after  5,
10,  and , 20 days, respectively.  The conclusion reached  by  the
study  of  these limited data, and general  observations  on  all
toxic organic pollutants relating molecular structure to ease  of
biochemcial  oxidation,  is that 2-chlorophenol is removed  to  a
high  degree  or completely by biological treatment  in  a  POTW.
Undegraded 2-chlorophenol is expected to pass through a POTW into
the   effluent  because  of  the  water  solubility.    Some   2-
chlorophenol  is  also expected to be generated  by  chlorination
treatments of POTW effluents containing phenol.

1,1-Dichloroethylene (29).   1,1-Dichloroethylene (1,1-DCE), also
called   vinylidene  chloride,  is  a  clear   colorless   liquid
manufactured  by  dehydrochlorination  of  1,1,2-trichloroethane.
1,1-DCE has the formula CC12CH2.  It has a boiling point of 32°C,
and  a vapor pressure of 591 mm Hg at 25°C.  1,1-DCE is  slightly
solu-ble  in  water  (2.5 mg/1) and is soluble  in  many  organic
solvents.  U.S.  production  is  in  the  range  of  hundreds  of
thousands of tons annually.

1,1-DCE  is  used  as a chemical intermediate and  for  copolymer
coatings or films.   It may enter the wastewater of an industrial
facility  as  the  result of  decomposition  of  1,1,1-trichloro-
ethylene  used  in degreasing operations,  or by  migration  from
vinylidene  chloride  copolymers exposed to  the  process  water.
Human toxicity of 1,1-DCE has not been demonstrated;  however, it
is a suspected human carcinogen.  Mammalian toxicity studies have
                               63

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           GENERAL DEVELOPMENT DOCUMENT
                SECT - VI
 focused   on   the  liver and kidney damage  produced  by   1,1-DCE.
 Various   changes occur in  those organs  in  rats and mice  ingesting
 1,1-DCE.

 For   the  maximum protection of human health from  the   potential
 carcinogenic  effects of exposure to 1,1-dichloroethylene  through
 ingestion of  water  and  contaminated  aquatic  organisms,  the
 ambient   water concentration is zero.  The concentration of  1,1-
 DCE estimated to result in an additional lifetime cancer risk  of
 1  in  100,000  is 0.0013 mg/1.

 Under laboratory conditions, dichloroethylenes have been shown to
 be toxic to  fish.   The primary effect of acute toxicity of  the
 dichloroethylenes  is  depression of the central nervous  system.
 The   octanol-water partition coefficient of 1,1-DCE indicates  it
 should not accumulate significantly in animals.

 The behavior of 1,1-DCE in a POTW has not been studied.   However,
 its   very high vapor pressure is expected to result in release of
 significant percentages of this material to the atmosphere in any
 treatment involving aeration.  Degradation of dichloroethylene in
 air is reported to occur, with a half-life of eight weeks.

 Biochemical oxidation of many of the toxic organic pollutants has
 been  investigated in laboratory-scale studies at  concentrations
 higher than would normally be expected in municipal  wastewaters.
 General   observations  relating molecular structure  to   ease  of
 degradation have been developed for all of these pollutants.  The
 conclusion  reached  by  study  to  the  limited  data   is   that
 biological  treatment produces little or no degradation   of  1,1-
 dichloroethylene.    No   evidence  is  available   for   drawing
 conclusions about the possible toxic or inhibitory effect of 1,1-
 DCE  on   POTW operation.  Because of  water  solubility,  1,1-DCE
 which is  not volatilized or degraded is expected to pass  through
 a  POTW.  Very little 1,1-DCE is expected to be found  in  sludge
 from a POTW.
1,2-trans-Dichloroethylene
trans-DCE)  is  a  clear,
CHC1CHC1.   1,2-trans-DCE
isomer   by  chlorination
  (30).     1,2-Dichloroethylene  (1,2-
 colorless  liquid  with  the  formula
is produced in mixture with  the  cis-
of  acetylene.   The  cis-isomer   has
distinctly  different  physical  properties.   Industrially,  the
mixture is used rather than the separate isomers.   1,2-trans-DCE
has a boiling point of 48°C, and a vapor pressure of 234 mm Hg at
25°C.

The  principal use of 1,2-dichloroethylene (mixed isomers) is  to
produce  vinyl  chloride.   It is used as  a  lead  scavenger  in
gasoline,  general  solvent, and for synthesis of  various  other
organic  chemicals.  When it is used as a solvent,  1,2-trans-DCE
can enter wastewater streams.

Although  1,2-trans-DCE is thought to produce fatty  degeneration
of mammalian liver,  there are insufficient data on which to base
any ambient water criterion.
                               64

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
In  the reported toxicity test of 1,2-trans-DCE on aquatic  life,
the  compound  appeared  to be about half as toxic as  the  other
dichloroethylene (1,1-DCE) on the toxic pollutants list.

The  behavior  of 1,2-trans-DCE in a POTW has not  been  studied.
However, its high vapor pressure is expected to result in release
of a significant percentage of this compound to the atmosphere in
any treatment involving aeration.   Degradation of the  dichloro-
ethylenes in air is reported to occur,  with a half-life of eight
weeks.

Biochemical oxidation of many of the toxic organic pollutants has
been  investigated in laboratory-scale studies at  concentrations
higher  than would normally be expected in municipal wastewaters.
General  observations  relating molecular structure  to  ease  of
degradation have been developed for all of these pollutants.  The
conclusion  reached  by  the study of the limited  data  is  that
biochemical  oxidation produces little or no degradation of  1,2-
trans-dichloroethylene.   No  evidence is available  for  drawing
conclusions about the possible toxic or inhibitory effect of 1,2-
trans-dichloroethylene  on POTW operation.  It is  expected  that
its  low  molecular weight and degree of  water  solubility  will
result in 1,2-trans-DCE passing through a POTW to the effluent if
it is not degraded or volatilized.  Very little 1,2-trans-DCE  is
expected to be found in sludge from a POTW.

2,4-Dichlorophenol (31).   2,4-Dichlorophenol, a white, low melt-
ing  solid, melts at 45°G.  it is soluble in alcohol  and  carbon
tetrachloride  and slightly soluble in water.  This  compound  is
moderately toxic by ingestion and is a strong irritant to tissue.

2,4-Dimethylphenol  (34)..'. -   2,4-Dimethylphenol  (2,4-DMP),  also
called  2,4-xylenol,  is a colorless,  crystalline solid at  room
temperature  (25°C),  but  melts at 27°C  to  28°C.   2,4-DMP  is
slightly  soluble  in water and, as a weak acid,  is  soluble  in
alkaline  solutions.  Its vapor pressure is less than 1 mm Hg  at
room temperature.

2,4-DMP   (C8H10O)  is a natural product,  occurring in coal  and
petroleum  sources.   It is used commercially as an  intermediate
for manufacture of pesticides,  dye stuffs,  plastics and resins,
and  surfactants.   It is found in the water runoff from  asphalt
surfaces.   It  can  find  its  way  into  the  wastewater  of  a
manufacturing plant from any of several adventitious sources.

Analytical procedures specific.to this compound are used for  its
identification and quantification in wastewaters.   This compound
does  not  contribute  to "Total Phenols" determined  by  the  4-
aminoantipyrene method.          .

Three  methylphenol  isomers  (cresols)  and  six  dimethylphenol
isomers  (xylenols) generally occur together in natural products,
industrial processes,  commercial products,  and phenolic wastes.
Therefore.  data are not available for human exposure to  2,4-DMP
                               65

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 alone.   In addition to this,  most mammalian tests for  toxicity of
 individual  dimethylphenol  isomers  have  been  conducted   with
 isomers other than 2,4-DMP.

 In   general,   the  mixtures  of  phenol,    methylphenols,    and
 dimethylphenols contain compounds which produced acute  poisoning
 in laboratory animals.   Symptoms were difficult breathing,   rapid
 muscular   spasms,    disturbance  of   motor   coordination,    and
 asymmetrical  body  position.   In a   1977   National   Academy  of
 Science publication the conclusion was reached that, "In view  of
 the ^   relative   paucity   of    data   on    the   mutagenicity,
 carcinogenicity,   teratogenicity, and long  term oral toxicity  of
 2,4-dimethylphenol,   estimates   of the effects  of  chronic   oral
 exposure  at low levels cannot  be made with any confidence."    No
 ambient  water  quality criterion can be set at  this   time.    In
 order to protect  public health,  exposure to this compound should
 be minimized as soon as possible.

 Toxicity  data for  fish and  freshwater aquatic life are  limited;
 however,   in  reported  studies  of 2,4-dimethylphenol   at  concen-
 trations as  high  as  2 mg/1 no adverse effects were observed.

 The behavior  of 2,4-DMP in  a  POTW has not been studied.   As  a
 weak  acid,   its  behavior may be somewhat dependent on the pH  of
 the influent to the  POTW.  However, over the normal limited range
 to POTW pH,  little  effect of  pH would be expected.

 Biological   degradability of  2,4-DMP  as determined in  one study,
 showed   94.5  percent  removal  based  on  chemical  oxygen demand
 (COD).    Thus,  substantial removal is expected for this  compound.
 Another   study determined that persistence of   2,4-DMP  in   the
 environment  is low,   and  thus any of  the compound which   remained
 in     the   sludge or passed  through  the POTW into  the   effluent
 would be     degraded  within moderate  length of  time (estimated  as
 two months     in  the  report).

 2,4-Dinitrotoluene   (35)   2,4-Dinitrotoluene  ((N02)2C6H3CH3),  a
 yellow  crystalline compound,  is  manufactured as. a co-product  with
 the 2,6-isomer by nitration  of  nitrotoluene.   It melts  at  71°C.
 2,4-Dinitrotoluene   is  insoluble in water (0.27  g/1 at  22°C)  and
 soluble  in a number of  organic  solvents.  Production data for the
 2,4-isomer alone  are  not  available.   The  2,4-  and 2,6-isomers are
manufactured in an 80:20  or 65:35  ratio,  depending on  the process
used.   Annual U.S. commercial production is  about  150   thousand
tons of the  two isomers.   Unspecified  amounts are Produced by the
U.S. government and further nitrated  to  trinitrotoluene  (TNT) for
military use.  The major  use  of  the dinitrotoluene mixture is for
production   of toluene  diisocyanate used  to  make  polyurethanes.
Another use  is in production  of  dyestuffs.

The  toxic   effect of 2,4-dinitrotoluene  in  humans  is   primarily
methemoglobinemia  (a blood condition  hindering oxygen    transport
by  the blood).    Symptoms  depend on severity of the disease.   but
include cyanosis,  dizziness,  pain in  joints, headache, and loss
of appetite  in workers  inhaling  the compound.  Laboratory animals
                               66

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
fed  oral doses of 2,4-dinitrotoluene exhibited many of the  same
symptoms.  Aside from the effects in red blood cells, effects are
observed in the nervous system and testes.

Chronic  exposure to 2,4-dinitrotoluene may produce liver  damage
and  reversible anemia.   No data were found on teratogenicity of
this  compound.   Mutagenic data are limited and are regarded  as
confusing.   Data  resulting from studies of  carcinogenicity  of
2,4-dinitrotoluene  point to a need for further testing for  this
property.

For  the  maximum protection of human health from  the  potential
carcinogenic  effects  of exposure to 2.4-dinitrotoluene  through
ingestion  of  water  and  contaminated  aquatic  organisms,  the
ambient  water  concentration is zero.  Concentrations   of  2,4-
dinitrotoluene estimated toresult in additional lifetime  cancer
risk  at  risk levels of 10~7, 10~6  and 10~5 are  0.00074  mg/1,
0.074 mg/1, and 0.740 mg/1, respectively.

Data  on  the behavior of 2,4-dinitrotoluene in a  POTW  are  not
available.    However, biochemical oxidation of 2,4-dinitrophenol
was  investigated  on a laboratory scale.   At 100 mg/1  of  2,4-
dinitrotoluene, a concentration considerably higher than expected
in municipal wastewaters, biochemical oxidation by an acclimated,
phenol-adapted  seed  culture produced 52 percent degradation  in
three  hours.   Based  on this limited  information  and  general
observations relating molecular structure to ease of  degradation
for  all  the  toxic organic pollutants, it  was  concluded  that
biological  treatment in a POTW removes 2,4-dinitrotoluene  to  a
high degree or completely.  No information is available regarding
possible  interference  by 2,4-dinitrotoluene in  POTW  treatment
processes,  or on the possible detrimental effect on sludge  used
to amend soils in which food crops are grown.

Ethylbenzene   (38).    Ethylbenzene  (CgHio)  is  a  colorless,
flammable  liquid  manufactured  commercially  from  benzene  and
ethylene.   Approximately  half of the benzene used in  the  U.S.
goes  into  the manufacture of more than three  million  tons  of
ethylbenzene  annually.  Ethylbenzene boils at 136°C  and  has  a
vapor  pressure  of 7 mm Hg at 20°C.  It is slightly  soluble  in
water (0.14 g/1 at 15°C) and is very soluble in organic solvents.

About  98 percent of the ethylbenzene produced in the  U.S.  goes
into  the  production of styrene,  much of which is used  in  the
plastics  and  synthetic rubber industries.   Ethylbenzene  is  a
constituent  of  xylene mixtures used as diluents  in  the  paint
industry, agricultural insecticide sprays, and gasoline blends.

Although  humans  are exposed to ethylbenzene from a  variety  of
sources  in  the environment,  little information on  effects  of
ethylbenzene  in  man or animals is  available.   Inhalation  can
irritate eyes, affect the respiratory tract, or cause vertigo. In
laboratory  animals, ethylbenzene exhibited low  toxicity.   There
are  no data available on teratogenicity,  mutagenicity,  or car-
cinogenicity of ethylbenzene.
                               67

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           GENERAL DEVELOPMENT DOCUMENT
SECT - -VI
Criteria  are  based  on data derived  from  inhalation  exposure
limits.   For  the  protection of human  health  from  the  toxic
properties   of   ethylbenzene   ingested   through   water   and
contaminated   aquatic  organisms,  the  ambient  water   quality
criterion is 1.1 mg/1.

The  behavior of ethylbenzene in a POTW has not been  studied  in
detail.  Laboratory-scale studies of the biochemical oxidation of
ethylbenzene  at  concentrations greater than would  normally  be
found  in municipal wastewaters have demonstrated varying degrees
of  degradation.   In  one  study  with  phenol-acclimated   seed
cultures,  27 percent degradation was observed in a half  day  at
250  mg/1 ethylbenzene.  Another study at unspecified  conditions
showed  32,  38, and 45 percent degradation after 5, 10,  and  20
days,   respectively.   Based  on  these  results   and   general
observations  relating molecular structure of degradation, it  is
concluded  that  biological  treatment  produces  only   moderate
removal of ethylbenzene in a POTW by degradation.

Other  studies  suggest that most of the ethybenzene  entering  a
POTW  is  removed from the aqueous stream  to  the  sludge.   The
ethylbenzene  contained  in the sludge removed from the POTW  may
volatilize.

Fluoranthene (39) .  Fluoranthene (1,2-benzacenaphthene) is one of
the compounds called polynuclear aromatic hydrocarbons (PAH).   A
pale yellow solid at room temperature, it melts at 111°C and  has
a  negligible  vapor pressure at 25°C.  Water solubility  is  low
(0.2 mg/1).  Its molecular formula is CisHiQ. Fluoranthene, along
with many other PAHs, is found throughout the environment.  It is
produced  by pyrolytic processing of organic raw materials,  such
as  coal and petroleum, at high temperature (coking  processes).
It   occurs  naturally  as  a  product  of  plant   biosynthesis.
Cigarette smoke contains fluoranthene. Although it is not used as
the  pure compound in industry, it has been found  at  relatively
higher  concentrations (0.002 mg/1) than most other PAH's  in  at
least one industrial effluent.  Furthermore, .in a 1977 EPA survey
to determine levels of PAH in U.S.  drinking water supplies,  none
of   the  110  samples  analyzed  showed  any  PAH   other   than
fluoranthene.

Experiments  with  laboratory animals indicate that  fluoranthene
presents  a relatively low degree of toxic potential  from  acute
exposure,  including oral administration.    Where death occurred,
no  information was reported concerning target organs or specific
cause of death.

There  is  no  epidemiological  evidence to  prove  that  PAH  in
general,   and fluoranthene,   in particular,  present in  drinking
water are related to the development of cancer.   The only studies
directed  toward determining carcinogenicity of fluoranthene have
been  skin tests on laboratory animals.   Results of these  tests
show  that fluoranthene has  no activity as a complete  carcinogen
(i.e.,   an  agent which produces cancer when applied by  itself),
                               68

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VI
but exhibits significant cocarcinogenicity (i.e.,  in combination
with a carcinogen, it increases the carcinogenic activity).

Based  on  the  limited  animal  study  data,  and  following  an
established  procedure, the  ambient water quality criterion  for
fluoranthene  alone  (not  in  combination  with  other  PAH)  is
determined to be 200 mg/1 for the protection of human health from
its toxic properties.

There  are  no  data on the chronic effects  of  fluoranthene  on
freshwater organisms.   One saltwater invertebrate shows  chronic
toxicity  at  concentrations below 0.016 mg/1.   For some  fresh-
water  fish species the concentrations producing  acute  toxicity
are substantially higher, but data are very limited.

Results   of   studies  of - the  behavior  of   fluoranthene   in
conventional sewage treatment processes found in a POTW have been
published.  Removal of fluoranthene during primary  sedimentation
            to  be 62 to 66 percent (from  an  initial  value  of
             0.04435 mg/ to a final value of 0.00122
             the removal was 91 to 99 percent
             0.00026  mg/1) after  biological
was  found
0.00323  to
mg/1),  and
0.00028  to
activated sludge processes.
       to  0.0146
(final  values  of
purification  with
A review was made of data on biochemical oxidation of many of the
toxic organic pollutants investigated in laboratory-scale studies
at  concentrations  higher  than would normally  be  expected  in
municipal  wastewaters.  General observations relating  molecular
structure  to ease of degradation have been developed for all  of
these pollutants.  The conclusion reached by study of the limited
data   is  that  biological  treatment • produces  little  or   no
degradation of fluoranthene. .The same study, however,  concludes
that fluoranthene would be readily removed by filtration and oil-
water   separation  and  other  methods  which  rely   on   water
insolubility, or adsorption on other particulate surfaces.   This
latter  conclusion  is supported by the  previously  cited  study
showing significant removal by primary sedimentation.

No  studies  were  found  to give data  on  either  the  possible
interference   of  fluoranthene  with  POTW  operation,  or   the
persistence  of fluoranthene in sludges or POTW effluent  waters.
Several  studies have documented the ubiquity of fluoranthene  in
the  environment  and  it cannot be readily  determined  if  this
results  from  persistence of anthropogenic fluoranthene  or  the
replacement of degraded fluoranthene by natural processes such as
biosynthesis in plants.  , .

Methylene   Chloride
      	   	   44).   Methylene  chloride,  also   called
dTchldromethane(CH2C12), is a colorless liquid manufactured  by
chlorination of .methane or methyl chloride followed by separation
from  the  .hrgher  chloni-nated methanes  formed  as  co-products.
Methylene chloride boils at 40°C, and has a vapor pressure of 362
mm Hg at 20°C. It is slightly soluble in water (20 g/1 at  20°C).
and very soluble in organic solvents.. U.S. annual production  is
about 250,000 tons.
                               69

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           GENERAL DEVELOPMENT DOCUMENT
                             SECT - VI
Methylene  chloride  is  a common  industrial  solvent  found  in
insecticides,  metal  cleaners,  paint,  and  paint  and  varnish
removers.

Methylene  chloride is not generally regarded as highly toxic  to
humans.  Most human toxicity data are for exposure by inhalation.
Inhaled  methylene  chloride  acts as a  central  nervous  system
depressant.   There  is  also evidence that the  compound  causes
heart failure when large amounts are inhaled.

Methylene  chloride  does  produce  mutation in  tests  for  this
effect.   in  addition, a bioassay recognized for  its  extremely
high sensitivity to strong and weak carcinogens produced  results
which  were marginally significant.  Thus potential  carcinogenic
effects  of methylene chloride are not confirmed or  denied,  but
are  under  continuous  study.   Difficulty  in  conducting
interpreting the test results at the low boiling point (40°C)
methylene  chloride increases the difficultg of  maintaining
compound  in  growth  media durihg incubation at  37°C;  and
                                                and
                                                 of
                                                the
                                                the
difficulty  of  removing  all impurities,
themselves be carcinogenic.
                             some  of  which  might
For  the protection of human health from the toxic properties  of
methylene  chloride  ingested  through  water  and   contaminated
aquatic organisms, the ambient water criterion is 0.002 mg/1. The
behavior  of methylene chloride in a POTW has not been studied in
any detail.   However, the biochemical oxidation of this compound
was  studied  in  one laboratory-scale  study  at  concentrations
higher  than  those expected to be contained  by  most  municipal
wastewaters.    After  five  days  no  degradation  of  methylene
chloride was observed.  The conclusion reached is that biological
treatment  produces  little  or  no  removal  by  degradation  of
methylene chloride in a POTW.

The  high  vapor pressure of methylene chloride  is  expected  to
result  in volatilization of the compound'from aerobic  treatment
steps  in a POTW.   It has been reported that methylene  chloride
inhibits anaerobic processes in a POTW.   Methylene chloride that
is  not volatilized in the POTW is expected to pass through  into
the effluent.
Dichlorobromomethane
	   (48).
Research   has
aliphatic.
carcinogenic
adverse effects on human health.
This  compound
 shown   that
                                is  a   halogenated
                                halomethanes   have
properties, and exposure to this compound may  have
Chlorodibromomethane
	   (51).
Research   has
aliphatic.
carcinogenic
adverse effects on human health.
This  compound
 shown   that
                                is  a   halogenated
                                halomethanes   have
properties, and exposure to this compound may  have
Isophorone  (54).    Isophorone is an industrial chemical produced
at a level of tens of millions of pounds annually in the U.S. The
chemical  name for isophorone is  3,5,5-trimethyl-2-cyclohexen-l-
                               70

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
one  and  it  is  also  known  as  trimethyl  cyclohexanone   and
isoacetophorone.   The formula is €5^(013)30.   Normally,  it is
produced  as the gamma isomer;   technical grades contain about 3
percent of the beta isomer  (3,5,5-trimethyl-3-cyclohexen-l-one).
The  pure  gamma  isomer  is a  water-white  liquid,  with  vapor
pressure  less  than 1 mm Hg at room temperature, and  a  boiling
point of 215.2°C.  It has a camphor- or peppermint-like  odor and
yellows upon standing.  It is slightly soluble (12 mg/1) in water
and dissolves in fats and oils.

Isophorone  is synthesized from acetone and is used  commercially
as a solvent or cosolvent for finishes,  lacquers,  polyvinyl and
nitrocellulose resins,  pesticides,  herbicides,  fats, oils, and
gums.  It is also used as a chemical feedstock.

Because isophorone is an industrially used solvent, most toxicity
data  are  for  inhalation  exposure.   Oral  administration   to
laboratory animals in two different studies revealed no acute  or
chronic   effects  during  90  days   and  no  hematological   or
pathological abnormalities were reported.  Apparently, no studies
have been completed on the carcinogenicity of isophorone.

Isophorone does undergo bioconcentration in the lipids of aquatic
organisms and fish.

Based  on subacute data,  the ambient water quality criterion for
isophorone ingested through consumption of water and fish is  set
at  460  mg/1 for the protection of human health from  its  toxic
properties

Studies  of  the  effects  of  isophorone  on  fish  and  aquatic
organisms reveal relatively low toxicity  compared to some  other
toxic pollutants.

The  behavior  of  isophorone in a POTW  has  not  been  studied.
However,  the biochemical oxidation of many of the toxic  organic
pollutants  has been investigated in laboratory scale studies  at
concentrations   higher  than  would  normally  be  expected   in
municipal  wastewaters.  General observations relating  molecular
structure  to ease of degradation have been developed for all  of
these  pollutants.   The conclusion reached by the study  of  the
limited  data  is that biochemical treatment in a  POTW  produces
moderate  removal of isophorone.  This conclusion  is  consistent
with  the  findings of an experimental study  of  microbiological
degradation of isophorone which showed about 45 percent oxidation
in  15 to 20 days in domestic wastewater, but only 9  percent  in
salt  water. No data were found on the persistence of  isophorone
in sewage sludge.

Naphthalene  (55).   Naphthalene is an aromatic hydrocarbon  with
two  orthocondensed  benzene  rings and a  molecular  formula  of
C10H8.  As such, it is properly classed as a polynuclear aromatic
hydrocarbon  (PAH).  Pure naphthalene is a white crystalline solid
melting  at  80°C.  For a solid, it has a relatively  high  vapor
pressure  (0.05 mm Hg at 20°C), and moderate water solubility  (19
                               71

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 mg/1 at 20°C).  Napthalene is the most abundant single  component
 of  coal tar. Production is more than a third of a  million  tons
 annually  in the U.S. About three fourths of the   production  is
 used  as feedstock for phthalic anhydride manufacture.   Most  of
 the  remaining production goes into manufacture  of  insecticide,
 dyestuffs,   pigments,  and  Pharmaceuticals.   Chlorinated   and
 partially  hydrogenated  naphthalenes are used  in  some  solvent
 mixtures.  Naphthalene is also used as a moth repellent.

 Naphthalene,  ingested  by humans.  has reportedly caused  vision
 loss  (cataracts),  hemolytic  anemia   and  occasionally   renal
 disease.  These effects of naphthalene ingestion are confirmed by
 studies  on laboratory animals.  No carcinogenicity  studies  are
 available which can be used to demonstrate carcinogenic  activity
 for  naphthalene.   Naphthalene does  bioconcentrate  in  aquatic
 organisms.

 For  the protection of human health from the toxic properties  of
 naphthalene  ingested  through  water  and  through  contaminated
 aquatic organisms,  the ambient water criterion is determined  to
 be 143 mg/1.

 Only a limited number of studies have been conducted to determine
 the  effects of naphthalene on aquatic organisms.    The data from
 those studies show only moderate toxicity.

 Naphthalene  has  been  detected in  sewage  plant  effluents  at
 concentrations  up  to 0.022 mg/1 in studies carried out  by  the
 U.S.  EPA.  Influent levels were not reported.   The  behavior  of
 naphthalene  in  a POTW has not been  studied.    However,   recent
 studies  have  determined  that naphthalene  will   accumulate  in
 sediments  at  100 times the concentration  in   overlying   water.
 These results suggest that naphthalene will be  readily removed by
 primary  and  secondary  settling 'in  a  POTW,   if  it  is   not
 biologically degraded.

 Biochemical oxidation of many of the toxic organic pollutants has
 been  investigated in laboratory-scale studies  at   concentrations
 higher  than would normally be expected in municipal wastewaters.
 General  observations  relating molecular  structure  to ease  to
 degradation have been developed for  all of these pollutants.   The
 conclusion  reached  by  study  of  the  limited  data  is   that
 biological  treatment produces a high removal by  degradation  of
 naphthalene.   One recent study has shown that microorganisms   can
 degrade naphthalene,  first to a dihydro compound,  and  ultimately
 to carbon dioxide and water.

.Nitrobenzene   (56) .     Nitrobenzene   (C6H5N02),    also   called
 nitrobenzol  and oil  of mirbane,   is a pale yellow,   oily  liquid,
 manufactured  by reacting benzene with nitric acid  and sulfuric
 acid.    Nitrobenzene   boils at 210°C and has a  vapor  pressure  of
 0.3g mm Hg at 25°C.    It is slightly soluble in  water  (1.9  g/1  at
 20°C)   and is miscible  with most  organic solvents.    Estimates  of
 annual  U.S  production  vary .widely,  ranging  from  100  to   350
 thousand tons.
                                72

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           GENERAL DEVELOPMENT .DOCUMENT
SECT - VI
Almost the entire volume of nitrobenzene produced (97 percent) is
converted  to  aniline,  which  is  used  in  dyes,   rubber,  and
medicinals.   Other uses for nitrobenzene include:   solvent  for
organic synthesis, metal polishes, shoe polish, and perfume.

The  toxic effects of ingested or inhaled nitrobenzene in  humans
are  related  to  its action  in  blood:   methemoglobinemia  and
cyanosis.  Nitrobenzene administered orally to laboratory animals
caused   degeneration  of  heart,  kidney   and   liver   tissue;
paralysis,   and   death.   Nitrobenzene   has   also   exhibited
teratogenicity  in laboratory animals  but studies  conducted  to
determine  mutagenicity or carcinogenicity did not reveal  either
of these properties

For  the  prevention of adverse effects due to  the  organoleptic
properties of nitrobenzene in water, the criterion is 0.030 mg/1.

Data  on the behavior of nitrobenzene in POTW are not  available.
However,   laboratory-scale  studies  have  been   conducted   at
concentrations  higher  than  those  expected  to  be  found   in
municipal   wastewaters.   Biochemical  oxidation   produced   no
degradation  after  5,  10, and 20 days.   A  second  study  also
reported  no  degradation after 28 hours,  using  an  acclimated,
phenol-adapted seed culture with nitrobenzene at 100 mg/1.  Based
on  these  limited  data, and on  general  observations  relating
molecular  structure  to  ease of  biological  oxidation,  it  is
concluded that little or no removal of nitrobenzene occurs during
biological  treatment in POTW.  The low water solubility and  low
vapor  pressure  of  nitrobenzene lead to  the  expectation  that
nitrobenzene  will  be removed,from POTW in the effluent  and  by
volatilization during aerobic treatment.

2-Nitrophenol  (57).   2-Nitrophenol.  (NO2C6H40H),  also   called
orthonitrophenol,   is   a  light   yellow   crystalline   solid,
manufactured commercially by hydrolysis of  2-chloro-nitrobenzene
with  aqueous sodium hydroxide.  2-Nitrophenol melts at 45PC  and
has  a  vapor  pressure of 1 mm Hg  at  49°C,   2-Nitrophenol  is
slightly  soluble  in  water (2.1 g/1 at  20°C)  and  soluble  in
organic  solvents.   This phenol does not react to give  a  color
with 4-amino-antipyrene, and therefore does not contribute to the
nonconventional pollutant parameter "Total.Phenols."  U.S. annual
production is 5,000 to 8,000 tons.

The   principle  use  of  ortho-nitrophenol  is   to   synthesize
ortho-aminophenol,   ortho-nitroanisole,   and   other   dyestuff
intermediates.

The  toxic  effects  of 2-nitrophenol on  humans  have  not  been
extensively  studied.   Data  from  experiments  with  laboratory
animals indicate that exposure to this compound causes kidney and
liver  damage.   Other; studies indicate that the  compound  acts
directly  on cell membranes,  and inhibits ,certain enzyme systems
in vitro.                                  .
                               73

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 No  information  regarding   pqtential   teratogencity   was   found.
 Available   data  indicate   that  this compound   does   not   pose   a
 mutagenic  hazard to humans.    Very  limited  data for 2-nitrophenol
 do not  reveal  potential  carcinogenic effects.

 The  available data base is  insufficient  to establish an   ambient
 water  criterion for protection  of  human  health from  exposure   to
 2-nitrophenol.    No  data are  available on  which to evaluate  the
 adverse effects of  2-nitrophenol on aquatic life.

 Data on the behavior of  2-nitrophenol  in  POTW were not available.
 However,    laboratory-scale  studies   have   been  conducted    at
 concentrations  higher   than  those expected   to be found    in
 municipal    wastewater.   Biochemical   oxidation using    adapted
 cultures from  various sources  produced 95 percent degradation   in
 three  to  six  days  in one study.  Similar results were  reported
 for other  studies.   Based on these  data,  and general  observations
 relating molecular  structure to  ease of biological oxidation,   it
 is expected that 2-nitrophenol will be biochemically  oxidized   to
 a   lesser  extent than domestic sewage  by  biological treatment   in.
 POTWs.

 4-Nitrophenol   (58).     4-Nitrophenol   (NO2C6H4OH).   also   called
 paranitrophenol,  is a colorless to yellowish   crystalline  solid
 manufactured commercially by hydrolysis of   4-chloro-nitrobenzene
 with aqueous   sodium hydroxide.  4-Nitrophenol  melts  at   114°C.
 Vapor pressure  is not cited  in the  usual  sources.   4-Nitrophenol
 is  slightly  soluble in water (15  mg/1 at  25°C)  and   soluble   in
 organic  solvents.    This phenol  does  not react  to give  a  color
 with 4-aminoantipyrene,  and  therefore  does  not  contribute  to  the
 nonconventional  pollutant parameter "Total  Phenols."   U.S.  annual
 production  is  about  20,000 tons.

 Paranitrophenol  is used  to prepare  phenetidine,  acetaphenetidine,
 azo and sulfur  dyes,  photochemicals, and  pesticides.

 The  toxic   effects   of  4-nitrophenol  on  humans  have  not  been
 extensively  studied.    Data   from  experiments   with  laboratory
 animals  indicate  that  exposure to   this   compound   results   in
methemoglobinemia   (a metabolic  disorder  of  blood),  shortness   of
 breath,  and stimulation followed by depression.   Other  studies
 indicate  that  the compound  acts directly on cell membranes,  and
 inhibits  certain  enzyme  systems  in  vitro.    No    information
 regarding  potential  teratogenicity was  found.   Available  data
 indicate  that  this  compound does not pose a mutagenic hazard   to
humans.   Very   limited  data  for   4-nitrophenol  do  not   reveal
potential  carcinogenic  effects, although the compound  has  been
 selected  by the National Cancer Institute for  testing under  the
Carcinogenic Bioassay Program.

No  U.S. standards for exposure to 4-nitrophenol  in ambient water
have been established.

Data  on  the  behavior  of  4-*-nitrophenol   in   a  POTW  are  not
available.   However, laboratory-scale studies have been conducted
                               74

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
at  concentrations  higher  than those expected to  be  found  in
municipal  wastewaters.   Biochemical  oxidation  using   adapted
cultures from various sources produced 95 percent degradation  in
three  to six days in one study.  Similar results  were  reported
for  other  studies.   Based  on  these  data,  and  on   general
observations  relating molecular structure to ease of  biological
oxidation,  it  is  concluded that complete  or  nearly  complete
removal of 4-nitrophenol occurs during biological treatment in  a
POTW.

2,4-Dinitrophenol  (59) .  2,4-Dinitrophenol (€5114^05),  a yellow
crystalline solid, is manufactured by hydrolysis of  2,4-dinitro-
1-chlorobenzene with sodium hydroxide. 2,4-Dinitrophenol sublimes
at  114°C.  Vapor pressure is not cited in usual sources.  It  is
slightly  soluble  in  water (7.0 mg/1 at 25°C)  and  soluble  in
organic   solvents.    This  phenol  does  not  react   with   4-
aminoantipyrene   and  therefore  does  not  contribute  to   the
nonconventional pollutant parameter "Total Phenols."  U.S. annual
production is about 500 tons.
2,4-Dinitrophenol  is used to manufacture sulfur and
photochemicals, explosives, and pesticides.
           azo  dyes,
The  toxic  effects of 2,4-dinitrophenol in humans  is  generally
attributed    to    their   ability   to    uncouple    oxidative
phosphorylation.   in  brief,  this means  that  sufficient  2,4-
dinitrophenol   short-circuits  cell  metabolism  by   preventing
utilization  of  energy provided by respiration  and  glycolysis.
Specific  symptoms are gastrointestinal  disturbances,  weakness,
dizziness,  headache, and loss to weight.  More  acute  poisoning
includes symptoms such as:  burning thirst, agitation,  irregular
breathing,  and  abnormally  high  fever.   This  compound   also
inhibits  other  enzyme systems, and acts directly  on  the  cell
membrane,  inhibiting chloride permeability.  Ingestion  of  2,4-
dinitrophenol also causes cataracts in humans.

Based   on   available  data  it  appears  unlikely   that  •2,4-
dinitrophenol  poses a teratogenic hazard to humans.  Results  of
studies  of mutagenic activity of this compound are  inconclusive
as far as humans are concerned.  Available data suggest that 2,4-
dinitrophenol does not possess carcinogenic properties.

To  protect  human  health  from  the  adverse  effects  of  2,4-
dinitrophenol  ingested  in  contaminated  water  and  fish,  the
suggested water quality criterion is 0.0686 mg/1.

Data  on  the  behavior of 2,4-dinitrophenol in a  POTW  are  not
available.  However, laboratory-scale studies have been conducted
at  concentrations  higher  than those expected to  be  found  in
municipal  wastewaters.   Biochemical  oxidation using a  phenol-
adapted  seed  culture  produced 92 percent  degradation  in  3.5
hours.   Similar results were reported for other studies.   Based
on  these data,  and on general observations  relating  molecular
structure ' to ease of biological oxidation,  it is concluded that
complete  or nearly complete removal of 2,4-dinitrophenol  occurs
                               75

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           GENERAL DEVELOPMENT DOCUMENT
:SECT  - VI
during biological treatment in a POTW.

4,6-Dinitro-o-cresol  (60).   4,6-Dinitro-o-cresol  (DNOC)  is  a
yellow  crystalline solid derived from o-cresol.   DNOC melts  at
85.8°C and has a vapor pressure of 0.000052 mm Hg at 20°C.   DNOC
is  sparingly soluble in water (100 mg/1 at 20°CJ,  while  it  is
readily  soluble in alkaline agueous solutions, "ether,  acetone,
and  alcohol.   DNOC  is  produced  by . sulfonation  of  o-cresol
followed by treatment with nitric acid.

DNOC is used primarily as a blossom thinning agent on fruit trees
and  as  a fungicide, insecticide, and miticide  on  fruit  trees
during  the dormant season.  It is highly toxic to plants in  the
growing  stage.   DNOC  is not manufactured in  the  U.S.  as  an
agricultural  chemical.   Imports of DNOC  have  been  decreasing
recently with only 30,000 pounds imported in 1976.

While  DNOC is highly toxic to plants, it is also very  toxic  to
humans  and  is  considered  to be  one  to  the  more  dangerous
agricultural  pesticides.   The available  literature  concerning
humans  indicates  that  DNOC may be absorbed  in  acutely  toxic
amounts  through the respiratory and gastrointestinal tracts  and
through the skin, and that it accumulates in the blood.  Symptoms
of  poisoning include profuse sweating, thirst, loss  of  weight,
headache, malaise, and yellow staining to the skin, hair, sclera,
and conjunctiva.
There  is  no  evidence  to suggest  that  DNOC  is
mutagenic, or carcinogenic.  The effects of DNOC in
to  chronic  exposure  are basically the same ' as
resulting  from  acute exposure..  Although DNOC is
cumulative  poison  in  humans, cataract formation
chronic  effect noted in any human or experimental
it  is believed that DNOC accumulates in the human
toxic symptoms may develop when blood levels exceed
          teratogenic,
         the human due
        those  effects
         considered  a
         is  the  only
        animal  study.
        body and  that
         20 mg/kg.
For  the protection of human health from the toxic properties  of
dinitro-o-cresol ingested through ,water and contaminated  aquatic
organisms, the ambient water criterion is determined to be 0.0134
mg/1.   If  contaminated  aquatic organisms alone  are  consumed,
excluding  the consumption of water,  the ambient water criterion
is determined to be 0.765 mg/1.   No data are available on  which
to  evaluate  the  adverse  effects  of  4,6-dinitro-o-cresol  on
aquatic life.

Some studies have been reported regarding the behavior of DNOC in
POTW.   Biochemical oxidation !of DNOC under laboratory conditions
at a concentration of 100 mg/1 produced 22 percent degradation in
3.5  hours,  using acclimated phenol adapted seed  cultures.   In
addition,   the nitro group in the number 4 (para) position seems
to  impart  a destablilizing effect on the  molecule.   Based  on
these  data and general conclusions relating molecular  structure
to  biochemical  oxidation,  it is expected  that  4.6-dinitro-o-
cresol  will  be biochemically oxidized to a lesser  extent  than
domestic sewage by biological treatment in POTW.
                               76

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           GENERAL DEVELOPMENT. DOCUMENT    SECT - VI
N-nitrosodiphenylamine (62) . N-nitrosodiphenylamine [ (CsHs) 2NNO] ,
also called nitrous diphenylamide,  is a yellow crystalline solid
manufactured  by nitrosation of diphenylamine.  it melts at  66°C
and  is  insoluble  in  water, but  soluble  in  several  organic
solvents  other  than hydrocarbons.  Production in the  U.S.  has
approached  1,500  tons  per year.  The compound  is  used  as   a
retarder for rubber vulcanization and as a pesticide for  control
of scorch (a fungus disease of plants) .

N-nitroso  compounds  are acutely toxic to every  animal  species
tested and are also poisonous to humans.   N-nitrosodiphenylamine
toxicity in adult rats lies in the mid range of the values for 60
N-nitroso compounds tested.  Liver damage is the principal  toxic
effect.     N-nitrosodiphenylamine,   unlike   many   other    N-
nitrosoamines,   does   not   show   mutagenic   activity.     N-
nitrosodiphenylamine has been reported by several  investigations
to  be  non-carcinogenic.  However, the compound  is  capable  of
trans-nitrosation  and  could  thereby convert  other  amines  to
carcinogenic N-nitrosoamines.  Sixty-seven of 87  N-nitrosoamines
studied  were reported to have carcinogenic activity.   No  water
quality criteria have been proposed for N-nitrosodipheriylamine.

No  data are available on the behavior of  N-nitrosodiphenylamine
in  a POTW.  Biochemical oxidation of many of the  toxic  organic
pollutants  have been investigated, at least in  laboratory-scale
studies,  at  concentrations  higher than those  expected  to  be
contained  in most municipal wastewaters.   General  observations
have  been  developed  relating molecular structure  to  ease  of
degradation for all the toxic organic pollutants.  The conclusion
reached by study of the limited data is that biological treatment
produces .little  or no removal of  N-nitrosodiphenylamine  in   a
POTW.    No   information   is   available   regarding   possible
interference  by N-nitrosodiphenylamine in POTW processes, or  on
the possible detrimental effect on sludge used to amend soils  in
which  crops are grown.  However, no interference or  detrimental
effects  are  expected  because N-nitroso -compounds  are  widely
distributed   in   the  soil  and  water  environment,    at   low
concentrations,  as a result of microbial action on nitrates  and
nitrosatable compounds.
Pentachlorophenol (64) .    Pentachlorophenol (CsClsOH) is a  white
crystalline solid produced commercially by chlorination of phenol
or  polychlorophenols.   U.S.  annual production is in excess  of
20,000  tons.   Pentachlorophenol melts at 190°C and is  slightly
soluble in water (14 mg/1).  Pentachlorophenol is not detected by
the 4-amino antipyrene method.

Pentachlorophenol  is a bactericide and fungicide and is used for
preservation of wood and wood products.   It is competitive  with
creosote in that application.   It is also used as a preservative
in glues,  starches, and photographic papers.   It is an effective
algicide and herbicide.

Although  data  are available on the human  toxicity  effects  of
                               77

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GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VI
pentachlorophenol,   interpretation   of   data   is   frequently
uncertain.  Occupational exposure observations must  be  examined
carefully  because  exposure to pentachlorophenol  is  frequently
accompanied   by   exposure   to   other   wood    preservatives.
Additionally,   experimental  results and  occupational  exposure
observations  must  be  examined  carefully  to  make  sure  that
observed effects are produced by the pentachlorophenol itself and
not    by    the   by-products    which    usually    contaminate
pentachlorophenol.

Acute  and chronic toxic effects of pentachlorophenol in  humans
are  similar:   muscle  weakness,  headache,  loss  of  appetite,
abdominal pain,  weight loss,  and irritation of skin,  eyes, and
respiratory   tract.    Available   literature   indicates   that
pentachlorophenol  does  not accumulate in body  tissues  to  any
significant   extent.    Studies   on   laboratory   animals   of
distribution  of the compound in body tissues showed the  highest
levels  of  pentachlorophenol in liver,  kidney,  and  intestine,
while the lowest levels were in brain, fat, muscle, and bone.

Toxic  effects of pentachlorophenol in aquatic organisms are much
greater  at  pH 6 where this weak acid is  predominantly  in  the
undissociated   form   than  at  pH  9  where  the   ionic   form
predominates.   Similar  results were observed in  mammals  where
oral  lethal  doses  of pentachlorophenol  were  lower  when  the
compound  was  administered in hydrocarbon  solvents  (un-ionized
form)  than when it was administered as the sodium salt  (ionized
form) in water.

There  appear  to be no significant  teratogenic,  mutagenic,  or
carcinogenic effects of pentachlorophenol.

For  the protection of human health from the toxic properties  of
pentachlorophenol ingested through water and through contaminated
aquatic organisms, the ambient water quality criterion is  deter-
mined to be 0.140 mg/1.

Only  limited data .are available for reaching  conclusions  about
the  behavior of pentachlorophenol in a POTW.   Pentachlorophenol
has been found in the influent to a POTW.  In a study of one POTW
the  mean  removal  was  59  percent  over  a
Trickling   filters   removed   44  percent
pentachlorophenol, suggesting that biological degradation occurs.
The same report compared removal of pentachlorophenol at the same
plant  and  two additional POTW facilities on a  later  date  and
obtained values of 4.4, 19.5, and 28.6 percent removal, the  last
value  being  for the plant which was 59 percent removal  in  the
original  study.   Influent concentrations  of  pentachlorophenol
ranged from 0.0014 to 0.0046 mg/1.  Other studies, including  the
general review of data relating molecular structure to biological
oxidation,  indicate  that pentachlorophenol is  not  removed  by
biological  treatment processes in a POTW.   Anaerobic  digestion
processes are inhibited by 0.4 mg/1 pentachlorophenol.

The low water solubility and low volatility of  pentachlorophenol
                                    seven-day  period.
                                   at   the   influent
                    78

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
lead  to the expectation that most of the compound will remain in
the sludge in a POTW.  The effect on plants grown on land treated
with   pentachlorophenol-containing  sludge   is   unpredictable.
Laboratory   studies  show  that  this  compound   affects   crop
germination   at  5.4  mg/1.   However,   photodecomposition   of
pentachlorophenol occurs in sunlight.  The effects of the various
breakdown products which may remain in the soil were not found in
the literature.

Phenol  (65) .   Phenol, also called hydroxybenzene  and  carbolic
acid, is a clear, colorless, hygroscopic, deliquescent,  crystal-
line  solid at room temperature.  Its melting point is  43°C  and
its vapor pressure at room temperature is 0.35 mm Hg.  It is very
soluble  in  water  (67  gm/1 at 1°C) and  can  be  dissolved  in
benzene,   oils,   and   petroleum  solids.    Its   formula   is
Although  a small percent of the annual production of  phenol  is
derived  from coal tar as a naturally occurring product, most  of
the  phenol  is synthesized.  Two of the methods  are  fusion  of
benzene sulfonate with sodium hydroxide, and oxidation of  cumene
followed  by cleavage with a catalyst.  Annual production in  the
U.S.  is  in  excess of one million tons.   Phenol  is  generated
during distillation of wood and the microbiological decomposition
of organic matter in the mammalian intestinal tract.

Phenol  is used as a disinfectant,  in the manufacture of resins,
dyestuffs,  and in Pharmaceuticals,  and in the photo  processing
industry.   In  this discussion,  phenol is the specific compound
which  is  separated  by  methylene  chloride  extraction  of  an
acidified sample and identified and quantified by GC/MS.   Phenol
also     contributes to the "Total Phenols," discussed  elsewhere
which are    determined by the 4-AAP colorimetric method.

Phenol  exhibits  acute  and  sub-acute toxicity  in  humans  and
laboratory animals.   Acute oral doses of phenol in humans  cause
sudden     collapse  and  unconsciousness by its  action  on  the
central  nervous    system.   Death occurs by respiratory arrest.
Sub-acute  oral     doses  in mammals are  rapidly  absorbed  and
quickly distributed to    various organs,  then cleared from  the
body by urinary excretion    and metabolism.   Long-term exposure
by   drinking  phenol-contaminated  water  has  resulted  in   a
statistically   significant  increase     in  reported  cases  of
diarrhea,   mouth  sores,   and  burning  of  the     mouth.   In
laboratory  animals, long-term oral administration at low  levels
produced  slight liver and kidney damage. No reports  were  found
regarding  carcinogenicity of phenol administered orally  —  all
carcinogenicity studies were skin test.

For  the protection of human health from phenol ingested  through
water   and   through   contaminated   aquatic   organisms,   the
concentration in water should not exceed 3.4 mg/1.

Fish-"  and  other aquatic organisms demonstrated a wide  range  of
sensitivities to phenol concentration.   However,  acute toxicity
                               79

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 values  were  at  moderate levels when compared
 organic pollutants.
      to  other  toxic
 Data  have  been developed on  the behavior of phenol  in  a  POTW.
 Phenol  is biodegradable by biota present in a POTW.   The  ability
 of  a   POTW   to  treat  phenol-bearing  influents  depends   upon
 acclimation   of  the  biota  and  the  constancy  of  the  phenol
 concentration. It appears that an induction period is required  to
 build   up the population of organisms which can  degrade  phenol.
 Too large a concentration will result in upset or pass though   in
 the  POTW,  but the specific level causing upset depends  on  the
 immediate past history of phenol concentrations in the  influent.
 Phenol  levels  as  high as 200 mg/1 have been  treated  with   95
 percent removal in a POTW, but more or less continuous  presence
 of   phenol   is  necessary  to  maintain   the   population    of
 microorganisms that degrade phenol.

 Phenol  which  is not degraded is expected to pass through the POTW
 because of its very high water solubility.   However,  in a  POTW
 where   chlorination  is  practiced for disinfection of  the  POTW
 effluent, chlorination of phenol may occur.  The products of that
 reaction may  be toxic pollutants.

 The   EPA   has   developed  data  on   influent   and   effluent
 concentrations   of  total  phenols  in  a  study  of  103   POTW
 facilities.   However,  the  analytical procedure was  the  4-AAP
 method  mentioned  earlier and not the GC/MS method   specifically
 for  phenol.  Discussion of the study,  which of course  includes
 phenol, is presented under the pollutant heading "Total Phenols."

 Phthalate   Esters  (66-71).    Phthalic  acid   or   1,2-benzene-
 dicarboxylic  acid,  is one of three isomeric  benzenedicarboxylic
 acids produced by the chemical industry.   The other  two isomeric
 forms are called isophthalic and terephthalic acids.  The formula
 for all three acids is C6H4(COOH)2.  Some esters of phthalic acid
 are designated as toxic pollutants.   They will be discussed as a
 group   here,,  and  specific  properties of  individual  phthalate
 esters will be discussed afterwards.

 Phthalic  acid esters are manufactured in the U.S. at  an  annual
 rate  in  excess  of  one  billion  pounds.   They  are  used  as
 plastiizers,  primarily in the production of  polyvinyl  chloride
 (PVC)    resins.   The most widely used  phthalate  plasticizer  is
 bis(2ethylhexyl)   phthalate (66)  which accounts for  nearly  one-
 third of the phthalate esters produced.   This particular ester is
 commonly referred to as dioctyl phthalate (OOP) and should not be
 confused  with one of the less used esters, di-n-octyl  phthalate
 (69),  which is also used as a plasticizer.   In addition to  these
 two  isomeric  dioctyl phthalates,  four  other esters,  also  used
 primarily  as plasticizers,  are designated as  toxic  pollutants.
 They  are:    butyl benzyl phthalate  (67),  . di-n-butyl  phthalate
 (68),  diethyl phthalate (70),  and dimethyl phthalate  (71).

 Industrially,    phthalate  esters  are  prepared  from   phthalic
anhydride  and  the  specific alcohol to form  the  ester.    Some
                               80

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           GENERAL DEVELOPMENT DOCUMENT  :, SECT - VI
evidence  is available suggesting that phthalic acid esters  also
may  be  synthesized by certain plant and  animal  tissues.   The
extent to which this occurs in nature is not known.

Phthalate   esters  used  as  plasticizers  can  be  present   in
concentrations  up to 60 percent of the total weight of  the  PVC
plastic. The plasticizer is not linked by primary chemical  bonds
to  the  PVC resin.  Rather, it is locked into the  structure  of
intermeshing polymer molecules and held by van der Waals  forces.
The   result  is  that  the  plasticizer  is  easily   extracted.
Plasticizers  are  responsible for the odor associated  with  new
plastic  toys  or  flexible sheet that has been  contained  in  a
sealed package.

Although  the phthalate esters are not soluble or are  only  very
slightly soluble in water, they do migrate into aqueous solutions
placed in contact with the plastic.   Thus, industrial facilities
with tank linings,  wire and cable coverings,  tubing,  and sheet
flooring  of PVC are expected to discharge some phthalate  esters
in  their raw waste.   In addition to their use as  plasticizers,
phthalate  esters  are  used in lubricating  oils  and  pesticide
carriers.   These also can contribute to industrial discharge  of
phthalate esters.

From the accumulated data on acute toxicity in animals, phthalate
esters  may  be  considered  as having  a  rather  low  order  of
toxicity.   Human toxicity data are limited.  It is thought  that
the toxic effects of the esters is most likely due to one of  the
metabolic  products,  in particular the  monoester.   Oral  acute
toxicity  in  animals is greater for the lower  molecular  weight
esters than for the higher mol'ecular weight esters.

Orally administered phthalate esters generally produced enlarging
of liver and kidney, and atrophy of testes in laboratory animals.
Specific   esters  produced  enlargement  of  heart  and   brain,
spleenitis, and degeneration of central nervous system tissue.

Sub-acute   doses  administered  orally  to  laboratory   animal,s
produced  some decrease in growth and degeneration of the testes.
Chronic studies in animals showed similar effects to those  found
in acute and sub-acute studies,  but to a much lower degree.  The
same  organs  were enlarged,  but pathological changes  were  not
usually detected.       :

A recent study of several phthalic esters produced suggestive but
not conclusive evidence that dimethyl and diethyl phthalates have
a cancer liability.   Only four of the six toxic pollutant esters
were  included in the study.   Phthalate esters do bioconcentrate
in  fish.   The  factors,  weighted fo-r relative  consumption  of
various  aquatic and marine ;food groups,  are used  to  calculate
ambient  water quality criteria for four phthalate  esters.   The
values are included in the discussion of the specific esters.

Studies  of  toxicity of phthalate esters in freshwater and  salt
water organisms are scarce.   A chronic toxicity test with bis(2-
                               81 GO

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
ethylhexyl)   phthalate  showed  that  significant   reproductive
impairment  occurred at 0.003 mg/1 in the freshwater  crustacean,
Daphnia  magna.   In acute toxicity studies,  saltwater fish  and
organisms  showed sensitivity differences of up to eight-fold  to
butyl benzyl,  diethyl  and dimethyl phthalates.   This  suggests
that each ester must be evaluated individually for toxic effects.

The  behavior of phthalate esters in a POTW has not been studied.
However,  the biochemical oxidation of many of the toxic  organic
pollutants  has "been investigated in laboratory-scale studies  at
concentrations   higher  than  would  normally  be  expected   in
municipal  wastewaters.   Three  of  the  phthalate  esters  were
studied.  Bis(2-ethylhexyl)  phthalate was found to  be  degraded
slightly or not at all and its removal by biological treatment in
a  POTW is expected to be slight or zero.   Di-n-butyl  phthalate
and  diethyl  phthalate were degraded to a  moderate  degree  and
their  removal by biological treatment in a POTW is  expected  to
occur  to  a  moderate  degree.   Using  these  data  and   other
observations relating molecular structure to ease of  biochemical
degradation of other toxic organic pollutants, the conclusion was
reached that butyl benzyl phthalate and dimethyl phthalate  would
be  removed  in  a  POTW  to  a  moderate  degree  by  biological
treatment.   On the same basis, it was concluded that  di-n-octyl
phthalate would be removed to a slight degree or not at all.   An
EPA study of seven POTW facilities revealed that for all but  di-
n-octyl phthalate, which was not studied, removals ranged from 62
to 87 percent.

No information was found on possible interference wirh POTW oper-
ation or the possible effects on sludge by the phthalate  esters.
The  water - insoluble phthalate esters (butyl benzyl  and  di-n-
octyl  phthalate)  would tend :to remain in sludge,  whereas  the
other   four   toxic  pollutant  phthalgte  esters   with   water
solubilities ranging from 50 mg/1 to 4.5 mg/1 would probably pass
through into the POTW effluent.

Bis(2-ethylhexyl)  Phthalate  (66) .   In addition to the  general
remarks and discussion on phthalate esters,  specific information
on  bis(2-ethylhexyl) phthalate is provided.  Little  information
is  available about the physical properties of  bis(2-ethylhexyl)
phthalate.   It  is a liquid boiling at 387°C at 5 mm Hg  and  is
insoluble  in water.  Its formula is CsH^COOCsHiy^* This  toxic
pollutant  constitutes  about one-third of  the  phthalate  ester
production  in  the U.S.  It is commonly referred to  as  dioctyl
phthalate, or OOP, in the plastics industry where it is the  most
extensively  used  compound for the plasticization  of  polyvinyl
chloride (PVC).  Bis(2-ethylhexyl) phthalate has been approved by
the  FDA for use in plastics in contact with food. Therefore,  it
may  be  found in wastewaters coming in  contact  with  discarded
plastic  food  wrappers  as  well as the  PVC  films  and  shapes
normally  found  in industrial plants.  This toxic  pollutant  is
also  a commonly used organic diffusion pump oil, where  its  low
vapor pressure is an advantage.

For  the protection of human health from the toxic properties  of
                               82

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 bis(2-ethylhexyl)   phthalate ingested through water  and  through
 contaminated   aquatic  organisms,  the  ambient  water   quality
 criterion  is determined to be 15 mg/1.  If contaminated  aquatic
 organisms alone are consumed,  excluding the consumption of water,
 the ambient water  criteria is  determined to be 50 mg/1.

 Although  the behavior of bis(2-ethylhexyl) phthalate in  a  POTW
, has  not  been  studied,  biochemical  oxidation  of  this  toxic
 pollutant   has   been   studied  on  a   laboratory   scale   at
 concentrations  higher  than   would  normally  be  expected   in
 municipal wastewater.   In fresh water with a non-acclimated  seed
 culture,  no biochemical oxidation was observed after 5, 10,  and
 20  days.  However, with an acclimated seed  culture,  biological
 oxidation occurred to  the extents of 13, 0, 6, and 23 percent  of
 theoretical  after 5,  10, 15,  and 20 days, respectively.   Bis(2-
 ethylhexyl)  phthalate concentrations were 3 to 10 mg/1.   Little
 or  no  removal of bis(2-ethylhexyl)  phthalate  by  biological
 treatment in a POTW is expected.

 Butyl Benzyl Phthalate (67).    In addition to the general remarks
 and discussion on  phthalate esters,  specific information on butyl
 benzyl  phthalate  is provided.    No information was found on  the
 physical properties of this compound.

 Butyl  benzyl phthalate is used as a plasticizer  for  PVC.    Two
 special   applications  differentiate  it  from  other  phthalate
 esters.   It  is  approved by  the U.S.  FDA for food  contact  in
 wrappers  and  containers,  and it is the industry  standard  for
 plasticization  of  vinyl  flooring  because  it  provides  stain
 resistance.

 No  ambient water  quality criterion is proposed for butyl  benzyl
 phthalate.
 Butyl  benzyl phthalate  removal  in  a  POTW  by  biological
 is  expected to  occur  to a moderate degree.
             treatment
 Di-n-butyl   Phthalate  (68) .    In  addition  to  the.general   remarks
 and  discussion on phthalate  esters,   specific  information on  di-
 n-butyl  phthalate  (DBP)  is provided.    DBF is  a   colorless    oil
 liquid,   boiling  at   340°C.   Its  water  solubility  at  room
 temperature   is  reported to be 0.4  g/1  and  4.5  g/1   in   two
 different    chemistry   handbooks.     The   formula   for    DBP,
 CsH4(COOC4H9)2  is   the  same as for  its   isomer,  di-isobutyl
 phthalate.    DBP  production   is  1 to  2  percent   of  total  U.S.
 phthalate ester production.

 Dibutyl  phthalate is  used to a limited  extent  as  a  plasticizer
 for  polyvinyl  chloride  (PVC).    It is  not approved for   contact
 with food.   It is used in liquid  lipsticks and  as  a dilluent   for
 polysulfide   dental  impression   materials.   DBP   is  used as  a
 plasticizer   for  nitrocellulose  in making gun  powder, and as  a
 fuel  in  solid  propellants   for rockets.   Further  uses    are
 insecticides,  safety   glass   manufacture,  textile   lubricating
 agents,  printing  inks,  adhesives, paper  coatings,  and resin
                               83

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           GENERAL DEVELOPMENT DOCUMENT    SECT - VI
solvents.
For  protection  of  human health from the  toxic  properties  of
dibutyl phthalate ingested through water and through contaminated
aquatic  organisms,  the  ambient  water  quality  criterion   is
determined  to  be 34 mg/1.  If  contaminated  aquatic  organisms
alone  are  consumed,  excluding the consumption  of  water,  the
ambient water criterion is 154 mg/1.

Although  the behavior of di-n-butyl phthalate in a POTW has  not
been  studied,  biochemical oxidation of this toxic pollutant has
been studied on a laboratory scale at concentrations higher  than
would normally be expected in municipal wastewaters.  Biochemical
oxidation of 35, 43, and 45 percent of theoretical oxidation were
obtained after 5,  10,  and 20 days,  respectively,  using sewage
microorganisms as an unacclimated seed culture.

Biological  treatment in a POTW is expected to remove  di-n-butyl
phthalate to a moderate degree.

Di-n-octyl  Phthalate (69).   In addition to the general  remarks
and discussion on phthalate esters, specific information on di-n-
octyl  phthalate is provided.   Di-n-octyl phthalate is not to be
confused  with the isomeric bis(2-ethylhexyl) phthalate which  is
commonly  referred  to in the plastics industry  as  DOP.   Di-n-
octyl phthalate is a liquid which boils at 220°C at 5 mm Hg.   It
is insoluble in water.  Its molecular formula is CeH^COOCsH]^^-
Its production constitutes about 1 percent of all phthalate ester
production in the U.S.

Industrially,   di-n-octyl  phthalate  is  used   to   plasticize
polyvinyl chloride (PVC) resins.

No  ambient  water quality criterion is proposed  for  di-n-octyl
phthalate.

Biological  treatment in a POTW is expected to lead to little  or
no removal of di-n-octyl phthalate.

Diethyl  Phthalate (70) .   In addition to the general remarks and
discussion oh phthalate esters,  specific information on  diethyl
phthalate is provided.  Diethyl phthalate, or DEP, is a colorless
liquid  boiling  at  296°C,  and  is  insoluble  in  water.   Its
molecular  formula  is  C6H4(COOC2H5)2-   Production  of  diethyl
phthalate  constitutes  about  1.5  percent  of  phthalate  ester
production in the U.S.

Diethyl phthalate is approved for use in plastic food  containers
by the U.S.  FDA.  In addition to its use as a polyvinyl chloride
(PVC)  plasticizer,  DEP is used to plasticize cellulose  nitrate
for gun powder, to dilute polysulfide dental impression materials
and   as  an  accelerator  for  dyeing  triacetate  fibers.    An
additional use which would contribute to its wide distribution in
the  environment is as an approved special denaturant  for  ethyl
alcohol.   The  alcohol-containing.products for which DEP   is  an


                               84

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
approved  denaturant include a wide range of personal care  items
such as bath preparations, bay rum, colognes, hair  preparations,
face  and hand creams, perfumes and toilet soaps.   Additionally,
this  denaturant  is  approved  for  use  in  biocides,  cleaning
solutions,  disinfectants,  insecticides,  fungicides,  and  room
deodorants  which have ethyl alcohol as part of the  formulation.
It is expected, therefore,  that people and buildings would  have
some surface loading of this toxic pollutant which would find its
way into raw wastewaters.

For  the protection of human health from the toxic properties  of
diethyl  phthalate ingested through water and through contaminate
aquatic organisms,  the ambient water quality criterion is deter-
mined  to be 350 mg/1.   If contaminated aquatic organisms  alone
are  consumed,  excluding the consumption of water,  the  ambient
water criterion is 1,800 mg/1.

Although the behavior of diethyl phthalate in a POTW has not been
studied,  biochemical oxidation of this toxic pollutant has  been
studied on a laboratory scale at concentrations higher than would
normally  be  expected  in  municipal  wastewaters.   Biochemical
oxidation  of 79, 84, and 89 percent of theoretical was  observed
after 5, 15, and 20 days, respectively.  Biological treatment  in
a  POTW  is expected to lead to a moderate degree of  removal  of
diethyl phthalate.

Dimethyl Phthalate (71).   In addition to the general remarks and
discussion on phthalate esters,  specific information on dimethyl
phthalate (DMP) is Provided.  DMP has the lowest molecular weight
of the phthalate esters - M.W. = 194 compared to M.W. of 391  for
bis(2-ethylhexyl)   phthalate.   DMP  has  a  boiling  point   of
282(->C.  It is a colorless liquid, soluble in water to the  extent
of 5 mg/1.  its molecular formula is C6H4(COOCH3)2•

Dimethyl phthalate production in the U.S. is just under 1 percent
of total phthalate ester production.   DMP is used to some extent
as a plasticizer in cellulosics; however,  its principal specific
use is for dispersion of polyvinylidene fluoride (PVDP).  PVDF is
resistant   to  most  chemicals  and  finds  use  as   electrical
insulation,  chemical process equipment (particularly pipe),  and
as a case for long-life finishes for exterior metal siding.  Coil
coating techniques are used to apply PVDF dispersions to aluminum
or galvanized steel siding.

For  the protection of human health from the toxic properties  of
dimethyl   phthalate   ingested   through   water   and   through
contaminated  aquatic organisms, the ambient water  criterion  is
determined  to  be 313 mg/1.  If contaminated  aquatic  organisms
alone  are  consumed  excluding the  consumption  of  water,  the
ambient water criterion is 2,900 mg/1.

B^sed  on  limited  data  and  observations  relating   molecular
structure  to  ease  of biochemical degradation  of  other  toxic
organic  pollutants, it is expected that dimethyl phthalate  will
be biochemically oxidized to a lesser extent than domestic sewage
                               85

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
by biological treatment in a POTW.

Polynuclear  Aromatic  Hydrocarbons  (72-84).   The   polynuclear
aromatic  hydrocarbons (PAH) selected as toxic pollutants  are  a
group of 13 compounds consisting of substituted and unsubstituted
polycyclic aromatic rings.  These compounds and their structurial
formulae  are shown in Figure VI-3 (page 143). The general  class
of PAH includes heterocyclics, but none of those were selected as
toxic  pollutants.  PAH are formed as the  result  of  incomplete
combustion  when  organic compounds are burned with  insufficient
oxygen.   PAH  are  found  in  coke  oven  emissions,   vehicular
emissions,  and  volatile products of oil and gas  burning.   The
compounds  chosen  as  toxic pollutants  are  listed  with  their
structural   formulae  and  melting  points   (m.p.).    All   are
relatively insoluble in water.

Some  of  these  toxic pollutants have commercial  or  industrial
uses.   Benzo(a)anthracene, benzo(a)pyrene, chrysene, anthracene,
dibenzo(a,h)anthracene,  and pyrene are all used as antioxidants.
Chrysene, acenaphthylene, anthracene, fluorene, phenanthrene, and
pyrene  are all used for synthesis of dyestuffs or other  organic
chemicals.  3,4-Benzofluoranthrene, benzo(k)fluoranthene,  benzo-
(ghi)perylene,   and  indeno  (l,2,3-cd)pyrene  have   no   known
industrial uses, according to the results of  a recent  literature
search.

Several of the PAH toxic pollutants are found in smoked meats, in
smoke  flavoring  mixtures,  in vegetable oils,  and  in  coffee.
Consequently,  they  are  also  found  in  many  drinking   water
supplies.  The wide distribution of these pollutants  in  complex
mixtures with the many other PAHs which have  not been  designated
as toxic pollutants results in exposures to humans that cannot be
associated with specific individual compounds.

The  screening and verification analysis procedures used for  the
toxic  organic pollutants are based on gas  chromatography  (GC).
Three pairs of the PAH have identical elution times on the column
specified in the protocol, which .means that the parameters of the
pair  are not differentiated.  For these three pairs  [anthracene
(78) - phenanthrene (81); 3,4-benzofluoranthene (74) -  benzo(k)-
fluoranthene  (75); and benzo(a)anthracene (72) - chrysene  (76)]
results  are obtained and reported as "either-or."   Either  both
are  present  in the combined concentration reported, or  one  is
present in the concentration reported.

There  are no studies to document the possible carcinogenic risks
to humans by direct ingestion.  Air pollution studies indicate an
excess  of lung cancer mortality among workers exposed  to  large
amounts of PAH containing materials such as coal gas,  tars,  and
coke-oven emissions.   However, no definite proof exists that the
PAH  present  in these materials are responsible for the  cancers
observed.

Animal studies have demonstrated the toxicity of PAH by oral  and
dermal  administration.   The  carcinogenicity  of PAH  has  been
                               86

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
traced  to  formation of PAH metabolites which,  in turn,  lead  to
tumor   formation.   Because  the levels of PAH which induce cancer
are very low,  little work has been done on other health  hazards
resulting  from  exposure.    It  has been established  in  animal
studies that tissue damage and systemic toxicity can result  from
exposure to non-carcinogenic PAH compounds.

Because  there  were no studies available regarding chronic  oral
exposures  to PAH mixtures,   proposed water quality criteria  were
derived using data on exposure to a single compound.  Two studies
were - selected,  one  involving benzo(a)pyrene ingestion and  one
involving  dibenzo(a,h)anthracene  ingestion.    Both  are  known
animal  carcinogens.

For  the   maximum protection of human health from  the  potential
carcinogenic   effects  of   exposure  to   polynuclear   aromatic
hydrocarbons  (PAH) through  ingestion of water  and  contaminated
aquatic  organisms,  the  ambient water  concentration  is  zero.
Concentrations of PAH estimated to result in additional risk of 1
in 100,000 were derived by the EPA and the Agency is  considering
setting criteria at an interim target risk level in the range  of
10 7,   10~6, or 10~5 with corresponding criteria  of  0.000000097
mg/1, 0.00000097 mg/1, and 0.0000097 mg/1, respectively.
No  standard toxicity tests have been reported for freshwater
saltwater organisms and any of the 13 PAH discussed here.
                    or
The behavior of PAH in a POTW has received only a limited  amount
of study.  It is reported that up to 90 percent of PAH entering a
POTW  will  be retained in the sludge generated  by  conventional
sewage  treatment  processes.   Some  of  the  PAH  can   inhibit
bacterial  growth when they are present at concentrations as  low
as  0.018 mg/1.  'Biological treatment in activated  sludge  units
has  been shown to reduce the concentration of  phenanthrene  and
anthracene  to  some  extent; however,  a  study  of  biochemical
oxidation of fluorene on a laboratory scale showed no degradation
after 5, 10, and 20 days.  On the basis of that study and studies
of other toxic organic pollutants, some general observations were
made relating molecular structure to ease of degradation.   Those
-observations  lead to the conclusion that the 13 PAH selected  to
represent  that  group as toxic pollutants will be  removed  only
slightly or not at all by biological treatment methods in a POTW.
Based  on  their  water insolubility and tendency  to  attach  to
sediment  particles,  very  little pass through of  PAH  to  POTW
effluent  is  expected.   Sludge  contamination  is  the   likely
environmental  fate, although no data are available at this  time
to support any conclusions about contamination of land by PAH  on
which sewage sludge containing PAH is spread.

Tetrachloroethylene (85).  Tetrachloroethylene (CC112sCCl2), also
called perchloroethylene and PCE,  is a  colorless,  nonflammable
liquid   produced  mainly  by  two  methods  - chlorination   and
pyrolysis   of  ethane  and  propane,  and   oxychlorination   of
dichloroethane.   U.S.  annual production exceeds  300,000  tons.
PCE boils at 121°C, a vapor pressure of 19 mm Hg at 20°C.  It  is
                               87

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
insoluble in water but soluble in organic solvents.

Approximately  two-thirds of the U.S.  production of PCE is  used
for dry cleaning.   Textile processing and metal  degreasing,  in
equal amounts consume about one-quarter of the U.S. production.

The  principal toxic effect of PCE on humans is  central  nervous
system  depression  when  the  compound  is  inhaled.   Headache,
fatigue,  sleepiness, dizziness, and sensations  of  intoxication
are   reported.   Severity  of  effects  increases   with   vapor
concentration.   High  integrated exposure  (concentration - times
duration) produces kidney and liver damage.  Very limited data on
PCE  ingested by laboratory animals indicate liver damage  occurs
when PCE is administered by that route.  PCE tends to  distribute
to fat in mammalian bodies.

One  report  found  in  the literature  suggests,  but  does  not
conclude, that PCE is teratogenic.  PCE has been demonstrated  to
be a liver carcinogen in B6C3-F1 mice.

For  the  maximum protection of human health from  the  potential
carcinogenic  effects  of exposure to tetrachlorethylene  through
ingestion  of  water  and  contaminated  aquatic  organisms,  the
ambient   water   concentration  is  zero.    Concentrations   of
tetrachloroethylene estimated ggo result . ng additional  lifetime
cancer  risk  levels of 10~7, 10~6, and 10~5  are  0.00002  mg/1,
0.0002 mg/1, and 0.002 mg/1, respectively.

No data were found regarding the behavior of PCE in a POTW.  Many
of the toxic organic pollutants have been investigated,  at least
in laboratory-scale studies,  at concentrations higher than those
expected to be contained by most municipal wastewaters.   General
observations have been developed relating molecular structure  to
ease of degradation for all of the toxic organic pollutants.  The
conclusion  reached  by. the .study of the limited  data  is  that
biological treatment produces a moderate removal of PCE in a POTW
by  degradation.  No information was found to indicate  that  PCE
accumulates  in,, the  sludge,  but some PCE  is  expected  to  be
adsorbed  onto  settling particles.  Some PCE is expected  to  be
volatilized in aerobic treatment processes and little, if any, is
expected to pass through into the effluent from the POTW.

Toluene  (86).   Toluene  is  a clear,  colorless liquid  with  a
benzene-like odor.   It is a naturally occurring compound derived
primarily  from  petroleum  or  petrochemical  processes.    Some
toluene  is obtained from the manufacture of metallurgical  coke;
Toluene is also referred to as toluol, methylbenzene,  methacide,
and  phenylmethane.   It  is an  aromatic  hydrocarbon  with  the
formula  C^R^CE^.  It boils at 111°C and has a vapor pressure  of
Hg  at room temperature.  The water solubility of toluene is  535
mg/1,  and  it is miscible with a variety  of  organic  solvents.
Annual  production  of toluene in the U.S. is  greater  than  two
million metric tons.  Approximately two-thirds of the toluene  is
converted  to  benzene and the remaining 30  percent  is  divided
approximately  equally  into chemical manufacture, and use  as  a
                               88

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
paint solvent and aviation gasoline additive.  An estimated 5,000
metric  tons  is  discharged to the  environment  annually  as  a
constituent in wastewater.

Most  data on the effects of toluene in human and  other  mammals
have been based on inhalation exposure or dermal contact studies.
There  appear to be no reports of oral administration of  toluene
to  human  subjects.  A long-term toxicity study on  female  rats
revealed no adverse effects on growth, mortality, appearance  and
behavior,  organ  to  body  weight  ratios,  blood-urea  nitrogen
levels,   bone  marrow  counts,  peripheral  blood   counts,   or
morphology  of major organs.  The effects of inhaled  toluene  on
the central nervous system, both at high and low  concentrations,
have  been  studied  in humans and  animals.   However,  ingested
toluene is expected to be handled differently by the body because
it is absorbed more slowly and must first pass through the  liver
before  reaching the nervous system.  Toluene is extensively  and
rapidly metabolized in the liver.  One of the principal metabolic
products  of toluene is benzoic acid, which itself seems to  have
little potential to produce tissue injury.

Toluene  does not appear to be teratogenic in laboratory  animals
or  man.   Nor is there any conclusive evidence that  toluene  is
mutagenic.   Toluene  has not been demonstrated to be positive in
any rn vitro mutagenicity or carcinogenicity bioassay system, nor
to be carcinogenic in animals or man.

Toluene  has  been found in fish caught in harbor waters  in  the
vicinity of petroleum and petrochemical plants.  Bioconcentration
studies  have not been conducted,  but  bioconcentration  factors
have been calculated on the basis of the octanol-water  partition
coefficient.

For  the protection of human health from the toxic properties  of
toluene  ingested through water and through contaminated  aquatic
organisms,  the ambient water criterion is determined to be  14.3
mg/1.   If  contaminated- aquatic  organisms alone  are  consumed
excluding  the consumption of water, the. ambient water  criterion
is  424  mg/1.  Available data show that the adverse  effects  on
aquatic life occur at concentrations as low as 5 mg/1.

Acute  toxicity  tests  have been conducted with  toluene  and  a
variety of freshwater fish and Daphnia magna.  The latter appears
to  be significantly more resistant than fish.   No test  results
have  been  reported  for  the  chronic  effects  of  toluene  on
freshwater fish or invertebrate species.

No  detailed  study of toluene behavior in a POTW  is  available.
However,   the  biochemical  oxidation  of  many  of  the   toxic
pollutants  has been investigated in laboratory scale studies  at
concentrations  greater  than those expected to be  contained  by
most  municipal wastewaters.  At toluene  concentrations  ranging
from 3 to 250 mg/1 biochemical oxidation proceeded to 50  percent
of  theoretical  or greater.  The time period varied from  a  few
hours to 20 days depending on whether or not, the seed culture was
                               89

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
acclimated.   Phenol  adapted acclimated seed cultures  gave  the
most rapid and extensive biochemical oxidation.

Based on study of the limited ^data,  it is expected that  toluene
will  be biochemically oxidized to a lesser extent than  domestic
sewage  by  biological treatment in a POTW.   The volatility  and
relatively   low  water  solubility  of  toluene  lead   to   the
expectation  that  aeration  processes  will  remove  significant
quantities  of  toluene from the POTW.  The EPA  studied  toluene
removal in seven POTW facilities.  The removals ranged from 40 to
100  percent. Sludge concentrations of toluene ranged from  54  x
10~3 to 1.85 mg/1.

Trichloroethylene      (87).       Trichloroethylene      (1,1,2-
trichloroethylene or TCE) is a clear, colorless liquid boiling at
87°C. It has a vapor pressure of 77 mm Hg at room temperature and
is  slightly  soluble  in water (1  gm/1).   U.S.  production  is
greater  than 0.25 million metric tons annually.  It is  produced
from tetrachloroethane by treatment with lime in the presence  of
water.

TCE  (CHCl=CCl2)  is  used for vapor phase  degreasing  of  metal
parts,  cleaning and drying electronic components, as  a  solvent
for  paints, as a refrigerant, for extraction of oils, fats,  and
waxes,  and for dry cleaning.  Its widespread use and  relatively
high volatility result in detectable levels in many parts of  the
environment.

Data on the effects produced by ingested TCE are  limited.   Most
studies  have  been  directed at  inhalation  exposure.   Nervous
system  disorders  and  liver , damage  are  frequent  results  of
inhalation exposure.  In the short term exposures, TCE acts as  a
central nervous system depressant - it was used as an  anesthetic
before its other long-term effects were defined.

TCE has been shown to induce transformation in a highly sensitive
in vitro Fischer rat embryo cell system (F1706) that is used  for
identifying, carcinogens.   Severe and persistent toxicity to the
liver  was  recently demonstrated when TCE was shown  to  produce
carcinoma  of the liver in mouse strain B6C3F1.  • One -systematic
study of TCE exposure and the incidence of human cancer was based
on  518 men exposed to TCE.  The authors of that study  concluded
that  although  the  cancer  risk to man  cannot  be  ruled  out,
exposure  to low levels of TCE probably does not present  a  very
serious and general cancer hazard.

TCE is bioconcentrated in aquatic species, making the consumption
of  such species by humans a significant source of TCE.   For the
protection  of  human  health '. from  the  potential  carcinogenic
effects  of  exposure to trichloroethylene. through  ingestion  of
water  and  contaminated  aquatic organisms,  the  ambient  water
concentration  is  zero.    Concentrations  of   trichloroethylene
estimated to result in additional lifetime cancer risks of 10~',
10 6,  and  10~5 are 0.00027 mg/1,  0,0027 mg/1, and  0,027  mg/1,
respectively.   If  contaminated  aquatic  organisms  alone   are

                               90

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
consumed,   excluding  the  consumption  of  water,   the   water
concentration  should  be  less  than  CK807  mg/1  to  keep  the
additional lifetime cancer risk below 10  .

Only  a  very  limited amount of data on the effects  of  TCE  on
freshwater aquatic life are available.  One species of fish (fat-
head  minnows)  showed  a loss of equilibrium  at  concentrations
below those resulting in lethal effects.

The behavior of trichloroethylene in a POTW has not been studied.
However, in laboratory-scale studies of toxic organic pollutants,
TCE was subjected to biochemical oxidation conditions.   After 5,
10,  and 20 days no biochemical oxidation occurred.  On the basis
of  this  study  and  general  observations  relating   molecular
structure to ease of degradation, the conclusion is reached  that
TCE  would undergo no removal by biological treatment in a  POTW.
The  volatility  and relatively low water solubility  of  TCE  is
expected  to  result  in volatilization of some  of  the  TCE  in
aeration steps in a POTW.

Vinyl  Chloride (88).   No freshwater organisms have been  tested
with vinyl chloride and no statement can be made concerning acute
or chronic toxicity.

For  the  maximum protection of human health from  the  potential
carcinogenic  effects  due to exposure of vinyl chloride  through
ingestion   of  contaminated  water  and   contaminated   aquatic
organisms, the ambient water concentrations should be zero  based
on the non-threshold assumption for this chemical.  However, zero
level may not be attainable at the present time.  Therefore,  the
levels  which may result in incremental_jncreas.e of  cancer,  risk
                                                              The
corresponding  recommended criteria are 0.020 mg/1, 0.0020  mg/1,
and  0.00020  mg/1,  respectively.  For  consumption
organisms  only, excluding consumption of water, the
5.246 mg/1, 0.525 mg/1, and 0.052 mg/1, respectively.
            10~7,
           0020
           of  aquatic
           levels  are
Vinyl  chloride  has  been used for over 40  years  in  producing
polyvinyl  chloride (PVC) which in turn is the most  widely  used
material in the manufacture of plastics throughout the world.  Of
the  estimated  18  billion pounds  of  vinyl  chloride  produced
worldwide  in  1972,  about 25 percent was  manufactured  in  the
United States. Production of vinyl chloride in the United  States
reached slightly over 5 billion pounds in 1978.

Vinyl chloride and polyvinyl chloride are used in the manufacture
of numerous products in building and construction, the automotive
industry,  for  electrical wire insulation  and  cables,  piping,
industrial and household equipment, packaging for food  products,
medical  supplies,  and is depended upon heavily by  the  rubber,
paper,  and  glass  industries.   Polyvinyl  chloride  and  vinyl
chloride copolymers are distributed and processed in a variety of
forms   including   dry   resins,   plastisol   (dispersions   in
plasticizers),  organosol   (dispersions  in  plasticizers   plus
volatile  solvent),  and latex (colloidal dispersion  in  water).
                               91

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           GENERAL DEVELOPMENT DOCUMENT
                                    SECT  - VI
Latexes are used to coat or  impregnate paper,  fabric, or leather.

Vinyl  chloride  (CH2CHC1:   molecular weight 62.5)   is  a  highly
flammable  chloroolefinic  hydrocarbon  which  emits  a  sweet  or
pleasant  odor  and has a vapor density slightly more than  twice
that  of air.   It has a boiling point of -13.9°C and  a  melting
point of -153.8°C.  Its solubility in water at 28°C  is 0.11 g/100
g  water and it is soluble in alcohol and very soluble  in  ether
and carbon tetrachloride.  Vinyl chloride is volatile and readily
passes from solution into the gas phase under most laboratory and
ecological  conditions.   Many salts such as soluble  silver  and
copper  salts,  ferrous  chloride,  platinous  chloride,  iridium
dichloride,  and  mercurous  chloride to name  a  few,  have  the
ability  to form complexes with vinyl chloride which  results  in
its  increased  solubility in water.   Conversely,  alkali  metal
salts  such  as  sodium or potassium chloride  may  decrease  the
solubility  of vinyl chloride in ionic strengths of  the  aqueous
solution.   Therefore,  the  amounts of vinyl  chloride  in  water
could be influenced significantly by the presence of salts.

Vinyl chloride introduced into aquatic systems will most probably
be  quickly transferred to the atmosphere through volatilization.
In  fact,  results  from model simulations  indicate  that  vinyl
chloride  should  not remain in an aquatic ecosystem  under  most
natural conditions.

Based on the information found, it does not appear that oxidation
hydrolysis,   biodegradation  or  sorption,  are  important  fate
processes for vinyl'chloride in the aquatic environment.

Based  on  the 1982 POTW study, "Fate of Priority  Pollutants  in
Publicly  Owned Treatment Works, Final Report,"  Effluent  Guide-
lines Division, U.S.  Environmental Protection Agency, EPA  440/1-
82/303, September 1983, the  removal efficiency for vinyl chloride
at a POTW with secondary treatment is 94 percent.

4,4'-ODD (94).   4,4'-DDD is toxic by ingestion, inhalation, 'skin
absorption, and is combustible.
a-Endosulfan-alpha  (95) .   Endosulfan
inhalation and skin absorption.
                                is  toxic  by  ingestion,
a-BHC-alpha  (102).     BHC-alpha  is  toxic  by  ingestion,  skin
absorption,  is  an eye irritant,  and a central  nervous  system
depressant.
b-BHC-beta
highly
absorption.
	  (103) .    BHC-beta is moderately toxic by  inhalation,
toxic  by  ingestion,  and is a strong irritant  by  skin
     It acts as a central nervous system depressant.
Polychlorinated Biphenyls (106 ^ 112).   Polychlorinated biphenyls
(G12H10-ncln'H10-ncln where n can range from 1 to 10),  designated
PCBs,  are  chlorinated derivatives of  biphenyls.  The commercial
products  are  complex mixtures of chlorobiphenyls,  but  are  no
longer produced in the U.S.  The, mixtures produced formerly  were
                               92

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           GENERAL DEVELOPMENT DOCUMENT
           SECT - VI
characterized by the percentage chlorination. Direct chlorination
of biphenyl was used to produce mixtures containing from 21 to 70
percent chlorine.  Seven of these mixtures have been selected  as
toxic pollutants:
 Toxic
 Pollu-
  tant
  No.

 106
 107
 108
 109
 110
 111
 112

Name .
Arochlor
1242
1254
1221
1232
1248
1260
1016
Percent
Chlorine

• 42
54
20.5-21.5
31.4-32.5
48
60
41
Range (°C)
Distilla-
   tion
 325-
 365-
 275-
 290-
 340-
 385-
 323-
366
390
320
325
375
420
356
          Pour
       Point (°C)
  Water
Solubility
-19
10
1
-35.5
- 7
31
—
240
12
<200
—
54
2.7
225-250
The arochlors 1221,  1232,  1016,  1242,  and 1248 are colorless,
oily liquids; 1254 is a viscous liquid; 1260 is a sticky resin at
room temperature.  Total annual U.S. production of PCBs  averaged
about 20,000 tons in 1972 to 1974.

Prior  to 1971,  PCBs  were used in several applications including
plasticizers,   heat   transfer   liquids,   hydraulic    fluids,
lubricants, vacuum pump and compressor fluids, and capacitor  and
transformer  oils.   After 1970, when PCB use was  restricted  to
closed  systems,  the latter two uses were  the  only  commercial
applications.

The  toxic effects of PCB's ingested by humans have been reported
to  range from acne-like skin eruptions and pigmentation  of  the
skin  to  numbness  of limbs,  hearing and vision  problems,  and
spasms.   Interpretation  of results is complicated by  the  fact
that  the very highly toxic polychlorinated dibenzofurans (PCDFs)
are  found in many commercial PCB  mixtures.   Photochemical  and
thermal  decomposition appear to accelerate the transformation of
PCBs to PCDFs.   Thus the specific effects of PCBs may be  masked
by  the  effects  of PCDFs.  However,  if  PCDFs  are  frequently
present to some extent in any PCB mixture, then their effects may
be properly included in the effects of PCB mixtures.

Studies  of effects of PCBs in laboratory animals indicate  that
liver and kidney damage, large weight losses, eye discharges, and
interference  with  some metabolic  processes  occur  frequently.
Teratogenic  effects  of  PCBs in laboratory animals  have  been
observed,  but are rare.   Growth retardations during  gestation,
and  reproductive  failure are more common  effects  observed  in
studies  of  PCB teratogenicity.  Carcinogenic effects   of  PCBs
have been studied in laboratory animals with results  interpreted
as positive.  Specific reference has been made to liver cancer in
rats in the discussion of water quality criterion formulation.

For  the  maximum protection of human health from  the  potential
                               93

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           GENERAL DEVELOPMENT DOCUMENT
                                   SECT - VI
For  the  maximum protection of human health from  the  potential
carcinogenic  effects of exposure to  PCBs through  ingestion  of
water  and  contaminated aquatic organisms,  the  ambient   water
concentration  should be zero.   Concentrations of PCBs  estimated
to  result in additional lifetime cancer risk at risk  levels  of
10
  -7
10
  -b
              and 10 ° are 0.0000000026 mg/1,  0.000000026  mg/1,
and  0.00000026 mg/1, respectively.

The  behavior of PCBs  in a POTW has received limited study.  Most
PCB's will be removed with sludge.   One study showed removals of
82   to  89 percent,  depending on suspended %olid  removal.   The
PCB's adsorb onto suspended sediments and other particulates.  In
laboratory-scale  experiments   with PCS  1221,  81  percent  was
removed by degradation in an activated sludge system in 47 hours.
Biodegradation  can form polychlorinated dibenzofurans which  are
more  toxic   than  PCBs   (as   noted   earlier).    PCBs    at
concentrations of 0.1 to 1,000 mg/1 inhibit or enhance  bacterial
growth  rates,  depending  on  the  bacterial  culture  and   the
percentage chlorine  in the PCB.  Thus, activated sludge may   be
inhibited by  PCBs.  Based on studies of bioaccumulation of  PCBs
in food crops grown on soils amended with PCB-containing  sludge,
the  U.S. FDA has recommended a limit of 10 mg PCB/kg dry  weight
of sludge used for application to soils bearing food crops.

Antimony  (114).    Antimony,   classified  as  a  non-metal   or
metalloid,   is  a  silvery  white,  brittle  crystalline  solid.
Antimony  is  found  in small ore bodies  throughout  the  world.
Principal  ores  are oxides of mixed antimony  valences,  and  an
oxysulfide  ore.   Complex ores with metals are important because
the  antimony is recovered as a by-product.   Antimony  melts  at
631°C, and is a poor conductor of electricity and heat.

Annual U.S. consumption of primary antimony ranges from 10,000 to
20,000  tons.   About half is consumed in metal products - mostly
antimonial lead for lead acid storage batteries,   and about  half
in non-metal products.   A principal compound is antimony trioxide
which 'is  used  as  a flame retardant  in .fabrics,  and  as  an
opacifier  in  glass, ceramics, and  enamels.   Several   antimony
compounds  are used as catalysts in organic chemicals  synthesis,
as fluorinating agents (the antimony fluoride), as pigments,  and
in   fireworks.   Semiconductor  applications  are   economically
significant.

Essentially  no  information  on  antimony-induced  human  health
effects has been derived from community epidemiology studies. The
available  data are in literature relating effects observed  with
therapeutic   or  medicinal  uses  of  antimony   compounds   and
industrial   exposure  studies.   Large  therapeutic   doses   of
antimonial compounds, usually used to treat schistisomiasis, have
caused  severe  nausea,  vomiting,  convulsions,  irregular  heart
action,   liver  damage,   and  skin  rashes.    Studies  of   acute
industrial  antimony  poisoning have revealed loss  of  appetite,
diarrhea,  headache,  and dizziness in addition to  the   symptoms
found in studies of therapeutic doses of antimony.
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For  the protection of human health from the toxic properties  of
antimony ingested through water and through contaminated  aquatic
organisms  the ambient water criterion is determined to be  0.146
mg/1.  If contaminated aquatic organisms are consumed,  excluding
the  consumption of water, the ambient water criterion is  deter-
mined to be 45 mg/1.  Available data show that adverse effects on
aquatic life occur at concentrations higher than those cited  for
human health risks.

Very  little  information is available regarding the behavior  of
antimony  in  a POTW.   The limited solubility of  most  antimony
compounds  expected  in a POTW (i.e.,  the oxides and  sulfides),
suggests that at least part of the antimony entering a POTW  will
be precipitated and incorporated into the sludge.  However,  some
antimony  is  expected to remain dissolved and pass  through  the
POTW  into  the effluent.  Antimony compounds  remaining  in  the
sludge  under  anaerobic conditions may be connected  to  stibine
(SbH3),  a  very soluble and very toxic compound.  There  are  no
data  to show antimony inhibits any POTW processes.  Antimony  is
not  known to be essential to the growth of plants, and has  been
reported  to be moderately toxic.  Therefore,  sludge  containing
large amounts of antimony could be detrimental to plants if it is
applied in large amounts to cropland.

Arsenic   (115).   Arsenic  is  classified  as  a  non-metal   or
metalloid.   Elemental  arsenic  normally exists  in  the  alpha-
crystalline metallic form which is steel gray and brittle, and in
the beta form which is dark gray and amorphous.  Arsenic sublimes
at  615°C.   Arsenic  is widely  distributed  throughout  the
world  in  a  large  number  of  minerals.   The  most  important
commercial source of arsenic is as a by-product from treatment of
copper, lead, cobalt, and gold ores.  Arsenic is usually marketed
as the trioxide (As203).  Annual U.S. production of the  trioxide
approaches 40,000 tons.

The  principal  use  of  arsenic  is  in  agricultural  chemicals
(herbicides) for controlling weeds in cotton fields.   Arsenicals
have  various  applications in. medicinal and veterinary  use,  as
wood preservatives, and in semiconductors.

The effects of arsenic in humans were known by the ancient Greeks
and  Romans.   The principal toxic effects  are  gastrointestinal
disturbances.   Breakdown of red blood cells occurs.  Symptoms of
acute  poisoning  include  vomiting,   diarrhea,  abdominal  pain
lassitude,  dizziness,  and  headache.   Longer exposure produced
dry, falling hair, brittle, loose nails, eczema, and exfoliation.
Arsenicals  also  exhibit teratogenic and  mutagenic  effects  in
humans.   Oral  administration  of  arsenic  compounds  has  been
associated  clinically  with skin cancer for nearly  one  hundred
years.   Since  1888  numerous studies have  linked  occupational
exposure  and therapeutic administration of arsenic compounds  to
increased incidence of respiratory and skin cancer.

For  the  maximum protection of human health from  the  potential
carcinogenic effects of exposure to arsenic through ingestion  of
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           GENERAL DEVELOPMENT DOCUMENT
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water  and  contaminated  aquatic organisms,  the  ambient  water
concentration  is zero.  Concentrations of arsenic  estimated  to
result  in additional lifetime cancer risk levels of 10~,  10~ ,
and  105 are 2.2 x 10-7 mg/1,  2.2 x 10-6 mg/1, and 2.2  x  10-5
mg/lf respectively.  If contaminated aquatic organisms alone  are
consumed,   excluding  the  consumption  of  water,   the   water
concentration  should  be  less  than 1.75 x  10~4  to  keep  the
increased  lifetime cancer risk below 10" .  Available data  show
that  adverse  effects on aquatic life  occur  at  concentrations
higher than those cited for human health risks.

A few studies have been made regarding the behavior of arsenic in
a POTW.  One EPA survey of nine POTW facilities reported influent
concentrations  ranging from 0.0005 to 0.693 mg/1; effluents from
three  POTW  facilities  having  biological  treatment  contained
0.0004 to 0.01 mg/1;  two POTW facilities showed arsenic  removal
efficiencies  of  50  and 71  percent  in  biological  treatment.
Inhibition of treatment processes by sodium arsenate is  reported
to  occur  at  0.1  mg/1 in activated sludge,  and  1.6  mg/1  in
anaerobic  digestion processes.  In another study based  on  data
from  60  POTW facilities, arsenic in sludge ranged from  1.6  to
65.6 mg/kg and the median value was 7.8 mg/kg.  Arsenic in sludge
spread on cropland may be taken up by plants grown on that  land.
Edible  plants can take up arsenic, but normally their growth  is
inhibited before the plants are ready for harvest.

Asbestos  (116).   Asbestos is a generic term used to describe  a
group of hydrated mineral silicates that can appear in a  fibrous
crystal  form (asbestiform) and, when crushed, can separate  into
flexible   fibers.    The  types  of  asbestos   presently   used
commercially  fall into two mineral groups:  the  serpentine  and
amphibole groups.  Asbestos is mineralogically stable and is  not
prone  to significant chemical or biological degradation  in  the
aquatic environment.  In 1978, ;the total consumption of  asbestos
in  the U.S. was 583,000 metric tons.  Asbestos is  an  excellent
insulating  material and is used in a wide variety  of  products.
Based  on  1975 figures, the total annual  identifiable  asbestos
emissions are estimated at 243,527 metric tons.  Land  .discharges
account for 98.3 percent of the emissions, air discharges account
for 1.5 percent, and water discharges account for 0.2 percent.

Asbestos  has  been  found to produce  significant  incidence  of
disease  among  workers  occupationally  exposed  in  mining  and
milling, in manufacturing, and in the use of materials containing
the fiber.  The predominant type of exposure has been inhalation,
although  some  asbestos may be swallowed  directly  or  ingested
after   being   expectorated   from   the   respiratory    tract.
Noncancerous  asbestos   has  been found  among  people  directly
exposed to high levels of asbestos as a result of excessive  work
exposure;  much less frequently, among those with lesser exposures
although  there is extensive evidence of pulmonary disease  among
people exposed to airborne asbestos.  There is little evidence of
disease among people exposed to waterborne fibers.

Asbestos  at  the concentrations currently found in  the  aquatic
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           GENERAL DEVELOPMENT DOCUMENT
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environment  does  not appear to exert toxic effects  on  aquatic
organisms.   For the maximum protection of human health from  the
potential  carcinogenic  effects of exposure to asbestos  through
ingestion  of  water  and  contaminated  aquatic  organisms,  the
ambient  water  concentration should be zero based  on  the  non-
threshold assumption of this substance.  However,  zero level may
not  be attainable at the present time.  Therefore, levels  which
may  result in incremental increase of cancer risk over the  life
time  are estimated at 10 5, 10 6, and 10 7.   The  corresponding
recommended  criteria are 300,000 fibers/1, 30,000 fibers/1,  and
3,000 fibers/1.

The  available  data indicate that technologies used at POTW  for
reducing  levels  of total suspended solids  in  wastewater  also
provide  a  concomitant reduction in asbestos  levels.   Asbestos
removal  efficiencies ranging from 80 percent to greater than  99
percent have been reported following sedimentation of wastewater.
Filtration and sedimentation with chemical addition  (i.e.,  lime
and polymer) have achieved even greater percentage removals.

Beryllium (117).   Beryllium is a dark gray metal of the alkaline
earth  family.  It is relatively rare, but because of its  unique
properties   finds  widespread  use  as  an   alloying   element,
especially  for  hardening  copper  which  is  used  in  springs,
electrical contacts  and non-sparking tools.  World production is
reported to be in the range of 250 tons annually.  However,  much
more  reaches  the  environment as emissions  from  coal  burning
operations.   Analysis  of coal indicates .an  average  beryllium
content of 3 ppm and 0.1 to 1.0 percent in coal ash or fly ash.

The  principal ores are beryl (3BeO'Al203*6Si02) and  bertrandite
(Be4Si2Oy(OH)2)•    Only   two   industrial  facilities   produce
beryllium  in the U.S.  because of limited demand and the  highly
toxic character.   About two-thirds of the annual production goes
into  alloys,  20 percent into heat sinks,  and 10  percent  into
beryllium oxide (BeO) ceramic products.

Beryllium has a specific gravity of 1.846, making it the lightest
metal with a high melting point (1,350° C).  Beryllium alloys
are  corrosion  resistant,   but  the metal corrodes  in  aqueous,
environments.   Most  common beryllium compounds are  soluble  in
water,  at  least  to  the extent necessary to  produce  a  toxic
concentration of beryllium ions.

Most data on toxicity of beryllium is for inhalation of beryllium
oxide  dust.   Some studies on orally administered  beryllium  in
laboratory animals have been reported.   Despite the large number
of  studies  implicating beryllium as a carcinogen,  there is  no
recorded   instance  of  .cancer  being  produced  by   ingestion.
However,   a  recently  convened  panel  of  uninvolved   experts
concluded   that   epidemiologic  evidence  is  suggestive   that
beryllium is a carcinogen in man.             •     .

In  the  aquatic environment,  beryllium is chronically toxic  to
aquatic  organisms at, 0.0053 mg/1.   Water softness has  a  large
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           GENERAL DEVELOPMENT DOCUMENT
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effect on beryllium toxicity to fish.   In soft water,
is  reportedly 100 times as toxic as in hard water.
             beryllium
For  the  maximum protection of human health from  the  potential
carcinogenic  effects of exposure to beryllium through  ingestion
of  water  and contaminated aquatic organisms the  ambient  water
concentration is zero.   Concentrations of beryllium estimatedto
result  in additional lifetime cancer risk levels of 10 ',  10~ ,
and 10 5 are 0.00000068 mg/1, 0.0000068 mg/1, and 0.000068  mg/1,
respectively.   If  contaminated  aquatic  grganisms  alone   are
consumed  excluding the consumption of water,  the  concentration
should  be less than_Q.00115 mg/1 to keep the increased  lifetime
cancer risk below 10~ .

Information  on  the behavior of beryllium in a POTW  is  scarce.
Because beryllium hydroxide is insoluble in water, most beryllium
entering a POTW will probably be in the form of suspended solids.
As  a  result, most of the beryllium will settle and  be  removed
with  sludge.   However,  beryllium has  been  shown  to  inhibit
several  enzyme  systems,  to interfere with  DNA  metabolism  in
liver, and to induce chromosomal and mitotic abnormalities.  This
interference  in cellular processes may extend to interfere  with
biological treatment processes.  The concentration and effects of
beryllium  in sludge which could be applied to cropland have  not
been studied.

Cadmium  (118).   Cadmium is a relatively rare  metallic  element
that  is seldom found in sufficient quantities in a pure state to
warrant  mining or extraction from the earth's  surface.   It  is
found  in  trace  amounts of about 1 ppm throughout  the  earth's
crust.   Cadmium  is,  however, a  valuable  by-product  of  zinc
production.

Cadmium is used primarily as an electroplated metal  and is found
as  an  impurity in the secondary refining  of  zinc,  lead,  and
copper.

Cadmium  is an extremely dangerous cumulative  toxicant,  causing
progressive  chronic poisoning in  mammals,  fish,  and  probably
other organisms.  The metal is not excreted.

Toxic  effects of cadmium on man have been reported from through-
out  the world.   Cadmium may be a factor in the  development  of
such human pathological conditions as kidney disease,  testicular
tumors,   hypertension,     arteriosclerosis,   growth  inhibition,
chronic  disease  of old age, and cancer.   Cadmium  is  normally
ingested by humans through food and water as well as by breathing
air  contaminated by cadmium dust.   Cadmium is cumulative in  the
liver, kidney, pancreas, and thyroid of humans and other animals.

A  severe bone and kidney syndrome known as ita-itai disease  has
been  documented  in  Japan as caused by  cadmium  ingestion  via
drinking water and contaminated irrigation water.   Ingestion  of
as  little as 0.6 mg/day has produced the disease.   Cadmium acts
synergistically with other metals.   Copper and zinc substantially
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
increase its toxicity.

Cadmium   is  concentrated  by  marine  organisms,   particularly
mollusks,  which accumulate cadmium in calcareous tissues and  in
the viscera.  A concentration factor of 1,000 for cadmium in fish
muscle has been reported, as have concentration factors of  3,000
in marine plants and up to 29,600 in certain marine animals.  The
eggs and larvae of fish are apparently more sensitive than  adult
fish  to poisoning by cadmium, and crustaceans appear to be  more
sensitive than fish eggs and larvae.

For  the protection of human health from the toxic properties  of
cadmium  ingested through water and through contaminated  aquatic
organisms,  the ambient water criterion is determined to be 0.010
mg/1.   Available data show that adverse effects on aquatic  life
occur  at  concentrations  in the same range as those  cited  for
human health, and they are highly dependent on water hardness.

Cadmium is not destroyed when it is introduced into a  POTW,  and
will  either pass through to the POTW effluent or be incorporated
into  the POTW sludge.   In addition,  it can interfere with  the
POTW treatment process.

In  a  study of 189 POTW facilities,  75 percent of  the  primary
plants,  57 percent of the trickling filter plants, 66 percent of
the  activated sludge plants,:  and 62 percent of  the  biological
plants  allowed  over 90 percent of the influent cadmium to  pass
through  to  the  POTW  effluent.   Only  two  of  the  189  POTW
facilities  allowed less than 20 percent pass-through,  and  none
less than 10 percent pass-through.  POTW effluent  concentrations
ranged  from  0.001  to  1.97 mg/1  (mean  0.028  mg/1,  standard
deviation 0.167 mg/1).

Cadmium  not  passed  through the POTW will be  retained  in  the
sludge where it is likely to build up in concentration.   Cadmium
contamination  of  sewage sludge limits its use on land since  it
increases  the  level of 'cadmium in the  soil.   Data  show  that
cadmium can be. incorporated into crops,  including vegetables and
grains, from contaminated soils.  Since the crops themselves show
no  adverse  effects  from  soils with levels  up  to  100  mg/kg
cadmium, these contaminated crops could have a significant impact
on  human health.  Two Federal agencies have  already  recognized
the  potential adverse human health effects posed by the  use  of
sludge  on cropland.  The FDA recommends that  sludge  containing
over 30 mg/kg of cadmium should not be used on agricultural land.
Sewage  sludge  contains 3 to 300 mg/kg (dry  basis)  of  cadmium
(mean  = 10 mg/kg, median = "16 mg/kg).  The USDA also  recommends
placing  limits  on  the total cadmium from sludge  that  may  be
applied to land.

Chromium (119).   Chromium is an elemental metal usually found as
a  chromite  (FeO'C^Os).   The  metal is  normally  produced  by
reducing  the oxide with aluminum.   A significant proportion  of
the  chromium  used  is in the form of compounds such  as  sodium
dichromate   (Na2CrO4),   and  chromic  acid   (CrO3)  - both   are
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
hexavalent chromium compounds.

Chromium  is found as an alloying  component of many steels and its
compounds  are  used in electroplating baths   and  as  corrosion
inhibitors for closed water circulation systems.

The  two  chromium  forms  most   frequently  found  in   industry
wastewaters  are hexavalent and trivalent  chromium.   Hexavalent
chromium  is the form used for metal treatments.  Some of  it  is
reduced   to trivalent chromium as part of the  process  reaction.
The  raw  wastewater containing both valence  states  is  usually
treated   first  to  reduce  remaining  hexavalent  to   trivalent
chromium,  and  second to precipitate the trivalent form  as  the
hydroxide.  The hexavalent form is not removed by lime treatment.

Chromium, in its various valence  states, is hazardous to man.  It
can   produce  lung  tumors  when  inhaled,   and  induces   skin
sensitizations.  Large doses of chromates have corrosive  effects
on  the   intestinal  tract  and can  cause  inflammation  of  the
kidneys. Hexavalent chromium is a known human carcinogen.  Levels
of  chromate ions that show no effect in man appear to be so  low
as to prohibit determination, to date.

The  toxicity  of chromium salts  to fish and other  aquatic  life
varies widely with the species,   temperature,  pH, valence of the
chromium, and synergistic or antagonistic effects, especially the
effect  of  water hardness.   Studies have shown  that  trivalent
chromium  is more toxic to fish of some types than is  hexavalent
chromium.  Hexavalent chromium retards growth of one fish species
at  0.0002  mg/1.   Fish food organisms and other lower forms  of
aquatic  life are extremely sensitive  to  chromium.   Therefore,
both hexavalent and trivalent chromium must be considered harmful
to particular fish or organisms.

For  the protection of human health from the toxic properties  of
chromium  (except hexavalent chromium) ingested through water and
contaminated   aquatic  organisms,  the  ambient ' water   quality
criterion  is 170 mg/1.  If contaminated aquatic organisms  alone
are  consumed   excluding the consumption of water,  the  ambient
water  criterion  for  trivalent chromium  is  3,443  mg/1.   The
ambient  water  quality  criterion  for  hexavalent  chromium  is
recommended  to   be  identical to the  existing  drinking  water
standard for total chromium which is 0.050 mg/1.

Chromium  is not destroyed when treated by a POTW  (although  the
oxidation state may change),  and will either pass through to the
POTW  effluent  or be incorporated into the  POTW  sludge.   Both
oxidation states can cause POTW treatment inhibition and can also
limit the usefulness of municipal sludge.

Influent concentrations of chromium to POTW facilities have  been
observed  by EPA to range from 0.005 to 14.0 mg/1,  with a median
concentration  of  0.1  mg/1.   The efficiencies  for  removal  of
chromium  by  the  activated sludge  process  can  vary  greatly,
depending  on chromium concentration in the influent,   and  other
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           GENERAL DEVELOPMENT DOCUMENT
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operating  conditions  at  the POTW.  Chelation  of  chromium  by
organic matter and dissolution due to the presence of  carbonates
can  cause  deviations from the predicted behavior  in  treatment
systems.

The   systematic  presence  of  chromium  compounds   will   halt
nitrification  in  a  POTW for short periods,  and  most  of  the
chromium  will  be  retained in the  sludge  solids.   Hexavalent
chromium  has been reported to severely affect the  nitrification
process,  but  trivalent chromium has little or  no  toxicity  to
activated sludge, except at high concentrations.  The presence of
iron,  copper, and low pH will increase the toxicity of  chromium
in a POTW by releasing the chromium into solution to be  ingested
by microorganisms in the POTW.

The amount of chromium which passes through to the POTW  effluent
depends on the type of treatment processes used by the POTW.   In
a study of 240 POTW facilities, 56 percent of the primary  plants
allowed more than 80 percent pass-through to POTW effluent.  More
advanced  treatment results in less pass-through.  POTW  effluent
concentrations ranged from 0.003 to 3.2 mg/1 total chromium (mean
=  0.197, standard deviation = 0.48), and from 0.002 to 0.1  mg/1
hexavalent chromium (mean = 0.017, standard deviation = 0.020).

Chromium  not  passed through the POTW will be  retained  in  the
sludge,  where it is likely to build up in concentration.  Sludge
concentrations of total chromium of over 20,000 mg/kg (dry basis)
have  been  observed.   Disposal of sludges containing very  high
concentrations  of  trivalent  chromium  can  potentially   cause
problems  in  uncontrolled landfills.  Incineration,  or  similar
destructive oxidation processes, can produce hexavalent  chromium
from  lower valence states.  Hexavalent chromium  is  potentially
more toxic than trivalent chromium.  In cases where high rates of
chrome  sludge  application  on land are  used,  distinct  growth
inhibition and plant tissue uptake have been noted.

Pretrea-tment    of   discharges   substantially    reduces    the
concentration  of  chromium  in sludge. . In  Buffalo,  New  York,
pretreatment  of electroplating waste resulted in a  decrease  in
chromium concentrations in POTW sludge from 2,510 to 1,040 mg/kg.
A  similar  reduction occurred in Grand  Rapids,  Michigan,  POTW
facilities  where the chromium concentration in sludge  decreased
from  11,000  to  2,700  mg/kg  when  pretreatment  was  made   a
requirement.

Copper   (120) .   Copper  is a metallic element that sometimes  is
found free,  as the native metal,  and is also found in  minerals
such  as  cuprite   (CU2O, malechite  [CuC03.Cu(OH)2],  azurite
[2CuCO3.Cu(OH)2!r  chalcopyrite (CuEeS2),  and bornite (CuS.FeS4).
Copper   is obtained from these ores by  smelting,  leaching,  and
electrolysis.   It is used in the plating,  electrical, plumbing,
and heating equipment industries,  as well as in insecticides and
fungicides.

Traces of copper are found in all forms of plant and animal life,
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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - VI
 and the  metal  is  an  essential  trace  element  for  nutrition.  Copper
 is   not  considered to  be  a  cumulative  systemic poison  for   humans
 as  it  is readily  excreted by the  body,   but  it can cause symptoms
 of   gastroenteritis,   with  nausea and  intestinal  irritations,  as
 relatively   low dosages.    The limiting  factor in domestic  water
 supplies is taste.  To prevent this adverse organoleptic   effect
 of  copper in water,  a  criterion of 1 mg/1 has been established.

 The toxicity of copper to aquatic organisms  varies significantly,
 not only  with   the   species,  but also  with  the  physical  and
 chemical characteristics  of  the water  including  temperature,
 hardness, turbidity, and  carbon dioxide  content.  In hard   water,
 the toxicity of copper salts may  be  reduced  by the  precipitation
 of   copper  carbonate or other,  insoluble  compounds.  The  sulfates
 of  copper and  zinc, and of  copper and  calcium are synergistic  in
 their  toxic effect on  fish.

 Relatively   high  concentrations  of  copper may  be  tolerated  by
 adult  fish for  short periods  of time;  the critical  effect  of
 copper   appears   to be its  higher toxicity to young  or  juvenile
 fish.    Concentrations of  0.02 to 0.03 mg/1 have proved fatal to
 some  common fish species.   In general, the salmonoids  are  very
 sensitive and  the sunfishes are less sensitive to copper.

 The recommended  criterion  to  protect  freshwater  aquatic life  is
 0.0056   mg/1  as  a  24-hour   average,  and  0.012  mg/1  maximum
 concentration  at a   hardness  of  50  mg/1  CaCO3.   For  total
 recoverable copper, the  criterion to protect freshwater  aquatic
 life is  0.0056 mg/1 as a .24-hour  average.

 Copper   salts  cause   undesirable color  reactions  in  the  food
 industry and  cause pitting when  deposited on some  other  metals
 such as aluminum and  galvanized  steel.  To  control  undesirable
 taste  and  odor quality of ambient water due to the  organoleptic
 properties   of copper, the estimated level is 1.0 mg/1 for  total
 recoverable copper.

 Irrigation  water  containing more  than minute quantities of copper
 can  be  detrimental to certain crops.   Copper  appears  in  all
 soils, and  its concentration ranges from 10  to 80 ppm.  In soils,
 copper occurs  in  association with  hydrous oxides of manganese and
 iron,  and   also  as soluble and insoluble complexes with  organic
matter.   Copper  is   essential to the life of  plants,  and  the
 normal   range  of concentration in plant tissue is from 5  to  20
ppm.  Copper concentrations in plants normally do not build up to
high   levels   when   toxicity    occurs.    For   example,   the
concentrations  of  copper in snapbean leaves and pods  was  less
 than  50 and 20 mg/kg, respectively,  under conditions  of  severe
copper toxicity.   Even under conditions of copper toxicity,  most
of   the  excess copper accumulates in the roots;  very  little  is
moved to the aerial part of the plant.

Copper is not destroyed when treated by a POTW,   and will  either
pass  through  to  the POTW effluent or be retained in  the  POTW
sludge.   It can  interfere with the POTW treatment processes  and
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           GENERAL DEVELOPMENT DOCUMENT
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can limit the usefulness of municipal sludge.

The  influent concentration of copper to a POTW has been observed
by  the  EPA  to  range from 0.01 to 1.97  mg/1,  with  a  median
concentration of 0.12 mg/1.  The copper that is removed from  the
influent stream of a POTW is absorbed on the sludge or appears in
the  sludge  as the hydroxide  of the metal.   Bench-scale  pilot
studies  have shown that from about 25 percent to 75  percent  of
the  copper passing through the activated sludge process  remains
in  solution  in the final effluent.  Four-hour slug  dosages  of
copper sulfate in concentrations exceeding 50 mg/1 were  reported
to   have  severe  effects  on  the  removal  efficiency  of   an
unacclimated system, with the system returning to normal in about
100 hours.  Slug dosages of copper in the form of copper  cyanide
were  observed to have much more severe effects on the  activated
sludge  system,  but the total system returned to  normal  in  24
hours.

In a recent study of 268 POTW facilities, the median pass-through
was  over 80 percent for primary plants and 40 to 50 percent  for
trickling  filter,  activated  sludge,  and biological  treatment
plants.  POTW effluent concentrations of copper ranged from 0.003
to 1.8 mg/1 (mean =0.126, standard deviation = 0.242).

Copper  which does not pass through the POTW will be retained  in
the sludge where it will build up in concentration.  The presence
of  excessive  levels of copper in sludge may limit  its  use  on
cropland.   Sewage  sludge contains up to 16,000 mg/kg of copper,
with  730  mg/kg as the mean  value.   These  concentrations  are
significantly  greater  than those normally found in  soil  which
usually  range from 18 to 80 mg/kg.   Experimental data  indicate
that  when dried sludge is spread over tillable land,  the copper
tends to remain in place down to the depth of the tillage, except
for copper which is taken up by plants grown in the soil.  Recent
investigation  has shown that the extractable copper  content  of
sludge-treated  soil  decreased  with  time,  which  suggests a
reversion of copper'to less soluble forms was occurring.

Cyanide  (121).   Cyanides are among the most toxic of pollutants
commonly  observed in industrial  wastewaters.   Introduction  of
cyanide  into  industrial processes is usually by dissolution  of
potassium  cyanide  (KCN)  or sodium cyanide  (NaCN)  in  process
waters.  However,  hydrogen cyanide (HCN), formed when the  above
salts are dissolved in water, is probably the most acutely lethal
compound.

The  relationship  of  pH to hydrogen cyanide formation  is  very
important.   As pH is lowered to below 7, more than 99 percent of
the cyanide is present as HCN and less than 1 percent as  cyanide
ions.   Thus,  at neutral pH, that of most living organisms,  the
more toxic form of cyanide prevails.

Cyanide  ions  combine  with numerous heavy metal  ions  to  form
complexes.  The complexes are in equilibrium with HCN.  Thus, the
stability  of  the metal-cyanide complex and the pH determine  the
                               103

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 concentration  of   HCN.    Stability of   the  metal-cyanide   anion
 complexes  is  extremely variable.   Those  formed with  zinc, copper,
 and  cadmium   are   not stable  -  they rapidly  dissociate,   with
 production of HCN,  in near  neutral or acid waters.   Some of  the
 complexes  are extremely stable.   Cobaltocyanide is very  resistant
 to  acid distillation  in the laboratory.   Iron cyanide   complexes
 are also stable, but undergo photodecomposition to give  HCN   upon
 exposure to sunlight.   Synergistic effects have been demonstrated
 for the metal cyanide  complexes making zinc,  copper,  and cadmium
 cyanides   more toxic   than  an  equal   concentration of  sodium
 cyanide.

 The  toxic mechanism of  cyanide is essentially an  inhibition of
 oxygen  metabolism   (i.e.,   rendering the tissues   incapable of
 exchanging oxygen).  The  cyanogen  compounds are true  noncumulative
 protoplasmic   poisons.    They  arrest the  activity of  all forms of
 animal life.   Cyanide  shows  a  very specific type of  toxic action.
 It  inhibits  the cytochrome  oxidase system.    This system is  the
 one which  facilitates  electron transfer  from reduced  metabolites
 to  molecular  oxygen.    The human body  can convert  cyanide  to  a
 non-toxic  thiocyanate  and eliminate it.   However, if  the quantity
 of cyanide ingested  is  too great  at one  time,   the inhibition of
 oxygen  utilization  proves fatal  before  the detoxifying  reaction
 reduces the cyanide  concentration to a safe level.

 Cyanides   are  more  toxic to fish than to lower  forms of aquatic
 organisms  such as  midge   larvae,   crustaceans,  and   mussels.
 Toxicity   to  fish  is  a  function of   chemical   form   and
 concentration,  and  is   influenced by  the  rate  of  metabolism
 (temperature),  the  level   of dissolved  oxygen,  and  pH.   In
 laboratory studies,  free  cyanide  concentrations  ranging  from 0.05
 to  O.lg   mg/1  have been proven  to be fatal   to  sensitive   fish
 species  including trout, bluegill,  and fathead minnows.   Levels
 above 0.2  mg/1  are rapidly fatal  to most  fish  species.   Long-term
 sublethal  concentrations  of  cyanide  as low as  0.01 mg/1  have  been
 shown  to  affect the ability of fish to function normally  (e.g.,
 reproduce, grow, and swim).

 For  the protection  of human health from  the  toxic properties  of
 cyanide  ingested through water and  through contaminated  aquatic
 organisms,  the ambient water  quality criterion  is determined  to
 be  0.200 mg/1.

 Persistence   of  cyanide  in  water  is  highly variable and  depends
 upon the chemical form of cyanide  in  the  water, the concentration
 of  cyanide, and the  nature of  other  constituents.  Cyanide may be
 destroyed  by   strong oxidizing agents such as  permanganate  and
 chlorine.    Chlorine is commonly used to  oxidize  strong  cyanide
 solutions.     Carbon  dioxide   and  nitrogen are  the  products  of
 complete  oxidation.   But if  the  reaction  is not  complete,   the
 very  toxic   compound,   cyanogen   chloride,  may  remain  in  the
 treatment system and subsequently  be  released to the environment.
 Partial  chlorination may occur as part of a POTW  treatment,  or
 during  the disinfection  treatment of surface water for  drinking
water preparation.
                               104

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           GENERAL DEVELOPMENT- DOCUMENT
SECT - VI
Cyanides  can interfere with treatment processes in  a  POTW,  or
pass  through to ambient waters.  At low concentrations and  with
acclimated    microflora,   cyanide   may   be   decomposed    by
microorganisms  in  anaerobic and aerobic environments  or  waste
treatment  systems.   However,  data indicate that  much  of  the
cyanide introduced passes through to the POTW effluent.  The mean
pass-through of 14 biological plants was 71 percent.  In a recent
study  of 41 POTW facilities the effluent  concentrations  ranged
from 0.002 to 100 mg/1 (mean = 2.518, standard deviation = 15.6).
Cyanide  also enhances the toxicity of metals commonly  found  in
POTW effluents, including the toxic pollutants cadmium, zinc, and
copper.

Data for Grand Rapids,  Michigan, showed a significant decline in
cyanide   concentrations   downstream   from   the   POTW   after
pretreatment regulations were put in force.  Concentrations  fell
from  0.66  mg/1  before, to 0.01  mg/1  after  pretreatment  was
required.

Lead (122).    Lead is a soft,  malleable,  ductile, blueish-gray,
metallic element,  usually obtained from the mineral galena (lead
sulfide,  PbS),  anglesite  (lead sulfate,  PbSO4),  or cerussite
(lead carbonate,  PbCO3).   Because it is usually associated with
minerals of zinc,  silver,  copper,  gold, cadmium, antimony, and
arsenic,  special purification methods are frequently used before
and  after  extraction of the metal from the ore  concentrate  by
smelting.

Lead  is  widely used for its  corrosion  resistance,  sound  and
vibration absorption, low melting point (solders), and relatively
high imperviousness to various forms of radiation.  Small amounts
of copper,  antimony and other metals can be alloyed with lead to
achieve greater hardness, stiffness, or corrosion resistance than
is afforded by the pure metal.  Lead compounds are used in glazes
and paints.    About one third of U.S.  lead consumption goes into
storage batteries.   About half of U.S.  lead consumption is from
secondary  lead  jrecovery.   U.S.  consumption of lead is. in  the
range of one million tons annually.

Lead  ingested  by  humans produces a variety  of  toxic  effects
including  impaired reproductive ability,  disturbances in  blood
chemistry,  neurological  disorders,  kidney damage, and  adverse
cardiovascular effects.   Exposure to lead in the diet results in
permanent increase in lead levels in the body.   Most of the lead
entering the body eventually becomes localized in the bones where
it  accumulates.   Lead  is a carcinogen or cocarcinogen in  some
species   of  experimental  animals.   Lead  is  teratogenic   in
experimental  animals.  Mutagenicity data are not  available  for
lead.

The ambient  water quality criterion for lead is recommended to be
identical to the existing drinking water standard which is  0.050
mg/1.   Available data show that adverse effects on aquatic  life
occur  at  concentrations  as low as 7.5 x  10-4  mg/1  of  total
                               105

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
recoverable lead as a 24-hour average with a water hardness of 50
mg/1 as
Lead  is not destroyed in a POTW,  but is passed through  to  the
effluent  or retained in the POTW sludge;  it can interfere  with
POTW  treatment  processes and can limit the usefulness  of  POTW
sludge  for  application to  agricultural  croplands.   Threshold
concentration  for inhibition of the activated sludge process  is
0.1  mg/1, and for the nitrification process is 0.5 mg/1.   In  a
study  of  214 POTW facilities, median pass-through  values  were
over  80  percent  for primary plants and  over  60  percent  for
trickling  filter,  activated  sludge,  and  biological   process
plants.   Lead concentration in POTW effluents ranged from  0.003
to 1.8 mg/1 (mean = 0.106 mg/1, standard deviation = 0.222).

Application of lead-containing sludge to cropland should not lead
to uptake by crops under most conditions because normally lead is
strongly bound by soil.   However, under the unusual condition of
low  pH  (less  than  5.5)  and  low  concentrations  of   labile
phosphorus,   lead  solubility  is  increased  and   plants   can
accumulate lead.

Mercury  (123) .   Mercury  is an elemental metal rarely found  in
nature as the free metal.   Mercury is unique among metals as  it
remains  a  liquid down to about 39 degrees below  zero.   it  is
relatively  inert  chemically  and is insoluble  in  water.   The
principal ore is cinnabar (HgS).

Mercury  is  used industrially as the metal and as mercurous  and
mercuric salts and compounds.   Mercury is used in several  types
of  batteries.   Mercury  released to the aqueous environment  is
subject  to  biomethylation - conversion to the  extremely  toxic
methyl mercury.

Mercury can be introduced into the body through the skin and  the
respiratory  system as the elemental vapor.   Mercuric salts  are
highly   toxic  to  humans  and  can  be  absorbed  through   the
gastrointestinal tract.  Fatal doses can vary from 1 to 30 grams.
Chronic  toxicity  of methyl mercury is  evidenced  primarily  by
neurological symptoms.  Some mercuric salts cause death by kidney
failure.

Mercuric  salts  are extremely toxic to fish  and  other  aquatic
life.   Mercuric chloride is more lethal than copper,  hexavalent
chromium,  zinc,  nickel, and lead towards fish and aquatic life.
In  the food cycle,  algae containing mercury up, to 100 times the
concentration  in  the surrounding sea water are  eaten  by  fish
which  further concentrate the mercury.   Predators that eat  the
fish in turn concentrate the mercury even further.

For  the protection of human health from the toxic properties  of
mercury  ingested through water and through contaminated  aquatic
organisms, the ambient water criterion is determined to be 0.0002
mg/1 .
                               106

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Mercury is not destroyed when treated by a POTW,  and will either
pass  through  to the POTW effluent or be incorporated  into  the
POTW  sludge.   At low concentrations it may reduce POTW  removal
efficiencies,  and  at high concentrations it may upset the  POTW
operation.

The  influent  concentrations  of mercury to  a  POTW  have  been
observed  by  the EPA to range from 0.002 to 0.24  mg/1,  with  a
median concentration of 0.001 mg/1.  Mercury has been reported in
the  literature  to  have inhibiting effects  upon  an  activated
sludge  POTW at levels as low as 0.1 mg/1.   At 5 mg/1 of mercury
losses  of COD removal efficiency of 14 to 40 percent  have  been
reported, while at 10 mg/1, loss of removal of 59 percent has been
reported.   Upset  of an activated sludge POTW is reported in the
literature  to  occur  near 200 mg/1.   The  anaerobic  digestion
process  is much less affected by the presence of  mercury,  with
inhibitory effects being reported at 1,365 mg/1.

In a study of 22 POTW facilities having secondary treatment,  the
range  of removal of mercury from the influent to the POTW ranged
from  4 to 99 percent with median removal of  41  percent.   Thus
significant pass-through of mercury may occur.               . ,  ."

In sludges,  mercury content may be high if industrial sources of
mercury  contamination  are present.   Little is known about  the
form  in  which mercury occurs in sludge.   Mercury  may  undergo
biological methylation in sediments,  but no methylation has been
observed in soils, mud, or sewage sludge.

The  mercury  content of soils not receiving  additions  of  POTW
sewage sludge lie in the range from 0.01 to 0.5-mg/kg.   In soils
receiving POTW sludges for protracted periods,  the concentration
of mercury has been observed to approach 1.0 mg/kg.  In the soil,
mercury  enters into reactions with the exchange complex of  clay
and  organic  fractions,  forming both ionic and covalent  bonds.
Chemical  and microbiological degradation of mercurials can  take
place  side  by side in the soil,  and the  products  - ionic  or
molecular  - are  retained by organic matter and clay or  may  be
volatilized  if  gaseous.   Because of the high affinity  between
mercury  and  the solid soil surfaces,  mercury persists  in  the
upper layer of the soil.

Mercury can enter plants through the roots,  it can readily- move
to  other parts of the plant,  and it has been reported to  cause
injury  to plants.   In many plants mercury concentrations  range
from  0.01 to 0.20 mg/kg,  but when plants are supplied with high
levels  of  mercury, these concentrations can exceed  0.5  mg/kg.
Bioconcentration occurs in animals ingesting mercury in food.

Nickel  (124).   Nickel  is seldom found in nature  as  the  pure
elemental  metal.  It is a relatively  plentiful element  and  is
widely  distributed throughout the earth's crust.  It  occurs  in
marine  organisms  and  is  found  in  the  oceans.   The   chief
commercial  ores for nickel are pentlandite [(Fe,Ni)9S8],  and   a
lateritic   ore  consisting  of  hydrated   nickel-iron-magnesium
                               107

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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - VI
 silicate.

 Nickel has many and varied  uses.   It  is  used  in alloys and as  the
 pure metal.  Nickel salts are  used for electroplating baths.

 The  toxicity  of  nickel to man  is thought  to be  very  low,   and
 systemic  poisoning of human beings by nickel or nickel salts  is
 almost  unknown.   In non-human  mammals  nickel  acts  to  inhibit
 insulin release, depress growth, and  reduce cholesterol.  A  high
 incidence  of  cancer of the lung  and nose  has been  reported  in
 humans engaged in  the refining of  nickel.

 Nickel salts can kill fish  at  very low concentrations.   However,
 nickel has been found to be less toxic to some fish than  copper,
 zinc,  and  iron.   Nickel  is present in coastal and open  ocean
 water  at  concentrations in the range of 0.0001  to  0.006  mg/1
 although the most  common values  are 0.002 to  0.003 mg/1.   Marine
 animals  contain up to 0.4  mg/1  and marine plants contain up to 3
 mg/1.   Higher nickel concentrations  have been reported to  cause
 reduction  in photosynthetic activity of the  giant kelp.   A   low
 concentration was  found to  kill  oyster eggs.

 For  the protection of human health based on  the toxic properties
 of nickel ingested through  water and  through  contaminated aquatic
 organisms, the ambient water criterion is determined to be 0.0134
 mg/1.   If contaminated aquatic  organisms are consumed, excluding
 consumption of water,  the  ambient  water criterion is  determined
 to  be 0.100 mg/1.   Available data show that adverse effects  on
 aquatic life occur for total recoverable nickel concentrations as
 low as 0.0071 mg/1 as a 24-hour average.

 Nickel  is not destroyed when; treated in a POTW,  but will either
 pass  through  to the POTW  effluent or be retained  in  the  POTW
 sludge.   It  can interfere with POTW treatment processes and  can
 also limit the usefulness of municipal sludge.

 Nickel salts have caused inhibition of'the biochemical  oxidation
 of  sewage  in a POTW.   In a  pilot plant,  slug doses of  nickel
 significantly  reduced  normal treatment efficiencies for  a   few
 hours,  but  the  plant acclimated  itself somewhat  to  the  slug
 dosage  and  appeared to achieve  normal  treatment  efficiencies
 within  40' hours.   It  has been   reported   that  the  anaerobic
 digestion  process  is inhibited only by high  concentrations  of
 nickel,  while  a  low  concentration  of  nickel  inhibits    the
 nitrification process.

 The  influent concentration of nickel to a POTW has been observed
 by the EPA to range from 0.01 ^to 3.19 mg/1,  with a median of 0.33
mg/1.  In a study of 190 POTW  facilities, nickel pass-through was
 greater  than  90 percent for  82 percent of  the.  primary  plants.
Median pass-through for trickling filter,  activated sludge,   and
 biological  process  plants was greater  than  80  percent.    POTW
 effluent  concentrations  ranged from 0.002  to 40 mg/1  (mean  =
 0.410,  standard deviation = 3..279).
                               108

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Nickel  not passed through the POTW will be incorporated into the
sludge.   In a recent two-year study of eight cities, four of the
cities  had median nickel concentrations of over 350  mg/kg,  and
two  were  over 1,000 mg/kg.   The maximum  nickel  concentration
observed was 4,010 mg/kg.

Nickel is found in nearly all soils,  plants, and waters.  Nickel
has  no known essential function in  plants.   In  soils,  nickel
typically  is found in the range from 10 to 100  mg/kg.   Various
environmental  exposures  to  nickel  appear  to  correlate  with
increased incidence of tumors in man.  For example, cancer in the
maxillary  antrum  of  snuff users may result  from  using  plant
materials grown on soil high in nickel.

Nickel  toxicity may develop in plants from application of sewage
sludge on acid soils.   Nickel has caused reduction of yields for
a variety of crops including oats, mustard, turnips, and cabbage.
In  one study,  nickel decreased the yields of oats significantly
at 100 mg/kg.

Whether nickel exerts a toxic effect on plants depends on several
soil factors,  the amount of nickel applied,  and the contents of
other metals in the sludge.   Unlike copper and zinc,  which  are
more  available from inorganic sources than from  sludge,  nickel
uptake  by  plants  seems to be promoted by the presence  of  the
organic  matter  in sludge.   Soil treatments,  such  as  liming,
reduce the solubility of nickel.  Toxicitry of nickel to plants is
enhanced in acidic soils.

Selenium (125).   Selenium is a non-metallic element existing  in
several  allotropic forms.   Gray selenium,  which has a metallic
appearance, is the stable form at ordinary temperatures and melts
at  220°C.   Selenium is a major component of 38 minerals  and  a
minor component of 37 others found in various parts of the world.
Most  selenium  is obtained as a  by-product of  precious  metals
recovery from electrolytic copper refinery slimes.   U.S.  annual
production at one time reached one million pounds.

Principal  uses  of selenium are  in  semi-conductors,  pigments,
decoloring of glass,  and metallurgy.  It also is used to produce
ruby glass used in signal lights.  Several selenium compounds are
important oxidizing agents in the synthesis of organic  chemicals
and drug products.

While  results  of some studies suggest that selenium may  be  an
essential  element  in  human nutrition,  the  toxic  effects  of
selenium  in humans are well  established.   Lassitude,  loss  of
hair,  discoloration  and  loss  of  fingernails are  symptoms  of
selenium  poisoning.   In a fatal case of ingestion or  a  larger
dose  of selenium acid,  peripheral  vascular collapse,  pulmonary
edema,  and  coma  occurred.   Selenium• produces  mutagenic  and
teratogenic    effects,  but  it  has  not  been  established   as
exhibiting carcinogenic activity.

For  the protection of human health  from the toxic properties  of
                                109

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 selenium ingested through water and through contaminated  aquatic
 organisms,  the ambient water criterion is determined to be 0.010
 mg/1,  (i.e., the same as the drinking water standard).  Available
 data   show  that  adverse  effects  on  aquatic  life  occur   at
 concentrations higher than that cited,for human toxicity.

 Very few data are available regarding the behavior of selenium in
 a POTW.   One EPA survey of 103 POTW facilities revealed one POTW
 using  biological treatment and having selenium in the  influent.
 Influent   concentration   was   0.0025   mg/1,    and   effluent
 concentration  was 0.0016 mg/1,  giving a removal of 37  percent.
 It  is not known to be inhibitory to POTW processes.   In another
 study,  sludge  from  POTW facilities in 16 cities was  found  to
 contain  from 1.8 to 8.7 mg/kg selenium,  compared to 0.01  to  2
 mg/kg  in  untreated soil.   These concentrations of selenium  in
 sludge  present  a potential hazard for humans or  other  mammals
 eating crops grown on soil treated with selenium-containing sludge.

 Silver  (126).   Silver is a soft  lustrous  white metal that  is
 insoluble in water and alkali.  In nature, silver is found in the
 elemental  state  (native  silver) and combined in ores  such  as
 argentite (Ag2S),  horn silver (AgCl),  proustite (Ag3AsS3),  and
 pyrargyrite  (Ag3SbS3).   Silver is used extensively  in  several
 industries, among them electroplating.
Metallic  silver is not considered to be toxic,
salts  are toxic to a large number of organisms.
by  humans,  many silver salts are absorbed  in
system  and  deposited  in various  body  tissues
generalized or sometimes localized gray pigmentat
and mucous membranes known as argyria.  There is
for  removing silver from the tissues once it is
the effect is cumulative.
      but  most  of  its
        Upon ingestion
      the   circulatory
      ,  resulting  in
      ion  of the  skin
      no known   method
      deposited,  and
Silver is recognized as a bactericide and doses from 0.000001  to
0.0005  mg/1 have been reported as sufficient to sterilize water.
The criterion for ambient water to protect human health from  the
toxic  properties  of silver ingested through water  and  through
contaminated aquatic organisms is 0.010 mg/1.

The  chronic  toxic effects of 'Silver on the aquatic  environment
have not been given as much attention as many other heavy metals.
Data  from  existing literature support the fact that  silver  is
very toxic to aquatic organisms',   Despite the fact that silver is
nearly the most toxic of the heavy metals, there are insufficient
data  to  adequately  evaluate even the effects  of  hardness  on
silver toxicity.   There are no data available on the toxicity of
different forms of silver.

There  is  no available literature on the incidental  removal  of
silver by a POTW.   An incidental removal of about 50 percent  is
assumed  as  being representative.   This is the highest  average
incidental  removal  of any metal for which data  are  available.
(Copper  has been indicated to have a'median  incidental  removal
rate of 49 percent.)
                               110

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Bioaccumulation  and  concentration of silver from sewage  sludge
has  not  been  studied  to any  great 'degree.   There  is  some
indication  that silver could be bioaccumulated in  mushrooms  to
the  extent that there could be adverse physiological effects  on
humans  if they consumed large quantities of mushrooms  grown  in
silver-enriched   soil.   The effect, however, would tend  to  be
unpleasant rather than fatal.

There are.little summary data available on the quantity of silver
discharged  to a POTW.   Presumably there would be a tendency  to
limit its discharge from a manufacturing facility because of  its
high intrinsic value.

Thallium  (127).    Thallium  is  a  soft,  silver-white,  dense,
malleable  metal.   Five major minerals contain 15 to 85  percent
thallium,  but they are not of commercial importance because  the
metal is produced in sufficient quantity as a by-product of lead-
zinc  smelting of sulfide ores.   Thallium melts at 304°C.   U.S.
annual  production of thallium and its compounds is estimated  to
be 1,500 pounds.

Industrial  uses  of thallium include the manufacture of  alloys,
electronic  devices and special glass.   Thallium  catalysts  are
used for industrial organic syntheses.

Acute  thallium  poisoning in humans has been  widely  described.
Gastrointestinal  pains  and  diarrhea are followed  by  abnormal
sensation in the legs and arms,  dizziness,  and,  later, loss of
hair.   The central nervous system is also affected.  Somnolence,
delirium  or  coma may occur.  Studies on the  teratogenicity  of
thallium  appear  inconclusive; no studies on  mutagenicity  were
found;  and no published reports on carcinogenicity  of  thallium
were found.

For  the protection of human health from the toxic properties  of
thallium   ingested  through  water  and   contaminated   aquatic
organisms, the ambient water criterion is 0.004 mg/1.

No  reports  were found regarding the behavior of thallium  in  a
POTW.   It will not be degraded;  therefore, it must pass through
to the effluent or be removed with the  sludge.   However,  since
the, sulfide (T1S) is very insoluble,  if appreciable sulfide  is
present,  dissolved  thallium in the influent to a  POTW  may  be
precipitated  into the sludge.  Subsequent use of sludge  bearing
thallium compounds as a soil amendment to crop bearing soils  may
result  in uptake of this element by food plants.  Several  leafy
garden  crops  (cabbage,  lettuce,  leek,  and  endive)   exhibit
relatively  higher  concentrations of thallium than  other  foods
such as meat.

Zinc  (128).   Zinc  occurs  abundantly  in  the  earth's  crust,
concentrated  in  ores.   It is readily refined  into  the  pure,
stable,  silver-white metal.  In addition to its use  in  alloys,
zinc is used as a protective coating on steel.  It is applied  by
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            GENERAL  DEVELOPMENT DOCUMENT
                    SECT - VI
 hot   dipping   (i.e.,
 electroplating.
dipping the steel in molten  zinc)  or  by
 Zinc   can   have   an  adverse  effect  on man   and  animals  at  high
 concentrations.    Zinc   at   concentrations  in excess  of   5  mg/1
 causes  an  undesirable  taste which  persists through  conventional
 treatment.    For  the prevention  of  adverse  effects due  to   these
 organoleptic  properties of  zinc,  5 mg/1  was  adopted  for  the
 ambient  water  criterion.    Available  data show  that  adverse
 effects  on aquatic  life occur at concentrations as low as   0.047
 mg/1 as  a 24-hour average.

 Toxic  concentrations of zinc compounds cause adverse changes  in
 the morphology and physiology of fish.  Lethal concentrations  in
 the  range  of  0.1   mg/1 have  been  reported.   Acutely   toxic
 concentrations  induce   cellular breakdown of  the  gills,  and
 possibly the  clogging of the gills  with   mucous.   Chronically
 toxic  concentrations of zinc compounds cause general enfeeblement
 and  widespread histological changes to many organs, but  not  to
 gills.   Abnormal swimming  behavior has been  reported  at  0.04
 mg/1.    Growth and maturation are retarded  by zinc.  It has  been
 observed that  the   effects of  zinc  poisoning  may  not  become
 apparent immediately, so that fish  removed  from zinc-contaminated
 water  may die as  long as 48  hours after removal.

 In  general,  salmonoids are most sensitive to elemental zinc  in
 soft   water;  the rainbow   trout is the most sensitive  in  hard
 waters.     A   complex  relationship   exists   between    zinc
 concentration, dissolved zinc concentration, pH, temperature, and
 calcium  and  magnesium  concentration.   Prediction  of  harmful
 effects  has been less  than  reliable and controlled studies  have
 not been extensively documented.

 The  major  concern  with zinc compounds in  marine waters  is  not
 with   acute  lethal  effects   but rather with the  long-term  sub-
 lethal   effects of the  metallic  compounds   and  complexes.   Zinc
 accumulates  in   some marine  species and marine animals  contain
 zinc in  the range  of  6  to 1,500  mg/kg.  From the point of view of
 acute  lethal effects,   invertebrate marine  animals seem to be the
most sensitive organism tested.

Toxicities  of zinc  in  nutrient  solutions have been  demonstrated
 for a number of plants.   A  variety of fresh water plants  tested
manifested  harmful   symptoms at concentrations of 0.030 to  21.6
mg/1.    Zinc  .sulfate   has also  been found  to be lethal  to  many
plants and it could  impair agricultural uses of the water.

Zinc   is not destroyed  when  treated by a POTW,  but  will  either
pass  through  to  the  POTW  effluent or be  retained in  the  POTW
sludge.   It  can  interfere with treatment processes in the  POTW
and can also limit the  usefulness of municipal sludge.

In  slug  doses,   and  particularly in the  presence  of  copper,
dissolved  zinc  can  interfere with  or  seriously  disrupt .the
operation  of  POTW  biological  processes  by  reducing  overall
                               112

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           GENERAL DEVELOPMENT .DOCUMENT
                                SECT - VI
removal efficiencies,  largely as a result of the toxicity of the
metal to biological organisms.   However, zinc solids in the form
of  hydroxides  or  sulfides  do not  appear  to  interfere  with
biological  treatment processes,  on the basis of available data.
Such solids     accumulate in the sludge.

The influent concentrations of zinc to a POTW have been  observed
by  the  EPA  to range from 0.017 to 3.91  mg/1,  with  a  median
concentration  of 0.33 mg/1.   Primary treatment is not efficient
in     removing zinc;  however,  the microbial floe of  secondary
treatment     readily adsorbs zinc.

In a study of 258 POTW facilities, the median pass-through values
were  70 to 88 percent for primary plants,  50 to 60 percent  for
trickling  filter  and biological process plants,  and 30  to  40
percent   for   activated   process   plants.     POTW   effluent
concentrations      of zinc ranged from 0.003 to 3.6 mg/1 (mean =
0.330, standard     deviation = 0.464).

The zinc which does not pass through the POTW is retained in  the
sludge.   The  presence  of zinc in sludge may limit its  use  on
cropland.   Sewage  sludge  contains 72 to over 30,000  mg/kg  of
zinc,  with 3,366 mg/kg as the mean value.   These concentrations
are  significantly  greater  than those normally found  in  soil,
which  range from 0 to 195 mg/kg,  with 94 mg/kg being  a  common
level.   Therefore,  application  of  sewage sludge to soil  will
generally increase the concentration of zinc in the  soil.   Zinc
can  be  toxic  to plants,  depending  upon  soil  pH.   Lettuce,
tomatoes,  turnips,  mustard,  kale,  and  beets  are  especially
sensitive to zinc contamination.

Oil  and  Grease.   Oil  and  grease are taken  together  as  one
pollutant parameter.   This is a conventional pollutant and  some
of its
components are:
    1.   Light  Hydrocarbons - These include light fuels such  as
gasoline, kerosene, and jet fuel, and miscellaneous solvents used
for industrial processing, degreasing, or cleaning purposes.  The
presence  of  these  light hydrocarbons may make the  removal  of
other heavier oil wastes more difficult.

    2.   Heavy Hydrocarbons,  Fuels, and Tars - These include the
crude oils,  diesel oils,  #6 fuel oil, residual oils, slop oils,
and in some cases, asphalt and road tar.

    3.   Lubricants  and  Cutting Fluids - These  generally  fall
into two classes:  non-emulsifiable oils such as lubricating oils
and  greases  and emulsifiable oils such as water  soluble  oils,
rolling oils,  cutting oils, and drawing compounds.  Emulsifiable
oils may contain fat, soap, or various other additives.

    4.   Vegetable  and  Animal Fats and Oils  - These  originate
primarily   from  processing  of  foods  and  natural   products.

These  compounds can settle or ,f3loat; and-may exist as  solids  or
                               113

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
 liquids  depending upon  factors  such as method of use,
 process,  and  temperature of water.
            production
 Oil   and  grease even  in  small quantities  cause troublesome  taste
 and  odor  problems.    Scum  lines  from  these agents are produced on
 water treatment basin walls and  other containers.  Fish and water
 fowl  are  adversely  affected by oils  in   their  habitat.   Oil
 emulsions  may  adhere to  the gills of  fish  causing  suffocation,
 and       the  flesh of fish is tainted  when  microorganisms   that
 were      exposed to  waste oil are eaten.    Deposition of oil in
 the   bottom     sediments of water can serve to  inhibit  normal
 benthic growth.     Oil  and grease exhibit an oxygen demand.

 Many  of  the  toxic organic pollutants will be  found  distributed
 between   the  oil  phase  and the  aqueous   phase  in  industrial
 wastewaters.  The presence of phenols,  PCBs, PAHs, and almost any
 other  organic   pollutant   in  the  oil   and   grease    make
 characterization of this parameter almost  impossible.   However,
 all   of these    other  organics add  to the  objectionable  nature
 of the oil and     grease.

 Levels of oil and grease which are  toxic to  aquatic  organisms
 vary  greatly,   depending   on the   type   and   the   species
 susceptibility.   However, it lhas been  reported that crude oil in
 concentrations   as   low  as  0.3  mg/1  is  extremely  toxic to
 freshwater fish.   It   has been recommended that  public  water
 supply sources be essentially free from oil  and grease.

 Oil  and grease in quantities of  100 1/sq  km  show up as a sheen on
 the   surface  of  a body of water.    The  presence of  oil  slicks
 decreases the aesthetic  value of a waterway.

 Oil  and grease is compatible with a POTW  activated sludge process
 in    limited   quantity.    However,    slug  loadings   or    high
 concentrations  of  oil  and  grease  interfere  with  biological
 treatment processes.  The  oils coat surfaces and solid particles,
 preventing access of  oxygen,  and sealing in some microorganisms.
 Land  spreading  of  POTW sludge  containing  oil  and   grease
 uncontaminated  by  toxic  pollutants  is not  expected  to  affect
 crops grown on the treated land  or animals  eating those crops.

 pH.    Although  not a specific pollutant, pH is  related  to  the
 acidity   or  alkalinity  of  a wastewater  stream.   It  is   not,
 however,   a measure of either.   The term  pH  is used  to  describe
 the   hydrogen ion concentration  (or activity) present in a  given
'solution.   Values for pH  range  from  0  to 14, and  these  numbers
 are   the  negative logarithms of  the hydrogen ion  concentrations.
 A pH of 7 indicates neutrality.  Solutions with a pH above 7  are
 alkaline,   while  those  solutions with  a  pH  below 7  are  acidic.
 The   relationship  of pH  and   acidity  and alkalinity  is  not
 necessarily  linear   or  direct.  Knowledge  of the  water  pH is
 useful in determining necessary measures for corrosion  control,
 sanitation, and disinfection.  Its value  is  also necessary in the
 treatment  of industrial  wastewaters  to  determine  amounts of
 chemicals  required   to  remove pollutants and  to  measure  their
                                114

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
effectiveness.   Removal  of  pollutants,  especially
solids is affected by the pH of the wastewater.
             dissolved
Waters  with  a  pH  below  6.0  are  corrosive  to  water  works
structures,  distribution lines, and household plumbing  fixtures
and  can  thus add constituents to drinking water such  as  iron,
copper, zinc, cadmium, and lead.  The hydrogen ion  concentration
can affect the taste of the water, and at a low pH, water  tastes
sour.  The bactericidal effect of chlorine is weakened as the  pH
increases,  and it is advantageous to keep the pH close  to  7.0.
This is significant for providing safe drinking water.

Extremes of pH or rapid pH changes can exert stress conditions or
kill  aquatic life outright.   Even moderate changes from accept-
able criteria limits of pH are deleterious to some species.

The  relative  toxicity  to aquatic life  of  many  materials  is
increased   by   changes   in  the  water   pH.    For   example,
metallocyanide complexes can increase a thousand-fold in toxicity
with a drop of 1.5 pH units.

Because  of  the universal nature of pH and its effect  on  water
quality  and treatment,  it is selected as a pollutant  parameter
for many industry categories.   A neutral pH range (approximately
6  to 9) is generally desired because either extreme beyond  this
range  has  a  deleterious  effect on  receiving  waters  or  the
pollutant nature of other wastewater constituents.

Pretreatment  for  regulation of pH is covered  by  the  "General
Pretreatment   Regulations  for  Existing  and  New  Sources   of
Pollution,"  40 CFR 403.5.  This section prohibits the  discharge
to  a POTW of "pollutants which will cause  corrosive  structural
damage  to the POTW but in no case discharges with pH lower  than
5.0  unless the works is specially designed to  accommodate  such
discharges."

Total Suspended Solids (TSS).  Suspended solids include both
organic and inorganic materials.  The inorganic compounds include
sand,  silt,  and  clay.   The  organic  fraction  includes  such
materials  as  grease, oil, tar, and animal and  vegetable  waste
products.      These  solids may settle out rapidly,  and  bottom
deposits  are  often  a mixture of  both  organic  and  inorganic
solids.   Solids  may be suspended in water for a time  and  then
settle to the bed of the stream or lake.  These solids discharged
with  man's wastes may be inert, slowly biodegradable  materials,
or   rapidly  decomposable  substances.   While  in   suspension,
suspended  solids  increase the turbidity of  the  water,  reduce
light  penetration,  and impair the  photosynthetic  activity  of
aquatic plants.

Suspended   solids  in  water  interfere  with  many   industrial
processes  and  cause  foaming in boilers  and  encrustations  on
equipment  exposed to such water, especially as  the  temperature
rises.      They  are undesirable in process water  used  in  the
manufacture of     steel, in the textile industry, in  laundries,
                               115

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
in dyeing, and in cooling systems.

Solids  in suspension are aesthetically displeasing.   When  they
settle  to form sludge deposits on the stream or lake  bed,  they
are  often  damaging to the life  in  the  water.   Solids,  when
transformed  to  sludge  deposit,  may do a variety  of  damaging
things,      including  blanketing  the stream or  lake  bed  and
thereby  destroying the living spaces for those benthic organisms
that would     otherwise occupy the habitat.   When of an organic
nature,  solids     use a portion or all of the dissolved  oxygen
available  in  the     area.   Organic materials also serve as  a
food source for     sludgeworms and associated organisms.

Disregarding any toxic effect attributable to substances  leached
out  by  water,  suspended solids may kill fish and shellfish  by
causing   abrasive  injuries  and  by  clogging  the  gills   and
respiratory  passages  of  various  aquatic  fauna.   Indirectly,
suspended      solids are inimical to aquatic life  because  they
screen   out      light,   and  they  promote  and  maintain  the
development  of noxious     conditions through oxygen  depletion.
This results in the killing   .  of fish and fish food  organisms.
Suspended  solids  also reduce     the recreational value of  the
water.

Total  suspended  solids  is a  traditional  pollutant  which  is
compatible  with  a  well-run POTW.   This  pollutant,  with  the
exception  of those components which are described  elsewhere  in
this section (e.g.,  heavy metal components),  does not interfere
with  the  operation of a POTW.   However,  since a  considerable
portion  of  the innocuous TSS may be inseparably  bound  to  the
constituents  which do interfere with POTW operation,  or produce
unusable    sludge,   or   subsequently   dissolve   to   produce
unacceptable POTW  effluent, TSS may be considered a toxic waste.

Aluminum.   Aluminum,  a nonconventional pollutant,  is the  most
common metallic element in the earth's crust,  and the third most
abundant  element  (8.1  percent).   It is never  found  free  -in
nature.   Most  rocks  and various clays contain aluminum in  the
form of aluminosilicate minerals.   Generally,  aluminum is first
converted to alumina (A1203) from bauxite ore.   The alumina then
undergoes  electrolytic reduction to form  the  metal.   Aluminum
powders  (used in explosives,  fireworks,  and rocket fuels) form
flammable mixtures in the air.   Aluminum metal resists corrosion
under  many conditions by forming a protective oxide film on  the
surface.   This oxide layer corrodes rapidly in strong acids  and
alkalis,  and  by  the electrolytic action of other  metals  with
which  it  comes  in  contact.   Aluminum  is  light,  malleable,
ductile,  possesses high thermal and electrical conductivity, and
is non-magnetic.   It can be formed, machined, or cast.  Aluminum
is used in the building and construction, transportation, and the
container  and  packaging industries and competes with  iron  and
steel  in  these  markets.   Total  U.S.  production  of  primary
aluminum  in 1981 was 4,948,000 tons.  Secondary  aluminum  (from
scrap) production in 1981 was 886,000 tons.
                               116

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Aluminum is soluble under both acidic and basic conditions,  with
environmental  transport  occurring  most  readily  under   these
conditions.   In water, aluminum can behave as an acid  or  base,
can   form  ionic  complexes  with  other  substances,  and   can
polymerize,  depending  on  pH and the  dissolved  substances  in
water.  Aluminum's high solubility at acidic pH conditions  makes
it  readily available for accumulation in aquatic  life.   Acidic
waters  consistently  contain higher levels of  soluble  aluminum
than  neutral  or  alkaline  waters.  Loss  of  aquatic  life  in
acidified  lakes and streams has been shown to be due in part  to
increased  concentrations  of aluminum in waters as a  result  of
leaching of aluminum from soil by acidic rainfall.

Aluminum  has  been  found to be toxic to freshwater  and  marine
aquatic  life.   In  freshwaters, acute  toxicity  and  solubility
increases  as pH levels increase above* pH 7.   This  relationship
also  appears  to be true as the pH levels decrease below  pH  7.
Chronic  effects  of  aluminum on aquatic  life  have  also  been
documented.   Aluminum  has  been found to be  toxic  to  certain
plants.  A  water quality standard for aluminum  was  established
(U.S.  Federal Water Pollution Control Administration, 1968)  for
interstate agricultural and irrigation waters, which set a  trace
element  tolerance at 1 mg/1 for continuous use on all soils  and
20 mg/1 for short-term use on fine-textured soils.

There  are no reported adverse physiological effects on man  from
exposure  to  low concentrations of aluminum in  drinking  water.
Large concentrations of aluminum in the human body,  however, are
alleged  to  cause  changes  in  behavior.   Aluminum  compounds,
especially  aluminum  sulfate, are major coagulants used  in  the
treatment  of drinking water.  Aluminum is not among  the  metals
for which a drinking water standard has been established.

The  highest aluminum concentrations in animals and humans  occur
in the lungs, mostly from the inhalation of airborne  particulate
matter.    Pulmonary  fibrosis  has  been  associated  with   the
inhalation of very fine particles of aluminum flakes and  powders
among  workers  in the explosives and fireworks  industries.   An
occupational  exposure Threshold Limit Value (TLV) of 5 mg/m^  is
recommended  for  pyro  powders to prevent lung  changes,  and  a
time weighted average  (TWA)  of  10  mg/m3  is  recommended  for
aluminum  dust.  High levels of aluminum have been found  in  the
brains, muscles, and bones of patients with chronic renal failure
who  are  being treated with aluminum hydroxide, and  high  brain
levels  of aluminum are found in those suffering from  Alzheimers
disease (presenile dementia) which manifests behavioral changes.

Aluminum  and some of its compounds used in food preparation  and
as  food  additives  are generally recognized  as  safe  and  are
sanctioned  by  the Food and Drug Administration.  No  limits  on
aluminum  content  in  food  and  beverage  products  have   been
established.

Aluminum   has   no  adverse  effects  on   POTW   operation   at
concentrations normally encountered.  The results of an EPA study
                                117

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            GENERAL DEVELOPMENT DOCUMENT
                          SECT - VI
 of 50  POTW revealed that  49  POTW contained aluminum with  effluent
 concentrations   ranging from less than  0.1 mg/1  to  1.07 mg/1   and
 with an average  removal of 82 percent.
 Ammonia.    Ammonia
 pollutant.    It
   (chemical;formula NH3) is  a  nonconventional
is  a  colorless gas with a very  pungent  odor,
 detectable  at  concentrations  of  20  ppm  in  air  by  the  nose,  and  is
 very   soluble  in  water  (570 gm/1  at 25°C).   Ammonia  is  produced
 industrially   in   very  large  quantities (nearly 20  million  tons
 annually  in the U.S.).    It is converted to  ammonium  compounds  or
 shipped in  the liquid form  (it liquifies at  -33°C).   Ammonia  also
 results from natural processes.   Bacterial  action on nitrates  or
 nitrites,   as  well  as dead  plant  and  animal  tissue  and   animal
 wastes produces ammonia.  Typical domestic wastewaters contain  12
 to  50  mg/1  ammonia.
                           »
 The principal  use of ammonia  and  its compounds is as  fertilizer.
 High   amounts  are introduced  into soils and  the water runoff  from
 agricultural land by this use.  Smaller quantities of ammonia are
 used as a refrigerant.  Aqueous ammonia (2 to  5 percent solution)
 is  widely used as a household cleaner.  Ammonium compounds  find a
 variety of  uses in various industries;  as an  example,  ammonium
 hydroxide is used as a  reactant in  the  purification of tungsten.

 Ammonia is  toxic  to humans by inhalation of  the gas or  ingestion
 of  aqueous  solutions.  The ionized  form, ammonium (NH4+), is  less
 toxic  than the un-ionized form.  Ingestion  of as little  as  one
 ounce  of   household ammonia  has  been reported as a   fatal  dose.
 Whether inhaled or ingested,  ammonia acts destructively on  mucous
 membrane  with resulting loss of  function.   Aside from breaks   in
 liquid ammonia refrigeration equipment, industrial  hazard  from
 ammonia  exists   where . solutions of ammonium  compounds  may  be
 accidentally treated with a strong  alkali, releasing ammonia gas.
 As  little  as  150  ppm ammonia  in  air  is  reported  to  cause
 laryngeal   spasms   and  inhalation  of  5,000  ppm  in  air   is
 considered  sufficient to result in  death.

 The  behavior  of  ammonia in POTW  is well documented because it i.s
 a   natural  component of domestic wastewaters.   Only  very  high
 concentrations  of ammonia compounds could  overload  POTW.   One
 study       has  shown that concentrations of  un-ionized  ammonia
 greater  than      90  mg/1   reduce  gasification  in   anaerobic
 digesters   and    concentrations  of  140  mg/1  stop   digestion
 completely.     Corrosion  of  copper      piping  and   excessive
 consumption   of  chlorine  also  result  from      high  ammonia
 concentrations.     Interference   with   aerobic   nitrification
processes   can  occur  when  large  concentrations  of   ammonia
 suppress dissolved oxygen.  Nitrites are then produced instead of
nitrates.    Elevated nitrite concentrations in drinking water are
known to cause infant methemoglobinemia.

Cobalt.  Cobalt is a nonconventional pollutant.  It is a brittle,
hard,  magnetic, gray metal with a reddish tinge.   Cobalt ores are
usually the  sulfide or arsenic [smaltite-(Co,  Ni)As2; cobaltite-
CoAsS]   and   are  sparingly distributed  in  the  earth's  crust.
                               118

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Cobalt  is  usually  produced as a by-product of  mining  copper,
nickel,  arsenic, iron, manganese, or silver.  Because of     the
variety  of  ores  and the very  low  concentrations  of  cobalt,
recovery  of  the  metal  is accomplished  by  several  different
processes.   Most  consumption  of cobalt is  for  alloys.   Over
two-thirds of U.S.  production goes to heat-resistant,  magnetic,
and wear-resistant alloys.   Chemicals and color pigments make up
most of the rest of consumption.

Cobalt  and  many  of its alloys  are  not  corrosion  resistant;
therefore,   minor  corrosion  of  any  of  the  tool  alloys  or
electrical      resistance alloys can contribute to its  presence
in  raw  wastewater from a variety of  manufacturing  facilities.
Additionally,     the use of cobalt soaps used in coatings may be
a  general source     of small quantities of the metal.   Several
cobalt  pigments  are     used in paints to  produce  yellows  or
blues.

Cobalt is an essential nutrient for humans and other mammals, and
is  present  at  a fairly constant level of about 1.2 mg  in  the
adult  human  body.   Mammals  tolerate low  levels  of  ingested
water-soluble  cobalt  salts without  any  toxic  symptoms;  safe
dosage levels in man have been stated to be 2-7 mg/kg body weight
per  day.   A goitrogenic effect in humans is observed after  the
systematic  administration of 3-4 mg cobalt as cobaltous chloride
daily  for  three weeks.   Fatal heart disease among  heavy  beer
drinkers was attributed to the cardiotoxic action of cobalt salts
which  were formerly used as additives to improve  foaming.   The
carcinogenicity  of cobalt in rats has  been  verified;  however,
there  is  no evidence for the involvement of dietary  cobalt  in
carcinogenisis in mammals.

There  are  no data available on the behavior of cobalt in  POTW.
There are no data to lead to an expectation of adverse effects of
cobalt  on POTW operation or the utility of sludge from POTW  for
crop application.   Cobalt which enters POTW is expected to  pass
through to the effluent unless sufficient sulfide ion is present,
or  generated  in  anaerobic  processes  in  the.  POTW  to  cause
precipitation of the very insoluble cobalt sulfide.

Fluoride.   Fluoride  ion  (F-) is a  nonconventional  pollutant.
Fluorine  is  an extremely reactive,  pale yellow  gas which  is
never found free in nature.   Compounds of fluorine - fluorides -
are found widely distributed in nature.   The principal  minerals
containing   fluorine   are   fluorspar   (CaF2)   and   cryolite
(Na2AlFs).    Although   fluorine  is  produced  commercially  in.
small  quantities  by  electrolysis of  potassium  bifluoride  in
anhydrous  hydrogen  fluoride, the elemental  form  bears  little
relation      to the combined ion.  Total production of  fluoride
chemicals  in  the U.S. is difficult to estimate because  of  the
varied uses. Large volume usage compounds are:  calcium  fluoride
(estimated  1,500,000  tons in U.S.)  and  sodium  fluoraluminate
(estimated  100,000 tons in U.S.).  Some fluoride  compounds  and
their  uses  are sodium fluoroaluminate  -  aluminum  production;
calcium  fluor-ide - steelmaking, hydrofluoric  acid  production,
                               119

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
enamel,  iron  foundry; boron trifluoride  -  organic  synthesis;
antimony penta-fluoride - fluorocarbon production; fluoboric acid
and fluobor-ates - electroplating; perchloryl fluoride (C103F)
rocket  fuel  oxidizer;  hydrogen  fluoride  -  organic  fluoride
manufacture, pickling acid in stainless steelmaking   manufacture
of  aluminum  fluoride  sulfur hexafluoride - insulator  in  high
voltage  trans-formers; polytetrafluoroethylene - inert
Sodium  fluoride  is used at a concentration of about 1
many  public  drinking water supplies to prevent tooth
children.
              plastic.
              mg/1  in
             decay  in
The   toxic   effects  of  fluoride  on  humans  include   severe
gastroenteritis,  vomiting,  diarrhea,  spasms, weakness, thirst,
failing pulse and delayed blood coagulation.   Most  observations
of toxic     effects are made on individuals who intentionally or
accidentally  ingest  sodium  fluoride intended for  use  as  rat
poison  or insecticide. Lethal doses for adults are estimated  to
be  as  low as 2.5 g. At 1.5 ppm in drinking water,  mottling  of
tooth  enamel is reported, and 14 ppm, consumed over a period  of
years,  may  lead to deposition of calcium fluoride in  bone  and
tendons.

Fluorides  found in irrigation waters in high concentrations have
caused damage to certain plants exposed to these waters.  Chronic
fluoride poisoning of livestock has been observed.  Fluoride from
waters  apparently  does  not  accumulate in  soft  tissue  to  a
significant degree; it is transferred to a very small extent into
the  milk  and to a somewhat greater degree in  eggs.   Data  for
fresh water indicate that fluorides are toxic to fish.

Very  few data are available on the behavior of fluoride in POTW.
Under usual operating conditions in POTW,  fluorides pass through
into  the  effluent.    Very  little  of  the  fluoride  entering
conventional   primary  and  secondary  treatment  processes   is
removed.  In    one study of POTW influents conducted by the U.S.
EPA,  nine  POTW    reported concentrations of  fluoride  ranging
from   0.7   mg/1  to  1.2     mg/1,   which  is  the  range   of
concentrations used for fluoridated drinking water.

Iron.   Iron is a nonconventional pollutant.  It is  an  abundant
metal found at many places in the earth's crust.  The most common
iron  ore  is  hematite (Fe2O3) from which iron  is  obtained  by
reduction  with  carbon.   Other forms  of  commercial  ores  are
magnetite  (F63O4)  and  taconite  (FeSiO).   Pure  iron  is  not
often  found  in commercial use, but it is usually  alloyed  with
other metals and minerals.  The most common of these is carbon.

Iron is the basic element in the production of steel.   Iron with
carbon is used for casting of major parts of machines and it  can
be machined,  cast,  formed, and welded.   Ferrous iron is used in
paints,  while  powdered iron can be sintered and used in  powder
metallurgy.   Iron  compounds are also used to precipitate  other
metals   and  undesirable  minerals  from  industrial  wastewater
streams.
                               120

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           GENERAL DEVELOPMENT DOCUMENT
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Corrosion  products of iron in water cause staining of  porcelain
fixtures,  and ferric iron combines with tannin to produce a dark
violet   color.    The  presence  of  excessive .iron  in   water
discourages cows from drinking and thus reduces milk  production.
High     concentrations of ferric and ferrous ions in water  kill
most fish    introduced to the solution within a few hours.   The
killing     action  is attributed to coatings of  iron  hydroxide
precipitates     on  the  gills.   Iron  oxidizing  bacteria  are
dependent  on iron in    water for growth.   These bacteria  form
slimes that can affect the    aesthetic values of bodies of water
and  cause  stoppage  of  flows     in  pipes.    However,   high
concentrations of iron can precipitate    on bottom sediments and
affect rooted aquatic and invertebrate    benthos.

Iron is an essential nutrient and micro-nutrient for all_forms of
growth.   Drinking water standards in the U.S. set a limit of 0-.3
mg/1  of  iron in domestic water supplies based on aesthetic  and
organoleptic  properties of iron in water.

High  concentrations of iron do not pass through a POTW into  the
effluent.   In  some  POTW  iron  salts are  added  to  coagulate
precipitates  and suspended sediments into a sludge.   In an  EPA
study  of POTW,  the concentration of iron in the effluent of  22
biological  POTW meeting secondary treatment  performance  levels
ranged from 0.048 to 0.569 mg/1 with a median value of 0.25 mg/1.
This represented removals of 76 to 97 percent with a median of 87
percent removal.

Iron  in  sewage  sludge spread on  land  used  for  agricultural
purposes  is  not expected to have a detrimental effect on  crops
grown on the land.

Molybdenum.   Molybdenum  is present in the environment in  trace
quantities.  It is estimated that 3.6 x 1010 grams of molybdenum
are  released  into  surface waters of the  world  each  year  by
natural  processes.  Most surface waters contain less than  0.020
mg  Mo/1, and sea water concentrations range from 0.004 to  0.012
mg Mo/1. Finished waters in the United States contain a median of
0.0014  mg  Mo/1  and  a  maximum  of  0,068  mg  Mo/1.    Normal
concentrations in stream sediments range from 1 to 5 ppm Mo,  and
the concentration of molybdenum tends to increase with decreasing
grain size.

Molybdenum  is vitally necessary to plants and animals as  it is a
constituent  of  essential  enzymes needed  for  life  processes.
Molybdenum  concentrations in plants normally range from 1  to   2
ppm,  though  a  range of tenths to hundredths of ppm  have  been
observed.   Legumes  tend  to take up more molybdenum than  other
plants.   Accumulation  of  molybdenum in plants  occurs   without
detrimental effects.

Disease   related  to  molybdenum  in  humans  and  animals   has
historically been a  result of excessive uptake of molybdenum.

Average  daily  intake of molybdenum in the United States  varies
                                121

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            GENERAL  DEVELOPMENT DOCUMENT
SECT - VI
 between   0.120   and  0.240  mg Mo/day,  depending  on  age,   sex,   and
 family   income.    Estimated  daily  intake  of  molybdenum  in   the
 U.S.S.R.  has  been  been  reported  to  be between 0.329  and  0.376   mg
 Mo/day.   Abnormally  high intakes, as  high  as 10 to 15 mg  Mo/day,
 have been documented in India, the  U.S.S.R., and are suspected in
 Turkey.  Diet  plays a large part  in  determining  molybdenum  uptake.
 Legumes,  cereal  grains, leafy vegetables,  liver, and kidney beans
 are  among the  foods  which contain   greater   concentrations   of
 molybdenum than fruits, root and stem vegetables, muscle  meats,
 and dairy products.

 The  only  clinical  symptom resulting from excessive  molybdenum
 uptake in humans is  described as a  gout-like disease.  Study of a
 human  population  receiving  10  to   15   mg  Mo/day found  high
 incidence of  this  gout-like disease.   In addition, increased uric
 acid levels were noted.  Another study where humans  were  exposed
 to 10 mg  Mo/day  found greatly increased blood and  urine  levels of
 molybdenum,   and  significant increases in uric acid  excretion,
 though   the levels of uric acid were  still within  an  acceptable
 range  for humans.   For daily intake  levels between  0.5  and   1.0
 mg  Mo,   increased urinary copper excretion was noted   in human
 subjects.   Increased  urinary excretion of molybdenum   has  been
 observed  in humans whose water supply contained 0.050 to 0.200 mg
 Mo/1.   No  biochemical or clinical effects are known  in  humans
 whose water supply contains less than 0.050 mg  Mo/1.

 Sources of molybdenum for  animals are primarily in pasture forage
 and  grain  feed.     Intake  from  water   sources  is  not  very
 significant.  Molybdenum is more toxic  to  animals  than to  humans,
 and   cattle  and sheep are more susceptible to  disease caused   by
 excessive molybdenum than  rats, poultry, horses, and pigs.  These
 species   differences  are not understood.   The  Registry  of Toxic
 Effects   for  Chemical  Substances states  the   lower  toxic  dose
 (oral) for rats  and  rodents is 6.050  mg/kg.

 All cattle are susceptible to molybdenosis, with dairy cattle  and
 calves  showing  a   higher  susceptibility.   The  characteristic
 scouring disease ..and  weight loss may  be debilitating to  the point
 of permanent  injury  or death.    Pastures containing  20 to  100  ppm
 Mo  (dry  weight   basis)  are likely  to  induce  the  disease   as
 compared  to  health  forage containing  3 to 5 ppm  molybdenum   or
 less.   It  is   difficult  to assign  a  firm  threshold   value   of
 molybdenum  contained  in pasture that will include  molybdenosis
 because of the effects of two other dietary  constituents.   High
 levels  of molybdenum act to decrease the  retention of copper   in
 an animal.    Increased copper  intake  could,  therefore,   mitigate
 the  effect of high amounts of molybdenum.    The second  factor  in
 the diet is sulfate.    It has  been shown that in animals   showing
 increasing  levels of molybdenum,  an increase  in dietary  sulfate
 causes more of the molybdenum to be excreted harmlessly.

A  study  of the effects on frogs to changes  in  the  molybdenum
 concentration  in  the aqueous environment  concluded  that  while
 high  concentrations  of aqueous molybdenum  increased blood levels
of  molybdenum in frogs,  no deleterious effects  were  observed.
                               122

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
Laboratory  bioassays  involving  rainbow trout  have  also  been
conducted   to   determine  long-term  and  acute   toxicity   of
molybdenum.   Long-term toxicity tests included sodium  molybdate
dissolved in demineralized water in concentrations ranging from 0
to  17  mg/1 Mo.  After one year, results showed  no  significant
differences in growth and mortality for the exposed fish.   Acute
toxicity  results determined that for rainbow trout averaging  55
mm  and 20 mm, the 96 hr LC50 is 1,320 mg/1 Mo and 800  mg/1  Mo,
respectively.   Generally  it was concluded  that  molybdenum  as
molybdate in the aquatic environment constitutes little danger to
rainbow trout.

A  third  study was done to determine whether or  not  molybdenum
mining  in Colorado was causing any environmental problems to the
natural  wildlife  in  geographic areas  impacted  by  molybdenum
mining and milling.   Animals in the area were assayed, fish were
placed a. mile downstream of mine tailings,  and tailings were fed
to  chicks.   No  serious  adverse  effects  were  discovered  in
animals,  and  chicks  fed  20  percent  mine  tailings  remained
healthy.   Some adverse effects and abnormal tissue were found in
the  fish,  but it was not certain whether these conditions  were
caused  by   excessive  molybdenum or  other  heavy  metals  also
present in the  stream.

In conclusion,  molybdenum is not very toxic to humans.  Clinical
effects have been reported at steady intake levels of 10 to 15 mg
Mo/day,  and  biochemical  effects in the range of 0.5 to  10  mg
Mo/day.  Below 0.5 mg Mo/day, there is no evidence of substantial
toxic effects of molybdenum to humans.

The  greatest problem of molybdenum toxicity involves cattle  and
other   ruminants.    These  animals  are  for  unknown   reasons
particularly susceptible to molybdenosis,  and in addition,  rely
entirely   on  forage  for food.   It is known  that  plants  can
accumulate  molybdenum  without  harmful  effects   but   herbage
containing  more   than  20 ppm Mo (dry weight basis)  may  cause
molybdenosis in cattle.

High molybdenum content in surface waters in the United States in
rare  and usually associated with molybdenum mining and  milling,
uranium mining and milling, copper mining and milling, molybdenum
smelting and purification,  or shale oil production.  Toxicity of
molybdenum  to  some  aquatic  life has been  shown  to  be  low.
Surface  or  ground waters high in molybdenum that are  used  for
farmland  irrigation may increase molybdenum content  of  plants.
This may have effects on animals further along the food chain.

Phenols (Total).  "Total Phenols"'  is a nonconventional pollutant
parameter"!   Total  phenols  is the result of analysis using  the
4-AAP  (4-aminoantipyrene)  method.   This  analytical  procedure
measures the color development of reaction products between 4-AAP
and  some phenols.   The results are reported  as  phenol.   Thus
"total phenol" is not total phenols because many phenols (notably
nitrophenols)  do not react.   Also,  since each reacting  phenol
contributes  to the color development to a different degree,  and
                               123

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            GENERAL  DEVELOPMENT  DOCUMENT.
                                           • SECT .-• 'VI
 each phenol  has  a molecular  weight  different  from  others  and  from
 phenol  itself,   analyses  of  several mixtures  containing the   same
 total    concentration   in mg/1   of  several  phenols  will   give
 different  numbers depending  on the  proportions  in  the  particular
 mixture.

 Despite these limitations of the  analytical method,  total phenols
 is  a   useful  parameter  when .the mix of  phenols   is  relatively
 constant and an  inexpensive  monitoring method is desired.  In any
 given   plant or even  in  an  industry  subcategory,   monitoring of
 "total  phenols" provides an indication of the , concentration of
 this  group  of priority pollutants  as well as those phenols  not
 selected as  priority pollutants.  A further advantage  is  that the
 method  is  widely used  in  water quality determinations.

 In an EPA  survey of 103 POTW the  concentration of  "total phenols"
 ranged  from 0.0001 mg/1 to 0.176  mg/1 in the influent,  with  a
 median  concentration of 0.016 mg/1.   Analysis of  effluents   from
 22  of  these  same POTW  which had  biological treatment  meeting
 secondary  treatment   performance levels showed  "total  phenols"
 concentrations ranging from  0 mg/1  to 0.203 mg/1 with  a median of
 0.007.   Removals  were  64  to 100  percent with a   median  of 78
 percent.

 It  must   be recognized, however,  that six of  the  11  priority
 pollutant  phenols could be present  in high concentrations and not
 be  detected.  Conversely, it is  possible, but not  probable,  to
 have  a  high  "total  phenol" concentration   without   any  phenol
 itself  or  any of the 10 other priority pollutant phenols present.
 A  characterization  of   the phenol mixture to  be  monitored to
 establish  constancy of  composition  will allow "total phenols"  to
 be used with confidence.
Titanium.   Titanium  is a nonconventional pollutant.   It  is  a
           white  metal  occurring  as  the  oxide  in   ilmenite
            and  rutile  (TiO2).   The metal  is  used  in  heat-
            high-strength, light-weight alloys for  aircraft  and
           It. is also used in surgical appliances because of  its
                and  light  weight.   Titanium  dioxide  is  used
lustrous
(PeO*TiO2)
resistant,
missiles.
high  strength
extensively as a white pigment; in paints, ceramics, and plastics.
Toxicity.data on titanium are not abundant.   Because of the lack
of  definitive data, titanium compounds are generally  considered
non-toxic.   Large  oral  doses of titanium  dioxide  (TiO2)  and
thiotitanic  acid (H4TiS03) were tolerated by rabbits for several
days  with no toxic symptoms.   However,  impaired  reproductive
capacity was observed in rats fed 5 mg/1 titanium as titanite  in
drinking  water.   There was also a reduction in the  male/female
ratio  and  in  the  number of animals  surviving  to  the  third
generation.   Titanium  compounds are reported to inhibit several
enzyme systems and to be carcinogenic.

The  behavior of titanium in POTW has not been studied.    On  the
basis of the insolubility of the titanium oxides in water,  it is
expected  that  most  of the titanium entering the POTW  will  be
                               124

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
removed by settling and will remain in the sludge.   No data were
found  regarding  possible  effects  on plants  as  a  result  of
spreading titanium-containing sludge on agricultural cropland.

SUMMARY OF POLLUTANT SELECTION

After  examining  the sampling  data,  pollutants  and  pollutant
parameters were selected by subcategory for further consideration
for  limitation.   The selection of a pollutant was based on  the
concentration  of the pollutant in the raw sampling data and  the
frequency   of   occurrence   above   concentrations   considered
treatable.   The  pollutants selected under  this  rationale  are
listed  in  Table VI-2 (page 131). The analysis that led  to  the
selection  of  these  priority pollutants and  the  exclusion  of
pollutants  is  presented  in  Section  VI  of  each  subcategory
supplement.
                               125

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                           Table VI-1

                 LIST OF 129 PRIORITY POLLUTANTS
Compound Name

  1.  acenaphthene
  2.  acrolein
  3.  acrylonitrile
  4.  benzene
  5.  benzidene
  6.  carbon tetrachloride (tetrachloromethane)

   Chlorinated benzenes (other than dichlorobenzenes)

  7.  chlorobenzene
  8.  1,2,4-trichlorobenzene
  9.  hexachlorobenzene

   Chlorinated ethanes (including 1,2-dichloroethane,
   1,1,1-trichloroethane and hexachloroethane)

 10.  If2-dichloroethane
 11.  1/lf1-trichloroethane
 12.  hexachloroethane
 13.  1,1-dichloroethane
 14.  1,1,2-trichloroethane
 15.  1,1,2,2-tetrachloroethane
 16.  chloroethane

   Chloroalkyl ethers  (chloromethyl, chloroethyl  and
   mixed  ethers)

 17.  bis(chloromethyl)  ether (deleted)
 18.  bis (2-chloroethyl)  ether
 19.  2-chloroethyl vinyl  ether (mixed)

   Chlorinated naphthalene

 20.  2-chloronaphthalene

   Chlorinated phenols (other than  those  listed elsewhere
   includes  trichlorophenols  and  chlorinated  cresols)

 21.   2,4,6-trichlorophenol
 22.   parachlorometa cresol
 23.   chloroform  (trichloromethane)
 24.   2-chlorophenol
                              126

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     Table Vl-1 (Continued)

                 LIST OF 129 PRIORITY POLLUTANTS
  Dichlorobenzenes

25.  1,2-dichlorobenzene
26.  1,3-dichlorobenzene
27.  1,4-dichlorobenzene
  Dichlorobenzidine

28.  3,3'-dichlorobenzidine

  Dichloroethylenes (lf1-dichloroethylene and
  1,2-dichloroethylene)

29.  1,1-dichloroethylene
30.  1,2-trans-dichloroethylene
31.  2,4-dichlorophenol

  Dichloropropane and dichloropropene

32.  I,2-dichloropropane
33.  1,2-dichloropropylene (1,3-dichloropropene)
34.  2,4-dimethylphenol

  Dinitrotoluene

35.  2,4-dinitrotoluene
36.  2,6-dinitrotoluene
37.  1,2-diphenylhydrazine
38.  ethylbenzene
39.  fluoranthene

  Haloethers (other than those listed elsewhere)

40.  4-chlorophenyl phenyl ether
41.  4-bromophenyl phenyl ether
42.  bis(2-chloroisopropyl) ether
43.  bis(2-choroethoxy) methane


  Halomethanes (other than those listed elsewhere)

44.  methylene chloride (dichloromethane)
45.  methyl chloride (chloromethane)
46.  methyl bromide (bromomethane)
                               127

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     Table VI-1 (Continued)

                 LIST OF 129 PRIORITY POLLUTANTS
  Halomethanes (Cont.)

47.  bromoform (tribromomethane)
48.  dichlorobromomethane
49.  trichlorofluoromethane (deleted)
50.  dichlorofluoromethane (deleted)
51.  chlorodibromomethane
52.  hexachlorobutadiene
53.  hexachlorocyclopentadiene
54.  isophorone
55.  naphthalene
56.  nitrobenzene

  Nitrophenols (including 2,4-dinitrophenol and dinitrocresol)

57.  2-nitrophenol
58.  4-nitrophenol
59.  2,4-dinitrophenol
60.  4,6-dinitro-o-cresol

  Nitrosamines

61.  N-nitrosodimethylamine
62.  N-nitrosodiphenylamine
63.  N-nitrosodi-n-propylamine
64.  pentachlorophenol
65.  phenol

  Phthalate esters

66.  bis(2-ethylhexyl) phthalate
67.  butyl benzyl phthalate
68.  di-n-butyl phthalate
69.  di-n-octyl phthalate
70.  diethyl phthalate
71.  dimethyl phthalate

  Polynuclear aromatic hydrocarbons

72.  benzo (a)anthracene (1,2-benzanthracene)
73.  benzo (a)pyrene (3,4-benzopyrene)
74.  3,4-benzofluoranthene
75.  benzo(k)fluoranthane (11,12-benzofluoranthene)
                               128

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           GENERAL DEVELOPMENT  DOCUMENT
SECT - VI
                     Table  VI-1  (Continued)

                 LIST OF  129  PRIORITY  POLLUTANT
  Polynuclear aromatic  hydrocarbons  (Cont.)

76.  chrysene
77.  acenaphthylene          L
78.  anthracene
79.  benzo(ghi)perylene (1,11-benzoperylene)
80.  fluorene
81.  phenanthrene
82.  dibenzo  (a,h)anthracene  (1,2,5,6-dibenzanthracene)
83.  indeno  (1,2,3-cd)pyrene  (w,e,o-phenylenepyrene)
84.  pyrene
85.  tetrachloroethylene
86.  toluene                  :••..•
.87.  trichloroethylene
88.  vinyl chloride  (chloroethylene)

  Pesticides and metabolites

89.  aldrin
90.  dieldrin
91.  chlordane (technical mixture and metabolites)

  DDT and metabolites

92.  4,4'-DDT
93.  4,4'-DDE(p,p'DDX)
94.  4,4'-DDD(p,p TDE)

  Polychlorinated biphenyls  (PCS's)

  Endosulfan and metabolites
95.  a-endosulfan-Alpha
96.  b-endosulfan-Beta
97.  endosulfan sulfate

  Endrin and metabolites

98.  endrin             . ,
99.  endrin aldehyde

  Heptachlor and mefab.o.li.tes-

100.  heptachlor
101.  heptachlor epoxide
                                1.29

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     Table Vl-rl  (Continued)

                 LIST OF 129 PRIORITY POLLUTANTS
  Hexachlorocyclohexane  (all isomers)

102.  a-BHC-Alpha
103.  b-BHC-Beta
104.  r-BHC  (lindane)-Gamma
105.  g-BHC-Delta
106.  PCB-1242  (Arochlor 1242)
107.  PCB-1254  (Arochlor 1254)
108.  PCB-1221  (Arochlor 1221)
109.  PCB-1232  (Arochlor 1232)
110.  PCB-1248  (Arochlor 1248)
111.  PCB-1260  (Arochlor 1260)
112.  PCB-1016  (Arochlor 1016)

  Other

113.  toxaphene

  Metals and Cyanide, and Asbestos

114.  antimony
115.  arsenic
116.  asbestos  (Fibrous)
117.  beryllium
118.  cadmium
119.  chromium  (Total)
120.  copper
121.  cyanide (Total)
122.  lead
123.  mercury
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
129.  2,3,7,8-tetra chlorodibenzo-p-dioxin (TCDD)
                               130

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                            TABLE VI-2

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Bauxite Refining

21.  2,4,6-trichlorophenol
24.  2-chlorophenol
31.  2,4-dichlorophenol
57.  2-nitrophenol
58.  4-nitrophenol
65.  phenol
     phenols (4-AAP)
     pH

Primary Aluminum Smelting Subcategory

  1.  acenaphthene
 39.  fluoranthene
 55.  naphthalene
 72.  benzo(a)anthracene (1,2-benzanthracene)
 73.  benzo(a)pyrene
 76.  chrysene
 78.  anthracene (a)
 79.  benzo(ghi)perylene (1,11-benzoperylene)
 80.  fluorene
 81.  phenanthrene  (a)
 82.  dibenzo(a,h)anthracene (1,2,5,6-dibenzanthracene)
 84.  pyrene
114.  antimony
115.  arsenic
116.  asbestos (Fibrous)
118.  cadmium
119.  chromium (Total)
120.  copper
121.  cyanide (Total)
122.  lead
124.  nickel
125.  selenium
128.  zinc
      aluminum
      fluoride
      oil and grease
      TSS
      pH

  (a)  Reported together
                               131

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2  (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Aluminum Subcategory

 65.  phenol
118.  cadmium
122.  lead
128.  zinc
      aluminum
      ammonia (N)
      total phenolics (by 4-AAP method)
      oil and grease
      TSS
      PH

Primary Electrolytic Copper Refining Subcategory

115.  arsenic
119.  chromium (Total)
120.  copper
122.  lead
124.  nickel
126.  silver
128.  zinc
      TSS
      pH

Primary Lead Subcategory

116.  asbestos (Fibrous)
118.  cadmium
122.  lead
128.  zinc
      TSS
      pH

Primary Zinc Subcategory

115.  arsenic
116.  asbestos (Fibrous)
118.  cadmium
119.  chromium (Total)
120.  copper
122.  lead
124.  nickel
126.  silver
128.  zinc
      TSS
      pH
                               132

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Metallurgical Acid Plants

114.  antimony
115.  arsenic
118.  cadmium
119.  chromium
120.  copper
122.  lead
123.  mercury
124.  nickel
125.  selenium
126.  silver
128.  zinc
      fluoride
      molybdenum
      total suspended solids (TSS)
      pH


Primary Tungsten Subcategory
 11.  1,1,1-trichloroethane
 55.  naphthalene
 65.  phenol
 73.  benzo(a)pyrene
 79.  benzo(ghi)perylene
 82.  dibenzo(a,h)anthracene
 85.  tetrachloroethylene
 86.  toluene
118.  cadmium
119.  chromium  (Total)
122.  lead
124.  nickel
126.  silver
127.  thallium
128.  zinc
      ammonia (N)
      TSS
      pH
                               133

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Primary Columbium-Tantalum Subcategory

  4.  benzene
  6.  carbon tetrachloride
  7.  chlorobenzene
  8.  1,2,4—trichlorobenzene
 10.  I,2-dichloroethane
 30.  If2-trans-dichloroethylene
 38.  ethylbenzene
 51.  chlorodibromomethane
 85.  tetrachloroethylene
 87.  trichloroethylene
114.  antimony
115.  arsenic
116.  asbestos (Fibrous)
118.  cadmium
119.  chromium (Total)
120.  copper
122.  lead
124.  nickel
125.  selenium
127.  thallium
128.  zinc
      ammonia (N)
      fluoride
      TSS
      PH
                               134

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Silver Subcategory

  4.  benzene
  6.  carbon tetrachloride (tetrachloromethane)
 10.  lf2-dichloroethane
 11.  1,1,1-trichloroethane
 29.  1,1-dichloroethylene
 30.  I,2-trans-dichloroethylene
 38.  ethylbenzene
 84.  pyrene
 85.  tetrachloroethylene
 86.  toluene
 87.  trichloroethylene
114.  antimony
115.  arsenic
118.  cadmium
119.  chromium (Total)
120.  copper
121.  cyanide
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
      ammonia (N)
      total phenolics (by 4-AAP method)
      TSS
      pH

Secondary Lead Subcategory

114.  antimony
115.  arsenic
118.  cadmium
119.  chromium (Total)
120.  copper
122.  lead
124.  nickel
126.  silver
127.  thallium
128.  zinc
      ammonia
      TSS
      pH
                               135

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Primary Antimony Subcategory

114.  antimony
115.  arsenic
118.  cadmium
120.  copper
122.  lead
123.  mercury
128.  zinc
      total suspended solids (TSS)
      pH

Primary Beryllium

117.  beryllium
119.  chromium
120.  copper
121.  cyanide
      ammonia (as N)
      fluoride
      total suspended solids (TSS)
      pH

Primary and Secondary Germanium and Gallium
114.
115.
118.
119.
120.
122.
124.
125.
126.
127.
128.

antimony
arsenic
cadmium
chromium
copper
lead
nickel
selenium
silver
thallium
zinc
fluoride
      germanium
      gallium
      total suspended solids (TSS)
      pH
                               136

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Indium

118.  cadmium
119.  chromium
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
      indium
      total suspended solids (TSS)
      PH

Secondary Mercury

122.  lead
123.  mercury
127.  thallium
128.  zinc
      total suspended solids (TSS)
      pH

Primary Molybdenum and Rhenium

115.  arsenic
119.  chromium (total)
120.  copper
122.  lead
124.  nickel
125.  selenium
128.  zinc
      ammonia (as N)
      fluoride
      molybdenum
      rhenium
      total suspended solids (TSS)
      PH
                               137

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Molybdenum and Vanadium

115.  arsenic
119.  chromium
120.  copper
122.  lead
124.  nickel
128.  zinc
      aluminum
      ammonia (as N)
      boron
      cobalt
      germanium
      iron
      manganese
      molybdenum
      tin
      titanium
      vanadium
      total suspended solids
      pH

Primary Nickel and Cobalt

120.  copper
124.  nickel
128.  zinc
      cobalt
      ammonia (as N)
      total suspended solids (TSS)
      PH

Secondary Nickel

115.  arsenic
119.  chromium
120.  copper
124.  nickel
128.  zinc
      total suspended solids (TSS)
      pH
                               138

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Primary Precious Metals and Mercury

115.  arsenic
118.  cadmium
119.  chromium
120.  copper
122.  lead
123.  mercury
124.  nickel
126.  silver
127.  thallium
128.  zinc
      gold
      oil and grease
      total suspended solids (TSS)
      PH

Secondary Precious Metals

114.  antimony
115.  arsenic
118.  cadmium
119.  chromium
120.  copper
121.  cyanide
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
      ammonia (as N)
      gold
      palladium
      platinum
      total suspended solids (TSS)
      pH
                               139

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Primary Rare Earth Metals

  4.  benzene
  9.  hexachlorobenzene
115.  arsenic
118.  cadmium
119.  chromium (total)
120.  copper
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
      total suspended solids (TSS)
      PH

Secondary Tantalum

114.  antimony
120.  copper
122.  lead
124.  nickel
126.  silver
128.  zinc
      tantalum
      total suspended solids (TSS)
      pH
                               140

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VI
                     TABLE VI-2 (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Tin

114.  antimony
115.  arsenic
118.  cadmium
119.  chromium
120.  copper
121.  cyanide
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium
128.  zinc
      aluminum
      barium
      boron
      fluoride
      iron
      manganese
      tin
      total suspended solids (TSS)
      PH


Primary and Secondary Titanium

114.  antimony
118.  cadmium
119.  chromium (total)
120.  copper
122.  lead
124.  nickel
127.  thallium
128.  zinc
      titanium
      oil and grease
      total suspended solids (TSS)
      pH
                               141

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VI
                     TABLE VI -2  (Continued)

  POLLUTANTS SELECTED FOR FURTHER CONSIDERATION BY SUBCATEGORY

Secondary Tungsten and Cobalt

115.  arsenic
118.  cadmium
119.  chromium
120.  copper
122.  lead
124.  nickel
126.  silver
128.  zinc
      ammonia (as N)
      cobalt
      tungsten
      oil and grease
      total suspended solids (TSS)
      PH

Secondary Uranium
114
115
118
119
120
122
124.
125.
126.
128.
      antimony
      arsenic
      cadmium
      chromium (total)
      copper
      lead
      nickel
      selenium
      silver
      zinc
      fluoride
      uranium
      total suspended solids (TSS)
Primary Zirconium and Hafnium

118.  cadmium
119.  chromium (total)
121.  cyanide (total)
122.  lead
124. , nickel
127.  thallium
128.  zinc
      ammonia (as N)
      hafnium
      radium-226
      zirconium
      total suspended solids (TSS)
      pH
                               142

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           GENERAL DEVELOPMENT DOCUMENT    SECT - VI
                           FIGURE VI-3
               POLYNUCULEAR AROMATIC HYDROCARBONS
                 (Toxic Pollutant No's 72 - 84)
72  Benzo(a)anthracene (1,2-benzanthracene)  ^^   m.p. 162°C
                                           Col
73  Benzo(a)pyrene (3,4-benzopyrene)
74  3,4-Benzofluoranthene
75  Benzo(k)fluoranthene
      (11,12-benzofluoranthene)
76  Chrysene (1,2-benzphenanthrene)
77  Acenaphthylene
                                                  m.p. 168°C
                                                  m.p. 217°C
                                       HC = CH
                                      -(PIP)
                                                  m.p. 255°C
m.p. 92°C
78  Anthracene
                                     SMS)
                                                  m.p.  216°C
79  Benzo(ghi)perylene
      (1,12-benzoperylene)
                                                  m.p.  not reported
80  Fluorene (alpha-diphenylenemethane)
                                                  m.p.  116°C
81  Phenanthrene
                               143
                                                  m.p.  101°C

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           GENERAL DEVELOPMENT DOCUMENT    SECT - VI
                     FIGURE VI-3 (Continued)

               POLYNUCULEAR AROMATIC HYDROCARBONS
                 (Toxic Pollutant No's 72 - 84)
82  Dibenzo(a,h)anthracene
      (1,2,5,6-dibenzoanthracene)
m.p. 269°C
83  Indeno (l,2,3-cd)pyrene
      (2,3-o-phenylenepyrene)
84  Pyrene
m.p. not available
m.p. 156°C
                               144

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           GENERAL DEVELOPMENT DOCUMENT    SECT - VI
                           FIGURE VI-3

               POLYNUCULEAR AROMATIC HYDROCARBONS
                 (Toxic Pollutant No's 72 - 84)
72  Benzo(a)anthracene (1,2-benzanthracene)  >>.   m.p. 162°C
73  Benzo(a)pyrene (3,4-benzopyrene)
74  3,4-Benzofluoranthene
75  Benzo(k)fluoranthene
      {11,12-benzofluoranthene)
                                                  m.p. 176°C
                                                  m.p. 168°C
                                                  m.p. 217°C
76  Chrysene (1,2-benzphenanthrene)
77  Acenaphthylene
                                       HC
                                          CH
                                                  m.p. 255°C
m.p. 92°C
78  Anthracene
                                                  m.p. 216°C
79  Benzo(ghiJperylene
      (1,12-benzoperylene)
                                                  m.p. not reported
80  Fluorene (alpha-diphenylenemethane)
                                                  m.p. 116°C
81  Phenanthrene
                               143
                                                  m.p. 101°C

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           GENERAL DEVELOPMENT DOCUMENT    SECT - VI
                     FIGURE VI-3 (Continued)

               POLYNUCULEAR AROMATIC HYDROCARBONS
                 (Toxic Pollutant No's 72 - 84)
82  Dibenzo(a,h)anthracene
      (1,2,5,6-dibenzoanthracene)
m.p. 269°C
83  Indeno (l,2,3-cd)pyrene
      (2,3-o-phenylenepyrene)
84  Pyrene
m.p. not available
m.p. 156°C
                               144

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
                 NONFERROUS METALS MANUFACTURING

                           SECTION VII

                CONTROL AND TREATMENT TECHNOLOGY
This section describes the treatment techniques currently used or
available to remove or  recover  wastewater  pollutants  normally
generated by the nonferrous metals manufacturing industrial point
source  category.  Included are discussions of individual end-of-
pipe treatment technologies  and  in-plant  technologies.   These
treatment   technologies  are  widely  used  in  many  industrial
categories,  and  data   and   information   to   support   their
effectiveness  has  been  drawn  from  a  similarly wide range of
sources and data bases.

               END-OF-PIPE TREATMENT TECHNOLOGIES

Individual recovery  and  treatment  technologies  are  described
which  are  used  or  are suitable for use in treating wastewater
discharges from nonferrous  metals  manufacturing  plants.   Each
description  includes  a functional description and discussion of
application  and   performance,   advantages   and   limitations,
operational  factors  (reliability,  maintainability, solid waste
aspects), and  demonstration  status.   The  treatment  processes
described include both technologies presently demonstrated within
the  nonferrous  metals  manufacturing category, and technologies
demonstrated  in treatment of similar wastes in other industries.

Nonferrous         metals       manufacturing         wastewaters
characteristically    may contain  treatable  concentrations   of
toxic    metals.    The  toxic  metals    antimony,      arsenic,
beryllium,     cadmium,    chromium,  copper,    lead,   mercury,
nickel,  selenium,  silver,  thallium  and  zinc  are   found  in
nonferrous    metals   manufacturing   wastewater   streams    at
treatable concentrations;   and  are  generally  free from strong
chelating agents.   Aluminum,   ammonia,  barium,  boron, cesium,
cobalt,  columbium,  cyanide, fluoride, gallium, germanium, gold,
hafnium,    indium,    iron,  manganese,  molybdenum,  palladium,
phosphorus,  platinum,  radium-226,  rhenium, rubidium, tantalum,
tin,  titanium,  tungsten,  uranium, vanadium, zirconium and some
toxic organics (polynuclear aromatic  hydrocarbons  and  phenols)
also  may  be present.  The toxic inorganic pollutants constitute
the most significant wastewater pollutants in this category.

In  general,   these   pollutants   are   removed   by   chemical
precipitation  and sedimentation or filtration.  Most of them may
be effectively removed by precipitation of  metal  hydroxides  or
carbonates utilizing the reaction with lime, sodium hydroxide, or
sodium  carbonate.   For  some, improved removals are provided by
the use of sodium sulfide or ferrous sulfide to  precipitate  the
pollutants as sulfide compounds with very low solubilities.
                               145

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           GENERAL DEVELOPMENT, DOCUMENT
                                         SECT - VII
Discussion  of end-of-pipe treatment technologies is divided into
three parts:  the major technologies; treatment effectiveness  of
major technologies; and minor technologies.

MAJOR TECHNOLOGIES

In  Sections  IX,  X,  XI,  and  XII  the rationale for selecting
model   treatment   systems   is   discussed.    The   individual
technologies  used in  the  system  are  described   here.    The
major    end-of-pipe  technologies   for   treating    nonferrous
metals  manufacturing wastewaters are:  (1) chemical reduction of
chromium,    (2)    chemical   precipitation,     (3)     cyanide
precipitation,   (4)  granular   bed filtration,   (5)   pressure
filtration,   (6)   settling,   and  (7) skimming.   In practice,
precipitation   of  metals  and   settling   of   the   resulting
precipitates  is , often a unified two-step  operation.  Suspended
solids    originally    present  in  raw  wastewaters   are   not
appreciably affected  by  the  precipitation  operation  and  are
removed  with the precipitated metals in the settling operations.
Settling operations can be evaluated independently  of  hydroxide
or  other  chemical  precipitation  operations, but hydroxide and
other chemical precipitation operations can only be evaluated  in
combination with a solids removal operation.

1. Chemical Reduction of Chromium

Desc r ip t ion  of the Process.  Reduction is a chemical reaction in
which electrons are transferred to  the  chemical  being  reduced
from  the  chemical initiating the transfer (the reducing agent).
Sulfur  dioxide,  sodium  bisulfite,  sodium  metabisulf ite,  and
ferrous  sulfate  form strong reducing agents in aqueous solution
and are often used in industrial waste treatment  facilities  for
the  reduction of hexavalent chromium to the trivalent form.  The
reduction allows removal of chromium from solution in conjunction
with other metallic salts by alkaline precipitation.   Hexavalent
chromium is not precipitated as the hydroxide.

Gaseous  sulfur  dioxide  is  a  widely  used  reducing agent and
provides a  good  example  of  the  chemical  reduction  process.
Reduction  using  other  reagents  is  chemically  similar.   The
reactions involved may be illustrated as follows:

  3 S02+ 3 H20   ---- > 3 H2S03
3 H2S03 +
                     ---- > ^2(804)3 + 5 H20
The above reaction is favored by low pH.  A pH of from 2 to 3  is
normal for situations requiring complete reduction.  At pH levels
above  5,  the  reduction rate is slow.  Oxidizing agents such as
dissolved oxygen and ferric iron  interfere  with  the  reduction
process by consuming the reducing agent.

A  typical  treatment  consists  of  45  minutes  retention  in a
reaction tank.  The reaction tank  has  an  electronic  recorder-
                               146

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
controller  device  to control process conditions with respect to
pH and  oxidation  reduction  potential  (ORP).    Gaseous  sulfur
dioxide  is  metered  to  the  reaction  tank to maintain the ORP
within the range of 250 to  300  millivolts.   Sulfuric  acid  is
added  to  maintain  a pH level of from 1.8 to 2.0.  The reaction
tank is equipped with a propeller agitator  designed  to  provide
approximately  one turnover per minute.  Figure VII-13 (Page 266)
shows a continuous chromium reduction system.

Application and Performance.  Chromium reduction is most  usually
required  to  treat  electroplating  and  metal  surfacing  rinse
waters,  but  may  also  be   required   in   nonferrous   metals
manufacturing  plants.  A study of an operational waste treatment
facility chemically reducing tiexavalent chromium has shown that a
99.7 percent reduction  efficiency  is  easily  achieved.   Final
concentrations   of   0.05   mg/1   are   readily  attained,  and
concentrations of 0.01 mg/1 are considered to  be  attainable  by
properly maintained and operated equipment.

Advantages  and  Limitations.   The  major  advantage of chemical
reduction to reduce hexavalent chromium is that  it  is  a  fully
proven  technology  based on many years of experience.  Operation
at ambient conditions results in minimal energy consumption,  and
the process, especially when using sulfur dioxide, is well suited
to  automatic  control.   Furthermore,  the  equipment is readily
obtainable from many suppliers, and operation is straightforward.

One limitation of chemical reduction of  hexavalent  chromium  is
that  for  high concentrations of chromium, the cost of treatment
chemicals may be prohibitive.  When this situation occurs,  other
treatment  techniques are likely to be more economical.  Chemical
interference by oxidizing agents is possible in the treatment  of
mixed  wastes,  and the treatment itself may introduce pollutants
if not properly  controlled.   Storage  and  handling  of  sulfur
dioxide is somewhat hazardous.

Operational   Factors.   Reliability:   Maintenance  consists  of
periodic removal of sludge; the frequency.of removal  depends  on
the input concentrations of detrimental constituents.

Solid  Waste Aspects;  Pretreatment to eliminate substances which
will interfere with the process may  often  be  necessary.   This
process  produces  trivalent  chromium which can be controlled by
further treatment.  However,  small  amounts  of  sludge  may  be
collected  as the result of minor shifts in the solubility of the
contaminants.  This sludge can be processed by  the  main  sludge
treatment equipment.

Demonstration  Status.  The reduction of chromium waste by sulfur
dioxide or sodium bisulfite is a classic process and is  used  by
numerous  plants  which  have  hexavalent  chromium  compounds in
wastewaters from operations such  as  electroplating,  conversion
coating and noncontact cooling.
                               147

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 2.  Chemical  Precipitation

 Dissolved toxic   metal  ions  and certain anions  may be chemically
 precipitated for  removal by physical  means  such  as  sedimentation,
 filtration,  or  centrifugation.    Several  reagents   are  commonly
 used to effect  this  precipitation:

 1)   Alkaline compounds   such  as lime  or sodium hydroxide  may  be
 used to precipitate  many toxic  metal  ions  as  metal  hydroxides.
 Lime   also   may   precipitate  phosphates  as  insoluble  calcium
 phosphate, fluorides as  calcium fluoride and arsenic  as  calcium
 arsenate.

 2)   Both  "soluble"   sulfides  such'as  hydrogen  sulfide or  sodium
 sulfide and  "insoluble"  sulfides such as ferrous sulfide  may   be
 used to precipitate  many heavy  metal  ions as metal  sulfides.

 3)   Ferrous  sulfate,  zinc sulfate or  both (as  is required)  may  be
 used to precipitate  cyanide  as  a  ferro  or  zinc  ferricyanide
 complex.

 4)   Carbonate precipitates  may  be used  to remove metals either  by
 direct  precipitation using  a  carbonate  reagent   such  as  calcium
 carbonate  or  by  converting  hydroxides  into   carbonates using
 carbon  dioxide.

 These treatment chemicals may be added  to a flash mixer or  rapid
 mix   tank,   to  a  presettling tank, or  directly  to  a clarifier  or
 other   settling  device.    Because metal  hydroxides  tend   to   be
 colloidal    in  nature,  coagulating agents  may also be  added   to
 facilitate settling.  After the solids  have been removed,  final
 pH adjustment may  be required to reduce the high  pH created   by
 the  alkaline  treatment chemicals.

 Chemical precipitation as a mechanism for   removing  metals from
 wastewater    is    a   complex  process   of at least  two  steps
•precipitation  of  the   unwanted  metals   and   removal of  the
 precipitate.  Some  very  small  amount   of  metal    will    remain
 dissolved     in    the  wastewater    after    precipitation    is
 complete.     The   amount  of  residual dissolved  metal depends   on
 the  treatment  chemicals   used  and    related   factors.    The
 effectiveness  of  this   method   of removing any  specific   metal
 depends  on   the   fraction  of   the specific  metal   in the  raw
waste   (and   hence in the precipitate)  and  the   effectiveness   of
 suspended solids removal.   In   specific  instances,  a   sacrifical
 ion  such as  iron  or aluminum may be added  to aid in  the  removal
of   toxic  metals  by co-precipitation  process  and  reduce  the
 fraction of a specific metal  in  the precipitate.

Application   and   Performance.  Chemical precipitation  is used  in
nonferrous metals manufacturing  for  precipitation   of  dissolved
metals.    It  can  be used to remove metal  ions  such as aluminum,
antimony, arsenic, beryllium,  cadmium,  chromium,   copper,  lead,
mercury,   nickel,   zinc,  cobalt,  iron,  manganese,  tungsten,
molybdenum  and tin.    The process  is  also  applicable  to  any
                               148

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VII
substance  that  can   be transformed into an insoluble form such
as fluorides,  phosphates,  soaps,  sulfides and others.  Because
it is simple and effective, chemical precipitation is extensively
used for  industrial  waste treatment.

The  performance  of  chemical  precipitation  depends on several
variables.  The more important  factors  affecting  precipitation
effectiveness are:

1. Maintenance of an appropriate (usually alkaline) pH throughout
the precipitation reaction and subsequent settling;

2. Addition of a sufficient excess of treatment ions to drive the
precipitation reaction to completion;

3.  Addition  of  an  adequate supply of sacrifical ions (such as
iron or aluminum) to ensure precipitation and removal of specific
target ions; and

4. Effective removal  of  precipitated  solids  (see  appropriate
solids removal technologies).

Control  of_  pH.   Irrespective  of the solids removal technology
employed, proper  control  of  pH  is  absolutely  essential  for
favorable     performance     of      precipitation-sedimentation
technologies.  This is clearly illustrated by  solubility  curves
for selected metals hydroxides and sulfides shown in Figure  VII-
1,  (page  254),  and by plotting  effluent  zinc  concentrations
against  pH  as shown  in  Figure  VII-2   (page  255).    Figure
VII-2   was  obtained   from   Development   Document   for   the
Proposed   Effluent
Performance
                      Limitations  Guidelines  and   New   Source
	   Standards   for  the  Zinc  Segment  of  Nonferrous
Metals  Manufacturing  Point Source Category,  U.S.  E.P.A.,  EPA
440/1-74/033,November, 1974.   Figure VII-2  was  plotted  from
the  sampling data from several facilities with  metal  finishing
operations.  It is partially illustrated  by data  obtained  from
3  consecutive  days of sampling at one metal  processing   plant
(47432)  as displayed in Table VII-1  (page 235).  Flow   through
this  system  is  approximately 49,263 1/h (13,000 gal/hr).

This treatment system uses  lime  precipitation  (pH  adjustment)
followed  by  coagulant addition and sedimentation.  Samples were
taken before (in) and after (out) the treatment system.  The best
treatment for removal of copper arid zinc was achieved on day one,
when the pH was maintained at a satisfactory level.  The  poorest
treatment  was found on the second day, when the pH slipped to an
unacceptably low level; intermediate values were achieved on  the
third day, when pH values were less than desirable but in between
those for the first and second days.

Sodium  hydroxide  is  used  by  one  facility (plant 439) for^pH
adjustment  and  chemical  precipitation,  followed  by  settling
(sedimentation  and  a  polishing lagoon) of precipitated solids.
Samples were taken prior to caustic addition  and  following  the
polishing  lagoon.   Flow  through  the  system  is approximately
                               149

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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - VII
 22,700  1/hr.  (6,000  gal/hr).   These data  displayed  in  Table VII-2
 (page 235)  indicate  that  the   system  was operated efficiently.
 Effluent  pH  was  controlled within the range of  8.6 to  9.3, and,
 while raw waste  loadings  were   not  unusually  high,   most  toxic
 metals  were removed  to  very low concentrations.

 Lime  and   sodium  hydroxide   (combined)  are  sometimes  used  to
 precipitate metals.  Data developed from  plant 40063,  a  facility
 with a  metal  bearing wastewater, exemplify efficient operation  of
 a   chemical precipitation and  settling system.  Table  VII-3 (page
 236) shows  sampling  data  from   this  system,   which   uses   lime
 and  sodium     hydroxide  for   pH  adjustment    and  chemical
 precipitation,     polyelectrolyte   flocculant    addition,    and
 sedimentation.   Samples  were   taken  of  the  raw  waste influent
 to  the system and of the clarifier effluent.   Flow through  the
 system  is  approximately 19,000 1/hr (5,000 gal/hr).

 At  this  plant,   effluent  TSS levels were below 15 mg/1 on each
 day, despite  average raw  waste  TSS concentrations   of  over  3500
 mg/1.   Effluent   pH was maintained  at  approximately  8, lime
 addition was  sufficient to precipitate the dissolved metal  ions,
 and the  flocculant addition  and clarifier retention served  to
 remove  effectively the precipitated solids.

 Sulfide precipitation is  sometimes  used  to  precipitate  metals
 resulting   in  improved metals  removals.  Most metal sulfides are
 less soluble  than  hydroxides, and the precipitates  are frequently
 more dependably  removed from water.   Solubilities  for  selected
 metal   hydroxide,  carbonate and sulfide precipitates are shown  in
 Table   VII-4,   (page 236).    (Source:   Lange's    Handbook     of
 Chemistry).   Sulfide  precipitation is particularly effective  in
 removing specific  metals  such as silver  and  mercury.   Sampling
 data  from  three  industrial  plants using sulfide precipitation
 appear  in   Table VII-5  (page 237),  In  all  cases  except  iron,
 effluent  concentrations  are  below  0.1  mg/1 and in many cases
 below 0.01  mg/1 for  the three plants studied.

 Sampling data, from several chlorine-caustic manufacturing  plants
 using   sulfide    precipitation   demonstrate   effluent  mercury
 concentrations varying between 0.009 and 0.03 mg/1.  As shown   in
 Figure  VII-1 (page  254), the solubilities  of  PbS and  Ag2S
 are  lower  at  alkaline pH levels than either the   corresponding
 hydroxides  or   other    sulfide    compounds.     This   implies
 that    removal performance for lead and silver sulfides should  be
 comparable   to  or  better than that for the  metal  hydroxides.
Bench-scale  tests on   several  types   of    metal    finishing
and   manufacturing wastewater  indicate  that metals removal   to
 levels  of  less  than 0.05  mg/1 and in  some cases   less   than
 0.01   mg/1  are   common  in systems using  sulfide  precipitation
followed   by  clarification.   Some  of  the  bench-scale   data,
particularly  in   the case of  lead,  do  not support   such   low
effluent    concentrations.      However,  lead   is   consistently
 removed  to very low  levels   (less   than 0.02      mg/1)       in
systems    using   hydroxide  and   carbonate  precipitation  and
sedimentation.
                               150

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Of-  particular  interest is the ability of sulfide to precipitate
hexavalent  chromium  (Cr+°)  without prior  reduction   to   the
trivalent   state  as  is  required  in  the  hydroxide  process.
When ferrous sulfide is used as the precipitant, iron and sulfide
act as  reducing  agents for the hexavalent chromium according to
the reaction:

 Cr03 + FeS + 3H2O 	> Fe(OH)3 + Cr(OH)3 + S

The sludge produced in this reaction consists  mainly  of  ferric
hydroxides,  chromic  hydroxides,  and various metallic sulfides.
Some excess hydroxyl ions are generated in this process, possibly
requiring a downward re-adjustment of pH.

Based on the available data, Table VII-6  {page 238)  shows   the
minimum  reliably  attainable effluent concentrations for sulfide
precipitation-sedimentation systems.  These values  are  used  to
calculate   performance  predictions  of  sulfide  precipitation-
sedimentation systems.

Sulfide precipitation is used  in  many  process  and  wastewater
treatment  applications in nonferrous metals manufacturing.  This
technology is used to treat process  wastewater  discharges  from
cadmium  recovery  and to recover metals from zinc baghouse dusts
at a U.S. nonferrous metals manufacturing plant.   Another  plant
achieves  complete  recycle  of  electrolyte from copper refining
through removal of metal impurities  via  sulfide  precipitation.
Primary  tungsten  is  frequently  separated  from molybdenum via
sulfide precipitation.  In  secondary  tin  production,  lead  is
recovered   from   alkaline   detinning  solutions  with  sulfide
precipitation just prior to electrowinning.  In the production of
beryllium hydroxide, sulfide  precipitation  is  used  to  remove
metal  impurities  prior  to  precipitating  beryllium hydroxide.
These demonstrations show that sulfide precipitation is in use in
the nonferrous metals manufacturing  category  that  may  present
equal or greater treatment difficulties as wastewater.

Sulfide  precipitation also is used as a preliminary or polishing
treatment  technology   for   nonferrous   metals   manufacturing
wastewater.   A  U.S.  nonferrous  metals  manufacturing facility
specifically uses sulfide precipitation operated at a low  pH  to
remove  specific toxic metals from the acid plant blowdown  prior
to discharging the wastewater to  a  lime  and  settle  treatment
system.   Hydrogen  sulfide  is  used  to  precipitate  selenium.
Arsenic is also precipitated as arsenic sulfide.  The arsenic and
selenium sulfides are removed in a plate and frame  filter.   EPA
sampling  at  this plant found three-day averages of arsenic  and
selenium in the untreated acid plant blowdown of  4.74  mg/1  and
21.5  mg/1  of  arsenic  and  selenium,  respectively.  Composite
samples of treated  (sulfide precipitation  and  filtration)  acid
plant  blowdown  collected  during  the EPA sampling visit showed
arsenic concentrations at 0.066, 0.348 and 0.472 mg/1.  Likewise,
the  treated  acid  plant  blowdown  samples  contained  selenium
concentrations at 0.015, 0.05, and 0.132 mg/1.
                                151

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 Performance  data  collected  by personnel  at  this  same  plant  over  a
 one-year   time   period   (24  data  points)   indicate the  long-term
 arithmetic mean for  arsenic is 1.2 mg/1.  Selenium data   gathered
 at   the   same  plant  over  one year   (33   data  points)   show  a
 long-term arithmetic mean  of  0.53 mg/1.     The  effluent  data
 submitted to  the   Agency  are quite  variable due to the methods
 used to control reagent  addition  by   the   plant.  In fact, there
 is   almost   as much  variability in the treated effluent  from  the
 filter press as there is  in  the raw  acid  plant     blowdown.
 This  is   not   characteristic of the well-operated  treatment
 systems where a significant reduction  in variability  of  raw waste
 loads is  observed.    Hydrogen sulfide  is added  to the acid plant
 blowdown  based on flow  rate,    not influent  concentration.   EPA
 sampling   data   demonstrate   that slight  increases  in   influent
 arsenic   concentration  also   produce    similar  increases     in
 effluent     arsenic    concentrations.     This  is characteristic
 of   a system in which treatment reagents   are  not being    added
 in   sufficient  quantities.    The  Agency  believes more uniform
 performance   would   be   achieved   if    sulfide    addition    were
 properly  controlled using  a  specific  ion electrode.   This  method
 of control is demonstrated  in sulfide  treatment  to recover   silver
 from photographic   solutions.   In this   way,  excess sulfide is
 consistently added to ensure  proper precipitation  of  arsenic  and
 selenium  sulfides.

 While the   average   for  arsenic from  this  plant is 1.2  mg/1, the
 system as operated was able to achieve concentrations  as low as
 0.04  mg/1.   Likewise,  for selenium, concentrations as  low as  0.01
 mg/1  were   achieved.    The Agency recognizes  that it  is unlikely
 that  plants  could consistently achieve 0.04  mg/1 and   0.01  mg/1,
 respectively;  however,   this   performance  indicates  that through
 proper control of reagent addition the plant would vastly improve
 the  performance.

 Data  are also available  from  a  Swedish copper  and  lead smelter
 that  operates  a full-scale  sulfide precipitation and  hydroxide
 precipitation unit on  acid  plant  blowdown,  storm   water,  .and
 facility  cleaning   wastewaters.    The       full-scale  sulfide-
 hydroxide  precipitation plant  was  started up  in May  1978 and has
 operated  since  that  time.    The  plant   personnel   compared
 hydroxide  and  sulfide precipitation for removal of  toxic  metals
 at the bench scale prior  to design  of the full-scale plant.    On
 the   basis   of  laboratory  data,  they determined that a combined
 sulfide-hydroxide process would be  best.    This approach resulted
 in the best  overall  removals and yielded a sludge that   could  be
 recycled into the smelting process.

 This  Swedish plant  operates the sulfide precipitation portion of
 the process  at a pH  in the  range of 3 to 5 standard units.   This
 results  in  good copper, lead, and zinc removals as well as some
 reduction of arsenic and selenium.   This mode  of  operation  was
 selected  to  yield  a sludge containing copper and lead sulfides
 that  could be reintroduced  readily  into  the  smelter   furnaces.
Arsenic  concentrations  as low as  1.9  mg/1  were achieved even in
                               152

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
this mode which is not optimized for arsenic removal.

There is a Japanese copper  smelter  with  a  metallurgical  acid
plant  that  operates  a  sulfide  precipitation  and  filtration
preliminary treatment system.  The plant uses  sulfide  to  treat
acid  plant  blowdown  containing arsenic concentrations of 8,530
mg/1, copper at 120 mg/1, lead at 30 mg/1, copper  at  120  mg/1,
lead  at  30 mg/1 and cadmium at 60 mg/1.  The filtrate from this
treatment system typically contains concentrations of  0.03  mg/1
for arsenic, 0.03 mg/1 for copper, 0.5 mg/1 for lead and 0.3 mg/1
for  cadmium.   Wastewater from the acid plant is pumped from the
acid   plant to a 50-cubic-meter  stirred   reaction   tank where
sodium    hydrosulfide    is    added.     Completion   of    the
precipitation  reaction  is  measured  by  a  oxidation-reduction
potentiometer.   After the reaction is complete the wastewater is
pumped to a filter press to separate the precipitated solids from
solution.  The  filtrate  is  pumped  for  additional  wastewater
treatment downstream.

EPA   also   conducted   bench-scale  tests   to  determine   the
effectiveness    of   sulfide   precipitation   on  metallurgical
acid   plant   discharges.   Wastewater  samples  were  collected
from    a   U.S.   copper   smelter   and   refinery    with    a
metallurgical  acid  plant  on site.  The U.S. plant did not have
raw wastewater arsenic concentrations as high  as  those  of  the
Japanese plant; however, the arsenic concentrations from the U.S.
facility    have   been  observed  to  range  from  50-150  mg/1.
Bench-scale tests were conducted using sulfide precipitation  and
filtration  preliminary  treatment  in  the  same  way   as   the
full-scale  Japanese  plant.   At a pH of 1.5 standard units with
excess sodium sulfide, an arsenic concentration of 1.5  mg/1  was
achieved  with  this  preliminary  treatment.   The fact that the
concentration  achieved for arsenic in the bench-scale  tests  is
higher  (1.5  mg/1 as opposed to 0.03 mg/1) than that observed in
the full-scale Japanese facility is not unexpected.  The  purpose
of  the  bench-scale  tests  was  to  .demonstrate that  effective
removal of arsenic was possible.  These operating conditions were
not optimized as they were  in  the., full-scale  facility.    The
bench-scale   tests  are  described in greater detail in a report
entitled Laboratory Studies on Sulfide Precipitation Applied   to
Metallurgical   Acid  Plant  Wastewaters,  found  in  the  record
supporting this rulemaking.

Sulfide  precipitation  may  also  be  applied  following  or  in
conjunction     with    hydroxide    precipitation     (two-stage
treatment-lime followed  by  sulfide).    In  these  applications
sulfide   precipitation   acts  to  further  reduce  toxic  metal
concentrations.   Responses  to  Section  308   data   collection
portfolios   indicate  that  there  are  four  nonferrous  metals
manufacturing plants using sulfide precipitation as  a  polishing
step - two primary zinc-and two secondary silver plants.

EPA   conducted bench-scale tests to examine the effectiveness of
sulfide precipitation used in conjunction with lime precipitation
and following lime and settle treatment.   Sulfide  precipitation
                               153

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
used in conjunction with lime precipitation applied to wastewater
from  a  primary  zinc  process wastewater containing 1.4 mg/1 of
arsenic, 15 mg/1 of cadmium, 7 mg/1 of copper, 5 mg/1 of lead and
114 mg/1 of zinc, achieved effluent concentrations of  0.04  mg/1
of  arsenic,  0.05  mg/1  of cadmium, 0.038 mg/1 of copper, 0.027
mg/1 of lead  and  0.31  mg/1  of  zinc.   Sulfide  precipitation
applied  as  a  polishing  step after lime precipitation achieved
0.04 mg/1 of arsenic,  0.004  mg/1  of  cadmium,  0.014  mg/1  of
copper,  0.003  mg/1 of lead and 0.036 mg/1 of zinc when treating
the same process wastewater.

Carbonate precipitation is sometimes used to precipitate  metals,
especially  where precipitated metals values are to be recovered.
The solubility of most metal carbonates is  intermediate  between
hydroxide  and sulfide solubilities; in addition, carbonates form
easily  filtered  precipitates.   Carbonate  ions  appear  to  be
particularly  useful  in precipitating lead and antimony.  Sodium
carbonate has been observed being added at treatment  to  improve
lead  precipitation  and  removal in some industrial plants.  The
lead hydroxide and lead carbonate solubility curves displayed  in
Figure  VII-3  (page 256)  (Source:  "Heavy  Metals Removal,"  by
Kenneth Lanovette, Chemical Engineering/Deskbook  Issue,  October
17, 1977) explain this phenomenon.

Co-precipitation   With   Iron.    The  presence,  of  substantial
quantities   of   iron  in  metal-bearing   wastewaters    before
treatment  has   been   shown to improve  the  removal  of  -toxic
metals.   In  some  cases this iron is an integral  part  of  the
industrial  wastewater;  in other cases  iron   is   deliberately
added   as   a   preliminary  treatment   or   first   step    of
treatment.  The iron functions to improve  toxic and other metals
(such as molybdenum)  removal  by three  mechanisms:   the   iron
co-precipitates with toxic metals forming  a  stable  precipitate
which   desolubilizes    the     toxic  metal;      the      iron
improves    the  settleability  of   the precipitate;    and   the
large    amount    of   iron  reduces   the fraction   of   toxic
metal  in  the precipitate.   Co-precipitation with    iron   has
been  practiced  for  many  years  incidentally when   iron ,.  was
a-  substantial  constituent of raw - wastewater and  intentionally
when  iron  salts  were  added  as  a  coagulant aid.     Aluminum
or mixed iron-aluminum salt also have been used.

Co-precipitation using large amounts of  ferrous  iron  salts  is
known  as ferrite co-precipitation because magnetic iron oxide or
ferrite is formed.  The addition of ferrous  salts  (sulfate)   is
followed   by   alkali  precipitation  and  air  oxidation.   The
resultant precipitate is easily removed by filtration  and may  be
removed  magnetically.   Data  illustrating  the  performance  of
ferrite co-precipitation is,shown in. Table VII-7, (page 239).

Removal of PAH                   ,   ,

EPA  and  its contractor conducted, a series of bench-  and  pilot-
scale  tests examining the effectiveness of removing  polynuclear
aromatic  hydrocarbons  (PAH)  from  primary  aluminum   smelting
                               154

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
potline wet air pollution control wastewater.   In the study, the
effectiveness of  lime  and  settle,  multimedia  filtration  and
activated carbon adsorption was examined.  The study demonstrated
that  PAH  commonly  found in potline wet air  pollution  control
wastewater  can be removed by lime and  settle  technology.   PAH
present   in   the   untreated   potline   scrubber   liquor   at
concentrations  ranging from 0.030 to 2.740 mg/1 were reduced  to
less  than  0.170  mg/1 (ND to 0.170 mg/1)  by  lime  and  settle
treatment.

Advantages and Limitations.  Chemical precipitation has proved to
be an effective  technique  for  removing  many  pollutants  from
industrial  wastewater.  It operates at ambient conditions and is
well  suited  to  automatic  control.   The   use   of   chemical
precipitation may be limited because of interference by chelating
agents,  because  of  possible  chemical  interference with mixed
wastewaters  and  treatment  chemicals,   or   because   of   the
potentially  hazardous  situation  involved  with the storage and
handling     of     those     chemicals.      Nonferrous   metals
manufacturing  wastewaters  do  not  normally  contain  chelating
agents    or  complex  pollutant matrix  formations  which  would
interfere with  or  limit the   use   of  chemical precipitation.
One  exception   to  this statement  is wastewaters generated  by
secondary precious  metals facilities.    These  wastewaters  are
expected  to  contain  metal complexes  which  may  require  lime
or sulfide addition  to  help overcome complexing effects.

Lime  is  usually  added  as a  slurry  when  used  in  hydroxide
precipitation.   The  slurry must  be kept  well  mixed  and  the
addition   lines  periodically checked to prevent blocking  which
may   result   from  a  build-up  of    solids.     Also,    lime
precipitation   usually  makes  recovery   of   the  precipitated
metals   difficult,   because  of  the  heterogeneous  nature  of
most lime sludges.

The major advantage of the sulfide precipitation process is  that
the extremely low solubility of most metal sulfides promotes very
high metal removal efficiencies; the sulfide process also has the
ability  to  remove chromates and dichromates without preliminary
reduction of the chromium to its trivalent state.   In  addition,
sulfide  can  precipitate  metals  complexed with most complexing
agents.  The process demands care, however, in maintaining the pH
of  the  solution at approximately 10 in order  to  restrict  the
generation   of   toxic   hydrogen   sulfide   gas.    For   this
reason,  ventilation  of the treatment tanks may be  a  necessary
precaution in most installations.  The use of insoluble  sulfides
reduces the problem  of  hydrogen  sulfide  evolution.   As  with
hydroxide precipitation,  excess  sulfide  ion must be present to
drive  the  precipitation reaction to  completion.    Since   the
sulfide  ion itself is toxic, sulfide addition must be  carefully
controlled  to  maximize  heavy  metals  precipitation   with   a
minimum  of  excess  sulfide   to   avoid   the   necessity    of
additional    wastewater  treatment.    At   very   high   excess
sulfide   levels and high pH, soluble  mercury-sulfide  compounds
may   also   be  formed.   Where excess   sulfide   is   present,
                               155

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           GENERAL DEVELOPMENT DOCUMENT
               SECT - VII
aeration  of  the effluent stream can aid in  oxidizing  residual
sulfide  to  the  less  harmful  sodium sulfate    (N32S04).   The
cost  of sulfide precipitants is high in comparison to  hydroxide
precipitants,  and  disposal   of metallic  sulfide  sludges  may
pose   problems.    An  essential element  in  effective  sulfide
precipitation  is the   removal   of precipitated   solids   from
the  wastewater  and  proper disposal  in  an  appropriate  site.
Sulfide  precipitation will also generate a higher    volume   of
sludge   than   hydroxide   precipitation, resulting   in  higher
disposal  and dewatering costs.    This   is  especially     true
when  ferrous  sulfide  is  used   as   the precipitant.

Sulfide  precipitation may be used as a polishing  treatment after
hydroxide    precipitation-sedimentation.      This     treatment
configuration  may  provide the better treatment effectiveness of
sulfide precipitation while minimizing the variability caused  by
changes   in  raw  waste  and  reducing  the  amount  of  sulfide
precipitant required.
Operational    Factors.
Reliability:
Alkaline
chemical
precipitation  is highly reliable, although proper monitoring and
control are  required.   Sulfide  precipitation  systems  provide
similar reliability.

Maintainability:   The  major  maintenance needs involve periodic
upkeep of  monitoring  equipment,  automatic  feeding  equipment,
mixing  equipment,  and  other  hardware.  Removal of accumulated
sludge is necessary for  efficient  operation  of  precipitation-
sedimentation systems.

Solid Waste Aspects:  Solids which precipitate out are removed in
a  subsequent  treatment  step.  Ultimately, these solids require
proper disposal.

Demonstration Status.  Chemical precipitation of metal hydroxides
is a classic waste treatment technology used by  most  industrial
waste treatment systems.  Chemical precipitation of metals in the
carbonate  form  alone  has  been  found  to  be  feasible and is
commercially used to permit  metals  recovery  and  water  reuse.
Pull-scale    commercial  sulfide  precipitation  units  are   in
operation at numerous installations, including several plants  in
the  nonferrous metals manufacturing category.  As noted earlier,
sedimentation to remove precipitates is discussed separately.

Use  in  Nonferrous  Metals  Manufacturing   Plants:    Hydroxide
chemical   precipitation   is   used  at  121  nonferrous  metals
manufacturing plants.  Sulfide  precipitation  is  used  in  four
nonferrous metals manufacturing plants.

3. Cyanide Precipitation

Cyanide  precipitation, although a method for treating cyanide in
wastewaters, does not destroy cyanide.   The cyanide  is  retained
in  the' sludge  that  is  formed.   Reports indicate that during
exposure to sunlight, the cyanide complexes can  break  down  and
                               156

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           GENERAL DEVELOPMENT DOCUMENT
                   SECT - VII
form  free  cyanide.   For  this  reason,  the
treatment method must be disposed of carefully,
                        sludge  from this
Cyanide may be precipitated and settled out of wastewaters by the
addition of zinc sulfate or ferrous sulfate.  In the presence  of
iron,  cyanide will form extremely stable cyanide complexes.  The
addition  of  zinc  sulfate  or  ferrous   sulfate   forms   zinc
ferrocyanide or ferro ferricyanide complexes.

Cyanide  precipitation occurs in two steps: reaction with ferrous
sulfate or zinc sulfate at an alkaline pH to form  iron  or  zinc
cyanide   complexes  followed  by  reaction  at  a  low  pH  with
additional  ferrous  sulfate  to  form  insoluble  iron   cyanide
precipitates.  Cyanide precipitation is applicable to all cyanide
containing wastewater and,  unlike many  oxidation  technologies,
is  not  limited  by  the  presence  of  complexed cyanides.  The
oxidation  technologies  discussed  later  in  this section   are
applicable   for   waste  streams  containing   only  uncomplexed
cyanides.    Cyanide  precipitation  has  been  selected  as  the
technology basis for cyanide control because of the  presence  of
iron,  nickel,  and zinc in wastewaters in this category.   These
toxic metals are known to form stable complexes with cyanide.

Cyanide-containing wastewater is introduced into a mixing chamber
where  ferrous  sulfate (as the heptahydrate  (FeSO4*7(H2O)),  is
added     to    form    a    hexacyanoferrate     complex.    The
hexacyanoferrate   complex   is most stable at  a   pH    of    9
(standard   units).     Thus,    the   complexation  reaction  is
performed  at  pH  9.  The amount or dosage  of  ferrous  sulfate
is  dependent   upon   the  chemical  form  of  the  cyanide   in
the  wastewater.    Cyanide  may  be present in   one   of    two
forms,  free  or  complexed  (sometimes referred  to  as  fixed).
Various  analytical   methods  to  determine  the   portions   of
free   and complexed  cyanides  in  wastewater  are discussed  in
the  open  literature.   Free cyanide refers to  the  portion  of
total cyanide that freely dissociates in water  (e.g.,  HCN).

When  ferrous  sulfate is added to the wastewater at  pH  9,  the
ferrous ion readily oxidizes to the ferric ion.  The complexation
step is then expected to occur as follows:
     FeSO4 +

To  a  lesser
according to:

     FeSO4  +
6CN~	>

  degree,


 6CN~	:
                            Fe(CN)6
                                   3-
                S04'
the free cyanide may


            .4-
+ e

also
                                                    be  complexed
     Fe(CN)g
                                         SO4'
Complexed   cyanide,   present   as   the   hexacyanoferrate   or
metallocyanide complexes, is  already  in  the  desired  chemical
form.   In  theory,  the  ferrous sulfate dosage is determined by
calculating the stoichiometric equivalent required for  the  free
cyanide  present,  that  is,  one mole of ferrous sulfate per six
moles of cyanide.  In actual practice,  the  dosage  requirements
are  greater  than  the  stoichiometric  equivalent.   One reason
                               157

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            GENERAL DEVELOPMENT DOCUMENT
                                       SECT  -  VII
 form  free  cyanide.    For   this  reason,   the  sludge
 treatment method must  be disposed of carefully.
                                                    from this
 Cyanide may be precipitated and settled out of wastewaters by the
 addition of zinc  sulfate or ferrous  sulfate.   In the presence  of
 iron,   cyanide will  form extremely stable  cyanide complexes.   The
 addition  of  zinc   sulfate .or  ferrous   sulfate   forms   zinc
 ferrocyanide or ferro  ferricyanide complexes.

 Cyanide  precipitation occurs  in two steps:  reaction with ferrous'
 sulfate or zinc sulfate at  an  alkaline  pH  to  form  iron  or  zinc
 cyanide   complexes  followed   by reaction  at  a  low  pH  with
 additional  ferrous  sulfate  to  form   insoluble  iron   cyanide
 precipitates.   Cyanide precipitation is applicable to all cyanide
 containing^wastewater  and,   unlike many oxidation  technologies,
 is^  not  limited  by  the  presence  "of complexed cyanides.   The
 oxidation  technologies  discussed  later   in   this section   are
 applicable   for   waste streams containing    only  uncomplexed
 cyanides.     Cyanide  precipitation  has  been  selected   as   the
 technology basis  for cyanide control because of the  presence  of
 iron,   nickel,  and  zinc in wastewaters in this category.   These
 toxic metals are  known to form stable complexes with cyanide.

 Cyanide-containing   wastewater   is  introduced  into  a    mixing
 chamber where  ferrous  sulfate   (as  the heptahydrate  (FeS04.
 7H20)),    is   added  to form  a hexacyanoferrate  complex.  The
 hexacyanoferrate   complex   is  most stable at   a   pH    of     9
 (standard    units).      Thus,     the   complexation  reaction  is
 performed   at   pH 9.   The  amount or dosage  of  ferrous   sulfate
 is   dependent   upon   the   chemical form of   the  cyanide    in
 the  wastewater.     Cyanide    may be present  in  one  of     two
 forms,   free   or  complexed  (sometimes referred  to  as  fixed).
 Various  analytical    methods   to determine   the   portions    of
 free    and  complexed  cyanides   in  wastewater   are discussed   in
 the  open   literature.    Free  cyanide  refers  to the   portion   of
 total cyanide  that freely dissociates in water   (e.g.,  HCN) .

 When  ferrous   sulfate  is added  to the  wastewater  at   pH   9,   the
 ferrous  ion  readily  oxidizes to  the  ferric ion.   The  complexation
 step is  then expected  to occur as  follows:
FeSO4
             6CN  ----
Fe(CN)6
                                   3-
S04"
                                              + c
To  a  lesser  degree,  the free cyanide may  also  be  complexed
according to:

                                    .4-
     FeSC-4  + 6CN" ---- >
 Fe(CN)6
                                    S04
Complexed   cyanide,   present   as   the   hexacyanoferrate   or
metallocyanide complexes, is  already  in  the  desired  chemical
form.   In  theory,  the  ferrous sulfate dosage is determined by
calculating the stoichiometric equivalent required for  the  free
cyanide  present,  that  is,  one mole of ferrous sulfate per six
moles of cyanide.  In actual practice,  the  dosage  requirements
are  greater  than  the  stoichiometric  equivalent.   One reason
                               157

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
that  excess   ferrous   sulfate  is   required   is   that   the
complexation  reaction  is  very slow and the excess of reactants
increases the reaction rate.  Another reason is that in treatment
systems, where lime or other sources of hydroxide ions are  added
to  raise  the  pH  to  8,  some  of the lime will react with the
ferrous sulfate to form calcium sulfate.

After forming the complex, the  wastewater  is  then  mixed  with
additional  ferrous  sulfate  and the  pH  adjusted  using   acid
(e.g.,  H2S04)  in  the range of 2 to 4.   The ferrous    sulfate
reacts with the hexacyanoferrate  to  form ferrohexacyanoferrate,
according to:
     3FeS04 + 2Pe(CN)6
              Fe(CN)5
Fe3(Fe(CN)6)2

Fe2(Fe(CN)6)
        3SO4'
It appears that it may also be possible to use ferric chloride in
the precipitation step, according to:

     4FeC13 + 3Fe(CN6)4	>  Fe4(Fe(CN)6)3 + 12C1"

However,  based  on data obtained from cyanide-bearing waters  in
the  primary aluminum industry,  ferric chloride did not increase
the  amount  of  cyanide  precipitate  formed.    In  wastewaters
obtained  from two different facilities,  the dosage  of  ferrous
sulfate was held constant while the dosage of ferric chloride was
varied.   Results  from both plants indicate that the addition of
ferric chloride has little,  if any,  effect on the precipitation
chemistry.

Following  complexation  the  wastewater  is  introduced  into  a
clarifier  to  allow  these  insoluble  precipitates  to  settle.
Sedimentation  (settling)  is discussed in a later subsection.

Adequate  complexation  of  cyanide  requires that the pH must be
kept at 9.0 and an appropriate retention  time be  maintained.   A
study  has  shown  that  the  formation   of  the  complex is very
dependent on pH.  At a pH of either 8 or  10, the residual cyanide
concentrations measured are  twice  that  of  the  same  reaction
carried  out  at  a  pH  of  9.  Removal  efficiencies also depend
heavily on the retention time  allowed.   The  formation  of  the
complexes  takes  place rather slowly.  Depending upon the excess
amount of zinc sulfate or ferrous sulfate added, at  least  a  30
minute  retention time should be allowed  for the formation of the
cyanide  complex before continuing on to  the clarification stage.

One experiment with  an  initial  concentration  of  10  mg/1  of
cyanide  showed  that 98 percent of the cyanide was complexed ten
minutes after the  addition  of  ferrous  sulfate  at  twice  the
theoretical  amount  necessary.   Interference  from  other metal
ions, such as cadmium,  might  result   in the  need  for  longer
retention times.
                                158
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           GENERAL DEVELOPMENT  DOCUMENT
                                           SECT - VII
 Table  VII-8   (page  239) presents  cyanide precipitation data  from
 three  coil  coating plants.  A  fourth plant was  visited   for   the
 purpose   of  observing plant testing of  the cyanide precipitation
 system.   Specific    data   from   this   facility   are      not
 included  because:   (1)   the pH was usually well below the optimum
 level  of  9.0;   (2)  the  historical  treatment  data  were    not
.obtained    using  the standard  cyanide  analysis  procedure;   and
 (3)  matched   input-output data  were not made  available  by   the
 plant.    Scanning    the available data  indicates that  the   raw
 waste  CN  level was  in the range  of 25.0;  the pH 7.5; and treated
 CN  level  was  from  0.1   to 0.2.

 The  concentrations   are those of  the  stream entering and leaving
 the  treatment system.  Plant 1057  allowed a  27-minute  retention
 time  for  the formation of the complex.  The retention  time for
 the  other plants  is  not  known.   The data suggest that over a  wide
 range  of  cyanide   concentration   in  the   raw   waste,    the
 concentration of  cyanide can be  reduced  in the effluent stream to
 under  0.15  mg/1.

 Application  and  Performance.   Cyanide  precipitation can be  used
 when cyanide  destruction is not  feasible because of the   presence
 of   cyanide  complexes   which  are  difficult to destroy.   Effluent
 concentrations of cyanide well below 0.15 mg/1 are possible.
 Advantages   and
 inexpensive
                 Limitations.    Cyanide
precipitation   is   an
Problems may occur when
             method of treating cyanide.
metal ions interfere with the formation of the complexes.

4. Granular Bed Filtration

Filtration occurs in nature as  surface  and ground  waters   are
cleansed  by  sand.  Silica sand, anthracite coal, and garnet are
common filter media used in water treatment  plants.   These  are
usually  supported by gravel.  The media may be used singly or in
combination.  The multi-media filters may be arranged to maintain
relatively distinct layers by virtue of balancing the  forces  of
gravity, flow, and buoyancy, on the individual particles.  This is
accomplished  by selecting appropriate filter flow rates (gpm/sq-
ft), media grain size, and density.

Granular bed filters may be classified  in  terms  of  filtration
rate,  filter  media,  flow pattern, or method of pressurization.
Traditional rate classifications are slow sand, rapid  sand,  and
high  rate  mixed  media.   In  the  slow  sand  filter,  flux or
hydraulic loading is relatively low,  and  removal  of  collected
solids  to  clean  the filter is therefore relatively infrequent.
The filter is often cleaned by scraping off the inlet face  (top)
of  the  sand  bed.   In  the  higher  rate  filters, cleaning is
frequent and is accomplished by a periodic backwash, opposite  to
the direction of normal flow.

A  filter  may  use  a single medium such as sand or diatomaceous
earth, but dual and mixed (multiple) media filters  allow  higher
flow  rates  and  efficiencies.   The  dual  media filter usually
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
consists of a fine bed of  sand under a coarser bed of  anthracite
coal.  The coarse coal removes most of the  influent solids, while
the  fine  sand performs a polishing function.  At the end of the
backwash, the fine sand settles  to  the  bottom  because  it  is
denser  than  the  coal,   and  the  filter  is  ready  for normal
operation.   The  mixed  media  filter  operates  on   the   same
principle,  with  the  finer,  denser media at the bottom and the
coarser, less dense media  at the top.  The  usual  arrangement  is
garnet at the bottom  (outlet end) of the bed, sand in the middle,
and  anthracite  coal  at  the  top.  Some  mixing of these layers
occurs and is, in fact, desirable.

The flow pattern is usually top-to-bottom,  but other patterns are
sometimes used.  Upflow filters are  sometimes  used,  and  in  a
horizontal  filter  the  flow is horizontal.  In a biflow filter,
the influent enters  both  the  top  and  the  bottom  and  exits
laterally.   The  advantage  of  an upflow  filter is that with an
upflow backwash, the particles of  a  single  filter  medium  are
distributed and maintained in the desired coarse-to-fine (bottom-
to-top)  arrangement.   The disadvantage is that the bed tends to
become fluidized, which ruins filtration efficiency.  The  biflow
design is an attempt to overcome this problem.

The  classic  granular  bed  filter  operates  by  gravity  flow;
however, pressure filters  are fairly widely  used.   They  permit
higher  solids loadings before cleaning and are advantageous when
the filter effluent must be pressurized  for  further  downstream
treatment.   In  addition, pressure filter  systems are often less
costly for low to moderate flow rates.

Figure VII-14 (page 267) depicts a high rate, dual media, gravity
downflow granular bed filter, with  self-stored  backwash.    Both
filtrate  and backwash are piped around the bed in an arrangement
that permits gravity upflow of  the  backwash,  with  the  stored
filtrate   serving   as  backwash.   Addition  of  the  indicated
coagulant and polyelectrolyte usually results  in  a  substantial
improvement in filter performance.

Auxiliary filter cleaning  is sometimes employed in the upper  few
inches  of  filter  beds.   This is conventionally referred to as
surface wash and is accomplished by water  jets  just  below  the
surface  of  the  expanded bed during the backwash cycle.   These
jets enhance the scouring  action in the  bed  by  increasing  the
agitation.

An important feature for successful filtration and backwashing is
the  underdrain.  This is  the support structure for the bed.  The
underdrain provides an area for collection of the filtered  water
without  clogging  from  either  the filtered solids or the media
grains.  In addition, the  underdrain prevents loss of  the  media
with  the  water,  and during the backwash cycle it provides even
flow  distribution  over   the  bed.   Failure  to  dissipate  the
velocity  head during the  filter or backwash cycle will result in
bed upset and the need for major repairs.
                               160

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Several standard approaches are employed for filter  underdrains.
The  simplest  one  consists  of  a parallel porous pipe embedded
under a layer of coarse gravel and manifolded to  a  header  pipe
for  effluent removal.  Other approaches to the underdrain system
are known as the Leopold and Wheeler  filter  bottoms.   Both  of
these  incorporate  false concrete bottoms with specific porosity
configurations to provide drainage and velocity head dissipation.

Filter system operation may be manual or automatic.   The  filter
backwash  cycle  may  be  on a timed basis, a pressure drop basis
with a terminal value which triggers backwash, or a solids carry-
over basis from turbidity monitoring of the outlet  stream.   All
of these schemes have been used successfully.

Application  and  Performance.  Wastewater treatment plants often
use granular  bed  filters  for  polishing  after  clarification,
sedimentation,   or   other  similar  operations.   Granular  bed
filtration  thus  has  potential  application   to   nearly   all
industrial plants.  Chemical additives which enhance the upstream
treatment  equipment may or may not be compatible with or enhance
the filtration process.  Normal operating flow rates for  various
types of filters are:
 Slow Sand      2.04 - 5.30 1/sq m-hr
 Rapid Sand    40.74 - 51.48 1/sq m-hr
 High Rate Mixed Media  81.48 - 122.22 1/sq m-hr
Suspended  solids are commonly removed from wastewater streams by
filtering through a deep 0.3-0.9 m  (1-3  feet)  granular  filter
bed.  The porous bed formed by the granular media can be designed
to  remove  practically  all suspended particles.  Even colloidal
suspensions (roughly 1  to  100  microns)  are  adsorbed  on  the
surface  of  the  media grains as they pass in close proximity in
the narrow bed passages.

Properly operated filters ^following some pretreatment  to  reduce
suspended  solids  below  200 mg/1 should produce water with less
than 10 mg/1 TSS.  For example, multimedia filters  produced  the
effluent qualities shown in Table VII-9 (page 240).

The  addition of multimedia filtration to lime precipitation  and
sedimentation resulted in further reduction of the PAH; all  less
than  0.110 mg/1.  Benzo(a)pyrene  was reduced to the  analytical
quantification  limit  of  0.010 mg/1.  The  study  conducted  on
potline scrubber liquor is discussed more fully in Section VII of
the  primary  aluminum  subcategory supplement and  in  a  report
entitled  Physical-Chemical Treatment of Aluminum  Plant  Potline
Scrubber Wastewater, found in the record supporting this rule.

Advantages and Limitations.  The principal advantages of granular
bed  filtration  are  its  comparatively  (to  other filters) low
initial and operating costs, reduced land requirements over other
methods  to  achieve  the  same  level  of  solids  removal,  and
                               161

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           GENERAL DEVELOPMENT DOCUMENT     SECT - VII


 elimination  of  chemical  additions  to   the  discharge   stream.
 However,  the filter may  require pretreatment if the solids   level
 is high  (over   100  mg/1).    Operator training must be   somewhat
 extensive due to the controls and periodic  backwashing  involved,
 and   backwash  must  be   stored  and  dewatered  for  economical
 disposal.

 Operational Factors.  Reliability:  The  recent  improvements  in
 filter    technology   have   significantly   improved  filtration
 reliability.   Control   systems,  improved  designs,   and   good
 operating procedures  have  made  filtration  a  highly reliable
 method of water treatment.

 Maintainability:  Deep bed filters may be   operated  with  either
 manual  or  automatic  backwash.   In  either  case, they must be
 periodically inspected for media attrition, partial plugging, and
 leakage.  Where backwashing is not used, collected solids must be
 removed by shoveling, and  filter media must be at least partially
 replaced.

 Solid Waste  Aspects:   Filter  backwash  is  generally  recycled
 within  the  wastewater  treatment  system,  so  that  the solids
 ultimately appear in the clarifier sludge stream  for  subsequent
 dewatering.   Alternatively, the backwash stream may be dewatered
 directly  or, if there is no backwash, the collected solids may be
 disposed  of  in  a  suitable  landfill.    In  either  of    these
 situations  there is a solids disposal problem similar to that of
 clarifiers.

 Demonstration Status.  Deep bed filters  are  in  common  use  in
 municipal  treatment  plants.   Their use in polishing industrial
 clarifier effluent is increasing, and the   technology  is  proven
 and   conventional.   Granular  bed  filtration  is  used  in  25
 nonferrous metals manufacturing  plants.   As  noted  previously,
 however,    little   data   is   available   characterizing   the
 effectiveness of filters presently in use within the industry.

 5. Pressure Filtration

 Pressure  filtration works by pumping the liquid through a  filter
material  which is impenetrable to the solid phase.   The positive
pressure  exerted by the feed  pumps  or  other  mechanical  means
provides  the pressure differential which is the principal driving
 force.   Figure VII-15 (page 268) represents the operation of one
 type of pressure filter.

A typical pressure filtration unit consists of a number of plates
or trays which are held rigidly in a frame  to  ensure  alignment
and  which  are  pressed  together  between  a  fixed  end  and a
 traveling end.   On the surface of each plate,  a  filter  made  of
cloth  or  synthetic fiber is mounted.  The feed stream is pumped
into the unit and passes through holes in  the  trays  along  the
length  of  the  press until the cavities or chambers between the
trays are completely filled.   The solids are then entrapped,  and
a cake begins to form on the surface of the filter material.  The


                               162

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 water  passes  through the  fibers,  and the  solids  are  retained.

 At   the  bottom of  the  trays  are  drainage ports.   The  filtrate  is
 collected and discharged  to a common drain.  As  the  filter medium
 becomes coated with sludge, the   flow  of  filtrate  through  the
 filter  drops sharply,  indicating that  the capacity  of the filter
 has  been exhausted.   The  unit must then be cleaned of  the sludge.
 After  the cleaning  or replacement of the  filter  media,   the  unit
 is again ready for  operation.

 Application   and Performance.    Pressure  filtration   is used  in
 nonferrous metals manufacturing for  sludge dewatering  and  also
 for  direct   removal of  precipitated  and other  suspended solids
 from wastewater.  Because dewatering is such a   common  operation
 in   treatment  systems,   pressure filtration is  a technique which
 can  be found  in many industries concerned  with   removing  solids
 from their waste stream.

 In   a   typical  pressure  filter,  chemically preconditioned sludge
 detained in the unit for  one  to  three   hours   under   pressures
 varying  from  5 to  13  atmospheres exhibited final solids content
 between 25 and 50 percent.

 Advantages and Limitations.   The  pressures which  may   be  applied
 to   a   sludge  for   removal   of   water  by filter  presses that are
 currently available  range from 5  to  13  atmospheres.  As  a result,
 pressure  filtration may  reduce   the   amount   of   chemical
 pretreatment   required  for sludge dewatering.  Sludge  retained  in
 the  form of the filter  cake has a higher  percentage  of  solids
 than  that from centrifuge  or   vacuum  filter.  Thus,  it can  be
 easily accommodated  by  materials  handling  systems.

 As   a   primary  solids  removal   technique,  pressure  filtration
 requires   less   space   than  clarification  and is well  suited  to
 streams  with  high solids  loadings.   The sludge  produced  may   be
 disposed   without further dewatering, but  the amount of  sludge  is
 increased  by  the   use   of  filter  precoat  materials  (usually
 diatomaceous   earth). .  Also,  cloth  pressure filters often do not
 achieve  as high  a degree  of effluent clarification as  clarifiers
 or granular media filters.

 Two  disadvantages associated with pressure filtration in the past
 have   been  the  short  life  of   the  filter  cloths and lack of
 automation.   New synthetic fibers have largely offset  the  first
 of   these  problems.   Also,  units  with  automatic  feeding and
 pressing cycles are  now available.

 For  larger operations, the relatively high space requirements,  as
 compared to those of a centrifuge, could be prohibitive  in  some
 situations.

Operational "Factors.   Reliability:   With  proper pretreatment,
design, and control, pressure  filtration is a  highly  dependable
 system.
                               163

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Maintainability:   Maintenance  consists  of periodic cleaning or
replacement of the filter media, drainage grids, drainage piping,
filter pans, and other parts of the system.  If  the  removal  of
the sludge cake is not automated, additional time is required for
this operation.

Solid  Waste  Aspects:   Because it is generally drier than other
types of sludges, the filter sludge  cake  can  be  handled  with
relative  ease.  The accumulated sludge may be disposed by any of
the accepted procedures depending on  its  chemical  composition.

Demonstration Status.  Pressure filtration  is  a  commonly  used
technology in a great many commercial applications.

6. Settling

Settling is a process which removes solid particles from a liquid
matrix  by  gravitational  force.   This  is done by reducing the
velocity of the feed stream in a large volume tank or  lagoon  so
that  gravitational settling can occur.  Figure VII-16 (page 269)
shows two typical settling devices.

Settling  is  often  preceded  by  chemical  precipitation  which
converts  dissolved  pollutants  to solid form and by coagulation
which enhances settling  by  coagulating  suspended  precipitates
into larger/ faster settling particles.

If no chemical pretreatment is used, the wastewater is fed into a
tank  or  lagoon where it loses velocity and the suspended solids
are allowed to settle out.  Long retention  times  are  generally
required.    Accumulated   sludge   can   be   collected   either
periodically or continuously,and either manually or mechanically.
Simple  settling,  however,   may   require   excessively   large
catchments,  and  long  retention  times   (days  as compared with
hours)  to achieve high removal efficiencies.   Because  of  this,
addition  of  settling aids such as alum or polymeric flocculants
is often economically attractive.

In practice, chemical precipitation often precedes settling,  and
inorganic  coagulants or "polyelectroly'tic  flocculants are usually
added as well.  Common coagulants  include  sodium sulfate,  sodium
aluminate,  ferrous  or  ferric  sulfate,  and  ferric  chloride.
Organic polyelectrolytes vary in structure, but all usually  form
larger  floe particles than coagulants used alone.

Following  this  pretreatment,   the  wastewater can be fed into  a
holding tank or lagoon for settling, but is more often piped into
a clarifier for the same  purpose.   A  clarifier  reduces  space
requirements,   reduces  retention time,  and  increases  solids
removal efficiency.  Conventional  clarifiers generally consist of
a circular  or  rectangular  tank with   a   mechanical   sludge
collecting device or with a sloping funnel-shaped  bottom designed
for   sludge  collection.   In advanced  settling devices, inclined
plates, slanted tubes, or a  lamellar   network  may  be  included
within  the  clarifier   tank  in   order to increase the effective
                                164

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
settling area, increasing capacity.  A  fraction  of  the  sludge
stream is often recirculated to the inlet, promoting formation of
a denser sludge.

Settling  is  based  on  the ability of gravity (Newton's Law) to
cause small particles to fall or settle (Stokes1 Law) through the
fluid  they  are  suspended  in.   Presuming  that  the   factors
affecting  chemical  precipitation  are  controlled  to achieve a
readily settleable precipitate, the principal factors controlling
settling are the particle characteristics and the upflow rate  of
the  suspending fluid.  When the effective settling area is great
enough to allow settling, any increase in the effective  settling
area will produce no increase in solids removal.

Therefore,  if  a plant has installed equipment that provides the
appropriate overflow rate,  the  precipitated  solids  (including
toxic  metals)  in  the effluent can be effectively removed.  The
number of settling devices operated in series or in parallel by a
facility  is  not  important  with  regard  to  suspended  solids
removal.   Rather,  it  is  important  that  the settling devices
provide sufficient effective settling area.

Another  important  facet  of  sedimentation   theory   is   that
diminishing  removal  of  suspended solids is achieved for a unit
increase in the effective settling area.   Generally, it has  been
found  that  suspended solids removal performance varies with the
effective up-flow rate.  Qualitatively the performance  increases
asymptotically  to a maximum level beyond which a decrease in up-
flow  rate  provides  incrementally  insignificant  increases  in
removal.   This  maximum  level  is  dictated  by  particle  size
distribution, density characteristic of  the  particles  and  the
water  matrix,  chemicals  used for precipitation and pH at which
precipitation occurs.

Application and Performance.  Settling and clarification are used
in  the  nonferrous  metals  manufacturing  category  to   remove
precipitated  metals.   Settling  can  be  used  to  remove  most
suspended solids in a particular waste stream; thus  it  is  used
extensively   by   many   different  industrial  waste  treatment
facilities.   Because  most  metal  ion  pollutants  are  readily
converted  to  solid metal hydroxide precipitates, settling is of
particular  use  in  those  industries  associated   with   metal
production,   metal  finishing,  metal  working,  and  any  other
industry  with  high  concentrations  of   metal  ions  in   their
wastewaters.   In addition to toxic metals, suitably precipitated
materials effectively removed by settling include aluminum, iron,
manganese, cobalt,  antimony,  beryllium,  molybdenum,  fluoride,
phosphate, and many others.

A  properly  operating  settling  system  can  efficiently remove
suspended  solids,  precipitated  metal  hydroxides,  and   other
impurities  from  wastewater.   The  performance  of  the process
depends on a  variety  of  factors,  including  the  density  and
particle  size  of  the  solids,  the  effective  charge  on  the
suspended  particles,  and  the  types  of  chemicals   used   in
                               165

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
pretreatment.   The site of flocculant or coagulant addition also
may significantly influence the effectiveness  of  clarification.
If the flocculant is subjected to too much mixing before entering
the  clarifier,  the  complexes  may  be sheared and the settling
effectiveness diminished.  At the same time, the flocculant  must
have  sufficient  mixing and reaction time in order for effective
set-up and settling to occur.  Plant personnel have observed that
the line or trough leading into the clarifier is often  the  most
efficient  site  for  flocculant  addition.   The  performance of
simple  settling  is a function of the  movement  rate,  particle
size and density, and the surface area of the basin.

The  data displayed in Table VII-10 (page 240) indicate suspended
solids removal efficiencies in settling systems.

The mean effluent TSS concentration obtained by the plants  shown
in  Table  VII-10 is 10.1 mg/1.  Influent concentrations averaged
838 mg/1.  The maximum effluent TSS value reported  is  23  mg/1.
These  plants all use alkaline pH adjustment to precipitate metal
hydroxides, and most add  a  coagulant  or  flocculant  prior  to
settling.

Advantages  and  Limitations.   The  major  advantage  of  simple
settling is its simplicity as demonstrated by  the  gravitational
settling  of solid particulate waste in a holding tank or lagoon.
The major problem with simple settling is the long retention time
necessary  to  achieve  complete  settling,  especially  if   the
specific  gravity  of  the  suspended  matter is close to that of
water.  Some materials cannot be practically  removed  by  simple
settling alone.

Settling  performed in a clarifier is effective in removing slow-
settling suspended matter in a shorter time  and  in  less  space
than  a  simple settling system.  Also, effluent quality is often
better from a clarifier.  The cost of installing and  maintaining
a  clarifier,  however,  is  substantially greater than the costs
associated with simple settling.

Inclined plate, slant tube, and lamella settlers have even higher
removal efficiencies than conventional  clarifiers,  and  greater
capacities per unit area are possible.  Installed costs for these
advanced  clarification  systems  are  claimed to be one half the
cost of conventional systems of similar capacity.

Operational Factors.  Reliability:   Settling  can  be  a  highly
reliable  technology  for  removing suspended solids.  Sufficient
retention time and regular sludge removal are  important  factors
affecting  the  reliability  of  all  settling  systems.   Proper
control of pH adjustment, chemical precipitation,  and  coagulant
or  flocculant addition are additional factors affecting settling
efficiencies  in  systems  (frequently  clarifiers)  where  these
methods are used.

Those  advanced settlers using slanted tubes, inclined plates, or
a lamellar network may require  pre-screening  of  the .waste  in
                               166

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
order  to eliminate any fibrous materials which could potentially
clog the system.  Some installations are especially vulnerable to
shock loadings, as from storm water  runoff,  but  proper  system
design will prevent this.

Maintainability:   When  clarifiers  or  other  advanced settling
devices are used, the associated  system  utilized  for  chemical
pretreatment  and  sludge dragout must be maintained on a regular
basis.   Routine  maintenance  of  mechanical   parts   is   also
necessary.    Lagoons   require  little  maintenance  other  than
periodic sludge removal.

Demonstration Status.  Settling represents the typical method  of
solids  removal  and  is employed extensively in industrial waste
treatment.  The advanced clarifiers are just beginning to  appear
in significant numbers in commercial applications.

7. Skimming

Pollutants  with  a  specific  gravity less than water will often
float unassisted to the  surface  of  the  wastewater.   Skimming
removes  these floating wastes.  Skimming normally takes place in
a tank designed to allow the floating debris to rise  and  remain
on the surface, while the liquid flows to an outlet located below
the floating layer.  Skimming devices are therefore suited to the
removal  of  non-emulsified  oils from raw waste streams.  Common
skimming mechanisms include the rotating drum type,  which  picks
up  oil  from  the  surface of the water as it rotates.  A doctor
blade scrapes oil from the drum and collects it in a  trough  for
disposal  or  reuse.   The water portion is allowed to flow under
the  rotating  drum.   Occasionally,  an  underflow   baffle   is
installed after the drum; this has the advantage of retaining any
floating  oil  which  escapes  the  drum  skimmer.  The belt type
skimmer is pulled vertically through the  water,  collecting  oil
which  is  scraped  off from the surface and collected in a drum.
Gravity separators, such as the API type,  utilize  overflow  and
underflow  baffles  to skim a floating oil layer from-the surface
of the wastewater.  An overflow-underflow baffle allows  a  small
amount of wastewater (the oil portion) to flow over into a trough
•for  disposition  or  reuse while the majority of the water flows
underneath the baffle.  This is followed by an  overflow  baffle,
which  is  set at a height relative to the first baffle such that
only the oil bearing portion will  flow  over  the  first  baffle
during  normal  plant  operation.   A diffusion device, such as  a
vertical slot baffle, aids in creating a uniform flow through the
system and in increasing oil removal efficiency.

Application and Performance.  Oil skimming is used in  nonferrous
metals  manufacturing  to  remove  free  oil  and  grease used as
lubricants in some types of metal casting.  Another source of oil
is lubricants for drive mechanisms and other machinery  contacted
by  process  water.   Skimming  is applicable to any waste stream
containing pollutants which float to the surface.  It is commonly
used to remove free oil, grease, and soaps.   Skimming  is  often
used  in conjunction with air flotation or clarification in order
                                167

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           GENERAL  DEVELOPMENT  DOCUMENT
SECT - VII
 to  increase  its  effectiveness.

 The removal  efficiency  of  a  skimmer  is partly a  function  of   the
 retention  time  of   the water  in  the tank.  Larger, more buoyant
 particles require  less  retention   time   than  smaller  particles.
 Thus, the efficiency  also  depends  on the composition of the waste
 stream.   The  retention   time  required  to allow phase separation
 and subsequent skimming varies  from  1 to 15 minutes, depending on
 the wastewater characteristics.

 API or other gravity-type  separators tend to be  more suitable  for
 use where the amount  of surface oil  flowing through the system is
 consistently  significant.   Drum  and   belt  type  skimmers  are
 applicable   to   waste  streams  which evidence smaller amounts of
 floating oil and where  surges of floating oil are not a  problem.
 Using  an  API   separator  system  in conjunction with a drum type
 skimmer would be a very effective  method of  removing  floating
 contaminants  from  non-emulsified  oily waste streams.  Sampling
 data shown in Table VII-11 (page 241) illustrate the capabilities
 of  the technology with  both  extremely   high  and  moderate  oil
 influent levels.

 These data are intended to be illustrative of the very high level
 of   oil  and  grease  removals attainable in a simple two-step oil
 removal system.  Based  on  the performance of installations  in  a
 variety  of manufacturing plants and permit requirements that are
 consistently achieved,  it  is determined  that effluent oil  levels
 may be  reliably  reduced  below  10 mg/1 with  moderate influent
 concentrations.  Very high concentrations of oil such as  the  22
 percent  shown   above  may  require  two-step treatment to achieve
 this level.

 Skimming which removes -oil may also  be used to remove base levels
 of   organics.    Plant   sampling  data  show  that  many   organic
 compounds  tend  to   be  removed in  standard wastewater treatment
 equipment.  Oil  separation not only  removes oil  but also organics
 that are more  soluble  in  oil  than  in  water.   Clarification
 removes  organic  solids  directly and probably  removes dissolved
 organics by adsorption  on inorganic  solids.

 The  source of these organic pollutants is not always  known  with
 certainty,  although  in  metal  forming  operations they seem to
 derive mainly from various process   lubricants.    They  are  also
 sometimes  present  in  the  plant   water supply, as additives to
proprietary  formulations  of  cleaners,  or  as  the  result  of
 leaching from plastic lines and other materials.

High  molecular  weight  organics  in  particular  are  much more
 soluble in organic solvents than in  water.  Thus  they  are  much
more  concentrated  in  the oil phase that is skimmed than in the
wastewater.   The ratio of solubilities of a compound in  oil  and
water  phases is called the partition coefficient.   The logarithm
of  the partition coefficients for selected  polynuclear  aromatic
hydrocarbon  (PAH)   and  other toxic organic compounds in octanol
and water are shown in Table VII-12  (page 241).
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           GENERAL DEVELOPMENT DOCUMENT
                     SECT - VII
A review of priority organic compounds commonly  found  in  metal
forming operation waste streams indicated that incidental removal
of  these  compounds  often  occurs as a result of oil removal or
clarification processes.  When all organics analyses from visited
plants are considered, removal  of  organic  compounds  by  other
waste  treatment  technologies  appears  to  be  marginal in many
cases.   However, when only raw waste concentrations of 0.05 mg/1
or greater are considered, incidental  organics  removal  becomes
much  more  apparent.    Lower values, those less than 0.05 mg/1,
are much more  subject  to  analytical  variation,  while  higher
values indicate a significant presence of a given compound.  When
these factors are taken into account, analysis data indicate that
most  clarification  and  oil  removal  treatment  systems remove
significant amounts of the toxic organic compounds present in the
raw waste.  The API oil-water separation system performed notably
in this regard, as shown in Table VII-13 (page 242).

Data from five plant days demonstrate removal of organics by  the
combined  oil  skimming and settling operations performed on coil
coating wastewaters.  Days were  chosen  where  treatment  system
influent  and  effluent  analyses provided paired data points for
oil and grease and the organics present.  All organics  found  at
quantifiable  levels  on those days were included.  Further, only
those days were  chosen  where  oil  and  grease  raw  wastewater
concentrations  exceeded 10 mg/1 and where there was reduction in
oil and grease going through the  treatment  system.   All  plant
sampling  days  which  met the above criteria are included below.
The conclusion is that when oil and grease are removed,  organics
also are removed.
                                  Percent Removal
Plant-Day

 1054-3
13029-2
13029-3
38053-1
38053-2
Mean
Oil & Grease

  95.9
  98.3
  95.1
  96.8
  98.5
  96.9
Organics

  98.2
  78.0
  77.0
  81.3
  86.3
  84.2
The  unit  operation most applicable to removal of trace priority
organics  is  adsorption,  and  chemical  oxidation  is   another
possibility.   Biological degradation is not generally applicable
because the organics are not present in sufficient  concentration
to  sustain  a  biomass  and  because  most  of  the organics are
resistant to biodegradation.

Advantages  and  Limitations.    Skimming  as  a  pretreatment  is
effective in removing naturally floating waste material.  It also
improves  the  performance  of  subsequent downstream treatments.
Many pollutants, particularly dispersed or emulsified  oil,  will
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
not  float "naturally" but require additional treatments.  There-
fore/ skimming alone may not remove all the pollutants capable of
being removed  by  air  flotation  or  other  more  sophisticated
technologies.

Operational  Factors.   Reliability:   Because of its simplicity,
skimming is a very reliable technique.

Maintainability:   The  skimming  mechanism   requires   periodic
lubrication, adjustment, and replacement of worn parts.

Solid  Waste  Aspects:   The  collected  layer  of debris must be
disposed of by contractor  removal,  landfill,  or  incineration.
Because  relatively  large quantities of water are present in the
collected wastes, incineration is not always  a  viable  disposal
method.

Demonstration  Status.   Skimming  is a common operation utilized
extensively by industrial waste treatment systems.  Oil  skimming
is used in four nonferrous metals manufacturing plants.

MAJOR TECHNOLOGY EFFECTIVENESS

The   performance   of   individual  treatment  technologies  was
presented above.  Performance of operating systems  is  discussed
here.   Two  different  systems  are  considered:  L&S (hydroxide
precipitation and sedimentation or  lime  and  settle)  and  LS&F
(hydroxide  precipitation, sedimentation, and filtration or lime,
settle, and filter).  Subsequently, an analysis of  effectiveness
of  such  systems is made to develop one-day maximum, ten-day and
thirty-day   average   concentration  levels  to   be   used   in
regulating  pollutants.   Evaluation  of  the  L&S  and  the LS&F
systems is carried out on the assumption that chemical  reduction
of  chromium, cyanide precipitation and oil removal are installed
and operating properly where appropriate.

L&S Performance — Combined Metals Data Base

A data base known as the "combined metals data base"  (CMDB)  was
used  to  determine  treatment  effectiveness  of lime and settle
treatment for certain pollutants.  The CMDB  was  developed  over
several  years  and  has  been  used  in a number of regulations.
During the development of  coil  coating  and  other  categorical
effluent  limitations  and standards, chemical analysis data were
collected of raw  wastewater  (treatment  influent)  and  treated
wastewater  (treatment  effluent)  from 55 plants (126 data days)
sampled by  EPA  (or  its  contractor)  using  EPA  sampling  and
chemical  analysis  protocols. .  These  data are the initial data
base for determining  the  effectiveness  of  L&S  technology  in
treating nine pollutants.  Each of the plants in the initial data
base   belongs   to  at  least  one  of  the  following  industry
categories: aluminum forming, battery manufacturing, coil coating
(including  canmaking),  copper   forming,   electroplating   and
porcelain  enameling.  All of the plants employ pH adjustment and
hydroxide  precipitation  using  lime  or  caustic,  followed  by
                               170

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Stokes1  law  settling  (tank,  lagoon  or  clarifier) for solids
removal.   An  analysis  of  this  data  was  presented  in   the
development  documents  for  the  proposed  regulations  for coil
coating  and  porcelain  enameling  (January  1981).   Prior   to
analyzing  the data, some values were deleted from the data base.
These deletions  were  made  to  ensure  that  the  data  reflect
properly operated treatment systems.  The following criteria were
used in making these deletions:


     Plants   where malfunctioning processes or treatment systems
     at   the time of sampling were identified.


     Data days where pH was less than 7.0 for  extended   periods
     of    time  or  TSS  was  greater  than  50 mg/1 (these  are
     prima facie   indications of poor operation).

In  response  to  the  coil  coating  and   porcelain   enameling
proposals,  some  commenters claimed that it was inappropriate to
use data from some categories for regulation of other categories.
In response to these comments, the Agency  reanalyzed  the  data.
An  analysis of variance was applied to the data for the 126 days
of sampling to test the hypothesis of homogeneous plant mean  raw
and treated effluent levels across categories by pollutant.  This
analysis  is  described  in the report "A Statistical Analysis of
the Combined Metals Industries Effluent Data"  which  is  in  the
administrative record supporting this rulemaking.  Homogeneity is
the  absence  of  statistically discernible differences among the
categories,  while  heterogeneity  is  the  opposite  (i.e.,  the
presence   of   statistically  discernible   differences).    The
main conclusion drawn from the analysis of variance is that, with
the exception  of electroplating, the categories included in  the
data  base  are  generally homogeneous  with   regard   to   mean
pollutant  concentrations   in  both raw  and  treated  effluent.
That is, when data from electroplating facilities are included in
the analysis, the hypothesis of  homogeneity  across   categories
is   rejected. When  the  electroplating  data are  removed  from.
the analysis the conclusion  changes   substantially   and    the
hypothesis   of homogeneity  across  categories is not  rejected.
On  the  basis  of this analysis, the  electroplating  data  were
removed from the data base used to determine limitations for  the
final   coil   coating, porcelain  enameling,   copper   forming,
aluminum  forming,  battery  manufacturing,   nonferrous   metals
manufacturing,   nonferrous  metals  forming,   and     canmaking
regulations.

Analytical data from nonferrous  metals  manufacturing  treatment
systems   which  include  paired  raw  waste  influent  treatment
and  treated  effluent  are  limited to nine  plants   with  lime
precipitation   and   sedimentation  systems.    Three  of  these
systems  were  deemed  to  be  inappropriate  for   consideration
in   establishing  treatment  effectiveness   concentration   for
nonferrous metals  manufacturing.   Two  of  the plants had large
non-scope flows entering the treatment system and the third   had
                               171

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            GENERAL  DEVELOPMENT  DOCUMENT
                      SECT - VII
 high   TSS  (N  1000 mg/1)  concentrations  at  the  outfall  of  its  lime
 and settle treatment  system;  concentrations  indicative   of   poor
 system  operation.    The  treated   data from six   of   these   nine
 nonferrous metals  manufacturing plants with  properly   operated
 lime precipitation  and  sedimentation  systems were  compared to the
 achievable concentrations derived  using the combined  metals  data
 base.    These data generally supported the combined metals   data
 base concentrations.  These data and  the analysis  performed using
 the  data   are   in  the  administrative record  supporting   this
 rulemaking.

 EPA    examined   the   homogeneity  among    nonferrous   metals
 manufacturing   subcategories,    as     well    as    across   the
 combined  metals  data   base.   Homogeneity  is  the   absence of
 statistically   discernible   differences  among   mean untreated
 pollutant  concentrations observed in  a  set of  data.  The  purpose
 of  these   analyses was  to corroborate  the  Agency's   engineering
 judgment   that   the   untreated   wastewater     characteristics
 observed  in  the nonferrous   category   were   similar  to   those
 observed   in the  combined   metals  data.    Establishment   of
 similarity of   raw  wastes through  a   statistical   assessment
 provides   further  support  to EPA's assumption   that  lime   and
 settle treatment reduces the  toxic  metal pollutant concentrations
 in  untreated nonferrous   metals   manufacturing   wastewater   to
 concentrations  achieved  by   the same  technology  applied to   the
 wastewater    from the categories   in  the  combined metals   data
 base.    In  general, the  results of  the  analysis showed that    the
 nonferrous  subcategories  are  homogeneous  with respect to   mean
 pollutant  concentrations   across    subcategories.    Comparison
 of     the  untreated   nonferrous  metals   manufacturing    data
 combined   across subcategories  and  the combined metals    data
 also  showed  good  agreement.

 The  homogeneity observed  among the nonferrous untreated data and
 the combined  metals   data   supports   the  hypothesis  of  similar
 untreated  wastewater  characteristics  and suggests that lime and
 settle   treatment   would   reduce   the  concentrations  of  toxic
 metal    pollutants    in  the nonferrous metals  manufacturing  to
 concentrations comparable  to those  achievable by lime and  settle
 treatment  of  wastewater  from the  categories  included  in  the
 combined metals data  base.

 There    were   several   exceptions  to  the  general  finding  of
 homogeneity among the industrial categories discussed above.   The
 exceptional cases include:

 1.    Primary  aluminum  -  cathode  reprocessing   wastewater   and
 potline  wet  air  pollution control  wastewater  commingled  with
 cathode  reprocessing wastewater.
2.   Primary  lead,
process wastewater.
zinc,  and metallurgical acid  plants  - all
3.  The  primary  beryllium  subcategory  has  higher   beryllium
concentrations  in the untreated wastewater than other plants  in
                               172

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           GENERAL DEVELOPMENT DOCUMENT
                             SECT - VII
phase II.

4. The secondary  precious metals  subcategory  has  higher  zinc
concentrations  in the untreated wastewater than other plants  in
phase II.

5.  The  untreated  nickel concentrations in specific   secondary
tungsten  and  cobalt plants are higher than in the plants in the
combined metals data base.
These  first
section.
two  special  cases are  discussed  later  in  this
EPA  is  considering  the  use  of   sulfide   precipitation   in
conjunction with lime and settle, and lime, settle and filtration
for   these  three  latter  cases  where   the   influent  metals
concentrations  are higher than those observed in  the   combined
metals  data  base.  These  special  cases  are  discussed  in  a
memorandum  entitled  "Analysis  of  the  Wastewater    Pollutant
Concentrations   from   the  Phase  II   Subcategories   of   the
Nonferrous  Metals  Manufacturing Category," found in the  record
supporting   this  rulemaking.  The combined metals data base  as
discussed   below  is  applicable  to  all  nonferrous     metals
manufacturing   wastewater  as demonstrated by the homogeneity.

Properly operated hydroxide precipitation and sedimentation  will
result  in  effluent  concentrations that are directly related to
pollutant   solubilities.    Since    the    nonferrous    metals
manufacturing  raw  wastewater  matrix  contains  the  same toxic
pollutants in the same order of magnitude as the combined  metals
data  base,  the treatment process effluent long-term performance
and   variability   will  be  quite   similar.    In    addition,
interfering  properties   (such  as  chelating  agents) usually do
not    exist    in  nonferrous  metals  manufacturing  wastewater
that    would  interfere  with   metal   precipitation  and   _ so
prevent  attaining concentrations calculated  from  the  combined
metals data base.

It should be noted,  however,  that statistical analyses indicate
that the raw wastewater matrix in nonferrous metals manufacturing
contains  higher concentrations of lead and cadmium than the  raw
wastewater  of  plants used for the combined  metals  data  base.
Because the precipitation (and ultimate removal by sedimentation)
of  these  metals is directly related to  their  solubility,  EPA
believes that the differences in raw waste concentrations,  while
statistically  significant,  are  not large enough to  alter  the
achievable concentrations following treatment.

The statistical  analysis  provides  support  for  the  technical
engineering     judgment    that    electroplating    wastewaters
are  sufficiently  different  from  the  wastewaters  of    other
industrial  categories    in the data base to warrant  removal  of
electroplating   data   from   the    data    base    used     to
determine   'treatment effectiveness.
                               173

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 For   the   purpose   of   determining   treatment   effectiveness,
 additional   data  were  deleted  from  the   data    base.     These
 deletions  were  made,   almost  exclusively,    in    cases    where
 effluent  data points   were  associated with low influent  values.
 This  was done in two steps.   First,  effluent  values  measured on
 the  same day as influent values  that were  less than or  equal   to
 0.1   mg/1   were deleted.    Second,   the remaining  data  were
 screened  for cases in  which  all  influent values at a  plant  were
 low   although  slightly above  the   0.1   mg/1   value.     These
 data    were   deleted  not as  individual data  points but  as  plant
 clusters  of   data   that  were  consistently low   and  thus  not
 relevant  to  assessing treatment.  A few     data    points  were
 also    deleted   where   malfunctions  not   previously  identified
 were  recognized.   The   data   basic  to   the CMDB   are    displayed
 graphically  in  Figures VII-4  to 12  (Pages 257 to 265).

 After  all deletions, 148 data points  from   19  plants  remained.
 These   data  were  used  to   determine  the  concentration basis  of
 limitations  derived  from  the  CMDB  used  for    the  proposed
 nonferrous metals manufacturing regulations.

 The CMDB  was reviewed following its use in  a  number  of proposed
 regulations   (including  nonferrous   metals     manufacturing).
 Comments  pointed  out   a few errors  in the data and the Agency's
 review identified a few transcription errors  and some  data points
 that were appropriate for inclusion in  the  data that had not been
 used previously because of errors in  data   record   identification
 numbers.   Documents in  the record of  this rulemaking identify all
 the changes,  the  reasons  for  the  changes, and the  effect of  these
 changes  on the data base.  Comments on  other proposed  regulations
 asserted   that   the  data  base  was   too  small   and  that  the
 statistical methods used were   overly complex.    Responses   to
 specific  comments  are   provided in   a document  included in the
 record of this  rulemaking.  The Agency   believes   that  the  data
 base   is  adequate  to determine  effluent  concentrations achievable
 with lime and  settle treatment.    The  statistical methods employed
 in  the   analysis   are   well   known  and  appropriate   statistical
 references  are  provided  in   the ..documents   in  the  record that
 describe  the analysis.

 The  revised   data  base  was    re-examined    for   homogeneity.
 The earlier  conclusions  were  unchanged.   The categories  show
 good overall homogeneity with respect to concentrations  of   the
 nine  pollutants   in both raw and treated  wastewaters  with  the
 exception of electroplating.

The     same   procedures   used  in  developing  limitations for
nonferrous  metals manufacturing  from the combined   metals  data
base   were    then   used  on the revised data  base.   That  is,
certain effluent data associated with low  influent  values  were
deleted,  and  then  the  remaining   data were fit  to a lognormal
distribution to determine limitations values.   The  deletion  of
data  was  done in two  steps.   First,  effluent values measured on
the same day as influent values  that'were less than or   equal  to
0.1  mg/1 were deleted.   Second, the remaining data were  screened
                               174

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
for cases in which all  influent  values  at  a  plant  were  low
although  slightly  above  the  0.1  mg/1 value.  These data were
deleted not as individual data points but as  plant  clusters  of
data  that  were  consistently  low  and  thus  not  relevant  to
assessing treatment.

One-day Effluent Values

The basic assumption underlying the  determination  of  treatment
effectiveness  is  that  the  data for a particular pollutant are
lognormally distributed by plant.  The lognormal has  been  found
to  provide a satisfactory fit to plant effluent data in a number
of effluent guidelines categories and there was no evidence  that
the lognormal was not suitable in the case of the CMDB.  Thus, we
assumed  measurements  of each pollutant from a particular plant,
denoted by X, followed a lognormal distribution with log mean "y"
and log variance  a . The mean, variance  and  99th percentile of
X are then:


      mean of X = E(X) = exp ( y + a2/2)

      variance of X = V(X) = exp (2 y + a2) [exp (a 2) - 1]

      99th percentile = X.gg = exp ( y + 2.33 CT)

where exp is e, the base of  the  natural  logarithm.   The  term
lognormal  is  used  because  the  logarithm  of  X  has a normal
distribution   with   mean  y  and variance   a2     Using    the
basic     assumption    of    lognormality    of   the     actual
treatment  effectiveness   was determined   using   a   lognormal
distribution that,  in a sense, approximates the distribution  of
an  average  of the  plants  in   the  data   base,    i.e.,   an
"average  plant" distribution.  The notion of an "average  plant"
distribution  is not  a  strict  statistical concept but is  used
here  to determine limits that would represent  the   performance
capability  of   an average of the plants in the data base.


This "average plant" distribution for a particular pollutant  was
developed  as  follows: the log mean was determined by taking the
average of all the observations for the pollutant across  plants.
The  log  variance  was  determined  by  the  pooled within plant
variance.  This is the weighted average of the  plant  variances.
Thus, the log mean represents the average of all the data for the
pollutant  and  the  log  variance  represents the average of the
plant  log  variances  or  average  plant  variability  for   the
pollutant.

The one day effluent values were determined as follows:


Let  Xij = the jth observation on a particular pollutant at plant
i where
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           GENERAL DEVELOPMENT DOCUMENT
                         SECT - VII
   i = 1,  ..., I
   j = 1,  ..., Ji
   I = total  number of plants
   Ji = number of observations at plant i.

 Then  Yij  =  In Xij

 where In means the natural logarithm.

 Then  y =  log mean over all plants
           I
           Z
Ji
S
where n = total number of observations
          I
          2
                   Ji
and  V(y) = pooled log variance


          S   (Ji - 1) Si2
          i = 1
          S  (Ji - 1)
          i = 1

where Si2 = log variance at plant i

          Jj           9
      =   EJ (yij - Yi)2/(Ji - 1)
          J  = 1

    Yi"~= log mean at plant i.

Thus, y and V(y) are the log mean and log variance, respectively,
of the lognormal distribution used  to  determine  the  treatment
effectiveness.   The  estimated  mean and 99th percentile of this
distribution form the basis for the long term average  and  daily
maximum effluent limitations, respectively.  The estimates are
mean = E(X) = exp(y)  yn (0.5 V(y))
99th percentile = X.gg = exp [y + 2.33 /V(y)  I

where   Y (•) is a Bessel function and exp is e,  the base of the
natural  logarithms (See Aitchison,  J.  and  J.A.C.  Brown,  The
Lognormal Distribution,  Cambridge University Press,  1963).   In
cases where zeros were present in the data, a generalized form of
                               176

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
the  lognormal,  known  as the delta distribution was  used  (See
Aitchison and Brown, op. cit., Chapter 9).

For  certain  pollutants,  this approach was modified slightly to
ensure that well-operated lime and  settle  plants  in  all  CMDB
categories  would  achieve  the  pollutant  concentration  values
calculated from the CMDB.   For  instance,  after  excluding  the
electroplating data and other data that did not reflect pollutant
removal  or  proper  treatment, the effluent copper data from the
copper forming plants were  statistically  significantly  greater
than  the copper data from the other plants.  This indicated that
copper forming plants might have difficulty achieving an effluent
concentration value calculated from copper  data  from  all  CMDB
categories.    Thus, copper effluent values shown in Table VII-14
(page 242) are based only on the copper effluent  data  from  the
copper  forming  plants.  That is, the log mean for copper is the
mean of the logs of all copper values  from  the  copper  forming
plants   only  and the log variance is the pooled log variance of
the copper forming plant data only.  A similar situation occurred
in the case of lead.  That is, after excluding the electroplating
data, the effluent lead  data  from  battery  manufacturing  were
significantly  greater than the other categories.  This indicated
that battery manufacturing plants might have difficulty achieving
a lead concentration calculated from, all  the  CMDB  categories.
The lead values proposed in nonferrous metals manufacturing phase
I   were  therefore  based on the battery manufacturing lead data
only.    Comments   on   the   proposed  battery    manufacturing
regulation  objected  to this procedure and asserted   that   the
lead  concentration  values  were  too  low. Following  proposal,
the Agency obtained additional lead effluent data from a  battery
manufacturing   facility   with  well-operated lime  and   settle
treatment.   These data were combined with the proposal lead data
and  analyzed  to determine the  final   treatment  effectiveness
concentrations.    The  mean  lead concentration is unchanged  at
0.12  mg/1  but  the  final one-day maximum  and  monthly  10-day
average   maximum   increased   to   0.42   and
respectively.  -A  complete  discussion  of  the
analysis  is  contained  in a memorandum  in  the
record for this rulemaking.
       0.20      mg/1,
       lead  data  and
        administrative
In the case of cadmium, after excluding the  electroplating  data
and  data that did not reflect removal or proper treatment, there
were insufficient data to estimate the log variance for  cadmium.
The   variance used to determine the values shown in Table VII-14
for cadmium was estimated by pooling .the within  plant  variances
for  all  the other metals.  Thus, the cadmium variability is the
average of the plant variability  averaged  over  all  the  other
metals.   The log mean for cadmium is the mean of the logs of the
cadmium observations only.  A complete discussion of the data and
calculations  for  all   the   metals   is   contained   in   the
administrative record for this rulemaking.

Average Effluent Values

Average  effluent  values  that  form  the  basis for the monthly
                               177

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
limitations were developed in a manner consistent with the method
used to develop  one-day  treatment  effectiveness  in  that  the
lognormal  distribution used for the one-day effluent values  was
also used as the basis for  the  average  values.   That  is,  we
assume  a  number  of consecutive measurements are drawn from the
distribution  of  daily  measurements.   The   average   of   ten
measurements  taken  during a month was used as the basis for the
monthly average  limitations.   The  approach  used  for  the  10
measurement   values  was  employed previously in regulations for
other categories.  That is, the distribution of the average of 10
samples   from   a   lognormal  was   approximated   by   another
lognormal   distribution.   Although  the  approximation  is  not
precise theoretically,  there  is  empirical  evidence  based  on
effluent  data  from a number of categories that the lognormal is
an adequate approximation for the distribution of small  samples.
In  the course of previous work the approximation was verified in
a  computer  simulation  study  (see  "Development  Document  for
Existing  Sources  Pretreatmeht  Standards for the Electroplating
Point Source Category",   EPA  440/1-79/003,  U.S.  Environmental
Protection  Agency, Washington, D.C., August 1979).  We also note
that the average values were developed assuming  independence  of
the  observations  although  no  particular  sampling  scheme was
assumed.

Ten-Sample Average;

The  formulas for the 10-sample limitations were derived  on  the
basis  of  simple  relationships between the mean and variance of
the distributions of the daily  pollutant  measurements  and  the
average  of  10  measurements.  We assume the daily concentration
measurements for a particular pollutant, denoted by X,  follow  a
lognormal  distribution with log mean and log variance denoted by
 y   and   a2,   respectively.     Let  XIQ  denote  the  mean  of
10 consecutive  measurements.   The following relationships  then
hold assuming the daily measurements are independent:
 mean of XIQ = EXX10) = E(X)

 variance of X10 = V(X10) = V(X)  10
Where E(X) and V(X) are the mean and variance of Xf respectively,
defined   above.     We  then  assume  that   X^O    follows    a
lognormal  distribution  with  log  mean  H 10  an^  Io9  standard
deviation a io«  The mean and variance of XIQ are then
E(X10) = exp ( y10 + 0.5 cr10)

V(Xio) = exp (2 y10 + cr210 [exp ( a2i0)-l]
              n                                      O
Now, PIQ anc^ CT 10 can be derived in terms of jj  and a^ as

 W 10  = u+cr2/2 - 0.5 In [1 + exp (a2/N]
                               178

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VII
 cr2io = In [1 + (exp(
                      a2)  -1)/N]

Therefore, MIQ and   a210   can  be  estimated  using   the 'above
relationships and  the estimates of y  and a2  obtained for   the
underlying   lognormal    distribution.      The    10     sample
limitation  value   was   determined  by  the   estimate  of  the
approximate 99th percentile of the distribution of the 10  sample
average given by
X10 (.99) = exp (V 10 + 2.33  a10|.

where ftio  and OIQ are the estimates of

respectively.
                                             and  °io
Thirty Sample Average
Monthly  average  values  based  on  the  average  of  30   daily
measurements  were  also  calculated.  These are included because
monthly limitations based on 30 samples have  been  used  in  the
past  and  for comparison with the 10 sample values.  The average
values based on 30 measurements are determined on the basis of  a
statistical  result  known  as  the  Central Limit Theorem.  This
Theorem   states   that/   under   general   and   nonrestrictive
assumptions,  the  distribution  of  a  sum of a number of random
variables, say n, is approximated  by  the  normal  distribution.
The  approximation  improves  as  the  number  of  variables,  n,
increases.  The Theorem is quite general in  that  no  particular
distributional  form  is  assumed  for  the  distribution  of the
individual variables.  In most applications (as in  approximating
the   distribution  of  30-day  averages)  the Theorem is used to
approximate the distribution of the average of n observations  of
a  random  variable.   The  result  makes  it possible to compute
approximate probability statements about J:he average  in  a  wide
range  of cases.  For instance, it is possible to compute a value
below which a specified percentage  (e.g.,  99  percent)  of  the
averages  of  n  observations are likely to fall.  Most textbooks
state  that  25  or  30  observations  are  sufficient  for   the
approximation  to  be  valid.   In  applying  the  Theorem to the
distribution  of  the  30-day   average   effluent   values,   we
approximate  the  distribution  of the average of 30 observations
drawn from the distribution of daily  measurements  and  use  the
estimated 99th percentile of this distribution.

Thirty Sample Average Calculation

The  formulas  for  the  30  sample  average  were  based  on  an
application of the  Central  Limit  Theorem.   According  to  the
Theorem,   the   average   of  30  observations  drawn  from  the
distribution   of  daily  measurements,   ' denoted  by    X30, is
approximately  normally  distributed.   The  mean and variance of
                               179

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           GENERAL  DEVELOPMENT DOCUMENT
                                           SECT - VII
X30 are:
 mean of X30 = E(X30) = E(X)

 variance of X30 = V(^30) = V(X)/30.
The 30 sample average value was determined by the estimate of the
approximate 99th percentile of the distribution of the 30  sample
average given by
                = 2.33   /V(X) -: 30

where

E?X) = exp(y) 
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           GENERAL DEVELOPMENT DOCUMENT
SECT
VII
in Table VII-14 (page 242) and are included in Table  VII-21.

Additional Pollutants

Thirty-three  additional  pollutant  parameters  were   evaluated
to determine the performance of lime and settle treatment systems
in removing  them  from industrial wastewater.   Performance data
for  these parameters are not  a  part  of  the  CMDB  so   other
available  data have been used to determine the long term average
performance   of   lime   and   settle   technology    for   each
pollutant.     These   data are displayed in Table  VII-15  (page
243).  Treatment   effectiveness  values   for  these  additional
pollutants  were calculated by multiplying the  mean  performance
from Table  VII-15  by  the   appropriate    variability  factor.
(The variability  factor  is  the ratio of the  value of  concern
to  the  mean).   The pooled variability  factors   are:  one-day
maximum   -  4.100;    ten-day  average      1.821;   and  30-day
average  - 1.618.  These one-,  ten-,  and thirty-day values  are
tabulated  in  Table VII-21 (page 248).

In establishing which data were suitable for use in Table  VII-15
two   factors  were  heavily  weighed:  (1)  the  nature  of  the
wastewater; and (2) the range of pollutants or  pollutant  matrix
in  the  raw  wastewater.   These  data  have  been selected from
processes that generate dissolved metals in  the  wastewater  and
which  are  generally free from complexing agents.  The pollutant
matrix  was  evaluated  by  comparing   the   concentrations   of
pollutants  found  in  the  raw  wastewaters  with  the  range of
pollutants in the raw wastewaters of  the  combined  metals  data
set.    The raw wastewater pollutant matrix for the CMDB is shown
in  Table VII-16 (page 243). Table VII-17   (page 244),  displays
the  raw waste pollutant matrix of  wastewaters from  which  long
term average treatment effectiveness data were derived for 18  of
the added pollutant(s).  Data for the remaining added  pollutants
were  developed from CMDB related manufacturing  facilities.  The
available  data  on  these  added  pollutants  do,  not  allow   a
homogeneity   analysis  as   was  performed   on   the   combined
metals data base. Because the concentrations of the componets  in
the  raw wastewaters is similar to or less than that of the  CMDB
it  is  appropriate to logically assume  transferability  of  the
treated  pollutant concentrations to  the  combined  metals  data
base.

Antimony  (Sb) - The achievable performance for antimony is  based
on data from a  battery  and  secondary  lead  plant.   Both  EPA
sampling   data  and  recent  permit data  (1978-1982) confirm the
achievability of 0.7 mg/1 in the battery manufacturing wastewater
matrix  included  in  the  combined  data  set.   The  0.7   mg/1
concentration  is  achieved  at a nonferrous metals manufacturing
and secondary lead plant with the comparable untreated wastewater
matrix shown in Table VII-17  (page 244).

Arsenic (As) -  The  achievable  performance  of  0.51  mg/1  for
arsenic   is  based  on  permit  data  from  two nonferrous metals
                               181

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            GENERAL DEVELOPMENT DOCUMENT
                                            SECT - VII
 manufacturing plants.   The untreated wastewater matrix  shown  in
 Table VII-17 (page 244) is comparable with the combined data  set
 matrix.
 Beryllium    (Be)  - The achievable performance of  beryllium   is
 from the nonferrous metals manufacturing industry.   The 0.3  mg/1
 performance  is achieved at a beryllium plant with  the comparable
 untreated wastewater matrix shown in Table VII-17.

 Mercury  (Hg)   - The achievable concentration of 0.06  mg/1  for
 mercury is based on data from four battery plants.   The untreated
 wastewater  matrix at these plants was considered in the combined
 metals data set.

 Selenium   (Se)   - The achievable concentration of  0.30 mg/1  for
 selenium  is based on  recent  permit  data  from  one   of   the
 nonferrous     metals  manufacturing   plants   also   used   for
 arsenic  performance.   The  untreated wastewater matrix for this
 plant  is  shown  in  Table VII-17.

 Silver   (S)   -   The  achievable concentration of  0.1  mg/1  for
 silver  is   based   on  an  estimate    from    the    inorganic
 chemicals   industry.     Additional     data    supporting     a
 treatability   as   stringent or more stringent than 0.1  mg/1   is
 also  available    from seven   nonferrous  metals   manufacturing
 plants.     The    untreated wastewater  matrix for these plants  is
 comparable and   summarized in Table  VII-17.

 Thallium  (Tl)      The  0.50  mg/1  treatability for thallium   is
 transferred from the inorganic chemicals  industry.    Although   no
 untreated  wastewater  data are available to  verify comparability
 with the combined  metals  data set  plants,   no  other  sources   of
 data for thallium  treatability could be  identified.

 Aluminum   (Al)  - The  2.24  mg/1  achievable  concentration   of
 aluminum  is  based  on  the mean performance   of  three  aluminum
 forming   plants  and  one  coil  coating plant.    These  plants  are
 from  categories   included in the  combined   metals    data   set,
 assuring  untreated wastewater  matrix comparability.

 Barium
^	  (Ba) - The achievable performance for barium (0.42  mg/1)
is based on data from one nonferrous metals forming  plant.   The
untreated  wastewater matrix shown in Table VII-17 is  comparable
with the combined metals data base.

Boron
	  (B) - The achievable performance of 0.36 mg/1 for boron is
based  on  data from a nonferrous metals  plant.   The  untreated
wastewater matrix shown  in Table VII-17 is comparable with   the
combined metals data base.

Cesium (Cs) - The achievable performance for cesium (0.124  mg/1)
is  based  on  the performance achievable for  sodium  using  ion
exchange technology.  This transfer of performance is technically
justifiable  because  of  the  similarity  of  the  chemical  and
physical behavior of these monovalent atoms.
                               182

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Cobalt    (Co)  - The   0.05  mg/1 achievable  concentration   is
based  on  nearly  complete  removal of  cobalt  at  a  porcelain
enameling  plant  with   a  mean   untreated  wastewater   cobalt
concentration  of  4.31  mg/1.   In  this  case,  the  analytical
detection   limit   using   aspiration   techniques   for    this
pollutant  is  used  as the basis of the treatability.  Porcelain
enameling  was  considered in the  combined  metals   data  base,
assuring untreated wastewater matrix comparability.

Columbium  (Nb) - Data collected at two refractory metals forming
plants  indicate that lime and settle reduces columbium to  below
the  level  of  detection (using  x-ray  fluorescence  analytical
methods)  when an operating pH of eight is  maintained.   Another
sampled lime and settle treatment system is operated at a  higher
pH, from 10.5 to 11.5.  Effluent concentrations of columbium from
this  system  are  significantly  higher.-  Therefore,  the  data
indicate that if the treatment system is operated at a pH near 8,
columbium should be removed,to below the level of detection.  The
level  of  detection (0.12 mg/1) is used as the  one-day  maximum
concentration  for lime and settle treatment effectiveness values
are  established  since it is impossible to  determine  precisely
what  concentrations are achievable.   The  untreated  wastewater
matrix  shown in Table VII-17 (page 244) is comparable with  the
combined metals data base.

Fluoride   (F) - The 14.5 mg/1 treatability of fluoride generally
applicable to metals processing is based on the mean  performance
(47  samples) from two electronics manufacturing phase II plants.
The untreated wastewater matrix for this  plant  shown  in  Table
VII-17 is comparable to the combined metals data set.

Gallium  (Ga) -  The  achievable  concentration  of  gallium  is
assumed to be the same as the level for chromium (0.084 mg/1) for
the  reasons discussed below for indium.

Germanium   (Ge)  - The achievable concentration of germanium  is
assumed  to  be the same as the level for chromium  (0.084  mg/1)
for the reasons  discussed  for  indium  (see below).

Gold  (Au).     The treatment effectiveness value for  gold  (0.1
mg/1)  is  based  on  the performance  achieved  at  a  secondary
precious  metals  manufacturing facility whose  treatment  scheme
includes lime,  settle,  filter and ion exchange.   This value is
supported  by  data  obtained  from  an  ion  exchange  equipment
manufacturer  (Rohm & Haas) for treatment of electroplating rinse
water.

Hafnium (Hf) - The achievable performance for hafnium  (7.28 mg/1)
is  based  on  the  performance achieved  for  zirconium  at  two
nonferrous  metals forming plants.    The Agency  believes   that
since  the water chemistry for zirconium and hafnium is  similar,
hafnium can be removed to the same levels as zirconium.

Indium  (In) - The achievable concentration for indium is assumed
to   be   the  same   as the level  for  chromium  (0.084  mg/1).
                               183

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
Lacking  any treated effluent data for indium,  a comparison  was
made  between the  theoretical  solubilities  of  indium  and the
metals in the Combined Metals  Data  Base:   cadmium,   chromium,
copper,   lead,  nickel  and  zinc.   The  theoretical solubility
of   indium   (2.5 x 10-7,) is more similar to  the   theoretical
solubility   of  chromium   (1.65 x 10-8   ) than  it  is  to   the
theoretical  solubilities of  cadmium,   copper,   lead,   nickel
or   zinc.    The theoretical solubilities of these metals  range
from 20 x 10-3 to 2.2 x 10-5 mg/1.   This  comparison  is further
supported  by  the  fact  that  indium  and  chromium  both  form
hydroxides in the trivalent   state.  Cadmium,    copper,   lead,
nickel  and  zinc  all  from  divalent hydroxides.

Molybdenum (Mo) -  The 1.83 mg/1 treatment effectiveness is based
on data from a nonferrous metals manufacturing and forming  plant
which   uses  coprecipitation  of  molybdenum  with  iron.    The
treatment effectiveness concentration of 1.83 mg/1 is  achievable
with  iron coprecipitation and lime and settle  treatment.    The
untreated   wastewater matrix shown in Table VII-17 (page 244) is
comparable with the combined metals data base.

Palladium (Pd) -  The treatment effectiveness value for palladium
(0.1  mg/1)  is based on the performance achieved at a  secondary
precious  metals  manufacturing facility whose  treatment  scheme
includes lime,  settle,  filter and ion exchange.   This value is
supported ' by  data  obtained  from  an  ion  exchange  equipment
manufacturer (Rohm & Haas) for treatment of electroplating  rinse
water.

Phosphorus  (P)  - The  4.08 mg/1   achievable  concentration  of
phosphorus   is based  on  the  mean  of 44 samples including  19
samples  from the Combined Metals Data Base and 25  samples  from
the   electroplating data  base.    Inclusion  of  electroplating
data   with   the   combined  metals    data    was    considered
appropriate,   since  the   removal mechanism for phosphorus is a
precipitation reaction with calcium rather than hydroxide.

Platinum  (Pt) -  The treatment effectiveness value for  platinum
(0.1  mg/1)  is based on the performance achieved at a  secondary
precious  metals  manufacturing facility whose  treatment  scheme
includes lime,  settle,  filter and ion exchange.   This value is
supported  by  data  obtained  from  an  ion  exchange  equipment
manufacturer (Rohm & Haas) for treatment of electroplating  rinse
water.

Radium   226  (Ra  226) - The  achievable  performance  of 6.17
picocuries per liter for radium 226 is based  on  data  from  one
facility  in  the  uranium  subcategory  of  the  Ore  Mining and
Dressing category which practices barium chloride coprecipitation
in conjunction with lime and  settle  treatment.   The  untreated
wastewater  matrix shown in Table VII-17 is  comparable with  the
Combined Metals Data Base.

Rhenium (Re)  - The achievable performance for rhenium (1.83 mg/1)
is  based  on  the  performance  achieved  for  molybdenum  at  a
                               184

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           GENERAL DEVELOPMENT DOCUMENT
                            SECT - VII
nonferrous metals manufacturing and forming plant.  This transfer
of   performance  is  technically  justifiable  because  of   the
similarity  of  the  physical  and  chemical  behavior  of  these
compounds.

Rubidium  (Rb) -  The achievable performance for rubidium  (0.124
mg/1) is based on the performance achievable for sodium using ion
exchange technology.  This transfer of performance is technically
justifiable  because  of  the  similarity  of  the  chemical  and
physical behavior of these monvalent atoms.

Tantalum  (Ta)  - As  with  columbium,   data  collected  at  two
refractory  metals  forming plants indicate that lime and  settle
reduces  tantalum  to below the level of detection  (using  x-ray
fluorescence analytical methods) when an operating pH of eight is
maintained.   Another sampled lime and settle treatment system is
operated  at  a  higher  pH,   from  10.5  to   11.5.    Effluent
concentrations     of    tantalum    from   this   system     are
significantly  higher.   Therefore,  the  data  indicate that  if
the   treatment  system  is operated at a pH  near  8,   tantalum
should be removed to below the level of detection.  The level  of
detection   (0.45   mg/1)  is  used  as   the   one-day   maximum
concentration for lime and  settle treatment  effectiveness.   No
long-term,     10-day,     and    30-day    average     treatment
effectiveness values are established since  it is  impossible  to
determine  precisely what  concentrations  are achievable.    The
untreated  wastewater matrix shown in Table VII-17 is  comparable
with the combined metals data base.

Tin  (Sn) - The achievable performance of 0.14  mg/1 for tin is
based  on  data  from  one  metal  finishing  tin   plant.    The
untreated  wastewater matrix shown in Table VII-17 is  comparable
with  the  combined metals data base.
Titanium
- The 0.19 mg/1 achievable concentration is  based
on the mean performance of four nonferrous metals forming plants.
A total of 9 samples were included in the calculation of the mean
performance.  The untreated wastewater matrix shown in Table VII-
17 is comparable with the combined metals data base.

Tungsten   (W)   - The  1.29  mg/1  treatability   (using   x-ray
fluorescence   analytical   methods)  is based on  data  collected
from the refractory metals forming plant where an operating pH of
10.5  to   11.5  was used.   The data indicate  that  maintaining
the   pH  within  this  range   achieves   significantly   better
removal  of tungsten  than  a  pH  near  8.   Therefore,   plants
that  treat wastewaters containing both tantalum and tungsten  or
other  metals that precipitate at a higher pH may need to  use  a
two-stage  lime and  settle system to remove all of these metals.
The  untreated  wastewater    matrix   shown   in   Table   VII-17
is comparable with the combined metals data base.

Uranium  (U) -  The  achievable  performance  of  4.0  mg/1   for
uranium  is  based  on  data  from  one  facility  in the uranium
                               185

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VII
subcategory  of  the  Ore  Mining  and  Dressing  category  which
practices  chemical  precipitation  and  sedimentation treatment.
The  untreated wastewater matrix shown in Table VII-17 (page 244)
is comparable with the combined metals data base.

Vanadium  (V) - Data collected at two nonferrous  metals  forming
plants  indicate  that lime and settle reduces vanadium to  below
the detection limit.   The level of detection (0.10 mg/1) is used
as  the  one-day  maximum  concentration  for  lime  and   settle
treatment.   No  long-term,  10-day  or 30-day average  treatment
effectiveness  values are established since it is  impossible  to
determine  precisely  what concentrations  are  achievable.    The
untreated  wastewater matrix shown in Table VII-17 is  comparable
with the combined metals data base.

Zirconium  (Zr
___^	   Zr)  - The zirconium treatment effectiveness of  7.28
mg/1is based on the mean performance of two  nonferrous  metals
forming  plants with lime and settle treatment.   One plant forms
zirconium  and  the other plant  forms  refractory  metals.   The
untreated  wastewater matrix shown in Table VII-17 is  comparable
with the combined metals data base,

Applicability  of  CMBD  and Additional Pollutant  Data  Base  to
Plants with Elevated Raw Wastewater Concentrations

Several  comments  on  the proposed  regulations  for  nonferrous
metals  manufacturing pointed out that plants in the category had
concentrated    process    wastewater    discharges    containing
significantly  higher concentrations of toxic metals  than  those
observed  in plants in the combined metals data base  and  plants
used to establish treatment effectiveness concentrations for  the
additional  pollutants.   Plants with elevated  cadmium,  copper,
lead, and zinc concentrations may apply sulfide precipitation and
filtration  as  a  polishing step following lime  and  settle  to
achieve  the  concentrations  based on  the  CMDB.   Plants  with
elevated  arsenic and selenium concentrations may  apply  sulfide
precipitation  and filtration as a preliminary treatment to  lime
and settle to achieve the CMDB concentrations.

Lime  and Settle Performance on Cathode Reprocessing Wastewater ^
Primary Aluminum

Treatment  performance data gathered during a  pilot-scale  study
conducted by EPA on primary aluminum wastewater demonstrated that
plants  operating cathode reprocessing operations and  using  the
wastewater  as makeup for potline scrubber liquor cannot  achieve
the  performance values proposed for aluminum, antimony,  nickel,
and  fluoride.  This is due to the matrix  differences  resulting
from cathode reprocessing.  The cathode reprocessing  wastewater,
and  subsequently the potline scrubber liquor, contain  dissolved
solids  levels in the five to six percent  range.   Consequently,
the  Agency  is promulgating effluent limitations  and  standards
based  on  specific treatment  effectiveness  concentrations  for
those  primary aluminum plants that operate cathode  reprocessing
                               186

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VII
and commingle resulting wastewater with potline scrubber  liquor.
To  receive these alternate limitations the plant may not  dilute
potline   scrubber  liquor  blowdown  or   cathode   reprocessing
wastewater with any process or nonprocess wastewater source.   If
the potline scrubber blowdown is diluted with other  wastewaters,
the   complexity   of   the  matrix  decreases   and   thus   the
concentrations  of the combined metals data base (as well as  the
transferred  aluminum, antimony and fluoride concentrations)  can
be achieved.  The derivation of the limitations and standards for
this wastewater is detailed in the primary aluminum supplement.
Cyanide   Precipitation  Performance  in
Wastewaters
                                           Cathode   Reprocessing
Cyanide   is
reprocessing
presence is
reduction of
detected  at
mg/1 in this
the cyanide
              present  in  wastewater  resulting   from   cathode
              in  the primary aluminum  smelting  industry.   Its
            due to the use of coke and pitch in the  electrolytic
             alumina to produce aluminum metal.  Cyanide has been
             concentrations ranging from approximately 50 to  800
             wastewater.  In general, approximately 90 percent of
            is present as a complex, hexacyanoferrate.
                                                  examining   the
                                                  wastewater   by
                                                 chloride.  These
                                                 the  performance
EPA  conducted  bench-scale and pilot-scale  studies  on  cathode
reprocessing  and  cryolite recovery wastewater  from  a  primary
aluminum  plant.   The  study  was  directed  at
effectiveness  of  removing  cyanide  from  this
precipitating  with  ferrous sulfate and ferric
treatment  performance  studies  revealed  that
limits for cyanide precipitation are not transferrable from  coil
coating  to  primary aluminum wastewater.    The pilot  study  is
summarized  in  Section VII of the primary  aluminum  subcategory
supplement.

Treatment  Effectiveness Concentrations for Fluoride  in  Primary
Aluminum and Primary Columbium-Tantalum Subcategories

The   Agency   has  re-evaluated  lime  and   settle   technology
performance   for  fluoride  removal.   The  proposed   treatment
performance  for  fluoride was transferred  from  electrical  and
electronic component manufacturing (phase I) lime and settle mean
performance.   However, examination of the electronics  data  has
lead  the  Agency  to conclude that  the  raw  concentrations  of
fluoride  in  nonferrous metals  manufacturing  wastewaters  more
closely  resemble the higher concentrations found  in  electrical
and  electronics  phase  II rather than phase I  (49  FR  55690).
Therefore, the Agency believes it is appropriate to use the  mean
performance   and   daily  maximum  variability   developed   for
electronics  phase  II to establish treatment  effectiveness  for
fluoride removal by lime and settle treatment.

The  fluoride  data from Electrical and Electronic  Components  -
Phase  II  were taken from self-sampling data  from  two  plants.
There were 20 observations from one plant and 27 from the  other,
totaling  47.  A geometrical form of the lognormal  distribution,
known as the delta lognormal distribution, was used to model  the
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
data.   The new long-term performance concentration of 14.5  mg/1
was  estimated  using the mean of the  distribution  of  effluent
concentrations.   The  daily maximum limitation of  35  mg/1  was
based  upon estimates of the 99th percentile of the  distribution
of effluent concentrations.  The monthly average limitation of 20
mg/1  was  based on the 99th percentile of  the  distribution  of
averages  of 10 samples drawn from the distribution  of  effluent
concentrations.

LS&F Performance

Tables VII-18 and VII-19 (pages 245 and 246) show long-term  data
from  two  plants which have well operated precipitation-settling
treatment followed by  filtration.   The  wastewaters  from  both
plants  contain  pollutants  from metals processing and finishing
operations  (multi-category).   Both  plants  reduce   hexavalent
chromium  before neutralizing and precipitating metals with lime.
A clarifier is used to remove much  of  the  solids  load  and  a
filter  is  used  to  "polish"  or  complete removal of suspended
solids.  Plant A uses a pressure filter, while  plant  B  uses  a
rapid sand filter.

Raw  wastewater  data  was  collected  only  occasionally at each
facility  and  the  raw  wastewater  data  is  presented  as   an
indication  of  the  nature of the wastewater treated.  Data from
plant A was received as a statistical summary and is presented as
received.  Raw laboratory data  was  collected  at  plant  B  and
reviewed  for  spurious  points and discrepancies.  The method of
treating the data base is discussed below under lime, settle, and
filter treatment effectiveness.

Table VII-20 (page 247) shows long-term data for zinc and cadmium
removal at plant C, a primary zinc smelter, which operates a LS&F
system.  This data represents about  4  months  (103  data  days)
taken  immediately  before  the  smelter was closed.  It has been
arranged similarly to Plants A and B for comparison and use.

These data  are  presented  to  demonstrate  the  performance  of
precipitation-settling-filtration  (LS&F) technology under actual
operating conditions and over a long period of time.

It should be noted that the iron content of the raw wastewater of
plants A and B is high while that  for  Plant  C  is  low.   This
results,  for plants A and B, in co-precipitation of toxic metals
with iron.  Precipitation using high-calcium lime for pH  control
yields  the  results  shown  above.   Plant  operating  personnel
indicate that this chemical treatment combination (sometimes with
polymer assisted coagulation) generally produces better and  more
consistent  metals removal than other combinations of sacrificial
metal ions and alkalis.

The LS&F performance data presented here  are  based  on  systems
that  provide polishing filtration after effective L&S treatment.
We have previously shown that L&S treatment is equally applicable
to  wastewaters  from  the  five  categories   because   of   the
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
homogeneity  of  its  raw  and  treated  wastewaters,  and  other
factors.  Because of the similarity of the wastewaters after  L&S
treatment,  the  Agency  believes  these  wastewaters are equally
amenable to treatment using polishing filters added  to  -the  L&S
treatment   system.    The Agency concludes that these LS&F  data
based in part on porcelain enameling are directly  applicable  to
nonferrous metals manufacturing.

Analysis of Treatment System Effectiveness

Data are presented in Table VII-14 showing  the  mean,   one-day,
10-day, and 30-day values for nine pollutants examined in the L&S
combined  metals  data  base.   The pooled variability factor for
seven metal pollutants (excluding cadmium because  of  the  small
number  of  data  points)  was determined and is used to estimate
one-day, 10-day and 30-day values.  (The  variability  factor  is
the  ratio  of  the  value  of  concern  to  the mean. The pooled
variability  factors  are:   one-day  maximum  -  4.100;  ten-day
average  - 1.821;   and 30-day average - 1.618.)  For values  not
calculated from the CMDB as previously discussed, the mean  value
for  pollutants  shown  in  Table  VII-15 were multiplied by  the
variability  factors to compute the one,  ten and 30-day  values.
These are tabulated in Table VII-21.

The   treatment   effectiveness  for  sulfide  precipitation  and
filtration has been  calculated  similarly.   Long-term   average
values   shown  in Table VII-6 (page 238) have been multiplied by
the appropriate variability factor, to estimate one-day   maximum,
and  ten-day  and  30-day  average values.   Variability  factors
developed in the combined metals data base were used because  the
raw  wastewaters  are  identical  and  the  treatment methods are
similar as both use chemical precipitation and solids removal  to
control metals.

LS&F   technology  data are presented in Tables VII-18 and VII-19
(pages 245 and 246). These data represent two operating plants (A
and  B) in which  the technology has been installed and  operated
for some years.   Plant A,  data  was  received  as a  statistical
summary  and  is  presented without change.   Plant B  data   was
received  as  raw  laboratory analysis  data.  ,  Discussions with
plant personnel indicated that operating experiments and  changes
in  materials and  reagents  and occasional   operating    errors
had  occurred  during  the  data' collection period.  No  specific
information  was  available  on those  variables.   To  sort  out
high values probably caused by .methodological factors from random
statistical   variability,   or data  noise,   the  plant  B data
were analyzed.   For each of four pollutants  (chromium,  nickel,
zinc,   and  iron),   the  mean  and standard  deviation  (sigma)
were calculated for the entire data set.   A data day' was removed
from  the  complete  data  set when   any  individual   pollutant
concentration  for  that day exceeded the sum of  the  mean  plus
three  sigma  for that pollutant.   Fifty-one  data days (from  a
total of about 1300) were eliminated by this method.

Another  approach was also used as a check on the above method of
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
eliminating certain high  values.   The  minimum  values  of  raw
wastewater   concentrations  from  Plant  B  for  the  same  four
pollutants were compared to the  total  set  of  values  for  the
corresponding   pollutants.    Any   day  on  which  the  treated
wastewater pollutant concentration  exceeded  the  minimum  value
selected  from  raw  wastewater concentrations for that pollutant
was discarded.  Forty-five days of data were eliminated  by  that
procedure.  Forty-three days of data in common were eliminated by
either  procedures.  Since common engineering practice (mean plus
3 sigma) and logic (treated wastewater concentrations  should  be
less  than  raw  wastewater concentrations) seem to coincide, the
data base with the 51 spurious data days eliminated is the  basis
for  all  further  analysis.  Range, mean plus standard deviation
and mean plus two standard deviations are shown in Tables  VII-18
and VII-19 (pages 245 and 246) for Cr, Cu, Ni, Zn and Fe.

The  Plant  B  data was separated into 1979, 1978, and total data
base (six years) segments.  With the  statistical  analysis  from
Plant  A  for 1978 and 1979 this in effect created five data sets
in which there is some overlap between the individual  years  and
total  data  sets from Plant B.  By comparing these five parts it
is apparent that they are quite similar and all appear to be from
the same family of numbers.  The largest  mean  found  among  the
five  data  sets for each pollutant was selected as the long-term
mean for LS&F technology and is used as the LS&F  mean  in  Table
VII-21.

Plant  C data was used as a basis for cadmium removal performance
and as a check on the zinc values derived from Plants  A  and  B.
The  cadmium  data is displayed in Table VII-20 (page 247) and is
incorporated into Table VII-21 (page 248) . for  LS&F.   The  zinc
data   was  analyzed  for compliance with the  1-day  and  30-day
values  in Table VII-21;   no  zinc value of the 103 data  points
exceeded the 1-day zinc value of 1.02 mg/1.   The 103 data points
were separated into blocks of 30 points and averaged.   Each   of
the   3  full  30-day averages  was  less  than  the  Table  VII-
21  value of 0.31 mg/1.  Additionally the Plant C raw  wastewater
pollutant  concentrations (Table  VII-20)  .are  well  within  the
range   of raw wastewater concentrations of the  combined  metals
data  base   (Table  VII-16),  further supporting the  conclusion
that Plant C wastewater data is compatible with similar data from
Plants A and B.

Concentration  values  for  regulatory use are displayed in Table
VII-21.   Mean one-day, ten-day and 30-day  values  for  L&S  for
nine   pollutants  were taken from Table VII-14  (page  242;  the
remaining  L&S  values were developed using the  mean  values  in
Table VII-15  and the mean variability factors discussed above.

LS&F  mean  values  for  Cd,  Cr,   Ni,  Zn and Fe are derived from
plants A, B,  and C as discussed above.   One-, ten- and thirty-day
values are derived by applying the variability  factor  developed
from  the pooled data base for the specific pollutant to the mean
for that pollutant.   Other LS&F values are calculated  using  the
long-term  average  or  mean  and  the  appropriate   variability
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
factors.

Copper levels achieved at Plants  A  and  B  may  be  lower  than
generally  achievable  because  of  the high iron content and low
copper content of  the  raw  wastewaters.   Therefore,  the  mean
concentration value from plants A and B achieved is not used; the
LS&F mean for copper is derived from the L&S technology.

L&S   cyanide  mean levels shown in Table VII-8  (page  239)  are
converted  to  one-day,  ten-day and 30-day  values  using   mean
variability   factors.  LS&P  mean  cyanide  is   calculated   by
applying   the   ratios  of removals L&S and  LS&P  as  discussed
previously   for   LS&F  metals limitations.     The    treatment
method   used  here  is  cyanide precipitation.  Because  cyanide
precipitation  is limited  by  the same  physical  processes   as
the    metal    precipitation,    it   is   expected   that   the
variabilities  will be similar.  Therefore,  the average  of  the
metal   variability  .factors  has  been  used  as  a  basis   for
calculating   the   cyanide  one-day,   ten-day   and  thirty-day
average treatment effectiveness values.

The filter performance for removing TSS as shown in  Table  VII-9
(page 240) yields a mean effluent concentration of 2.61 mg/1 and
corresponds  to  a 10-day average of 4.33,  30-day   average   of
3.36  mg/1  and a  one-day  maximum of  8.88.   These  calculated
values more than amply support the classic thirty-day and one-day
values  of 10 mg/1 and 15 mg/1,  respectively, which are used for
LS&F.

Although   iron   concentrations  were  decreased  in  some  LS&F
operations, some facilities using that treatment  introduce  iron
compounds  to  aid settling.  Therefore, the one-day, ten-day and
30-day values for iron at LS&F were held at the L&S level  so  as
to  not  unduly  penalize the operations which use the relatively
less objectionable iron compounds to enhance  removals  of  toxic
metals.

The .removal of.additional fluoride by adding polishing filtration
is  suspect  because  lime  and settle technology removes calcium
fluoride  to  a  concentration  near  its  solubility.   The  one
available  data  point appears to question the ability of filters
to achieve high removals of additional  fluoride.   The  fluoride
concentrations  demonstrated  for  L&S  are used as the treatment
effectiveness for LS&F.

MINOR TECHNOLOGIES

Several other treatment technologies were considered for possible
application  in  this  subcategory.    These   technologies   are
presented here.

8. Carbon Adsorption

The  use  of  activated  carbon to remove dissolved organics from
water and wastewater is a long demonstrated  technology.  ' It  is
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
one  of  the  most efficient organic removal processes available.
This sorption process is reversible, allowing activated carbon to
be regenerated for reuse by the application of heat and steam  or
solvent.   Activated  carbon  has  also proved to be an effective
adsorbent for many toxic metals, including mercury.  Regeneration
of carbon which has adsorbed significant metals, however, may  be
difficult.

The term activated carbon applies to any amorphous form of carbon
that   has   been  specially  treated  to  give  high  adsorption
capacities.  Typical raw materials include  coal,  wood,  coconut
shells,  petroleum  base  residues,  and  char from sewage sludge
pyrolysis.   A  carefully  controlled  process  of   dehydration,
carbonization,  and  oxidation  yields  a product which is called
activated  carbon.   This  material  has  a  high  capacity   for
adsorption  due primarily to the large surface area available for
adsorption,  500 to 1500 m2/sq m resulting from a large number of
internal pores.   Pore  sizes  generally  range  from  10  to 100
angstroms in radius.

Activated  carbon  removes contaminants from water by the process
of  adsorption,  or  the  attraction  and  accumulation  of   one
substance   on   the   surface   of  another.   Activated  carbon
preferentially adsorbs organic compounds  and,  because  of  this
selectivity,   is  particularly  effective  in  removing  organic
compounds from aqueous solution.

Carbon  adsorption  requires  pretreatment   to   remove   excess
suspended  solids,  oils,  and  greases.  Suspended solids in the
influent should  be  less  than  50  mg/1  to  minimize  backwash
requirements; a downflow carbon bed can handle much higher levels
(up to 2000 mg/1) but requires frequent backwashing.  Backwashing
more  than  two or three times a day is not desirable; at 50 mg/1
suspended solids, one backwash  will  suffice.   Oil  and  grease,
should  be  less  than  about 10 mg/1.  A high level of dissolved
inorganic material  in  the  influent  may  cause  problems  with
thermal  carbon reactivation (i.e., scaling and loss of activity)
unless appropriate preventive steps are taken.  Such steps  might
include  pH control, softening, or the use of an acid wash on the
carbon prior to reactivation.

Activated carbon is available in both powdered and granular form.
An adsorption column packed with granular  activated  carbon   is
shown  in  Figure  VII-17  (page 270).   Powdered carbon is  less
expensive per unit weight and may have slightly higher adsorption
capacity, but it is more difficult to handle and to regenerate.

Application and Performance.  Carbon adsorption is used to remove
mercury from wastewaters.  The removal rate is influenced by  the
mercury  level  in the influent to the adsorption unit.  In Table
VII-24, removal levels found at  three  manufacturing  facilities
are listed.

In  the  aggregate  these  data  indicate  that very low effluent
levels could be attained from any raw waste by  use  of  multiple
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
adsorption   stages.    This   is  characteristic  of  adsorption
processes.

Isotherm tests have  indicated  that  activated  carbon  is  very
effective  in  adsorbing  65  percent  of  the  organic  priority
pollutants and is reasonably effective for  another  22  percent.
Specifically/  for the organics of particular interest, activated
carbon  was  very  effective  in   removing   2,4-dimethylphenol,
fluoranthene,   isophorone,   naphthalene,  all  phthalates,  and
phenanthrene.    It   was   reasonably   effective   on    1,1,1-
trichloroethane,  1,1-dichloroethane, phenol, and toluene.  Table
VII-22 (page 249) summarizes the treatment effectiveness for most
of  the  organic  priority  pollutants  by  activated  carbon  as
compiled  by  EPA.  Table VII-23 (page 250) summarizes classes of
organic compounds together with examples  of  organics  that  are
readily adsorbed on carbon.

In  response  to comments from companies in the primary  aluminum
subcategory on the proposed mass limitations for  benzo(a)pyrene,
the  Agency  conducted  bench and pilot-scale  tests  or  potline
scrubber   liquor  to  determine  the  effectiveness  of  various
wastewater treatment technologies,  including carbon  adsorption,
in  removing  polynuclear aromatic hydrocarbons (PAH) from  these
wastewaters.  The study is discussed in greater detail in Section
VII  of  the primary aluminum subcategory supplement and  in  the
record supporting this rulemaking.

The  pilot tests demonstrated that;activated carbon  will  reduce
the    polynuclear   aromatic   hydrocarbons   to   the   nominal
quantification limit of 0.010 mg/1.

Advantages  and  Limitations.  -The  major  benefits  of   carbon
treatment include applicability to a wide variety of organics and
high  removal  efficiency.  Inorganics such as cyanide, chromium,
and  mercury  are  also  removed  effectively.    Variations   in
concentration  and  flow  rate are well tolerated.  The system is
compact,  and  recovery  of  adsorbed  materials   is   sometimes
practical.  ^However,  destruction  of  adsorbed  compounds often
occurs  during  thermal  regeneration.   If  carbon   cannot   be
thermally  desorbed,  it  must  be  disposed  of  along  with any
adsorbed pollutants.  The capital and operating costs of  thermal
regeneration are relatively high'.  Cost surveys show that thermal
regeneration  is  generally  economical  when  carbon 'use exceeds
about 1,000 Ib/day.  Carbon cannot remove low molecular weight or
highly soluble  organics.   It  also  has  a  low  tolerance  for
suspended  solids,  which  must be removed to at least 50 mg/1 in
the influent water.

Operational Factors.  Reliability:  This system  should  be  very
reliable  with  upstream  protection  and  proper  operation  and
maintenance procedures.

Maintainability:  This system requires periodic  regeneration  or
replacement  of spent carbon and is dependent upon raw waste load
and process efficiency.
                               193

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 Solid  Waste  Aspects:   Solid  waste  from   this   process   is
 contaminated  activated  carbon  that  requires disposal.  Carbon
 undergoes   regeneration,    which  reduces   the   solid   waste
 problem  by reducing the frequency of carbon replacement.

 Demonstration   Status.   Carbon  adsorption  systems  have  been
 demonstrated to be practical and economical in reducing COD, BOD,
 and  related parameters  in  secondary  municipal  and  industrial
 wastewaters;  in  removing  toxic  or  refractory  organics  from
 isolated  industrial  wastewaters;  in  removing  and  recovering
 certain organics from wastewaters; and in removing and some times
 recovering  selected  inorganic  chemicals  from  aqueous wastes.
 Carbon adsorption is a viable and economic  process  for  organic
 waste  streams  containing  up to 1 to 5 percent of refractory or
 toxic organics.  Its applicability for removal of inorganics such
 as metals has also been demonstrated.

 9. Centrifugation

 Centrifugation  is  the  application  of  centrifugal  force   to
 separate  solids  and  liquids  in  a  liquid-solid mixture or to
 effect  concentration  of  the  solids.    The   application   of
 centritugal   force   is   effective   because   of  the  density
 differential normally found between the insoluble solids and  the
 liquid  in  which  they  are  contained.   As  a  waste treatment
 procedure, Centrifugation is applied to  dewatering  of  sludges.
 One  type of centrifuge is shown in Figure VII-18 (page 271).

 There  are  three common types of centrifuges;  disc, basket, and
 conveyer.   All  three  operate  by  removing  solids  under  the
 influence of centrifugal force.  The fundamental difference among
 the  three  types  is the method by which solids are collected in
 and  discharged from the bowl.

 In the disc centrifuge, the sludge feed  is  distributed  between
 narrow  channels  that  are  present  as  spaces  between stacked
 conical discs.  Suspended particles are collected and  discharged
 continuously  through  small  orifices  in  the  bowl .wall.  The
 clarified effluent is discharged through an overflow weir.

A second type of centrifuge which is useful in dewatering sludges
 is the basket centrifuge.   In this  type  of  centrifuge,  sludge
 feed  is  introduced  at  the  bottom  of  the basket,  and solids
 collect at the bowl wall while clarified effluent  overflows  the
 lip  ring  at the top.   Since the basket centrifuge does not have
provision for continuous discharge of collected  cake,   operation
 requires interruption of the feed for cake discharge for a minute
or two in a 10 to 30 minute overall cycle.

The  third  type of centrifuge commonly used in sludge  dewatering
 is the conveyer type.   Sludge is fed through  a  stationary  feed
pipe  into  a  rotating  bowl in which the solids are settled out
against the bowl wall by centrifugal force.   From the bowl  wall,
the  solids  are  moved  by a screw to the end of the machine,  at
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
which  point  they  are  discharged.    The  liquid  effluent   is
discharged  through  ports  after  passing the length of the bowl
under centrifugal force.

Application And  Performance.   Virtually  all  industrial ^waste
treatment  systems  producing  sludge  can  use centrifugation^to
dewater it.  Centrifugation is currently being  used  by  a  wide
range of industrial concerns.

The performance of sludge dewatering by centrifugation depends on
the  feed  rate,  the  rotational  velocity  of the drum, and the
sludge composition and concentration.  Assuming proper design and
operation, the solids content of the sludge can be  increased  to
20 to 35 percent.

Advantages  And  Limitations.  Sludge dewatering centrifuges have
minimal space requirements and show a  high  degree  of  effluent
clarification.   The  operation  is simple, clean, and relatively
inexpensive.   The  area  required  for   a   centrifuge   system
installation  is  less  than that required for a filter system or
sludge drying bed of equal capacity,  and  the  initial  cost  is
lower.

Centrifuges have a high power cost that partially offsets the low
initial  cost.   Special  consideration  must  also  be  given to
providing sturdy foundations and  soundproofing  because  of  the
vibration  and  noise  that  result  from  centrifuge  operation.
Adequate electrical power  must  also  be  provided  since  large
motors  are  required.   The  major difficulty encountered in the
operation of centrifuges has been the disposal of the concentrate
which is relatively high in suspended, non-settling solids.

Operational  Factors.   Reliability:   Centrifugation  is  highly
reliable  with  proper  control  of  factors such as sludge feed,
consistency, and temperature.  Pretreatment such as grit  removal
and  coagulant  addition  may  be  necessary,  depending  on  the
composition of the sludge and on the type of centrifuge employed.

Maintainability:  Maintenance consists of  periodic  lubrication,
cleaning, and inspection.  The frequency and degree, of inspection
required  varies  depending  on  the  type of sludge solids being
dewatered and the maintenance service conditions.  If the  sludge
is  abrasive,  it is recommended that the first inspection of the
rotating assembly be made  after  approximately  1,000  hours  of
operation.   If the sludge is not abrasive or corrosive, then the
initial inspection might be delayed.   Centrifuges  not  equipped
with  a  continuous  sludge  discharge  system  require  periodic
shutdowns for manual sludge cake removal.

Solid Waste Aspects:    Sludge  dewatered  in  the  centrifugation
process  may  be disposed of by landfill.  The clarified effluent
(centrate), if high in  dissolved or  suspended solids, may require
further treatment prior to discharge.

Demonstration Status.   Centrifugation  is  currently  used  in   a
                               195

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            GENERAL DEVELOPMENT DOCUMENT
                                            SECT - VII
 great  many  commercial  applications to dewater  sludge.   Work  is
 underway to improve the efficiency,  increase   the  capacity,  and
 lower the costs associated with centrifugation.

 10.  Coalescing

 The   basic  principle  of  coalescence  involves  the  preferential
 wetting of a coalescing medium by oil droplets which  accumulate
 on   the  medium  and  then rise to the surface of the solution  as
 they^combine  to  form  larger  particles.    The   most important
 requirements  for  coalescing   media  are wettability for  oil and
 large surface area.   Monofilament line is  sometimes   used as  a
 coalescing medium.

 Coalescing  stages   may  be integrated  with a   wide variety  of
 gravity oil separation devices,  and  some systems  may   incorporate
 several   coalescing  stages.    In  general,   a   preliminary  oil
 skimming step is desirable to  avoid  overloading the coalescer.

 One   commercially  marketed system   for oily waste  treatment
 combines   coalescing   with    inclined  plate    separation  and
 filtration.   In  this  system,   the   oily  wastes  flow into   an
 inclined  plate  settler.   This   unit  consists   of   a stack  of
 inclined baffle plates in a cylindrical  container  with   an  oil
 collection chamber  at the top.   The  oil droplets  rise and  impinge
 upon the undersides  of the plates.   They then migrate upward to a
 guide   rib  which  directs the  oil to the oil collection chamber,
 from which oil  is discharged for  reuse or disposal.

 The  oily water  continues  on through  another   cylinder   containing
 replaceable   filter   cartridges,  which remove suspended particles
 from the  waste.    From  there   the   wastewater   enters  a  final
 cylinder in  which the coalescing  material is  housed.   As the oily
 water   passes   through  the many small,   irregular,   continuous
 passages in  the coalescing material,  the  oil  droplets  coalesce
 and  rise to  an  oil  collection chamber.

 Application  and  Performance.    Coalescing is used to  treat oily
 wastes  which do not  separate readily  in  simple  gravity  systems.
 The  three-stage  system   described   above  has achieved effluent
 concentrations  of 10  to 15  mg/1 oil and  grease  from   raw   waste
 concentrations  of 1000 mg/1 or more.
Advantages  _
droplets  too
            and  Limitations.   Coalescing  allows removal of oil
                finely   dispersed   for   conventional   gravity
separation-skimming technology.  It also can significantly reduce
   ^ residence times (and therefore separator volumes) required to
achieve  separation  of  oil  from  some  wastes.  Because of its
simplicity, coalescing provides generally  high  reliability  and
low  capital  and  operating  costs.  Coalescing is not generally
effective in removing soluble or chemically. stabilized emulsified
oils.   To  avoid  plugging,  coalescers  must  be  protected  by
pretreatment from very high concentrations of free oil and grease
and  suspended solids.  Frequent replacement of pref liters may be
necessary when raw waste oil concentrations are high.
                               196

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           GENERAL DEVELOPMENT DOCUMENT
       SECT - VII
Operational  Factors.   Reliability:  Coalescing  is   inherently
highly  reliable  since  there  are  no  moving  parts,  and  the
coalescing  substrate  ( monof i lament,  etc. )    is  inert  in  the
process  and  therefore  not  subject to frequent regeneration or
replacement   requirements.    Large    loads    or    inadequate
pretreatment,  however,  may  result  in  plugging  or  bypass of
coalescing stages.

Maintainability: Maintenance requirements are  generally  limited
to replacement of the coalescing medium on an infrequent basis.

Solid  Waste  Aspects: No appreciable solid waste is generated by
this process.

Demonstration Status.  Coalescing has been fully demonstrated  in
industries   generating   oily   wastewater,   although  none  are
currently  in  use  at  any   nonferrous   metals   manufacturing
facilities.

11. Cyanide Oxidation by Chlorine


Cyanide  oxidation  using  chlorine  is widely used in industrial
waste treatment to oxidize cyanide.  Chlorine can be utilized  in
either   the  elemental  or  hypochlorite  forms.   This  classic
procedure can be illustrated by the following two  step  chemical
reaction:
       + NaCN + 2NaOH ---- > NaCNO

2.  3C12 + 6NaOH + 2NaCNO ---- >
2NaCl + H20

   + N2 + 6NaCl
                                                      2H20
The reaction presented as Equation 2 for the oxidation of cyanate
is the final step in the oxidation of cyanide.  A complete' system
for  the alkaline chlorination of cyanide is shown in Figure VII-
19 (page 272) .


The alkaline chlorination process  oxidizes  cyanides  to  carbon
dioxide  and  nitrogen.   The  equipment  often  consists  of  an
equalization tank followed by two reaction  tanks/  although  the
reaction  can  be carried out in a single tank.  Each tank has an
electronic recorder-controller to  maintain  required  conditions
with  respect  to pH and oxidation reduction potential (ORP) .  In
the first reaction  tank,  conditions  are  adjusted  to  oxidize
cyanides  to  cyanates.   To  effect  the  reaction,  chlorine is
metered to the reaction tank as required to maintain the  ORP  in
the  range  of  350  to  400  millivolts,  and 50 percent aqueous
caustic soda is added to maintain a pH range of 9.5  to  10.   In
the  second  reaction  tank, conditions are maintained to oxidize
cyanate to carbon dioxide and nitrogen.  The desirable , ORP and pH
for this reaction are 600 millivolts and a pH of  8.0.   Each  of
                               197

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            GENERAL  DEVELOPMENT  DOCUMENT
                                            SECT  - VII
 the  reaction  tanks  is  equipped with  a  propeller agitator  designed
 to   provide   approximately  one turnover per minute.  Treatment  by
 the  batch process is accomplished  by using  two   tanks,   one  for
 collection of water over a  specified time period, and  one for the
 treatment  of  an   accumulated  batch.   If dumps of concentrated
 wastes  are frequent, another  tank  may  be required to equalize the
 flow to the treatment  tank.   When  the  holding  tank is  full,  the
 liquid   is transferred to the reaction tank for treatment.  After
 treatment, the  supernatant  is discharged  and the  sludges  are
 collected for removal  and ultimate disposal.
Application  and  Performance.
chlorine  is a classic process and  is
                                The oxidation of cyanide waste by
                                      found  in  most   industrial
                                process   is  capable of achieving
plants  using  cyanide.   This
effluent  levels  that  are  nondetectable.

Advantages  and  Limitations.   Some   advantages   of   chlorine
oxidation for handling process effluents are operation at ambient
temperature,  suitability  for  automatic  control, and low cost.
Disadvantages include the need for careful pH  control,  possible
chemical  interference  in the treatment of mixed wastes, and the
potential hazard of storing and handling chlorine gas.

Operational Factors.  Reliability:  Chlorine oxidation is  highly
reliable  'with   proper   monitoring   and  control  and  proper
pretreatment to control interfering substances.
Maintainability:  Maintenance consists  of
sludge and recalibration of instruments.
                                            periodic  removal  of
Solid  Waste Aspects:  There is no solid waste problem associated
with chlorine oxidation.
Demonstration  Status.   The  oxidation  of  cyanide  wastes   by
chlorine  is  a  widely  used  process in plants using cyanide in
cleaning and metal processing baths.   Alkaline  chlorination  is
also used for cyanide treatment in a number of inorganic chemical
facilities producing hydrocyanic^acid and various metal  cyanides.

12. Cyanide Oxidation By Ozone

Ozone is a highly reactive oxidizing agent which is approximately
ten  times  more  soluble than oxygen on a weight basis in water.
Ozone  may  be  produced  by  several  methods,  but  the  silent
electrical  discharge  method  is  predominant in the field.  The
silent electrical discharge process  produces  ozone  by  passing
oxygen  or  air  between  electrodes  separated  by an insulating
material.  A complete ozonation system is represented  in  Figure
VII-20 (page 273) .

                    Performance.
Application   and
commercially
organometal   complexes.
         	     Ozonation  has  been  applied
to  oxidize  cyanides,   phenolic  chemicals,   and
            Its  applicability  to    photographic
wastewaters  has   been   studied' in  the  laboratory  with  good
results.   Ozone is used in industrial waste treatment  primarily
                               198

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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 to  oxidize  cyanide to  cyanate  and  to  oxidize  phenols
 dyes to a variety of colorless nontoxic products.

 Oxidation of cyanide to cyanate is illustrated below:
                   and
 CN- + 03 	> CNO- +02

 Continued exposure to ozone will convert the  cyanate  formed  to
 carbon  dioxide  and  ammonia;   however, this is not economically
 practical.

 Ozone oxidation of cyanide to cyanate requires 1.8 to 2.0  pounds
 ozone  per  pound  of CN ; complete oxidation requires 4.6 to 5.0
 pounds  ozone  per pound  of  CN .     Zinc,   copper,  and  nickel
 cyanides  are  easily destroyed to  a nondetectable   level,   but
 cobalt  and iron cyanides are more  resistant to ozone  treatment.

 Advantages  and  Limitations.   Some advantages of ozone oxidation
 for handling process effluents  are  its suitability  to  automatic
 control  and  on-site  generation  and  the   fact  that  reaction
 products are not chlorinated organics and no dissolved solids are
 added in the treatment step.  Ozone in the presence of  activated
 carbon,   ultraviolet,  and  other   promoters  shows  promise  of
 reducing reaction time and improving ozone utilization,   but   the
 process  at  present is limited by  high capital expense,  possible
 chemical interference in the treatment of mixed  wastes,   and  an
 energy  requirement   of 25 kwh/kg of ozone generated.   Cyanide is
 not economically oxidized beyond the cyanate form.

 Operational Factors.   Reliability:    Ozone  oxidation   is   highly
 reliable   with   proper   monitoring  and  control,   and   proper
 pretreatment to control interfering substances.

 Maintainability:   Maintenance consists   of  periodic   removal   of
 sludge,   and periodic renewal of  filters  and desiccators  required
 for  the input  of  clean dry air;  filter   life  is  a  function   of
 input  concentrations  of detrimental  constituents.

 Solid   Waste Aspects:   Pretreatment  to  eliminate  substances which
 will interfere  with  the  process may  be  necessary.  Dewatering   of
 sludge   generated  in   the  ozone   oxidation process or in an  "in
 line" process may  be  desirable prior  to disposal.

 13. Cyanide Oxidation  By_ Ozone With  UV Radiation

One  of   the  modifications  of  the  ozonation  process  is   the
 simultaneous  application  of ultraviolet  light and ozone for  the
 treatment  of  wastewater,  including  treatment  of  halogenated
organics.   The  combined  action  of  these  two  forms produces
 reactions  by  photolysis,   photosensitization,   hydroxyla.tion,-
oxygenation,  and  oxidation.   The  process  is  unique  because
several  reactions and  reaction species are active simultaneously.

Ozonation is facilitated by ultraviolet absorption  because  both
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
the  ozone  and  the  reactant  molecules  are raised to a higher
energy state so that they react more rapidly.  In addition,  free
radicals  for  use  in the reaction are readily hydrolyzed by the
water present.  The energy and reaction intermediates created  by
the introduction of both ultraviolet and ozone greatly reduce the
amount  of  ozone  required  compared  with  a system using ozone
alone.  Figure VII-21 (page 274)  shows  a  three-stage  UV-ozone
system.   A  system to treat mixed cyanides requires pretreatment
that involves chemical coagulation, sedimentation, clarification,
equalization, and pH adjustment.

Application and Performance.  The ozone-UV radiation process  was
developedprimarily  for cyanide treatment in the electroplating
and color  photo-processing  areas.   It  has  been  successfully
applied  to  mixed  cyanides  and organics from organic chemicals
manufacturing processes.  The process is particularly useful  for
treatment  of  complexed  cyanides  such  as ferricyanide, copper
cyanide,  and nickel cyanide, which are resistant to ozone alone.

14. Cyanide Oxidation By_ Hydrogen Peroxide

Hydrogen peroxide oxidation removes both cyanide  and  metals  in
cyanide containing wastewaters.  In this process, cyanide bearing
waters   are  heated  to 49 to  54° C  (120 to 130°F) and the pH is
adjusted to 10.5 to 11.8.   Formalin  (37 percent  formaldehyde) is
added  while  the  tank  is  vigorously  agitated.     After 2 to
5   minutes,   a proprietary peroxygen compound     (41  _  percent
hydrogen  peroxide   with  a catalyst and  additives)  is  added.
After an hour of mixing,  the  reaction is complete.   The cyanide
is  converted  to cyanate,  and the metals   are   precipitated  as
oxides  or hydroxides.  The metals are then  removed from solution
by  either  settling  or filtration.

The main equipment required for this  process  is  two holding  tanks
equipped  with  heaters  and air spargers or mechanical stirrers.
These  tanks may be used in a batch or  continuous  fashion,  with
one  tank  being  used  for  treatment  while   the  other  is  being
filled.  A settling  tank or a  filter  is needed to concentrate  the
precipitate.

Application  and Performance.    The  hydrogen  peroxide  oxidation
process  is applicable  to cyanide-bearing wastewaters,   especially
those  containing  metal-cyanide  complexes.    In  terms  of  waste
reduction performance,  this process can  reduce total   cyanide   to
less  than  0.1 mg/1  and  the  zinc or  cadmium  to  less  than 1.0  mg/1.

Advantages   and Limitations.   Chemical  costs are similar  to  those
 for alkaline chlorination  using chlorine and lower  than those  for
 treatment  with hypochlorite.   All   free  cyanide  reacts   and   is
 completely    oxidized   to   the  less   toxic  cyanate   state.    In
addition,  the metals precipitate and  settle quickly,  and  they_may
 be recoverable in many instances.   However,  the process   requires
 energy expenditures  to heat  the wastewater  prior to treatment.

 Demonstration  Status.    This  treatment  process was introduced in
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           GENERAL DEVELOPMENT  DOCUMENT
SECT - VII
 1971 and  is used  in  several   facilities.    No   nonferrous  metals
 manufacturing plants are  known  to  use  oxidation by  hydrogen peroxide,

 15. Evaporation

 Evaporation is a  concentration  process.  Water  is evaporated  from
 a  solution,  increasing   the  concentration  of solute   in   the
 remaining solution.  If the  resulting  water vapor   is  condensed
 back  to  liquid  water,   the evaporation-condensation process  is
 called distillation.  However,  to  be  consistent   with  industry
 terminology,  evaporation is  used  in this  report to describe  both
 processes.  Both  atmospheric  and vacuum evaporation are  commonly
 used  in  industry   today.    Specific  evaporation  techniques  are
 shown in Figure VII-22  (page  275)  and  discussed below.

 Atmospheric evaporation could be accomplished simply by   boiling
 the  liquid.   However,   to   aid   evaporation,   heated  liquid  is
 sprayed on an evaporation surface, and air is blown  over   the
 surface  and  subsequently   released   to   the   atmosphere.  Thus,
 evaporation occurs by humidification of the air stream,   similar
 to  a  drying  process.    Equipment  for carrying out atmospheric
 evaporation is quite similar  for most  applications.   The  major
 element  is generally a packed  column  with  an accumulator  bottom.
 Accumulated wastewater is pumped from  the   base of  the   column,
 through  a  heat  exchanger,  and back  into  the  top  of the  column,
 where it is sprayed  into  the  packing.   At  the same  time,  air
 drawn  upward  through  the   packing   by  a fan is heated as  it
 contacts the hot  liquid.   The  liquid partially   vaporize's  and
 humidifies the air stream.  The fan then blows  the  hot, humid air
 to  the  outside  atmosphere.   A  scrubber  is  often unnecessary
 because the packed column itself acts  as a  scrubber.

 Another form of atmospheric evaporator  also  works  on  the  air
 humidification  principle,  but the evaporated  water is recovered
 for reuse by condensation.  These air  humidification  techniques
 operate  well  below  the  boiling point of water and can utilize
 waste process heat to supply  the energy required.

 In vacuum evaporation, the evaporation  pressure  is  lowered   to
 cause  the  liquid  to  boil  at reduced temperature.  All of the
 water vapor is condensed,  and to maintain the   vacuum  condition,
 noncondensible  gases (air in particular)  are removed by a vacuum
 pump.  Vacuum evaporation may be either single or double  effect.
 In  double  effect evaporation,  two evaporators  are used,  and the
 water vapor from the first evaporator  (which  may  be  heated  by
 steam)   is  used  to supply heat to the second evaporator.   As it
 supplies  heat,   the  water  vapor  from  the   first   evaporator
 condenses.   Approximately  equal  quantities  of  wastewater are
 evaporated  in  each  unit;   thus,  the  double   effect   system
 evaporates  twice the amount of  water  that a single effect  system
 does, at nearly the same cost in energy but  with  added  capital
 cost   and   complexity.    The    double   effect   technique  is
 thermodynamically  possible  because   the   second  evaporator  is
maintained  at  lower  pressure   (higher  vacuum) and,  therefore,
 lower evaporation temperature.  Vacuum evaporation equipment  may
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
be  classified  as  submerged  tube  or climbing film evaporation
units.

Another  means  of  increasing   energy   efficiency   is   vapor
recompression  evaporation,  which enables heat to be transferred
from the condensing water vapor to  the  evaporating  wastewater.
Water  vapor generated from incoming wastewaters flows to a vapor
compressor.   The  compressed  steam  than  travels  through  the
wastewater  via an enclosed tube or coil in which it condenses as
heat is transferred to the surrounding solution.   In  this  way,
the   compressed   vapor  serves  as  a  heating  medium.   After
condensation, this distillate is drawn off  continuously  as  the
clean  water  stream.  The heat contained in the compressed vapor
is used to heat the  wastewater,  and  energy  costs  for  system
operation are reduced.

In  the most commonly used submerged tube evaporator, the heating
and condensing coil are contained in a single  vessel  to  reduce
capital  cost.   The  vacuum  in  the  vessel is maintained by an
eductor-type pump, which creates the required vacuum by the  flow
of  the  condenser  cooling  water through a venturi.  Wastewater
accumulates in the bottom of the vessel, and it is evaporated  by
means  of  submerged  steam  coils.   The  resulting  water vapor
condenses as it contacts the condensing coils in the top  of  the
vessel.   The condensate then drips off the condensing coils into
a  collection  trough  that  carries  it  out  of   the   vessel.
Concentrate is removed from the bottom of the vessel.

The  major  elements  of  the  climbing  film  evaporator are the
evaporator, separator, condenser, and vacuum pump.  Wastewater is
"drawn" into the system by the vacuum so that a  constant  liquid
level  is  maintained in the separator.  Liquid enters the steam-
jacketed evaporator tubes, and part of it evaporates  so  that  a
mixture  of vapor and liquid enters the separator.  The design of
the separator is such that the liquid is continuously  circulated
from  the  separator  to  the evaporator.  The vapor entering the
separator flows out through a mesh entrainment separator  to  the
condenser,  where  it  is  condensed as it flows down through the
condenser tubes.  The condensate, along with any  entrained  air,
is  pumped  out  of  the bottom of the condenser by a liquid ring
vacuum pump.  The liquid seal provided by  the  condensate  keeps
the vacuum in the system from being broken.

Application   and   Performance.   Both  atmospheric  and  vacuum
evaporation are used in many industrial plants,  mainly  for  the
concentration  and  recovery of process solutions.  Many of these
evaporators also recover water for rinsing.  Evaporation has also
been applied to recovery of phosphate metal cleaning solutions.

In theory, evaporation should yield a concentrate and a deionized
condensate.  Actually,  carry-over  has  resulted  in  condensate
metal concentrations as high as 10 mg/1, although the usual level
is  less  than  3  mg/1,  pure enough for most final rinses.  The
condensate may also contain organic brighteners  and  antifoaming
agents.   These  can  be removed with an activated carbon bed, if
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
necessary.  Samples from one plant showed 1,900 mg/1 zinc in  the
feed,  4,570  mg/1  in  the  concentrate,  and  0.4  mg/1  in the
condensate.  Another plant had 416 mg/1 copper in  the  feed  and
21,800 mg/1 in the concentrate.  Chromium analysis for that plant
indicated  5,060  mg/1  in  the  feed  and  27,500  mg/1  in  the
concentrate.  Evaporators are available in a range of capacities,
typically from 15  to  75  gph,  and  may  be  used  in  parallel
arrangements for processing of higher flow rates.

Advantages   and  Limitations.   Advantages  of  the  evaporation
process are that it permits recovery of a wide variety of process
chemicals, and it is often applicable to concentration or removal
of compounds which cannot be accomplished  by  any  other  means.
The  major  disadvantage is that the evaporation process consumes
relatively large amounts of energy for the evaporation of  water.
However,   the  recovery  of  waste  heat  from  many  industrial
processes (e.g., diesel  generators,  incinerators,  boilers  and
furnaces)  should  be  considered  as a source of this heat for a
totally integrated evaporation system.  Also, in some cases solar
heating  could  be  inexpensively  and  effectively  applied   to
evaporation   units.    Capital   costs   for  vapor  compression
evaporators are substantially higher  than  for  other  types  of
evaporation equipment.  However, the energy costs associated with
the operation of a vapor compression evaporator are significantly
lower   than   costs   of   other  evaporator  types.   For  some
applications, pretreatment may be required to  remove  solids  or
bacteria  which  tend  to  cause  fouling  in  the  condenser  or
evaporator.    The  build-up  of   scale   on   the    evaporator
surfaces  reduces   the   heat   transfer  efficiency   and   may
present   a  maintenance  problem  or  increase  operating  cost.
However,  it   has been  demonstrated that fouling  of  the  heat
transfer  surfaces can be  avoided  or  minimized   for   certain
dissolved    solids    by  maintaining   a   seed  slurry   which
provides  preferential  sites  for  precipitate  deposition.   In
addition, low temperature differences in  the  evaporator    will
eliminate    nucleate   boiling   and  supersaturation   effects.
Steam  distillable  impurities in the process stream are  carried
over with the product water  and  must be handled by pre-or  post
treatment.

Operational   Factors.   Reliability:   Proper  maintenance  will
ensure a high degree of reliability for the system.  Without such
attention, rapid fouling or deterioration  of  vacuum  seals  may
occur, especially when corrosive liquids are handled.

Maintainability:    Operating  parameters  can  be  automatically
controlled.  Pretreatment may be required, as  well  as  periodic
cleaning of the system.  Regular replacement of seals, especially
in a corrosive environment, may be necessary.

Solid  Waste  Aspects:   With  only a few exceptions, the process
does not generate appreciable quantities of solid waste.
Demonstration  Status.   Evaporation  is
    fully
commercially  available  wastewater treatment system.
developed,
It is used
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
extensively to recover plating chemicals  in  the  electroplating
industry, and a pilot-scale unit has been used in connection with
phosphating  of  aluminum.  Proven performance in silver recovery
indicates that evaporation could be a useful treatment  operation
for  the  photographic  industry, as well as for metal finishing.
Vapor compression evaporation has been  practically  demonstrated
in a number of industries, including chemical manufacturing, food
processing, pulp and paper, and metal working.

16. Flotation

Flotation  is  the  process  of  causing  particles such as metal
hydroxides or oil to float to the surface of a  tank  where  they
can  be  concentrated  and  removed.   This  is  accomplished  by
releasing gas  bubbles  which  attach  to  the  solid  particles,
increasing   their  buoyancy  and  causing  them  to  float.   In
principle, this process is the opposite of sedimentation.  Figure
VII-23 (page 276) shows one type of flotation system.

Flotation is  used  primarily  in  the  treatment  of  wastewater
streams that carry heavy loads of finely divided suspended solids
or  oil.   Solids having a specific gravity only slightly greater
than 1.0,  which  would  require  abnormally  long  sedimentation
times,  may be removed in much less time by flotation.  Dissolved
air flotation is of greatest interest in removing oil from  water
and is less effective in removing heavier precipitates.

This  process  may be performed in several ways:  foam, dispersed
air, dissolved air, gravity, and vacuum flotation  are  the  most
commonly  used  techniques.  Chemical additives are often used to
enhance the performance of the flotation process.

The principal difference among types of flotation is  the  method
of   generating  the  minute  gas  bubbles  (usually  air)  in  a
suspension of water and small particles.  Chemicals may  be  used
to  improve  the  efficiency  with any of the basic methods.  The
following paragraphs describe the different flotation  techniques
and the method of bubble generation for each process.

Froth  Flotation - Froth flotation is based on differences in the
physiochemical properties in various particles.  Wettability  and
surface  properties  affect  the  particles'  ability  to  attach
themselves to  gas  bubbles  in  an  aqueous  medium.   In  froth
flotation, air is blown through the solution containing flotation
reagents.   The  particles with water repellant surfaces stick to
air bubbles as they rise and  are  brought  to  the  surface.   A
mineralized  froth  layer, with mineral particles attached to air
bubbles, is  formed.   Particles  of  other  minerals  which  are
readily wetted by water do not stick to air bubbles and remain in
suspension.

Dispersed Air Flotation - In dispersed air flotation, gas bubbles
are  generated  by  introducing  the  air  by means of mechanical
agitation with impellers or by forcing air through porous  media.
Dispersed  air  flotation  is  used  mainly  in the metallurgical
                               204

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
industry.
       i
Dissolved Air Flotation - In dissolved air flotation, bubbles are
produced by releasing air from a  supersaturated  solution  under
relatively high pressure.  There are two types of contact between
the  gas bubbles and particles.  The first type is predominant in
the  flotation  of  flocculated  materials   and   involves   the
entrapment  of rising gas bubbles in the flocculated particles as
they increase in size.  The bond between the bubble and  particle
is  one  of physical capture only.  The second type of contact is
one  of  adhesion.   Adhesion  results  from  the  intermolecular
attraction  exerted  at  the interface between the solid particle
and gaseous bubble.

Vacuum Flotation -  This  process  consists  of  saturating  the
wastewater  with  air  either directly in an aeration tank, or by
permitting air to enter on the suction of a wastewater  pump.   A
partial vacuum is applied, which causes the dissolved air to come
out  of  solution as minute bubbles.  The bubbles attach to solid
particles and rise to the,surface to form a scum  blanket,  which
is  normally  removed  by  a  skimming mechanism.  Grit and other
heavy solids that settle to the bottom are generally raked  to  a
central sludge pump for removal.  A typical vacuum flotation unit
consists  of a covered cylindrical tank in which a partial vacuum
is maintained.  The tank is equipped with scum and sludge removal
mechanisms.  The floating material is continuously swept  to  the
tank  periphery, automatically discharged into a scum trough, and
removed from the unit  by  a  pump  also  under  partial  vacuum.
Auxiliary  equipment includes an aeration tank for saturating the
wastewater with air, a tank  with  a  short  retention  time  for
removal of large bubbles, vacuum pumps, and sludge pumps.

Application and Performance.  The primary variables for flotation
design  are  pressure,  feed  solids concentration, and retention
period.  The suspended solids, in the effluent decrease,  and  the
concentration  of  solids  in the float increases with increasing
retention period.  When the flotation process is ' used  primarily
for clarification, a retention period .of 20 to 30 minutes usually
is adequate for separation and concentration.

Advantages   and  Limitations.  Some  advantages of the  flotation
process are the high levels of solids separation achieved in many
applications, the relatively low  energy  requirements,  and  the
adaptability  to  meet  the  treatment  requirements of different
waste types.  Limitations of flotation are that it often requires
addition of chemicals to enhance process performance and that  it
generates large quantities of solid waste.

Operational. Factors.   .Reliability:   Flotation systems normally
are very reliable with proper maintenance of the sludge collector-
mechanism and the motors and pumps used for aeration.

Maintainability:  Routine maintenance is required  on  the  pumps
and  motors.   The  sludge  collector  mechanism  is  subject  to
possible  corrosion  or  breakage  and   may   require   periodic
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
replacement.

Solid  Waste  Aspects:   Chemicals  are  commonly used to aid the
flotation process by creating a surface or a structure  that  can
easily  adsorb  or entrap air bubbles.  Inorganic chemicals, such
as the aluminum and ferric salts, and activated silica, can  bind
the  particulate  matter together and create a structure that can
entrap air bubbles.  Various organic  chemicals  can  change  the
nature  of  either  the  air-liquid interface or the solid-liquid
interface, or both.   These  compounds  usually  collect  on  the
interface   to  bring  about  the  desired  changes.   The  added
chemicals plus the particles in solution combine to form a  large
volume  of  sludge  which  must  be  further  treated or properly
disposed.

Demonstration Status.  Flotation is a fully developed process and
is readily available for the  treatment  of  a  wide  variety  of
industrial    waste    streams.     Flotation    separation    is
demonstrated  in  one primary aluminum  plant,  namely,  at the a
smelter as a part of a system for oil removal.

17. Gravity Sludge Thickening

In the gravity thickening process, dilute sludge is  fed  from  a
primary  settling  tank  or  clarifier to a thickening tank where
rakes stir the sludge gently to densify it and to push  it  to  a
central  collection  well.   The  supernatant  is returned to the
primary settling tank.  The thickened sludge that collects on the
bottom of the tank is pumped to dewatering  equipment  or  hauled
away.   Figure  VII-24  (page 277)  shows  the construction of  a
gravity thickener.

Application and Performance.  Thickeners are  generally  used  in
facilities  where  the  sludge  is  to  be further dewatered by a
compact mechanical device such as a vacuum filter or  centrifuge.
Doubling  the  solids  content  in  the  thickener  substantially
reduces capital and operating cost of the  subsequent  dewatering
device  and  also  reduces  cost  for  hauling.   The  process is
potentially applicable to almost any industrial plant.

Organic sludges from sedimentation units of one  to  two  percent
solids  concentration  can usually be gravity thickened to six to
ten percent; chemical sludges can be thickened  to  four  to  six
percent.

Advantages and Limitations.   The principal advantage of a gravity
sludge  thickening  process is that it facilitates further sludge
dewatering.  Other advantages are high  reliability  and  minimum
maintenance requirements.

Limitations  of the sludge thickening process are its sensitivity
to the flow rate through the thickener  and  the  sludge  removal
rate.   These  rates  must  be  low  enough  not  to  disturb the
thickened sludge.
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           GENERAL DEVELOPMENT DOCUMENT
                                            SECT - VII
Operational Factors.   Reliability:   Reliability  is  high  with
proper  design and operation.  A gravity thickener is designed on
the basis of square feet per pound of solids per  day,  in  which
the  required  surface area is related to the solids entering and
leaving the unit.  Thickener area requirements are also expressed
in terms of mass loading, grams of solids per  square  meter  ner
day (.lbs/sq f t/day).                                            .

Maintainability:  Twice a year, a thickener must be shut down for
lubrication of the drive mechanisms.  Occasionally, water must be
pumped back through the system in order to clear sludge pipes.

Solid  Waste Aspects:   Thickened sludge from a gravity thickening
process  will  usually  require  further  dewatering   prior   to
disposal,  incineration,  or  drying.   The clear effluent may be
recirculated in part,  or it may be subjected to further treatment
prior to discharge.
               Status.    Gravity  sludge  thickeners   are   used
 Demonstration   	          ^     ...__   	    	    	^
 throughout   industry  to  reduce  water  content  to  a  level where the
 sludge  may  be  efficiently  handled.  Further dewatering  is usually
 practiced to minimize costs  of  hauling  the   sludge   to approved
 landfill areas.

 18.  Insoluble  Starch  Xanthate

 Insoluble   starch  xanthate  is  essentially an ion  exchange  medium
 used to remove dissolved heavy  metals from wastewater.   The water
 may  then either be reused  (recovery  application)  or   discharged
 (end-of-pipe   application).    In  a  commercial   electroplating
 operation,   starch xanthate  is  coated on a filter  medium.    Rinse
 water   containing  dragged   out  heavy  metals   is     circulated
 through  the   filters   and then  reused    for   rinsing.    The
 starch-heavy  metal  complex   is  disposed   of    and    replaced
 periodically.    Laboratory  tests  indicate   that   recovery   of
 metals  from  the complex  is feasible, with regeneration  of  the
 starch   xanthate.    Besides electroplating,  starch xanthate   is
 potentially  applicable  to  any other  industrial  plants   where
 dilute  metal  wastewater streams are generated.  Its present  use
 is   limited  to  one  electroplating plant.

 19.  Ion Exchange


 Ion  exchange  is  a process in which ions, held by electrostatic
 forces  to charged functional groups on the  surface  of  the   ion
 exchange resin, are exchanged for ions of similar charge from  the
 solution in which the resin  is immersed.  This is classified as a
 sorption  process  because  the exchange occurs on the surface of
 the  resin,  and the exchanging ion must undergo a  phase  transfer
 from  solution phase to solid phase.   Thus, ionic contaminants in
 a waste stream can be exchanged for  the  harmless  ions  of   the
 resin.

Although the precise technique may vary slightly according to  the
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
application  involved, a generalized process description follows.
The wastewater stream being treated passes through  a  filter  to
remove  any  solids,  then flows through a cation exchanger which
contains the ion exchange resin.  Here, metallic impurities  such
as copper, iron, and trivalent chromium are retained.  The stream
then passes through the anion exchanger and its associated resin.
Hexavalent  chromium,.for example, is retained in this^stage.  If
one pass does not reduce the contaminant levels sufficiently, the
stream may then enter another series  of  exchangers.   Many  ion
exchange   systems  are  equipped  with  more  than  one  set  of
exchangers  for  this reason.   A strongly basic  anion  exchange
resin may be used alone to remove precious metals,  such as gold,
palladium and platinum.

The other major portion of the ion exchange process concerns  the
regeneration  of  the  resin,  which  now  holds those impurities
retained from the waste stream.  An ion exchange  unit  with  in-
place  regeneration  is shown in Figure VII-25 (page 278).  Metal
ions such as nickel are  removed  by  an  acid,  cation  exchange
resin,  which  is regenerated with hydrochloric or sulfuric acid,
replacing the metal ion with one or more hydrogen  ions.   Anions
such  as dichromate are removed by a basic, anion exchange resin,
which is regenerated with sodium hydroxide, replacing  the  anion
with  one  or  more  hydroxyl  ions.  The three principal methods
employed by industry for regenerating the spent resin are:

A) Replacement Service:   A  regeneration  service   replaces  the
spent  resin  with  regenerated  resin, and regenerates the spent
resin at its own facility.  The service then has the  problem  of
treating and disposing of the spent regenerant.

B)  In-Place  Regeneration:  Some establishments may find  it less
expensive to do their own regeneration.  The spent   resin  column
is  shut  down  for  perhaps  an  hour,  and   the  spent  resin is
regenerated.  This  results in one or  more  waste  streams  which
must  be  treated   in  an  appropriate  manner.   Regeneration is
performed as the resins require it, usually every few months.

C) Cyclic Regeneration:  In  this process, the  regeneration of the
spent resins takes  place within the ion exchange unit   itself  in
alternating  cycles with the ion  removal process.  A regeneration
frequency of twice  an hour is  typical.   This  very  short   cycle
time  permits   operation  with  a  very  small quantity of resin and
with  fairly concentrated solutions, resulting  in a   very   compact
system.  Again, this  process varies according  to application, but
the regeneration cycle generally  begins with caustic being pumped
through   the  anion  exchanger, carrying out hexavalent chromium,
for example, as sodium dichromate.  The sodium dichromate stream
then  passes  through a   cation  exchanger, converting  the sodium
dichromate  to chromic  acid.  After  concentration  by  evaporation
or  other   means,  the chromic  acid  can be  returned  to  the process
line.   Meanwhile,   the  cation  exchanger  is  regenerated  with
sulfuric  acid,   resulting   in a  waste acid stream  containing the
metallic  impurities removed   earlier.   Flushing   the   exchangers
with  water  completes  the cycle.   Thus,  the  wastewater  is  purified
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
and,  in  this  example,  chromic  acid  is  recovered.   The ion
exchangers, with newly regenerated  resin,  then  enter  the  ion
removal cycle again.

Application  and  Performance.   The list of pollutants for which
the ion exchange system has proved effective  includes  aluminum,
arsenic,  cadmium,  chromium  (hexavalent and trivalent), copper,
cyanide,   gold,   iron,   lead,  manganese,  nickel,  palladium,
platinum, selenium,  silver, tin,  zinc,  arid more.  Thus, it can
be applied to a wide variety of industrial concerns.   Because of
the  heavy  concentrations  of metals  in  their wastewater,  the
metal finishing industries utilize ion exchange in several  ways.
As  an  end-of-pipe   treatment,   ion   exchange  is   certainly
feasible, but its greatest value is in recovery applications.  It
is   commonly   used  as  an  integrated treatment   to   recover
rinse    water  and  process  chemicals.    Some   electroplating
facilities   use  ion   exchange   to   concentrate   and  purify
plating  baths.   Also,  many industrial  concerns,  including  a
number  of  nonferrous  metals  manufacturing  plants,   use  ion
exchange to reduce salt concentrations in incoming water sources.

The  ion  exchange  process  may  be  used to remove cyanide in a
ferrocyanide complex from wastewater.  The  process  generates  a
concentrated  stream  of  the complex, which may be treated using
cyanide precipitation.

Ion exchange is applicable to cyanide removal when the cyanide is
complexed  with  iron.   Experimental  data  have  shown  that  a
specific  resin  (Rohm  & Haas IRA-958) is very selective to  the
removal of iron cyanide complexes.  The process  described  below
is  based  on  the  use  of  this  resin  and upon operating data
obtained from  the  vendor  and  from  an  actual  operating  ion
exchange facility.

Two  downflow  columns  are  used.  The columns are operated in a
merry-go-round  configuration (see the granular activated  carbon
adsorption process description in this section for  a  discussion
on this type of operation).  The.regeneration step is carried out
in  two  stages.   The first step uses regeneration solution from
the previous second regeneration  step.   The  second  step  uses
fresh  regeneration  solution.   This  is  done  because  a large
majority of the pollutant ions are eluted in the first step.  The
solution used in the second step yields a dilute solution of  the
pollutant  and  can  be  used  in  the  first  step  of  the next
regeneration cycle.  Separation of the regeneration  solution  in
this  manner  results  in  a  50  percent savings in regeneration
solution costs and a more concentrated product.  The regeneration
solution used is 15 percent brine (NaCl).

Unless the cyanide in the influent is already in complexed  form,
the wastewater must be treated to convert the : free cyanide to the
ferrocyanide complex.

The spent brine solution produced in the regeneration step may be
disposed   of   as   a   hazardous   waste  or   sent  to  cyanide
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           GENERAL DEVELOPMENT DOCUMENT
                 SECT - VII
precipitation.  In this module the cyanide  complex  is  combined
with more iron at low pH to produce an insoluble complex.

Ion exchange is highly  efficient  at  recovering  metal  bearing
solutions.  Recovery of chromium, nickel, phosphate solution, and
sulfuric  acid  from  anodizing  is  commercial.   A chromic acid
recovery  efficiency  of  99.5  percent  has  been  demonstrated.
Typical  data  for purification of rinse water have been reported
and are displayed in Table VII-25 (page 251).  Sampling  at   one
nonferrous  metals  manufacturing  plant  characterized  influent
and effluent streams for an ion exchange unit on a silver bearing
waste.   This  system was in start-up at the  time  of  sampling,
however, and  was not found to be operating effectively.

Advantages   and   Limitations.   Ion  exchange  is  a  versatile
technology  applicable  to  a  great   many   situations.    This
flexibility, along with its compact nature and performance, makes
ion  exchange  a  very  effective me'thod of wastewater treatment.
However, the resins in these systems can prove to be  a  limiting
factor.  The thermal limits of the anion resins, generally in the
vicinity    of    60°C,    could  prevent  its  use  in   certain
situations.  Similarly,  nitric acid,  chromic acid, and hydrogen
peroxide  can all  damage  the resins,  as will iron,  manganese,
and  copper  when present  with  sufficient   concentrations   of
dissolved  oxygen.  Removal  of  a  particular  trace contaminant
may  be  uneconomical  because  of the presence  of  other  ionic
species  that are preferentially removed.    The regeneration  of
the  resins  presents  its  own problems.    The   cost   of  the
regenerative  chemicals  can be  high.  In  addition,  the  waste
streams originating from the  regeneration process  are extremely
high in pollutant concentrations, although low in volume.   These
must  be  further  processed  for  proper disposal.
Operational   Factors.
Reliability:   With
occasional clogging or fouling of the resins,
proved to be -a highly dependable technology.
the  exception  of
ion  exchange  has
Maintainability:   Only  the normal maintenance of pumps, valves,
piping and other hardware used in  the  regeneration  process  is
required.

Solid  Waste  Aspects:  Few, if any, solids accumulate within the
ion  exchangers,  and those which do appear are  removed  by  the
regeneration  process.  Proper prior treatment and  planning  can
eliminate   solid   build-up   problems  altogether.   The  brine
resulting  from regeneration of the  ion  exchange   resin   must
usually  be treated  to  remove  metals  before discharge.   This
can generate solid waste.

Demonstration Status.  All of the applications mentioned in  this
document  are  available for commercial use, and industry sources
estimate the number of units currently in the field at well  over
120.  The research" and development in ion exchange is focusing on
improving  the  quality and efficiency of the resins, rather than
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
new applications.   Work  is  also  being  done  on  a  continuous
regeneration  process  whereby  the resins  are  contained  on  a
fluidtransfusible     belt.      The   belt   passes   through    a
compartmentalized    tank   with  ion   exchange,   washing,   and
regeneration  sections.   The resins  are  therefore  continually
used and regenerated.  No such system, however, has been reported
beyond the pilot stage.

Ion exchange has been used to treat cyanide containing wastewater
at  two  plants  in  the primary  aluminum   subcategory  in  the
nonferrous metals  manufacturing category.

Ion  exchange has  also been used to treat wastewaters from  three
secondary    precious    metals   facilities in  the   nonferrous
metals  manufacturing  category.    These   wastewaters   contain
gold, platinum and palladium, as well as base metals.

20. Membrane Filtration

Membrane   filtration   is   a   treatment  system  for  removing
precipitated metals from a wastewater stream.  It must  therefore
be  preceded  by  those  treatment techniques which will properly
prepare the wastewater for solids removal.  Typically, a membrane
filtration unit is preceded by pH adjustment or sulfide  addition
for precipitation of the metals.  These steps are followed by the
addition  of  a  proprietary  chemical  reagent  which causes the
precipitate to be non-gelatinous, easily  dewatered,  and  highly
stable.   The  resulting  mixture  of  pretreated  wastewater and
reagent is continuously recirculated through a filter module  and
back  into  a  recirculation  tank.   The  filter module contains
tubular membranes.  While the reagent-metal hydroxide precipitate
mixture flows through the inside of the tubes, the water and  any
dissolved  salts  permeate  the membrane.  When the recirculating
slurry reaches a concentration of 10 to 15 percent solids, it  is
pumped out of the system as sludge.

Application  and  Performance.  Membrane filtration appears to be
applicable to any wastewater or process  water  containing  metal
ions  which  can  be  precipitated  using  hydroxide,  sulfide or
carbonate  precipitation.   It  could  function  as  the  primary
treatment  system, but also might find application as a polishing
treatment (after precipitation and settling) to ensure  continued
compliance  with metals limitations.  Membrane filtration systems
are  being  used  in  a  number   of   industrial   applications,
particularly  in  the  metal finishing area.  They have also been
used for toxic metals removal in the metal  fabrication  industry
and the paper industry.

The  permeate is claimed by one manufacturer to contain less than
the  effluent  concentrations  shown  in  Table VII-26 (page     )
regardless  of  the  influent  concentrations.  These claims have
been largely substantiated by the analysis of  water  samples  at
various plants in various industries.

In  the  performance  predictions  for this technology, pollutant
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           GENERAL  DEVELOPMENT DOCUMENT
                 SECT - VII
 concentrations  are  reduced  to  the  levels   shown  below   in   Table
 VII-26  (page  252) unless  lower  levels are  present  in the influent
 stream.

 Advantages  and Limitations.
	    A major advantage of the membrane
 installations  can  use  most  of  the
 systems  that may already be in place.
claimed  to  be  excellent,  even  with
pollutant  input  rates;  however,  the
 filtration  system  is  that
 conventional  end-of-pipe
 Removal efficiencies  are
 sudden   variation   of
 effectiveness of the  membrane filtration system can be limited by
 clogging of the filters.  Because pH changes in the waste  stream
 greatly  intensify clogging  problems/  the pH must be carefully
 monitored  and controlled.   Clogging can force the shutdown   of
 the system  and  may  interfere  with  production.   In addition,
 the  relatively  high capital cost of this system may  limit  its
 use.

 Operational Factors.  Reliability:  Membrane filtration has  been
 shown  to  be  a   very  reliable  system, provided that the pH is
 strictly controlled.  Improper pH can result in the  clogging  of
 the  membrane.  Also, surges in the flow rate of the waste stream
 must be controlled in  order  to  prevent  solids  from  passing
 through the filter and into the effluent.

 Maintainability:    The   membrane   filters  must  be  regularly
 monitored, and cleaned or replaced as  necessary.   Depending  on
 the  composition   of  the waste stream and its flow rate, frequent
 cleaning  of  the  filters  may  be  required.    Flushing   with
 hydrochloric  acid for  6  to 24 hours will usually suffice.  In
 addition, the routine maintenance of  pumps,  valves,  and  other
 plumbing is required.

 Solid  Waste Aspects:  When the recirculating reagent-precipitate
 slurry reaches 10  to  15 percent solids, it is pumped out  of  the
 system.   It can then be disposed of directly or it can undergo a
 dewatering process.  Because this sludge contains  toxic  metals,
 it requires proper disposal.

 Demonstration Status. .There are more than 25 membrane filtration
 systems   presently   in  use  on  metal  finishing  and  similar
 wastewaters.  Bench-scale and pilot-studies are being run  in  an
 attempt to expand  the list of pollutants for which this system is
 known to be .effective.

 21. Peat Adsorption

 Peat moss is a complex natural organic material containing lignin
 and   cellulose    as  major  constituents.    These  constituents,
particularly  lignin,  bear  polar  functional  groups,  such  as
alcohols,   aldehydes,  ketones,   acids,   phenolic hydroxides, and
ethers, that can be involved in chemical bonding.   Because of the
polar nature of the material,  its adsorption of dissolved  solids
such  as  transition  metals and polar organic molecules is quite
high.   These properties  have led to the use of peat as  an  agent
for the purification of  industrial wastewater.
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           GENERAL DEVELOPMENT DOCUMENT
                     SECT  - VII
Peat  adsorption  is a "polishing" process which can achieve very
low effluent  concentrations  for  several  pollutants.   If  the
concentrations  of  pollutants  are  above  10  mg/1,  then  peat
adsorption  must  be  preceded  by  pH  adjustment   for   metals
precipitation and subsequent clarification.  Pretreatment is also
required  for  chromium  wastes  using ferric chloride and sodium
sulfide.  The wastewater  is  then  pumped  into  a  large  metal
chamber  called  a  kier  which  contains a layer of peat through
which the waste stream passes.  The water flows to a second  kier
for  further  adsorption.   The  wastewater  is  then  ready  for
discharge.  This system may be automated or manually operated.

Application and Performance.  Peat  adsorption  can  be  used  in
nonferrous metals manufacturing for removal of residual dissolved
metals  from  clarifier effluent.  Peat moss may be used to treat
wastewaters containing heavy metals  such  as  mercury,  cadmium,
zinc,  copper,  iron,  nickel,  chromium,  and  lead,  as well as
organic  matter  such  as  oil,  detergents,  and   dyes.    Peat
adsorption  is  currently used commercially at a textile plant, a
newsprint facility, and a metal reclamation operation.

Table VII-27  (page 252)  contains  performance  figures  obtained
from  pilot-plant  studies.    Peat adsorption was preceded by pH
adjustment for precipitation and by clarification.

In addition, pilot plant studies have shown that  chelated  metal
wastes,  as  well as the chelating agents themselves, are removed
by contact with peat moss.

Advantages and Limitations.  The major advantages of  the  system
include  its  ability  to yield low pollutant concentrations, its
broad scope in  terms  of  the  pollutants  eliminated,  and  its
capacity to accept wide variations of waste water composition.

Limitations   include   the  cost  of  purchasing,  storing,  and
disposing of  the peat moss; the necessity for regular replacement
of the peat may lead to high  operation  and  maintenance  costs.
Also,  the  pH  adjustment  must  be  altered  according  to  the
composition of the waste stream.

Operational Factors.  Reliability:  The  question  of  long-term
reliability is not yet fully answered.  Although the manufacturer
reports  it   to be a highly reliable system, operating experience
is needed to  verify the claim.

Maintainability:   The  peat  moss  used  in  this  process  soon
exhausts  its  capacity  to adsorb pollutants.  At that time, the
kiers must be opened, the peat removed,  and  fresh  peat  placed
inside.    Although   this   procedure   is  easily  and  quickly
accomplished, it must  be  done  at  regular  intervals,  or  the
system's efficiency drops, drastically.
 Solid Waste Aspects:
 must  be eliminated.
After removal from the kier, the spent peat
If incineration is used, precautions should
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           GENERAL  DEVELOPMENT  DOCUMENT
                   SECT - VII
be  taken  to  insure  that  those pollutants  removed  from   the  water
are not   released  again  in the  combustion  process.   Presence of
sulfides  in  the  spent peat, for example,  will  give  rise to  sulfur
dioxide in the fumes from  burning.  The presence  of   significant
quantities  of   toxic    heavy   metals   in   nonferrous   metals
manufacturing wastewater will in  general  preclude incineration of
peat used in treating these wastes.
Demonstration  Status.
 Only  three  facilities  currently   use
systems  in the United States - a textile
commercial  adsorption
manufacturer, a newsprint facility, and a metal  reclamation firm.
No data have been reported showing the use of peat adsorption  in
nonferrous metals manufacturing plants.

22. Reverse Osmosis

The process of osmosis involves the passage of a liquid through a
semipermeable  membrane  from  a  dilute  to  a more concentrated
solution.  Reverse osmosis (RO) is an operation  in which pressure
is applied to the more concentrated solution,  forcing  the  per-
meate  to  diffuse  through the membrane and into the more dilute
solution.  This filtering action produces  a  concentrate  and  a
permeate  on opposite sides of the membrane.  The concentrate can
then be further treated or returned to the original operation for
continued use, while the permeate water can be recycled  for  use
as  clean  water.   Figure  VII-26  (page 279) depicts a  reverse
osmosis system.

As illustrated in Figure VII-27,  (page 280),  there  are   three
basic  configurations  used in commercially available RO modules:
tubular, spiral-wound, and hollow fiber.  All of these operate on
the principle described above, the major difference  being  their
mechanical and structural design characteristics.

The  tubular  membrane module uses a porous tube with a cellulose
acetate membrane lining.  A common tubular module consists  of  a
length  of  2.5  cm  (1 inch) diameter tube wound on a supporting
spool and_encased in a plastic shroud.  Feed water is driven .into
the tube under pressures varying from 40 to 55 atm (600-800 psi).
The permeate  passes  through  the  walls ' of  the  tube  and  is
collected  in  a manifold while the concentrate is drained off at
the end of the tube.  A less widely used tubular RO module uses a
straight tube contained in a housing,  under  the  same  operating
conditions.

Spiral-wound  membranes  consist  of  a porous backing sandwiched
between two cellulose acetate membrane sheets  and  bonded  along
three  edges.   The fourth edge of the  composite sheet is attached
to a large permeate collector tube.    A  spacer  screen  is  then
placed  on  top of the membrane sandwich,  and the entire stack is
rolled around the centrally located tubular  permeate  collector.
The  rolled  up package is inserted into a pipe able to withstand
the high operating pressures employed  in this process, up  to  55
atm  (800  psi)  with the spiral-wound  module.   When the system is
operating, the pressurized product water permeates  the  membrane
                               214

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            GENERAL DEVELOPMENT DOCUMENT
                                            SECT - VII
 and  flows  through the backing material  to the central collector
 tube.   The concentrate  is  drained off  at  the end of  the container
 pipe  and  can  be   reprocessed  or  sent  to  further   treatment
 facilities.

 The hollow fiber membrane  configuration is  made up of a bundle of
 polyamide  fibers   of   approximately 0.0075 cm  (0.003 in.)  OD and
 0.0043 cm (0.0017 in.)  ID.   A commonly used hollow   fiber   module
 contains   several hundred  thousand of  the fibers placed in  a  long
 tube,  wrapped  around a  flow  screen, and   rolled  into   a spiral.
 The  fibers  are  bent in a  U-shape and  their ends are supported by
 an epoxy  bond.   The hollow fiber  unit  is  operated under 27   atm
 (400  psi),  the  feed water being  dispersed  from the  center  of the
 module through a porous distributor tube.   Permeate  flows through
 the membrane to  the hollow  interiors   of  the fibers and  is
 collected at the ends of the fibers.

 The   hollow  fiber and spiral-wound  modules   have a distinct
 advantage over the  tubular system in that they  are able to  load a
 very  large  membrane surface   area  into   a    relatively   small
 volume.   However,    these    two  membrane   types  are   much  more
 susceptible  to  fouling  than  the tubular  system,   which   has  a
 larger flow channel. This characteristic also  makes the tubular
 membrane   much   easier  to  clean  and  regenerate than  either  the
 spiral-wound  or hollow fiber modules.  One  manufacturer   claims
 that  its  helical   tubular  module  can   be    physically   wiped
 clean   by  passing a  soft porous polyurethane plug under  pressure
 through the  module.

 Application  and  Performance.  In  a  number  of  metal   processing
 plants,   the  overflow   from the first rinse in a countercurrent
 setup  is   directed   to   a  reverse  osmosis  unit,  where   it   is
 separated  into  two  streams.    The concentrated stream contains
 dragged out  chemicals and is returned to the bath to replace  the
 loss   of   solution  caused by evaporation and dragout.  The  dilute
 stream (the permeate) is routed to the last rinse tank  to provide
 water  for  the rinsing operation.  The rinse flows from   the  last
 tank to the  first tank,  and  the cycle is complete.

 The_closed-loop system described above may be supplemented by the
 addition  of  a  vacuum  evaporator after  the RO unit in order to
 further reduce the volume of reverse  osmosis  concentrate.    The
 evaporated  vapor can be condensed and returned to the last rinse
 tank or sent on for further treatment.

The  largest  application  has been for the   recovery  of  nickel
solutions.  It has been  shown that RO can   generally   be  applied
to   most   acid   metal   baths   with   a    high   degree     of
performance,  providing    that   the    membrane   unit    is    not
overtaxed.     The  limitations  most   critical   here    are  the
           pH  range and maximum operating  pressure    for    each
             configuration.  Adequate    prefiltration   is    also
             Only three  membrane types  are readily available   in
            RO  units,   and  their overwhelming  use  has been  for
allowable
particular
essential.
commercial
the  recovery  of various acid metal baths.   For the  purpose  of
                               215

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           GENERAL DEVELOPMENT DOCUMENT
                        SECT - VII
calculating   performance  predictions  of  this  technology,   a
rejection  ratio of 98 percent is  assumed  for dissolved  salts,
with 95 percent permeate recovery.

Advantages  and  Limitations.   The  major  advantage  of reverse
osmosis  for  handling  process  effluents  is  its  ability_  to
concentrate  dilute solutions for recovery of salts and chemicals
with low power requirements.  No latent heat of  vaporization  or
fusion  is  required  for  effecting separations; the main energy
requirement is for a high pressure .pump.  It requires  relatively
little  floor  space  for  compact,  high  capacity units, and it
exhibits good recovery  and  rejection  rates  for  a  number  of
typical  process  solutions.  A,limitation of the reverse osmosis
process  for  treatment  of  process  effluents  is  its  limited
temperature  range  for  satisfactory  operation.   For cellulose
acetate systems, the preferred limits are 18   to 30 C (65    to
85°F);  higher  temperatures  will increase the rate of membrane
hydrolysis and reduce system life, while lower temperatures  will
result  in  decreased  fluxes  with  no  damage  to the membrane.
Another limitation is  inability  to  handle  certain  solutions.
Strong  oxidizing  agents,  strongly  acidic  or basic solutions,
solvents, and other organic compounds can  cause  dissolution  of
the  membrane.   Poor rejection of some compounds such as berates
and low molecular weight organics is another problem.  Fouling_of
membranes by slightly soluble components in solution or  colloids
has caused failures, and fouling of membranes by feed waters with
high   levels  of  suspended solids can be a  problem.   A   final
limitation  is inability to treat or achieve high   concentration
with  some  solutions.   Some  concentrated  solutions  may  have
initial  osmotic   pressures which are so high that  they_ either
exceed  available  operating  pressures or  are  uneconomical  to
treat.                  •       .:•;•»    .  ; .

Operational Factors.   Reliability:  .Very;  good^ reliability  _is
achievedso long as the proper precautions are  taken to minimize
the chances of fouling or   degrading  the  membrane.   Sufficient
testing  of the waste stream prior to application of an RO system
will provide  the  information. needed  to  dnsure  a  successful
application.

Maintainability:   Membrane life  is estimated  to  range  from  six
months to three years,  depending  on   the  use  of  the  system.
Downtime for flushing or cleaning  is on the order of two  hours as
often  as  once  each  week; a  substantial portion  of maintenance
time must be spent on cleaning  any prefilters  installed ahead  of
the reverse osmosis unit.     :

Solid  Waste Aspects:   In  a closed-loop system utilizing  RO  there
is a  constant  recycle of concentrate  and  a   minimal  amount  of
solid  waste.   Prefiltration   eliminates many solids before_they
reach  the  module  and helps  keep the  ;build-up  to  a   minimum.
These  solids require proper disposal.
 Demonstration  Status.
 reverse  osmosis
       There are presently at least one hundred
was~tewater  applications  in   a   variety   of
                                216

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
industries.  In addition to these, there are 30 to 40 units being
used  to  provide  pure  process  water  for  several industries.
Despite the many types and configurations of membranes, only  the
spiral-wound   cellulose   acetate membrane  has  had  widespread
success in commercial 'applications.

23. Sludge Bed Drying

As a waste treatment procedure, sludge bed drying is employed  to
reduce  the  water  content  of a variety of sludges to the point
where they are amenable to mechanical collection and  removal  to
landfill.   These  beds  usually  consist of 15 to 45 cm (6 to 18
in.) of sand over a 30 cm (12 in.) deep gravel drain system  made
up  of  3  to 6 mm (1/8 to 1/4 in.) graded gravel overlying drain
tiles.  Figure VII-28 (page 281)  shows  the  construction  of  a
drying bed.

Drying   beds   are   usually   divided   into   sectional  areas
approximately 7.5 meters (25 ft) wide x 30 to 60 meters  (100  to
200  ft) long.  The partitions may be earth embankments, but more
often are made of planks and supporting grooved posts.

To apply liquid sludge to the sand bed, a  closed  conduit  or  a
pressure pipeline with valved outlets at each sand bed section is
often  employed.  Another method of application is by means of an
open channel with appropriately placed side  openings  which  are
controlled  by slide gates.  With either type of delivery system,
a concrete splash slab should be provided to receive the  falling
sludge and prevent erosion of the sand surface.

Where  it  is necessary to dewater sludge continuously throughout
the year regardless of the weather, sludge beds  may  be  covered
with  a  fiberglass  reinforced  plastic  or other roof.  Covered
drying beds permit a greater volume of sludge drying per year  in
most  climates  because  of  the protection afforded from rain or
snow and  because  of  more  efficient  control  of  temperature.
Depending on the climate, a combination of open and enclosed beds
will  provide  maximum  utilization  of  the  sludge  bed  drying
facilities.

Application and Performance.  Sludge drying beds are a  means  of
dewatering  sludge  from  clarifiers  and  thickeners.   They are
widely  used  both  in   municipal   and   industrial   treatment
facilities.                  .

Dewatering  of  sludge  on  sand  beds  occurs by two mechanisms:
filtration of water "through the bed and evaporation of water as a
result of radiation  and  convection.   Filtration  is  generally
complete   in   one   to  two  days  and  may  result  in  solids
concentrations as  high  as  15: to  20  percent.   The  rate  of
filtration depends on ,the drainability of the sludge.

The  rate  of  air  drying  of  sludge is related to temperature,
relative humidity, and air velocity.  Evaporation will proceed at
a constant rate to a critical moisture content, then at a falling
                              .217

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
rate to an equilibrium moisture content.  The average evaporation
rate for a sludge is about 75 percent of that from a  free  water
surface.

Advantages  and Limitations.  The main advantage of sludge drying
beds over other types of sludge dewatering is the relatively  low
cost of construction, operation, and maintenance.

Its  disadvantages  are  the large area of land required and long
drying times that depend, to  a  great  extent,  on  climate  and
weather.
Operational  Factors.   Reliability:   Reliability
favorable climactic conditions, proper bed  design
avoid  excessive  or  unequal  sludge  application.
         is  high with
         and  care  to
           If climatic
conditions in a given area are not favorable for adequate drying,
a cover may be necessary.

Maintainability:   Maintenance  consists  basically  of  periodic
removal  of  the  dried sludge.  Sand removed from the drying bed
with the sludge must be replaced and the sand layer resurfaced.

The resurfacing of sludge beds  is  the  major  expense  item  in
sludge  bed  maintenance,  but  there  are  other areas which may
require attention.  Underdrains occasionally become  clogged  and
have to be cleaned.  Valves or sludge gates that control the flow
of  sludge  to  the  beds must be kept watertight.  Provision for
drainage of lines in winter should be provided to prevent  damage
from  freezing.   The  partitions between beds should be tight so
that sludge will not flow from one compartment to  another.   The
outer walls or banks around the beds should also be watertight.

Solid  Waste  Aspects:  The full sludge drying bed must either be
abandoned or the collected solids must be removed to a  landfill.
These  solids  contain  whatever  metals  or other materials were
settled in the clarifier.  Metals will be present as  hydroxides,
oxides,  sulfides,  or  other salts.  They have the potential for
leaching and contaminating ground water, whatever the location of
the~semidried solids.  Thus the abandoned bed or landfill  should
include provision for runoff control and leachate monitoring.

Demonstration  Status.   Sludge  beds  have been in common use in
both  municipal  and  industrial  facilities  for   many   years.
However,  protection  of  ground  water from contamination is not
always adequate.

24. Ultrafiltration

Ultrafiltration  (UF)  is  a  process  which  uses  semipermeable
polymeric membranes to separate emulsified or colloidal materials
suspended in a liquid phase by pressurizing the liquid so that it
permeates  the  membrane.  The membrane of an ultrafilter forms a
molecular screen which retains molecular particles based on their
differences in size, shape, and chemical structure.  The membrane
permits passage of solvents and lower molecular weight molecules.
                               218

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
At present, an ultrafliter is capable of -removing materials  with
molecular  weights in the range of 1,000 to 100,000 and particles
of comparable or larger sizes.

In an  ultrafiltration  process,  the  feed  solution  is  pumped
through . a  tubular  membrane unit.  Water and some low molecular
weight materials pass through  the  membrane  under  the  applied
pressure of 2 to 8 atm (10 to 100 psiq).  Emulsified oil droplets
and  suspended  particles are retained, concentrated, and removed
continuously.   In  contrast  to  ordinary  filtration,  retained
materials  are washed off the membrane filter rather than held by
it.  Figure VII-29  (page 282)  represents  the   ultrafiltration
process.

Application   and  Performance.   Ultrafiltration  has  potential
application to nonferrous metals manufacturing for separation  of
oils  and  residual  solids  from a variety of waste streams.  In
treating nonferrous metals manufacturing wastewater, its greatest
applicability  would  be  as  a  polishing  treatment  to  remove
residual  precipitated  metals  after  chemical precipitation and
clarification.  Successful  commercial  use,  however,  has  been
primarily  for  separation  of  emulsified  oils from wastewater.
Over one hundred such units now operate  in  the  United  States,
treating  emulsified oils from a variety of industrial processes.
Capacities of currently operating units range from a few  hundred
gallons  a week to 50,000 gallons per day.  Concentration of oily
emulsions  to  60  percent  oil  or  more   is   possible.    Oil
concentrates  of  40  percent  or more are generally suitable for
incineration, and the permeate can be treated further and in some
cases recycled back to the process.  In this way, it is  possible
to  eliminate  contractor  removal  costs  for oil from some oily
waste streams.

The test data in Table VII-28 (page 253) indicate ultrafiltration
performance (note that UF is not  intended  to  remove  dissolved
solids).
The  removal  percentages  shown  are  typical,
influenced by pH and other conditions.
      but  they can be
The  permeate  or  effluent  from  the  ultrafiltration  unit  is
normally   of   a  quality  that  can  be  reused  in  industrial
applications or discharged directly.  The  concentrate  from  the
ultrafiltration  unit  can  be  disposed  of as any oily or solid
waste.

Advantages and  Limitations.   Ultrafiltration  is  sometimes  an
attractive  alternative  to  chemical  treatment because of lower
capital equipment, installation, and operating costs,  very  high
oil   and   suspended   solids   removal,   and  little  required
pretreatment.  It places a positive  barrier  between  pollutants
and effluent which reduces the possibility of extensive pollutant
discharge due to operator error or upset in settling and skimming
systems.   Alkaline  values in alkaline cleaning solutions can be
recovered and reused in process.                           	
                               219

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           GENERAL DEVELOPMENT DOCUMENT
                 SECT - VII
A  limitation  of  ultrafiltration,  for  treatment   of   process
effluents   is   its   narrow   temperature  range  (18°C  to
30°C) for satisfactory operation.   Membrane  life  decreases
with   higher temperatures,    but  flux  increases  at  elevated
temperatures.  Therefore,   surface  area  requirements   are   a
function    of  temperature  and  become   a   tradeoff   between
initial  costs  and  replacement  costs  for  the  membrane.   In
addition,  ultrafiltration  cannot   handle  certain   solutions.
Strong   oxidizing    agents,   solvents,    and  other   organic
compounds  can  dissolve  the membrane.  Fouling is  sometimes  a
problem,  although  the high velocity of the wastewater  normally
creates enough turbulence to keep fouling,  at a  minimum.   Large
solids  particles can sometimes puncture the membrane and must be
removed  by  gravity   settling   or   filtration  prior  to  the
ultrafiltration unit.
Operational   Factors.
Reliability:
The
the
reliability  of  an
proper  filtration,
Q£            	
ultrafiltration system is dependent  on
settling  or other treatment of incoming waste streams to prevent
damage to the membrane.  Careful pilot studies should be done  in
each  instance  to determine necessary pretreatment steps and the
exact membrane type to be used.

Maintainability:  A limited  amount  of  regular  maintenance  is
required  for  the  pumping system.   In addition, membranes must
be  periodically changed.   Maintenance associated with  membrane
plug-ging can be reduced by selection of a membrane with  optimum
phy-sical   characteristics   -and  sufficient  velocity  of   the
waste  stream.    It   is  occasionally  necessary  to   pass   a
detergent  solution  through  the  system  to  remove an oil  and
grease film which accumulates on  the  membrane.    With   proper
maintenance, membrane life can be greater than twelve months.

Solid  Waste  Aspects:   Ultrafiltration  is  used  primarily  to
recover solids and liquids.  It therefore eliminates solid  waste
problems  when the solids (e.g., pain-t solids) can be recycled to
.the process.  Otherwise, the stream  containing  solids  must  be
treated   by   end-of-pipe   equipment.   In  the  most  probable
applications within the nonferrous metals manufacturing category,
the ultrafilter would remove hydroxides  or  sulfides  of  metals
which have recovery value.

Demonstration   Status.   The  ultrafiltration  process  is  well
developed and commercially available for treatment of  wastewater
or  recovery  of  certain  high molecular weight liquid and solid
contaminants.

25.  Vacuum Filtration

In wastewater  treatment  plants,   sludge  dewatering  by  vacuum
filtration  generally uses cylindrical'drum filters.  These drums
have a filter medium which  may  be  cloth  made  of  natural  or
synthetic  fibers  or  a wire-mesh fabric.   The drum is suspended
above and dips into a vat of sludge.   As the drum rotates slowly,
                               220

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           GENERAL DEVELOPMENT;: DOCUMENT
SECT. - VII
part of its circumference is subject to an internal  vacuum  that
draws  sludge  to  the. filter medium.  Water, is drawn through the
porous filter cake to a discharge port, and the dewatered sludge,
loosened by compressed air, is'  scraped  from  the  filter  mesh.
Because  the dewatering of sludge on vacuum filters is relativley
expensive per kilogram of .water removed,  the  liquid  sludge  is
frequently  thickened  prior . to  processing.  A vacuum filter is
shown in Figure VII-30 (page  ,,:.,).  •     .

Application and Performance.  -Vacuum filters are frequently  used
both  in  municipal  treatment :• plants  and  in a wide variety of
industries.  They are most commonly used  in  larger  facilities,
which  may  have  a  thickener  to  double  the solids content of
clarifier sludge before vacuum filtering.

The function of vacuum filtration is to reduce the water  content
Of  sludge,  so  that  the  solids content increases from about 5
percent to about 30 percent.  .  .    :

Advantages and Limitations.  Although the initial cost  and  area
requirement of the vacuum filtration system are higher than those
of  a  centrifuge,  the  operating  cost is lower, and no special
provisions for sound and vibration protection need be made.   The
dewatered sludge from this process is in the form of a moist cake
and can be conveniently handled.

Operational  Factors.   Reliability:   Vacuum filter, systems have
proven  reliable  at  many .industrial  and  municipal  treatment
facilities.  At present, the largest municipal installation is at
the   West  Southwest  wastewat.er  treatment  plant  of  Chicago,
Illinois,  where  96  large  filters  were  installed  in   1925,
functioned  approximately, 25 >years, and then were replaced with
larger units.  Original!vacuum.filters: at  Minneapolis-St,  Paul,
Minnesota,  now  have  over  28  years of continuous service, and
Chicago has some units with similar or greater service life.

Maintainability:   Maintenance ,> .consists;  of:, the   cleaning   or
replacement of. the filter> media,;;,drainage grids, drainage piping,
filter  pans,  and other/; parts, of •• the equipment.  Experience in a
number  of  vacuum  filter  plants,  indicates  that   maintenance
consumes  approximately  5  to:  .15; percent-of the total time.  If
carbonate  buildup  or  other  problems  are  unusually   severe,
maintenance  time may be as high as 20 percent.  For this reason,
it is desirable to maintain one or more spare units.

If intermittent operation is used., the filter equipment should be
drained and washed each time it is  taken  out  of  service.   An
allowance for this wash time must be made in filtering schedules.

Solid  Waste Aspects:  Vacuum filters generate a solid cake which
is usually trucked directly  to;,  landfill.   All  of  the  metals
extracted   from   the plant wastewater are concentrated  in  the
filter cake as hydroxides,, oxides, sulfides, or other salts.

Demonstration Status.  Vacuum filtration has been widely used for.
                               221,

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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
many  years.   It is a fully proven,  conventional technology for
sludge  dewatering.   Vacuum filtration is used in 20  nonferrous
metals manufacturing plants for sludge dewatering.

26.  Permanganate Oxidation

Permanganate oxidation is a chemical reaction by which wastewater
pollutants  can  be oxidized.   When the reaction is  carried  to
completion,   the   by-products   of  the   oxidation   are   not
environmentally  harmful.   A large number of pollutants  can  be
practically   oxidized  by  permanganate,   including   cyanides,
hydrogen  sulfide, and phenol.  In addition, the chemical  oxygen
demand  (COD)  and many odors in wastewaters and sludges  can  be
significantly  reduced by permanganate oxidation carried  to  its
end point.  Potassium permanganate can be added to wastewater  in
either dry or slurry form.  The oxidation occurs optimally in the
8  to  9 pH range.  As an example of the  permanganate  oxidation
process,  the following chemical equation shows the oxidation  of
phenol by potassium permanganate:
3CgH5(OH)
28KMn04
5H20 ---- >  18C02
    28KOH
                                                         28MnO2
One  of  the by-products of this oxidation is  manganese  dioxide
(Mn02),  which  occurs  as a relatively  stable  hydrous  colloid
usually having a negative charge.  These properties, in  addition
to  its large surface area, enable manganese dioxide to act as  a
sorbent  for metal cation, thus enhancing their removal from  the
wastewater .

Application  and  Performance.   Commercial use  of  permanganate
oxidation  has been primarily for the control of phenol and waste
odors.   Several municipal waste treatment facilities report that.
initial  hydrogen  sulfide concentrations (causing  serious  odor
problems)  as high as 100 mg/1 have been reduced to zero  through
the  application  of  potassium  permanganate.    A  variety   of
industries  (including metal finishers and agricultural  chemical
manufacturers)  have  used  permanganate  oxidation  to   totally
destroy phenol in their wastewaters.

Advantages  and Limitations.   Permanganate oxidation has several
advantages  as a wastewater treatment  technique.   Handling  and
storage  are  facilitated  by  its  non-toxic  and  non-corrosive
nature.  Performance has been proved in a number of municipal and
industrial  applications.   The tendency of the manganese dioxide
by-product to act as a coagulant aid is a distinct advantage over
other types of chemical treatment.

The  cost  of permanganate oxidation treatment  can  be  limiting
where  very  large  dosages are required  to  oxidize  wastewater
pollutants.   In  addition,  care  must  be taken in  storage  to
prevent  exposure to intense heat,  acids,  or  reducing  agents;
exposure  could  create a fire hazard or  cause  explosions.   Of
greatest  concern  is the environmental hazard which the  use  of
manganese chemicals in treatment could cause.  Care must be taken
to remove the manganese from treated water before discharge.
                               222

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           GENERAL DEVELOPMENT DOCUMENT
                                SECT - VII
Operation  Factors.    Reliability:    Maintenance  consists   of
periodic   sludge  removal  and  cleaning  of  pump  feed  lines.
Frequency    of   maintenance   is   dependent   on    wastewater
characteristics.

Solid  Waste Aspects:   Sludge is generated by the process  where
the manganese dioxide by-product tends to act as a coagulant aid.
The  sludge  from  permanganate oxidation can  be  collected  and
handled  by standard sludge treatment and  processing  equipment.
No  nonferrous metals manufacturing facilities are known  to  use
permanganate oxidation for wastewater treatment at this time.

Demonstration Status.
	   The oxidiation of wastewater pollutants by
permanganate is a proven treatment process in  several
             It has been shown effective in treating a
                            municipal  and  industrial
potassium
types  of industries.
wide  variety  of  pollutants in both
wastes.
27.  Activated Alumina Adsorption

Application,  Performance, Advantages and Limitations.  Activated
alumina  adsorbs  arsenic  and  fluorides.
                                   Alumina's   removal
efficiency  depends  on  the  wastewater  characteristics.   High
concentrations  of  alkalinity  or chloride and  high  pH  reduce
activated  alumina's  capacity  to  adsorb.   This  reduction  in
adsorptive  capacity  is  due to the  alkalinity  causing  (e.g.,
hydroxides,  carbonates, etc.) and chlorine anions competing with
arsenic and fluoride ions for removal sites on the alumina.

While chemical precipitation can reduce fluoride to less than  14
mg/1  by  formation of calcium fluoride,  activated  alumina  can
reduce  fluoride levels to below 1.0 mg/1 on a  long-term  basis.
An initial concentration of 30 mg/1 of fluoride can be reduced by
as much as 85 to 99+ percent.  Influent arsenic concentrations of
0.3  to  10 mg/1 can be reduced by 85 to 99+  percent.   However,
some  complex  forms  of fluoride are not  removed  by  activated
alumina.  Caustic, sulfuric acid, hydrochloric acid, and alum are
used to chemically regenerate activated alumina.

Operational Factors—Reliability and Maintainability:   Activated
alumina  has been used at potable water treatment plants for many
years.   Furthermore,  the equipment is similar to that found  in
ion-exchange  water  softening plants which are commonly used  in
industry to prepare boiler water.

Demonstration Status.   The use of activated alumina has not been
reported by any nonferrous metals manufacturing plants nor is  it
widely applied in any other industrial categories.   High capital
and  operation costs generally limit the wide application of this
process in industrial applications.

28.  Ammonia Stripping

Ammonia,  often used as a process reagent,  dissolves in water to
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           GENERAL DEVELOPMENT DOCUMENT
                              SECT - VII
an extent governed by the partial pressure of the gas in  contact
with  the  liquid.   The  ammonia  may be  removed  from  process
wastewaters by stripping with air or steam.

Air  stripping takes place in a packed or lattice tower;  air  is
blown through the packed bed or lattice,  over which the ammonia-
laden stream flows.   Usually,  the wastewater is heated prior to
delivery to the tower, and air is used at ambient temperature.

The  term  "ammonia  steam stripping" refers to  the  process  of
desorbing  aqueous  ammonia  by  contacting  the  liquid  with  a
sufficient amount of ammonia-free steam.  The steam is introduced
countercurrent to the wastewater to maximize removal of  ammonia.
The  operation  is  commonly carried out in packed  bed  or  tray
columns,  and the pH is adjusted to 12 or more with lime.  Simple
tray  designs are used in steam stripping because of the presence
of appreciable suspended solids and the scaling produced by lime.
These  allow  easy  cleaning of the  tower,  at  the  expense  of
somewhat lower steam water contact efficiency,  necessitating the
use of more trays for the same removal efficiency.
Application
and Performance.   The evaporation of water and  the
                generally produces a  drop  in  both
volatilization  of  ammonia
temperature and pH, which ultimately limit the removal of ammonia
in  a  single air stripping tower.   However,  high removals  are
favored by:

1.   High  pH values,  which shift the equilibrium from  ammonium
toward free ammonia;

2.   High temperature,  which decreases the solubility of ammonia
in aqueous solutions; and
3.   Intimate  and extended contact between the wastewater to
stripped and the stripping gas.
                                                  be
Of   these   factors,  pH  and -temperature  are  generally  more
cost-effective  to optimize than increasing contact  time  by  an
increase  in  contact  tank  volume  or recirculation ratio.  The
temperature will, to some extent, be controlled by  the  climatic
conditions;  the  pH  of the wastewater can be adjusted to assure
optimum stripping.

Steam stripping offers better  ammonia  removal  (99  percent  or
better) than air stripping for high ammonia wastewaters found in
the   primary  columbium-tantalum,    primary   molybdenum    and
rhenium,   primary   tungsten,   secondary   silver,    secondary
molybdenum  and vanadium,  primary nickel and  cobalt,  secondary
precious   metals,  primary    and   secondary   tin,   secondary
tungsten   and  cobalt,  secondary uranium and primary  zirconium
and hafnium subcategories of this category.

The performance of an ammonia stripping column is influenced   by
a   number  of  important  variables  that  are associated   with
the wastewater being treated and column design. Brief discussions
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
of these variables follow.

Wastewater pH: Ammonia in water exists in  two  forms,  NH3   and
NH4+,  the   distribution  of which is pH dependent.   Since only
the molecular form of ammonia (NH3 ) can be stripped,  increasing
the  fraction  of  NH3  by increasing the pH enhances the rate of
ammonia desorption.

Column Temperature:  The  temperature  of  the  stripping  column
affects the equilibrium between gaseous and dissolved ammonia, as
well  as  the equilibrium between the molecular and ionized forms
of ammonia in water.  An increase in the temperature reduces  the
ammonia  solubility and increases the fraction of aqueous ammonia
that is in the molecular form, both exhibiting favorable  effects
on the desorption rate.

Steam  rate:  The rate of ammonia transfer from the liquid to gas
phase  is  directly  proportional  to  the  degree   of   ammonia
undersaturation  in  the  desorbing  gas.  Increasing the fate of
steam supply, therefore, increases  undersaturation  and  ammonia
transfer.

Column  design:  A  properly  designed  stripper  column achieves
uniform distribution of the feed liquid across the cross  section
of  the  column,  rapid renewal of the liquid  gas interface, and
extended liquid-gas contacting area and time.

Chemical   analysis   data  were  collected   for    raw    waste
(treatment  influent)   and  treated waste  (treatment  effluent)
from one plant of the iron and steel manufacturing category.  EPA
collected   six paired  samples  in a two-month  period.    These
data  are  the  data base for determining  the  effectiveness  of
ammonia  steam stripping technology and are contained within  the
public record  supporting this rulemaking.   Ammonia treatment at
this  coke plant consisted of two  steam  stripping  columns   in
series  with  steam  injected countercurrently to the flow of the
wastewater.  A  lime  reactor for pH adjustment separated the two
stripping columns.

An  arithmetic  mean  of  the treatment effluent data produced an
ammonia  long-term  mean  value  of  32.2  mg/1.    The   one-day
maximum,  10-day  and 30-day average concentrations attainable by
ammonia steam stripping were calculated using the long-term  mean
of  the,  32.2  mg/1 and the variability factors developed for the,
combined  metals  data  base.  This  produced  ammonia  treatment
effectiveness   concentrations of  133.3,   58.6, and  52.1  mg/1
ammonia  for  the one-day maximum, 10-day  and  30-day  averages,
respectively.

As discussed below, steam stripping is  demonstrated  within  the
nonferrous  metals  manufacturing  category.   EPA  believes  the
performance data from the iron and steel  manufacturing 'category
provide  a  valid  measure  of  this  technology's performance on
nonferrous category wastewater.
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
The Agency has verified the steam  stripping  performance  values
using     steam  stripping data collected at a  zirconium-hafnium
manufacturing  plant/  which is in   the   nonferrous   category.
Data collected  by  the  plant  represent  almost  two  years  of
daily  operations,   and support the long-term   mean   used   to
establish treatment effectiveness.

The Agency also has corroborated the steam stripping  performance
values  with data submitted by a facility manufacturing columbium
and tantalum.   This facility has high influent concentrations of
ammonia  and  also  high  influent  concentrations  of  dissolved
solids.

Steam  stripping  can  recover  significant quantities of reagent
ammonia  from  wastewaters  containing  extremely  high   initial
ammonia  concentrations,  which partially offsets the capital and
energy costs of the technology.

Advantages  and  Limitations.   Strippers  are  widely  used   in
industry  to  remove  a  variety of materials, including hydrogen
sulfide  and  volatile  organics  as  well   as   ammonia,   from
aqueous streams.   The basic techniques have been applied both in
process  and  in wastewater treatment applications and  are  well
understood.  The  use of steam strippers with  and   without   pH
adjustment   is  standard practice for the  removal  of  hydrogen
sulfide and ammonia in   the   petroleum  refining  industry  and
has   been  studied extensively in this context.   Air  stripping
has   treated  municipal  and  industrial  wastewater   and    is
recognized  as  an  effective technique  of  broad applicability.
Both  air and steam stripping have successfully treated  ammonia-
laden   wastewater,    both   within  the    nonferrous    metals
manufacturing   category   or   for  similar  wastes  in  closely
related industries.

The major drawback of air stripping is the low efficiency in cold
weather  and  the  possibility  of  freezing  within  the  tower.
Because  lime  may cause scaling problems and the types of towers
used in air stripping are not easily  cleaned,  caustic  soda  is
generally  employed  to  raise the feed pH.  Air stripping simply
transfers  the ammonia  from  one medium to another   (water   to
air),  whereas   steam stripping  allows  for  recovery  and,  if
so  desired, reuse of ammonia.  Pour primary tungsten plants  use
steam  stripping  to recover  ammonia from process wastewater and
reuse   the   ammonia   in   the    manufacture    of    ammonium
paratungstate.     The    two    major  limitations   of    steam
strippers   are the critical column design required  for   proper
operation    and   the   operational   problems  associated  with
fouling of the packing material.

Operational  Factors.  Reliability and Maintainability: Strippers
are relatively easy to operate.  The most complicated part  of  a
steam  stripper is the boiler.  Periodic maintenance will prevent
unexpected shutdowns of the boiler.

Packing  fouling  interferes  with  the  intimate  contacting  of
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
liquid-gas,    thus   decreasing   the   column  efficiency,  and
eventually  leads  to   flooding.    The   stripper   column   is
periodically   taken   out of service and cleaned with  acid  and
water  with air sparging.   Column cutoff  is  predicated  on   a
maximum allowable   pressure   drop   across   the   packing   of
maximum  "acceptable"  ammonia content in the stripper   bottoms.
Although packing   fouling   may   not  be  completely  avoidable
due  to endothermic  CaS04  precipitation,    column  runs  could
be  prolonged  by  a  preliminary  treatment  step   designed  to
remove suspended  solids  originally present in  the  feed    and
those precipitated after lime addition.

Demonstration  Status.   Steam  stripping  has  proved  to  be an
efficient, reliable process for the removal of ammonia from  many
types  of industrial wastewaters that contain high concentrations
of ammonia.  Industries using ammonia steam stripping  technology
include  the  fertilizer  industry, iron and steel manufacturing,
petroleum  refining,   organic   chemicals   manufacturing,   and
nonferrous  metals manufacturing.  Eight plants in the nonferrous
metals manufacturing category currently practice steam stripping.

IN-PLANT TECHNOLOGY

The intent of  in-plant  technology  for  the  nonferrous  metals
manufacturing point source category is to reduce or eliminate the
waste  load  requiring  end-of-pipe treatment and thereby improve
the efficiency of an  existing  wastewater  treatment  system  or
reduce  the  requirements  of  a  new treatment system.  In-plant
technology involves water conservation, automatic controls,  good
housekeeping   practices,   process   modifications,   and  waste
treatment.

Process Water Recycle

EPA  has  promulgated  BAT for most subcategories  based  on   90
percent recycle   of  wet  air  pollution  control  and   contact
cooling  wastewater.   The Agency promulgated a higher  rate  for
certain waste  streams  where  reported rates of recycle are even
higher.  Water is used in wet air pollution  control  systems  to
capture   particulate    matter    or   fumes   evolved    during
manufacturing.  Cooling  water is used to  remove   excess   heat
from  cast  metal products.

Recycle   is  part  of  the  technical  basis  for  many  of  the
promulgated regulations in the  nonferrous  metals  manufacturing
category.   The  Agency identified both demonstrated and feasible
recycle opportunities as  early  as  1973  in  proposed  effluent
limitations for secondary aluminum.

Recycling of process water is the practice of recirculating water
to  be  used again for the same purpose.  An example of recycling
process water is the return of casting contact cooling  water  to
the  casting  process  after  the  water passes through a cooling
tower.  Two types of recycle are possible—recycle with  a  bleed
stream  (blowdown)  and  total  recycle.   Total  recycle  may be
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            GENERAL DEVELOPMENT DOCUMENT
SECT - VII
 prohibited  by  the  presence  of  dissolved  solids.   Dissolved  solids
 (e.g.,  sulfates  and  chlorides)  entering  a  totally recycled   waste
 stream  may  precipitate,  forming scale  if the  solubility  limits  of
 the   dissolved  solids   are exceeded.   A bleed  stream  may  be
 necessary to   prevent  maintenance  problems   (pipe  plugging   or
 scaling,  etc.)  that  would   be created  by  the  precipitation  of
 dissolved solids.  While the   volume  of   bleed   required   is   a
 function  of   the  amount of dissolved  solids  in the waste stream,
 10 percent  bleed is  a common value  for a variety  of process waste
 streams in  the nonferrous  metals   manufacturing   category.   The
 recycle of process  water is currently practiced  where it is cost
 effective,  where it  is necessary due to  water  shortage,  or   where
 the   local  permitting   authority   has   required  it.  Recycle,  as
 compared to the  once-through   use of  process   water,    is   an
 effective method of  conserving  water.

 Application and  Performance.   Required   hardware necessary for
 recycle is  highly  site-specific.  Basic  items  include  pumps and
 piping.   Additional  materials  are necessary if  water  treatment
 occurs  before  the  water  is   recycled.    These   items   will   be
 discussed   separately  with each unit process.   Chemicals  may  be
 necessary    to    control   scale    build-up,     slime,     and
 corrosion problems,  especially  with recycled cooling water.

 The   Agency based  its zero  discharge of  pollutants  regulation for
 PSES  in  the  secondary  copper  subcategory  on  the  use of  cooling
 towers  in conjunction with  lime  precipitation  and   sedimentation.
 The   lime precipitation  and sedimentation  technology was  included
 to reduce the  metals concentrations so that the wastewater   could
 be  completely recycled  and reused  without  corrosion and  scaling
 problems.   Maintenance   and  energy  use   are  limited   to  that
 required by the  pumps, and  solid waste generation  is dependent  on
 the type of treatment system in place.

 Recycling   through  cooling towers  is  the most common practice.
 One   type   of  application  is   shown  in   Figure   VII-31   (page
 284).    Casting   contact -  cooling water is recycled  through  a
 cooling tower  with a blowdown discharge.

 A cooling tower  is a device which cools  water  by  bringing  the
 water   into  contact  with  air.   The  water  and  air flows are
 directed in such a way as to provide maximum heat transfer.    The
 heat  is  transferred  to   air primarily by evaporation  (about  75
 percent),  while   the  remainder  is  removed  by   sensible  heat
 transfer.

 Factors  influencing  the   rate of heat transfer and,  ultimately,
 the temperature  range of  the tower,  include water   surface  area,
 tower packing and configuration, air flow,  and packing height.   A
 large  water surface area promotes evaporation, and sensible heat
 transfer rates are lower  in proportion to the water surface  area
provided.    Packing  (an  internal  latticework  contact area)   is
often used  to produce small droplets  of   water  which  evaporate
more  easily,   thus increasing the total  surface area  per unit  of
throughput.   For a given water  flow,   increasing   the  air   flow
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
increases  the  amount  of  heat  removed  by  maintaining higher
thermodynamic potentials.  The packing height in the tower should
be high enough so that the air leaving  the  tower  is  close  to
saturation.

A  mechanical-draft cooling tower consists of the following major
components:  (1)   Inlet-water  distributor  (2)    Packing   (3)
Air   fans   (4)  Inlet-air  louvers  (5)   Drift  or  carry-over
eliminators (6)  Cooled water storage basin.

Advantages  and  Limitations.  Recycle offers economic as well as
environmental  advantages.   Water  consumption  is  reduced  and
wastewater  handling  facilities (pumps, pipes, clarifiers, etc.)
can thus be  sized  for  smaller  flows.   By  concentrating  the
pollutants  in  a much smaller volume (the bleed stream), greater
removal efficiencies can be attained  by  any  applied  treatment
technologies.    Recycle  may  require  some  treatment  such  as
sedimentation or cooling of water before it is reused.

The ultimate benefit of recycling process water is the  reduction
in  total  wastewater  discharge and the associated advantages of
lower  flow streams.   A  potential  problem  is   the   build-up
of dissolved  solids  which  could  result  in scaling.   Scaling
can usually be controlled by depressing the  pH  and   increasing
the bleed flow.

Operational  Factors.   Reliability and Maintainability: Although
the principal construction material in mechanical-draft towers is
wood, other materials are used extensively.  For  long  life  and
minimum  maintenance,  wood  is generally pressure-treated with a
preservative.  Although the tower structure is  usually  made  of
treated redwood, a reasonable amount of treated fir has been used
in  recent  years.   Sheathing  and louvers are generally made of
asbestos cement, and the fan stacks of fiberglass.   There  is  a
trend  to  use  fire-resistant  extracted  PVC  as fill which, at
little or no increase in cost, offers the advantage of  permanent
fire-resistant properties.

The  major  disadvantages of wood are its susceptibility to decay
and fire.  Steel construction is occasionally used,  but  not  to
any  great  extent.   Concrete may be used but has relatively high
construction labor costs, although it does offer the advantage of
fire protection.

Various chemical additives are used in cooling water  systems  to
control  scale,  slime,  and  corrosion.   The chemical additives
needed depend  on  the  character  of  the  make-up  water.   All
additives have definite limitations and cannot eliminate the need
for  blowdown.    Care  should  be  taken in selecting nontoxic or
readily degraded additives, if possible.

Solid Waste  Aspects:   The  only  solid  waste  associated  with
cooling towers may be removed scale.

Demonstration  Status.   Predominantly two types of waste streams
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           GENERAL DEVELOPMENT DOCUMENT
            SECT - VII
in the nonferrous metals  manufacturing  category  are  currently
being  recycled;  casting contact cooling water and air pollution
control scrubber liquor.  Two variations  of  recycle  are  used:
(1)  a  wastewater  is recycled within a given process, and (2) a
wastewater is combined with others,  treated,  and  the  combined
wastewater is recycled to the processes from which it originated.

For example, scrubber liquor may be recycled within the scrubber,
or treated by sedimentation and recycled back to the scrubber.

Total  recycle  may  become  more  wide-spread  in  the future if
methods for removal of dissolved solids, such as reverse  osmosis
and ion exchange, become more common and less expensive.

The  Agency  observed  extensive recycle of contact cooling water
and scrubber liquor throughout the category.  Indeed, some plants
reported 100 percent recycle of  process  wastewater  from  these
operations.   The  Agency believes, however, that most plants may
have to discharge a portion of the recirculating flow to  prevent
the   excessive  build-up  of  dissolved  solids  unless  dragout
of  solids in  products  or  slags  is  sufficient   to   prevent
this build-up.

Existing  practice supports the selection of a 90 percent recycle
rate.   Twenty-nine  of 61 aluminum smelting and  forming  plants
practice  greater  than 90 percent recycle of  the  direct  chill
casting contact cooling water.  Two of the five aluminum smelters
practicing  continuous rod casting recycle 90 percent or more  of
their  contact  cooling water.  Four of  eight  primary  aluminum
plants using wet air pollution control on anode bake ovens,  five
of 11 plants using wet scrubbers on potlines, and three of  eight
plants  using  wet scrubbers for potrooms recycle 90  percent  or
more of their scrubber water.

Five  of 10 primary electrolytic copper plants currently  recycle
90  percent or more of their casting contact cooling water.   Two
of  three primary zinc plants with leaching scrubbers recycle  90
percent  or  more.   Two  of five primary  tungsten  plants  with
scrubbers  on reduction furnaces practice 90 percent  or  greater
recycle.   Six  of  seven  secondary silver plants  with  furnace
scrubbers  currently recycle 90 percent or more of  the  scrubber
water.

Process Water Reuse

Reuse  of  process  water  is the practice of recirculating water
used in one production process for subsequent use in a  different
production process.
Application  and Performance.
process  can   include  using
for  another  application,  or
Reuse of wastewater in a different
a  relatively   clean   wastewater
 using  a relatively  dirty  water
for an application where water quality is of no concern.

Advantages and Limitations.  Advantages of reuse are  similar  to
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
the  advantages  of  recycle.   Water  consumption is reduced and
wastewater treatment facilities can be sized for  smaller  flows.
Also, in areas where water shortages occur, reuse is an effective
means of conserving water.

Operational Factors.  The hardware necessary for reuse of process
wastewaters  varies,  depending on the specific application.  The
basic elements include pumps and piping.   Chemical  addition  is
not  usually  warranted,  unless  treatment  is required prior to
reuse.  Maintenance and energy use are limited to  that  required
by  the  pumps.  Solid waste generated is dependent upon the type
of treatment used and will be discussed separately with each unit
process.

Demonstration  Status.   Reuse  applications  in  the  nonferrous
metals   manfuacturing  category  are  varied.   For  example,  a
secondary uranium facility reuses wastewater from evaporation and
calcination wet air pollution control in  raw  material  leaching
operations.  Bauxite refineries commonly reuse water from red mud
inpoundments  in digestion operations.   A primary aluminum plant
reuses wastewater from casting for air scrubbing.  A lead smelter
uses  wastewater from air scrubbing for slag  granulation,  where
all  the water is evaporated.   A primary copper refinery  reuses
precipitated  spent  electrolyte,   known  as  "black  acid,"  in
leaching operations that are part of an ore beneficiation plant.

Process Water Use Reduction

Process  water  use  reduction  is  the decrease in the amount of
process water used as an influent to  a  production  process  per
unit  of  production.   Section  V  of  each  of  the subcategory
supplements discusses water use in  detail  for  each  nonferrous
metals  manufacturing  operation.   A  range  of water use values
taken from the data collection portfolios is presented  for  each
operation.   The  range  of values indicates that some plants use
process  water  more  efficiently  than  others  for   the   same
operation.

Application   and  Performance.   Noncontact  cooling  water  can
replace contact cooling water i-n some applications.  The  use  of
noncontact  heat exchangers eliminates concentration of dissolved
solids by evaporation and minimizes scaling problems.   A  copper
refinery   is   currently  using  this  method  to  achieve  zero
discharge.   However,  industry-wide  conversion  to   noncontact
cooling  may  not  be  possible  because  of a need for extensive
retrofitting. Certain molten metals require  contact  cooling  to
produce  desired  surface characteristics.  Some plants produce a
metal shot by allowing molten metal to flow through a screen into
a tank of water, immediately quenching the metal and producing  a
spherical  shot  product.   Shot,  generally  cannot  be produced
without contact cooling water.

Air Cooling of Cast Metal Products

Application and Performance.  Air cooling, for  some  operations,
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
is  an alternative to contact cooling water but limited potential
except in low tonnage situations.  For example,  air  cooling  is
not  generally used in the production of high tonnage casting for
several reasons.  The casting line can be inordinately  long  (or
large),  a  result  of an increased number of molds to compensate
for the slower cooling of the metal.

Operational Factors.   Maintenance  costs  are  generally  higher
because  of the longer conveyer, the added heat load on equipment
and lubricants, and the need for added air blowers.  Air  cooling
without these process appurtenances might greatly reduce finished
metal production from rates now possible with water cooling.

Conversion  to  dry  air  pollution  control equipment, discussed
further on in this section, is another  way  to  eliminate  water
use.

         Processing and Granulation

Slag  from pyrometallurgical processes is a solid waste that must
be disposed of or reprocessed.  Slag can be prepared for disposal
by slag granulation or slag dumping.

Application and  Performance.   Slag  granulation  uses  a  high-
velocity  water  jet to produce a finely divided and evenly sized
rock, which can be used  as  concrete  agglomerate  or  for  road
surfacing.    Slag   dumping   is   "the  dumping  and  subsequent
solidification of slag, composed almost entirely  of  insolubles,
which  can  be  crushed  and  sized for such applications as road
surfacing.  Slag can be reprocessed if the metal content is  high
enough  to  be  economically  recovered.  Wet or dry milling, and
recovery of metal by melting can be used  to  process  slag  with
recoverable  amounts  of  metal.   Of  course,  in all slag reuse
processes, ultimate disposal of  the  reprocessed  slag  must  be
considered.                   .  .  .  •

Operational   Factors-.   Although  slag  dumping  eliminates  the
wastewater associated with slag'granulation, an additional factor
is that large volumes of dust  are  generated  during  subsequent
crushing operations and dust control systems may be necessary.

Demonstration  Status.   Four  of the seven primary lead smelters
currently granulate slag prior to  disposal.   One  of  the  four
plants granulates the slag, mixes the granulated slag in with ore
concentrate  feed  to  sintering  to  control lead content of the
feed.

Dry Air Pollution Control Devices

Application and  Performance.   The  use  of  dry  air  pollution
control devices would allow the elimination of waste streams with
high  pollution  potentials.  The choice of air pollution control
equipment is complicated, and  sometimes  a  wet  system  is  the
necessary  choice.    The important, difference between wet and dry
devices is that wet devices control gaseous pollutants as well as
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           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
particulates.

Wet devices may be chosen  over  dry  devices  when  any  of  the
following   factors   are   found:   (1)  the  particle  size  is
predominantly under 20 microns, (2) flammable particles or  gases
are to be treated at minimal combustion risk, (3) both vapors and
particles  are  to  be  removed  from the carrier medium, (4) the
gases are corrosive and may  damage  dry  air  pollution  control
devices,  and  (5)  the  gases  are  hot  and  may damage dry air
pollution control devices.

Equipment for dry control of air emissions includes cyclones, dry
electrostatic precipitators, fabric  filters,  and  afterburners.
These  devices  remove  particulate  matter,  the  first three by
entrapment and the afterburners by combustion.

Afterburner use is limited to air emissions consisting mostly  of
combustible  particles.  Characteristics of the particulate-laden
gas which affect the design and use of a device are gas  density,
temperature,  viscosity,  flammability,  corrosiveness, toxicity,
humidity,  and  dew  point.   Particulate  characteristics  which
affect  the  design and use of a device are particle size, shape,
density, resistivity,  concentration,  and  other  physiochemical
properties.

In  the  primary and secondary  aluminum  subcategories,  melting
prior  to  casting requires wet air pollution control  only  when
chlorine  gas  is present in the  offgases.   Dry  air  pollution
control  methods with inert gas or salt furnace fluxing have been
demonstrated in the category.   It is possible to perform all the
metal   treatment  tasks  of  removing   hydrogen,   non-metallic
inclusions,  and  undesirable trace elements and  meet  the  most
stringent  quality  requirements without furnace  fluxing,  using
only in-line metal treatment units.  To achieve this, the  molten
aluminum  is treated in the transfer system between  the  furnace
and  casting units by flowing the metal through a region of  very
fine,  dense, mixed-gas bubbles generated by a spinning rotor  or
nozzle. .No process wastewater is generated in this operation.  A
schematic   diagram  depicting  the  spinning   nozzle   refining
principle is shown in Figure VII-32 (page xxx).  Another  similar
alternate  degassing  method  is  to  replace  the  chlorine-rich
degassing  agent with a mixture of inert gases and a  much  lower
proportion   of  chlorine.   The  technique   provides   adequate
degassing while permitting dry scrubbing.

To  the extent that nonferrous metals manufacturing processes are
designed to limit the volume or severity of  air  emissions,  the
volume  of scrubber water used for air pollution control also can
be reduced.  For example, new,  or  replacement  furnaces  can  be
designed to minimize emission volumes.

Advantages  and Limitations.  Proper application of a dry control
device can result in  particulate! removal  efficiencies  greater
than  99  percent  by  weight  for fabric filters,  electrostatic
precipitators,  and  afterburners,  and  up  to  95  percent  for
                               233

-------
           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
cyclones.

Common  wet  air  pollution control devices are wet electrostatic
precipitators, venturi scrubbers,  and  packed  tower  scrubbers.
Collection  efficiency for gases will depend on the solubility of
the contaminant  in  the  scrubbing  liquid.   Depending  on  the
contaminant removed, collection efficiencies usually approach  99
percent for particles and gases.

Demonstration   Status.   Plants  in  the primary  and  secondary
aluminum, primary zinc, primary lead, secondary copper, secondary
silver,  primary  precious  metals  and  mercury,  and  secondary
precious  metals  subcategories all  report  the use of  dry  air
pollution control devices on furnaces and smelting operations.

Good Housekeeping

Good  housekeeping and proper equipment maintenance are necessary
factors  in  reducing  wastewater  loads  to  treatment  systems.
Control  of  accidental  spills  of  oils, process chemicals, and
wastewater from washdown and filter cleaning or removal  can  aid
in  abating or maintaining the segregation of wastewater streams.
Curbed areas should be used to contain or control these wastes.

Leaks in pump casings, process piping, etc., should be  minimized
to  maintain efficient water use.  One particular type of leakage
which may cause a water pollution problem is the contamination of
noncontact cooling water by hydraulic oils,  especially  if  this
type of water is discharged without treatment.

Good housekeeping is also important in chemical, solvent, and oil
storage  areas  to  preclude  a  catastrophic  failure situation.
Storage areas should be isolated from high fire-hazard areas  and
arranged  so  that  if  a  fire  or  explosion  occurs, treatment
facilities will not  be  overwhelmed  nor  excessive  groundwater
pollution  caused  by  large  quantities  of chemical-laden fire-
protection- water.

A conscientiously applied program of water use reduction can be a
very effective method of curtailing unnecessary wastewater flows.
Judicious use of  washdown  water  and  avoidance  of  unattended
running hoses can significantly reduce water use.
                               234

-------
GENERAL DEVELOPMENT DOCUMENT

pH CONTROL
Day 1
In Out
pH Ranqe 2.4-3.4 8.5-8.
(mg/1)
TSS 39 8
Copper 312 0.22
Zinc 250 0.31

TABLE VII-1
SECT -

VII



EFFECT ON METALS REMOVAL
Day 2
In
7 1.0-3.0 5.

16
120
32.5
TABLE VI.I-2
EFFECTIVENESS OF SODIUM HYDROXIDE
Day 1
In Out
pH Range 2.1-2.9 9.0-9.
(mg/1)
Cr 0.097 0.0
Cu 0.063 O.O18
Fe 9.24 0.76
Pb 1.0 0.11
Mn 0.11 0.06
Ni 0.077 0.011
Zn 0.054 0.0
TSS 13
Day 2
In
3 2.0-2.4 8.
0.057 0
0.078 0
15.5 0
1.36 0
0.12 0
0.036 0
0.12 0
11
Out
0-6.0 2.

19
Day
In
0-5.0 6

16
5.12 107
25.0 43.8

FOR METALS
Out
7-9.1 2.
.005 0
.014 0
.92 9
.13 1
.044 0
.009 0
.0 0


REMOVAL
Day 3
In
0-2.4 8
.068
.053
.41
.45
.11
.069
.19

3
Out
. 5— 8 . 1

7
0.66
0.66


Out
.6-9.1
0.005
0.019
0.95
0.11
0.044
0.011
0.037
11
235

-------
           GENERAL DEVELOPMENT DOCUMENT
                                            SECT - VII
                           TABLE VI1-3

  EFFECTIVENESS OF LIME AND SODIUM HYDROXIDE FOR METALS  REMOVAL
                 Day 1
                                    Day  2
                     Day 3


In
pH range 9.2-9.6
(xng/1)
Al
Co
Cu
Fe
Mn
Ni
Se
Ti
Zn
37
3
0
137
175
6
28
143
18
.3
.92
.65


.86
.6

.5
Out
8.3-9.8
O.
0.
0.
0.
0.
0.
0.
0.
0.
35
0
003
49
12
0
0
0
027
In
9.
38.
4.
0.
110
205
5.
30.
125
16.
2
1
65
63


84
2

2
7.
0
0
0
0
0
0
0
0
0
Out
6-8.1
.35
.0
.003
.57
.012
.0
.0
.0
.044
In
9.
29.
4.
0.
208
245
5.
27.
115
17.
6
9
37
72


63
4

0
Out
7.8-8.2
0.35
0.0
0.003
0.58
0.12
0.0
0.0
0.0
0.01
TSS
          4390
3595
13
2805
13
                             TABLE VII-4

       THEORETICAL SOLUBILITIES OF HYDROXIDES AND SULFIDES
                OF SELECTED METALS IN PURE WATER
Metal

Cadmium (Cd++)
Chromium (Cr   )
Cobalt (Co++)

Copper (Cu++)
Iron (FeJJ)
Lead (Pb++)

Manganese  (Mn~*"+)
Mercury (Hg++)
Nickel    *"1"
Silve
Tin (
Zinc
          +>
                        Splubility of metal ion, me
                                   As Carbonate
As
2.
8.
2.
2.
8.
2.
1.
3.
6.
13.
1.
1.
Hydroxide
3
4
2
2
9
1
2
9
9
3
1
1
x
X
X
X
X


X
X

X

10
10
10
10
10


10
10

10

-5
-4
-1
-2
-1


-4
-3

-4

                                   10 x 10
                                          -4
                                  7.0 x 10
                                          -3
                                  3.9 x 10
                                  1.9 x 10
           -2
           -1
                                          -1
                                  2.1 x 10

                                  7.0 x 10~4
                     As Sulfide

                    6.7 x lO"10
                 No precipitate
                    1.0 x 10~8
5
3
3
2
9
6
7
3
2
.8
.4
.8
.1
.0
.9
.4
.8
.3
x
x
X
X
X
X
X
X
X
10
10
10
10
10
10
10
10
10
-18
-5
-9
-3
-20
-8
-12s
— ft
-7
                               236

-------
           GENERAL DEVELOPMENT DOCUMENT
SECT - VII
                           TABLE VI1-5

                   SAMPLING DATA FROM SULFIDE
               PRECIPITATION-SEDIMENTATION SYSTEMS
              Lime, FeS,       Lime, FeS/       NaOH, Ferric
           Polyelectrolyte, Polyelectrolyte, Chloride, Na2§
Treatment  Settle, Filter   Settle, Filter   Clarify (1 stage)
+ In Out
pH 5.0-6.8 8-9
Cr*6 25.6 <0.014
Cr 32.3 <0.04
Cu
Fe 0.52 0.10
Ni
Zn 39.5 <0.07
These data were obtained
Summary Report, Control
Metal Finishing Industry:
In Out
7.7 7.38
0.022 <0.020
2.4 <0.1
',; .-- '
108 0.6
0.68 <0.1
33.9 0.01
In

11.45
18.35
0.029


0.060
Out

<.005
<.005
0.003


0.009
from three sources:
and Treatment
Technology
for
Sulfide Precipitation, USEPA, E
                                                              the
625/8/80-003, 1979.

Industrial Finishing, Vol. 35, No. 11, November, 1979.

Electroplating sampling data from plant 27045.
                               237

-------
           GENERAL DEVELOPMENT DOCUMENT
        SECT - VII
                           TABLE VII ^6

         SULFIDE PRECIPITATION-SEDIMENTATION PERFORMANCE

              Parameter    Treated Effluent  (mq/1)
                  Cd
                  Cr (T)
                  Cu

                  Pb
                  Hg
                  Ni

                  Ag
                  Zn
0.01
0.05
0.05

0.01
0.03
0.05

0.05
0.01
Table VII-6 is based on two reports:

Summary   Report/   Control  and  Treatment  Technology  for  the
Metal  Finishing  Industry;  Sulfide  Precipitation/  USEPA,  EPA
No. 625/8/80-003, 1979.

Addendum  to  Development Document   for   Effluent   Limitations
Guidelines   and   New  Source   Performance   Standards/   Major
Inorganic   Products   Segment  of   Inorganics   Point    Source
Category/  USEPA.,  EPA Contract No.  EPA  68-01-3281  (Task  7),
June/ 1978.
                               238

-------
           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - VII
Metal

Mercury
Cadmium
Copper

Zinc
Chromium
Manganese

Nickel
Iron
Bismuth

Lead
                           TABLE VII-7

              FERRITE CO-PRECIPITATION PERFORMANCE

               Influent (mg/1)      Effluent (mg/1)
    7.4
  240
   10

   18
   10
   12
1,000
  600
  240

  475
                                       0.001
                                       0.008
                                       0.010

                                       0.016
                                      <0.010
                                       0.007

                                       0.200
                                       0.06
                                       0.100

                                       0.010
NOTE: These data are from:
Sources and Treatment of Wastewater in the Nonferrous
Metals Industry, USEPA, EPA No. 600/2-80-074, 1980.
                           TABLE VII-8

                CONCENTRATION OF TOTAL CYANIDE
                            (mg/1)
       Plant

       1057



       33056


       12052


       Mean
                    Method
                     FeS04
                   In

                  2.57
                  2.42
                  3.28

                  0.14
                  0.16

                  0.46
                  0.12
 Out

0.024
0.015
0.032

0.09
0.09

0.14
0.06

0.07
                               239

-------
            GENERAL DEVELOPMENT DOCUMENT
                               SECT - VII
                            TABLE VI1-9

                   MULTIMEDIA FILTER PERFORMANCE

        Plant ID £     TSS Effluent Concentration,  mg/1

          06097      0.0,  0.0, 0.5
          13924      1.8,  2.2, 5.6,  4.0, 4.0,  3.0,  2.2,  2.8
                    3.0,  2.0, 5.6,  3.6, 2.4,  3.4

          18538      1.0
          30172      1.4,  7.0, 1.0
          36048      2.1,  2.6, 1.5

          mean      2.61
PLANT ID
01057
09025
11058


12075

19019

33617
40063
.44062
46050
              TABLE VII-10

PERFORMANCE OF SELECTED SETTLING SYSTEMS

 SETTLING   SUSPENDED SOLIDS CONCENTRATION (mg/1)
)EVICE

Lagoon
Clarifier .
& Settling
Ponds
Clarifier
Settling
Pond
Settling
Tank
Clarifier
& Lagoon
Clarifier
Clarifier
Settling
Tank
Day
in
54
1100


451
284

170



4390
182
295

1
Out
6
9


17
6

1



9
13
10

Day
1
56
1900



242

50

1662

3595
118
42

2
Out
6
12



10

1

16

12
14
10

Day
In
50
1620



502



1298

2805
174
153

3
Out
5
5



14



4

13
23
8

                               240

-------
     GENERAL DEVELOPMENT DOCUMENT'
                                      SECT - VII
                     TABLE VII-11

                 SKIMMING PERFORMANCE

                             Oil & Grease
  Plant

  06058
  06058
              Skimmer Type      In
                  API
                  Belt
224,669
     19.4
 (mg/1)
Out

17.9
 8.3
                     TABLE VII-12

            SELECTED PARITION COEFFICIENTS
Priority Pollutant

  1  Acenaphthene
 11  1,1,1-Trichloroethane
 13  1,1-Dichloroethane
                            Log Octanol-Water
                            Partition Coefficient

                                  4.33
                                  2.17
                                  1.79
15  1,1,2,2-Tetrachloroethane     2.56
18  Bis(2-chloroethyl)ether       1.58
23  Chloroform                    1.97

29  1,1-Dichloroethylene          1.48
39  Fluoranthene                  5.33
44  Methylene chloride            1.25

64  Pentachlorophenol            : 5.01
66  Bis(2-ethylhexyl)
    phthalate                     8.73
67  Butyl benzyl phthalate        5.80

68  Di-n-butyl phthalate          5.20
72  Benzo(a)anthracene            5.61
73  Benzo(a)pyrene                6.04

74  3,4-benzofluoranthene         6.57
75  Benzo(k)fluoranthene          6.84
76  Chrysene                      5.61

77  Acenaphthylene                4.07
78  Anthracene                    4.45
79  Benzo(ghiJperylene            7.23

80  Fluorene                      4.18
81  Phenanthrene                  4.46
82  Dibenzo(a,h)anthracene        5.97

83  lndeno(l,2,-.3, cd)pyrene        7.66
84  Pyrene                        5.32
85  Tetrachloroethylene           2.88

86  Toluene                       2.69
                         241.-

-------
    GENERAL DEVELOPMENT  DOCUMENT
                               SECT  - VII
                    TABLE  VII-13

         TRACE  ORANIC  REMOVAL  BY  SKIMMING
               API  PLUS  BELT SKIMMERS
                 (From Plant 06058)
 Pollutant
Oil  &  Grease
Chloroform
Methylene Chloride

Naphthalene
N-nitrosodiphenylamine
Bis-2-ethylhexyl phthalate

Diethyl phthalate
Butylbenzyl phthalate
Di-n-octyl phthalate

Anthracene - phenanthrene
Toluene
                            Influent
                             (mg/1)

                       225,000
                             0.023
                             0.013
                             2.31
                            59.0
                            11.0
                              0.005
                              0.019

                             16.4
                              0.02
                                Effluent
                                  (mg/1)

                                  14.6
                                  0.007
                                  0.012
                                  0.004
                                  0.182
                                  0.027
                                  0.002
                                  0.002

                                  0.014
                                  0.012
                   TABLE VII-14

   COMBINED METALS DATA EFFLUENT VALUES (mg/1)
Cd
Cr
Cu

Pb
Ni
Zn
Mean

0.079
0.084
0.58

0.12
O.74
0.33
Fe   0.41
Mn   0.16
TSS 12.0
One Day
   Max.

   0.34
   0.44
   1.90

   0.42
   1.92
   1.46

   1.20
   0.68
  41.0
10 Day Avg,
     Max.

     0.15
     0.18
     1.00

     0.20
     ].27
     0.61

     0.61
     0.29
    19.5
30 Day Avg,
   Max.

   0.13
   0.12
   0.73

   0.16
   1.00
   0.45

   0.50
   0.21
  15.5 .
                       242

-------
           GENERAL DEVELOPMENT DOCUMENT
                           SECT - VII
                           TABLE VI1-15

                         L&S PERFORMANCE
                      ADDITIONAL POLLUTANTS
                             (mg/1)
    Pollutant

     Sb
     As
     Be

     Hg
     Se
     Ag

     Th
     Al
     Ba

     B
     Cz
     Co

     Nb
     F
     Ga

     Ge
     Au
  Average
Performance

     0.7
     0.51
     0.30

     0.06
     0.30
     0.10

     0.50
     2.24
     0.42

     0.36
     0.124
     0.05

    0.12
    14.5
     0.084

     0.084
     0.01
Pollutant

   Hf
   In
   Mo

   Pd
   P
   Pt

   Ra-226
   Re
   Rb

   Ta
   Sn
   Ti

   W
   U
   V

   Xr
  Average
Performance

   7.28
   0.084
   1.83

   0.01
   4.08
   0.01

   6.17
   1.83
   0.124

  <0.12
   0.14
   0.19

   1.29
   4.0
  <0.10

   7.28
NOTE: Ra-226 is in picocurries per liter




                           TABLE VI1-16

         COMBINED METALS DATA SET - UNTREATED WASTEWATER
         Pollutant

            Cd
            Cr
            Cu

            Pb
            Ni
            Zn

            Fe
            Mn
            TSS
       Min. Cone,  (mg/1)
            <0.1
            <0.1
            <0.1
             4.6
        Max. Cone,  (mg/1)

            3.83
          116
          108

           29.2
           27.5
          337

          263
            5.98
        4,390
                               243

-------
GENERAL DEVELOPMENT DOCUMENT   SECT - V









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-------
    GENERAL DEVELOPMENT DOCUMENT
SECT - VII
                    TABLE VI1-18

PRECIPITATION-SETTLING-FILTRATION (LS&F) PERFORMANCE
                      Plant A
Parameters No Pts
For 1979-Treated
Cr
Cu
Ni
Zn
Fe
For 1978-Treated
Cr
Cu
Ni
Zn
Fe
Raw Waste
Cr
Gu
Ni
Zn
Fe
Range mq/
1
Mean +_
std. dev
Mean + 2
std. dev.
Wastewater
47
12
47
47

0.
0.
0.
0.

015 -
01 -
08 -
08 -

0.
0.
0.
0.

13
03
64
53

0.
0.
ft.
0.

045
019
22
17

+0
+ 0
+ 0
+ 0

.029
.006
.13
.09

0.10
0.03
0.48
0.35

Wastewater
47
28
47
47
21

5
5
5
5
5
0.
0.
0.
0.
0.

32.
0.
1.
33.
10.
01 -
005 -
10 -
08 -
26 -

0
08 -
65 -
2
0
0.
0.
0.
2.
1.

72
0
20
32
95
07
055
92
3.5
1

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.45
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.0
.0
0.
0.
0.
0.
0.






06
016
20
23
49






+
+"
T
T
T






0.10
0.010
0.14
0.34
0.18






0.26
0.04
0.48
0.91
0.85






                        245

-------
     GENERAL DEVELOPMENT DOCUMENT
SECT - VII
                    TABLE VI1-19

PRECIPITATION-SETTLING-FILTRATION (LS&F) PERFORMANCE
                       Plant B
Parameters
No Pts.
Range mq/1
Mean +_
std. dev.
For 1979-Treated Wastewater
Cr
Cu
Ni
Zn
Fe
TSS
175
176
175
175
174
2
0.0
0.0
0.01
0.01
0.01
1.00
- 0.40
- 0.22
- 1.49
- 0.66
- 2.40
- 1.00
0.068 +0.075
0.024 +0.021
0.219 +0.234
0.054 +0.064
0.303 +0.398

For 1978-Treated Wastewater
Cr
Cu
Ni
Zn
Fe
144
143
143
131
144
Total 1974-1979-Treated
Cr
Cu
Ni
Zn
Fe
Raw Waste
Cr
Cu
Ni
Zn
Fe
TSS
1288
1290
1287
1273
12B7

3
3
3
2
3
2
0.0
0.0
0.0
0.0
0.0
- 0.70
- 0.23
- 1.03
- 0.24
- 1.76
0.059 +0.088
0.017 +0.020
0.147 +0.142
0.037 +0.034
0.200 +0.223
Wastewater
0.0
0.0
0.0
0.0
0.0

2.80
0.09
1.61
2.35
3.13
177
- 0.56
- 0.23
- 1.88
- 0.66
- 3.15

- 9.15
- 0.27
- 4.89
- 3.39
- 35.9
- 466.
0.038 +0.055
0.011 +0.016
0.184 +0.211
0.035 +0.045
0.402 +0.509

5.90
0.17
3.33

22.4

                                                 Mean + 2
                                                 std. dev,
                                                   0.22
                                                   0.07
                                                   0.69
                                                   0.18
                                                   1.10
                                                   0.24
                                                   0.06
                                                   0.43
                                                   0.11
                                                   0.47
                                                   0.15
                                                   0.04
                                                   0.60
                                                   0.13
                                                   1.42
                         246

-------
           GENERAL DEVELOPMENT DOCUMENT
                            SECT - VII
                          TABLE VI1-20

      PRECIPITATION-SETTLING-FILTRATION (LS&F) PERFORMANCE
                             Plant C
Parameters
No Pts.
Range (mg/1)
Mean +_
  std. dev.
For Treated Wastewater
Cd
Zn
TSS
PH
103
103
103
103
0.010 -
0.039 -
0.100 -
7.1
                                  0.500  0.049
                                  0.899  0.290
                                  5.00   1.244
                                  7.9    9.2*
                                 +0.049
                                 +0.131
                                 +1.043
                                                       Mean + 2
                                                        std. dev,
                               0.147
                               0.552
                               3.33
For Untreated Wastewater
Cd
Zn
Fe
TSS
pH
103
103
3
103
103
0
0
0
0
6
.039
.949
.107
.80
.8
- 2
- 29
- 0
- 19
- 8
.319
.8
.46
.6
.2
0
11
0
5
7
.542
.009
.255
.616
.6*
+ 0.
+6.

+ 2.

381
933

896

1.
24.

11.

304
956

408

* pH value is median of 103 values.
                                247

-------
GENERAL DEVELOPMENT DOCUMENT
SECT - VII
SUMMARY OF TREATMENT EFFECTIVENESS (mg/1)
L £ S Technology System L S & F Technology System Sulfide & Filter Technology System
Pollutant One-day 10-day 30-day One-day 10-day 30-day One-day 10-day 30-day
Parameter Mean Maximum Average Average Mean Maximum Average Average Mean Maximum Average Average
vo in CN
r*- m ro
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000
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cn
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cocno
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CN in
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CN VO
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r- VD
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rH rH rH
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rH CN rH
O CD O
cn oj in
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r- CN vo
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0 CM K
rH CN CO'
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cn cn
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cn ro o
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cn co o
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CD rH O
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VD CN CO
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rH rH
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VD
CN
O 0
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0
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in
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in
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CO
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CN O O
ro
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rH 2; a
CN
in
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in
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CM 0 0

-------
               GENERAL DEVELOPMENT DOCUMENT
                                               SECT -  VII
                          TABLE VII-22

           TREATABILITY RATING OF PRIORITY POLLUTANTS
                   UTILIZING CARBON ADSORPTION
Priority Pollutant
 1.
 2.
 3.
 4.
 5.
 6.
 7.
 8.
 9.
10.
11.
12.
13.
14.
15.
16.
18.
19.
20.
21.
22.
23.
24.
25.
26.
27.
28.
29.
30.
31.
32.
33.
34.
35.
36.
37.
38.
39.
40.
41.
42.
43.
44.
45.
46.
47.
 acenaphthene
 acrolein
 acrylonitrile
 benzene
 benzidene
 carbon tetrachloride
 chlorobenzene
 1,2,4-trichlorobenzene
 hexachlorobenzene
 1,2-dichloroethane
 1,1,1-trichloroethane
 hexachloroethane
 1,1-dichloroethane
 1,1,2-trichloroethane
 1,1,2,2-tetrachloroethane
 chloroethane
 bis  (2-chloroethyl) ether
 2-chloroethyl vinyl ether
 2-chloronaphthalene
 2,4,6-trichlorophenol
 parachlorometa cresol
H
L
L
M
H
H
H
H
H
M
M
H
M
M
H
L
M
L
H
H
H
 chloroform (trichloromethane) L
 2-chlorophenol                H
 1,2-dichlorobenzeneH
 1,3-dichlorobenzene           H
 1,4-dichlorobenzene           H
 3,3'-dichlorobenzidine        H
 1,1-dichloroethylene         L
 1,2-trans-dichloroethylene    L
 2,4-dichlorophenol            H
 1,2-dichloropropane           M
 1,2-dichloropropylene         M
 2,4-dimethylphenol            H
 2,4-dinitrotoluene            H
 2,6-dinitrotoluene            H
 1,2-diphenylhydrazine         H
 ethylbenzene                  M
 fluoranthene                  H
 4-chlorophenyl  phenyl ether   H
 4-broraophenyl phenyl ether    H
 bis(2-chloroisopropyl)  ether  M
-bis(2-choroethoxy) methane    M
 methylene  chloride            L
 methyl  chloride              L
 methyl  bromide                L
 bromoform  (tribromomethane)   H
48.  dichlorobromomethane          M
51.  chlorodibromomethane          H
52.  hexachlorobutadiene           H
53.  hexachlorocyclopentadiene     H
54.  isophorone                    H
55.  naphthalene                   H
56.  nitrobenzene                  H
57.  2-nitrophenol                 H
58.  4-nitrophenol                 H
59.  2,4-dinitrophenol             H
60.  4,6-dinitro-o-cresol          H
61.  N-nitrosodimethylamine        M
62.  N-nitrosodiphenylamine        H
63.  N-nitrosodi-n-propylamine     M
64.  pentachlorophenol             H
65.  phenol                        M
66.  bis(2-ethylhexyl) phthalate   H
67.  butyl benzyl phthalate '       H
68.  di-n-butyl phthalate          H
69.  di-n-octyl phthalate          H
70.  diethyl phthalate             H
71.  dimethyl phthalate            H
72.  benzo (a)anthracene           H
73.  benzo (a)pyrene               H
74.  3,4-benzofluoranthene         H
75.  benzo(k)fluoranthane          H
76.  chrysene                      H
77.  acenaphthylene                H
78.  anthracene                    H
79.  benzo(ghi)perylene            H
80.  fluorene                      H
81.  phenanthrene                  H
82.  dibenzo (a,h)anthracene       H
83.  indeno (l,2,3-cd)pyrene       H
84.  pyrene
85.  tetrachloroethylene           M
86.  toluene                       M
87.  trichloroethylene             L
88.  vinyl chloride                L
106.  PCB-1242 (Arochlor 1242)     H
107.  PCB-1254 (Arochlor 1254)     H
108.  PCB-1221 (Arochlor 1221)     H
109.  PCB-1232 (Arochlor 1232)     H
110.  PCB-1248 (Arochlor 1248)     H
111.  PCB-1260 (Arochlor 1260)     H
112.  PCB-1016 (Arochlor 1016)     H
    Category  H
        Adsorbs
        Adsorbs
    Category  M
        Adsorbs
        Adsorbs
    Category  L
        Adsorbs
        Adsorbs
    Cf = final
           (high removal)
            at levels >100 mg/g carbon  at  Cf =10 mg/1
            at levels >100 mg/g carbon  at  Cf <10 mg/1
           (high removal)
            at levels >100 mg/g carbon  at  Cf =10 mg/1
            at levels <100 mg/g carbon  at  Cf <10 mg/1
           (high removal)
            at levels <100 mg/g carbon  at  Cf =10 mg/1
            at levels <100 mg/g carbon  at  Cf <10 mg/1
           concentration of priority pollutant  at equilibrium.
                              249

-------
           GENERAL DEVELOPMENT DOCUMENT
        SECT - VII
                          TABLE VI1-23

         CLASSES OF ORGANIC COMPOUNDS ADSORBED ON CARBON
Organic Chemical Class

Aromatic Hydrocarbons

Polynuclear Hydrocarbons


Chlorinated Aromatics


Phenolics


Chlorinated Phenolics
High Molecular Weight Alphatic
and Branch Chain Hydrocarbons
Example of Chemical Class

Benzene, toluene, xylene

Napthalene, anthracene,
biphenols

Chlorobenzene, pollychlorinated
biphenyls, aldrin, endrin

Phenol, cresol, resorcenol,
polyphenyls

Trichlorophenol,
pentachlorophenol

Gasoline, kerosine
Chlorinated Alphatic Hydrocarbons  Carbon tetrachloride,
                                   chlorethylenes
High Molecular Weight Alphatic
Acids and Aromatic Acids

High Molecular Weight Alphatic
Amines and Aromatic Amines

High Molecular Weight Ketones,
Esters, Ethers and Alcohols

Surfactants

Soluble Organic Dyes
Tar acids, benzoic acid


analine, toluene, diamine


Hydroquinone, polyethylene
glycol

alkyl benzene sulfonates

Melkylene blue, Indigo carmine
High molecular weight includes compounds in the broad range  from
four to 20 carbon atoms.
                               250

-------
   GENERAL DEVELOPMENT DOCUMENT
                   SECT - VII
                  TABLE VII-24

     ACTIVATED CARBON PERFORMANCE (MERCURY)

    Plant          Mercury levels (mg/1)
    A
    B
    C
   28.0
    0.36
    0.008
         0.9
         0.015
         0.0005
Parameter
                  TABLE VII-25

            ION EXCHANGE PERFORMANCE
                     (mg/1)
                  Plant A
In
Out
                     Plant B
In
Out
Al
2+3
Cr+6
Cu
CN
Au
Fe
Pb
Mn
Ni
Ag
S04
Sn
Zn
5.6
5.7
3.1
7.1
4.5
9.8
—
7.4
—
4.4
6.2
1.5
1.7
14.8
0.20
0.00
0.01
0.01
0.09
0.04
_
0.01
—
0.00
0.00
13.00
0.00
0.40
_
-
«.
43.0
3.40
2.30
_
1.79
_
1.60
9.10
210.00
1.10
-
_
""*
_
0.10
0.09
0.10
• -
0.01
_
0.01
0.01
2.00
0.10
-
                       251

-------
           GENERAL DEVELOPMENT DOCUMENT
                                SECT - VII
                          TABLE VII-26
               MEMBRANE FILTRATION SYSTEM EFFLUENT
Specific
Metal
Cr (T)
Cu

Fe
Pb
CN

Ni
Zn
TSS
Manufacturers
  Guarantee
Plant 19066
 In    Out
Plant 31022
 In    Out
Predicted
Performance
0.5
0.02
0.03
0.1
0.1
0.05
0.02
0.1
0.1


0.46
4.13
18.8
288
0.652
<0.005
9.56
2.09
632

0.01
0.018
0.043
0.3
0.01
<0.005
0.017
0.046
0.1

5.25
98.4
8.00
21.1
0.288
<0.005
194
5.00
13.0

<0.005
0.057
0.222
0.263
0.01
<0.005
0.352
0.051
8.0


0.05
0.02
0.30
0.05
0.02
0.40
0.10
1.0
                          TABLE VII-27

                   PEAT ADSORPTION PERFORMANCE
                             (mg/1)
             Pollutant
                Cr
                Cu
                CN
                Pb
                Hg
                Ni

                Ag
                Sb
                Zn
                  +6
                       In

                    35000
                      250
                       36.0

                       20.0
                        1.0
                        2.5

                        1.0
                        2.5
                        1.5
                    Out

                    0.04
                    0.24
                    0.7

                    0.025
                    0.02
                    0.07

                    0.05
                    0.9
                    0.25
                               252

-------
           GENERAL DEVELOPMENT DOCUMENT
                        SECT - VII
     Parameter
       TABLE VI1-28

ULTRAFILTRATION PERFORMANCE

        Feed (mg/1)       Permeate (mg/1)
Oil (Freon extractable)    1230
COD                        8920
TSS                        1380
Total Solids               2900
                               4
                             148
                              13
                             296

-------
        GENERAL DEVELOPMENT DOCUMENT     SECT -  VII
  10
  101 —
                           7    a    9   10   n
FIGURE VII-1. COMPARATIVE SOLUBILITIES OF METAL HYDROXIDES
             AND SULFIDE AS A FUNCTION OF pH
                         254

-------
GENERAL DEVELOPMENT  DOCUMENT
SECT  -  VII
















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          GENERAL DEVELOPMENT DOCUMENT     SECT - VII
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        FIGURE VII- 3 LEAD SOLUBILITY IN THREE ALKALIES
                            256

-------
GENERAL DEVELOPMENT DOCUMENT     SECT - VII
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-------
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-------
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-------
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-------
GENERAL  DEVELOPMENT  DOCUMENT     SECT  -  VII
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-------
  GENERAL DEVELOPMENT DOCUMENT
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-------
             GENERAL DEVELOPMENT DOCUMENT
                     SECT  - VII
EFFLUENT
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                             LEVEL
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                                267

-------
            GENERAL  DEVELOPMENT DOCUMENT    SECT - VII
 PERFORATED
 BACKING PLATE
FABRIC
FILTER MEDIUM
              \
  SOLID
  RECTANGULAR
  END PLATE
INLET
SLUDGE
                                                  FABRIC
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                                                 ENTRAPPED SOLIDS
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                                                 PRESSED TOGETHER DURING
                                                 FILTRATION CYCLE
                                                 RECTANGULAR
                                                 METAL PLATE
                                           RECTANGULAR FRAME
                 FIGURE VII-15. PRESSURE FILTRATION
                                268

-------
              GENERAL  DEVELOPMENT DOCUMENT     SECT -  VII
SEDIMENTATION BASIN

         INLET ZONE
   INLET LIQUID
                             BAFFLES TO MAINTAIN
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                                                          OUTLET ZONE
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                         REMOVED
                            SLUDGE DRAWOFF
        FIGURE VII-16.  REPRESENTATIVE TYPES OF SEDIMENTATION
                                  269

-------
        GENERAL DEVELOPMENT DOCUMENT
SECT - VII
                                      FLANGE
WASTE WATER
 WASH WATER
                                           SURFACE WASH
                                           MANIFOLD
    BACKWASH
         INFLUENT
         DISTRIBUTOR
                                                BACKWASH
                                                REPLACEMENT CARBON
                                        CARBON REMOVAL PORT
                                                w-TREATED WATER
                                           SUPPORT PLATE
     FIGURE VII-17.  ACTIVATED CARBON ADSORPTION COLUMN
                           270

-------
GENERAL DEVELOPMENT DOCUMENT    SECT - VII
CONVEYOR DRIVE

  I—BOWL DRIVE
                                        LIQUID
                                        OUTLET
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                              REGULATING
                              RING
                                         IMPELLER
    FIGURE VII-18. CENTRIFUGATION
                271

-------
GENERAL DEVELOPMENT DOCUMENT
SECT -  VII
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-------
       GENERAL DEVELOPMENT DOCUMENT     SECT - VII
    CONTROLS
                   OZONE
                 GENERATOR
     DRY AIR
                       D
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REACTION
TANK
      RAW WASTE-
                                          *. ^
                                        —CXI
                 TREATED
                 WASTE
         x
FIGURE VII-20.  TYPICAL OZONE PLANT FOR WASTE TREATMENT
                        273

-------
GENERAL DEVELOPMENT DOCUMENT
                                          SECT - VII
               MIXER
WASTEWATER
FEED TANK
                                EXHAUST
                                GAS
                           TEMPERATURE
                           CONTROL

                           PH MONITORING
                           TEMPERATURE
                           CONTROL-

                           PH MONITORING
                           TEMPERATURE
                           CONTROL

                           PH MONITORING
                       OZONE
                                    OZONE
                                    GENERATOR
       TREATED WATER
       FIGURE VII-21. UV/OZONATION
                  274

-------
GENERAL DEVELOPMENT DOCUMENT
SECT  -  VII
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                    275

-------
                GENERAL DEVELOPMENT DOCUMENT.
SECT - VII
OILY WATER
INFLUENT
                                             WATER
                                             DISCHARGE
                                  OVERFLOW
                                  SHUTOFF
                                  VALVE
                                               AIR IN
                                                          BACK PRESS
                                                          VALVE
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      TANK   "
                                                               EXCESS
                                                               AIR OUT
                                                               LEVEL
                                                               CONTROLLER
                FIGURE VII-23. DISSOLVED AIR FLOTATION
                                  276

-------
            GENERAL DEVELOPMENT  DOCUMENT  ,  SECT - VII
  CONDUIT
  TO MOTOR
INFLUENT
 CONDUIT TO
 OVERLOAD
 ALARM
                                         COUNTERFLOW
                                         INFLUENT WELL
                                              DRIVE UNIT
                      OVERLOAD ALARM

                         EFFLUENT WEIR
                             DIRECTION OF ROTATION
    EFFLUENT PIPE
                                                    EFFLUENT CHANNEL
                                    PLAN
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 INFLUENT 	•
 CENTER COLUMN
  CENTER CAGE
                                                              WEIR
                 STILTS

                 CENTER SCRAPER
                                                             SQUEEGEE
SLUDGE PIPE
                  FIGURE VII-24.  GRAVITY THICKENING
                                277

-------
                 GENERAL DEVELOPMENT DOCUMENT
 SECT  - VII
 WASTE WATER CONTAINING
' DISSOLVED METALS OR
 OTHER IONS
                                              DIVERTER VALVE
     REGENERANT
     SOLUTION
                                                   DISTRIBUTOR
                                                   SUPPORT
     REGENERANT TO REUSE.
     TREATMENT. OR DISPOSAL
                                              -DIVERTER VALVE
METAL-FREE WATER
FOR REUSE OR DISCHARGE
               FIGURE VII - 25.  ION EXCHANGE WITH REGENERATION
                                    278

-------
          GENERAL DEVELOPMENT DOCUMENT   SECT - VII
                           MACROMOLECULES
                           AND SOLIDS
MEMBRANE
                                          AP - 450 PSlI
                          WATER
        PERMEATE (WATER)
   FEED-
                 o . •
                                MEMBRANE CROSS SECTfON.
                                IN TUBULAR, HOLLOW TIBER,
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                                . o
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                                      o
          ••!'••     -r        -t
        O SALTS OR SOLIDS

        • WATER MOLECULES
       FIGURE VII-26. SIMPLIFIED REVERSE OSMOSIS SCHEMATIC
                        279

-------
                   GENERAL DEVELOPMENT DOCUMENT
                                          SECT  -VII
                         PERMEATE
                         TUBE
                  FEED
      PERMEATE
               FLOW
                           ADHESIVE BOUND

                                  SPIRAL MODULE
                                                        CONCENTRATE
                                                        FLOW
                                               BACKING MATERIAL
                                       •MESH SPACER
                                 •MEMBRANE

                             SPIRAL MEMBRANE MODULE
                                PRODUCT WATER
           POROUS SUPPORT TUBE   PERMEATE FLOW
           WITH MEMBRANE
             .'.•* BRACKISH
             *   WATER
                FEED FLOW
                                                             BRINE
                                                             CONCENTRATE
                                                             FLOW
                                 PRODUCT WATER

                         TUBULAR REVERSE OSMOSIS MODULE
   SNAP
   RING

"O" RING
SEAL
                                                  OPEN ENDS
                                                  OF FIBERS
                                                   ,— EPOXY
                                                     TUBE SHEET
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                                                         BACK-UP DISC
                                                              SNAP
                                                              RING
CONCENTRATE
OUTLET
   END PLATE
                         POROUS FEED
                         DISTRIBUTOR TUBE —'
                                                                         PERMEATE
                                                                        END PLATE
                              HOLLOW FIBER MODULE
           FIGURE VII - 27.  REVERSE OSMOSIS MEMBRANE CONFIGURATIONS
                                     . 280

-------
         GENERAL DEVELOPMENT  DOCUMENT
                                     SECT  - VII
     6-IN. VITRIFIED PIPE LAID-
     WITH PLASTIC JOINTS
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                                  3-IN. COARSE SAND
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                                  3 TO 6 IN. COARSE GRAVEL
                                                V
  /*

J
                                                    2-IN. PLANK
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                                         6-IN. UNDERDRAIN LAID
                                         WITH OPEN JOINTS
                             SECTION A-A
              FIGURE  VII-28.  SLUDGE DRYING BED
                               281

-------
        GENERAL  DEVELOPMENT DOCUMENT    SECT  - VII
  ULTRAFILTRATION
                            MACROMOLECULES
 f - 10-SO fSl
MEMBRANE
                                  *
                                  WATER       SALTS
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          • DISSOLVED SALTS AMD LOW-MOLECULAR-WEIGHT ORGANICS
  FIGURE VII-29.  SIMPLIFIED ULTRAFILTRATION FLOW SCHEMATIC
                           282

-------
                GENERAL DEVELOPMENT  DOCUMENT
SECT  - VII
         FABRIC OR WIRE
         FILTER MEDIA
         STRETCHED OVER
         REVOLVING DRUM
  DIRECTION OF ROTATION
           ROLLER
SOLIDS SCRAPED
OFF FILTER MEDIA
                                                MEDIA
                                                MEANS
                                                VACUUM
    SOLIDS COLLECTION
    HOPPER
                                                                   INLET LIQUID
                                                                   TO BE
                                                                   FILTERED
                                -TROUGH
                                                      FILTERED LIQUID
                     FIGURE VII-30.  VACUUM FILTRATION
                                    283

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      GENERAL DEVELOPMENT DOCUMENT   SECT - VII
                          EVAPORATION
CONTACT COOLING
WATER
COOLING
 TOWER
SLOWDOWN
DISCHARGE
                                  MAKE-UP WATER
     RECYCLED  FLOW
                 Figure VII-31

  FLOW DIAGRAM FOR RECYCLING WITH A COOLING TOWER
                      284

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
                          SECTION VIII

            COST OF WASTEWATER .TREATMENT AND CONTROL
This section contains a summary of cost estimates,  a  discussion
of  the  cost methodology used to develop  these  estimates,  and
descriptions of the equipment and assumptions for each individual
treatment  technology.  These cost estimates, together  with  the
estimated pollutant reduction performance for each treatment  and
control  option presented in Sections IX, X, XI, and XII  of  the
subcategory  supplements,  provide a basis  for  evaluating  each
regulatory  option,  as well as- for identification  of  the  best
practicable technology currently available (BPT), best  available
technology  economically  achievable  (BAT),  best   demonstrated
technology (BDT), and the appropriate technology for pretreatment
standards.  The  cost  estimates  also  provide  the  basis   for
determining  the  probable economic impact of regulation  on  the
category  at different pollutant discharge levels.  In  addition,
this section addresses nonwater quality environmental impacts  of
wastewater  treatment  and control  alternatives,  including  air
pollution, solid wastes, and energy requirements.

SUMMARY OF COST ESTIMATES      ; ,,  '

The  total  capital  and  annual costs  of  compliance  with  the
promulgated  regulation  are presented by subcategory  in  Tables
VIII-1 through VIII-3 (pages 327-329) for regulatory options BPT,
BAT,  and PSES, respectively.  The number of direct and  indirect
discharging  plants  in  each  subcategory  is  also  shown.  The
methodology  used  to  obtain  these  plant  cost  estimates   is
described in the following sections.

COST ESTIMATION METHODOLOGY   {

Two  general  approaches to cost estimation  are  possible.   The
first  is a plant-by-plant approach in which costs are  estimated
for  each individual plant in the category.  Alternatively, in  .a
model  plant  approach,  costs can be  projected  for  an  entire
category  (or  subcategory)  based  on  cost  estimates  for   an
appropriately selected subset of plants.  The plant-by-plant cost
estimation  procedure is usually more accurate compared with  the
model  plant  approach  because it affords  a  higher  degree  of
flexibility  and maximizes the use of plant specific  data.   For
the nonferrous metals manufacturing category, the  plant-by-plant
approach was adopted.

For  the  primary aluminum, secondary  aluminum,  primary  copper
smelting,  primary  copper electrolytic refining,  primary  lead,
primary  zinc,  primary  columbium-tantalum,  primary   tungsten,
secondary   silver,   secondary  copper,  secondary   lead,   and
metallurgical  acid plants subca.tegories, the Agency revised  its
cost estimation methodology between proposal and promulgation  of
effluent limitations.
                               285

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
The  revisions are based on a more detailed engineering  analysis
of  each  plant so that estimated costs better  represent  actual
cost  to  each plant for compliance with  the  regulations.   The
revised  methodology also reflects the comments received  by  the
Agency  on  its  cost estimation approach.   The  pre- and  post-
proposal  cost estimation methodologies  are,  in  general,  very
similar.   The  major  revisions  in the methodology  are  listed
below.

     (1)  The revised approach made greater use of plant-specific
data  for treatment system design and equipment  information  for
costs.

     (2)  Treatment-in-place was considered.

     (3)   The method of determining the flow rate of  wastewater
into the treatment system was revised.

     (4)  Specific design and cost assumptions were revised.

     (5)  The method of calculating the pollutant loading in each
waste stream was revised.

     (6)   The  chemical precipitation system  configuration  was
simplified.

     (7)   Costs for contract hauling of nonhazardous wastes were
revised.

     (8)  Enclosure costs were revised.

To implement the revised approach, the wastewater characteristics
and  appropriate  treatment technologies for  the  category  were
identified.  These are discussed in Section V of each subcategory
supplement and Section VII of this document, respectively.  Based
on  a  preliminary technical and economic evaluation,  the  model
treatment systems were developed for each regulatory option  from
the  available  set of treatment processes.  When  these  systems
were  established,  a  cost data  base  is  developed  containing
capital and  operating costs for each applicable technology.   To
apply  this   data base to each plant for  cost  estimation,  the
following steps  were taken:

    1.    Define  the  components of the treatment  system  (e.g.,
chemical precipitation, multimedia filtration)  and their sequence
that are  applicable to the waste streams under consideration.

    2.    Define  the  flows and pollutant concentrations  of  the
waste streams entering the treatment system.

    3.    Estimate  capital  and annual costs for  this  treatment
system.

    4.    Estimate  the actual compliance costs  by accounting  for
existing treatment inplace.
                               286

-------
         GENERAL DEVELOPMENT DOCUMENT
                                 SECT - VIII
    5.  Repeat steps 1-4 for each regulatory option.
Because  of  the  large number of plants in the category  and  to
provide  a  greater  degree of accuracy,  the  above  steps  were
accomplished  by development of a computer-based cost  estimation
model  for  the  nonferrous  metals  manufacturing  category  and
related categories with similar treatment technology.  This model
represents the key element in the plant-by-plant cost  estimation
approach.
Each  of  the steps involved in the cost  estimation
outlined above is described in more detail below.

Cost Data Base Development
                                             methodology
A  step required prior to cost estimation is the      development
of  a cost data base, which includes the compilation     of  cost
data  and  standardization  of  the  data  to  a  common   dollar
basis.   Capital and annual cost data for the selected  treatment
processes  were  obtained  from  three  sources:   (1)  equipment
manufacturers and vendors, (2) literature data, and (3) cost data
from  existing plants.  The major source of equipment  costs  was
contacts  with  equipment vendors, while the majority  of  annual
cost  information  was  obtained  from  in-house  files  and  the
literature.   Additional cost and design data were obtained  from
data collection portfolios when possible.  The components of  the
cost  estimates,  the sources of cost     data,  and  the  update
factors  used  for standardization (to March  1982  dollars)  are
described below.

Components of Costs

The   components  of  the  capital  and  annual  costs  and   the
terminology  used  in this study are presented here in  order  to
ensure unambiguous interpretation of the cost estimates; and  cost
curves included in this section.
Capital  	
components:
or system capital costs.
Costs.   The  total capital costs consist of  two  major
     direct, or total module capital costs and indirect,
                 The direct capital costs include:
    (1)  Purchased equipment cost.

    (2)  Delivery charges (based on a shipping distance of 500
         miles), and

    (3)  Installation (including labor, excavation, site work,
         and materials).

The  direct  components  of the total capital  cost  are  derived
separately for each unit process,  or treatment technology.  Each
unit  process  cost comprises individual  equipment costs  (e.g.,
pumps,  tanks,  feed systems,  etc.).  The  correlating equations
                               287

-------
         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
used to generate the individual equipment
Table VIII-4 (page 330).
 costs are presented in
Indirect  capital costs consist of contingency, engineering   and
contractor fees.  These indirect costs are derived from  factored
estimates (i.e., they are estimated as percentages of a  subtotal
of the total capital cost, as shown i'n Table VIII-5 (page 341)).

Annual  Costs.   The  total  annualized costs also consist  of  a
direct  and  a system component as in the case of  total  capital
costs.   The components of the total annualized costs are  listed
in  Table  VIII-6 (page 340).   Direct annual costs  include  the
following:

     Raw  materials  - These  costs are for chemicals  and  other
     materials used in the treatment processes, which may include
     lime,  caustic,  sodium sulfide,  activated carbon, sulfuric
     acid, ferrous sulfate, and polyelectrolyte.

     Operating labor and materials - These costs account for  the
     labor  and  materials directly associated with operation  of
     the process equipment.   Labor requirements are estimated in
     terms of hours per year.   A labor rate of $21 per hour  was
     used  to convert the hour requirements into an annual  cost.
     This  composite labor rate included a base labor rate of  $9
     per  hour  for skilled labor,  15 percent of the base  labor
     rate  for supervision and plant overhead at 100  percent  of
     the total labor rate.  The base labor rate was obtained from
     the "Monthly Labor Review," which is published by the Bureau
     of  Labor Statistics of the U.S.  Department of Labor.   For
     the metals industry, this wage rate was approximately $9 per
     hour in March of 1982.

     Maintenance  labor and materials - These costs  account  for
     the  labor  and  materials required for repair  and  routine
     maintenance of the equipment.  They are based on information
     gathered  from  the  open  literature  and  from   equipment
     vendors.

     Energy  - Energy,  or power,  costs are calculated based  on
     total energy requirements (in kw-hrs). an electricity charge
     of  $0.0483/kilowatt-hour  and an operating schedule  of  24
     hours/day,  250 days/year unless  otherwise specified.   The
     electricity charge rate (March 1982) is based on the average
     retail electricity prices charged for industrial service  by
     selected Class A privately-owned  utilities,  as reported in
     the Department of Energy's Monthly Energy Review.

System   annual   costs   include   monitoring,   insurance   and
amortization.   Monitoring  refers to the  periodic  analysis  of
wastewater  effluent samples to ensure that discharge limitations
are  being  met.  The annual cost of  monitoring  was  calculated
using an  analytical lab fee of $120 per wastewater sample and  a
sampling   frequency based on the wastewater discharge  rate,  as
shown  in   Table VIII-7 (page 343).  The values shown  in  Table
                               288

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
VIII-7 represent typical requirements contained in NPDES permits.
For  the  economic  impact analysis, the  Agency  also  estimated
monitoring  costs  based  on  10  samples  per  month,  which  is
consistent  with the statistical basis for the  monthly  effluent
limitations.
The  cost of taxes and insurance is assumed to be one percent
the total depreciable capital investment.
                     of
Amortization  costs,  which account for depreciation and the cost
of  financing,  were calculated using a capital  recovery  factor
(CRF).   A  CRF  value of 0.177 was used,  which is based  on  an
interest rate of 12 percent,  and a taxable lifetime of 10 years.
The  CRF  is  multiplied by the total depreciable  investment  to
obtain the annual amortization costs.

Standardization of Cost Data

All  capital and annual cost data completed were standardized  by
adjusting  to  March  1982 dollars based on  the  following  cost
indices.

Capital  Investment.   Investment costs were adjusted  using  the
EPA-Sewage Treatment Plant Construction Cost Index.  The value of
this index for March 1982 is 414.0.

Chemicals.   The  Chemical  Engineering Producer Price Index  for
industrial chemicals was used.   This index is published biweekly
in Chemical Engineering magazine.   The March 1982 value of  this
index is 362.6.

Energy.   Power  costs  were  adjusted  by  using  the  price  of
electricity  on the desired date and multiplying it by the energy
requirements for the treatment module in kw-hr equivalents.   The
industrial charge rate for electricity for March 1982 is  $0.0483
per kw-hr as mentioned previously in the annual costs discussion.

Labor.   Annual  labor  costs were adjusted  by  multiplying  the
hourly  labor rate by the labor requirements (in  man-hours),  if
the latter is known.   The labor rate for March 1982 was computed
to be 21 dollars per hour as discussed above.  In cases where the
man-hour   requirements are unknown, the annual labor  costs  are
updated using cost indices.  The ENR Skilled Labor Index was used
for the primary aluminum, primary copper smelting, primary copper
electrolytic  refining,  primary  lead,  primary  zinc,   primary
columbium-tantalum,   primary   tungsten,   secondary   aluminum,
secondary   silver,   secondary  copper,  secondary   lead,   and
metallurgical acid plants subcategories.  The value of this index
for March 1982 is 3,256.23.  For all other subcategories in  this
rulemaking  the  EPA-Sewage  Treatment  Plant  Construction  Cost
Index was used.  The value of this index for March 1982, is 414.0
as stated above.

Plant Specific Flowsheet
                               289

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
When the cost data base has been developed, the first step of the
cost  estimation  procedure is the selection of  the  appropriate
treatment technologies and their sequence for a particular plant.
These  are determined for a given option by applying the  general
treatment  diagram  for that subcategory to the plant,  which  is
then   modified   as  appropriate  to   reflect   the   treatment
technologies that the plant will require. For instance, one plant
in a subcategory may generate wastewater from a certain operation
that  requires  oil-water separation. Another plant in  the  same
subcategory may not generate this waste stream and thus does  not
require  oil-water  separation  technology.  The  specific  plant
flowsheets will reflect this difference.

Wastewater Characteristics

Upon establishing the flowsheet required for a given  plant,  the
next  step is to define the influent waste stream characteristics
(flow and pollutant concentrations).

The  list of pollutants which may influence the design (and  thus
the cost) of the treatment system is shown in Table VIII-8.  This
list includes the conventional pollutants, and priority metal and
selected  nonconventional pollutants that are generally found  in
metal-bearing  waste  streams.   Inclusion of   these  pollutants
allows  the model to account for the effects of varying  influent
concentrations upon the various wastewater  treatment  processes.
For  example,  influent waste streams with  high metals  loadings
require  a  greater  volume  of precipitant (such  as  lime)  and
generate a greater amount of sludge than  wastestreams with lower
metals concentrations.

The  raw  waste  concentrations  of  pollutants  present  in  the
influent  waste streams for cost estimation were based  primarily
on field sampling data.  A production normalized raw waste  value
in  milligrams  of  pollutant per metric ton  of  production  was
calculated  for  each  pollutant  by  multiplying  the   measured
concentration by the corresponding waste stream flow and dividing
this  result  by  the corresponding^  production  associated  with
generation  of  the  waste stream.  These raw  waste  values  are
averaged  across  all sampled plants where the  waste  stream  is
found.   These  final  raw  waste values are  used  in  the  cost
estimation procedure to establish influent pollutant loadings  to
each plant's treatment system.  The underlying assumption in this
approach is that the amount of pollutant that is discharged by  a
process  is  a  function only of the amount of  product  that  is
generated  by  the process (or in some cases, the amount  of  raw
material  used in the process).  The amount of water used in  the
processes  is  assumed  to not have an affect  on  the  pollutant
quantity discharged. This assumption is also called the  constant
mass  assumption since the mass of pollutant  discharged  remains
the  same  even if the flow of water carrying  the  pollutant  is
changed.

The individual flows for cost estimation are determined for each
waste  stream.   The procedure used to derive these flows  is  as
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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
follows:

    (1)  The production normalized flows (1/kkg)  were  determined
for  each waste stream based on production (kkg/yr) and   current
flow (1/yr) data obtained from each plant's dcp   or trip  report
data where possible.

    (2)  This flow was compared to the regulatory flow  allowance
(1/kkg) established by the Agency for each waste   stream.

    (3)   The  lower  of the two flows was selected as  the  cost
estimation flow.  The flow in 1/yr is calculated by   multiplying
the selected flow by the production   associated with that  waste
stream.

    (4)   The  regulatory flow was assigned to waste streams  for
which actual flow rate data were unavailable for a   plant.

Treatment System Cost Estimation

Once  the treatment system and waste stream characteristics  have
been  defined,  they can be used as input to the cost  estimation
step,  which  is based on the cost estimation model  and  general
cost assumptions described below.

Cost Estimation Model

The  computer-based cost estimation model was designed to provide
conceptual  wastewater treatment design and cost estimates  based
on wastewater flows, pollutant loadings, and unit operations that
are  specified  by  the user. The model  was  developed  using  a
modular  approach;  that  is,  individual  wastewater   treatment
processes   such   as   gravity   settling   are   contained   in
semiindependent  entities  known as modules.  These  modules  are
used  as building  blocks in the determination of  the  treatment
system  flow  diagram. Because this approach  allows  substantial
flexibility  in treatment system cost estimation, the  model  did
not require modification  for each regulatory option.

Each module was developed by coupling design information from the
technical  literature  with  actual design  data  from  operating
plants.   This  results  in a more realistic  design  than  using
either theoretical or actual data alone, and correspondingly more
accurate   cost  estimates.   The  fundamental  units  for   cost
estimation  are  not the modules themselves  but  the  components
within each module.  These components range in configuration from
a  single  piece of equipment such as a pump to  components  with
several  individual  pieces, such as a lime  feed  system.   Each
component  is sized based on one or more fundamental  parameters.
For    instance, the lime feed system is sized by calculating  the
lime   dosage required to adjust the pH of the influent to 9  and
precipitate  dissolved  pollutants.  Thus, a larger  feed  system
would  be  designed for a chemical  precipitation  unit  treating
effluent containing high concentrations to dissolved metals  "than
for one treating effluent of the same flow rate but lower  metals
                               291

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          GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
 loadings.    This   flexibility  in  design  results   in   a   treatment
 system tailored to each  plant's wastewater  characteristics.

 The   cost   estimation  model   consists to   four   main parts,   or
 categories  of programs:

      User input programs,
      Design and simulation programs,
      Cost estimation programs, and
      Auxiliary programs.

 A  general   logic   diagram depicting  the   overall  calculational
 sequence is shown  in Figure VIII-1  (page 350).

 The   user input programs allow entry of all data  required by  the
 model,_  including  the  plant-specific  flowsheet,   flow   and
 composition data   for each waste stream,   and  specification   of
 recycle  loops.  The  design portion of the model calculates  the
 design  parameter  for each module of the flowsheet based  on  the
 user    input and material balances performed around each  module.
 Figure  VIII-2 (page 351) depicts the logic flow  diagram for  the
 design portion of  the model.

 The   design parameters are used as input to the   cost  estimation
 programs  to  calculate  the  costs  for  each  module  equipment
 component   (individual correlating cost equations were  developed
 for   each   of  these components). The total direct   capital  and
 annual  costs  are equal to the sum of the module   capital  and
 annual  costs,  respectively. System, or  indirect  costs  (e.g.,
 engineering, amortization) are then calculated (see Tables  VIII-
 5, and  VIII-6 (pages 341 and 342)) and added to  the  total direct
 costs  to obtain the total system costs. The logic flow  for  the
 cost  estimation   programs is displayed in  Figure  VIII-3  (page
 352).   The auxiliary programs store and transfer the final  cost
 estimates   to data  files, which are then used to  generate  final
 summary tables (see Table VIII-10, page 347, for a sample summary
 table).
General Cost Assumptions

The  following general assumptions apply to cost
in all subcategories:
       estimation
    (1)   Unless otherwise specified,  all
sludges are considered to be nonhazardous.
 wastewater   treatment
    (2)   In  cases  in  which  a  single  plant  has  wastewater
generating processes associated with different nonferrous  metals
manufacturing  subcategories,  costs are estimated for  a  single
treatment  system.  In most cases, the combined treatment  system
costs  are  then apportioned between  subcategories  on  a.  flow-
weighted basis since hydraulic flow is the primary determinant of
equipment  size  and  cost.  It is  possible,  however,  for  the
combined  treatment system to include a treatment module that  is
required  by  only one of the associated subcategories.  In  this
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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
case, the total costs for that particular module are included  in
the costs for the subcategory   which requires the module.  Where
the  module in   question involves flow reduction, the costs  are
apportioned based on an influent flow weighted basis.   Such cost
apportioning  is  essentially  only  a  bookkeeping  exercise  to
allocate costs  because the total costs calculated for the  plant
remain the same.

    (3)   In  most cases,  where a plant has  wastewater  sources
from  the nonferrous metals manufacturing category and a category
other  than  nonferrous manufacturing  (for  example,  nonferrous
forming)  costs are calculated for segregating   these  different
wastewaters.   This  means of cost estimation accounts   for  the
possibility  that respective regulations for   each category  are
based  on  different technologies (and    may  control  different
pollutants).

Consideration of Existing Treatment

The cost estimates calculated by the model represent  "greenfield
costs"  that do not account for equipment that plants may already
have  in  place,  i.e.. these costs  include  existing  treatment
equipment.  In  order  to estimate  the  actual  compliance  cost
incurred  by  a plant to meet the effluent  guidelines,  "credit"
should be given to account for treatment in place at that  plant.
This  was accomplished by subtracting capital costs of  treatment
in-place (as estimated by the model) from the "greenfield  costs"
to  obtain  the actual or required capital costs  of  compliance.
Annual costs associated with treatment in place (as estimated  by
the model), however, are not subtracted because these costs recur
and must be borne by the facility each year.  Further,  inclusion
of  these annual costs ensures that EPA adequately considers  the
costs  for  proper  operation of each  module  in  the  treatment
system.  For an example the reader is referred to Table  VIII-10,
(page  347 which presents compliance cost estimates for  a  plant
that has chemical precipitation of sufficient capacity already in
place.

Existing treatment is considered as such only if the capacity and
performance  of  the  existing equipment (measured  in  terms  of
estimated   ability   to  meet  the  effluent   limitations)   is
equivalent  to that of the technologies considered by the Agency.
The  primary source of information regarding  existing  treatment
was data collection portfolios (dcps).

General  assumptions  applying  to  all  subcategories  used  for
determining   treatment  in  place  qualifications  in   specific
instances include:

     (1)   In  cases  in which  existing  equipment  has  adequate
performance but insufficient capacity, the plant is   assumed  to
comply  by  either installing additional   required  capacity  to
supplement the existing equipment   or disregarding the  existing
equipment  and  installing   new equipment to  treat  the  entire
flow.  This selection   was based on the lowest total  annualized
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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
cost.

     (2)   When  a  plant  reported  recycle  of  treatment  plant
sludges,  capital and annual costs for sludge handling    (vacuum
filtration  and  contract  hauling) are  not    included  in  the
compliance costs.  It is assumed that   it is economical for  the
plant  to  practice recycle in   this case,  and  therefore,  the
related costs are considered to be process associated, or a  cost
of doing   business.

     (3)   Capital  costs for flow reduction (via recycling)  were
not   included  in  the  compliance  costs  whenever  the   plant
reported recycle to the stream, even it the specific   method  of
recycle was not reported.

     (g)   Settling  lagoons  were assumed  to  be  equivalent  to
vacuum  filtration  for  dewatering  treatment  plant    sludges.
Thus,   whenever  a  plant  reported  settling    lagoons  to  be
currently in use for treatment plant   sludges, the capital costs
of  vacuum  filtration were   not included.  It was assumed  that
annual  vacuum    filtration costs were comparable to  those  for
operation   of settling lagoons and were thus retained.

COST ESTIMATES FOR INDIVIDUAL TREATMENT TECHNOLOGIES

Treatment  technologies have been selected from among the  larger
set  of  available  alternatives discussed in Section  VII  after
considering  such factors as raw waste  characteristics,  typical
plant  characteristics  (e.g.,  location,  production  schedules,
product  mix,  and  land  availability),  and  present  treatment
practices.   Specific  rationale  for selection is  addressed  in
Sections IX,  X, XI, and XII of this document and the subcategory
supplements.   Cost  estimates for each technology  addressed  in
this  section  include  investment  costs and  annual  costs  for
amortization, operation and maintenance, and energy.

The  specific -design and cost assumptions  for  each  wastewater
treatment  module  are  listed^.under the subheadings  to  follow.
Costs  are  presented as a function of influent  wastewater  flow
except where noted in the unit process assumptions.
Costs are presented for the following control and
technologies:

   Cooling towers,
   Flow equalization,
   Cyanide precipitation and gravity settling,
   Ammonia steam stripping.
   Oil-water separation,
   Chemical precipitation and gravity settling,
   Sulfide precipitation and gravity settling,
   Vacuum filtration,
   Holding tanks,
   Multimedia filtration,
   Activated carbon adsorption,
         treatment
                               294

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         GENERAL DEVELOPMENT DOCUMENT
            SECT  - VIII
   Chemical oxidation, and
   Contract hauling.

In  addition,  costs  for  the following  items  associated  with
compliance costs are also discussed:

   Enclosures
   Segregation

Cooling Towers

Cooling  towers are used to reduce discharge flows  by  recycling
cooling  water waste streams.   Holding tanks are used to recycle
flows  less  than  3,400 liters per hour  (15  gpm).   This  flow
represents the effective minimum cooling tower capacity generally
available.

The  cooling  tower  capacity  is based on  the  amount  of  heat
removed,  which takes into account both the design flow  and  the
temperature  decrease  needed  across  the  cooling  tower.   The
influent flow to the cooling tower and the recycle rate are based
on the assumptions given in Table VIII-9 (page 346). It should be
noted  that for BAT a cooling tower is not included for cases  in
which  the actual flow is less than the reduced  regulatory  flow
(BAT  flow)  since flow reduction is not required.   The  recycle
ratios  for  waste streams undergoing flow  reduction  (based  on
cooling  tower  technology)  are discussed in Section  X  of  the
pertinent subcategory supplement.

The temperature decrease is calculated as the difference  between
the hot water (inlet) and cold water (outlet) temperatures.   The
cold  water  temperature  was assumed to be 29°C  (85°F)  and  an
average  value calculated from sampling data is used as  the  hot
water temperature for a particular waste stream.  When such  data
were   unavailable, or resulted in a temperature less  than  35°C
(95°F),  a  value  of 35°C (95°F) was  assumed,  resulting  in, a
cooling requirement for a 6°C (10°F) temperature drop.  The other
two  design  parameters, namely the wet bulb  temperature  (i.e.,
ambient   temperature at 100 percent relative humidity)  and  the
approach (thf difference between the outlet water temperature and
the  wet  bulb  temperature),  were assumed  to  be  constant  at
25°C (77°F) and 4°C (8°F), respectively.

For flow rates above 3,400 1/hr, a cooling tower is designed. The
cooling  tower is sized by calculating the required  capacity  in
evaporative tons.   Cost data were gathered for cooling towers up
to 700 evaporative tons.

The  capital costs of cooling tower systems include the following
equipment:          •                                   f
  Cooling  tower (crossflow,
  accessories
mechanically-induced) and   typical
  Piping and valves (305 meters (1,000 ft.),  carbon
                               295

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
  steel)

  Cold water storage tank (1-hour retention time)

  Recirculation pump, centrifugal

  Chemical treatment system (for pH, slime and corrosion
  control)
For  heat  removal requirements exceeding 700
multiple cooling towers are designed.
     evaporative  tons,
The  direct  capital  costs  include  purchased  equipment  cost,
delivery,  and  installation.   Installation  costs  for  cooling
towers  are assumed to be 200 percent to the cooling  tower  cost
based on information supplied by vendors.

Direct annual costs include raw chemicals for water treatment and
fan  energy  requirements.   Maintenance and operating labor  was
assumed to be constant at 60 hours per year.  The water treatment
chemical  cost is based on a rate to $220/1,000 Iph  ($5/gpm)  of
recirculated water.

For  small recirculating flows (less than 15 gpm),  holding tanks
were  used for recycling cooling water.   A holding  tank  system
consists  of  a steel tank,  61 meters (200 feet) piping,  and  a
recirculation pump.  The capacity of the holding tank is based on
the cooling  requirements of the water to be cooled.  Calculation
of  the  tank volume is based on a surface  area  requirement  of
0.025  m2/lph  (60  ft2/gpm) to recirculated  flow  and  constant
relative tank dimensions.

Capital  costs  for  the holding tank  system  include  purchased
equipment cost, delivery, and installation.  The annual costs are
attributable  to  the operation of the pump  only   (i.e.,  annual
costs for tank and piping are assumed to be negligible).

Capital  and  annual  costs  for cooling  towers  and  tanks  are
presented in Figure VIII-4 (page 353).

Flow Equalization

Flow  equalization  is  accomplished through  steel  equalization
tanks which are sized based on a retention time of  8 or 16  hours
and  an  excess capacity factor of 1.2. .  A retention time of  16
hours  was  assumed only when the equalization  tank  preceded  a
chemical  precipitation  system  with "low flow"  mode,  and  the
operating  hours were greater than or equal to 16 hours per  day.
In this case,  the additional retention time is required to  hold
wastewater during batch treatment,  since treatment is assumed to
require  16  hours and only one reaction tank is included in  the
"low  flow"  batch  mode.   Cost data were  available  for  steel
equalization  tank up to a capacity of 1,893,000 liters  (500,000
gallons);  multiple units were required for volumes greater  than
1,893,000  liters (500,000 gallons).   Fiberglass tanks are  used
                               296

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         GENERAL DEVELOPMENT DOCUMENT
                                          SECT - VIII
for capacities below 24,000 gallons.    The tanks are fitted with
agitators  with a horsepower requirement of 0.006 kw/1,000 liters
(0.03 hp/1,000 gallons) of capacity to prevent sedimentation.  An
effluent  transfer  pump  is also included  in  the  equalization
system.   Cost curves for capital and annual costs are  presented
in Figure VIII-5 (page 354),  for equalization at 8 hours and  16
hours  retention  time.   Figure VIII-5 presents cost curves  for
capital  and  annual costs that are applicable to  the  following
list  of subcategories:   primary aluminum,  secondary  aluminum,
primary copper,  secondary copper,  primary lead,  primary  zinc,
primary tungsten,  primary columbium-tantalum,  secondary silver,
and secondary lead.

Cyanide Precipitation and Gravity Settling

Cyanide precipitation is a two-stage process to remove  complexed
and uncomplexed cyanide as a precipitate.  In the first step, the
wastewater  is  contacted  with  an excess of  FeSO4.7H20  at  pH
9.0  to  ensure that all cyanide is converted  to  the  complexed
form:
    FeSO4
7H20 + 6CN ----- > Fe(CN)6
                                      3~
7H20 + S04
                                                     2~
                                                          e-
The  hexacyanoferrate is then routed to the second  stage,  where
additional FeSO4'7H2O and acid are added.   In this stage, the pH
is  lowered  to  4.0   or  less,  causing  the  precipitation  of
Fe3(Fe(CN)g)2 (Turnbull's blue) and its analogues:

3FeSO4*7H20 + 2Fe(CN)63~ ---- > Fes (Fe(CN) 6 ) 2 + 21H20 + 3S042~
A  chemical  defoamer  may  be added prior to  pH  adjustment  to
inhibit foaming,  as carbon dioxide degassing may occur when  the
pH is lowered.
The  blue  precipitate is settled and the overflow is
for further treatment.
                                                       discharged
Since the complexation step adjusts the pH to 9, metal hydroxides
will  precipitate.   These hydroxides may either be  settled  and
removed  at  pH  9  or  resolubilized  at  pH  4  in  the   final
precipitation  step  and removed later in a  downstream  chemical
precipitation   unit.   Advantages  of  removal  of   the   metal
hydroxides  include  reduced  acid  requirements  in  the   final
precipitation  step, since the metals will resolubilize when  the
pH  is  adjusted  to  4. However, the  hydroxide  sludge  may  be
classified  as  hazardous  due to the presence  of  cyanide.   In
addition, the continuous mode of operation requires an additional
clarifier between the complexation and precipitation step.  These
additional   costs   make  the  settling  of   metal   hydroxides
economically  unattractive in the continuous mode.  However,  the
batch  mode  requires no extra  equipment.   Consequently,  metal
hydroxide  sludge  removal in this case is desirable  before  the
precipitation  step.  Therefore, the batch cyanide  precipitation
step  settles two sludges:  metal hydroxide sludge (at pH 9)  and
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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
cyanide sludge (at pH 4).

Costs  were estimated for both batch and continuous systems  with
the operating mode selected on a least cost basis.  The equipment
and assumptions used in each mode are detailed below.

Costs  for the complexation step in the continuous mode are based
on the following:

     (1)   Ferrous  sulfate  feed system

           ferrous  sulfate  steel
           storage hoppers with dust collectors (largest hopper
           size is  170 mg  (6,000  ft3);  15 days storage)
           enclosure for  storage  tanks
           volumetric  feeders  (small installations)
           mechanical weigh  belt feeders (large installations)
           dissolving tanks   (5-minute detention time,
           6 percent solution)
           dual-head diaphragm metering pumps
           instrumentation and,controls

     (2)  Lime feed system

          hydrated lime
          feeder                                ,
          slurry mix tank (5-minute retention time)
          feed pump
          instrumentation (pH control)

     (3)  H2S04 feed system (used when influent pH is >9)

          93 percent 1*2804 delivered in bulk or in drums
          acid storage tank (15 days retention) when
          delivered in bulk
          metering pump (standby provided)
          pipe and -valves                                   •    ,
          instrumentation and controls

     (4) Reaction  tank  and  agitator  (fiberglass,  60-minute
         retention  time,  20 percent excess capacity,  agitator
         mount, concrete slab)

     (5)  Effluent transfer pump
For  the primary aluminum subcategory,  the lime feed system  was
replaced  with a caustic feed system.   This system consisted  of
day  tanks  (2) with mixers and feeders for feed rates less  than
200 Ibs/day, a fiberglass tank with a 15-day storage capacity for
feed  rates greater than 200 Ibs/day,  chemical  metering  pumps,
pipes and values, and instruments and controls.
Costs for the second step (precipitation) in the continuous
are based on the following equipment:
                   mode
                               298

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
      (1)  FeSC>4  feed  system - as  above

      (2)  H2SO4  feed  system - as  above

      (3)   Polymer  feed  system

           chemical mix tank with agitator
           chemical metering pump
           system storage hopper

      (4)   Reaction   tank with  agitator   (fiberglass,   30-minute
           retention  time,  20 percent  excess  capacity,   agitator
           mount, concrete slab)

      (5)   Clarifier

           sized based on 709 lph/m2  (17.4 gph/ft2),   3
             percent  solids  in  underflow
           steel  or  concrete,   above  ground
           support  structure, sludge scraper, and other  internals
           center feed

      (6)  Effluent transfer pump

      (7)  Sludge transfer pump


A  chemical  defoaming system may be included.   Defearning  costs
consist of the antifoam chemical  and the chemical feed system.

Operation  and maintenance costs  for continuous mode cyanide pre-
cipitation include labor  requirements to operate and maintain the
system, electric power for mixers, pumps, clarifier and controls,
and  treatment  chemicals.    Electrical  requirements  are  also
included  for  the chemical storage enclosures for  lighting  and
ventilation  and in the case of caustic  storage,  heating.   The
following assumptions are used in establishing OEM costs  for  the
complexation step in the  continuous mode:

     (1)   Ferrous  sulfate feed  system

           stoichiometry of  1  mole
             FeS(p4  7H20  to  6 moles CN-
           1.5 times stoichiometric  dosage  to
             drive   reaction   to   completion
           operating   labor   at    10 min/feeder/shift
          - maintenance  labor  at  8 hr/yr  for  liquid   metering
•   '   ;••'•••   • pumps ~ .•:•..•:-. I '-..
 "-'•    •    "power  based  on  a'gitators,  metering  pumps
• '-•". '• -'i-  V  maintenance materials  at 3 percent of capital cost
           chemical cost at  $0.1268 per kg ($0.0575 per  Ib)

     (2)   Lime feed system
                               299

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
             dosage based on pH and metals content to raise pH
               to 9
             operating and maintenance labor requirements are
               based on 20 min/day; in addition, 8 hr/7,260 kg
               (8 hr/16,000 Ibs) are assumed for delivery of
               hydrated lime
             maintenance materials cost is estimated as 3
               percent of the purchased equipment cost
             chemical cost of lime is based on $0.0474/kg
               ($0.0215 per Ib) for hydrated lime delivered in
               bags

     (3)   Acid feed system (if required)

             dosage based on pH and metals to bring pH to 9
             labor unloading - 0.25 hr/drum acid
             labor operation - 15 min/day
             annual maintenance - 8 hrs
             power (includes metering pump)
             maintenance materials - 3 percent of capital
               cost
             chemical cost at $0.082 per kg ($0.037 per Ib)

     (4)   Reaction tank with agitator

             operating and maintenance labor at 120 hrs/yr
             maintenance materials
             — tank:  2 percent of tank capital cost
             — pump:  5 percent of pump capital cost
             For the primary aluminum subcategory
               maintenance materials costs were estimated
               at 5 percent of capital cost.
             power based on agitator (70 percent efficiency)
               at 0.099 kW/1,000 liters (0.5 hp/1,000 gallons)
               of tank volume

     (5)   Pump

             operating labor at 0.04 hr/operating day
             maintenance labor at 0.005 hr/operating hour for
               flow <22,700 liters per hour (100 gpm)
             maintenance materials at 5 percent of capital
               cost
             power based on pump hp

For  the primary aluminum subcategory,  the lime feed system  was
replaced  by  a caustic feed system.   The costs for the  caustic
feed system are as follows:

           Caustic feed system

             dosage based on pH and metals content to raise pH
               to 9
             maintenance materials - 3 percent of manufactured
               equipment cost (excluding storage tank cost)
                               300

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         GENERAL DEVELOPMENT DOCUMENT
                               SECT - VIII
             labor unloading
             —dry NaOH - 8 hrs/16,000 Ibs
             —liquid 50 percent NaOH - 5 hrs/50,000 Ibs
             labor operation (dry NaOH only) 10 min/day/feeder
             labor operation for metering pump - 15 min/day
             annual maintenance - 8 hrs
             power [includes metering pump hp, instrumentation
               and control, volumetric feeder (dry NaOH)]
             chemical cost at $0.183 per Ib

The  following  assumptions  were used for  the  continuous  mode
precipitation step:

     (1)   Ferrous sulfate feed system

               stoichiometric dosage based on 3 moles
                  FeS04*7H20 to 2 moles of iron-complexed
                  cyanide (Fe (CN)63~)
               total dosage is 10 times stoichiometric dosage
                  based on data from an Agency treatability study
               other assumptions as above

     (2)   H2SO4 feed system

               dosage based on pH adjustment to 4 and
                  resolubilization of the metal hydroxides
                  from the complexation step
               other assumptions as above

     (3)   Polymer feed system

               2 mg/1 dosage
               operation labor at 134 hr/yr, maintenance labor at
                  32 hr/yr
               maintenance materials at 3 percent of the capital
                  cost
               energy at 17,300 kWh/yr
               chemical cost at $4.96/kg ($2.25/lb)

     (4)   Reaction tank with agitator
     (5)
               see assumptions above
Clarifier
               sized based on 417 gpd/ft2, 3 percent solids
                  in underflow
               maintenance materials range from 0.8 percent to
                  2 percent as a function of increasing size
               labor - 150 to 500 hr/yr (depending on size)
               power - based on horsepower requirements for
                  sludge pumping and sludge scraper drive unit
     (•'6)   Effluent transfer pump
                               301

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
             see assumptions above

     (7)  Sludge pump

            sized on underflow from clarifier
            operation and maintenance labor varies with flow
              rate
            maintenance materials - varies from 7 percent to
              10 percent of capital cost depending on flow rate

The  batch  mode  cyanide precipitation  step  accomplishes  both
complexation  and precipitation in the same  vessel.   Costs  for
batch  mode  cyanide complexation and precipitation are based  on
the following equipment:

     (1)   Ferrous sulfate addition

             from bags
             added manually to reaction tank

     (2)   Lime addition'

             from bags
             added manually to reaction tank

     (3)  H2SO4 addition

            from 208 liter (55 gallon) drums
            stainless steel valve to control flow

     (4)  Reaction tank and agitator (fiberglass, 8.5 hour
          minimum retention time/ 20 percent excess capacity,
          agitator mount, concrete slab)

     (5)  Pump

            effluent transfer pump
            sludge pump

Operation   and   maintenance  costs  for  batch   mode   cyanide
complexation  and  precipitation  include  costs  for  the  labor
required to operate and maintain the equipment, electrical  power
for   agitators,  pumps,  and  controls,  and   chemicals.    The
assumptions used in estimating costs are as follows:
     (1)  Ferrous sulfate addition

          stoichiometric dosage
          —complexation:  1 mole FeS04'7H20 per 6 moles
            CN-
          —precipitation:  3 moles FeS04 7H20 per 2
            moles of the iron cyanide complex
            actual   dosage   in   excess   of   stoichiometric
              complexation: 1.5 times stoichiometric dosage added
     (Fe(CN63 )
                               302

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
              precipitation: 10 times stoichiometric dosage added
            operating  labor  at  0.25  hr/batch
            chemical cost at $0.1268/kg ($0.0575/lb)
            no maintenance labor or materials or power costs

      (2)  Lime addition

          dosage based on pH and metals content to raise pH
             to 9           •
          operating labor at 0.25 hr/batch
          chemical cost at $0.0474/kg ($0.0215/lb)
          no maintenance labor or materials or power costs

      (3)  H2S04 addition

          dosage based on pH and metals content to lower pH
            to 9 (for complexation if required) and/or to lower
          pH to 4 (for precipitation)
          operating labor at 0.25 hr/batch
          chemical cost at $0.082/kg ($0.037/lb)
          no maintenance labor or materials or power costs

      (4)  Reaction tank with agitator

          maintenance materials
          —tank:  2 percent of tank capital cost  ,
          —pump:  5 percent of pump capital cost
          power based on agitator (70 percent efficiency) at
            0.099 kW/1,000 liters (0.5 hp/1,000 gallons) of tank
            volume

      (5)  Pumps

          effluent transfer pump
          —operating labor at 0.04 hr/operating day
          —maintenance labor at 0.005 hr/operating day (or
              flows < 22,700 1/hr (100 gpm)
          —maintenance materials at.5 percent of capital cost
          —power based on pump hp
          sludge pump
          —operation and maintenance costs vary with flow
              rate
          —maintenance materials costs vary from 7 to 10 per-
            cent of capital cost depending on flow rate

Capital  and  annual costs for continuous and batch mode  cyanide
precipitation are presented in Figure VIII-6 (page 355).   Figure
VIII-6 presents cost curves for capital and annual costs that are
applicable  to  the following  list  of  subcategories:   primary
aluminum,  secondary aluminum,  primary copper, secondary copper,
primary lead,  primary zinc, primary tungsten, primary columbium-
tantalum, secondary silver, and secondary lead.

Ammonia Steam Stripping
                               303

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
Ammonia removal using steam is a proven technology that is in use
in many industries.   Ammonia is more volatile than water and may
be   removed   using   steam  to  raise   the   temperature   and
preferentially  evaporate  the ammonia.   This  process  is  most
economically      done  in  a plate or packed  tower,  where  the
method of contacting     the liquid and vapor phases reduces  the
steam requirement.

The  pH of the influent wastewater is raised to approximately  12
to convert almost all of the ammonia present to molecular ammonia
(NH3)  by  the  addition of lime.   The water is  then  preheated
before it is sent to the   column.   This process takes place  by
indirectly  contacting the influent with the column effluent  and
with  the gaseous product via heat exchangers.   The water enters
the  top  of  the column and  travels  downward.   The  steam  is
injected  at the bottom and rises through the column,  contacting
the water in a countercurrent fashion.   The source of the  steam
may  be  either reboiled wastewater or another  steam  generation
system, such as the plant boiler system.

The  presence of solids in the wastewater, both those present  in
the influent and those which may be generated by adjusting the pH
(such as metal hydroxides), necessitates periodic cleaning of the
column.   This requires an acid cleaning system and a surge  tank
to hold wastewater while the column is being cleaned.  The column
is assumed to require cleaning approximately once per week  based
on the demonstrated long-term cleaning requirements of an ammonia
stripping  facility.   The volume of cleaning solution  used  per
cleaning operation is assumed to be equal to the total volume  of
the empty column (i.e., without packing).

For  the estimation of capital and annual  costs,  the  following
pieces  of  equipment  were included in the design of  the  steam
stripper:


    (1)  Packed tower

           3-inch Rashig rings
           hydraulic loading rate = 2 gpm/ft2
           height equivalent to a theoretical plate = 3ft

    (2)  pH adjustment system

           lime feed system (continuous) - see chemical
             precipitation section for discussion
           rapid mix tank, fiberglass (5-minute retention time)
           agitator (velocity gradient is 300 ft/sec/ft)
           control system
           pump

    (3)  Heat exchangers (stainless steel)

    (4)  Reboiler (gas-tired)
                               304

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         GENERAL DEVELOPMENT DOCUMENT
  SECT - VIII
     (5)  Acid cleaning system

           batch tank, fiberglass
           agitator  (velocity gradient is 60/sec.)
           metering  pump

     (6)  Surge tank  (8-hour retention time)

The  direct capital cost to the lime feed system was based on  the
chemical  feed  rate as  noted in  the  discussion  on  chemical
precipitation.   Sulfuric acid used in the acid  cleaning  system
was  assumed to be added manually, requiring no special equipment.
Other  equipment costs were direct or indirect functions  of  the
influent  flow rate.  Direct annual costs include  operation  and
maintenance  labor for the lime feed system, heat exchangers  and
reboiler,  the  cost  of  lime  and  sulfuric  acid,  maintenance
materials, energy costs required to run the agitators and  pumps,
and  natural gas costs to operate the reboiler.  The total direct
capital  and  annual costs are presented in Figure  VIII-7  (page
356).

Oil-Water Separation

Oil  skimming costs apply to the removal of free  (non-emulsified)
oil  using either a coalescent plate oil-water separator or a belt
skimmer  located  on the  equalization  tank.    The  latter  is
applicable to low oily waste flows (less than 189 liters per day)
whereas  the  coalescent plate separator is used for  oily  flows
greater than 189 liters/day (50 gpd).

Although  the  required coalescent plate  separator  capacity  is
dependent on many factors, the sizing was based primarily on  the
influent  wastewater flow rate, with the following design  values
assumed for the remaining parameters of importance:
    Parameter

    Specific gravity of oil
    Operating temperature (°F)
    Influent oil concentration (mg/1)
    Effluent oil concentration (mg/1)
 Design Value

     0.85
68
30,000
    10.0
Extreme operating conditions, such as influent oil concentrations
greater  than  30,000  mg/1,  or  temperatures  much  lower  than
20°C  (68°F) were accounted for in the sizing of  the  separator.
Additional  capacity  for such extreme  conditions  was  provided
using   correlations   developed  from   actual   oil   separator
performance data.

The  capital and annual costs of oil-water separation include the
following equipment:

       Coalescent plate separator with automatic shutoff
         valve and level sensor
                               305

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
       Oily waste storage tanks (2-week retention time)
       Oily waste discharge pump
       Effluent discharge pump

Influent flow rates up to 159,100 1/hr (700 gpm) are treated in a
single unit. Flows greater than this require multiple units.

The direct annual costs for oil-water separation include the cost
of operating and maintenance labor and replacement parts.  Annual
costs  for the coalescent plate separators alone are minimal  and
involve only periodic cleaning and replacement of the plates.

If  the  amount of oil discharged is 189 liters/day (50  gpd)  or
less,  it is more economical to use a belt skimmer rather than  a
coalescent plate separator.  This belt skimmer may be attached to
the  equalization basin which is usually necessary to equilibrate
flow surges.   The belt skimmer-equalization basin  configuration
is assumed to achieve 10 mg/1 oil in the effluent.

The  equipment  included in the belt oil skimmer  and  associated
design parameters and assumptions are presented below.

    1.  Belt oil skimmer

        12-inch width
         6-foot length

    2.  Oily waste storage tank

        2-week storage
        fiberglass


Capital  costs  for belt skimmers were  obtained  from  published
vendor  quotes.   Annual costs were estimated from the energy arid
operation arid maintenance requirements.   Energy requirements are
calculated from the skimmer motor horsepower-.  Operating labor is
assumed  constant  at 26 hours per year.   Maintenance  labor  is
assumed  to require 24 labor hours per year and belt  replacement
once  a  year.   Cost  curves for capital  and  annual  costs  of
oil-water   separation  are  presented  in  Figure  VIII-8   (page
357).   Figure VIII-8 presents cost curves for capital and annual
costs that are applicable to the following list of subcategories:
primary aluminum,  secondary aluminum,  primary copper, secondary
copper,  primary lead,  primary zinc,  primary tungsten,  primary
columbium-tantalum, secondary silver, and secondary lead.

Chemical Precipitation and Gravity Settling

Chemical precipitation using lime or caustic followed by  gravity
settling  is  a fundamental technology for  metals  removal.   In
practice,  quicklime  (CaO),  hydrated lime (Ca(OH)2),  or caustic
(NaOH) can be used to precipitate toxic and other metals.   Where
lime is selected, hydrated lime is generally more economical  for
low  lime  requirements  since  the use  of  slakers,  which  are
                               306

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
necessary for quicklime usage, is practical only for large volume
applications  of  lime (greater than 50  Ibs/hr).   The  chemical
precipitant  used  for compliance cost estimation  depends  on  a
variety  of factors  in  the subcategory being  considered.   The
basis  for the chemical precipitant (lime or caustic) used for  a
particular   subcategory   may  be  found  in   the   appropriate
supplement.

Lime  or  caustic is used to adjust the pH of the influent  waste
stream  to a value of approximately 9,  at which optimum  overall
precipitation  of  the metals as metal hydroxides is  assumed  to
occur.   The  chemical  precipitant  dosage is  calculated  as  a
theoretical  stoichiometric requirement based on the pH  and  the
influent  metals concentrations.  In addition,  particular  waste
streams  may  contain significant amounts of  fluoride,  such  as
those  found in the secondary tin and primary  columbium-tantalum
subcategories.   The fluoride will  form calcium fluoride  (CaF2)
when combined with free calcium ions which are present if lime is
used  as the chemical precipitant.  The additional sludge due  to
calcium fluoride formation is  included in the sludge  generation
calculations.   In cases where  the calcium consumed  by  calcium
fluoride  formation  exceeds  the calcium  level  resulting  from
dosing  for  pH  adjustment and metal  hydroxide  formation,  the
additional  lime  needed  to consume the  remaining  fluoride  is
included in the total theoretical dosage calculation.  The  total
chemical dosage requirement is obtained by assuming an excess  of
10 percent of the theoretical dosage. The effluent concentrations
are  generally  based on the Agency's combined metals  data  base
treatment   effectiveness  values  for   chemical   precipitation
technology described in Section VII (see Table VII-21, page 248).

The  costs  of chemical precipitation and  gravity  settling  are
based on one of three operating modes,  depending on the influent
flow:   continuous, "normal" batch, or "low flow" batch.  The use
of  a particular mode for cost estimation purposes is  determined
on  a least cost (total annualized) basis.   The economic  break-
point  between  continuous and normal batch was estimated  to  be
10,600 1/hr (46.7 gpm).   Below.2,200 1/hr, it was found that the
low  flow batch was the most economical.   The direct capital and
annual  costs  are presented in Figure VIII-9 (page 358  for  all
three  operating modes.   Figure VIII-9 presents cost curves  for
capital  and  annual costs that are applicable to  the  following
list  of subcategories:   primary aluminum,  secondary  aluminum,
primary copper,  secondary copper,  primary lead,  primary  zinc,
primary tungsten,  primary columbium-tantalum,  secondary silver,
and secondary lead.

Continuous  Mode.    For  continuous  operation,   the  following
equipment is included in the determination of capital and  annual
costs:

    (1)  Chemical precipitant feed system (continuous)

         lime
         —bags (for hydrated lime) or storage units (30-day
                               307

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         GENERAL  DEVELOPMENT  DOCUMENT
SECT - VIII
               storage  capacity)  for  quicklime
          —slurry mix  tank  (5-minute retention  time) or
               slaker
          —feed pumps  (for  hydrated  lime  slurry) or gravity
               feed  (for quicklime  slurry)
          —instrumentation  (pH control)
          caustic
          —day tanks  (2) with mixers and  feeders for feed
               rates less than 200  Ibs/day;  fiberglass  tank with
               15-day storage capacity otherwise
          —chemical metering pumps
          —pipe and valves
          —instrumentation  (pH control)

     (2)   Polymer feed  system

          storage hopper
          chemical mix  tank  with  agitator
          chemical metering  pump

     (3)   Reaction system

          rapid mix tank, fiberglass  (5-minute retention time)
          agitator (velocity gradient is 300 ft/sec/ft)
          instrumentation and control

     (4)   Gravity settling system

          clarifier, circular, steel  (overflow rate of  360
          gpd/ft. and underflow solids of  5 percent) were
          used  for most subcategories.  However, for the
          following subcategories, an overflow rate of
          500 gpd/ft2 and an underflow solids of 3 percent
          was used:  primary aluminum, secondary aluminum,
          primary copper, secondary copper, primary lead,
          primary zinc, primary tungsten, primary
          columbium-tantalum, secondary silver, and secondary
          lead.

     (5)   Sludge pump

Ten  percent of the clarifier underflow stream is recycled to the
pH  adjustment  tank to serve as seed material for  the  incoming
waste stream.

The direct capital costs of the  chemical precipitant and  polymer
feed  are based on the respective feed rates (dry Ibs/hr),  which
are dependent  on the influent waste  stream characteristics.   The
flexibility of this feature (i.e., costs are independent of other
module components) was previously noted in the description of the
cost estimation model.   The remaining equipment costs (e.g., for
tanks,  agitators,  pumps)   were developed as a function  of  the
influent  flow (either directly or indirectly,  when coupled with
the design assumptions).
                               308

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
Direct  annual costs for the continuous system are based  on  the
following assumptions:

    (1)  Lime feed system

           Operating and maintenance labor requirements are
              based on 3 hrs/day for the quicklime feed system and
              20 min/day for the hydrated lime feed system.  In
              addition, 5 hrs/50,000 Ibs are required for bulk
              delivery of quicklime and 8 hrs/16,000 Ibs are
              assumed for delivery of hydrated lime.
           Maintenance materials cost is estimated as 3 percent
              of the purchased equipment cost.
           Chemical cost of lime is based on $47.40/kkg
              ($43.00/ton) for hydrated lime delivered in bags and
              $34.50/kkg ($31.30/ton) for quicklime delivered on a
              bulk basis.  These costs were obtained from the
              Chemical Weekly Reporter (March 1982).

    (2)  Caustic feed system

           Labor for unloading of dry NaOH requires 8 hours per
              16,000 Ibs delivered.  Liquid 50 percent NaOH
              requires 5 hours per 50,000 Ibs.
           Operating labor for dry NaOH feeders is 10
              min/day/feeder
           Operating labor for metering pump is 15 min/day
           Maintenance materials cost is assumed to be 3
              percent of the purchased equipment cost.
           Energy cost is based on the horsepower requirements
              for the feed pumps and mixers.  Energy requirements
              generally represent less than 5 percent of the total
              annual costs for the caustic feed system.
           Chemical cost is $1.183 per Ib.

    (3)  Polymer feed system

           Polymer requirements ajre based on a dosage of 2
              mg/1.
           The operating labor is assumed to be 134 hrs/yr,
              which includes delivery and solution preparation
              requirements.  Maintenance labor is estimated at 32
              hrs/yr.
           Energy costs for the feed pump and mixer are based
              on 17,300 kw-hr/yr.
           Chemical cost for polymer is based on $5.00/kkg
              ($2.225/lb).
                               309

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
      (4)  Reaction system

           Operating and maintenance labor requirements are 120
              hrs/yr.
           Pumps are assumed to require 0.005 hrs of mainte-
              nance/operating hr  (for flows less than 100 gpm)
              or 0.01 hrs/operating hr (flows greater than 100
              gpm), in addition to 0.05 hrs/operating day for
              pump operation.
           Maintenance materials costs are estimated as 5
              percent of the purchased equipment cost.
           Energy costs are based on the power requirements for
              the pump (function of flow) and agitator (0.06 hp/
              1,000 gal).  An agitator efficiency of 70 percent
              was assumed.

      (5)  Gravity settling system

            Annual operating and maintenance labor requirements
               range from 150 hrs for the minimum size clarifier
               (300 ft.2) to 500 hrs for a clarifier of 30,000
               ft.2.  In addition, labor hrs for operation and
               maintenance of the sludge pumps were assumed to
               range from 55 to 420 hrs/yr, depending on the pump
               capacity (10 to 1,500 gpm).
            Maintenance material costs are estimated as 3
               percent of the purchased equipment cost.
            Energy costs are based on power requirements for the
               sludge pump and rake mechanism.

Normal Batch Mode.   The normal batch treatment system,  which is
used  for  flows between 2,200 and 10,600 1/hr, consists  of  the
following equipment:

      (1)  Chemical precipitant feed system

          lime (batch)
          —slurry tank (5-minute retention time)
          —agitator
          —feed pump

          caustic (batch)
          —fiberglass  tank (1-week storage)
          —chemical metering pump

     (2)  Polymer feed  system

            chemical mix  tank
            agitator
            chemical metering pump

     (3)  Reaction system

            reaction tanks  (minimum of  2)  (8-hour retention
               time  each)
                               310

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
            agitators (2) (velocity gradient is 300 ft/sec/ft)
            pH control system

The  reaction tanks used for pH adjustment are sized to hold  the
wastewater volume accumulated for one batch period (assumed to be
8  hours).  The tanks are arranged in a parallel setup  to  allow
treatment  in  one tank while wastewater is  accumulated  in  the
other  tank.  A separate gravity settler is not  necessary  since
settling  can occur in the reaction tank after precipitation  has
taken place.  The settled sludge is then pumped to the dewatering
stage if necessary.

Direct  annual costs for the batch treatment system are based  on
the following assumptions:

     (1)  Lime feed system (batch)

            Operating labor requirements range from 15 to 60
               min/batch, depending on the feedrate (5 to 1,000 Ibs
               of hydrated lime/batch).
            Maintenance labor is assumed to be constant at 52
               hrs/yr (1 hr/week).
            Energy costs for the agitator and feed pump are
               assumed to be negligible.
            Chemical costs are based on the use of hydrated lime
               (see continuous feed system assumptions).

      (2) Caustic feed system (batch)

            Operating labor requirements are based on 30
               min/metering pump/shift.
            Maintenance labor requirements are 16 hrs/metering
               pump/yr.
            Energy costs are assumed to be negligible.
            Chemical costs are based on the use of 50 percent
               liquid caustic solution (see continuous feed
               system).

     (3)  Polymer feed system (batch)

            Polymer requirements are based on a dosage of
               2 mg/1.
            Operating and maintenance labor are assumed to
               require 50 hrs/yr.
            Chemical cost for polymer is based on $5.00/kkg
               ($2.25/lb).

     (4)  Reaction system

            Required operating labor is assumed to be 1 hr/batch
               (for pH control,  sampling, valve operation, etc.)
            Maintenance labor requirements are 52 hrs/yr.
            Energy costs are based on power requirements for
               operation of the sludge pump and agitators.
                               311

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         GENERAL DEVELOPMENT DOCUMENT
      SECT - VIII
Low-Flow  Batch Mode.   For small influent flows (less than 2,200
1/hr),it is more economical on a total annualized cost basis to
select  the "low flow" batch treatment system.   The lower  flows
allow an assumption of up to five days for the batch duration, or
holding  time,  as opposed to  eight hours for the  normal  batch
system.   However,  whenever the total batch volume (based  on  a
five-day  holding  time)  exceeds 10,000 gallons,  which  is  the
maximum single batch tank capacity, the holding time is decreased
accordingly  to maintain the batch volume under this level.   The
cutoff value used for maximum single batch tank capacity for  the
following  list of subcategories was 25,000 gallons, rather  thein
10,000  gallons:  primary aluminum, secondary  aluminum,  primary
copper,  secondary  copper, primary lead, primary  zinc,  primary
tungsten,   primary  columbium-tantalum,  secondary  silver   and
secondary lead.  Capital costs for the low flow system are  based
on the following     equipment:

    (1)  Reaction system

            reaction/holding  tank  (5-day or less retention  time)
            agitator
            transfer pump

    (2)  Polymer feed system (batch)

            chemical  mix  tank  (5-day  retention  time)
            agitator
            chemical metering pump


The  polymer feed system is included for the low flow system  for
manufacturing processes operating in excess of 16 hours per  day.
The addition of polymer for plants operating 16 hours or less per
day  is assumed to be unnecessary due to the additional  settling
time available.
Only  one  tank is required for both
since  sedimentation  is assumed to
production hours (since the holding
required  for treatment).  Costs for
system  are  not included since lime
application  rates  can  be assumed
operator.   A  common  pump  is used
supernatant   and   sludge   through
arrangement.
 equalization  and ' treatment
be accomplished  during  non-
time is greater than the time
 a chemical precipitant  feed
 or caustic addition  at  low
to be done  manually  by  the
 for  transfer  of  both  the
   an   appropriate   valving
As in the normal batch case, annual costs consist mainly of labor
costs  for  the low flow system and are based  on  the  following
assumptions:

(1)  Reaction system

       Operating labor is assumed to be constant at 1 hr/
          batch (for pH control, sampling, filling, etc.).
          For the primary aluminum, secondary aluminum,
                               312

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
          primary copper, secondary copper, primary lead, primary
          zinc, primary tungsten, primary columbium-tantalum,
          secondary silver, and secondary lead subcategories
          operating labor value of 2 hrs/batch is used.
          Additional labor is also required for the manual
          addition of lime or caustic, ranging from 15 minutes
          to 1.5 hrs/batch depending on the feed requirement
          (1 to 500 Ibs/batch).
       Maintenance labor is 52 hrs/yr  (1 hr/wk).
       Energy costs are based on power requirements
          associated with the agitator and pump.
       Chemical costs are based on the use of hydrated lime
          or liquid caustic (50 percent).

 (2)  Polymer feed system (batch)

       See assumptions for normal batch treatment.

The  capital  and  annual costs for  chemical  precipitation  are
presented  in Figure VIII-9 (page 358), for all  three  operating
modes.

Sulfide Precipitation and Gravity Settling

Precipitation  using  sulfide followed by gravity settling  is  a
technology  similar to lime precipitation.   In general,  sulfide
precipitation  removes  more  metals from  wastewater  than  lime
precipitation  because metal sulfides are less soluble than metal
hydroxides.   Another configuration using sulfide precipitation is
appropriate for removal of arsenic and selenium (as well as other
metals) in the metallurgical acid plant subcategory.  That system
is  discussed  in  Section VIII of the metallurgical  acid  plant
subcategory supplement.

Sulfide  precipitants  can be either soluble  sulfides  (such  as
sodium  sulfide,  or  sodium hydrosulfide) or insoluble  sulfides
(such as ferr-ous sulfide).   Soluble sulfides generate less sludge
than  insoluble  sulfides,   are  less  expensive,   and  are  more
commonly used in industry.    As such, • the sulfide  precipitation
module is based on the use of sodium sulfide.

The sulfide  precipitation system generally used for this category
consists  of the use of sulfide precipitation as a polishing step
following  chemical  precipitation  (described  above).    Sodium
sulfide  is  added to the wastewater.    The sodium sulfide  reacts
with the remaining dissolved metals to form metal  sulfides.    The
sodium  sulfide  concentration is calculated as  the  theoretical
stoichiometric   requirement   based  on  the   influent   metals
concentration.    To calculate chemical requirements,  the  sodium
sulfide dosage is obtained  by assuming an excess of 25 percent of
the theoretical sodium sulfide dosage.   This 25 percent excess of
sodium sulfide is needed to ensure complete reaction to the metal
sulfides within the time allowed in the reaction tank.  As  noted
below,  the sulfide dosage would actually be controlled in a plant
by  a specific-ion electrode.   Effluent concentrations are  based
                               313

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
on treatment effectiveness values for sulfide precipitation.

The reaction tank is equipped with a specific-ion electrode which
monitors  the  solution potential during the addition  of  sodium
sulfide.  The  sulfide ion reacts with the metals in solution  to
form  insoluble metal sulfides as discussed above.   When all  of
the metal is reacted,  excess sulfide ion causes a sharp negative
potential change,  which automatically stops the sulfide addition
at the correct point.   This control equipment helps to eliminate
the  release of H2S gas from the reaction  tank.   A  ventilation
hood  is included in the cost estimate to control any H2S  which
would be released.   As a final protection, an aeration system is
included to remove any excess sulfide prior to discharge.

As with lime precipitation costs,  the costs for sulfide precipi-
tation,  and gravity settling are based on one of three operation
modes,  depending on the influent flow rate:   continuous, normal
batch, and low flow batch.  The use of a particular mode for cost
estimation  purposes  was  determined  on  a  least  cost  (total
annualized) basis for a given flow rate.  The economic breakpoint
between  continuous  and  normal batch is assumed  to  be .10,600
liters/hour.  Below 2,200 liters/hour, it is assumed that the low
flow  batch system is most economical.  Although all three  modes
of  operation  were  available  for  cost  estimations  for   the
category,  the  flow  rates  for  all  plants  requiring  sulfide
precipitation  were in the continuous range of operation.   Since
only the continuous mode was used, the normal batch and low  flow
batch   operation  modes  are  not  included  in  the   following
discussion.
For a continuous operation, the following equipment were included
in the determination of the capital and annual costs:

(1)  Sodium sulfide feed system (continuous)

        storage  units (sized for 15-day storage)
        mix tank (5-minute retention time)
        feed pumps
        hood for ventilation

(2)  Polymer feed system

        storage hopper
        chemical mix tank with agitator
        chemical metering pump

(3)  pH adjustment system

        rapid mix tank, fiberglass
        agitator (velocity gradient is 300 ft/sec/ft)
        control system

(4)  Sulfide precipitation system

        rapid mix tank, fiberglass
                               314

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         GENERAL DEVELOPMENT DOCUMENT
                         SECT - VIII
        agitator  (velocity gradient is 300 ft/sec/ft)
        hood for ventilation
        a specific-ion electrode

(5)  Flocculation system

        slow mix tank, fiberglass
        agitator  (velocity gradient is 100 ft/sec/ft)
        2.0 mg/1 polymer dosage

(6)  Gravity settling system
        clarifie
          gpd/ft ,
        sludge pump (1)
,  circular,  steel (overflow rate is  500
  underflow  is 3 percent solids)
Lime is added to adjust pH as necessary.  Lime costs are included
in  the subcategory supplements where appropriate.   An  aeration
system  (tank and spargers) for removing excess hydrogen  sulfide
is also included in the costs.

The direct capital costs of the lime, sodium sulfide, and polymer
feed  systems  were based on the respective chemical  feed  rates
(dry Ibs/hour),  which are dependent on the influent waste stream
characteristics.   Direct  annual costs for the continuous system
include operating and maintenance labor for the feed systems  and
the  clarifier,  the cost of lime,  sodium sulfide,  and polymer,
maintenance  materials  and  energy costs  required  to  run  the
agitators  and  pumps.   The assumptions for each  of  these  are
similar  to those used for lime precipitation.  Cost  curves  are
presented  in  Figure VIII-10 (page 359), page  for  capital  and
annual  costs of the continuous system.  Figure VIII-10  presents
cost  curves for capital and annual costs that are applicable  to
the following list of subcategories:  primary aluminum, secondary
aluminum, primary copper, secondary copper, primary lead, primary
zinc,  primary  tungsten, primary  columbium-tantalum,  secondary
silver, and secondary lead.

Vacuum Filtration

The underflow from the clarifier at 3 percent solids is routed to
a  rotary precoat vacuum filter,  which dewaters sludge to a cake
of 20 percent dry solids.  The dewatered sludge is disposed of by
contract  hauling  and the filtrate is recycled to  the  chemical
precipitation step.

The  capacity of the vacuum filter,  expressed as square feet  of
filtration area,  is based on a yield of 14.6 kg of dry solids/hr
per square meter of filter area (3 lbs/hr/ft2),  a solids capture
of  95  percent and an excess capacity of  30  percent.   It  was
assumed that the filter operates eight hours/operating day.

Cost  data  were compiled for vacuum filters ranging from 0.9  to
69.7 m  (9.4 to 750 ft) of filter surface area.  Based on a total
annualized  cost  comparison,  it was assumed that  it  was  more
                               315

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         GENERAL DEVELOPMENT DOCUMENT
                          SECT - VIII
economical  to directly contract haul clarifier underflow streams
which were less than 50 1/hr (0.23 gpm),  rather than dewater  by
vacuum  filtration  before hauling.   For the following  list  of
subcategories,  a  flow  cutoff value of 42 1/hr (0.19  gpm)  was
used:   primary  aluminum,  secondary aluminum,  primary  copper,
secondary copper,  primary lead,  primary zinc, primary tungsten,
primary columbium-tantalum, secondary silver, and secondary lead.

The  costs for the vacuum filtration system include the following
equipment:

(1)  Vacuum filter with precoat but no sludge conditioning
(2)  Housing
(3)  Influent transfer pump
(4)  Slurry holding tank
(5)  Sludge pumps

The  vacuum filter is sized based on 8  hrs/day  operation.   The
slurry  holding  tank  and pump are excluded when  the  treatment
system operates 8 hrs/day or less.   It was assumed in this  case
that  the underflow from the clarifier directly enters the vacuum
filter and that holding time volume for the slurry in addition to
the clarifier holding time was unnecessary.   For cases where the
treatment system is operated for more than 8 hrs/day,  the under-
flow  is  stored during vacuum filter non-operating  hours.   The
filter  is sized accordingly to filter the stored slurry in an  8
hour period each day.   The holding tank capacity is based on the
difference  between the plant and vacuum filter  operating  hours
plus  an excess capacity of 20 percent.   Cost curves for  direct
capital  and annual costs are presented in Figure  VIII-11  (page
360), for vacuum filtration.  Figure VIII-11 presents cost curves
for capital and annual costs that are applicable to the following
list  of subcategories:   primary aluminum,  secondary  aluminum,
primary  copper,  secondary copper,  primary lead,  primary zinc,
primary tungsten,  primary columbium-tantalum,  secondary silver,
and secondary lead.
The  following
annual costs:
assumptions were made for developing capital  and
     (1)  Annual  costs  associated  with the vacuum filter  were
          developed  based on continuous operation  (24  hrs/day!
          365 days/yr).  These costs were adjusted for a plant  s
          individual  operating schedule by assuming that  annual
          costs  are proportional to the hours the vacuum  filter
          actually operates.  Thus, annual costs were adjusted by
          the  ratio of actual vacuum filter operating hours  per
          year  (8 hrs/day x no. days/yr) to the number of  hours
          in continuous operation (8,760 hrs/yr).

     (2)  Annual  vacuum  filter  costs  include   operating  and
          maintenance labor (ranging from 200 to 3,000 hrs/yr  as
          a  function  of  filter  size),  maintenance  materials
          (generally less than five percent of capital cost), and
          energy requirements (mainly for the vacuum pumps).
                               316

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
     (3)  Enclosure  costs  for  vacuum filtration were based  on
          applying rates of $45/ft2 and $5/ft /yr for capital and
          annual costs,  respectively to the estimated floor area
          required by the vacuum filter system.  The capital cost
          rate  for enclosure is the standard value as  discussed
          below  in  the  costs for  enclosures  discussion.  The
          annual   cost  rate  accounts  for  electrical   energy
          requirements  for the filter housing.   Floor area  for
          the enclosure is based on equipment dimensions reported
          in  vendor  literature,  ranging from 300 ft2  for  the
          minimum size filter (9.4 ft2) to 1,400 ft2 for a vacuum
          filtration capacity of 1,320 ft2.

Holding Tanks-Recycle

A  holding tank may be used to recycle water back to a process or
for miscellaneous purposes,  e.g.,  storage for hose washdown for
plant equipment.   Holding tanks are usually implemented when the
recycled water need not be cooled.   The equipment used to deter-
mine  capital  costs are a fiberglass  tank,  pump,  and  recycle
piping.   Annual  costs are associated only with the  pump.   The
capital  cost of a fiberglass tank is estimated on the  basis  of
required tank volume.   Required tank volume is calculated on the
basis of influent flow rate, 20 percent excess capacity, and four
hour retention time.  The influent flow and the degree of recycle
were derived from the assumptions outlined in Table VIII-9.

Cost  curves for direct capital and annual costs are presented in
Figure VIII-12 (page 361).

Multimedia Filtration

Multimedia filtration is used as a wastewater treatment polishing
device  to  remove  suspended  solids  not  removed  in  previous
treatment processes.  The filter beds consist of graded layers of
coarse  anthracite  coal  and fine sand. The  equipment  used  to
determine capital and annual costs are as follows:

(1)  Gravity flow,  vertical steel cylindrical filters with media
     (anthracite  and sand)
(2)  Influent storage tank sized  for  one backwash  volume
(3)  Backwash tank sized for one backwash volume
(4)  Backwash  pump  to  provide necessary  flow  and  head  for
        backwash  operations including an air scour system
(5)  Influent  transfer  pump including  piping,  valves,  and  a
         control system

The hydraulic loading rate is 7,335 Iph/m2 (180 gph/ft2) and  the
backwash loading rate is 29,340 lph/m2 (720 gph/ft2).  The filter
is  backwashed  once per 24 hours for 10 minutes.   The  backwash
volume is provided from the stored filtrate.

Effluent  pollutant  concentrations  are based  on  the  Agency's
combined  metals  data  base for treatability  of  pollutants  by
                               317

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          GENERAL DEVELOPMENT  DOCUMENT
SECT - VIII
 filtration  technology.

 Cartridge-type  filters are  used  instead of multimedia  filters   to
 treat  small flows  (less  than  800  liters/hour)  since  they are more
 economical   than  multimedia  filters at these  flows  (based  on   a
 least   total annualized  cost  comparison).   The effluent  quality
 achieved by these filters was equivalent to the level  attained  by
 multimedia  filters.   The equipment used to determine  capital and
 annual costs for membrane filtration are as follows:

 (1)  influent holding tank  sized  for eight hours  retention

 (2)  pump

 (3)  prefilter
     —prefilter cartridges
     —prefilter housings

 (g)  membrane filter
     —membrane filter cartridges
     —housing

 The majority of annual cost is attributable to replacement of the
 spent   prefilter  and membrane filter  cartridges.   The  maximum
 loading for  the  prefilter  and membrane filter  cartridges  was
 assumed to be  0.225 kg  per 0.254 meter length of cartridge.  The
 annual  energy and maintenance costs associated with  the pump  are
 also included in the total annual costs.  Cost curves  for  direct
 capital and annual costs are presented in Figure  VIII-13  (page
 362) for cartridge and multimedia filtration.

 Activated Carbon Adsorption

 Activated carbon is used to remove dissolved organic contaminants
 from wastewater.   As the wastewater is pumped through the carbon
 column,  organic  contaminants diffuse into the carbon  particles
 through pores and are adsorbed onto the pore walls.   As organic
 material accumulates, the carbon loses its effectiveness and must
 be replaced or regenerated periodically.

 Two  downflow  carbon columns in series are  used.   The  leading
 column  loses its effectiveness first, since most of  the  organics
 are  adsorbed  in it.  When breakthrough occurs (i.e.,  when  the
 column  effluent concentration of a specified organic  exceeds  a
 specified  maximum), the column is taken off-line and the  second
 column  becomes the leading column.  When the carbon  in the  first
 column  is  regenerated  or replaced, it  becomes  the  following
 column. This configuration, known as a merry-go-round, results in
 a  more consistent effluent quality than a single, larger  column
 or  a   system  where one column is active  and  one  on  standby.
 During  column operation,  solids accumulate in the interstices  of
 the  carbon  bed.   To prevent the column from plugging,  the  bed
must be periodically backwashed to remove these solids.  Also,  a
method   for   replacing  spent  carbon  is   required.    Either
 replacement  with virgin carbon and disposal of the spent  carbon
                               318

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GENERAL DEVELOPMENT DOCUMENT
                                          SECT - VIII
                                   off-site  or  on-site
                                     included   in   the
or  regeneration  of  the spent carbon via
regeneration may be used.

The   following  pieces  of  equipment  were
determination of capital and annual costs:

(1)  Carbon adsorption system

        adsorption columns (2), downflow, merry-go-round
           configuration
        —hydraulic loading of 2.5 gpm/ft2
        initial carbon charge
        pump

(2)  Backwash facilities
                                                 r\
        backwash hold tank - to provide 15 gpm/ft  per
           column for 15 min.
        pump

(3)  Influent surge tank (1-hour retention time)

(4)  Carbon replacement/regeneration facilities

        replacement
        off-site regeneration
        on-site regeneration

The direct capital costs for the adsorption system pump, backwash
facilities,  and  surge tank are direct or indirect functions  of
the influent flow rate.   Direct capital costs for the adsorption
columns and replacement or regeneration facilities are  functions
of  the influent flow rate and the rate at which carbon is  used,
or  the carbon exhaustion rate.  The rate (expressed in  kg/1  or
Ibs/  1,000  gal) used depended upon the data available  for  the
types of organic contaminants being adsorbed.  Carbon  adsorption
data  for  a  specific type of  wastewater  were  preferred  when
available;  otherwise,.isotherm data for selected  organics  were
used  with conservative design factors.  The specific  exhaustion
rates selected are provided in the subcategory supplements.

The  direct  annual costs for the  adsorption  columns,  backwash
facilities,  and  surge tank included operation  and  maintenance
labor  for  the  columns  and  backwash  facilities,  maintenance
materials, and energy costs for pumping.

The  carbon usage rate (kg carbon exhausted/hr) is a function  of
the  influent flow rate combined with the carbon exhaustion  rate
expressed as a carbon usage rate (Ibs carbon exhausted/hr).   One
of  three  operating  regimes is chosen on a  least  cost  (total
annualized)  basis for a given carbon usage rate.  Below a  usage
rate of about 1.6 Ibs/hr, replacement of spent carbon with virgin
carbon and disposal of the spent carbon as a hazardous waste  was
found  to  be  most  economical.   Between  1.6  and  53  Ibs/hr,
regeneration  by  an off-site regeneration service is  more  cost
                      319

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
effective.  On-site regeneration facilities are
above 53 Ibs/hr.
       more  economical
For   the  carbon  replacement  option,  no  additional   capital
investment is required.  Direct annual costs consist of  contract
hauling  the spent carbon as a hazardous waste and  the  purchase
and installation of virgin carbon.

Direct capital costs for the off-site regeneration option include
hoppers  for  dewatering  and  storage  of  spent  carbon.   Also
included  is the cost of acquiring an increased carbon  inventory
where the actual required inventory is less than the minimum  for
economical  off-site  regeneration (about  20,000  Ibs).   Direct
annual costs include the charge for regeneration,  transportation
of  the carbon to and from the regeneration facility,  and  costs
for placing carbon into the column.

Direct capital costs for an on-site regeneration facility include
costs  for  a multiple hearth furnace and  associated  equipment,
spent  carbon  storage,  exhaust gas scrubbers,  a carbon  slurry
system,  quench tank,  housing, and controls and instrumentation.
Direct  annual costs include operation and maintenance labor  for
the regeneration facility, maintenance materials, and electricity
and natural gas costs for the building, electrical equipment, and
furnace.   Also included is the cost of replacing carbon lost  in
the  regeneration process (10 percent of the spent carbon passing
through the furnace) with virgin carbon.

The  total  direct  capital and annual costs  for  the  activated
carbon  adsorption system are presented in Figure  Vlll-14  (page
363).  Figure VIII-14 presents cost curves for capital and annual
costs that are applicable to the following list of subcategories:
primary aluminum,  secondary aluminum,  primary copper, secondary
copper,  primary lead,  primary zinc,  primary tungsten,  primary
columbium-tantalum, secondary silver, and secondary lead.

Chemical Oxidation

Chemical  oxidation using ozone is an alternative  technology  to
activated  carbon adsorption in the bauxite refining  subcategory
for  removing dissolved organics from the red mud impoundment net
precipitation  discharges.   Compliance  costs  for  the  bauxite
subcategory  were based on activated carbon adsorption  since  it
was more cost-effective than chemical oxidation based on a  total
annualized cost comparison.  Chemical oxidation with ozone proved
to be uneconomical due to the capital intensive ozone  generation
equipment  required  for the relatively  high  ozone  consumption
rates encountered.

Ozone  and hydrogen peroxide are considered as chemical  oxidants
because  they  do  not  result  in  the  release  of    secondary
pollutants,  such as manganese or residual chlorine.   Given  the
high  pH of the red mud impoundment net  precipitation  discharge
(11.5),  ozone  was selected over hydrogen peroxide  because  the
peroxide reaction occurs optimally at a pH of 4 or less,  whereas
                               320

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
ozone only requires neutralization to a pH of 7. An ozone  dosage
level of 50 mg/1 was assumed for the particular organics and  COD
loadings   found  in  the  red  mud  impoundment  waste   stream.
Neutralization  of the waste stream to a pH of 7 with lime  prior
to contact with ozone was accounted for in developing costs.

The  costs  for chemical oxidation with ozone were based  on  the
following equipment:

(1)  Ozone generator
     —  ozone preparation and dissolution equipment
         electrical and instrumentation
     —  safety and monitoring equipment

(2)  Contact chamber, concrete (90 minute contact time)

(3)  Neutralization system
     —  mixing tank
     —  pump
         agitator

Annual  costs  comprise mainly the labor  and  electricity  costs
required  to operate the ozone generation equipment and operation
and maintenance cost of the neutralization system.

Contract Hauling

Concentrated  sludge  and waste oils are removed  on  a  contract
basis  for  off-site  disposal.   The cost  of  contract  hauling
depends  on  the  classification  of the waste  as  being  either
hazardous or nonhazardous.   For nonhazardous wastes,  a  rate of
$0.106/liter  ($0.40/gallon)  was used  in  determining  contract
hauling  costs.   The cost for contract hauling hazardous  wastes
was developed from a survey of waste disposal services and varies
with the amount of waste hauled.  No capital costs are associated
with  contract hauling.   Annual cost curves for contract hauling
nonhazardous  and hazardous wastes are presented in Figure  VIII-
15 (page 364).

Enclosures

The  costs  of  enclosures for equipment  considered  to  require
protection  from inclement weather were accounted for  separately
from  the  module  costs  (except  for  vacuum  filtration).   In
particular,  chemical  feed  systems were  generally  assumed  to
require enclosure.

Costs  for  enclosures  were  obtained by  first  estimating  the
required  enclosure area and then multiplying this value  by  the
unit  cost  in dollars per unit area. A capital cost  of  $485/m^
($45/ft2) was estimated, based on the following:
        structure  (including  roofing,  materials,
        etc.)
        site work (masonry, installation, etc.)
            insulation,
                               321

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
   —   electrical and plumbing

The rate for annual costs of enclosures is $54/m2 ($5/ft2)  which
accounts  for  energy requirements for heating and  lighting  the
enclosure.

The required enclosure area is determined as the amount to  total
required   enclosure  area  which  exceeds  the  enclosure   area
estimated to be available at a particular plant.  It was  assumed
that  a common structure could be used to enclose  all  equipment
needing housing unless information was available to indicate that
separate enclosures are needed (e.g., due to plant layout).   The
individual areas are estimated from equipment dimensions reported
by  vendors  and  appropriate  excess  factors.   The   available
enclosure  areas were assumed as a function of plant site,  based
on experience from site visits at numerous plants.

Segregation

Costs  for  segregation  of  wastewaters  not  included  in  this
regulation  (e.g.,  noncontact  cooling  water)  or  for  routing
regulated  waste streams not currently treated to  the  treatment
system  were  included  in the compliance  cost  estimates.   The
capital  costs for segregating the above streams were  determined
using  a  rate of $6,900 for each stream  requiring  segregation.
This rate is based on the purchase and installation of 50 feet of
10  cm (4-inch) piping (with valves, pipe racks, and elbows)  for
each  stream.   Annual  costs  associated  with  segregation  are
assumed to be negligible.

Where  a common stormwater-process wastewater piping  system  was
used at a plant, costs were included for both segregation of each
process  waste stream to treatment (based on the above rate)  and
segregation  of  stormwater  for rerouting around  the  treatment
system.

Stormwater  segregation cost is $8,800 based on  the  underground
installation  of  305 m (300 feet) of 0.61 m  J24-inch)  diameter
concrete pipe.

COMPLIANCE COST ESTIMATION

To  calculate  the compliance cost estimates,  the model was  run
using  input  data as described previously.   A cost  summary  is
prepared for each plant.  An example of this summary may be found
in Table VIII-10 (page 347).  Referring to this table, four types
of data are included for each option:  run number, total  capital
costs,  required  capital costs, and annual  costs.   Run  number
refers to the computer run from which the costs were derived.

Total  capital costs include the capital cost estimate  for  each
piece  of wastewater treatment equipment necessary to  meet  mass
limitations.    Required   capital  costs   are   determined   by
considering the equipment and wastewater treatment system a plant
currently  has in place.  As discussed previously,  the  required
                               322

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
capital  costs reflect the estimates of the actual  capital  cost
the  facility  will incur to purchase and install  the  necessary
treatment equipment by accounting for what that facility  already
has installed. Adequate operation and size of equipment currently
at a facility must be demonstrated before equipment is considered
to  be in place.  This prevents compliance cost  underestimation.
Annual costs are based on all equipment in the treatment  system,
as discussed previously.

NONWATER QUALITY ASPECTS

The  elimination  or  reduction  of one  form  of  pollution  may
aggravate  other  environmental  problems.   Therefore,  Sections
304(b)  and 306 of the Act require EPA to consider  the  nonwater
quality environmental impacts (including energy requirements)  of
certain  regulations.  In compliance with these  provisions,  EPA
has  considered the effect of this regulation on  air  pollution,
solid  waste generation, water scarcity, and energy , consumption.
This  regulation was circulated to and reviewed by EPA  personnel
responsible  for nonwater quality environmental programs.   While
it is difficult to balance pollution problems against each  other
and against energy utilization, the Administrator has  determined
that  the impacts identified below are justified by the  benefits
associated  with compliance with the limitations  and  standards.
The  following  are the nonwater  quality  environmental  impacts
associated with compliance with BPT, BAT, NSPS, PSES, and PSNS.

Air Pollution, Radiation, and Noise

In general, none of the wastewater treatment or control processes
causes air pollution.  Steam stripping of ammonia has a potential
to  generate atmospheric emissions,  however, with proper  design
and  operation, air pollution impacts are prevented.  Air  strip-
ping  to  ammonia also has a potential  to  generate  atmospheric
emissions,  because air stripping transfers ammonia from a  water
to an air medium.  Because air stripping was only considered as a
technology  option for plants which presently use air  stripping,
the  Agency  does . not  believe it will  create  an  air  quality
problem.   Sulfide precipitation operations can involve  hydrogen
sulfide  vapors  if not properly controlled.   EPA's  design  for
sulfide   precipitation  includes  an   automatic   pH-controller
equipped  with  a specific-ion electrode that  monitors  solution
potential  during  sulfide addition.  When all to  the  available
metal ions are sequestered by the sulfide, the excess sulfide ion
causes a sharp negative potential change, automatically  stopping
the sulfide addition.  None of the wastewater treatment processes
cause  objectionable  noise or have any potential  for  radiation
hazards.

Solid Waste Disposal

As shown in the subcategory supplements, the waste streams  being
discharged  contain large quantities of toxic and  other  metals:
the  most  common method to removing the metals  is  by  chemical
precipitation.    Consequently,  significant  volumes  of   heavy
                               323

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
metal  laden  sludge  are  generated that  must  be  disposed  of
properly.

The technologies that directly generate sludge are:

1.  Cyanide precipitation

2.  Chemical  precipitation  (lime,  caustic,   sulfide,   iron
    co-precipitation, etc.)

3.  Multimedia filtration

4. Oil-water separation

Spent  carbon from activated carbon adsorption also represents  a
solid  waste  stream  requiring  disposal.   The  sludge  volumes
generated by plants complying with these effluent limitations and
standards  are  estimated for each subcategory in  Table  VIII-12
(page 348).

The  estimated sludge volumes generated from wastewater treatment
were  obtained from material balances performed by  the  computer
model  during  cost estimation.   The sludges resulting from  the
technologies listed above will vary in characteristics  depending
on the subcategory and combination of streams being treated.  The
majority  of sludge produced will be either dewatered sludge from
filtration or sludge from chemical precipitation.

A  major concern in the disposal of sludges is the  contamination
of  soils,  plants,  and animals by the heavy metals contained in
the  sludge.   The  leaching  of heavy  metals  from  sludge  and
subsequent   movement  through  soils  is  enhanced   by   acidic
conditions. Sludges formed by chemical precipitation possess high
pH  values and thus are more resistant to acid  leaching.   Since
the  largest amount of sludge that results from the  alternatives
is  generated by chemical precipitation, it is not expected  that
metals  will  be readily leached from the  sludge.   Disposal  of
sludges  in  a lined sanitary landfill will  further  reduce  the
possibility  of heavy metals contamination of soil,  plants,  and
animals.

Other methods of treating and disposing sludge are available. One
method  currently  being used at a number of plants is  reuse  or
recycle,   usually   to   recover  metals.    Since   the   metal
concentrations in some sludges may be substantial, it may be cost
effective for some plants to recover the metal fraction of  their
sludges prior to disposal.

The  Solid Waste Disposal Act Amendments of 1980  prohibited  EPA
from  regulating  certain wastes under Subtitle C of  RCRA  until
completion of certain studies and certain rulemaking. Among these
wastes  are "solid waste from the extraction,  beneficiation  and
processing  of  ores and minerals."  EPA has  therefore  exempted
from  hazardous  waste  status  any  solid  wastes  from  primary
smelting and refining,  as well as from exploration,  mining, and
                               324

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
milling.

The  Agency  has  not  made  a  determination  of  the  hazardous
character  of  sludges  and  solid  wastes  generated  from   the
secondary  metals processing plants covered by  this  regulation.
Each  sludge generator in the secondary metals  subcategories  is
subject   to  the  RCRA  tests  for  ignitability,   corrosivity,
reactivity,  and  toxicity.  Costs for treatment and disposal  of
such  sludges and solid wastes, as well as  nonhazardous  sludges
and solid wastes, have been presented in this section.

Wastewater  treatment sludges from this category are expected  to
be  non-hazardous  by the E.P.   Toxicity test  under  RCRA  when
generated using the model technology.   The only sludges expected
to  be hazardous under RCRA,  generated as a result of wastewater
treatment, are those from sulfide or cyanide precipitation steps..
The  Agency  has included costs for disposal of  those  hazardous
sludges  in  its estimates of  compliance  costs.   Treatment  of
similar  wastewaters from other categories using this  technology
has  resulted  in non-hazardous sludges.   Costs for disposal  of
non-hazardous wastes are included in the annual costs.

Consumptive Water Loss

Treatment   and  control  technologies  that  require   extensive
recycling  and  reuse of water may  require  cooling  mechanisms.
Evaporative   cooling   mechanisms  can  cause  water  loss   and
contribute to water scarcity problems,  a primary concern in arid
and  semi-arid  regions.   While  this regulation  assumes  water
reuse,  the  overall amount of reuse through evaporative  cooling
mechanisms  is  low  and the quantity of water  involved  is  not
significant.   The  Agency has concluded that  consumptive  water
loss  is insignificant and that the pollution reduction  benefits
of  recycle  technologies  outweigh their impact  on  consumptive
water loss.

Energy Requirements

The  incremental  energy requirements of a  wastewater  treatment
system  have been determined in order to consider the  impact  of
this  regulation  on  natural resource depletion and  on  various
national economic factors associated with energy consumption. The
calculation  of  energy  requirements  for  wastewater  treatment
facilities  proceeded  in  two  steps.   First,  the  portion  jof
operating  costs which were attributable to  energy  requirements
was estimated for each wastewater treatment module.  Then,  these
fractions, or energy factors, were applied to each module in  all
plants  to  obtain the energy costs  associated  with  wastewater
treatment  for  each  plant.  These costs were  summed  for  each
subcategory and converted to kW-hrs using the electricity  charge
rate  previously mentioned ($0.0483/kW-hr for March  1982).   The
total  plant  energy  usage  was calculated  based  on  the  data
collection portfolios.

Table VIII-12 (page 349),  presents these energy requirements for
                               325

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         GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
each  regulatory option on each subcategory.   From the  data  in
this table, the Agency has concluded that the energy requirements
of  the proposed treatment options will not significantly  affect
the  natural resource base nor energy distribution or consumption
in communities where plants are located.
                               326

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         GENERAL DEVELOPMENT DOCUMENT
      SECT - VIII
                          Table VIII-1

                 BPT COSTS OF COMPLIANCE FOR THE
            NONFERROUS METALS MANUFACTURING CATEGORY
                                      Final Regulation Cost
                                        Estimates ($1982)
   Subcategory

Primary Lead
Primary Tungsten
Primary Columbium-Tantalum

Secondary Silver
Secondary Lead
Primary Antimony

Primary Beryllium
Primary and Secondary
  Germanium and Gallium
Primary Molybdenum and Rhenium

Metallurgical Acid Plants
  (associated with molybdenum
   roasters)
Secondary Molybdenum and
  Vanadium
Primary Nickel and Cobalt

Primary Precious Metals and
  Mercury
Secondary Precious Metals
Primary Rare Earth Metals

Secondary Tantalum
Secondary Tin
Primary and Secondary Titanium

Secondary Tungsten and Cobalt
Secondary Uranium
Primary Zirconium and Hafnium
   Capital

  242,000
  619/000
  680,000

  110,000
1,631,000
  196,400

  226,500
     B
  Annual

  112,000
1,008,000
1,139,000

  309,000
1,124,000
  554,200

  211,200
     B
B
B
B
B
2,200
B
A
B
841,300
644,500
B
54,800
B
B
B
B
B
26,800
B
28,700
B-
692,600
505,300
B
90,400
B
NOTES:  A = no incremental costs
        B = based on confidential data

*Costs are shown for the selected option only.
                               327

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         GENERAL DEVELOPMENT DOCUMENT.
       SECT - VIII
                          Table' VIII-2

                 BAT COSTS OF COMPLIANCE FOR THE
            NONFERROUS METALS MANUFACTURING CATEGORY
   Subcategory

Primary Lead
Primary Tungsten
Primary Columbium-Tantalum

Secondary Silver
Secondary Lead
Primary Antimony

Bauxite Refining
Primary Beryllium
Primary and Secondary
  Germanium and Gallium

Primary Molybdenum and Rhenium
Metallurgical Acid Plants
  (associated with molybdenum
  roasters)
Secondary Molybdenum and
  Vanadium

Primary Nickel and Cobalt
Primary Precious Metals and
  Mercury
Secondary Precious Metals

Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin

Primary and Secondary Titanium
Secondary Tungsten and Cobalt
Secondary Uranium

Primary Zirconium and Hafnium
 Number of
Dischargers
     3
     1
     0
     2.
     2
     1
     1
     1
     3
     3

     4
     4
     1
    Promulgated
  Regulation Cost
 Estimates  ($1982)*
  Capital    Annual

  242,000   112,000
  619,000 1,008,000
  680,000 1,139,000

  110,000   309,000
1,631,000 1,124,000
  196,400   554,200
     A
  226,500
     B
     B
     B
                  B
     B
    3,025

     B

     B
     B
     B

1,030,000
     B
   88,000

     B
   B
211,200
   B
   B
   B
   B
 27,300

   B

   B
   B
   B

585,000
   B
106,700

   B
NOTES:  A = no incremental costs
        B = based on confidential data
*Costs are shown for the selected option only,
                               328

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         GENERAL DEVELOPMENT DOCUMENT
          SECT - VIII
                          Table VIII-3

                PSES COSTS OF COMPLIANCE FOR THE
            NONFERROUS METALS MANUFACTURING CATEGORY
   Subcategory

Primary and Secondary
  Germanium and Gallium

Secondary Indium

Secondary Nickel

Secondary Precious Metals

Primary Rare Earth Metals

Secondary Tin

Primary and Secondary Titanium

Secondary Tungsten and Cobalt
   Number
of Indirect
Dischargers
     1

     1

    30

     1

     2

     2

     1
     Promulgated
   Regulation Cost
  Estimates ($1982)*
  Capital    Annual
                 B
               B
   17,300    25,400

  320,000   161,200

1,734,300 1,059,400

     B         B

  160,200    50,000

     B         B

   16,300     8,800
NOTES:  B = based on confidential information

*Costs are shown for the selected option only.
                               329

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                GENERAL  DEVELOPMENT  DOCUMENT
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-------
  GENERAL DEVELOPMENT DOCUMENT
  SECT - VIII
                   TABLE  VIII-7
           WASTEWATER SAMPLING FREQUENCY
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                        343

-------
GENERAL DEVELOPMENT DOCUMENT
SECT -. VIII
                 TABLE  VIII-8
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-------
                    GENERAL  DEVELOPMENT DOCUMENT
                                             SECT  -  VIII
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SECT -  VIII































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-------
GENERAL  DEVELOPMENT DOCUMENT
SECT  -  VIII

































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                              347

-------
         GENERAL DEVELOPMENT DOCUMENT
          SECT - VIII
                          TABLE VI11-11

        NONPERROUS METALS MANUFACTURING WASTE GENERATION
                             (tons/yr)
Subcategory                        Direct

Primary Aluminum
Secondary Aluminum
Primary Copper

Secondary Copper
Secondary Silver
Primary Lead

Primary Zinc
Metallurgical Acid Plants
Primary Tungsten

Primary Columbium & Tantalum
Secondary Lead
Primary Antimony

Bauxite Refining
Primary Beryllium
Primary Boron

Primary Cesium and Rubidium
Primary & Secondary Germanium
  & Gallium
Secondary Indium                     0

Secondary Mercury                    0
Primary Molybdenum & Rhenium      1682
Secondary Molybdenum & Vanadium    850

Primary Nickel and Cobalt           10.4
Secondary Nickel                     0
Primary Precious Metals & Mercury   11.4

Secondary Precious Metals          524
Primary Rare Earth Metals            0
Secondary Tantalum                 173

Secondary Tin'                    2762
Primary & Secondary Titanium       339
Secondary Tungsten & Cobalt        562

Secondary Uranium                  320
Primary Zirconium & -Hafnium       2624
                                        Discharger Type
734336
     *
     *
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    65a

     3.5a
    88a
   896

 17932

  3361

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   695
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     0
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   NA
 5697
   NA

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 1212

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  170

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  423
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   17
    0

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   50.2
    0.2

    0
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* Solid waste generation accounted for by existing BPT regulation
a -  Sulfide precipitation sludge
                               348

-------
         GENERAL DEVELOPMENT DOCUMENT
                                          SECT - VIII
                          TABLE VII1-12

        NONFERROUS METALS MANUFACTURING ENERGY CONSUMPTION
                           (kW-hr/yr)
Subcategory

Primary Aluminum
Secondary Aluminum          -,:
Primary Copper

Secondary Copper
Secondary Silver
Primary Lead

Primary Zinc
Metallurgical Acid Plants
Primary Tungsten

Primary Columbium & Tantalum
Secondary Lead
Primary Antimony

Bauxite Refining
Primary Beryllium
Primary Boron               :

Primary Cesium and Rubidium
Primary & Secondary Germanium
  & Gallium                t
Secondary Indium
                                  BPT
                                     *
                                     *
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                                125247

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                               3373589
                               1727280
                                393800

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                                    NA

Secondary Mercury                    0
Primary Molybdenum & Rhenium   1261200
Secondary Molybdenum & Vanadium 926000

Primary Nickel and Cobalt        20600
Secondary Nickel            ;     „   NA
Primary Precious Metals & Mercury 4224

Secondary Precious Metals       489000
Primary Rare Earth Metals        43500
Secondary Tantalum               16000

Secondary Tin                   576000
Primary & Secondary Titanium    680340
Secondary Tungsten & Cobalt  .. 1150000

Secondary Uranium                57000
Primary Zirconium & Hafnium -  12210000
  BAT

11079204
  884061
  166302

       *
  711872
 1100028

   69564
  469968
 4641860

 3406603
 1813408
  396500

       0
 1137000
       0

       0
       0

      NA

       0
 1267200
  936000

   28570
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  497000
   39400
   18000

  581000
  687150
 1185000

   66000
12264000
  PSES

     NA
1613178
     NA

 179190
 217053
     NA

  13706
  16666
 904665

1859916
3607300
     NA

     NA
     NA
      0

      0
   6253

   5900

      0
     NA
     NA

     NA
  88300
     NA

4981000
  26000
     NA

 319200
 340300
   3700

     NA
     NA,
NOTE: NA = not applicable
      * Energy consumption was considered for the promulgated BPT
      regulation; no additional energy consumption is attributed .
      to this regulation.
                               349

-------
   GENERAL DEVELOPMENT  DOCUMENT
SECT -  VIII
       Input
    User-Specified
      Variables
                Figure VIII-1

GENERAL LOGIC DIAGRAM OF COMPUTER COST MODEL
                     350

-------
GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
             Figure VIII-2




LOGIC DIAGRAM OF MODULE DESIGN PROCEDURE
                 351

-------
   GENERAL DEVELOPMENT DOCUMENT
SECT - VIII
                  DESIGN VALUES
                AND CONFIGURATION
                  FROM MATERIAL
                BALANCE PROGRAM
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                Figure VIII-3

LOGIC  DIAGRAM OF THE COST ESTIMATION  ROUTINE
                     352

-------
GENERAL DEVELOPMENT DOCUMENT
SECT  -  VIII
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-------
GENERAL DEVELOPMENT DOCUMENT
SECT  -  VIII
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-------
             GENERAL DEVELOPMENT DOCUMENT
SECT  -  VIII
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                            Figure VIII-6



        CAPITAL AND ANNUAL COSTS FOR CYANIDE  PRECIPITATION
                                355

-------
        GENERAL DEVELOPMENT DOCUMENT
                            SECT -  VIII


























































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GENERAL DEVELOPMENT  DOCUMENT
SECT  - VIII
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-------
     GENERAL DEVELOPMENT DOCUMENT
SECT  -  VIII
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                SECT  - VIII
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                         359

-------
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SECT  -  VIII








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-------
           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
                           SECTION IX

     EFFLUENT QUALITY ATTAINABLE THROUGH APPLICATION OF THE
     BEST PRACTICABLE CONTROL TECHNOLOGY CURRENTLY AVAILABLE
This  section  sets  forth the  effluent  limitations  attainable
through  the  application of best practicable control  technology
currently available  (BPT).   It also serves to summarize  changes
from  previous rulemakings in the nonferrous metals manufacturing
category,  and presents the development and use of the mass-based
production related effluent limitations.

A  number  of  considerations guide  the  BPT  analysis.   First,
effluent  limitations based on BPT generally reflect  performance
levels  achieved at plants in each subcategory equipped with  the
best   wastewater  treatment  facilities.    The   BPT   analysis
emphasizes  treatment  facilities  at the end of a  manufacturing
process  but  can also include in-plant control  techniques  when
they are considered to be normal practice within the subcategory.
Finally,  the  Agency closely examines the effectiveness  of  the
various treatment technologies by weighing the pollutant removals
achievable   by  each  treatment  alternative  and  by  assessing
installation and operational costs.

The  limitations are organized by subcategory,  and are presented
in  Section II of each subcategory supplement..  The  limitations
were  developed based on the sampling,  treatment  effectiveness,
and cost data that have been presented in this document.

TECHNICAL APPROACH TO BPT

In  the  past, the technical approach for the  nonferrous  metals
manufacturing   category  considered  each  plant  as  a   single
wastewater source, without specific regard to the different  unit
processes  that are used in plants within the  same  subcategory.
This approach may be appropriate for BPT which is generally based
upon  end-of-pipe technology.  In-process controls are  generally
not used to establish BPT; however, they may be used as the basis
of  BPT when they are widely used in the category.  In  reviewing
the existing BAT regulations and developing new BAT  regulations,
the  Agency closely examined each process and the  potential  for
implementing in-process controls.  It became apparent that it was
best to establish effluent limitations and standards  recognizing
specific  waste  streams associated with  specific  manufacturing
operations.   This  also  results  in  more  effective  pollution
abatement  by tailoring the regulation to reflect  these  various
wastewater   sources.    Currently   promulgated   BPT   effluent
limitations  and standards which have been developed  using  this
approach generally have not been modified.

This  approach,  referred  to  as the  building  block  approach,
establishes  pollutant discharge limitations for each  source  of
wastewater  identified within the subcategory.   Each  wastewater
                               365

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
source  is  allocated a discharge based on the  average  reported
discharge  rates  for that source.   These flows  are  normalized
(related  to  a common basis) using a  characteristic  production
parameter  associated with the wastewater source (e.g.  volume  of
wastewater  discharged  per unit mass of production).   The  mass
limitations  established for a wastewater source are obtained  by
multiplying   the  effluent  concentrations  attainable  by   the
selected   BPT   technology  by   the   regulatory    (production
normalized) flow for each wastewater source.  Thus, the  specific
pollutant  discharge  allowances for a  plant's  final  discharge
permit  are calculated by multiplying the appropriate  production
rates with the corresponding mass limitations for each wastewater
source  in  that  plant,  and  then  summing  the  results.  This
calculation  is performed to obtain the one-day maximum  and  the
monthly  average limitations.  It is important to note  that  the
plant  need only comply with the total mass limitations  for  the
discharge   and  not the flow allowances or  concentrations.   In
cases  where  process  wastewaters  and  nonprocess  waters   not
specifically  regulated by this proposal are discharged  together
from  a facility, the permit authority must treat the  nonprocess
segment on a case-by-case basis.

Although  each  waste  stream  may  not  include  each   selected
pollutant,  discharge allowances are provided for all  pollutants
in  every  waste stream from the same  subcategory  because  each
waste stream contributes to the total loading of a combined waste
treatment  system.  Since a discharge allowance is  included  for
each  pollutant  in every waste stream, facilities would  not  be
required to reduce pollutant concentrations below the performance
limits of the technology. Instead, this approach allows plants to
achieve  the  performance determined for the  technology  at  the;
plant  discharge point. Therefore, the mass limitation  for  each
pollutant   in  each  building  block  is  the  product  of   the
concentration   achievable  by  the  technology  basis   of   the
limitation and the regulatory flow for that building block.

In determining the technology basis for BPT,  the Agency reviewed
a wide range of technology options and selected four alternatives
which could be applied to nonferrous metals manufacturing as  BPT
options.  These options include:

1.  Option  A  -  End-of-pipe treatment  consisting  of  chemical
    precipitation  and clarification, and preliminary  treatment,
    where   necessary,  consisting  of  oil   skimming,   cyanide
    precipitation,  sulfide precipitation, iron  coprecipitation,
    and  ammonia  air  or steam stripping.  This  combination  of
    technologies reduces toxic metals and cyanide,  conventional,
    and  nonconventional  pollutants.  Ion  exchange  end-of-pipe
    treatment  is  also included in Option A where  necessary  to
    reduce certain nonconventional pollutants.

2.  Option B - Option B is equal to Option A preceded by     flow
    reduction  of process wastewater through the use  of  cooling
    towers  for contact cooling water and holding tanks  for  all
    other process wastewater subject to recycle.
                               366

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
 3.  Option C - Option C is equal to Option B plus end-of-
     pipe polishing filtration for further reduction of
     priority metal pollutants and TSS.

 4.  Option  E  - Option E consists of Option  C  plus  activated
     carbon adsorption applied to the total plant discharge as  a
     polishing step to reduce toxic organic concentrations.

Two  additional  technologies,   activated  alumina  and  reverse
osmosis,  were evaluated prior to proposing mass limitations  for
this  category.   Activated  alumina treatment was  included  for
reduction  of  fluoride  and  arsenic  concentrations.    Reverse
osmosis  was  considered so that complete recycle of all  process
wastewater   could  be  attained.    However,   both   of   these
technologies  were rejected because they are not demonstrated  in
the  nonferrous  metals  manufacturing  category,  nor  are  they
clearly . transferable.

For  each of the selected options,  the mass of pollutant removed
and  the  costs associated with application of  the  option  were
estimated.   A  description  of the pollutant  removal  estimates
associated  with  the application of each option is presented  in
Section  X,  while the cost methodology is presented  in  Section
VIII.

MODIFICATIONS TO EXISTING BPT EFFLUENT LIMITATIONS

Prior  to this rulemaking session,  BPT effluent limitations were
promulgated  for nine of the 31 nonferrous  metals  manufacturing
subcategories:

     1.  bauxite refining,
     2.  primary aluminum smelting,
     3.  secondary aluminum smelting,
     4.  primary copper smelting,
     5.  primary electrolytic copper refining,
     6.  secondary copper,
     7.  primary lead,
     8.  primary zinc, and
     9.  metallurgical acid plants.

On  February 17,  1983, four new subcategories were proposed  for
inclusion  in  the nonferrous metals manufacturing  point  source
category   (48 FR 7032).  No effluent limitations had  previously
been promulgated for these subcategories.

     1.  primary tungsten,
     2.  primary columbium-tantalum,
     3.  secondary silver, and
     4.  secondary lead;

On  June  27,  1984,  20  new  subcategories  were  proposed  for
inclusion  in  the nonferrous metals manufacturing  point  source
category  (49  FR 26352.)  There had been  no  previous  effluent
                               367

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
limitations  developed  for these  20  subcategories.   Following
proposal,  EPA  decided to exclude two of the  20  subcategories,
primary boron and primary cesium and rubidium,  from  regulation.
The  20 new subcategories EPA proposed for regulation are  listed
below:
                           »
1.  primary antimony
2.  primary beryllium
3.  primary boron
4.  primary cesium & rubidium
5.  primary and secondary germanium and gallium
6.  secondary indium
7.  secondary mercury
8.  primary molybdenum and rhenium
9.  secondary molybdenum and vanadium
10. primary nickel and cobalt
11. secondary nickel
12. primary precious metals and mercury
13. secondary precious metals
14. primary rare earth metals
15. secondary tantalum
16. secondary tin
17. primary and secondary titanium
18. secondary tungsten and cobalt
19. secondary uranium
20. primary zirconium and hafnium

EPA  modified  BPT  effluent limitations  for  the  primary  lead
subcategory  and secondary aluminum subcategory because new  data
and  information  submitted to the Agency made  it  necessary  to
revise  these  limits.  EPA is modified  the  metallurgical  acid
plants subcategory to include acid plants associated with primary
molybdenum,   primary  zinc  and  primary  lead.   In   addition,
modifications were promulgated for existing stormwater exemptions
previously promulgated in the primary lead subcategory.

PRIMARY LEAD

The  1975  promulgated BPT for this subcategory is based  on  the
complete recycle and reuse of slag granulation wastewater (or dry
slag dumping),  dry air scrubbing,  and treatment and impoundment
(subject  to  allowances for net precipitation  and  catastrophic
precipitation  events)  of  acid plant  blowdown.   As  mentioned
earlier,   acid   plant  wastewater  is  now  included   in   the
metallurgical  acid plants subcategory.   This suggests that  BPT
for primary lead should be zero discharge.   Since 1975,  however,
additional  data  collected  by the Agency support the  need  for
discharge of wastewater from slag granulation.   Although it  was
previously thought that slag granulation is a net water consuming
operation,  the additional data show that at least one plant uses
an ore with a lead content sufficiently high to justify recycling
blast  furnace  slag into the sintering machine  to  recover  the
remaining  lead content.  For this reason, EPA modified the  1975
promulgated  BPT for this subcategory to allow a  discharge  from
dross slag granulation operations.
                               368

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - IX
METALLURGICAL ACID PLANTS

On  February 17,  1983,  EPA proposed to expand the metallurgical
acid  plants subcategory to include metallurgical acid plants  at
primary  lead  and  primary zinc smelters as  well  as  those  at^
primary copper smelters.
                                                     subcategory.
                                                     under  their
On  June  27,  1984,  EPA proposed to include  metallurgical  acid
plants    associated  (i.e.,  on-site)  with  primary   molybdenum
roasters  as part of the metallurgical acid  plants
These  operations,  which were previously regulated
respective  primary  metal  subcategories,  are  now  subject  to
limitations  for acid plants. All these plants would  accordingly
have  identical  effluent  limitations and  standards,  with  one
exception:   acid  plants  associated  with  primary   molybdenum
roasters  would  also have fluoride and molybdenum  regulated  in
their  effluent.   In making this determination,  that  all  acid
plants be regulated in one subcategory, the Agency considered the
way  in which acid plants are operated when associated  with  the
primary   smelters  and  the  characteristics  of  the  wastewater
generated by  each type to acid plant.  Our conclusion  is  that
these  processes,  rate  of  process  discharge,  and  wastewater
matrices  are  similar, justifying a single subcategory  for  all
acid plants.

Metallurgical  acid  plants are constructed on-site with  primary
copper,   lead, zinc, and molybdenum smelters to treat the smelter
emissions,  remove the sulfur dioxide,  and produce sulfuric acid
as  a marketable by-product.   Although two  basic  technologies,
single contact and double contact,  are used in the industry, the
Agency  found  no predominance of either technology in  place  in
plants  of the four metal types.   Finally,  the Agency found  no
difference  in  the characterization of the wastewater at  plants
which burn supplemental sulfur.

The  processes  are  also  similar  in  terms  of  waste  streams
generated. Wastewaters are typically combined in acid plants into
a  single waste stream (acid plant blowdown).  Principal  streams
going  into  the blowdown (compressor condensate,  blowdown  from
acid  plant scrubbing,  mist precipitation, mist elimination,  and
steam generation) are common to all four types of plants.

The  wastewater matrices from all four types of acid plants  also
are  similar.   The Agency reviewed the analytical data that were
obtained  in sampling programs described in Section V and compared
the characteristics of untreated acid plant blowdown from  plants
associated with each of the four primary metals considered. There
were   similar  concentrations  (i.e.,  in  the  same  order   of
magnitude) of antimony, arsenic, chromium, mercury,  and selenium,
among   the   four.   All  of  these  metals  were   present   at
concentrations   that   are  treatable  to  the   same   effluent
concentration  upon  application of  chemical  precipitation  and
sedimentation   or  chemical  precipitation,  sedimentation   and
multimedia   filtration,   and  are  within  the  range  used   in
                               369

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           GENERAL DEVELOPMENT DOCUMENT
  SECT - IX
calculating treatment effectiveness for these technologies.   One
dissimilarity  which was observed between molybdenum  acid  plant
wastewater  matrices and the matrices associated with other  acid
plants   is  that  treatable  concentrations  of   fluoride   and
molybdenum  are present in molybdenum acid plant wastewaters  and
not in the wastewaters from other metallurgical acid plants.  The
Agency is establishing limitations for fluoride and molybdenum in
discharges from metallurgical acid plants associated with primary
molybdenum  roasters.  Molybdenum limitations are based  on  iron
co-precipitation preliminary treatment.

Therefore,  in light of these essential similarities of  process,
wastewater  flow and composition,  we have chosen to include  all
acid plants in a single subcategory.

MODIFIED APPROACH TO STORMWATER

Stormwater,  in all effluent limitations and standards, is  only
considered process wastewater when commingled with actual process
wastewater.  If commingling occurs, the stormwater, which usually
does not contain significant pollutant loadings,  is contaminated
with  the pollutants contained in the process wastewater,  and as
such should be subject to treatment.   No allowance,  however, is
given  for this additional flow,  since stormwater is or  can  be
segregated  from  the process wastewater.

Existing  BPT  effluent  limitations for  the  nonferrous  metals
subcategories  primary  copper smelting,  secondary  copper,  and
primary lead have promulgated stormwater exemptions.   Facilities
in  these  three subcategories are subject to  a  zero  discharge
requirement  according  to promulgated BPT effluent  limitations;
however,  facilities meeting certain design capacity requirements
could  discharge,  regardless of effluent quality,  a  volume  of
water  falling  within the impoundment in excess of the  10-year,
24-hour storm,  when a storm of at least that magnitude occurred.
Further,  facilities  in  the secondary copper and  primary  lead
subcategories   can  discharge  once  per   month,   subject   to
concentration-based effluent limitations, a volume of water equal
to  the difference between precipitation and evaporation  falling
on the impoundment in that month.

The Agency made some revisions to some of these impoundment-based
regulations  in 1980 for primary copper smelting and electrolytic
refining  BPT.   The  1983-1989  rulemaking  session  promulgated
revisions to others.   The revised regulations are based on  end-
of-pipe   treatment   using  hardware  (lime  precipitation   and
sedimentation  technology  using  clarifiers).    By  eliminating
impoundments,  the  need  for a net precipitation  allowance  and
stormwater discharge (subject to an exception discussed below) is
eliminated.
The   Agency   is  reluctant  to  issue
impoundments for a number of reasons:
limitations   based   on
     1.   Discharge from impoundments can be as a "slug,"
                               370

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
          allowing potentially heavy and damaging pollutant
          loadings to be discharged all at once;

     2.    Impoundments allow dilution of heavily contaminated
          process wastewaters with relatively cleaner process
          streams;

     3.    Net precipitation limitations are hard to calculate
          because of periodic shifts between net precipitation
          and net evaporation;

     4.    Impoundments pose a risk of groundwater contamination;
          and,

     5.    Impoundment-based regulations effectively require the
          Agency to specify impoundment design.

For  reference,  see  generally 45 FR at 44926  (July  2,  1980),
revising  impoundment-based  regulations  in the  primary  copper
smelting and electrolytic refining subcategories.   In  addition,
plants  within these subcategories have,  in many cases,  already
installed  hardware-based  lime precipitation  and  sedimentation
technology,  so  that these technologies are now BPT or  BAT  for
these subcategories.

In   light  of  these  considerations,   an  allowance  for   net
precipitation  is  not  included for BPT  for  the  primary  lead
subcategory  because  the  effluent limitations for BPT  are  not
based  on  settling and evaporation  impoundments.   EPA  is  not
promulgating  any  modifications  to previously  promulgated  BPT
effluent   limitations  for  the  primary  copper  smelting   and
secondary copper subcategories.

It  is  recognized that this approach to  catastrophic  rainfalls
varies  from  the approach .used for the ore mining  and  dressing
category  (47 FR 54603).   In that regulation EPA  required  only
that the- impoundments be designed and operated so as to contain a
10-year,   24-hour  storm,   while  this  promulgated  regulation
requires  that no discharge from the impoundment may occur except
when  a  10-year,  24-hour  storm  occurs.   This  difference  is
justified  by the fact that the nonferrous  metals  manufacturing
allowance  applies  only to water falling on the surface  of  the
impoundment  while the ore mining allowance applies to stormwater
drainage  from various processing locations at the ore  mine  and
mill.   The  relative surface area of a nonferrous  manufacturing
impoundment  is  a small fraction of the area drained at  an  ore
mine or mill.  Therefore, the quantity of stormwater that must be
contained  at  a nonferrous plant impoundment  is  much  smaller,
making containment of the stormwater under the provisions of this
regulation  achievable.   The  Agency  believes  that   decisions
regarding stormwater are site-specific and are best handled based
on the judgment of individual permit writers.
                               371

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
BPT  OPTION SELECTION

The   treatment  option selected for the technology basis  of  BPT
throughout  the category  is Option A  (chemical precipitation  and
sedimentation, with ammonia steam or  air stripping, oil skimming,
sulfide   precipitation,   iron  co-precipitation   and   cyanide
precipitation   pretreatment,   and   ion-exchange    end-of-pipe
treatment    where    appropriate).    Chemical    precipitation,
sedimentation,  and ammonia stripping are widely demonstrated  at
plants with the best treatment practices in the nonferrous metals
manufacturing  category.  Of the 240 discharging plants (shown  by
subcategory in table IX-1, (page 384), 133 plants have  treatment
to   remove metals and suspended solids, one plant  practices  oil
skimmig,  one  plant has  technology   for  cyanide  precipitation,
eight have technology for cyanide oxidation, 11 practice  ammonia
stripping, three employ ion exchange  and 13 practice  end-of-pipe
filtration.  The remainder of the dischargers did not report  any
treatment for their nonferrous metals manufacturing  wastewaters.
The  preponderance  of technology is  chemical  precipitation  and
sedimentation equipment.  Multimedia  filtration (Option C) as  an
add-on  polishing  step to the  precipitation  and  sedimentation
system  was  not  selected  at  BPT   since  it  was  less  widely
demonstrated.

Recycle  after  treatment  consisting of lime  precipitation  and
sedimentation  is  practiced at ""one   plant.   Thirty-nine  plants
practice recycle of scrubber water without any treatment, and two
plants practice recycle of process water using cooling towers.

Between 1975 and 1980, BPT effluent limitations were  promulgated
for nine of the 36 nonferrous metals  manufacturing subcategories,
namely,  bauxite refining, primary aluminum, secondary  aluminum,
primary  copper smelting,.primary electrolytic  copper  refining,
secondary  copper, primary lead, primary zinc, and  metallurgical
acid plants.  Of the remaining 27 subcategories, EPA has reserved
setting  BPT  limitations for the following  three  subcategories
because there are no existing direct  discharging plants in  these
subcategories:

1.  Secondary Indium
2.  Secondary Mercury
3.  Secondary Nickel

As discussed earlier, EPA has excluded the following five sub-
categories from limitations.

1.  Primary Boron
2.  Primary Cesium and Rubidium
3.  Primary Lithium
4.  Primary Magnesium
5.  Secondary Zinc
Effluent  BPT limitations were promulgated for the
subcategories in 1985:
        following   18
                               372

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
1.  Primary Tungsten
2.  Primary Columbium-Tantalum
3.  Secondary Silver
4.  Secondary Lead
5.  Primary Antimony
6.  Primary Beryllium
7.  Primary and Secondary Germanium and Gallium
8.  Primary Molybdenum and Rhenium
9.  Secondary Molybdenum and Vanadium
10. Primary Nickel and Cobalt
11. Primary Precious Metals and Mercury
12. Secondary Precious Metals
13. Secondary Tantalum
14. Secondary Tin
15. Primary and Secondary Titanium
16. Secondary Tungsten and Cobalt
17. Secondary Uranium
18. Primary Zirconium and Hafnium

Briefly discussed below are descriptions of the options  selected
for each of these 18 subcategories.  A discussion of primary lead
and   secondary  aluminum  BPT  option  selection  will  also  be
presented   since  limitations  for  these   subcategories   were
modified. The mass limitations developed for these  subcategories
are   presented   in  Section  II  of  this  document   and   the
corresponding supplements.  Table IX-2 (page 386)    presents the
pollutants selected for limitation in each of the subcategories.


PRIMARY LEAD

The   technology   basis   for  the  BPT  limitations   is   lime
precipitation  and sedimentation technology to remove metals  and
solids  from  combined  wastewaters  and  to  control  pH.   This
technology is demonstrated at two primary lead smelters and  will
remove  an  estimated  4,286  kg/yr  of  toxic  metals  from  the
estimated  raw discharge.   Removal of TSS from raw discharge  is
estimated, at  261,130 kg/yr.   The capital and annual costs  for
achieving BPT are estimated at $0.24 million (March 1982 dollars)
and $0.11 million, respectively.

PRIMARY TUNGSTEN

The   technology   basis  for  the  BPT   limitations   is   lime
precipitation  and sedimentation technology to remove metals  and
solids  from combined wastewaters and to control pH,  and ammonia
steam stripping to remove ammonia.  Lime and settle technology is
already inplace at three direct dischargers for this subcategory.
Ammonia steam stripping is used by one direct discharger.

Implementation of the promulgated BPT limitations will result  in
the  removal  of 5,350 kg/yr of toxic metals from  raw  discharge
estimates.   Removal  estimates from raw discharge for ammonia is
141,000  kg/yr and 50,300 kg/yr of TSS.   The capital  and annual
costs  for  achieving BPT are estimated at $0.62  million  (March
                               373

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           GENERAL DEVELOPMENT DOCUMENT
                        SECT - IX
1982 dollars) and $1.0 million, respectively.

PRIMARY COLUMBIUM-TANTALUM

The  technology basis for BPT effluent mass limitations  is  lime
precipitation and sedimentation to control toxic metals,  TSS, pH
and  fluoride,  and  ammonia steam stripping.   Lime  and  settle
technology  is currently inplace at all three direct dischargers.
Ammonia  steam  stripping is currently used at two of  the  three
direct discharging facilities.

Application of BPT treatment will result in the removal of 61,000
kg/yr  of  toxic  pollutants,  1,692,000  kg/yr  of  conventional
pollutants,  and  941,000  kg/yr  of ammonia from  raw  discharge
estimates.   The  estimated  capital investment cost  of  BPT  is
$0.680 million (March 1982 dollars) and the estimated annual cost
is $1.14 million.  These costs represent wastewater treatment not
currently in place.

SECONDARY SILVER

The technology basis for BPT effluent mass limitations is lime
precipitation  and sedimentation to remove toxic metals  and  TSS
and  to  control  pH.   Ammonia  steam stripping  is  applied  as
pretreatment for removal of ammonia.   Lime and settle  treatment
is  currently in place at five direct dischargers,  while ammonia
steam  stripping is transferred from the  columbium-tantalum  and
tungsten subcategories.

The promulgated BPT will result in the removal of 30,900 kg/yr of
toxic  pollutnts and 664,000 kg/yr of ammonia from estimated  raw
discharge levels.   The estimated capital investment cost of  BPT
is  $0.11  million (March 1982 dollars) and the estimated  annual
cost  is  $0.31  million.    These  costs  represent   wastewater
treatment equipment not currently in place.

SECONDARY LEAD

The  technology  basis for BPT effluent mass limitations for  the
secondary   lead   subcategory   is   lime   precipitation    and
sedimentation  to  control  toxic  metals,  pH,  and  TSS.   This
technology is currently inplace at five discharging facilities in
the secondary lead subcategory.

The promulgated BPT will result in the removal of 25,350 kg/yr of
toxic  pollutants and 2,852,000 kg/yr of conventional  pollutants
from  estimated  raw  discharge levels.   The  estimated  capital
investment  cost of BPT is $1.6 million (March 1982 dollars)  and
the  estimated  annual  cost  is  $0.684  million.   These  costs
represent wastewater treatment equipment not currently in place,,
PRIMARY ANTIMONY

The   technology
basis  for  the  BPT
limitations
is
     lirne
                               374

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
precipitation  and sedimentation technology to remove metals  and
solids  from combined wastewaters and to control pH  and  sulfide
precipitation preliminary treatment.  Lime and settle  technology
is   inplace at the one discharger in this  subcategory.   Sulfide
precipitation  is  necessary  to ensure  that  large  amounts  of
arsenic  present  in the raw wastes are removed  to  the  desired
level.

Implementation  of  the BPT limitations will remove  annually  an
estimated  17,522  kg  of  priority  metals  and  26,156  kg   of
pollutants including TSS from the current discharge.  We  project
a  capital cost of approximately $196,350 and an annualized  cost
of approximately $554,180 for achieving BPT.

More stringent technology option were not selected for BPT  since
they  require in-process changes or end-of-pipe technologies less
widely practiced in the subcategory,  and,  therefore,  are  more
appropriately considered under BAT.

PRIMARY BERYLLIUM

The   technology  basis  for  the  BPT  limitations  is  chemical
precipitation  and sedimentation technology to remove metals  and
solids  from combined wastewaters and to control pH and  fluoride
along with scrubber liquor recycle, and cyanide precipitation and
ammonia steam stripping preliminary treatment.   Lime and  settle
technology  is  already  in place at the one  discharger  in  the
subcategory.

Implementation  of BPT limitations will remove an estimated 2,698
kg/yr of priority metal pollutants and cyanide,  69,943 kg/yr  of
ammonia,  and  131,734 kg/yr of pollutants including TSS from the
raw  wastewater.   We  project  $226,500  in  capital  costs  and
$211,200 in annual costs for achieving promulgated BPT.

PRIMARY AND SECONDARY GERMANIUM AND GALLIUM

The  technology  basis  for  the  BPT  limitations  is   chemical
precipitation  and  sedimentation  technology to  remove  metals,
fluoride, and solids from combined wastewaters and to control pH.
The  pollutants specifically included for regulation at  BPT  are
arsenic, lead, zinc, fluoride, TSS, and pH.                    "

Although  there  are  no  existing  direct  dischargers  in  this
subcategory,  BPT is promulgated for any existing zero discharger
that  elects  to  discharge at some point in  the  future.    This
action  is  necessary  because  wastewaters   from  germanium  and,
gallium operations which contain significant loadings of priority
pollutants are currently being disposed of in a RCRA -  permitted
surface impoundment.

More stringent technology options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies less
widely practiced in the subcategory,  and,   therefore,   are  more
appropriately considered under BAT.
                               375

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
The  cost and specific removal data for this subcategory are  not
presented here because the data on which they are based have been
claimed to be confidential.

PRIMARY MOLYBDENUM AND RHENIUM

The   technology  basis  for  the  BPT  limitations  is  chemical
precipitation  and sedimentation technology to remove metals  and
solids from combined wastewaters and to control pH,  and  ammonia
steam  stripping and iron co-precipitation preliminary treatment.
All  to  these  technologies  except  iron  co-precipitation  are
already   in-place  at  one  to  the  two  dischargers   in   the
subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated  73,644  kg to priority metals,  737 kg of  molybdenum,
63,443  kg  of  ammonia, and 51,529 kg of TSS  from  the  current
discharge.  While one discharging plant has the equipment inplace
to  comply  with BPT, we do not believe that plant  is  currently
achieving  the  BPT  mass limitations.  The cost  data  for  this
subcategory are not presented here because the data on which they
are based have been claimed to be confidential.

More stringent technology options were not selected for BPT since
they require in-process changes or end-of-pipe technologies  less
widely  practiced in the subcategory,  and,  therefore,  are more
appropriately considered under BAT.

SECONDARY MOLYBDENUM AND VANADIUM

The  technology  basis  for  the  BPT  limitations  is  iron  co-
precipitation,    chemical  , precipitation   and    sedimentation
technology  to remove metals and solids from combined wastewaters
and to control pH,  and air stripping to remove ammonia.   Except
for  iron  co-precipitation,  these technologies are  already  in
place at the one discharger -in the subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated  319 kg of  priority metals and cyanide,  18,477 kg  of
molybdenum,  563,160 kg of ammonia, and 28,136 kg of TSS from the
raw  waste load.   Although the one discharging facility in  this
subcategory  has  some of the technology in place to comply  with
BPT,  we do not believe that the plant is currently achieving the
BPT mass limitations.  The cost data for this subcategory are not
presented here because the data on which they are based have been
claimed to be confidential.

More stringent technology options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies  not
practiced   at   the  one  plant  in  the   subcategory.    These
technologies   must,   therefore,  be  transferred   from   other
subcategories  where  the technologies have been defined  as  BAT
rather than BPT.
                               376

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
PRIMARY NICKEL AND COBALT

The  technology  basis  for  the  BPT  limitations  is   chemical
precipitation  and sedimentation technology to remove metals  and
solids  from combined wastewaters and to control pH, and  ammonia
steam  stripping to remove ammonia.  Chemical  precipitation  and
sedimentation technology is already inplace at the one discharger
in the subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated  241  kg  of  priority  metals  and  252  kg  of  total
pollutants from the current discharge.  While the one discharging
plant  has the equipment  inplace to comply with BPT, we  do* not
believe  that  the  plant is currently  achieving  the  BPT  mass
limitations.   The  cost  data  for  this  subcategory  are   not
presented here because the data on which they are based have been
claimed to be confidential.

More  stringent  technology  options were not  selected  for  BPT
since    they   require   in-process   changes   or   end-of-pipe
technologies  not practiced at the one plant in the  subcategory.
These technologies must,  therefore,  be transferred from  other
subcategories  where  the technologies have been defined  as  BAT
rather than BPT.

PRIMARY PRECIOUS METALS AND MERCURY

The  technology  basis  for  the  BPT  limitations  is   chemical
precipitation,  sedimentation  and  ion  exchange  technology  to
remove metals and solids from combined wastewaters and to control
pH,  and oil skimming to remove oil and grease.  Lime and  settle
technology is in place at the one discharger in this subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated  50,442  kg of priority metals and 53,768 kg  of  total
pollutants including TSS from the raw waste load.   We project  a
capital  cost  of  $2,200 and an annualized cost of  $26,814  for
achieving proposed BPT limitations.

More stringent technology options were not selected for BPT since
they require in-process changes or end-of-pipe technologies  less
widely  practiced in the subcategory,  and,  therefore,  are more
appropriately considered under BAT.

SECONDARY PRECIOUS METALS

The  technology  basis  for  the  ,BPT  limitations  is   chemical
precipitation,  sedimentation  and  ion  exchange  technology  to
remove  metals  and  solids  from  combined  wastewaters  and  to
control  pH,  ammonia  steam  stripping  pretreatment  to  remove
ammonia,  and cyanide precipitation pretreatment to  remove  free
and complexed cyanide.  Chemical precipitation and  sedimentation
technology  is already in place at 20 of the dischargers  in  the
subcategory.  One  plant  has  cyanide  precipitation  in  place.
Although  ammonia steam stripping is not currently  practiced  by
                               377

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
any of the plants  in  this  subcategory, air stripping is practiced
at  one  plant and steam stripping  is demonstrated at  plants  in
other nonferrous metals manufacturing subcategories.

Some  of the plants in this subcategory have unusually high  zinc
levels.   For  those  plants,  costs were developed for  two-stage
precipitation  using  sulfide  polishing  as  the  second  stage.
Sulfide  controls  zinc to the desired levels and helps  overcome
complexation problems.  Sulfide costs were included in the economic
impact analysis.

Implementation  of the BPT limitations will remove  annually  an
estimated  94 kg of priority pollutants (which include 63  kg  of
cyanide),  and 4,677  of total pollutants, which include 494 kg of
ammonia,  and  2,946  kg of TSS from the current  discharge.   The
cost  and  specific   removal data for this  subcategory  are  not
presented here because the data on which they are based have been
claimed to be confidential.

More stringent technology  options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies less
widely practiced in the subcategory,  and,  therefore,  are  more
appropriately considered under BAT.

PRIMARY RARE EARTH METALS

EPA  has withdrawn the BPT limitations that were promulgated  for
the Primary Rare Earth Metals Subcategory on September 20,  1985.
These limitations  were withdrawn because EPA failed to adequately
address  the  sole  direct discharging plant's  comments  in  the
Administrative Record.   Therefore,  national BPT limitations are
not  available  for   this  subcategory,  and  applicable  plant's
effluent  limitations  will . need to be developed  by  the  local
permitting authority  through the NPDES program.

SECONDARY TANTALUM

The   technology   basis  for .the  BPT  limitations  is  chemical
precipitation  and sedimentation technology to remove metals  and
solids  from  combined  wastewaters and  to  control  pH.    These
technologies  are  already inplace  at three dischargers  in  the
subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated 26,268 kg of priority metals, 1,490 kg of tantalum, and
51,392  kg  of total pollutants including TSS  from  the  current
discharge.    The   cost  and  specific  removal  data   for   this
subcategory are not presented here because the data on which they
are based have been claimed to be confidential.

More stringent technology options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies  not
practiced by any of the three existing plants in the subcategory.
These  technologies must,   therefore,   be transferred from  other
subcategories  where  the technologies have been defined  as  BAT
                               378

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
rather than BPT.

SECONDARY TIN

The  .technology  basis  for  the  BPT  limitations  is   chemical
precipitation  and  sedimentation technology  to  remove  metals,
fluoride, and solids from combined wastewaters and to control pH,
with  preliminary treatment consisting of  cyanide  precipitation
for   certain  building  blocks.   Chemical   precipitation   and
sedimentation technology is already inplace  at two of the  three
direct dischargers in the subcategory.

Implementation  of the BPT limitations will remove annually  from
raw discharge an estimated 688 kg of priority metals,  144 kg  of
cyanide,  237,220  kg of fluoride,  and 506,900 kg of TSS,  for a
total pollutant removal of 800,967 kg.   Projected capital  costs
are estimated to be approximately $841,285 while annual costs are
estimated  to  be $692,625.   The Agency has determined that  the
pollutant  reduction benefits associated with  compliance  justify
the costs for this subcategory.

More stringent technology options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies less
widely 'practiced in the subcategory,  and,  therefore,  are  more
appropriately considered under BAT.

PRIMARY AND SECONDARY TITANIUM

The   technology  basis  for  the  BPT  limitations  is  chemical
precipitation  and sedimentation technology to remove metals  and
solids  from  combined wastewaters and to  control  pH,  and  oil
skimming   preliminary  treatment  for  streams  with   treatable
concentrations of oil and grease.  These technologies are already
in  place  at  two  of  the   four  direct  dischargers  in   the
subcategory.   The pollutants specifically regulated at  BPT  are
chromium, lead, nickel, titanium, oil and grease, TSS, and pH. We
have  exempted from regulation facilities which do  not  practice
electrolytic  ,. recovery  of  magnesium  and  which   use   vacuum
distillation  instead of leaching to purify titanium  sponge.  We
are promulgating these regulations for all other titanium  plants
and the two-tiered regulation as proposed is not promulgated. '

Implementation  of  the BPT limitations will remove  annually  an
estimated  217 kg of priority metals,  5,791 kg of titanium,  and
64,446 kg of TSS from the raw waste load.   While two plants have
the  equipment  in place  to comply with BPT, we do  not  believe
that the plants are currently achieving the BPT limitations.   We
project  a  capital  cost  of $644,500  and  annualized  cost  of
$505,300 for achieving the BPT limitations.

More stringent technology options were not selected for BPT since
they require in-process changes or end-of-pipe technologies  less
widely  practiced in the subcategory,  and,  therefore,  are more
appropriately considered under BAT.
                               379

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
SECONDARY TUNGSTEN AND COBALT

The  technology  basis  for  the  BPT  limitations  is   chemical
precipitation  and sedimentation technology to remove metals  and
solids from combined wastewaters and to control pHr ammonia steam
stripping  to remove ammonia and oil skimming to remove  oil  and
grease.  Chemical precipitation and sedimentation  technology  is
already inplace at three direct dischargers in the subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated 150,600 kg of priority metals,  108,700 kg of TSS,  and
420,200 of total pollutants from the current discharge.  The cost
and  specific removal data for this subcategory are not presented
here  because the data on which they are based have been  claimed
to be confidential.

More stringent technology options were not selected for BPT since;
they require in-process changes or end-of-pipe technologies  less
widely  practiced in the subcategory,  and,  therefore,  are more
appropriately considered under BAT.

SECONDARY URANIUM

The  technology  basis  for  the  BPT  limitations  is   chemical
precipitation  and sedimentation technology to remove metals  and
solids  from  combined wastewaters and to control  pH.   Chemical
precipitation  and sedimentation technology is already  in  place
at the one discharger in the subcategory.

Implementation  of  the BPT limitations will remove  annually  an
estimated  100  kg  of  priority metals and  5,034  kg  of  total-
pollutants  including 651 kg of TSS from the estimated raw  waste
load. While the one discharging plant has the  equipment in place
to comply with BPT, we do not believe that the plant is currently
achieving  the  BPT limitations.  We project capital  and  annual
costs  of $54,800 and $90,400 (1982 dollars),  respectively,  for
modifications to technology presently in-place at the discharging
facility to achieve BPT regulations.

More stringent technology options were not selected for BPT since
they  require in-process changes or end-of-pipe technologies  not
practiced  by  any  of  the plants  in  the  subcategory.   These
technologies   must,   therefore,  be  transferred   from   other
subcategories  where  the technologies have been defined  as  BAT
rather than BPT.
PRIMARY ZIRCONIUM AND HAFNIUM

The  technology  basis  for the BPT  limitations  is  recycle  of
scrubber   liquors,   chemical  precipitation  and  sedimentation
technology to remove metals and solids from combined  wastewaters
and  to  control  pH,  plus ammonia steam stripping  and  cyanide
precipitation preliminary treatment to streams containing ammonia
                               380

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
and cyanide.  Chemical precipitation and sedimentation technology
and ammonia steam stripping is already in-place at one discharger
in the subcategory.  The pollutants specifically regulated at BPT
are chromium,  cyanide,  lead,  nickel, ammonia, TSS, and pH.  We
are now exempting from national regulation facilities which  only
produce   zirconium  or  zirconium-nickel  alloys  by   magnesium
reduction  of  ZrO2-   These BPT limitations apply to  all  other
zirconium-hafnium facilities.

Implementation  of  the BPT limitations will remove  annually  an
estimated  14,110  kg of priority metals and  cyanide,  and  19.4
million  kg of pollutants, including 38,240 kg of TSS from the raw
waste load.  The cost data for this subcategory are not presented
here  because the data on which they are based have been  claimed
to be confidential.

More stringent technology options were not selected for BPT since
they require in-process changes or end-of-pipe technologies  less
widely  practiced in the subcategory,  and,  therefore,  are more
appropriately considered under BAT.

THE BUILDING BLOCK APPROACH IN DEVELOPING PERMITS

A  plant  is to receive a discharge allowance  for  a  particular
building  block only it it is actually operating that  particular
process.  In this way, the building block approach recognizes and
accommodates the fact that not all plants use identical steps  in
manufacturing  a  given metal.  However, the plant  need  not  be
discharging wastewater from the process to receive the allowance.
Thus,  for  example,  if  the  regulation  contains  a  discharge
allowance  for wet scrubber effluent and a particular  plant  has
dry  scrubbers, it cannot include a discharge allowance  for  wet
scrubbers  as  part of its aggregate limitation.   On  the  other
hand,  if  it  has wet scrubbers and  discharges  less  than  the
allowable  limit  or does not discharge from  the  scrubbers,  it
would  receive  the full regulatory allowance in  developing  the
permit.                   ,-,...••;      • :     ••

There  are  several  facilities within this  category  that  have
integrated  manufacturing  operations;  that  is,  they   combine
wastewater  from smelting and refining operations which are  part
of  this  point  source  category,  with  wastewater  from  other
manufacturing  operations which are not a part of this  category,
and  treat  the combined stream prior to  discharge.  For  direct
dischargers, this problem would be appraoached using the building
block  approach and and developing discharge allowances  for  the
additional  wastewater  streams from  other  applicable  effluent
limitations  and standards or, if such are not  available,  using
best professional judgment (BPJ). For indirect dischargers,  this
problem   would  be  approached  by  determining  the   discharge
allowances  for the nonferrous metals, manufacturing  segment  and
applying  the combined waste formula to1 determine  the  discharge
allowand  for  the entire wastewater stream  being  treated.  The
combined  wastewater  formula is presented in 40 CFR 403  and  is
specifically   intended  to  apply  .to  those  situations   where
                               18 Ir

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           GENERAL DEVELOPMENT DOCUMENT
SECT - IX
wastewaters   from   various  categories   or   non   categorical
wastewaters are comingled before treatment and discharge.

Additional discussion of the development of discharge  allowances
from  the mixed wastewaters within this category is presented  at
the end of Section X.

A  summary of the BPT limitations (and also BAT, NSPS,  PSES  and
PSNS)   is   presented  in  Section  II   of   each   supplement.
Additionally,  in each supplement, a table is presented  for  BPT
(also  for BAT, NSPS, PSES and PSNS) showing the levels at  which
all  of the pollutants found at treatable levels would have  been
regulated if the Agency had deemed it necessary or appropriate to
directly   limit  all  of  these  pollutants.   This   additional
information  is presented so it may be used by permit writers  as
the  Agency's  best  professional judgment  whenever  it  becomes
necessary  or  desirable  to set limitations  on  the  additional
pollutants.
                               382

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GENERAL DEVELOPMENT DOCUMENT    SECT - IX


























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-------
                GENERAL  DEVELOPMENT DOCUMENT
                                                                  SECT  -   IX
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-------
          GENERAL DEVELOPMENT DOCUMENT
  SECT - IX
                          Table IX-2

              BPT REGULATED POLLUTANT PARAMETERS
Subcategory

Primary Lead




Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Secondary Lead
Pollutant Parameters

122.  lead
128.  zinc
      TSS
      PH

122.  lead
128.  zinc
      ammonia (N)
      TSS
      PH

122.  lead
128.  zinc
      ammonia (N)
      fluoride
      TSS
      pH

120.  copper
128.  zinc
      ammonia (N)
      TSS
      PH

114.  antimony
115.  arsenic
122.  lead
128.  zinc
      ammonia (N)
      TSS
      pH
Primary Antimony
Primary Beryllium
114.  antimony
115.  arsenic
123.  mercury
      TSS
      pH

117.  beryllium
119.  chromium (total)
120.  copper
121.  cyanide
      ammonia (as N)
      fluoride
      TSS
      pH
                              386

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          GENERAL DEVELOPMENT DOCUMENT
       SECT - IX
                    Table IX-2 (Continued)

              BPT REGULATED POLLUTANT PARAMETERS
  Subcategory

Primary and Secondary Germanium
and Gallium
Primary Molybdenum and Rhenium
Secondary Molybdenum and Vanadium
Primary Nickel and Cobalt
Primary Precious Metals and Mercury
Pollutant Parameters

    115.  arsenic
    122.  lead
    128.  zinc
          fluoride
          TSS
          pH

    115.  arsenic
    122.  lead
    124.  nickel
    125.  selenium
          fluoride
          molybdenum
          ammonia (as N)
          TSS
          pH

    115.  arsenic
    119.  chromium
    122.  lead
    124.  nickel
          molybdenum
          ammonia (as N)
          iron
          TSS
          pH
   120.  copper
   124.  nickel
         cobalt
         ammonia  (as .N)
         TSS
         pH

   122.  lead
   123.  mercury
   126.  silver
   128.  zinc
         gold
         oil and  grease
         TSS
         pH
                               387

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           GENERAL  DEVELOPMENT  DOCUMENT
     SECT  -  IX
                     Table  IX-2  (Continued)

               BPT REGULATED POLLUTANT PARAMETERS
 Subcategory
Pollutant Parameters
 Secondary Precious Metals
Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin
Primary and Secondary Titanium
120.  copper
121.  cyanide
128.  zinc
      ammonia  (as N)
      gold
      palladium
      platinum
      TSS
      PH

119.  chromium (Total)
122.  lead
124.  nickel
      TSS
      pH

120.  copper
122.  lead
124.  nickel
128.  zinc
      tantalum
      TSS
      pH

115.  arsenic
121.  cyanide
122.  lead
      iron
      tin
      fluoride
      TSS
      pH

119.  chromium (total)
122.  lead
124.  nickel
      titanium
      oil and grease
      TSS
      pH
                              388

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          GENERAL DEVELOPMENT DOCUMENT
    SECT - IX
                    Table IX-2 (Continued)

              BPT REGULATED POLLUTANT PARAMETERS
Subcategory
Pollutant Parameters
Secondary Tungsten and Cobalt
Secondary Uranium
Primary Zirconium and Hafnium
120.  copper
124.  nickel
      cobalt
      tungsten
      oil and grease
      ammonia (as N)
      TSS
      PH

119.  chromium (total)
120.  copper
124.  nickel
      fluoride
      TSS
      pH

119.  chromium (total)
121.  cyanide (total)
122.  lead
124.  nickel
      ammonia (as N)
      TSS
      pH
                              389

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GENERAL DEVELOPMENT DOCUMENT    SECT - IX
    THIS PAGE INTENTIONALLY LEFT BLANK
                    390

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
                            SECTION X

       EFFLUENT QUALITY ATTAINABLE THROUGH APPLICATION OF
      THE BEST AVAILABLE TECHNOLOGY ECONOMICALLY ACHIEVABLE
This  section  sets  forth the  effluent  limitations  attainable
through the application of best available technology economically
achievable  (BAT).   It  also serves to  summarize  changes  from
previous  rulemakings  in  the  nonferrous  metals  manufacturing
category,  and presents the development and use of the mass-based
effluent limitations.

A  number of factors guide the BAT analysis including the age  of
equipment  and  facilities  involved,  the  processes   employed,
process   changes,   non-water  quality   environmental   impacts
(including energy requirements), and the costs of application  of
such  technology.  BAT technology represents the  best  available
techndlogy  economically  achievable at plants of  various  ages,
sizes,  processes,  or other characteristics.   BAT  may  include
process  changes  or internal controls, even when these  are  not
common   industry  practice.   This  level  of  technology   also
considers  those  plant  processes  and  control  and   treatment
technologies  which,  at  pilot  plant  and  other  levels,  have
demonstrated   both   technological  performance   and   economic
viability at a level sufficient to justify investigation.

The  required assessment of BAT "considers" costs,  but does  not
require  a balancing of costs against effluent reduction benefits
(see Weyerhaeuser v.  Costle,  11 ERC 2149 (D.C. Cir. 1978)).  In
developing  the proposed and promulgated BAT,  however,  EPA  has
given  substantial  weight to the economic achievability  of  the
technology.   The Agency has considered the volume and nature  of
discharges  expected  after  application  of  BAT,   the  general
environmental  effects  of  the pollutants,  and  the  costs  and
economic impacts of the required pollution control levels.

The  BAT  effluent limitations are organized by  subcategory  for
individual sources of wastewater.  The limitations were developed
based  on  the attainable effluent concentrations and  production
normalized  flows  that  have been presented  in  this  document.
Implementation  of  the BAT effluent limitations is  expected  to
remove  1,968,000  kg/yr  of  priority  pollutants  from  current
discharge.   The  estimated capital cost of BAT is $28.4  million
(1982  dollars),  and the estimated annual cost is $22.7  million
(1982 dollars).

TECHNICAL APPROACH TO .BAT

In  the past,   the technical approach for the  nonferrous  metals
manufacturing  category considered each plant as a single  waste-
water  source,  without  specific  regard to the  different  unit
processes  that  are used in plants within the  same  subcategory.
For  this rulemaking,  end-of-pipe treatment technologies and in-
process  controls  were  examined in the selection  of  the  best
                               391

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           GENERAL DEVELOPMENT DOCUMENT
                            SECT - X
available technology.   After examining in-process  controls,  it
became   apparent  that  it  was  best  to   establish   effluent
limitations and standards recognizing specific wastewater streams
associated with specific manufacturing operations.  The  approach
adopted for this rule considers the individual wastewater sources
within  a plant, resulting in more effective pollution  abatement
by  tailoring the regulation to reflect these various  wastewater
sources. This approach, known as the building block approach, was
presented  in  Section IX.  Another example to this  approach  is
given at the end of this section.
INDUSTRY  COST  AND POLLUTANT REDUCTION BENEFITS OF
TREATMENT OPTIONS
                                      THE  VARIOUS
Under these guidelines, four treatment 'options were evaluated  in
selection  of  BAT  for the category.   Because  of  the  diverse
processes and raw materials used in the nonferrous category,  the
pollutant  parameters  found  in various waste  streams  are  not
uniform.    This  required  the  identification  of   significant
pollutants  in  the  various waste streams  so  that  appropriate
treatment technologies could be selected for further  evaluation.
The  options  considered  applicable  to  the  nonferrous  metals
manufacturing subcategories are presented in Table X-l (page   ).
A  thorough discussion of the treatment  technologies  considered
applicable   to   wastewaters   from   the   nonferrous    metals
manufacturing  category  is  presented in  Section  VII  of  this
document.  In Section VII, the attainable effluent concentrations
of  each  technology  are  presented  along  with  their  uniform
applicability  to all subcategories.  Mass limitations  developed
from  these options may vary, however, because of the  impact  of
different production normalized wastewater discharge flows.

In summary,  the treatment technologies considered for nonferrous
metals manufacturing are:

Option A is based on:

Chemical precipitation of metals followed by sedimentation,  and,
where  required,  cyanide precipitation,  sulfide  precipitation,
iron  co-precipitation,  ammonia air or steam stripping and  oil
skimming  pretreatment,  with ion-exchange end-of-pipe treatment.
(This  option
based.)
is equivalent to the technology on  which  BPT  is
Option B is based on:

Option  A (chemical precipitation and sedimentation with  cyanide
precipitation,   sulfide  precipitation,  iron  co-precipitation,
ammonia  air or steam stripping,  and oil skimming  pretreatment,
with  ion  exchange  end-of-pipe  treatment  where  needed)  plus
process wastewater flow reduction by the following methods:

  - Contact  cooling  water  recycle through  cooling towers.
  - Holding  tanks  for all other process  wastewater subject
                               392

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            GENERAL DEVELOPMENT DOCUMENT
SECT - X
     to recycle.

 Option C is based on:

 Option  B (chemical  precipitation and  sedimentation with  cyanide
 precipitation,    sulfide  precipitation,   iron  co-precipitation,
 ammonia  air or  steam  stripping,   and  oil  skimming   pretreatment,
 with ion exchange end-of-pipe  treatment where  needed,  preceded by
 in-process  flow  reduction),  plus  multimedia  filtration.

 Option E is based on:

 Option  C  (chemical precipitation,  sedimentation   with  cyanide
 precipitation,    sulfide  precipitation,   iron  co-precipitation,
 ammonia  air or  steam  stripping,   and  oil  skimming   pretreatment,
 with ion exchange end-of-  pipe  treatment where needed, in-pr
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           GENERAL DEVELOPMENT DOCUMENT
SECT
X
The first step in the calculation of the removal estimates is the
calculation  of  production normalized raw waste values  (mg/kkg)
for  each pollutant in each waste stream.   The raw waste,  values
were  calculated  using one of three  methods.   When  analytical
concentration data (mg/1) and sampled production normalized  flow
values   (1/kkg)  were  available  for  a  given  waste   stream,
individual  raw waste values for each sample were calculated  and
averaged.    This   method  allows  for  the  retention  of   any
relationship  between concentration,  flow and production.   When
sampled  production  normalized flows were not  available  for  a
given  waste stream,  an average concentration was calculated for
each pollutant,  and the average production normalized flow taken
from  the  dcp  information for that waste  stream  was  used  to
calculate  the  raw  waste.   When  analytical  values  were  not
available  for a given waste stream,  the raw waste values for  a
strJam of similar water quality was used.

The  total  flow (1/yr) for each option for each subcategory  was
calculated  by the following three steps:  first,  comparing  the
actual  discharge to the regulatory flow for each  waste  stream;
second,  selecting  the  smaller of the two  values;  and _third,
summing  the  smaller  flow values for each waste stream  in  the
subcategory  for each option.   The regulatory flow  values  were
calculated  by  multiplying the total production associated  with
each   waste  stream  in  each  subcategory    (kkg/yr)   by   the
appropriate  production  normalized flow (1/kkg) for  each  waste
stream for each option.

The  raw  waste  mass values  (kg/yr) for each pollutant  in  each
subcategory  were  calculated  by summing  individual  raw  waste
masses for each waste stream  in the subcategory.   The individual
raw  waste mass values were calculated by multiplying  the  total
production  associated with each waste stream  in each subcategory
(kkg/yr)  by the raw waste value  (mg/kkg) for  each  pollutant  in
each waste stream.

The  mass  discharged  (kg/yr) for each pollutant for each  option
for each subcategory was calculated by multiplying the total flow
(1/yr)   for  those  waste  streams  which  enter   the   central
pretreatment system, by  the treatment effectiveness concentration
(mg/1)   (Table  VII-21   page  xxx)  for   each   pollutant   for  the
appropriate option.

The total mass  removed  (kg/yr)  for  each  pollutant for each option
for each subcategory was calculated by subtracting the total mass
discharged  (kg/yr)  from  the total raw mass  (kg/yr).

Total  treatment  performance values for  each  subcategory  were
calculated  by  using the total  production  (kkg/yr) of all  plants
in the subcategory  for  each waste stream.   Treatment performance
values for direct dischargers in  each subcategory were calculated
by using  the  total production  (kkg/yr)  of all direct dischargers
in the subcategory  for  each waste stream.

MODIFICATION OF EXISTING BAT  EFFLUENT LIMITATIONS
                                394

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
Modifications  were promulgated to all existing  promulgated  BAT
effluent  limitations  in  the  nonferrous  metals  manufacturing
category.  In general, the existing BAT effluent limitations have
been  modified  to incorporate the building  block  approach.   A
detailed discussion regarding the development of mass limitations
from   this   approach  is  presented  in  Section   IX.    Other
modifications to the primary lead subcategory, secondary aluminum
subcategory,  primary  zinc subcategory, and  metallurgical  acid
plants  subcategory  were  made as a result  of  new  information
supplied to the Agency.

To  reflect the changes in stormwater allowances promulgated  for
BPT   in  the  primary  copper  smelting  and  secondary   copper
subcategories,  the  Agency is promulgating modifications to  the
stormwater  allowances promulgated under  BAT.   The  promulgated
changes   allow   a  discharge  resulting  from  a   catastrophic
rainstorm,  but  they  eliminate the  monthly  net  precipitation
discharge   allowance.    The  building  block  approach  is  not
developed for these two subcategories since they are required  to
maintain zero discharge of all process wastewater pollutants.

The technology basis for BAT has been modified, in most cases  to
be    lime precipitation, sedimentation and  filtration.  Sulfide
precipitation  is also included as the technology basis  for  the
primary  lead,  primary  zinc,  and  metallurgical  acid   plants
subcategories  and  for  one primary copper  plant.   The  Agency
believes   this   represents  the   best   available   technology
economically  achievable.

Allowances for Net Precipitation in Bauxite Refining

Promulgated  BPT  and BAT limitations for  the  bauxite  refining
subcategory  are  based  on  the use  of  settling  impoundments.
Facilities  in this subcategory are subject to a  zero  discharge
requirement;  however,  during  any  month they can  discharge  a
volume  of  water equal to the difference  between  precipitation
that  falls  within  the impoundment and  evaporation  from  that
impoundment for that month (net precipitation).

We  are  promulgating  minor technical amendments  to  delete  or
correct  references  to  PDF considerations under  Part  125  and
pretreatment  references  to Part 128.   We are not altering  the
existing BAT (promulgated on April 8,  1974 under Subpart A to 40
CFR Part 421) which prohibits the discharge of process wastewater
except  for an allowance for net precipitation that falls"  within
process wastewater impoundments.
                               395

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
Primary Aluminum Smelting

The   previous  BAT  effluent  limitations  were   developed   by
considering  each  plant  as  a  single  wastewater  source   and
allocating one discharge rate from which the effluent limitations
were calculated.  The technology basis from which these  effluent
limitations  were  developed  are  lime  and  settle  performance
values.  The modified BAT effluent limitations were developed for
individual  wastewater  sources  identified  within  the  primary
aluminum subcategory, and effluent concentrations attainable with
lime   precipitation,  sedimentation,  filtration,  and   cyanide
precipitation.  This technology is discussed in greater detail in
the BAT option selection of this section.

Secondary Aluminum Smelting

The  previously promulgated BAT for this  subcategory  prohibited
the  discharge of process wastewater.  However,  new  information
supports  the  need  for discharge of  wastewater  from  chlorine
demagging,   an   operation  considered  and  included   in   the
promulgated  zero  discharge  regulation.   Three  dry  processes
existed  at  the time of promulgation: the  Durham  process;  the
Alcoa process; and the Teller process.  The Agency believed  that
each of these processes were sufficiently well demonstrated to be
installed and become operational by 1984, the compliance date for
BAT.   Consequently, there was no justification for  a  discharge
allowance associated with this waste stream.

New  information shows that the technologies are not sufficiently
demonstrated  nor are they applicable to plants on  a  nationwide
basis.   For this reason,  the promulgated BAT has been modified;
the modified BAT is based on the use of wet scrubbing on chlorine
demagging operations.

Information  received  through  comments  on  the  1983  proposed
regulation  and through data requests shows a need for  discharge
of water from ingot conveyer casting*  A discharge allowance will
be  provided, but is intended only for those plants that  do  not
practice chlorine demagging wet air pollution control.   Complete
reuse  of  ingot  conveyer  casting  contact  cooling  water   in
demagging wet air scrubber operations is demonstrated.

Comments  and  information received in response to  dcp  requests
subsequent  to  the  1983  proposal also  show  the  need  for  a
discharge  allowance  for  wet  scrubbers  used  in  delacquering
operations, where paint and lacquers are burned from the  surface
of aluminum can scrap.  The promulgated BAT effluent  limitations
include this waste stream, which was not considered nor  included
in the 1974 BAT regulation.

Primary Electrolytic Copper Refining

The   previous  BAT  effluent  limitations  were   developed   by
considering  each  plant  as  a  single  wastewater  source   and
allocating one discharge rate from which the effluent limitations
                               396

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
were calculated.  The technology basis was lime precipitation and
sedimentation  performance  values.  The  modified  BAT  effluent
limitations  were  developed for  individual  wastewater  sources
identified  within  the  primary  electrolytic  copper   refining
subcategory,  and  effluent concentrations attainable  with  lime
precipitation,  sedimentation,  in-process  flow  reduction,  and
multimedia  filtration.  This technology is discussed in  greater
detail in the BAT option selection of this section.

Primary Lead

With  the  exception of stormwater exemptions, the  previous  BAT
effluent  limitations  required  zero discharge  of  all  process
wastewater pollutants.  Before proposing modified limitations  in
1983, information supplied to the Agency showed that slag removed
from the smelting furnace may contain recoverable  concentrations
of  lead.   For  the smelter slag to be recycled  back  into  the
production  process,  it  must  be  granulated  so  that  it   is
compatible with concentrated ore.  The Agency has determined that
this waste stream requires a discharge to control the build-up of
suspended solids.

However,  in  the  final rule,  EPA has moved the  proposed  flow
allowance   for   blast  furnace  slag   granulation   to   dross
reverberatory   slag  granulation.    The  Agency  changed   this
allowance  so that a plant that achieves zero discharge of  blast
furnace  slag granulation would not receive a discharge allowance
that is not needed.

Primary Zinc

The  previous  BAT effluent limitations were developed  from  one
wastewater discharge rate and lime and settle performance values.
The   modified  BAT  effluent  limitations  were  developed   for
individual wastewater sources identified within the primary  zinc
subcategory,  and  effluent concentrations attainable  with  lime
precipitation,   sedimentation,   sulfide   precipitation    (and
sedimentation),   in-process  flow  reduction,   and   multimedia
filtration.   This technology is discussed in greater  detail  in
the BAT option selection of this section.

Metallurgical Acid Plants

As  discussed in Section IX,  the metallurgical acid plants  sub-
category has been modified to include acid plants associated with
primary lead and zinc smelters,  and primary molybdenum roasters.
This  is  based  on the similarity between  discharge  rates  and
effluent  characteristics of wastewaters from  all  metallurgical
acid   plants.    The  Agency  is  also   establishing   effluent
limitations  for fluoride and molybdenum in discharges from  acid
plants  associated  with  primary  molybdenum  operations.     The
existing  BAT limitations are based on the BPT  technology  (lime
precipitation    and   sedimentation),   in-process    wastewater
reduction,  with  sulfide  precipitation,  iron  co-precipitation
preliminary treatment and filtration.  Flow reductions are  based
                               397

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
on 90 percent recycle of scrubber liquor.

Compliance  with the BAT limitations for the  metallurgical  acid
plants   subcategory  by  the  two  direct  discharging   primary
molybdenum  facilities  which operate sulfuric acid  plants  will
result in the annual removal of an estimated 4,651 kg of priority
pollutants  which is 219 kg of priority pollutants  greater  than
the  estimated  BPT  removed and 67,539 kg  of  total  pollutants
including molybdenum.

The costs for this subcategory are not presented here because the
data   on  which  they  are  based  have  been  claimed   to   be
confidential.  The Agency has determined that BAT limitations for
this  subcategory  are  technically  feasible  and   economically
achievable.

MODIFIED APPROACH TO STORMWATER

For  the  same  reasons discussed in detail  in  Section  IX,  no
allowance will be given for stormwater under BAT.   Stormwater is
or can be segregated from the process  wastewater.   Furthermore,
stormwater  is site-specific and is best addressed on a  case-by-
case  basis by the permit writer.   Should a sufficient number of
plants demonstrate that segregation of stormwater would result in
excessive  costs or is not technically feasible,  or  demonstrate
that  contamination of stormwater with process pollutants  is  an
unavoidable  result of manufacturing processes,  the Agency  will
consider   modification   of   the  promulgated   regulation   as
appropriate.

The  BAT  regulations  on  catastrophic  and  net   precipitation
exemptions are modified for several subcategories.  These changes
are presented in Table X-2 (page xxx).  The reasons for modifying
the  BAT relief provisions for primary copper  smelting,  primary
copper electrolytic refining,  secondary copper and primary  lead
are as follows:

     1.   The  technology . basis  for BAT has been  changed  from
          wastewater  impoundments to equipment such  as  holding
          tanks,  cooling towers,  and clarifiers.   This type of
          equipment  is  not  influenced to the  same  degree  as
          cooling impoundments.  As a result, storm relief is not
          necessary   to  treat  process  wastewater  (with   the
          exception noted in (2) below).

     2.   For  primary  copper  smelting  and  secondary  copper,
          impoundments  to  treat cooling water are used at  many
          facilities  as an alternative to cooling  towers.   EPA
          has  thus  provided that stormwater may  be  discharged
          from these impoundments when a 25-year,  24-hour  storm
          or  larger has been experienced by the  facility.   The
          volume  of  water that may be discharged is  only  that
          which   falls  directly  on  the  impoundment  surface.
          Further,  since  the  size required for  cooling  water
          impoundments is substantially smaller than impoundments
                               398

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
          that   treat   other  process   wastewaters,   no   net
          precipitation  relief  is  necessary.   The  amount  of
          freeboard available in the proper design and  operation
          of  these  cooling water ponds is sufficient  for  most
          facilities  to  accommodate the fluctuations in  volume
          resulting  from the precipitation cycle without  having
          to discharge.
BAT OPTION SELECTION

The option generally selected throughout the category is Option C
-   chemical   precipitation,  sedimentation,   in-process   flow
reduction,  and  multimedia  filtration,  along  with  applicable
pretreatment,  including ammonia air or steam stripping,  cyanide
precipitation, sulfide precipitation, iron co-precipitation,  and
oil   skimming   pretreatment,  and  ion   exchange   end-of-pipe
treatment. The Agency has selected BPT plus in-process wastewater
flow reduction and the use of filtration as an effluent polishing
step  as  BAT  for  all of  the  subcategories  except  secondary
aluminum, which includes preliminary treatment of phenolics  with
activated  carbon adsorption, where applicable, and  primary  and
secondary  germanium and gallium, where BAT is based on lime  and
settle.

This  combination  of treatment technologies  has  been  selected
because they are technically feasible and are demonstrated within
the nonferrous metals manufacturing category.   Implementation of
this treatment scheme would result in the removal of an estimated
1,968,000  kg/yr  of priority pollutants from  current  discharge
estimates.   Although the Agency is not required to  balance  the
costs  against effluent reduction benefits (see  Weyerhaeuser  v.
Costle,  supra), the Agency has given substantial weight  to  the
reasonableness  of cost.  The Agency's current economic  analysis
shows   that  this  combination  of  treatment  technologies   is
economically  achievable.   Price increases are not  expected  to
exceed 2.5 percent for any subcategory.

Of   the  36  subcategories  considered  in   nonferrous   metals
manufacturing,  EPA has reserved setting BAT limitations for  the
following three subcategories:

1.  Secondary Indium
2.  Secondary Mercury
3.  Secondary Nickel

As  discussed earlier,  EPA has excluded the following five  sub-
categories  from limitations under the provisions of Paragraph  8
of the Settlement Agreement:

1.  Primary Boron
2.  Primary Cesium and Rubidium
3.  Primary Lithium
4.  Primary Magnesium
5.  Secondary Zinc
                               399

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           GENERAL DEVELOPMENT DOCUMENT
                                SECT - X
BAT Effluent limitations have been promulgated for the  following
28 subcategories:

  1.  Bauxite Refining
  2.  Primary Aluminum Smelting
  3.  Secondary Aluminum Smelting
  4.  Primary Copper Smelting
  5.  Primary Electrolytic Copper Refining
  6.  Secondary Copper
  7.  Primary Lead
  8.  Primary Zinc
  9.  Metallurgical Acid Plants
 10.  Primary Tungsten
 11.  Primary Columbium-Tantalum
 12.  Secondary Silver
 13.  Secondary Lead
 14.  Primary Antimony
 15.  Primary Beryllium
 16.  Primary and Secondary Germanium and Gallium
 17.  Primary Molybdenum and Rhenium
 18.  Secondary Molybdenum and Vanadium
 19.  Primary Nickel and Cobalt
 20.  Primary Precious Metals and Mercury
 21.  Secondary Precious Metals
 22.  Primary Rare Earth Metals
 23.  Secondary Tantalum
 24.  Secondary Tin
 25.  Primary and Secondary Titanium
 26.  Secondary Tungsten and Cobalt
 27.  Secondary Uranium
 28.  Primary Zirconium and Hafnium

The  general  approach taken by the Agency for BAT regulation  of
this category and the BAT option selected for each subcategory is
presented  in this section.  The actual limitations may be  found
in Section II of each subcategory suppliment.

After   publication   of  the  nonferrous  metals   manufacturing
regulations/  some  petitioners challenged the promulgated  rule.
EPA  developed  settlement  agreements based  on  somw  of  these
petitions.   The  results  of  these  settlement  agreements  are
discussed in the pertinent subcategory supplements.

In  the regulatory sections of each subcategory  supplement,  the
pollutants
regulatory
pollutants
pollutants
pollutants
presented
discharge
pollutants
  considered  for  regulation  are  included  in   the
 tables  for  that subcategory.  Only  some  of  these
 were  selected  for  regulation  and  the   regulated
 are  indicated with an asterisk in  each  table.  The
 found  at  treatable levels  but  not  regulated  are
to  assist the permit writer by advising  him  of  the
allowance  that  would have  been  assigned  if  these
had been regulated.
                               400

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           GENERAL DEVELOPMENT DOCUMENT
SECT «- X
Primary Aluminum Smelting

The  BAT option selected is flow reduction,  lime  precipitation,
sedimentation,  and  filtration for control of toxic  metals  and
fluoride, and cyanide precipitation preliminary treatment.

This  combination of treatment technologies was selected  because
it  provides  additional  pollutant  removal  achievable  by  the
primary  aluminum subcategory and it is economically  achievable.
Lime  precipitation  and sedimentation are  widely  practiced  at
primary  aluminum  plants,  and  as  indicated  in  the  previous
section,  form  the  basis for the BPT  limitations.   Filtration
serves  as  an  important  polishing  step  in  BAT.    For  this
subcategory,  it results in the removal of 271,350 kg/yr of toxic
pollutants and 5,231,000 kg/yr of nonconventional pollutants from
the  estimated raw discharge.   Further,  lime precipitation  and
sedimentation  are demonstrated at 11 primary aluminum  smelters,
while  filtration is demonstrated at 23 plants in the  nonferrous
metals manufacturing category including one plant in the  primary
aluminum  subcategory.   The estimated capital investment cost of
BAT  is $16 million (1982 dollars) and the annual cost  is  $10.5
million.

Cyanide   precipitation  preliminary  treatment  is  directed  at
control  of free and complexed cyanides in waste  streams  within
the primary aluminum subcategory that result from use of coke and
pitch in the electrolytic reduction process.  These waste streams
collectively  discharge  approximately 62,000 kg/yr  of  cyanide.
The  Agency  conducted a pilot-scale treatment performance  study
for   cyanide   precipitation  on  wastewater  from   a   cathode
reprocessing  operation,  the only primary aluminum operation  to
generate cyanide.   The treatment effectiveness concentration for
cyanide  achieved  from  this study is the  basis  for  the  mass
limitation.   The  mean  was also shown,  in data submitted by  a
primary  aluminum  facility,  to be achievable  by  ion  exchange
technology  applied  to  cyanide-contaminated  groundwater.    In
developing   variability   factors  for   'cyanide   precipitation
technology,  EPA  will continue, to use the mean variability  from
the  combined metals data base because only two data points  were
generated by the treatability study.

Flow  reduction is an important element of BAT because it results
in  reduced dilution of pollutants and smaller  hydraulic  flows,
which in turn lead to more efficient treatment, smaller treatment
systems,   and  an  associated  reduction  in  the  net  cost  of
treatment.   Wastewater  flow  reduction  is based  on  increased
recycle of scrubber liquor from potline,  potline SO2  emissions,
potroom, and anode bake scrubbers, in addition to casting contact
cooling water.

Secondary Aluminum Smelting

The   BAT  effluent  limitations  for  the   secondary   aluminum
subcategory  are  based  on  lime  precipitation,  sedimentation,
filtration,   ammonia  steam  stripping,   and  activated  carbon
                               401

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            GENERAL DEVELOPMENT DOCUMENT
SECT - X
 adsorption.    Ammonia  steam stripping is selected by the  Agency
 over   air  stripping  because  air   stripping  reduces    ammonia
 concentrations  by simply transferring pollutants  from one  media
 (water)   to   another   (air).    Steam  stripping   reduces   ammonia
 concentrations  by stripping  the ammonia from   wastewater  with
 steam.   The  ammonia is  concentrated  in the steam phase and may be
 condensed,  collected,   and sold as  a by-product or disposed off-
 site.   Ammonia steam  stripping is demonstrated by  five facilities
 in the  nonferrous  metals manufacturing category.   Filtration  is
 not demonstrated in the secondary aluminum subcategory;   however,
 it   is   demonstrated  in  the  nonferrous  metals  manufacturing
 category.

 Activated carbon adsorption preliminary treatment  to remove 4-AAP
 phenols    applies   to  plants  discharging  scrubber  water  from
 delacquering furnace  operations (an  operation  that removes  paint
 and other surface  coatings from aluminum scrap).

 Application   of the promulgated BAT  will result  in the removal of
 9,590 kg/yr  of toxic  pollutants,  526 kg/yr of  phenols, and 90,300
 ^9/Yr   °f aluminum  from  the  estimated  raw  discharge.     The
 estimated capital  investment  cost of the promulgated BAT  is  $1.1
 million   (1982  dollars)  and  the  estimated annual  cost is  $0.64
 million.

 Primary  Copper Electrolytic Refining

 The BAT  effluent limitations for  Primary Copper  Electrolytic
 Refining  are based on  in-process flow reduction and  end-of-pipe
 treatment    technology    consisting    of   lime     precipitation,
 sedimentation,   and multimedia filtration.   Sulfide precipitation
 is  added  for one  integrated  copper  refiner and  smelter based  on
 the demonstrated inability of this plant to meet the arsenic mass
 limitations  with lime and settle  technology.   The  Agency  believes
 that  the   mass   limitations are   achievable    using    sulfide
 precipitation  based  on bench-scale performance tests using  the
•plant's   wastewater.    Filtration is not  demonstrated   in  this
 subcategory,   but   it  is transferred from the primary  aluminum.,
 secondary  copper,  primary zinc, primary lead,  secondary lead,  and
 secondary  silver subcategories.

 Application   of the promulgated BAT  will result  in the removal of
 48,700    kg/yr   of toxic  pollutants  from the  estimated   raw
 discharge.     The   estimated   capital  investment   cost   of   the
 promulgated   BAT is $2.7  million  (1982  dollars)  and the estimated
 annual cost  is  $1.7 million.

 Primary  Lead

 The effluent  limitations  for  the primary  lead  subcategory  are
 based on  the  existing BPT with additional  reduction in  pollutant
 discharge  achieved through  in-process wastewater flow reduction,
 sulfide precipitation technology, and the  use  of filtration as an
 effluent   polishing step.   Wastewater  flow  reduction is based   on
 the complete recycle of  process  wastewater  from zinc fuming  wet
                               402

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
air  pollution control, blast furnace slag granulation, and  hard
lead  refining  wet air pollution control.   Extensive  treatment
performance  data  submitted to the Agency from  a  well-operated
plant  in this subcategory indicate that, for this facility,  the
proposed  BAT  mass  limitations are not  achievable  with  lime,
settle and filter technology.  The principal reason for not being
able  to attain the proposed effluent limits is the inability  to
achieve  the  combined metals data base lime, settle  and  filter
concentration  values.   The specific technical factors  in  this
failure could not be determined from the data submitted. However,
the  Agency  believes the addition of sulfide  precipitation,  in
conjunction   with  multimedia  filtration,  will   achieve   the
treatment effectiveness values because of the lower solubility of
metal  sulfides  (i.e., lower than metal hydroxides) as  well  as
performance  data for sulfide technology obtained  from  treating
nonferrous  metals and inorganic chemical  wastewaters.   Sulfide
precipitation  is currently demonstrated at a primary  molybdenum
plant with a metallurgical acid plant, and at a cadmium plant  in
the   primary   zinc,  subcategory.    Filtration   is   currently
demonstrated by one facility in the primary lead subcategory.

Application of the promulgated BAT will result in the removal  of
734  kg/yr  of toxic pollutants over the estimated  BPT  removal.
The primary lead subcategory is estimated to incur a capital cost
of  $0.2  million  (1982  dollars) and an annual  cost  of  $0.11
million  to  implement  the BAT technology.

Primary Zinc

The BAT effluent limitations for the primary zinc subcategory are
based  on  BPT with additional reduction in  pollutant  discharge
achieved  through in-process wastewater flow  reduction,  sulfide
precipitation  technology,  and  the  use  of  filtration  as  an
effluent  polishing step.  Wastewater flow reduction is based  on
increased  recycle of casting scrubber water and casting  contact
cooling  water.   As discussed above, sulfide  precipitation  and
filtration  is  added  to ensure achievability  of  the  combined
metals data base treatment effectiveness,, concentration values for
lime,  settle  and filter technology.  Sulfide  precipitation  is
currently  demonstrated  at a cadmium plant in the  primary  zinc
subcategory,   and   at  a  primary  molybdenum  plant   with   a
metallurgical  acid plant.  Filtration is currently in  place  at
one  of the three direct discharging plants in the  primary  zinc
subcategory.

Application of the promulgated BAT effluent mass limitations will
result in the removal of 1,159,000 kg/yr of toxic pollutants from
the  estimated raw discharge.   The estimated capital  investment
cost  of the promulgated BAT is $0.46 million (1982 dollars)  and
the  estimated annual cost is $0.24 million.   Activated  alumina
and  reverse  osmosis  were  also considered  for  BAT  but  were
rejected.    These  technologies  are  not  demonstrated  in  the
category, nor are they clearly transferable.
                               403

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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - X
Metallurgical Acid Plants

The   BAT  effluent limitations  for metallurgical acid plants  are
based on  BPT with additional  reduction  in  pollutant  discharge
achieved  through in-process wastewater flow   reduction,  sulfide
precipitation  technology,  and the  use  of  filtration  as  an
effluent  polishing step.  Wastewater flow reduction is based  on
increased  recycle of acid plant scrubber liquor.   As  discussed
above,  sulfide precipitation and filtration is added  to  ensure
achievability   of  the  combined  metals  data  base   treatment
effectiveness  concentration values for lime,  settle  and  filter
technology. Sulfide precipitation is currently demonstrated at  a
cadmium  plant in the primary zinc subcategory, and at a  primary
molybdenum plant with a metallurgical acid plant.  Filtration  is
currently  demonstrated  at two of the seven   direct  discharging
plants in the metallurgical acid plants subcategory.

Application  of the promulgated BAT mass  limitations will  result
in  the  removal  of 136,800 kg/yr of toxic pollutants  from  the
estimated raw discharge.   The  estimated  capital investment  cost
of  BAT  is $1.97 million (1982 dollars) and the annual  cost  is
$1.24 million.

Filtration, option C, was selected instead of  option B because it
is  demonstrated and results in removal of 7,590 kg/yr  of  toxic
pollutants.

Primary Tungsten

The  BAT  limitations  for the  primary tungsten  subcategory  are
based  on  BPT with additional  reduction in  pollutant  discharge
achieved through in-process wastewater flow reduction and the use
of  filtration as an effluent polishing  step.   Wastewater  flow
reduction  is  based on 90 percent recycle of  scrubber  liquors.
Filtration   is  currently  demonstrated  at   23  plants  in  the
category.

Application ,of the promulgated  BAT will remove an estimated 5,140
kg/yr  °f  toxic pollutants,  which is 318 kg/yr of toxic  metals
over the estimated BPT removal.  No additional ammonia is removed
at  BAT,  nor  are any toxic  organics  removed.  -The  estimated
capital  investment  cost of BAT is $0.77 million (1982  dollars)
and the estimated annual cost is $1.0 million.

Primary Columbium-Tantalum

The   BAT   limitations  for    the   primary   columbium-tantalum
subcategory  are  based  on  BPT  with  additional  reduction  in
pollutant  discharge achieved through in-process wastewater  flow
reduction  and  the  use of filtration as an  effluent  polishing
step.   Wastewater flow reduction is based on increased recycle of
scrubber  liquors  associated with  three  sources:    concentrate
digestion   scrubber,     solvent   extraction    scrubber,     and
precipitation scrubber.    Filtration is currently demonstrated at
23 nonferrous metals manufacturing plants.
                               404

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
Application of the promulgated BAT will result in the removal  of
283  kg/yr of toxic pollutants and 1,980 kg/yr of nonconventional
pollutants over the estimated BPT removal.  The estimated capital
investment  cost of BAT is $0.83 million (1982 dollars)  and  the
estimated annual cost is $1.2 million.

Filtration, option C, was selected instead of option B because it
is  demonstrated  and  results in removal of 57  kg/yr  of  toxic
pollutants and 94 kg/yr of nonconventional pollutants.

Secondary Silver

The  BAT  limitations  for the secondary silver  subcategory  are
based  on  BPT with additional reduction in  pollutant  discharge
through  in-process  wastewater  flow reduction and  the  use  of
filtration  as  an  effluent  polishing  step.   Wastewater  flow
reduction is based on complete recycle of furnace scrubber water.
Filtration  is currently demonstrated at two of the seven  direct
discharging secondary silver plants.

Application of the promulgated BAT will result in the removal  of
132  kg/yr  of toxic pollutants over the estimated  BPT  removal.
The  estimated capital investment cost of the promulgated BAT  is
$0.28  million  (1982  dollars)  and the  annual  cost  is  $0.39
million.

Filtration, option C, was selected instead of option B because it
is  demonstrated  and results in removal of 132  kg/yr  of  toxic
pollutants.

Secondary Lead

The BAT limitations for the secondary lead subcategory are  based
on  BPT with additional reduction in pollutant discharge  through
in-process wastewater flow reduction and the use of filtration as
an  effluent polishing step.   Wastewater flow reduction is based
on  90  percent  recycle of casting . contact  cooling  water  and
complete  recycle  of  facility washdown water and  battery  case
classification wastewater.   Filtration is currently demonstrated
at  one  of eight direct discharging secondary  lead  plants  and
seven plants in this subcategory.

Application of the promulgated BAT will result in the removal  of
350  kg/yr  of toxic pollutants over the estimated  BPT  removal.
The estimated capital investment cost of this technology is $1.86
million,  (1982  dollars) and the estimated annual cost is  $1.24
million.


Primary Antimony

The  BAT  limitations  for the primary antimony  subcategory  are
based  on  chemical precipitation and sedimentation  and  sulfide
precipitation  preliminary  treatment (BPT technology)  with  the
                               405

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
addition of filtration.

The  pollutants  specifically  limited under  BAT  are  antimony,
arsenic,  and mercury.   The priority pollutants cadmium, copper,
lead,  and  zinc were also considered for regulation because they
were  found  at treatable concentrations in the  raw  wastewaters
from  this subcategory.   These pollutants were not selected  for
specific regulation because they will be effectively  controlled
when  the  regulated  priority metals are treated to  the  levels
achievable by the model BAT technology.

Implementation  of the BAT limitations would remove  annually  an
estimated  18  kg  of  priority metals  over  the  estimated  BPT
discharge.  Estimated capital cost for achieving BAT is $208,300,
and annualized cost is $560,400.

Primary Beryllium

The  BAT  limitations for the primary beryllium  subcategory  are
based  on  chemical precipitation and sedimentation  preceded  by
scrubber  liquor  recycle,  ammonia steam stripping  and  cyanide
precipitation (BPT technology),  with the addition of  filtration
and  scrubber water recycle. Flow reduction is based  on  greater
than 90 percent recycle of beryllium oxide calcining furnace  wet
air  pollution  control.   The  one  beryllium  plant   currently
generating  beryllium oxide calcining furnace wet  air  pollution
control wastewater does practice recycle.

The  pollutants  specifically limited under  BAT  are  beryllium,
chromium, copper, cyanide, ammonia, and fluoride.

Implementation  of the BAT limitations would remove  annually  an
estimated  8 kg of priority metals and 0.5 kg of cyanide over the
estimated BPT discharge.  No additional ammonia is removed.

The  costs and specific removal data for this subcategory are not
presented here because the data on which they are based has  been
claimed to be confidential.

Primary and Secondary Germanium and Gallium

The  BAT limitations for the primary and secondary germanium  and
gallium  subcategory  are  based on  chemical  precipitation  and
sedimentation (BPT technology).

The pollutants specifically limited under BAT are arsenic,  lead,
zinc,  and fluoride.   The priority pollutants antimony, cadmium,
chromium, copper, nickel, selenium, silver and thallium were also
considered  for regulation because they were found  at  treatable
concentrations  in  the  raw wastewaters from  this  subcategory.
These  pollutants  were  not " selected  for  specific  regulation
because  they will be effectively controlled when  the  regulated
priority  metals are treated to the concentrations achievable  by
the  model •" BAT  technology.    EPA is including  limitations  for
gallium and germanium as guidance for permitting authorities.
                               406

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
Although  there  are  no  existing  direct  dischargers  in  this
subcategory, BAT is promulgated for any existing zero  discharger
who elects to discharge at some point in the future.  This action
was  necessary  because wastewaters from  germanium  and  gallium
operations   which  contain  significant  loadings  of   priority
pollutants  are currently being disposed of in a  RCRA  permitted
surface impoundment.

The costs and specific removal data for this subcategory are  not
presented  here because the data on which they are based has been
claimed to be confidential.

Primary Molybdenum and Rhenium

The  BAT  limitations  for  the primary  molybdenum  and  rhenium
subcategory  are  based on preliminary  treatment  consisting  to
ammonia  steam stripping, iron co-precipitation, and  end-of-pipe
treatment consisting of chemical precipitation and  sedimentation
(BPT technology), with the addition of in-process wastewater flow
reduction  and  filtration.   Flow reductions  are  based  on  90
percent recycle of scrubber liquor, a rate demonstrated by one of
the two direct discharger plants.

The pollutants specifically limited under BAT are arsenic,  lead,
molybdenum,   nickel,  selenium,  fluoride,  and  ammonia.    The
priority   pollutants  chromium,  copper,  and  zinc  were   also
considered  for regulation because they were found  at  treatable
concentrations  in  the raw wastewaters  from  this  subcategory.
These  pollutants  were  not  selected  for  specific  regulation
because  they will be effectively controlled when  the  regulated
priority metals are treated to the levels achievable by the model
BAT technology.

Implementation  of the BAT limitations would remove  annually  an
estimated 11 kg of priority metals greater than the estimated BPT
removal.  No additional ammonia is removed at BAT.

The  costs and specific removal data for this subcategory are not
presented here because the data on which they are based has  been
claimed to be confidential.

Secondary Molybdenum and Vanadium

The  BAT  limitations for the secondary molybdenum  and  vanadium
subcategory  are  based .on preliminary  treatment  consisting  of
ammonia   air   stripping  followed  by   end-of-pipe   treatment
consisting  of iron co-precipitation, chemical precipitation  and
sedimentation (BPT technology) and filtration.

The  pollutants  specifically  limited  under . BAT  are  arsenic,
chromium,  lead,  molybdenum,  nickel, iron,  and  ammonia.   The
priority  pollutants antimony, beryllium, cadmium, and zinc  were
also  considered  for  regulation  because  they  were  found  at
treatable  concentrations  in  the  raw  wastewaters  from   this
                               407

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            GENERAL DEVELOPMENT DOCUMENT
SECT - X
 subcategory.   These   pollutants  were  not   selected   for   specific
 regulation  because  they  will  be effectively  controlled  when   the
 regulated   priority   metals  are treated   to   the   concentrations
 achievable  by  the   model   BAT   technology.    EPA   is   providing
 limitations   for  the  following  pollutants  as   guidance    for
 permitting  authorities:  copper,  zinc,  aluminum,  boron,   cobalt,
 germanium,  manganese, tin, titanium,  and  vanadium.

 Implementation  of   the BAT  limitations would remove annually   an
 estimated 76  kg  of priority  metals  greater  than the estimated  BPT
 removal.

 The  costs and specific removal data for this  subcategory  are   not
 presented   here  because the  data  on which they  are  based  has been
 claimed to  be confidential.

 Primary Nickel and Cobalt

 The  BAT limitations  for the  primary nickel  and  cobalt subcategory
 are  based  on preliminary treatment consisting  of   ammonia  steam
 stripping   followed by  end-of-pipe   treatment  consisting    of
 chemical    precipitation and sedimentation  (BPT technology),   and
 filtration.    A  filter is presently utilized  by the one plant   in
 this subcategory.

 The pollutants specifically  limited under BAT are cobalt, copper,
 nickel,  and   ammonia.   The priority   pollutant  zinc  was  also
 considered  for  regulation  because  it was   found  at  treatable
 concentrations  in   the raw  wastewaters   from   this  subcategory.
 This  pollutant  was  not selected  for  specific regulation  because
 it  will  be  effectively controlled when  the  regulated  priority
 metals  are   treated to the  levels  achievable by  the  model   BAT
 technology.

 Implementation  of the BAT limitations would remove  annually   an
 estimated   5   kg of  toxic metals  greater  than the  estimated   BPT
 removal'.

 The  costs and specific removal data for  this subcategory are  not
 presented here because the data on  which  they are based has  been
 claimed to be  confidential.

 Primary Precious Metals and Mercury

 The  BAT limitations for the primary precious metals and  mercury
 subcategory  are based on preliminary treatment consisting of oil
 skimming   and  end-of-pipe  treatment  consisting  of   chemical
precipitation  and   sedimentation   (BPT  technology),   with  the
addition of in-process wastewater flow reduction,   filtration and
 ion-exchange.

The  pollutants specifically limited under BAT  are  gold,  lead,
mercury,  silver,  and zinc.   The  priority  pollutants  arsenic,
cadmium,   chromium,   copper,  nickel  and  thallium  were   also
considered  for regulation because they were found  at  treatable
                               408

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
concentrations  in  the raw wastewaters  from  this  subcategory.
These  pollutants  were  not  selected  for  specific  regulation
because  they will be effectively controlled when  the  regulated
priority metals are treated to the levels achievable by the model
BAT technology.                                                *

Implementation  of  the BAT limitations would remove annually  an
estimated  1.0 kg of priority metals greater than  the  estimated
BPT removal.  Estimated capital cost for achieving BAT is $3,025,
and annualized cost is $27/300.

Secondary Precious Metals

The BAT limitations for the secondary precious metals subcategory
are   based  on  preliminary  treatment  consisting  of   cyanide
precipitation   and  ammonia  steam  stripping  and   end-of-pipe
treatment consisting of chemical precipitation and  sedimentation
(BPT technology), with the addition of in-process wastewater flow
reduction,  filtration  and ion exchange.   Flow  reductions  are
based  on  recycle  of scrubber effluent. Twenty-one  of  the  29
existing  plants currently have scrubber liquor recycle rates  of
90  percent or greater.  A filter is also presently  utilized  by
one plant in the subcategory.

The  pollutants  specifically  limited  under  BAT  are   copper,
cyanide,  zinc,  ammonia,  gold, palladium,  and  platinum.   The
priority  pollutants antimony, arsenic, cadmium, chromium,  lead,
nickel,  selenium, silver and thallium were also  considered  for
regulation because they were found at treatable concentrations in
the raw wastewaters from this subcategory.  These pollutants were
not  selected  for  specific  regulation  because  they  will  be
effectively  controlled  when the regulated priority  metals  are
treated to the levels achievable by the model BAT technology.

Implementation  to the BAT limitations would remove  annually  an
estimated 10 kg of priority pollutants greater than the estimated
BPT removal.  No additional ammonia or cyanide is removed at BAT.

The costs and specific removal data for this subcategory are  not
presented  here because the data on which they are based has been
claimed to be confidential.
Primary Rare Earth Metals

The  BAT limitations that were promulgated for
earth  metals  subcategory  on  September  20,
withdrawn.   These  limitations were withdrawn
to   adequately  address  the  sole  plant's
Administrative Record.   Therefore,  national
not  available  for  this subcategory,  and a
manufacturing  plant's  effluent  limitations
developed  by  the local permitting authority
program.

Secondary Tantalum
    the  primary  rare
      1985  have  been
    because EPA failed
   comments   in   the
   BAT limitations are
    rare  earth  metal
    will  need  to  be
   through  the  NPDES
                               409

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
The  BAT limitations for the secondary tantalum  subcategory  are
based   on   chemical   precipitation  and   sedimentation    (BPT
technology) with the addition of filtration.

The pollutants specifically limited under BAT are  copper,  lead,
nickel,  zinc,  and tantalum.   The priority pollutants antimony,
beryllium, cadmium, chromium, and silver were also considered for
regulation because they were found at treatable concentrations in
the raw wastewaters from this subcategory.  These pollutants were
not  selected  for  specific  regulation  because  they  will  be
effectively  controlled  when the suggested priority  metals  are
treated to the levels achievable by the model BAT technology.

Implementation  of  the BAT limitations would remove annually  an
estimated  4.8  kg  of metal priority pollutants  more  than  the
estimated BPT removal.

The costs and specific removal data for this subcategory are not
presented here because the data on which they are based has  been
claimed to be confidential.

Secondary Tin

The  BAT limitations for the secondary tin subcategory are  based
on preliminary treatment consisting of cyanide precipitation when
required,   and  end-of-pipe  treatment  consisting  of  chemical
precipitation  and  sedimentation  (BPT  technology),   with  the
addition of filtration.

The  pollutants  specifically  limited  under  BAT  are  arsenic,
cyanide,  lead, iron, tin, and fluoride.  The priority pollutants
antimony,  cadmium,  chromium,  copper, nickel, selenium, silver,
thallium,  and  zinc were also considered for regulation  because
they  were  found at treatable concentrations in the  raw  waste-
waters from this subcategory.  These pollutants were not selected
for   specific  regulation  because  they  will  be   effectively
controlled when the regulated priority metals, are treated to  the
levels achievable by the model BAT technology.

Implementation  to the BAT limitations would remove  annually  an
estimated  26  kg  of  priority metals  over  the  estimated  BPT
discharge.  An additional 128 kg of fluoride is removed  annually
at BAT.  The costs and specific removal data for this subcategory
are  not presented here because the data on which they are  based
has been claimed to be confidential.

Primary and Secondary Titanium

EPA is exempting from limitations those titanium plants which  do
not  practice  electrolytic recovery of magnesium and  which  use
vacuum  distillation  instead  of  leaching  to  purify  titanium
sponge.   BAT  limitations are promulgated for all other titanium
plants' based on chemical precipitation,  sedimentation,  and  oil
skimming pretreatment where required (BPT technology),  plus flow
                               410

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
reduction and filtration.   Flow reduction is based on 90 percent
recycle of scrubber effluent through holding tanks and 90 percent
recycle of casting contact cooling water through cooling towers.

The pollutants specifically limited under BAT are chromium, lead,
nickel, and titanium.  The priority pollutants antimony, cadmium,
copper,  thallium,  and  zinc were also considered for regulation
because  they were found at treatable concentrations in  the  raw
wastewaters  from  this subcategory.   These pollutants were  not
selected for specific regulation because they will be effectively
controlled when the regulated priority metals are treated to  the
levels achievable by the model BAT technology.

Implementation  of the BAT limitations would remove  annually  an
estimated  299  kg  to  priority  pollutants  from  the   current
discharge.    Estimated  capital  cost  for  achieving   BAT   is
$1,030,000, and annualized cost is $585,000.

Secondary Tungsten and Cobalt

The  BAT  limitations  for  the  secondary  tungsten  and  cobalt
subcategory  are  based on preliminary  treatment  consisting  of
ammonia  steam  stripping  and  oil  skimming,   and  end-of-pipe
treatment  consisting of chemical precipitation and sedimentation
(BPT technology), plus filtration.

The pollutants specifically limited under BAT are cobalt, copper,
nickel,  tungsten, and ammonia.  The priority pollutants arsenic,
cadmium,  chromium,  lead,  silver, and zinc were also considered
for   regulation   because   they   were   found   at   treatable
concentrations  in  the raw wastewaters  from  this  subcategory.
These  pollutants  were  not  selected  for  specific  regulation
because  they will be effectively controlled when  the  regulated
priority metals are treated to the levels achievable by the model
BAT technology.

Implementation  of  the BAT limitations would remove annually  an
estimated  100 kg of priority., pollutants more than estimated  BPT
removal.

The costs and specific removal data for this subcategory are  not
presented  here because the data on which they are based has been
claimed to be confidential.

Secondary Uranium

The  BAT  limitations for the secondary uranium  subcategory  are
based   on   end-of-pipe   treatment   consisting   of   chemical
precipitation and sedimentation (BPT technology), and filtration.
Flow reduction of laundry wastewater is included in BAT.

The  pollutants  specifically  limited under  BAT  are  chromium,
copper, nickel, and fluoride.  The priority pollutants  antimony,
arsenic,   cadmium,  lead,  selenium,  silver,  zinc,   and   the
nonconventional  pollutant  uranium  were  also  considered   for
                               411

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            GENERAL  DEVELOPMENT  DOCUMENT
SECT - X
 regulation  because  they  were  found at  treatable concentrations  in
 the  raw wastewaters from the  subcategory.  These pollutants   were
 not   selected   for   specific   regulation  because   they  will  be
 effectively controlled   when the regulated priority  metals  are
 treated  to the  levels  achievable by  the model  BAT  technology.
 Guidance  is being  provided to permit  writers for  the control  of
 uranium.

 Implementation  of   the  BAT limitations would remove annually  an
 estimated  126  kg of priority metals from the current  discharge.
 Estimated  capital   cost for achieving  BAT  is   $88,000,   and
 annualized  cost is  $107,000 (1982 dollars).

 Primary Zirconium and Hafnium

 EPA  is  exempting  from limitations those plants which only produce
 zirconium  or   zirconium-nickel alloys by magnesium reduction  of
 ZrO2.   Limitations  apply to  all other plants in the subcategory.
 BAT  limitations are  based on  the same  flow allowances provided  at
 BPT   (cyanide precipitation,  ammonia steam stripping and chemical
 precipitation and sedimentation), plus in-process wastewater  flow
 reduction and filtration.

 The  pollutants  specifically limited under  BAT   are  chromium,
 cyanide,  lead,   nickel,  and ammonia.   The priority pollutants
 cadmium,  thallium,  zinc,  and  the   nonconventional  pollutants
 zirconium and hafnium were also considered for regulation because
 they  were  found at treatable concentrations in the  raw  waste-
 waters  from this  subcategory.   These pollutants were not selected
 for  specific   regulation because they will be  effectively   con-
 trolled  when   the  regulated  priority metals are treated  to  the
 levels  achievable by the model BAT technology.

 The costs and specific removal data for this subcategory are  not
 presented   here because  the data on which they are  based has  been
 claimed to  be confidential.

 REGULATED POLLUTANT PARAMETERS

 Presented   in   Section  VI  of this document is  a  list  of  the
 pollutant  parameters  found  at  concentrations  and  frequencies
 above     treatable    concentrations   that    warrant    further
 consideration.  Although these pollutants were found at  treatable
 concentrations, the Agency is not promulgating regulation of  each
 pollutant  selected  for further consideration.    The  high   cost
 associated  with  analysis  of  metal  priority  pollutants   has
 prompted EPA to develop an alternative method for regulating  and
monitoring toxic pollutant discharges from the nonferrous  metals
manufacturing category.   Rather than developing specific effluent
mass  limitations and standards for each of the  priority  metals
 found   in treatable concentrations in the raw wastewater  from  a
 given   subcategory,   the  Agency is  promulgating  effluent  mass
 limitations  only for those pollutants generated in the  greatest
quantities as shown by the pollutant reduction benefit analysis.
                               412

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           GENERAL DEVELOPMENT DOCUMENT
SECT - X
By  establishing  limitations  and standards  for  certain  metal
pollutants,  dischargers  will attain the same degree of  control
over metal pollutants as they would have been required to achieve
had  all  the  metal  pollutants  been  directly  limited.   This
approach   is   technically   justified   since   the   treatable
concentrations   achievable  with  chemical   precipitation   and
sedimentation  technology  are based on optimized  treatment  for
concomitant  multiple metals removal.  Thus, even though  metals
have  somewhat different theoretical solubilities, they  will  be
removed at very nearly the same rate in a chemical  precipitation
and  sedimentation treatment system operated for multiple  metals
removal.  Filtration as part of the technology basis is  likewise
justified   because   this   technology   removes   metals   non-
preferentially.

The  Agency  has excluded several toxic organic  pollutants  from
specific  regulation in the primary tungsten,  primary columbium-
tantalum,  and  secondary silver subcategories because they  were
found  in  trace (deminimus quantities) amounts and  are  neither
causing nor likely to cause toxic effects.

The  conventional pollutants oil and grease,  pH,  and  TSS  are
excluded  from  regulation in BAT.  They are  regulated  by  BCT.
Table  X-2  (page  416)  presents  the  pollutants  selected  for
specific  regulation  in BAT and Table X-3  (page  419)  presents
those pollutants that are effectively controlled by  technologies
upon  which are based other effluent limitations and  guidelines.
Table  X-4 (page 424) presents those pollutants excluded  because
they  are neither causing nor likely to cause toxic effects.    A
more  detailed  discussion  on the  selection  and  exclusion  of
priority  pollutants  is presented in Sections VI and X  of  each
subcategory supplement.

EXAMPLE OF THE BUILDING BLOCK APPROACH IN DEVELOPING PERMITS

That  there  is  a wide range  of  differences  in  manufacturing
facilities   has been emphasized by industry representatives  and
observed  by Agency personnel. This diversity of processes  makes
it  virtually  impossible to establish effluent  limitations  and
standards  on  a whole plant basis such that they  are  fair  and
achievable  for  industry and protective of the  environment.  To
better  accomplish these seemingly mutually exclusive goals,  the
Agency  has  adopted the building block  approach  to  developing
discharge limits for use in water discharge permits. The building
block approach allows the permit.writer to establish  appropriate
and  achievable  effluent  limits  for  any  discharge  point  by
combining   appropriate  limitations  based  upon   the   various
processes that contribute wastewater to the discharge point.

Each  building  block represents a single ,, process  or  discharge
stream  from  a  process  within, - the  subcategory.  Because   of
differences in manufacturing-processes, all'building blocks  will
not occur in every plant in a subcategory. Similarly, the  amount
of  material processed through any building block may  vary  from
plant  to plant both because of  the product output of  the  plant
                               413.

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           GENERAL DEVELOPMENT  DOCUMENT
                            SECT - X
and  the manufacturing processes  used. The building block approach
takes both of  these variables  into account; the first by allowing
the  selection of only  those building blocks that are in use  and
the  second by relating the quantity of pollutant allowed  to  be
discharged  to the materials processed or produced by a  building
block.  This   measure   of  production  is  called  a   production
normalizing  parameter  (PNP)  and is specific  to  each  building
block.

As   a  simplified  example, consider a  facility  which  produces
aluminum  from bauxite and   treats  the  wastewater  prior   to
discharge.   The facility in this example  discharges  wastewater
from potroom wet air pollution control and direct chill  casting.
Only a part of the aluminum reduced in the potroom is  processed
through the direct chill casting operation; the remainder is cast
into  sow  molds  and  generates  no  process   wastewater.   By
multiplying  the production for  each of these operations  by  the
limitations  or  standards  in 40 CFR 421  for  potroom  wet  air
pollution  control  and direct chill casting and by  summing  the
products  obtained  for each of  these waste streams,  the  permit
writer can obtain the allowable mass discharge.

The  permit writer must develop a quantification of the  PNP  for
each building  block so  that it is a reasonable representation  of
the  actual production level of the building block. The factors to
be   taken into account  in this quantification and the  procedures
for  calculating  the   reasonable representation  of  the  actual
production  have been reviewed in the development of 40 CFR  126.
The  permit  writer is  expected to take into  account  production
variations  in establishing a reasonable measure of  the  actual
production for use in the calculation of the discharge allowance.

If,  for  example, the  reasonable representation  of  the  actual
production associated with the potroom wet air pollution  control
system  is 550 kkg/day  and the reasonable representation  of  the
production  of  aluminum  through direct  chill  casting  is  410
kkg/day the maximum for any one day discharge limit based on  the
best  available technology economically achievable (BAT) for  the
pollutant nickel is 0.72486 kg/day as calculated below:

Potroom Wet Air Pollution Control

(550 kkg/day)   x (0.733 mg/kg)  x  (10~3mg/kg)
  =  0.42515 kg nickel, maximum for any one day

Direct Chill Casting

(410 kkg/day)   x (0.731 mg/kg)  x (10~3mg/kg)
  =  0.29971 kg nickel, maximum for any one day
Total
0.72486 kg nickel, maximum for any one day
                               414

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           GENERAL DEVELOPMENT DOCUMENT
      SECT - X
                            Table X-l

          OPTIONS CONSIDERED FOR EACH OF THE NONFERROUS
               METALS MANUFACTURING SUBCATEGORIES
   Subcategory

 Primary Aluminum Smelting
 Secondary Aluminum Smelting
 Primary Copper  Electrolytic
  Refining

 Primary Zinc
 Primary Lead
 Metallurgical Acid Plants

 Primary Tungsten
 Primary Columbium-Tantalum
 Secondary Silver

 Secondary Lead
 Primary Antimony
 Primary Beryllium
 Primary and Secondary
   Germanium and  Gallium

 Secondary Indium
 Secondary Mercury
 Primary Molybdenum and
   Rhenium

 Secondary Molybdenum and
   Vanadium
 Primary  Nickel and  Cobalt
 Secondary Nickel

 Primary  Precious  Metals and
   Mercury
 Secondary  Precious Metals
 Primary  Rare Earth Metals

 Secondary  Tantalum
 Secondary  Tin
 Primary and Secondary Titanium

 Secondary Tungsten and Cobalt
 Secondary Uranium
Primary Zirconium and Hafnium
Options Considered
                   E
                   X
A
X
X
X
X
X
X
X
X
X
X
X
x-*-
X
X
X
X
X
X
X
X
X
X
X,
X1
X
X
x
X1
B
X
X
X
X
X
X
X
X
X
X





X



X
X
X


X



c
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
                  X
Includes recycle of scrubber liquors as part of Option A.
                              415

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          GENERAL DEVELOPMENT DOCUMENT
SECT - X
                           Table X-2

              BAT REGULATED POLLUTANT PARAMETERS
     Subcategory

Primary Aluminum Smelting
Secondary Aluminum
Primary Electrolytic Copper
  Refining
Primary Lead


Primary Zinc




Metallurgical Acid Plants
Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Pollutant Parameters

 73.  benzo(a)pyrene
114.  antimony
121.  cyanide (total)
124.  nickel
      aluminum
      fluoride

122.  lead
128.  zinc
      aluminum
      ammonia (N)
      phenolics
       (total; by
        4-AAP method)

114.  arsenic
120.  copper
124.  nickel

122.  lead
128.  zinc

118.  cadmium
120.  copper
122.  lead
128.  zinc

115.  arsenic
118.  cadmium
120.  copper
122.  lead
128.  zinc

122.  lead
128.  zinc
      ammonia (N)

122.  lead
128.  zinc
      ammonia (N)
      fluoride

120.  copper
128.  zinc
      ammonia (N)
                               416

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            GENERAL  DEVELOPMENT DOCUMENT
    SECT - X
                      Table X-2  (Continued)

               BAT REGULATED POLLUTANT PARAMETERS
    Subcateqory

 Secondary Lead
 Primary Antimony
 Primary Beryllium
 Primary and Secondary Germanium
 and Gallium
 Primary Molybdenum  and Rhenium
Secondary Molybdenum and Vanadium
Primary Nickel and Cobalt
Primary Precious Metals and Mercury
Pollutant Parameters

    114.  antimony
    115.  arsenic
    122.  lead
    128.  zinc
          ammonia (N)
                      t
    114.  antimony
    115.  arsenic
    123.  mercury

    117.  beryllium
    119.  chromium (total)
    120.  copper
    121.  cyanide
          ammonia (as  N)
          fluoride

    115.  arsenic
    122.  lead
    128.   zinc
          fluoride

    115.   arsenic
    122.   lead
    124.   nickel
    125.   selenium
          fluoride
         molybdenum
         ammonia  (as N)

   115.  arsenic
   119.  chromium
   122.  lead
   124.  nickel
         molybdenum
         ammonia  (as N)
         iron

   120.. copper
   124.  nickel
         cobalt
         ammonia  (as N)

   122.  lead
   123.  mercury
   126.  silver
   128.  zinc
         gold
                              417

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r
                     GENERAL DEVELOPMENT DOCUMENT
  SECT - X
                                Table X-2 (Continued)

                         BAT REGULATED POLLUTANT PARAMETERS
               Subcategory

          Secondary Precious Metals
          Primary Rare Earth Metals
           Secondary Tantalum
           Secondary Tin
           Primary and Secondary  Titanium
           Secondary Tungsten and Cobalt
           Secondary Uranium
           Primary Zirconium and Hafnium
Pollutant Parameters

120.  copper
121.  cyanide
128.  zinc
      ammonia (as N)
      gold
      palladium
      platinum

  9.  hexachlorobenzene
119.  chromium (total)
122.  lead
124.  nickel

120.  copper
122.  lead
124.  nickel
128.  zinc
      tantalum

115.  arsenic
121.  cyanide
122.  lead
      iron
      tin
      fluoride

119.  chromium  (total)
122.  lead
124.  nickel
      titanium

120.  copper
124.  nickel
      cobalt
      tungsten
      ammonia  (as  N)

119.  chromium  (total)
120.  copper
124.  nickel
      fluoride

119.  chromium  (total)
121.  cyanide  (total)
122.  lead
124.  nickel
      ammonia  (as  N)
                                          418

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            GENERAL DEVELOPMENT DOCUMENT
          SECT - X
                             Table X-3

  PRIORITY POLLUTANTS EFFECTIVELY CONTROLLED BY TECHNOLOGIES UPON
     WHICH ARE BASED OTHER EFFLUENT LIMITATIONS AND GUIDELINES
      Subcategory

 Primary Aluminum Smelting
 Secondary Aluminum
 Primary Electrolytic
 Copper Refining
• Primary Lead
 Primary Zinc
Pollutant Parameters

  1.  acenaphthene
 39.  fluoranthene
 55.  naphthalene
 72.  benzo(a)anthracene
      (1,2-benzanthracene)
 76.  chrysene
 78.  anthracene (a)
 79.  benzo(ghi)perylene
      {1,11-benzoperylene)
 80.  fluorene
 81.  phenanthrene  (a)
 82.  dibenzo(a,h)anthracene
      (1,2,5,6-dibenzanthracene)
 84.  pyrene
115.  arsenic
116.  asbestos (Fibrous)
118.  cadmium
119.  chromium (Total)
120.  copper
122.  lead
125.  selenium
128.  zinc

(a)  Reported together.

 65.  phenol
118. ,cadmium

119.  chromium (Total)
122.  lead
126.  silver
128.  zinc

116.  asbestos (Fibrous)
118.  cadmium

115.  arsenic
116.  asbestos (Fibrous)
119.  chromium (Total)
124.  nickel
126.  silver
                                419

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           GENERAL DEVELOPMENT DOCUMENT
          SECT - X
                      Table X-3  (Continued)

     TOXIC POLLUTANTS EFFECTIVELY CONTROLLED BY TECHNOLOGIES
 UPON WHICH ARE BASED OTHER EFFLUENT LIMITATIONS AND GUIDELINES
     Subcategory

Metallurgical Acid Plants
Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Secondary Lead
Primary Antimony
Pollutants

114.  antimony
119.  chromium  (Total)
123.  mercury
124.  nickel
125.  selenium
126.  silver

118.  cadmium
119.  chromium  (Total)
124.  nickel
125.  silver
127.  thallium

114.  antimony
115.  arsenic
116.  asbestos  (Fibrous)
118.  cadmium
119.  chromium  (Total)
120.  copper
124.  nickel
125.  selenium
127.  thallium

114.  antimony
115.  arsenic
118.  cadmium
119.  chromium  (Total)
121.  cyanide
122.  lead
124.  nickel
125.  selenium
126.  silver
127.  thallium

118.  cadmium
119.  chromium  (Total)
120.  copper
124.  nickel
126.  silver
127.  thallium

118.  cadmium
120.  copper
128.  zinc
                               420

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           GENERAL DEVELOPMENT DOCUMENT
           SECT - X
                      Table X-3 (Continued)

     TOXIC POLLUTANTS EFFECTIVELY CONTROLLED BY TECHNOLOGIES
 UPON WHICH ARE BASED OTHER EFFLUENT LIMITATIONS AND GUIDELINES
     Subcategory
 Pollutants
Primary and Secondary Germanium  114.  antimony
and Gallium                      118.  cadmium
                                 119.  chromium
                                 120.  copper
                                 124.  nickel
                                 125.  selenium
                                 126.  silver
                                 127.  thallium

Primary Molybdenum and Rhenium   119.  chromium (total)
                                 120.  copper
                                 128.  zinc
Secondary Molybdenum and
Vanadium
Primary Nickel and Cobalt

Primary Precious Metals and
Mercury
114.
117.
118.
128.
Secondary Precious Metals
115.
118.
119.
120.
124.
127.

114.
115.
118.
119.
122.
124.
125.
126.
127.
      antimony
      beryllium
      cadmium
                                      zinc
128.  zinc
      arsenic
      cadmium
      chromium
      copper
      nickel
      thallium

      antimony
      arsenic
      cadmium
      chromium
      lead
      nickel
      selenium
      silver,
      thallium
                               421

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           GENERAL DEVELOPMENT DOCUMENT
           SECT - X
                      Table X-3 (Continued)

 PRIORITY POLLUTANTS EFFECTIVELY CONTROLLED BY TECHNOLOGIES UPON
    WHICH OTHER EFFLUENT LIMITATIONS AND GUIDELINES ARE BASED
     Subcategory

Primary Rare Earth Metals
Pollutant Parameters
Secondary Tantalum
Secondary Tin
Primary and Secondary
Titanium
Secondary Tungsten and
Cobalt
4.
115.
118.
120.
125.
126.
127.
128.
114.
117.
118.
119.
126.
114.
118.
119.
120.
124.
125.
126.
127.
128.
114.
118.
120.
128.
115.
118.
119.
124.
126.
128.
benzene
arsenic
cadmium
copper
selenium
silver
thallium
zinc
antimony
beryllium
cadmium
chromium (total)
silver
antimony
cadmium .
chromium
copper
nickel
selenium
silver
thallium
zinc
antimony
cadmium
copper
zinc
arsenic
cadmium
chromium
lead
silver
zinc
                               422

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           GENERAL DEVELOPMENT DOCUMENT
            SECT - X
                      Table X-3 (Continued)

 PRIORITY POLLUTANTS EFFECTIVELY CONTROLLED BY TECHNOLOGIES UPON
    WHICH OTHER EFFLUENT LIMITATIONS AND GUIDELINES ARE BASED
      Subcategory

Secondary Uranium
Pollutant Parameters
114.
115.
118.
122.
125.
126.
128.
antimony
arsenic
cadmium
lead
selenium
silver
zinc
Primary Zirconium and Hafnium  118.  cadmium
                               127.  thallium
                               128.  zinc
                               423

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           GENERAL DEVELOPMENT DOCUMENT
          SECT - X
                            Table X-4

       TOXIC POLLUTANTS DETECTED BUT ONLY IN TRACE AMOUNTS
    AND ARE NEITHER CAUSING NOR LIKELY TO CAUSE TOXIC EFFECTS
     Subcategory

Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
Pollutants

11.  Iflr1-trichloroethane
55.  naphthalene
65.  phenol
73.  benzo(a)pyrene
79.  benzo(ghi)perylene
82.  dibenzo(a,h)anthracene
85.  tetrachloroethylene
86.  toluene

 4.  benzene
 6.  carbon tetrachloride
 7.  chlorobenzene
 8.  lf2,4-trichlorobenzene
10.  1,2-dichloroethane
30.  1,2-trans-dichloroethylene
38.  ethylbenzene
51.  chlorodibromomethane
85.  tetrachloroethylene
87.  trichloroethylene

 4.  benzene
 6.  carbon tetrachloride
     (tetrachloroemethane)
10.  1,2-dichloroethane
11.  Iflf1-trichloroethane
29.  1,1-dichloroethylene
30.  1,2-trans-dichloroethylene
38.  ethylbenzene
84.  pyrene
85.  tetrachloroethylene
86.  toluene
87.  trichloroethylene
     total phenolics (by 4-AAP
       method)
                               424

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
                           SECTION XI

                NEW SOURCE PERFORMANCE STANDARDS
The  basis  for  new source performance  standards  (NSPS)  under
Section  306  of  the  Clean Water  Act  is  the  best  available
demonstrated  technology (BDT).   New plants have the  opportunity
to  design the best and most efficient production  processes  and
wastewater  treatment  technologies.   Therefore/  NSPS  includes
process  changes,  in-plant controls  (including  elimination  to
wastewater  discharges  for some  streams),  operating  procedure
changes,   and  end-of-pipe  treatment  technologies  to   reduce
pollution to the maximum extent possible.  This section describes
the  control  technology  for treatment of  wastewater  from  new
sources  and  presents mass discharge  limitations  of  regulated
pollutants for NSPS, based on the described control technology.

TECHNICAL APPROACH TO NSPS

All wastewater treatment technologies applicable to a new  source
in  the  nonferrous  metals  manufacturing  category  have   been
considered previously for the BAT options.  For this reason, four
options  were considered as the basis for NSPS, all identical  to
BAT options in Section X.  In summary, the treatment technologies
considered for nonferrous metals manufacturing new facilities are
outlined below:

Option A is based on:

     Chemical precipitation of metals followed by  sedimentation,
     and,  where required, ion exchange,  sulfide  precipitation,
     iron co-precipitation, cyanide precipitation, ammonia air or
     steam stripping,.and oil skimming.

Option B is based on:

     Option A plus process wastewater flow reduction by the
     following methods:

     Contact cooling water recycle through cooling
     towers.
     Holding tanks for all other process wastewater
     subject to recycle.

Option C is based on:

     Option B plus multimedia filtration.

Option E is based on:

     Option  C  plus activated carbon adsorption applied  to  the
     total plant discharge as a polishing step.
                               425

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           GENERAL DEVELOPMENT DOCUMENT
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The  options  listed above are general and can be applied to  all
subcategories.   Wastewater flow reduction within the  nonferrous
metals  manufacturing category is generally based on the  recycle
of   scrubbing  liquors  and  casting  contact   cooling   water.
Additional  flow reduction is achievable for new sources  through
alternative  process  methods  which  are   subcategory-specific.
Additional  flow  reduction attainable for  each  subcategory  is
discussed  later  in  this  section  regarding  the  NSPS  option
selection.

For  several subcategories,  the regulatory production normalized
flows  for NSPS are the same as the production  normalized  flows
for the selected BAT option.  The mass of pollutant allowed to be
discharged  per mass of product is calculated by multiplying  the
appropriate  treatment  effectiveness value (one-day maximum  and
10-day average values) (mg/1) by the production normalized  flows
(1/kkg).   When these calculations are performed,  the mass-based
NSPS   can  be  derived  for  the  selected   option.    Effluent
concentrations  attainable  by  the NSPS  treatment  options  are
identical  to  those presented in Section VII  of  this  document
(Table VII-21 page xxx).

MODIFICATIONS TO EXISTING NSPS

New source performance standards had been promulgated  previously
for  the primary and secondary aluminum  smelting  subcategories.
The technology basis for these standards was lime  precipitation,
sedimentation,   and   in-process  flow  reduction   of   process
wastewater.   EPA is promulgating modifications to these NSPS "to
incorporate changes promulgated for BAT and to include additional
flow  reductions possible at new sources in the primary  aluminum
subcategory.

As  discussed  in  Section  IX,  the  metallurgical  acid  plants
subcategory  has been modified to include acid plants  associated
with  primary  lead  and zinc smelters,  and - primary  molybdenum
roasters,.   This  is based on the  similarity  between  discharge
rates  and  effluent  characteristics  of  wastewaters  from  all
metallurgical acid plants.

NSPS OPTION SELECTION

In   general,  EPA  is  promulgating  that  the  best   available
demonstrated  technology  be equivalent to BAT  technology  (NSPS
Option C).  For the subcategories where EPA has reserved  setting
BAT  limitations,  chemical  precipitation,  sedimentation,   and
filtration  is  generally selected as the  technology  basis  for
NSPS.  The principal treatment method for Option C is  in-process
flow   reduction,  chemical  precipitation,  sedimentation,   and
multimedia  filtration.   Option C also  includes  ion  exchange,
sulfide   precipitation,   cyanide   precipitation,   iron    co-
precipitation, ammonia air or steam stripping, and oil  skimming,
where  required.   As  discussed  in Sections  IX  and  X,  these
technologies  are  currently  used at plants  within  this  point
                               426

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
source category.  The Agency recognizes that new sources have the
opportunity  to  implement  more advanced levels to treatment
without incurring the costs to retrofit equipment, and the  costs
of  partial  or  complete  shutdown  to  install  new  production
equipment.  Specifically the design of new plants can be based on
recycle of contact cooling water through cooling towers,  recycle
of  air pollution control scrubber liquor or the use of  dry  air
pollution   control   equipment.   New  plants  also   have   the
opportunity  to consider alternate degassing or slag  granulation
methods during the preliminary design of the facility.

The  data  relied upon for selection of NSPS were  primarily  the
data  developed  for existing sources which included costs  on  a
plant-by-plant  basis along with retrofit costs where applicable.
The Agency believes that compliance costs could be lower for  new
sources  than the cost estimates for equivalent existing sources,
because  production  processes can be designed on  the  basis  of
lower   flows  and  there  will  be  no  costs  associated   with
retrofitting  the  in-process controls.  Therefore,  new  sources
will have costs that are not greater than the costs that existing
sources  would incur in achieving equivalent pollutant  discharge
reduction.  Based on this analysis, the Agency believes that  the
selected NSPS (NSPS Option C) is an appropriate choice.

Section  II of each subcategory supplement presents a summary  of
the  NSPS  for the Nonferrous Metals Manufacturing  Point  Source
Category.   The  pollutants  selected  for  regulation  for  each
subcategory  are  identical to those selected for  BAT  with  the
addition of conventional pollutant parameters (e.g., TSS, oil and
grease,  and  pH).   The  pollutants  regulated  under  NSPS  are
presented  for  each  subcategory  in  Table  XI-1  (page   435).
Presented  below is a brief discussion describing the  technology
option selected for NSPS for each subcategory.

Primary Aluminum Smelting

New  source performance standards for primary aluminum are  based
on BAT plus additional flow reduction.  Additional flow reduction
is  achievable through the use of dry air pollution scrubbing  on
potlines,   anode  bake  plants,   and  anode  paste  plants  and
elimination   of  potroom  and  degassing  scrubber   discharges.
Potroom   scrubbing  discharges  are  eliminated  by  design   of
efficient   potline  scrubbing  (eliminating  potroom   scrubbing
completely)  or  100 percent recycle (with blowdown  recycled  to
casting).   Degassing scrubbers are limited by replacing chlorine
degassing with inert gases.

These  flow reductions are demonstrated at existing  plants,  but
are  not  included in BAT because they might involve  substantial
retrofit costs at other existing plants.  However, new plants can
include  these  reductions  in plant  design  at  no  significant
additional cost.

The  Agency  does  not  believe that the  promulgated  NSPS  will
provide  a  barrier  to  entry  for  new  facilities.   In  fact,
                               427

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
installation  of  dry scrubbing instead of wet scrubbing  in  new
facilities reduces the cost of end-of-pipe treatment by  reducing
the overall volume of wastewater discharged.

Secondary Aluminum Smelting

The  technology  basis  and  discharge allowances  for  NSPS  are
equivalent to that of the promulgated BAT,  with the exception of
dross  washing.   Dross  washing  is  not  provided  a  discharge
allowance in the NSPS because of the demonstration of dry milling
in  the subcategory.   Dry milling is not required  for  existing
sources  due  to  the  extensive  retrofit  costs  of  installing
milling,   grinding,  and  screening  operations.   However,  new
sources  have  the  opportunity  to install  the  best  equipment
without  the cost of major retrofits.   The Agency also does  not
believe  that  new  plants  could  achieve  any  additional  flow
reduction  for  chlorine demagging and  casting  contact  cooling
beyond that promulgated for BAT.

Primary Copper Smelting

The  promulgated NSPS for the primary copper smelting subcategory
is   zero   discharge  of  all  process  pollutants   without   a
catastrophic storm discharge allowance.  The Agency believes that
new  smelting facilities can be constructed using cooling  towers
to  cool and recirculate casting contact cooling water  and  slag
granulation   wastewater   instead  of   large   volume   cooling
impoundments.    This   technology  is   demonstrated   in   this
subcategory.   Thus, this modification eliminates  the  allowance
for the catastrophic precipitation discharge allowed at BAT.  The
costs  associated  with construction and operation of  a  cooling
tower system are not significantly greater than those for cooling
impoundments,   and  as  such,  the  Agency  believes  that   the
promulgated  NSPS will not constitute a barrier for entry of  new
facilities.   As a result of this modification, the discharge  of
toxic   metals  during  months  of  net  precipitation  will   be
eliminated.

Primary Electrolytic Copper Refining

The promulgated NSPS for the primary electrolytic copper refining
subcategory  are equivalent to promulgated BAT.   Review  of  the
subcategory    indicates   that   no   additional    demonstrated
technologies exist that improve on BAT.  The Agency also believes
that  new plants could not achieve any additional flow  reduction
beyond that promulgated for BAT.

Secondary Copper

New   source  performance  standards  for  the  secondary  copper
subcategory  are  promulgated as zero discharge  of  all  process
wastewater  pollutants.     It is believed that new sources can be
constructed   with   demonstrated   cooling   tower    technology
exclusively  and  that  the  cost of cooling  towers  instead  of
cooling impoundments is minimal.   This eliminates the  allowance
                               428

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
needed  for catastrophic stormwater provided at BAT.   Therefore,
NSPS,  as defined, does not constitute a barrier to entry for new
plants.

Primary Lead

The  promulgated  NSPS  prohibit the  discharge  of  all  process
wastewater  pollutants  from primary lead smelting  except  those
industrial  hygiene streams provided an allowance at BAT and  for
which   an  allowance  remains  necessary.    Zero  discharge  is
achievable through complete recycle and reuse of dross and  blast
furnace  slag  granulation  wastewater or through  slag  dumping.
Elimination  of  discharge  from  dross  or  blast  furnace  slag
granulation  is demonstrated in four of the six existing  plants,
but  it  is  not  included  at  BAT  because  it  would   involve
substantial  retrofit  costs for the one existing  discharger  by
requiring the installation of a modified sintering machine.   New
plants  can  include elimination of the discharge from  the  slag
granulation  process  in  the  plant  design  at  no  significant
additional  cost.   Elimination  of  the sinter  plant  materials
handling  wet air pollution control waste stream is based on  dry
scrubbing  to  control fugitive lead emissions  during  materials
handling.   Therefore, NSPS does not present any barrier to entry
for new plants.

Primary Zinc

New source performance standards for the primary zinc subcategory
are  promulgated  equal  to  BAT.    Review  of  the  subcategory
indicates  that  no  new  demonstrated  technologies  exist  that
improve on BAT.

Dry scrubbing is not demonstrated for controlling emissions  from
zinc  reduction furnaces,  leaching,  and product  casting.   The
nature of these emissions (acidic fumes,  hot particulate matter)
technically  precludes the use of dry  scrubbers.   Therefore,  a
discharge   allowance  is  included  from  this  source  at  NSPS
equivalent to that promulgated,, for BAT.  The Agency believes that
new plants could not achieve any additional flow reduction beyond
that promulgated for BAT.

Metallurgical Acid Plants

New  source  performance  standards for  the  metallurgical  acid
plants subcategory are promulgated equal to BAT.   Review of  the
subcategory indicates that no new demonstrated technologies exist
that  improve on BAT.   The Agency also does not believe that new
plants  could achieve any additional flow reduction  beyond  that
promulgated for BAT.

Primary Tungsten

For  the  primary tungsten subcategory,  NSPS are promulgated  as
equal  to BAT.   Review of the subcategory indicates that no  new
demonstrated technologies that improve on BAT exist.
                               429

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            GENERAL  DEVELOPMENT DOCUMENT
SECT - XI
 Dry scrubbing  is  not  demonstrated  for  controlling emissions   from
 acid  leaching,   APT  conversion  to oxides and  tungsten   reduction
 furnaces.    The   nature   of   these  emissions   (acid  fumes,  hot
 particulate    matter)  technically  precludes   the  use  of   dry
 scrubbers.   Therefore,   a   discharge  allowance is included  for
 these   sources at NSPS  equivalent to  that promulgated   for   BAT.
 Also,   the Agency does not believe that  new plants could achieve
 any additional   flow reduction beyond  the 90  percent  scrubber
 effluent recycle  promulgated for BAT.

 Primary Columbium-Tantalum

 The   promulgated  NSPS for  the  primary    columbium-tantalum
 subcategory  is   equivalent  to BAT.    Review of  the  subcategory
 indicates  that no new demonstrated technologies that improve on
 BAT exist.

 Dry scrubbing  is  not  demonstrated  for  controlling emissions   from
 concentration  digestion,    solvent  extraction,   precipitation,
 oxides calcining,  and reduction of  tantalum salt to metal.   The
 nature of these emissions (acidic  fumes,  hot particulate matter)
 technically  precludes the use of  dry  scrubbers.   Therefore,  a
 discharge  allowance  is included  for  these  sources  at   NSPS
 equivalent to  that promulgated for  BAT.   The Agency also does not
 believe  that  new  plants   could   achieve  any  additional   flow
 reduction beyond  that promulgated  for  BAT.

 Secondary Silver

 The promulgated  NSPS   for  the  secondary silver  subcategory  is
 equivalent to  BAT.   Review  of the  subcategory indicates that  no
 new demonstrated  technologies that  improve on BAT exist.

 Dry scrubbing is not demonstrated  for controlling emissions  from
 film  stripping   and precipitation of  film  stripping  solutions,
 precipitation  and  filtration   of  photographic  solutions,  and
 leaching  and  precipitation of  non-photographic  solutions.   The
 nature of these emissions (acidic  fumes,  hot particulate matter)
 technically  precludes the use of  dry  scrubbers.   Therefore,  a
 discharge  allowance  is  included  for  these  sources  at  NSPS!
 equivalent to  that promulgated for BAT.  The Agency also does not
 believe  that  new  plants  could  achieve  any  additional  flow
 reduction beyond  that promulgated  for BAT.

 Secondary Lead

The  promulgated  NSPS   for the  secondary  lead  subcategory  is
equivalent  to BAT with additional flow reduction over BAT levels
using  dry scrubbing to control emissions from  kettle  refining.
Review   of   the  subcategory   indicates  that  no   other   new
demonstrated technologies that improve on BAT exist.

Existing  wet scrubbers are used to control emissions and prevent
baghouse fires caused by sparking when sawdust and phosphorus are
                               430

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
applied  to the surface of the metal while in  the  kettle.   Dry
scrubbers  can  be used for this purpose if spark  arresters  and
settling  chambers are installed to trap sparks.    According  to
the  Secondary Lead Smelters Association,  this is a demonstrated
and viable technology option.   Dry scrubbing is not required  at
BAT because of the extensive retrofit costs of switching from wet
to dry scrubbing.   Dry scrubbing,  however,  is not demonstrated
for  controlling emissions from blast and reverberatory furnaces,
and  the  nature  of these  emissions  (hot  particulate  matter)
precludes  the  use of dry  scrubbing.   Therefore,  "a  discharge
allowance  is included for this source at NSPS equivalent to that
promulgated for BAT.   The Agency also does not believe that  new
plants  could  achieve any additional flow reduction beyond  that
promulgated for BAT.

Primary Antimony

The promulgated NSPS for primary antimony are equal to  BAT.   We
do  not  believe that new plants could achieve any  reduction  in
flow  beyond  the flows prom-ulgated for BAT.   Because  NSPS  is
equal to BAT, we believe that the NSPS will-not pose a barrier to
the entry of new plants into this subcategory.

Primary Beryllium

The promulgated NSPS for primary beryllium are equal to BAT.   We
do  not believe that new plants could achieve any flow  reduction
beyond the allowances promulgated for BAT.  Because NSPS is equal
to  BAT,  we  believe that the NSPS will not have  a  detrimental
impact on the entry of new plants into this subcategory.

Primary and Secondary Germanium and Gallium

The  promulgated  NSPS  for primary and secondary  germanium  and
gallium  are  equal to BAT.   We do not believe that  new  plants
could  achieve any reduction in flow beyond the  flow  allowances
promulgated  for BAT.  Because NSPS is equal to BAT,  we  believe
that the NSPS will not have a detrimental impact on the entry  of
new plants into this subcategory.

Secondary Indium

The  NSPS  for  the secondary indium  subcategory  are  based  on
chemical   precipitation  and  sedimentation,   (the  same  model
technology  as PSES).   The pollutants and  pollutant  parameters
specifically limited under NSPS are cadmium,  lead, zinc, indium,
total  suspended  solids,   and  pH.    The  priority  pollutants
chromium,  nickel,  selenium,  silver,  and  thallium  were  also
considered  for regulation because they are present at  treatable
concentrations  in  the  raw wastewaters from  this  subcategory.
These  pollutants  were  not  selected  for  specific  regulation
because  they will be effectively controlled when  the  regulated
priority metals are treated to the levels achievable by the model
technology.
                               431

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
The  costs and specific removal data for this subcategory are not
presented here because the data on which they are based has  been
claimed to be confidential.   We believe the promulgated NSPS are
economically  achievable,  and that they do not pose a barrier to
entry of new plants into this subcategory.

Secondary Mercury

The  promulgated NSPS for secondary mercury are based on chemical
precipitation, sedimentation, and filtration.  This technology is
fully  demonstrated in many nonferrous metals manufacturing  sub-
categories and would be expected to perform at the same level  in
this subcategory.

The pollutants specifically limited under NSPS are lead, mercury,
TSS,  and pH.   The priority pollutants arsenic, cadmium, copper,
silver, and zinc were also considered for regulation because they
are  present  at treatable concentrations in the raw  wastewaters
from  this subcategory.   These pollutants were not selected  for
specific  regulation because they will be effectively  controlled
when  the  regulated priority metals are treated  to  the  levels
achievable by the model technology.

We believe the promulgated NSPS are economically achievable,  and
that  they  are  not a barrier to entry of new plants  into  this
subcategory.

Primary Molybdenum and Rhenium

The promulgated NSPS for primary molybdenum and rhenium are equal
to BAT.  We do not believe that new plants could achieve any flow
reduction  beyond  the allowances promulgated for  BAT.   Because
NSPS are equal to BAT,  we believe that the NSPS will not have  a
detrimental   impact  on  the  entry  to  new  plants  into  this
subcategory.

Secondary Molybdenum and Vanadium

The  promulgated NSPS for secondary molybdenum and  vanadium  are
equal  to BAT.   We do not believe that new plants could  achieve
any reduction in flow beyond the flow allow-ances promulgated for
BAT.   Because  NSPS are equal to BAT,  we believe that the  NSPS
will  not  pose a barrier to the entry of new  plants  into  this
subcategory.

Primary Nickel and Cobalt

The  promulgated NSPS for primary nickel and cobalt are equal  to
BAT.   We  do  not  believe  that new plants  could  achieve  any
reduction  in  flow beyond the flow allow-ances  promulgated  for
BAT.   Because  NSPS are equal to BAT,  we believe that the  NSPS
will  not  pose a barrier to the entry of new  plants  into  this
subcategory.
                               432

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XI
 Secondary Nickel

 The  promulgated NSPS for secondary nickel are equivalent to PSES
 (chemical precipitation and sedimentation technology).   We do not
 believe  that  new  plants could achieve any  reduction  in  flow
 beyond  the flow allowances promulgated for PSES.    Because  NSPS
 are _equal  to  PSES, we believe that the NSPS will  not  pose  a
 barrier to the entry of new plants into this subcategory.

 Primary Precious Metals and Mercury

 The  promulgated NSPS for primary precious metals  and mercury are
 equal  to BAT.   We do not believe that new plants could  achieve
 any reduction in flow beyond the allowances promulgated for  BAT.
 Because NSPS are equal to BAT,   we believe that the NSPS will not
 have  a  detrimental impact on  the entry of new plants  into  this
 subcategory.

 Secondary Precious Metals

 The  promulgated NSPS for secondary precious metals are equal  to
 BAT.    We  do  not  believe  that new plants  could  achieve  any
 reduction  in  flow beyond the  allowances   promulgated   for  BAT.
 Because  NSPS  are  equal to BAT,   we believe that the   NSPS  are
 economically achievable,  and that they are not a barrier to entry
 of  new plants into this  subcategory.

 Primary Rare Earth Metals

 The promulgated NSPS for primary rare earth metals  are equal  to
 BAT,   which  is based on  in-process  flow reduction,   lime,   settle
 and filter   treatment, ,  followed  by  activated carbon   polishing
 technology for control of toxic  inorganic  and organic pollutants.
 Although the  BPT  and BAT  limitations  were  remanded   for   this
 subcategory,   EPA  feels   that   new   sources   would  be   able  to
 economically achieve  these new source  standards.

 The  NSPS for  this  subcategory are based on  in-process wastewater
 flow   reduction,    followed  by   lime,   settle,  and  filter  and
 activated  carbon   adsorption  end  of  pipe   treatments.     Flow
 reduction  is  based on 90 percent recycle of   scrubber   effluent.
 Activated  carbon   technology  is transferred  from the   iron  and
 steel category where  it is a demonstrated technology for  removal
 of  toxic organic pollutants.

 The    pollutants    specifically   limited   under   NSPS    are
 hexachlorobenzene,  chromium,  lead,  and nickel.   The  priority
pollutants benzene,  arsenic,  cadmium, copper, selenium, silver,
 thallium,  and  zinc were also considered for regulation  because
 they   were   found  at  treatable  concentrations   in  the   raw
wastewaters  from this subcategory.   These pollutants  were  not
selected for specific regulation because they will  be effectively
controlled  when the regulated priority pollutants  are treated to
the levels achievable by the model NSPS technology.
                               433

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XI
Secondary Tantalum

The promulgated NSPS for secondary tantalum are equal to BAT.  We
do  not  believe that new plants could achieve any  reduction  in
flow beyond the allowances promulgated for BAT.  Because NSPS are
equal to BAT, we believe that the NSPS will not pose a barrier to
the entry of new plants into this subcategory.

Secondary Tin

The promulgated NSPS for secondary tin are equal to BAT.   We  do
not  believe that new plants could achieve any reduction in  flow
beyond  the  allowances promulgated for BAT.   Because  NSPS  are
equal to BAT, we believe that the NSPS will not pose a barrier to
the entry of new plants into this subcategory.

Primary and Secondary Titanium

The promulgated NSPS for primary and secondary titanium are equal
to  BAT  plus  flow  reduction technology  with  additional  flow
reduction  for four streams.   Zero discharge  is promulgated  for
chip crushing,  sponge crushing and screening,  and scrap milling
wet  air  pollution control wastewater based   on  dry  scrubbing.
Zero  discharge is also promulgated for chlorine liquefaction wet
air  pollution control based on by-product recovery  of  scrubber
liquor as hypochlorous acid. Cost for dry scrubbing air pollution
control  in  a new facility is no greater than the cost  for  wet
scrubbing  which was the basis for BAT cost   estimates.   Because
NSPS  are equal to BAT,  we believe that the  NSPS will not pose a
barrier to the entry of new plants into this  subcategory.

Secondary Tungsten and Cobalt

The  promulgated NSPS for  secondary tungsten  and cobalt are  equal
to  BAT.   We  do not believe that new plants could  achieve  any
reduction  in  flow beyond the allowances  promulgated  for  BAT.
Because NSPS are equal to  BAT,  we- believe that the NSPS will not
pose a barrier to the entry of new plants  into this subcategory.

Secondary Uranium

The  promulgated NSPS for  secondary uranium are equal to BAT.   We
do  not  believe that new  plants  could achieve any   reduction   in
flow beyond  the allowances promulgated for BAT.  Because NSPS are
equal  to BAT, we believe  that the NSPS will not pose a  barrier  to
the entry of new plants  into this subcategory.

Primary  Zirconium and Hafnium

The  promulgated NSPS  for  primary zirconium and hafnium are  equal
to  BAT.   We   do not believe that new plants could achieve  any
reduction   in   flow beyond the  allowances   promulgated  for   BAT.
Because  NSPS are  equal  to BAT,   we believe that  the NSPS will  not
pose a barrier  to the  entry  of  new plants  into this subcategory.
                                434

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           GENERAL DEVELOPMENT DOCUMENT
    SECT - XI
                           Table XI-1

                 REGULATED POLLUTANT PARAMETERS
        Subcategory

Primary Aluminum Smelting
Secondary Aluminum Smelting
Primary Electrolytic Copper
  Refining
Primary Lead
Primary Zinc
Metallurgical Acid Plants
 Pollutant Parameters

 73.  benzo(a)pyrene
114.  antimony
121.  cyanide (total)
124.  nickel
      aluminum
      fluoride
      oil and grease
      TSS
      pH

122.  lead
128.  zinc
      aluminum
      ammonia (N)
      oil and grease
      phenolics (total;
       by 4-AAP method)
      TSS
      pH

114.  arsenic
120.  copper
124.  nickel
      TSS
      pH

122.  lead
128.  zinc
      TSS
      pH

118.  cadmium
120.  copper
122.  lead
128.  zinc
      TSS
      pH

115.  arsenic
118.  cadmium
120.  copper
122.  lead
128.  zinc
      TSS
      PH
                               435

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           GENERAL DEVELOPMENT DOCUMENT
   SECT - XI
                     Table XI-1 (Continued)

                 REGULATED POLLUTANT PARAMETERS
     Subcategory

Primary Tungsten
Pollutant Parameters
Primary Columbium-Tantalum
122.
128.
122.
128.
Secondary Silver
Secondary Lead
Primary Antimony
Primary Beryllium
120.
128.
114.
115.
122.
128.
114.
115.
123.
117.
119.
120.
121.
Primary and Secondary Germanium
and Gallium
115.
122.
128.
      lead
      zinc
      ammonia (N)
      TSS
      pH

      lead
      zinc
      ammonia (N)
      fluoride
      TSS
      pH

      copper
      zinc
      ammonia (N)
      TSS
      pH

      antimony
      arsenic
      lead
      zinc
      ammonia (N)
      TSS
      antimony
      arsenic
      mercury
      TSS
      PH

      beryllium
      chromium (total)
      copper
      cyanide
      ammonia (as N)
      fluoride
      TSS
      PH

      arsenic
      lead
      zinc
      fluoride
      TSS
      pH
                               436

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           GENERAL DEVELOPMENT DOCUMENT
  , SECT - XI
                     Table XI-1 (Continued)

                 REGULATED POLLUTANT PARAMETERS
     Subcategory

Secondary Molybdenum and Vanadium
Primary Nickel and Cobalt
Primary Precious Metals and Mercury
Secondary Precious Metals
Primary Rare Earth Metals
Pollutant Parameters

115.  arsenic
119.  chromium
122.  lead
124.  nickel
      molybdenum
      ammonia (as N)
      iron
      TSS
      PH

120.  copper
124.  nickel
      cobalt
      ammonia (as N)
      TSS
      pH

122.  lead
123.  mercury
126.  silver
128.  zinc
      gold
      oil and grease
      TSS
      pH

120.  copper
121.  cyanide
128.  zinc
      ammonia (as N)
      gold
      palladium
      platinum
      TSS
      pH

119.  chromium (Total)
122.  lead
124.  nickel
      TSS
                               437

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           GENERAL DEVELOPMENT DOCUMENT
   SECT - XI
                     Table XI-1 (Continued)

                 REGULATED POLLUTANT PARAMETERS
     Subcategory
Pollutant Parameters
Secondary Tantalum
Secondary Tin
Primary and Secondary Titanium
Secondary Tungsten and Cobalt
Secondary Uranium
120.  copper
122.  lead
124.  nickel
128.  zinc
      tantalum
      TSS
      pH

115.  arsenic
121.  cyanide
122.  lead
      iron
      tin
      fluoride
      TSS
      PH

119.  chromium (total)
122.  lead
124.  nickel
      titanium
      oil and grease
      TSS
      pH

120.  copper
124.  nickel
      cobalt
      tungsten
      oil and grease
      ammonia (as N)
      TSS
      pH

119.  chromium (total)
120.  copper
124.  nickel
      fluoride
      TSS
                               438

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           GENERAL DEVELOPMENT DOCUMENT
   SECT - XI
                     Table XI-1 (Continued)

                 REGULATED POLLUTANT PARAMETERS
     Subcategory
Primary Zirconium and Hafnium
Pollutant Parameters
119.  chromium (total)
121.  cyanide (total)
122.  lead
124.  nickel
      ammonia (as N)
      TSS
      PH
                               439

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GENERAL DEVELOPMENT DOCUMENT    SECT - XI
    THIS PAGE INTENTIONALLY LEFT BLANK
                   440

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XII
                            SECTION XII

                      PRETREATMENT STANDARDS
 Section 307(b) of the Clean Wajter Act requires EPA to  promulgate
 pretreatment standards for existing sources (PSES), which must be
 achieved  within three years of promulgation.  PSES are  designed
 to  prevent  the  discharge ofl  pollutants  which  pass  through,
 interfere with, or are otherwise incompatible with the  operation
 of publicly owned treatment wqjrks (POTW).  The Clean Water Act of
 1977   adds  a  new  dimension!  by  requiring  pretreatment   for
 pollutants,  such  as  heavy ..petals,  that  limit  POTW   sludge
 management alternatives, inducing the beneficial use of  sludges
 on  agricultural lands.  The legislative history of the 1977  Act
 indicates that pretreatment standards are to be technology-based,
 analogous  to  the  best  available  technology  for  removal  of
 priority pollutants.

 Section 307(c) of the Act requires EPA to promulgate pretreatment
 standards  for  new  sources:"(PSNS) at the  same  time  that  it
 promulgates  NSPS.  New indirect discharge facilities,  like  new
 direct discharge facilities, have the opportunity to  incorporate
 the  best available demonstrated technologies, including  process
 changes,    in-plant   controls,   and   end-of-pipe    treatment
 technologies, and to use plant site selection to ensure  adequate
 treatment system installation.

 General Pretreatment Regulations for Existing and New Sources  of
 Pollution were published in the Federal Register,  Vol. 46, No.
 18, Wednesday, January 28, 1981.  These regulations describe  the
 Agency's   overall   policy  for   establishing   and   enforcing
 pretreatment  standards for new and existing users of a POTW  and
 delineates the responsibilities and deadlines applicable to  each
 party  in  this effort.  In addition,  40 CFR  Part  403,  Section
 403.5 (b,), outlines prohibited discharges which apply to all users
 of a POTW.
 This  section describes the treatment and control technology  for
 pretreatment of process wastewaters from existing sources and new
 sources,   and  presents mass discharge limitations  of  regulated
 pollutants  for existing and new sources, based on the
 control   technology.    It also serves to summarize
 previous   rulemakings   in  the  nonferrous  metals
 category.

 REGULATORY APPROACH     • 'i-^
             described
         changes   from
         manufacturing
 There   are   125   faciliti'es,   representing  28  percent  of   the
 nonferrous    metals    manufacturing   category,    who   discharge
 wastewaters   to  POTW.   Pretreatment standards  are established  to
 ensure  removal of pollutants  discharged by these facilities which
 may  interfere with, pas;s  through,  or  be incompatible  with  POTW
.operations.   A determination  of  which  pollutants may pass through
 or   be  incompatible wi|€h?POTW operations,  and  thus be subject  to
                                441

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - XII
pretreatment standards, depends on the level of treatment used by
the  POTW.   In  general, more pollutants will  pass  through  or
interfere  with a POTW using primary treatment (usually  physical
separation  by settling) than one which has  installed  secondary
treatment (settling plus biological treatment).

Many   of   the  pollutants  contained   in   nonferrous   metals
manufacturing   wastewaters  are  not  biodegradable   and   are,
therefore, not effectively treated by such systems.  Furthermore,
these  pollutants  have been known to pass through  or  interfere
with the normal operations of these systems.  Problems associated
with the uncontrolled release of pollutant parameters  identified
in  nonferrous metals manufacturing process wastewaters  to  POTW
were discussed in Section VI.

The Agency based the selection of pretreatment standards for  the
nonferrous  metals manufacturing category on the minimization  of
pass-through   of   priority  pollutants  at  POTW.    For  _ each
subcategory, the Agency compared removal rates for each  priority
pollutant limited by the pretreatment options to the removal rate
for that pollutant at well-operated POTW.  The POTW removal rates
were  determined through a study conducted by the Agency at  over
40  POTW  and a statistical analysis of the data.  (See  Fate  of
Priority Pollutants in Publicly Owned Treatment Works, EPA  440/1-
80-301,  October, 1980; and Determining National Removal  Credits
for  Selected Pollutants for Publicly Owned Treatment Works,  EPA
                                             removal  rates
440/82-008,  September,
presented below:

 Priority Pollutant
1982.)   The  POTW
                       POTW Removal Rate
                                                              are
 Antimony                     0%
 Arsenic                      0%
 Cadmium                     38%
 Chromium                    65%
 Copper                      58%
 Cyanide                     52%
 Lead                        48%
 Mercury                     69%
 Nickel                      19%
 Selenium                     0%
 Silver                      66%
 Zinc                        65%
 Hexachlorobenzene           12%
 Ammonia                     40%
 Fluoride                     0%
 Total Regulated Metals      62%

 There were  no  data  concerning POTW  removals  for  beryllium,  boron,
 cobalt, germanium,  indium,  molybdenum,  radium  226,  thallium,  tin,
 titanium, and  uranium, to  compare with  our estimates  of   in-plant
 treatment.   Removal  of  these pollutants  is  solubility   related.
 Since  the   removal  of  metal  pollutants   for   which  data   are
 available   is   also'solubility  related, EPA  believes   that  these
 pollutants   may pass  through a  POTW.   It  was assumed,   therefore,
                                442

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
that these metals pass"- through "a POTW because they are soluble in
water  and  are  not  degradable.   Pass-through  data  are   not
available for benzo(aJ^Syrene; however, pass-through data for five
other polynuclear aromatic hydrocarbons do not exceed 83 percent.
This value was used for organics pass-through calculations.

A  pollutant is deemed to pass through the POTW when the  average
percentage  removed  nationwide by  well-operated  POTW,  meeting
secondary  treatment  requirements, is less than  the  percentage
removed  by  direct  dischargers  complying  with  BAT   effluent
limitations guidelines for that pollutant.  (See generally, 46 FR
9415-16  (January 28, 1981).)  For example, if the selected  PSES
option  removed  90  percent  of the  cadmium  generated  by  the
subcategory, cadmium would be considered to pass through  because
a  well-operated  POTW would be expected to  remove  38  percent.
Conversely,  if the selected PSES option removed only 30  percent
of  the  cadmium generated by the subcategory, it  would  not  be
considered  to pass through.  In the latter case,  cadmium  would
not  be selected for specific regulation because a  well-operated
POTW would have a greater removal efficiency.
                                     *'; '. '•
The  analysis described above was performed for each  subcategory
starting with the pollutants selected for regulation at BAT.  The
conventional pollutant parameters (TSS,  pH,  and oil and grease)
and   aluminum   were  not  considered   for   regulation   under
pretreatment   standards.   The   conventional   pollutants   are
effectively controlled by POTW, while aluminum is used to enhance
settling.  For those subcategories where ammonia was selected for
specific  limitation,  it  will also be selected  for  limitation
under pretreatment standards.  Most .POTW in the United States are
not  designed for nitrification.   Hence,  aside from  incidental
removal,  most,  if not all,  of the ammonia introduced into POTW
will pass through into receiving waters without treatment.

An   examination  of  the  percent  removal  for   the   selected
pretreatment  options  indicated  that  the  pretreatment  option
selected  removed at least 95 percent of the priority  pollutants
generated  in  the nonferrous metals manufacturing  point  source
category.  Consequently,  the priority pollutants  regulated  for
each   subcategory  under  BAT  will  also  be  regulated   under
pretreatment  standards.   Table XII-1 (page  460)  presents  the
pollutants selected for regulation for pretreatment standards.

MODIFICATIONS TO EXISTING PRETREATMENT STANDARDS

Existing  pretreatment  standards  proposed  for  the  nonferrous
metals  manufacturing  category are being revised to  incorporate
the building block approach as discussed earlier.   In  addition,
information  has become available regarding proposed pretreatment
standards that warrant.revision of promulgated standards.

Primary Aluminum Smelting                   ?

Pretreatment  standards  for  new sources  hjad  been  promulgated
previously  to  limit the quantity of  fluoride  discharged  from
                               443

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
primary aluminum smelters to POTW.  The technology basis for this
limitation  was lime precipitation and sedimentation.   PSNS  for
primary  aluminum  has been revised to incorporate  the  building
block approach and the same technology basis as for new  sources.
Since   the  PSNS  regulation  was  proposed,  three   additional
technologies have been identified as demonstrated or transferable
to   the  primary  aluminum  subcategory.   These   technologies,
filtration,  activated  carbon,  and dry  alumina  for  scrubbing
systems,  would  greatly reduce the amount  of  toxic  pollutants
discharged  by  a  new  source.  A  thorough  discussion  of  the
building  block  approach and selection  of  regulated  pollutant
parameters is presented in the primary aluminum supplement.

Secondary Aluminum Smelting

The  previously promulgated pretreatment standards  for  existing
secondary  aluminum  facilities limited the quantity of  oil  and
grease  allowed to be discharged from metal cooling, the pH  from
demagging fume scrubbers, and the quantity of ammonia  discharged
from  residue milling.  These mass limitations have been  revised
to include additional waste streams that warrant regulations  and
to  upgrade the technology basis so that it is analogous  to  the
promulgated BAT.

Pretreatment  standards  previously promulgated for  new  sources
require  zero discharge of all process generated pollutants  into
POTW  with the exception of demagging fume  scrubber  liquor.   A
discharge  from  this scrubber was allowed only when chlorine  is
used as a demagging agent.   Mass limitations developed for  this
discharge  were based on chemical precipitation and sedimentation
technology.   Revision of the promulgated  pretreatment  standard
was  necessary in light of comments and information received  and
to  incorporate  the more thorough building block  approach  (see
Section X).  An extensive description of the development of these
standards can be found in the secondary aluminum supplement.

Secondary Coppe'r

The promulgated pretreatment standards for existing sources allows
the  discharge  of  process wastewaters  subject  to  limitations
developed   from   chemical   precipitation   and   sedimentation.
technology.   Currently  promulgated  BAT  limitations,  however,
require  zero discharge of all process  wastewaters.   Therefore,
PSES  is being promulgated as zero discharge through recycle  and
reuse making it equivalent to BAT.

Metallurgical Acid Plants

As  discussed in Section IX,  the metallurgical acid plants  sub-
category has been modified to include acid plants associated with
primary  molybdenum  roasters.   This is based on the  similarity
between  discharge rates and effluent characteristics  of  waste-
waters from all metallurgical acid plants.

EPA   sis   not  extend  the  applicability   of   the   existing
                               444

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           GENERAL DEVELOPMENT .DOCUMENT
SECT - XII
metallurgical  acid  plant  pretreatment  standards  to   include
molybdenum acid plants because there are no indirect  discharging
molybdenum acid plants.                       ,

We  have  extended  the applicability of the  existing  PSNS  for
metallurgical  acid plants to include metallurgical  acid  plants
associated with primary molybdenum roasters.  It is necessary  to
promulgate  PSNS  to prevent pass-through  of  arsenic,  cadmium,
copper, lead, and zinc.  These priority pollutants are removed by
a well-operated POTW achieving secondary treatment at an  average
of  42 percent, while BAT level technology removes  approximately
83 percent.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  newj: plants  into  this
subcategory.                                 ^

OPTION SELECTION                             \:

The  treatment schemes considered for pretreatment standards  for
existing sources are identical to those considered for BAT.   The
treatment  schemes considered for pretreatment standards for  new
sources  are also identical to those considered for BAT with  the
exception  of  primary  aluminum  smelting,  secondary  aluminum,
primary lead, arid secondary lead, where additional flow reduction
is required.   Each of the options considered builds upon the BPT
technology  basis  of chemical precipitation and  sedimentation.
Depending  on  the pollutants present in  the  subcategories' raw
wastewaters,  a  combination of the treatment technologies listed
below were considered:

 o  Option A - End-of-pipe treatment consisting of chemical
    precipitation, sedimentation, and ion-exchange, and
    preliminary treatment, where necessary, consisting of
    oil skimming, cyanide precipitation, sulfide precipi-
    tation, iron co-precipitation, and ammonia air or steam
    stripping.  This combination of technology reduces
    priority metals and cyanide, conventional, and
    nonconventional pollutants.

 o  Option B - Option B is equal to Option A preceded by
    flow reduction of process wastewater through the use
    of cooling towers for contact cooling water and holding
    tanks for all other process wastewater subject to
    recycle.

 o  Option C - Option C is equal to Option ;B plus end-of-
    pipe polishing filtration for further reduction of
    priority metals and TSS.

 o  Option E - Option E consists of Option C plus activated
    carbon adsorption applied to the total plant discharge
    as a polishing step to reduce priority organic concen-
    trations.                             V
                                445

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            GENERAL DEVELOPMENT  DOCUMENT
SECT - XII
 The  general   approach  taken   by   the   Agency  for   pretreatment
 standards   for this  category is presented  below.   The  mass-based
 standards  for  each subcategory  may  be found  in Section  II  of  each
 subcategory supplement.  The options selected for  the  category  on
 which to base  pretreatment standards are discussed below.

 Primary Aluminum  Smelting

 Pretreatment    standards for   existing  sources   will   not    be
 promulgated for  the primary aluminum smelting subcategory since
 there are  no existing  indirect  dischargers.

 The  technology basis  for PSNS  is identical  to NSPS and includes
 flow  reduction, lime precipitation,  sedimentation, and  filtration
 for   control   of   toxic  metals,   and  cyanide   precipitation
 preliminary treatment.

 Secondary  Aluminum Smelting

 The technology basis for PSES is in-process  flow  reduction lime,
 precipitation,    sedimentation,   and  filtration.    Preliminary
 treatment   consisting  of ammonia steam  stripping  and  activated
 carbon  adsorption  is  included   for   selected   streams.    The
 achievable concentration for ammonia steam stripping  is based  on
 iron   and  steel manufacturing category data.    Flow reduction for
 the  selected   technology  option over   current  discharge rates
 represents a   75  percent  reduction  in  flow.   Ammonia steam
 stripping   and  lime  precipitation and sedimentation,  and  filter
 technologies are presently demonstrated  in the  nonferrous  metals
 manufacturing  category.  Ammonia air stripping  was the  technology
 basis  for the previously promulgated PSES.   Steam stripping  was
 promulgated j.n  this  rule instead of  air  stripping because  it  is a
 superior   technology in  that it does not transfer  the  pollutant
 from   one  media  to another.   Activated  carbon  adsorption  is
 selected   to  control  phenolics  in  the  scrubber   stream   from
 delacquering operations.

 Implementation  of the promulgated PSES would  remove  annually an
 estimated  11,300 kg/yr of toxic pollutants,   96 kg/yr of ammonia,
 and  212   kg/yr  of  phenolics  over  estimated  raw  discharges.
 Capital cost for achieving promulgated PSES  is  $2.3 million (1982
 dollars),  and annual cost of $1.4 million.

 The technology basis used to develop standards  for new  sources is
 identical  to  those  used for existing  sources.   There  is  no
 demonstrated technology  that is better than  the PSES  technology.

 Primary Copper Smelting

No  pretreatment standards for existing sources  are  promulgated
 for  the  primary copper smelting subcategory since there  are  no
 existing indirect dischargers.

The  technology basis for promulgated PSNS is identical  to  NSPS
                               446

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             GENERAL DEVELOPMENT DOCUMENT
SECT - XII
   n,n-                       dlschar<3e  of  all   process   wastewater
  pollutants,   with    no   allowance   for   catastrophic   stormwater
  discharge.   New  indirect  discharger^will be  constructed  with
  cooling   towers,  not cooling  impoundments,   since  they will  be
  located   near  POTW,   suggesting  that  they will  be   near  heavily
  populated areas where land  is scarce making the  cost of acquiring
  land to install an  impoundment  relatively high.   Thus,  we do not
  believe there are any incremental costs associated with PSNS.
 Primary Electrolytic Copper Refining
 No  pretreatment standards for existing sources  are  promulgated
 for  the  primary electrolytic copper refining subcategory  since
 there are no existing indirect dischargers.

 The technology basis of pretreatment for new sources is identical
 to   BAT   and  NSPS  and  is  based   on   lime   precipitation,
 sedimentation,  filtration,  and  90 percent recycle for  casting
 ™oaC^ -C00iin9  "ater.   As in NSPS,  all other  waste  stream!
 generated  at  copper  refineries are not included  in  the  flow
 allowance.                                         .          j-j-uw
 Secondary Copper

 As  mentioned earlier in this section,  PSES for secondary copper
 is  being  modified  to  make  it  equivalent  to  BAT,  or  zero
 discharge.    Implementation of the promulgated PSES would  remove
 an estimated 9,500 kg/yr of toxic pollutants from raw discharges?
 en *C!S fcimat(rd capital cost for achieving the promulgated PSES is
 $0 654  million  (1982  dollars)  and the annual  cost  is  $0.277
 HI i x j_ j. o n •
 no  techn?lo9v basis  for  promulgated PSNS  is  identical to  NSPS,
 PSES,    and   BAT.    NO allowance   for   catastrophic  stormwater
 discharges is provided as  is  discussed in Chapter  XI  for NSPS.

 Primary  Lead

 The-   technology   for   promulgated   PSES  is   equivalent  to BAT
 treatment _ and consists   of   in-process  flow  reduction,    lime
 precipitation,     sedimentation,   sulfide   precipitation    (and
 sedimentation), and multimedia filtration.  Implementation  of the
 promulgated   PSES  will remove an estimated 117  kg/yr   of   toxic
            over raw discharge.   The  capital  cost for   achieving
       1S-i?-'°57   million  <1982 dollars)  and the annual   cos??!
       million.
The  technology basis for promulgated PSNS is equivalent to  NSPS
or  zero discharge except for industrial hygiene streams provided
an allowance at NSPS.   As discussed in Chapter XI for NSPS, slaa
removed  from  dross reverberatory furnaces  contains  economical
recoverable amounts of lead that are granulated before recycling
New  facilities  will have the opportunity to  install  dry  slaq
conditioning devices to eliminate the usage of wastewater in this
process  or  implement  a  100 percent  recycle  system  of  slag
                               447

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
granulation   wastewater.    Elimination  of  the  sinter   plant
materials  handling wet air pollution control stream can also  be
accomplished with dry methods or 100 percent recycle.  The Agency
believes  the elimination of these process wastewater sources can
be  accomplished  without additional cost  beyond  BAT-equivalent
costs.

Primary Zinc

The technology basis for the promulgated PSES in the primary zinc
subcategory is equivalent to BAT.   The treatment consists of in-
process  flow  reduction,   lime  precipitation,   sedimentation,
sulfide   precipitation  (and  sedimentation),   and   multimedia
filtration.  Implementation of the PSES would remove an estimated
650,000  kg/yr  of  toxic pollutants  over  raw  discharge.   The
estimated capital cost for achieving PSES is $0.12 million   (1982
dollars) and the annual  cost is $0.058 million.

The   technology basis for promulgated pretreatment standards  f or
new   sources is equivalent to the NSPS basis of  flow  reduction,
lime  precipitation,  sedimentation,  sulfide  precipitation  and
sedimentation,  and  filtration.   The  PSNS flow allowances  are
based on  minimization  of process wastewater  wherever  possible
through  the  use of cooling "towers to  recycle  contact  cooling
water and sedimentation  basins for wet scrubbing wastewater.  The
discharges  from  contact  cooling and scrubbers is  based  on  90
percent  recycle.   Elimination of wastewater from   scrubbers  by
installing  dry  scrubbers   is not demonstrated  for  controlling
emissions  from zinc reduction furnaces,  leaching,  and  product
casting.   The  nature   of emissions from these  sources   (acidic
fumes,  hot particulate  matter) technically precludes the use  of
dry scrubbers.
                    the
                    The
 Metallurgical  Acid  Plants

 The   technology   basis    for   the   promulgated  PSES    in
 metallurgical  acid  plants  subcategory is  equivalent  to  BAT.
 treatment   consists    of    in-process   flow   reduction,
 precipitation, sedimentation, and multimedia filtration.   Sulfide
 precipitation   is included for  all primary lead and  primary _  zinc
 acid plants and one primary copper acid plant.   Implementation of
 the  promulgated PSES would remove approximately 12,500 kg/yr  o£
 toxic metals over raw discharge.  The capital cost for  PSES  is an
 estimated  $0.16 million  (1982 dollars)  and the annual  cost  is
 $0.085 million.

 The promulgated technology basis for pretreatment for new sources
 is  equivalent  to   the NSPS  basis  of   flow  reduction,    lime
 precipitation,   sedimentation,   sulfide   precipitation,    and
 filtration.   There  is no demonstrated technology that  provides
 better  pollutant  removal than that promulgated for  PSNS.    The
 acid  plant blowdown  allowance  allocated  for PSNS is based on  90
 percent  recycle.   The Agency  believes that no  additional   flow
 reduction  is   feasible  for new sources  because the  only  other
 available  flow reduction  technology,  reverse  osmosis,  is  not
                                448

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XII
 demonstrated nor  is  it clearly transferable  for  this  subcategory.

 Primary Tungsten

 The   technology   basis    for  the   promulgated  PSES    in    the
 primary tungsten  subcategory is equivalent to  BAT.    The  selected
 treatment  _  consists   of    in-process    flow    reduction,    lime
 precipitation  and sedimentation,  ammonia steam  stripping,   and
 filtration.

 Implementation  of the promulgated PSES  limitations would remove
 an   estimated 3,400  kg/yr  of toxic pollutants  over estimated   raw
 discharge, and  an estimated 63,320 kg/yr  of  ammonia.  The capital
 cost  for  achieving  promulgated PSES is $0.568  million   (1982
 dollars), and annual cost  of $0.445 million.

 The technology  basis for promulgated  PSNS is identical to PSES.
 The  PSES  flow allowances are based  on minimization  of  process
 wastewater wherever  possible through  the  use of  cooling towers to
 recycle contact  cooling  water and sedimentation basins  for  wet
 scrubbing wastewater.   These discharges  are based on 90  percent
 recycle  of    these  waste  streams.     Dry   scrubbing   is   not
 demonstrated  for controlling emissions from acid  leaching,  APT
 conversion to oxides and tungsten reduction  furnaces.  The nature
 of   these  emissions  (acidic  fumes,   hot  particulate  matter)
 technically precludes  the  use of dry  scrubbers.

 Primary Columbium-Tantalum

 The   technology   basis    for   the   promulgated  PSES    in   the
 primary columbium-tantalum subcategory is equivalent to BAT.  The
 selected treatment  consists  of  in-process flow  reduction,  lime
 precipitation  and sedimentation,  ammonia steam  stripping,  and
 filtration.   Flow   reduction is based on 90 percent  recycle  of
 scrubber effluent that  is  the flow basis of BAT.   This flow rate
 is  achieved by  both  indirect  dischargers  in the subcategory,  and
 filters  are  demonstrated at  23 plants in the nonferrous  metals
 manufacturing category.

 Implementation  of the promulgated PSES limitations would  remove
 18,590   kg/yr of  toxic pollutants,  290,460 kg/yr of ammonia  and
 400,175  kg/yr of  fluoride  from  raw discharges.    Capital cost for
 achieving promulgated PSES  is $1.03 million (1982  dollars),  and
 annual  cost of  $0.7 million.

 The  technology basis for promulgated PSNS is identical to  NSPS,
 PSES   and  BAT.    There   is  no  known  economically  feasible,
 demonstrated  technology that  is better than PSES technology.   The
PSES  flow  allowances  are  based  on  minimization  of  process
wastewater wherever possible  through the use of cooling towers to
 recycle  contact cooling water and sedimentation basins  for  wet
scrubbing  wastewater.   The  discharges are based on 90  percent
 recycle   of  these  waste  streams.     Dry  scrubbing   is   not
demonstrated   for   controlling  emissions  from   concentration
digestion,   solvent extraction,  precipitation, oxides calcining,
                               449

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
and  reduction of tantalum salt to metal.   The nature  of  these
emissions  (acidic  fumes,  hot particulate  matter)  technically
precludes the use of dry scrubbers.

Secondary Silver

The  technology basis for the promulgated PSES in  the  secondary
silver subcategory is equivalent to BAT.  The selected  treatment
consists  of  in-process  flow  reduction,  lime   precipitation,
sedimentation,  and  multimedia filtration,  along  with  ammonia
steam  stripping preliminary treatment.  Flow reduction is  based
on  complete  recycle  of  furnace  wet  air  pollution  control.
Filtration  is  currently in place at eight of  the  26  indirect
discharging  secondary  silver plants.   Promulgated  PSES  would
remove   an  estimated  4,259  kg/yr  of  toxic  pollutants   and
approximately 42,400 kg/yr of ammonia generated by the  industry.
Capital  cost  for achieving promulgated PSES  is  $0.63  million
(1982 dollars), with an annual cost of $0.42 million.

The  promulgated  technology basis for PSNS is equivalent to  the
NSPS basis of in-process flow reduction,  lime precipitation  and
sedimentation,  filtration,  and ammonia steam stripping.  Review
of   the   subcategory   indicates  that  no   new   demonstrated
technologies that improve on this BAT technology exist.

Dry scrubbing is not demonstrated for controlling emissions  from
film  stripping  and precipitation of film  stripping  solutions,
precipitation  and  filtration  of  photographic  solutions,  and
leaching  and  precipitation of non-photographic  solutions.   The
nature of these emissions (acidic fumes,  hot particulate matter)
technically precludes the use of dry  scrubbers.   Therefore,  an
allowance  is  included for these sources at PSES  equivalent  to
that  promulgated  for BAT and PSES.   The Agency also  does  not
believe  that  new  plants  could  achieve  any  additional  flow
reduction beyond that promulgated for BAT.

Secondary Lead
The  technology basis for the promulgated PSES in  the  secondary
lead  subcategory  is equivalent to BAT.  The selected  treatment
consists  of  in-process  flow  reduction,   lime  precipitation,
sedimentation,  and  multimedia filtration.   Flow
based  on  90  percent recycle of casting contact
         reduction  is
        cooling  water
through cooling towers.  Filtration is achieved by five of the 26
indirect discharging secondary lead plants.

Implementation  of the promulgated PSES would remove an estimated
46,500  kg/yr of toxic pollutants over estimated  raw  discharge.
Capital  cost  for  achieving promulgated PSES is  $4.26  million
(1982 dollars), with an annual cost of $2.51 million.

Pretreatment standards for new sources are equivalent to the NSPS
basis   of  in-process  flow   reduction,   lime   precipitation,
sedimentation  and filtration with the additional flow  reduction
over  BAT  levels using dry scrubbing to control  emissions  from
                               450

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
kettle  refining.    Flow reduction is based on 90 percent recycle
of  scrubber  effluent and casting contact  cooling  water  using
cooling towers and holding tanks.   There is no known demonstrated
technology  that is better than the technology basis  promulgated
for  new secondary lead plants.   Existing wet scrubbers are used
to  control  emissions  and  prevent  baghouse  fires  caused  by
sparking  when sawdust and phosphorus are applied to the  surface
of the metal while in the kettle.    Dry scrubbers can be used for
this  purpose  if   spark  arresters  and  settling  chambers  are
installed  to  trap  sparks.    According to  the  Secondary  Lead
Smelters   Association,   this  is  a  demonstrated  and   viable
technology option.   Dry scrubbing is not required at BAT because
of  the  extensive retrofit costs  of switching from  wet  to  dry
scrubbing.   Dry  scrubbing  is not demonstrated for  controlling
emissions from blast and reverberatory furnaces,  and the  nature
of  these emissions (hot particulate matter) precludes the use of
dry scrubbing.

Primary Antimony

Pretreatment  standards for existing sources were not promulgated
for the primary antimony subcategory because there are no  exist-
ing indirect dischargers.  We have promulgated PSNS equivalent to
NSPS and BAT.  The technology basis for PSNS is identical to NSPS
and  BAT.   It was necessary  to promulgate PSNS to prevent  pass-
through of priority metals.   These metals are removed by a well-
operated  POTW achieving secondary treatment at an average of  61
percent.   PSNS technology removes these pollutants at an average
of  98 percent.   No additional flow reduction for new sources is
feasible beyond the allowances promulgated for BAT.   We  believe
that  the PSNS are not a barrier to entry of new plants into this
subcategory  because  they do not  include  any  additional  costs
compared to BAT.

Primary Beryllium

Pretreatment  standards for existing sources were not promulgated
for the primary beryllium subcategory since there are no indirect
dischargers.   The  technology  basis  for  promulgated  PSNS  is
identical  to NSPS and BAT.  It was necessary to promulgate  PSNS
to prevent pass-through of beryllium, chromium, copper,  cyanide,
and  fluoride.   These  priority  pollutants  are  removed  by  a
well-operated POTW achieving  secondary treatment at an average of
41 percent while BAT technology removes approximately 93 percent.
The  PSNS  flow allowances are based on minimization  to  process
wastewater wherever possible  through the use of holding tanks for
wet  scrubbing wastewater.  The flow allowances are identical  to
those promulgated for BAT.

Primary and Secondary Germanium and Gallium

EPA  promulgated  PSES and PSNS limitations for this  subcategory
based on chemical precipitation and sedimentation treatment.

We  have  promulgated PSES to prevent  pass-through  to  arsenic,
                               451

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
lead,  zinc,  and  fluoride.   These pollutants are removed by  a
well-operated POTW achieving secondary treatment at an average of
33 percent while BAT technology removes approximately 87 percent.
Implementation  of the PSES limitations would remove annually
estimated 564 kg of priority metal pollutants.
                    an
The  costs and specific removal data for this subcategory are not
presented here because the data on which they are based have been
claimed to be cponfidential.  The promulgated PSES will not result
in adverse economic impacts.

We have promulgated PSNS equivalent to PSES,  NSPS and BAT.   The
technology basis for promulgated PSNS is identical to NSPS, PSES,
and BAT.   The same pollutants pass through as at PSES,  for  the
same  reasons.   We  believe that the promulgated PSNS are not  a
barrier to entry of new plants into this subcategory because they
do not include any additional costs compared to BAT.

Secondary Indium

PSES  limitations for this subcategory are promulgated  based  on
chemical   precipitation  and  sedimentation   technology.    The
pollutants  specifically regulated under PSES are cadmium,  lead,
zinc,  and  indium.   The priority pollutants  chromium,  nickel,
selenium,  silver,  and thallium were also considered for regula-
tion because they are present at treatable concentrations in  the
raw wastewaters from this subcategory.  These pollutants were not
selected for specific regulation because they will be effectively
controlled  when the regulated priority metals are treated to the
levels  achievable by the model technology.   It is necessary  to
promulgate  PSES to prevent pass-through of  cadmium,  lead,  and
zinc.  These toxic pollutants are removed by a well-operated POTW
achieving  secondary treatment at an average of 38 percent  while
this BAT level technology removes approximately 90 percent.
Implementation  of the PSES limitations would remove annually
estimated 586 kg of priority metals and 288 kg of indium.
                    an
We have promulgated PSNS equal to NSPS.  The technology basis for
PSNS  is identical to NSPS.   The same pollutants pass through as
at PSES, for the same reasons.

We  believe that the promulgated PSNS are  achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory.

Secondary Mercury

Pretreatment  standards for existing sources were not promulgated
for the secondary mercury subcategory since there are no existing
indirect dischargers.

We have promulgated PSNS equivalent to NSPS for this subcategory.
It  was necessary to promulgate PSNS to prevent  pass-through  of
                               452

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
lead,  and  mercury.   These  pollutants are removed  by  a  well-
operated  POTW achieving secondary treatment at an average of  59
percent  while  PSNS  level technology removes  approximately  99
percent.

We  believe that the promulgated PSNS are  achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory.

Primary Molybdenum and Rhenium

Pretreatment  standards for existing sources were not promulgated
for  the primary molybdenum and rhenium subcategory  since  there
are no existing indirect dischargers.

We  have  promulgated  PSNS  equal  to  BAT  and  NSPS  for  this
subcategory.   It  was  necessary to promulgate PSNS  to  prevent
pass-through of arsenic,  lead, nickel, selenium, molybdenum, and
ammonia.   These  priority  pollutants  are removed  by  a  well-
operated  POTW achieving secondary treatment at an average of  13
percent,   while  the  NSPS  and  BAT  level  technology  removes
approximately 79 percent.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory.

Secondary Molybdenum and Vanadium

Pretreatment standards for existing sources were not  promulgated
for the secondary molybdenum and vanadium subcategory since there
are no existing indirect dischargers.

We  have  promulgated  PSNS  equal  to  BAT  and  NSPS  for  this
subcategory. It was necessary to promulgate PSNS to prevent pass-
through of arsenic, chromium, lead, nickel, molybdenum, iron, and
ammonia.   These  priority  pollutants are  removed  by  a  well-
operated  POTW achieving secondary treatment at an average of  23
percent,  while  the  NSPS  and  BAT  level  technology   removes
approximately 98 percent.

The technology basis for PSNS is ammonia air stripping,  iron co-
precipitation,   chemical   precipitation,   sedimentation,   and
filtration.    The  achievable  concentration  for  ammonia   air
stripping  is based on nonferrous metals  manufacturing  category
data,   as  explained  in the discussion of BPT and  BAT  in  this
subcategory supplement.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT.

Primary Nickel and Cobalt
                               453

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
Pretreatment standards for existing sources were not  promulgated
for  the primary nickel and cobalt subcategory since there are no
existing indirect dischargers.

We  have  promulgated  PSNS  equal  to  BAT  and  NSPS  for  this
subcategory.   It  was necessary to promulgate  PSNS  to  prevent
pass-through  to  copper,  nickel, cobalt,  and  ammonia.   These
priority  pollutants  are removed by a well-operated POTW  at  an
average of 26 percent, while SAT technology removes approximately
58 percent.

The  technology  basis  for  PSNS  is  ammonia  steam  stripping,
chemical precipitation and sedimentation,  and  filtration.   The
achievable  concentration for ammonia steam stripping is based on
iron and steel manufacturing category data,  as explained in  the
discussion of BPT and BAT for this subcategory.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT.

Secondary Nickel

PSES  for  this  subcategory are promulgated  based  on  chemical
precipitation  and sedimentation.   The  pollutants  specifically
regulated  under  PSES are chromium,  copper,  and  nickel.   The
priority  pollutants  arsenic and zinc were also  considered  for
regulation  because they are present at treatable  concentrations
in the raw wastewaters from this subcategory.   These  pollutants
were  not  selected for specific regulation because they will  be
effectively  controlled  when the regulated priority  metals  are
treated to the levels achievable by the model technology.  We are
promulgating  PSES to prevent pass-through to  chromium,  copper,
and nickel.  These pollutants are removed by a well-operated POTW
at  an  average  of  32 percent  while  PSES  technology  removes
approximately 84 percent.

Implementation  of the promulgated PSES limitations would  remove
annually  an  estimated 1,624 kg of priority metals from the  raw
waste  loads.   We  estimate a capital cost of  $320,000  and, • .an
annualized  cost  of $161,233 to achieve PSES.   The  promulgated
PSES will not result in adverse economic impacts.

We have promulgated PSNS equivalent to NSPS and PSES.   The  same
pollutants pass through at PSNS as at PSES, for the same reasons.
The  PSES  flow allowances are based on minimization  of  process
wastewater wherever possible.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory.

Primary Precious Metals and Mercury
                               454

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
Pretreatment standards for existing sources were not  promulgated
for  the primary precious metals and mercury subcategory  because
there are no existing indirect dischargers.

We  have  promulgated  PSNS  equal  to  BAT  and  NSPS  for  this
subcategory. It was necessary to promulgate PSNS to prevent pass-
through of gold, lead, mercury, silver, and zinc.  These priority
pollutants  are removed by a well-operated POTW at an average  of
62   percent,   while  the  NSPS  and  BAT   technology   removes
approximately 93 percent.

The   technology  basis  for  PSNS  is  oil  skimming,   chemical
precipitation  and  sedimentation,  wastewater  flow   reduction,
filtration  and  ion  exchange.  Flow reduction is  based  on  90
percent  recycle of scrubber effluent that is the flow  basis  of
BAT.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  to  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT.

Secondary Precious Metals

The  technology basis for the promulgated PSES in  the  secondary
precious  metals  subcategory  is  equivalent  to  BAT.    It  is
necessary  to promulgate PSES to prevent pass-through of  copper,
cyanide,  zinc,  ammonia,  gold,  palladium,  and  platinum.  The
priority pollutants are removed by a well-operated POTW achieving
secondary  treatment at an average of 32 percent while BAT  level
technology  removes  approximately 99  percent.   The  technology
basis  for  PSES  is chemical  precipitation  and  sedimentation,
ammonia  steam stripping, cyanide precipitation, wastewater  flow
reduction,   filtration,  and  ion  exchange.    The   achievable
concentration  for ammonia steam stripping is based on  iron  and
steel manufacturing category data, as explained in the discussion
of BPT and BAT for this subcategory.  Flow reduction is based  on
the same recycle of scrubbej effluent and granulation water  that
is  the flow basis of BAT.  Recycle is practiced by 21 of the  29
existing plants in the subcategory.

Implementation  of the promulgated PSES limitations would  remove
annually an estimated 110,300 kg of priority pollutants including
866 kg of cyanide, and an estimated 10,530 kg of ammonia from the
raw  waste load.   Capital cost for achieving PSES is  $1,734,265
and  annualized cost of $1,059,367.   The proposed PSES will  not
result in adverse economic impacts.

We  have  promulgated  PSNS  equivalent to  NSPS  and  BAT.   The
technology  basis for promulgated PSNS is identical to  NSPS  and
BAT. The same pollutants pass through at PSNS as at PSES, for the
same reasons.  The NSPS flow allowances are based on minimization
of  process  wastewater  wherever possible  through  the  use  of
holding tanks to recycle wet scrubbing wastewater and granulation
water.  The  discharges  are  based on  recycle  of  these  waste
                               455

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
streams.   We believe that the promulgated PSNS  are  achievable,
and that they are not a barrier to entry of new plants into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT and PSES.

Primary Rare Earth Metals

PSES  and  PSNS  for  this  subcategory  are  based  on  chemical
precipitation  and  sedimentation,   in-process  wastewater  flow
reduction,  filtration,  and  activated carbon adsorption.   Flow
reduction  is based on 90 percent recycle of  scrubber  effluent.
Activated  carbon  technology  is transferred from the  iron  and
steel category where it is a demonstrated technology for  removal
of priority organic pollutants.

The  pollutants  specifically  limited under PSES  and  PSNS  are
hexachlorobenzene,  chromium,  lead,  and  nickel.   The priority
pollutants benzene,  arsenic,  cadmium, copper, selenium, silver,
thallium,  and  zinc were also considered for regulation  because
they   were  found  at  treatable  concentrations  in   the   raw
wastewaters  from  this subcategory.   These pollutants were  not
selected for specific regulation because they will be effectively
controlled when the regulated priority pollutants are treated  to
the levels achievable by the model PSES and PSNS technology.

Secondary Tantalum

Pretreatment  standards for existing sources were not promulgated
for  the  secondary  tantalum  subcategory  since  there  are  no
existing indirect dischargers.

We have promulgated PSNS equal to NSPS and BAT.  It was necessary
to  promulgate  PSNS  to prevent pass-through  of  copper,  lead,
nickel,  zinc,  and  tantalum.   These  priority  pollutants  are
removed by a well-operated POTW achieving secondary treatment  at
an  average  of 48 percent,  while BAT level  technology  removes
approximately 99 percent.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  to  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT.

Secondary Tin

The  technology basis for the promulgated PSES in  the  secondary
tin  subcategory  is  equivalent to  BAT.   It  is  necessary  to
promulgate  PSES  to prevent pass-through  to  arsenic,  cyanide,
lead,  iron,  tin,  and fluoride.   These priority pollutants and
fluoride  are removed by a well-operated POTW achieving secondary
treatment  at  an  average of 17  percent  while  BAT  technology
removes approximately 97 percent.   The technology basis for PSES
is  chemical precipitation,  sedimentation,  and filtration  with
preliminary  treatment consisting of cyanide precipitation  where
required.
                               456

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XII
 Implementation  of the promulgated PSES limitations would  remove
 annually an estimated 167 kg of priority metals,  6,227 kg of tin,
 20 kg of cyanide,   and 25,105 kg of fluoride over estimated  cur-
 rent discharge.   Capital cost for achieving PSES  is $160,187, and
 annual cost of $50,044.   The promulgated PSES will not result in
 adverse economic impacts.

 We have promulgated PSNS equivalent to PSES,  NSPS, and BAT.  The
 technology  basis  for PSNS is identical to NSPS,   PSES,  and BAT.
 The same pollutants pass through at PSNS as at PSES,  for the same
 reasons.   The  PSNS  flow allowances are identical to  the  flow
 allowances for BAT, NSPS, and PSES.

 There  would  be  no additional cost for  PSNS above  the  costs
 estimated  for  BAT.   We believe that the  promulgated  PSNS  are
 achievable,   and  that  they are not a barrier to  entry  of  new
 plants  into  this subcategory because they do not  include  any
 additional costs compared to BAT and PSES.

 Primary and  Secondary Titanium

 We  have promulgated PSES equal to BAT for  this subcategory.    It
 is  necessary  to   promulgate PSES  to  prevent   pass-through  of
 chromium,  lead,  nickel,  and titanium.   These priority  pollutants
 are removed  by a well-operated POTW achieving secondary treatment
 at  an  average  of  14   percent  while  BAT  technology  removes
 approximately 76 percent.   Implementation of the  promulgated PSES
 limitations  would  remove annually an estimated 1.7  kg of priority
 pollutants,  and  147 kg of titanium from the  current discharge.

 The cost data for  this subcategory are not presented  here because
 the _data  on which   they  are based  have   been  claimed  to  be
 confidential.    The  promulgated PSES  will not result in  adverse
 economic impacts.

 We  have  promulgated PSNS equivalent  to  NSPS.   The  technology
 basis   for   promulgated.  PSNS  is  identical   to  NSPS.    The   same
 pollutants are regulated at  PSNS  as  at  PSES  and they  pass  through
 at PSNS  as at PSES, for  the  same  reasons.  The PSNS and  NSPS  flow
 allowances   are  based  on  minimization  to  process  wastewater
 wherever  possible  through the  use of  cooling  towers   to   recycle
 contact  cooling  water   and  holding   tanks   for  wet   scrubbing
 wastewater.   The discharge  allowance  for pollutants  is  the   same
 at  PSNS  and  NSPS.   The discharges are  based on 90 percent  recycle
 of  these waste streams  (see  Section  IX  -  recycle of wet   scrubber
 and  contact cooling  water).  As  in NSPS, flow  reduction  beyond
 BAT   (zero   discharge) is  promulgated  for chip  crushing,  sponge
 crushing  and  screening,  and  scrap milling  wet  air  pollution
 control wastewater based on dry scrubbing.  Also,  zero  discharge
 is  promulgated  for   chlorine  liquification  wet  air  pollution
 control wastewater based on by-product  recovery.

We  believe  that the promulgated PSNS are achievable,  and  that
 they  are  not  a  barrier  to entry  of  new  plants  into  this
                               457

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
subcategory  because  they do not include  any  additional  costs
compared to BAT and PSES.

Secondary Tungsten and Cobalt

The  technology basis for the promulgated PSES in  the  secondary
tungsten  and  cobalt subcategory is equivalent to BAT and  PSNS.
It  was  necessary to promulgate PSES and PSNS to  prevent  pass-
through to copper,  nickel, cobalt, tungsten, and ammonia.  These
priority pollutants are removed by a well-operated POTW achieving
secondary treatment at an average of 26 percent,  while the  NSPS
and BAT level technology removes approximately 97 percent.


The  technology  basis for PSES and PSNS is ammonia steam_ strip-
ping, oil skimming, chemical precipitation and sedimentation, and
filtration.   The  achievable  concentration  for  ammonia  steam
stripping is based on iron and steel manufacturing category data,
as  explained  in  the  discussion  of  BPT  and  BAT  for   this
subcategory.

Implementation  of the PSES limitations would remove annually  an
estimated 13 kg of priority pollutants.  Capital and annual costs
expected  to be incurred to achieve PSES are $16,293 and  $8,765,
respectively.    The   Agency  has  determined  that   PSES   are
economically  achievable and will not result in adverse  economic
impacts.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT.

Secondary Uranium

Pretreatment  standards  for existing sources were not'promulgated
for the secondary uranium subcategory since there are no existing
indirect dischargers.

We  Have  promulgated  PSNS  equal  to  BAT  and  NSPS  for  this
subcategory.  It  was  necessary to promulgate  PSNS  to  prevent
passthrough  of  chromium, copper, nickel, and  fluoride.   These
priority pollutants are  removed by a well-operated POTW achieving
secondary  treatment at  an average of 40 percent, while the  NSPS
and BAT level technology removes approximately  88 percent.

The   technology  basis  for  PSNS  is  chemical   precipitation,
sedimentation,  and filtration, plus in-process  wastewater  flow
reduction.

We  believe  that  the promulgated PSNS are  achievable,  and  that
they  are  not  a  barrier   to entry  of  new   plants  into  this
subcategory  because  they do not  include  any  additional   costs
compared to  BAT.
                                458

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XII
Primary Zirconium and Hafnium

EPA  did  not  promulgate  pretreatment  standards  for  existing
sources  for the primary zirconium and hafnium  subcategory.   We
had  proposed PSES for this subcategory in a two tier  regulatory
approach.   However,  we  are excluding from national  regulation
plants  which  only reduce zirconium or  zirconium-nickel  alloys
from  zirconium dioxide with magnesium or  hydrogen.   Since  the
only  indirect  discharger in the subcategory complies with  this
requirement,  we  have  decided not to establish  PSES  for  this
subcategory.   However,  this  facility will still be subject  to
general pretreatment standards.

We  are  promulgating  PSNS  equivalent to  NSPS  and  BAT.   The
technology basis for promulgated PSNS is identical to NSPS.   The
following  priority pollutants pass through:  chromium,  cyanide,
lead, nickel, and ammonia.  It is necessary to promulgate PSNS to
prevent  pass-through.  These pollutants are removed by  a  well-
operated  POTW achieving secondary treatment at an average of  30
percent,  while BAT technology removes approximately 80  percent.
We know of no economically feasible, demonstrated technology that
is better than BAT and NSPS technology.

We  believe  that the promulgated PSNS are achievable,  and  that
they  are  not  a  barrier  to entry  of  new  plants  into  this
subcategory  because  they do not include  any  additional  costs
compared to BAT and PSES.
                               459

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           GENERAL DEVELOPMENT DOCUMENT
  SECT - XII
                           Table XII-1

       POLLUTANTS SELECTED FOR REGULATION FOR PRETREATMENT
                    STANDARDS BY SUBCATEGORY
     Subcategory
Pollutant Parameters
Primary Aluminum Smelting*
Secondary Aluminum Smelting
Primary Copper Smelting

Primary Electrolytic Copper
  Refining*
Primary Lead
Primary Zinc
Metallurgical Acid Plants
Primary Tungsten
Primary Columbium-Tantalum
Secondary Silver
 73.  benzo(a)pyrene
114.  antimony
121.  cyanide (total)
124.  nickel
      fluoride

122.  lead
128.  zinc
      ammonia (N)
      phenolics
       (by 4-AAP
        Method)
114.  arsenic
120.  copper
124.  nickel

122.  lead
128.  zinc

118.  cadmium
120.  copper
122.  lead
128.  zinc

115.  arsenic
118.  cadmium+
120.  copper
122.  lead
128.  zinc+

122.  lead
128.  zinc
      ammonia (N)

122.  lead
128.  zinc
      ammonia (N)
      fluoride

120.  copper
128.  zinc
      ammonia (N)
                               460

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            GENERAL DEVELOPMENT DOCUMENT
   SECT - XII
                      Table XII-1 (Continued)

        POLLUTANTS SELECTED FOR REGULATION FOR PRETREATMENT
                     STANDARDS BY SUBCATEGORY
      Subcategory

 Secondary  Lead
Primary Antimony
Primary Beryllium
Primary and Secondary
  Germanium and Gallium
Secondary Indium
Secondary Mercury
Primary Molybdenum
  and Rhenium
Secondary Molybdenum
  and Vanadium
 Pollutant  Parameters

 114.   antimony
 115.   arsenic
 122.   lead
 128.   zinc
       ammonia  (N)

 114.   antimony
 115.   arsenic
 123.   mercury

 117.   beryllium
 119.   chromium
 120.   copper
 121.   cyanide
       ammonia (as N)
       fluoride

 115.   arsenic
 122.   lead
 128.   zinc
       fluoride

 118.   cadmium
 122.   lead
 128.   zinc
       indium

 122.   lead
 123.  mercury

 115.  arsenic
 122.  lead
 124.  nickel
 125.  selenium
      fluoride
      molybdenum
      ammonia (as N)

115.  arsenic
119.  chromium
122.  lead
124.  nickel
      iron
      molybdenum
      ammonia (as N)
                               461

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           GENERAL DEVELOPMENT DOCUMENT
  SECT - XII
                     Table XII-1 (Continued)

       POLLUTANTS SELECTED FOR REGULATION FOR PRETREATMENT
                    STANDARDS BY SUBCATEGORY
  Subcategory

Primary Nickel and Cobalt




Secondary Nickel
Primary Precious Metals
  and Mercury
Secondary Precious Metals
Pollutant Parameters

120.  copper
124.  nickel
      cobalt
      ammonia (as N)

119.  chromium
120.  copper
124.  nickel

122.  lead
123.  mercury
126.  silver
128.  zinc
      gold

120.  copper
121.  cyanide
128.  zinc
      ammonia (as N)
      gold
      palladium
      platinum
Primary Rare Earth Metals
Secondary Tantalum
Secondary Tin
9.
119.
122.
124.
120.
122.
124.
128.

115.
121.
122.



hexachlorobenzene
chromium
lead
nickel
copper
lead
nickel
zinc
tantalum
arsenic
cyanide
lead
iron
tin
fluoride
(total)










                               462

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           GENERAL DEVELOPMENT DOCUMENT
   SECT - XII
                     Table XII-1 (Continued)

       POLLUTANTS SELECTED FOR REGULATION FOR PRETREATMENT
                    STANDARDS BY SUBCATEGORY
    Subcategory

Primary and Secondary
  Titanium
Secondary Tungsten
  and Cobalt
Secondary Uranium
Primary Zirconium
  and Hafnium
Pollutant Parameters

119.  chromium (total)
122.  -lead
124.  nickel
      titanium

120.  copper
124.  nickel
      cobalt
      tungsten
      ammonia (as N)

119.  chromium (.total)
120.  copper
124.  nickel
      fluoride

119.  chromium (total)
121.  cyanide (total)
122.  lead
124.  nickel
      ammonia  (as N)
*Regulated by PSNS only.
+Regulated by PSES only.
                               463

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                    464

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          GENERAL DEVELOPMENT DOCUMENT
SECT -XIII
                       SECTION XIII

         BEST CONVENTIONAL POLLUTANT CONTROL TECHNOLOGY
EPA  is  not  promulgating best  conventional  pollutant  control
technology (BCT) for the nonferrous metals manufacturing category
at this time.
                               465

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                     466

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XIV
                           SECTION XIV

                        ACKNOWLEDGMENTS
The nonferrous metals manufacturing project has been ongoing as a
regulation  development  project since the Consent  Agreement  of
1976  required  EPA to re-study and expand the regulation of  this
industry category.   During this eleven year period many  persons
have  contributed  in  a  meaningful way  toward  the  successful
completion of the project.   This section is intended to  provide
some  recognition  to  those who have labored in behalf  of  this
regulation development effort.

Much  of  the sampling,  analysis,  data  compilation  and  draft
manuscript  preparation has been conducted by contractors for the
EPA.   The  initial  contractor in this effort was  Sverdrup  and
Parcel and Associates under Contact  No.  68-01-4409.   Technical
personnel  of this contractor who worked on the project included:
Mr.  Donald Washington,  Project Manager, Mr. Garry Aronberg, Ms.
Claudia O'Leary,  Mr.  Antony Tawa,  Mr. Charles Amelotti and Mr.
Jeff Carlton.  The second and final contractor in this effort was
Radian Corporation under Contracts N.  68-01-6529, 68-01-6999 and
68-03-3411.  Technical personnel of this contractor who worked on
the project included:   Mr.  James Sherman,  Program Manager, Mr.
Mark  Hereth,   Project  Director,  Mr.  Ron  Dickson,  Mr.  John
Vidumsky, Mr. Richard Weisman, Mr. Tom Grome, Mr. Marc Papai, Ms.
Lori Stoll,  Mr.  John Collins,  Mr. Mike Zapkin, Mr. Andrew Oven
and Ms.  Diane Neuhaus.  Acknowledgment and appreciation is also
made  to the Radian secretarial staff,  Ms.  Nancy  Johnson,  Ms.
Sandra Zapkin and Ms. Daphne Phillips for their tireless efforts.

This regulation development project has been under the  direction
of  Mr.  Ernst  P.  Hall,  Chief of the Metals  Industry  Branch,
Industrial   Technology  Division  of  EPA.    Technical  Project
Officers  for  this  project were (in order  of  succession)  Ms.
Patricia Williams,  Mr. James Berlow, Ms. Maria Irizarry, and Ms.
Eleanor Zimmerman,  with assistant project Officers Mr.  Geoffery
Grubbs and Mr.  Stuart Colton.   The final review and editing  of
this document has been under the immediate direction of Mr. Hall.

Special  note is made of the contribution of the word  processing
staff of the Industrial Technology Division,  Ms. Kaye Starr, Ms.
Nancy Zubric,  Ms.  Pearl Smith,  Ms.  Carol Swann and Ms. Glenda
Nesby  and a special commendation is given to Ms.  Smith for  her
tireless  efforts in producing the final drafts and camera  ready
copy of the entire document.

The  cooperation  of the Aluminum  Association,  American  Mining
Congress,  Aluminum  Recycling  Association,  Tantalum  Producers
Association  and  Secondary Lead Smelters Association along  with
their technical committees and individual companies that supplied
information   and  whose  plants  were  sampled   is   gratefully
acknowledged.
                               467

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
                           SECTION XV

                           REFERENCES


1.   Sampling and Analysis Procedures for Screening of Industrial
Effluents for Priority Pollutants, USEPA Environmental Monitoring
and  Support  Laboratory,  Cincinnati,  OH  45268  (March,  1977,
revised April, 1977).

2.   "Mineral  Facts and Problems," Bureau to Mines Bulletin 667,
Washington. D.C., Department to the Interior (1975).

3.   Development Document for Effluent Limitations Guidelines and
New Source Performance Standards for the Primary Aluminum  Smelt-
ing  Subcategory,  EPA-4401/l-74-019d.  Environmental  Protection
Agency (March, 1974).

4.   Development Document for Effluent Limitations Guidelines and
New  Source  Performance  Standards for  the  Secondary  Aluminum
Subcategory,  EPA-400/l-74-019e,  Environmental Protection Agency
(March, 1974).

5.   Development  Document for Interim Final Effluent Limitations
Guidelines and Proposed New Source Performance Standards for  the
Primary  Copper Smelting Subcategory and Primary Copper  Refining
Subcategory,  EPA-440/l-75/032b,  Environmental Protection Agency
(February, 1975).

6.   Development  Document for Interim Final Effluent Limitations
Guidelines and Proposed New Source Performance Standards for  the
Secondary  Copper Subcategory,  EPA-440/l-75/032c,  Environmental
Protection Agency (February, 1975).

7.   Development Document for Interim Final Effluent  Limitations
Guidelines  and Proposed New Source Performance Standards for the
Lead Segment,  EPA-440/l-75/032a, Environmental Protection Agency
(February, 1975).

8.   Development Document for Interim Final Effluent  Limitations
Guidelines  and Proposed New Source Performance Standards for the
Zinc Segment,  EPA-440/1-75/032,  Environmental Protection Agency
(February, 1975).

9.   Draft  Development Document for Effluent Limitations  Guide-
lines and New Source Performance Standards for the  Miscellaneous.
Nonferrous   Metals  Segment,   EPA-440/1-76/067,   Environmental
Protection Agency (March, 1977).

10.  "National Resources Defense Council v. Train", Environmental
Reporter - Cases 8 ERC 2120 (1976).
                               469

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
11.  Development Document for Effluent Limitations Guidelines and
New Source Performance Standards for the Bauxite Refining  Indus-
try,  EPA-440/1-74/019C,  Environmental Protection Agency (March,
1974).

12.  Pound, C. E. and Crites, R. W., "Land Treatment of Municipal
Wastewater  Effluents,  Design Factors - Part 1," Paper presented
at USEPA Technology Transfer Seminars (1975).
13.   Wilson,  Phillip  R.,  Brush  Wellman,
Personal Communication (August, 1978).
   Inc.,  Elmore,  OH,
14.   Description  of the Beryllium Production Processes  at  the
Brush Wellman,  Inc.  Plant in Elmore,  OH,  Brush Wellman,  Inc.
(1977).  (Photocopy).

15.   Phillips, A. J., "The World's Most Complex Metallurgy (Cop-
per,  Lead and Zinc),"  Transactions to the Metallurgical Society
of AIME, 224, 657 (August, 1976).

16.  Schack, C. H. and Clemmons, B. H., "Review and Evaluation of
Silver-Production Techniques," Information Circular 8266,  United
States Department of the Interior, Bureau of Mines (March, 1965).

17.   Technical Study Report:  BATEA-NSPS-PSES-PSNS-Textile Mills
Point  Source Category,  Report submitted to EPA-Effluent  Guide-
lines  Division  by  Sverdrup  &  Parcel  and  Associates,   Inc.
(November, 1978).

18.   The Merck Index, 8th edition, Merck & Co., Inc., Rahway, NJ
(1968).

19.   Rose,  A.  and Rose, E., The Condensed Chemical Dictionary,
6th ed., Reinhold Publishing Company, New York (1961).

20.  McKee, J. E. and Wolf, H. W. (eds.), Water Quality Criteria,
2nd  edition,  California  State Water  Resources  Control  Board
(1963).

21.   Quinby-Hunt,  M. S., "Monitoring Metals in Water," American
Chemistry (December, 1978), pp. 17-37.

22.   Fassel,  V.  A.  and Kniseley,  R. N., "Inductively Coupled
Plasma  - Optical  Emission Spectroscopy," Analytical  Chemistry,
46,13 (1974)
23.   Study  of Selected Pollutant Parameters in  Publicly  Owned
Treatment  Works,  Draft report submitted to EPA-Effluent  Guide-
lines  Division  by  Sverdrup  &  Parcel  and  Associates,   Inc.
(February, 1977).

24.   Schwartz,  H.  G.  and Buzzell,  J. C., The Impact of Toxic
Pollutants  on  Municipal  Wastewater  Systems,   EPA  Technology
Transfer,  Joint  Municipal/Industrial Seminar on Pretreatment of
Industrial Wastes, Dallas, TX (July, 1978).
                               470

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
25.  Class notes and research compiled for graduate class, Autumn
Qtr.,  1976-77 School year at Montana State University by  G.  A.
Murgel.

26.   Gough, P. and Shocklette, H. T., "Toxicity of Selected Ele-
ments to Plants, Animals and Man—An Outline," Geochemical Survey
of  the  Western Energy Regions,  Third Annual  Progress  Report,
July,  1976,  US  Geological  Survey  Open  File  Report  76-729,
Department of the Interior, Denver (1976).

27.   Second  Interim Report - Textile Industry BATEA-NSPS-PSES-
PSNS Study,  report submitted to EPA-Effluent Guidelines Division
by Sverdrup & Parcel and Associates, Inc. (June, 1978).

28.   Proposed Criteria for Water Quality,  Vol. 1, Environmental
Protection  Agency  (October,   1973)  citing  Vanselow,  A.  P.,
"Nickel,  in  Diagnostic Criteria for Plants and  Soils,"  H.  D.
Chapman,  ed., University of California, Division of Agricultural
Science, Berkeley, pp. 302-309 (1966).

29.  Morrison, R. T. and Boyd, R. N., Organic Chemistry, 3rd ed.,
Allyn and Bacon, Inc., Boston (1973).

30.  McKee, J. E. and Woll, H. W. (eds), Water Quality Criteria,
2nd  edition,  California  State Water Resources  Control  Board
(1963)  citing  Browning,  E.,  "Toxicity of  Industrial  Metals,
Butterworth, London, England (1961).

31.  citing Stokinger,  H.  E.  and Woodward,  R.  L., "Toxicologic
Methods for Establishing Drinking Water Standards," Journal AWWA,
50, 515 (1958).

32.  citing Waldichuk, M., "Sedimentation of Radioactive Wastes
in the Sea," Fisheries Research Board of Canada,  Circular No. 59
(January, 1961).

33.  citing  "Quality Criteria for Water,"  U.S.  Environmental
Protection Agency; Washington, D.C., Reference No. 440/9-76-023.

34.  Bronstein,  M.  A., Priviters, E. L., and Terlecky, P. M.,
Jr.,   "Analysis  of  Selected Wastewater Samples  of  Chrysotile
Asbestos  and Total Fiber Counts - Nonferrous Metals Point Source
Category," Calspan Advanced Technology Center,  Report No.    ND-
5782-M-19  for USEPA,   Effluent Guidelines Division (November  1,
1978).

35.  Hallenbeck,  W.  H.  and Hesse, C. S.,  "A Review of the
Health    Effects of Ingested Asbestos," Review of  Environmental
Health, 2,    3, 157 (1977).

36.   McKee, J. E. and Wolf,  H.  W. (eds), Water quality Criteria,
2nd  edition,  California  State Water Resources  Control  Board,
(1963)  citing  The Merck Index,  7th ed.,  Merck  &  Co.,  Inc.,
Rahway, NJ (1960) .
                               471

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
37.  citing  Pomelee,  C.  S.,  "Toxicity of Beryllium," Sewage
and Industrial Wastes, 25, 1424 (1953).

38.  citing  Rothstein,  "Toxicology  of  the  Minor  Metals,"
University of Rochester, AEC Project, UR-262 (June 5, 1953).

39.  citing Truhout, R. and Boudene, C., "Enquiries Into    the
Pacts  of  Cadmium  in the Body  During  Poisoning:   Of  Special
Interest to Industrial Medicine," Archiv. Hig. Roda 5, 19 (1954);
AMA Archives of Industrial Health 11, 179 (February, 1955).

40.  citing Fairhall, L. T., "Toxic Contaminants of    Drinking
Water," Journal New England Water Works Association,  55,     400
(1941).

41.  citing  Ohio  River  Valley Water  Sanitation  Commission,
"Report  on  the  Physiological Effects of Copper  on  Man,"  The
Kettering  Laboratory,   College  of  Medicine,   University   of
Cincinnati, Cincinnati, OH (January 28, 1953).
42.  citing "Copper and the Human Organism," Journal
Water Works Association, 21, 262 (1929).
             American
43.  citing  Taylor,  E.  W.,  "The  Examination of Waters  and
Water Supplies," P. Blakiston's Son and Co. (1949).
44.  citing  "Water  Quality  and  Treatment,"
(1950).
     2nd  ed.,   AWWA
45.  citing Hale,  F.  E.,  "Relation to Copper and Brass  Pipe
to Health," Water Works Eng., 95, 240, 84, 139, 187 (1942).

46.  citing "Drinking Water Standards," Title 42 - Public Health
Chapter   1  - Public  Health  Service,   Department  to  Health,
Education,  and Welfare;  Part 72 - Interstate Quarantine Federal
Register 2152 (March 6, 1962).

47.  citing Derby,  R. L., Hopkins, 0. C., Gullans, 0., Baylis,
J.  R.,  Bean,  E. L., and Malony, F., "Water Quality Standards,"
Journal American Water Works Association,  52,  1159  (September,
1960).

48.  McKee,  J.  E.  and  Wolf,  H.  W.,  (eds.).  Water Quality
Criteria,  2nd edition,  California State Water Resources Control
Board,  (1963) citing Klein,  L.,  "Aspects of River  Pollution,"
Butterworth  Scientific Publications,  London and Academic Press,
Inc., New York (1957) .

49.  citing Fuchess,  H.,  Bruns, H., and Haupt, H., "Danger of
Lead Poisoning From Water Supplies," Theo.  Steinkopff  (Dresden)
(1938);  Journal  American  Water  Works  Association,  30,  1425
(1938).

50.  citing  "Ohio  River Valley Water  Sanitation  Commission,
Subcommittee  on  Toxicities,  Metal Finishing  Industries  Action
                               472

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XV
 Committee,"  Report  No.  3  (1950).

 51.   Pickering,  Q.  H. and Henderson,  C.,  "The  Acute  Toxicity of
 Some  Heavy   Metals  to Different  Species of   Warm  Water   Fish,"
 Intnat.  J. Air-Water  Pollution,  10:  453-463  (1966).

 52.   Murdock,  H. R. Industrial Wastes,"  Ind. Eng.  Chem.  99A-102A
 (1953).

 53.   Calabrese,   A., et.  al., "The  Toxicity of  Heavy  Metals of
 Embryos   of  the  American  Oyster,   Crassostrea  Virginicia,"  Marine
 Biology  38:  162-166 (1973).

 54.   citing  Russell,  F. C.,  "Minerals in  Pasture,  Deficien-cies
 and   Excesses  in Relation to Animal  Health," Imperial  Bureau  of
 Animal  Nutrition,  Aberdeen,  Scotland,   Tech.  Communication  15
 (1944).

 55.   citing  Hurd-Kaner,   A., "Selenium Absorption  by Plants and
 their Resulting  Toxicity to Animals,"   Smithsonian  Inst.   Ann.
 Rept., p. 289  (1934-35).

 56.   citing  Byers,  H. G.,  "Selenium Occurrence in  Certain Soils
 in   the  United States with a Discussion of Related Topics,"   U.S.
 Department of Agr.  Tech.  Bull. No. 582 (August,  1935).

 57.   citing  Fairhall,   L.  T.,   "Toxic Contaminants  of Drinking
 Water,"   Journal New England Water  Works  Association,  55,  400
 (1941).

 58.   citing  Smith,  M.  I., Franke, K. W., and Westfall, B.  B.,
 "Survey   to  Determine the  Possibility of  Selenium  Detoxification
 in   the   Rural Population  Living on   Seleniferous  Soil,"   Public
 Health Repts. 51, 1496  (1936).

 59.   citing  Kehoe, R.  A.,  Cholak, J., and Largent,  E. J.,  "The
 Hygienic - Significance of  the Contamination of Water with Certain
 Mineral Constituents," Journal American Water Works  Association,
 36,  645  (1944).

 60.   citing  Schwarz, K.,  "Effects of Trace Amounts of Selenium,"
 Proc.  Conf.  Physical. Effects of Water Quality,  U.S.P.H.S., p. 79
 (September,  1960).

 61.  Water Quality Criteria of 1972.   NAS Report.

 62.  US  Department  of   Agriculture,   Agricultural  Research
 Science,  Consumer  and  Food Economics Research  Division,   "Food
 Consumption of Households  in the United States "  (Spring,  1965),
 Preliminary  Report,  Agricultural Research Service,   Washington,
 D.C.

 63.  Hill,  W. R. and  Pillsburg"  D. M., "Argyria  Investigation -
Toxicity  Properties  of  'Silver,"   American  Silver   Producers
Research Project Report, Appendix 11.
                               473

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
64.  citing Brown, A. W. A., "Insect Control by Chemicals," John
Wiley and Sons (1951).

65.  Lougis, P., "The Physiological Effect of Zinc in Seawater,"
Comptes Rendu, Paris, 253:740-741 (1961).

66.  Wisely,  B.  and  Blick,  R.  A.,  "Mortality  of  Marine
Invertebrate Larvae in Mercury, Copper and Zinc Solutions," Aust.
J. of Mar. Fresh. Res., 18:63-72 (1967).

67.  Clarke,  G.  L.,  "Poisoning and Recovery in Barnacles and
Mussels," Biol. Bull., 93:73-91 (1947).

68.  Foreman, C. T., "Food Safety and the Consumer," EPA Jour. 4,
10, 16 (November/December, 1978).

69.  Marnahan,  S. E., Environmental Chemistry, 2nd ed., Willard
Grant Press, Boston (1975).

70.  Methods for Chemical Analysis of Water and Wastes, Environ-
mental  Monitoring  and  Support  Laboratory,   EPA-625/6-74-003a
USEPA, Cincinnati, OH (1976).

71.  Krocta,  H. and Lucas, R. L., "Information Required for the
Selection  and Performance Evaluation of Wet Scrubbers,"  Journal
of Pollution Control Association, 22, 6, 459.

72.  Pourbaix,  M.,   Atlas  of  Electrochemical  Equilibria  in
Aqueous  Solutions,  Pergamon  Press,  New York (1966)  cited  in
Development  Document  for  Interim  Final  Effluent  Limitations
Guidelines  and Proposed New Source Performance Standards for the
Primary  Copper Smelting Subcategory and Primary Copper  Refining
Subcategory,  EPA-440/l-75/032b,  Environmental Protection Agency
(February, 1975).

73.  Draft Development Document for Effluent Limitations  Guide-
lines  and New Source Performance Standards for the Miscellaneous
Nonferrous  Metals   Segment,   EPA-440/1-76/067,   Environmental
Protection Agency (March,  1977) citing Miller,  D. G., "Fluoride
Precipitation  in Metal Finishing Waste Effluent,"  Water-1974:I.
Industrial  Waste  Treatment,   American  Institute  of  Chemical
Engineers Symposium Series, 70, 144 (1974).

74.  Parker  and Fong,  "Fluoride Removal:   Technology and Cost
Estimates," Industrial Wastes  (November/December, 1975).

75.  Rohrer,  L.,  "Lime,  Calcium Chloride Beat Fluoride Waste-
water,"  Water and Wastes Engineering   (November,  1974),  p.  66
cited  in  Draft Development Document   for  Effluent  Limitations
Guidelines   and   New  Source  Performance  Standards  for   the
Miscellaneous   Nonferrous  Metals   Segment,   EPA-440/1-76/067,
Environmental Protection Agency  (March, 1977).

76.  Zabben,  W.  and Jewett,  H. W.,  "The Treatment of Fluoride
                               474

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - XV
Wastes," Proceedings of 22nd Industrial Waste Conference,
University  (May 2-4, 1967), pp. 706-716.
                                                           Purdue
77.  Manual  of  Treatment Techniques for  Meeting  the  Interim
Primary    Drinking    Water    Regulations,    EPA-600/8-77-005,
Environmental Protection Agency (April, 1978).
78.  Patterson,  J.W.
Pollution  Abatement,"
(1976).
                        "Technology  and Economics of Industrial
                        IIEQ  Document  #76/22  Project  #20.070A
79.  Maruyama,  T.,  Hannah,  S.  A.,  and Cohen,  J. M. , "Metal
Removal by Chemical Treatment Processes," Journal Water Pollution
Control Federation, 47, 5, 962.

80.  Gulp,  G.  L.  and  Gulp,  R.  L.,  New Concepts  in  Water
Purification,  (Van  Nostrand,  Reinhold  and Company,  New  York
(1974), pp. 222-224.

81.  Jenkins,  S.  N. , Knight, D. G., and Humphreys, R. E., "The
Solubility of Heavy Metal Hydroxides in Water, Sewage, and Sewage
Sludge,  I.   The Solubility of Some Metal Hydroxides,"  Interna-
tional Journal of Air and Water Pollution, 8, 537 (1964).
82.  Sittig,  M., Pollutant Removal Handbook.
Park Ridge, NJ  (1973).
                                               Noyes Data Corp.,
83.  Link,  W.  E.  and Rabosky,  J.  G., "Fluoride Removal from
Wastewater  Employing Calcium Precipitation and Iron Salt  Coagu-
lation,"  Proceedings  of the 31st Industrial  Waste  Conference,
Purdue University, pp. 485-500 (1976).

84.  Beychak, M. R., Aqueous Wastes from Petroleum and Petrochem-
ical  Plants,  John Wiley and Sons (1967) cited in Draft Develop-
ment Document for Effluent Limitations Guidelines and New  Source
Performance  Standards  for the Miscellaneous  Nonferrous  Metals
Segment,   EPA-440/1-76-067,   Environmental   Protection  Agency
(March, 1977).  '

85.  "Stripping,  Extraction,  Adsorption,  and  Ion  Exchange,"
Manual on Disposal of Refinery Wastes - Liquid  Wastes,  American
Petroleum  Institute,  Washington,  D.  C.  (1973) cited by Draft
Development Document for Effluent Limitations Guidelines and  New
Source  Performance  Standards for the  Miscellaneous  Nonferrous
Metals Segment, EPA-440/1-76/067, Environmental Protection Agency
(March, 1977).

86.  Grantz, R. G., "Stripper Performance Tied to NH3 Fixation,"
Oil and Gas Journal, 73, 24, 80 (1975) cited by Draft Development
Document  for  Effluent  Limitations Guidelines  and  New  Source
Performance  Standards  for the Miscellaneous  Nonferrous  Metals
Segment,   EPA-440/1-76/067,   Environmental   Protection  Agency
(March, 1977).

87.  Wrek,  W. J. and Snow, R. H., "Design to Cross Flow Cooling
                               475

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
Towers  and  Ammonia Stripping  Towers,"  Industrial  Engineering
Process Design Development,  11, 3 (1972) cited by Draft Develop-
ment  Document for Effluent Limitations Guidelines and New Source
Performance Standards for the Miscellaneous Metals Segment,  EPA-
440/1-76-067, Environmental Protection Agency (March, 1977).

88.  Mioderszewski,  D.,  "Ammonia Removal - What's Best," Water
and  Wastes Engineering (July,  1975) cited by Draft  Development
Document  for  Effluent  Limitations Guidelines  and  New  Source
Performance Standards for the Miscellaneous Metals Segment,  EPA-
440/1-76-067, Environmental Protection Agency (March, 1977).

89.  Schlauch,  R.  M.,  and Epstein,  A. C., Treatment to Metal
Finishing Wastes by Sulfide Precipitation, EPA 600/2-77-049.

90.  Coleman, R. T., Colley, D. J., Klausmeier, R. F., Malish, D.
A.,  Meserole,  N.  P.,  Micheletti, W. C., and Schwitzgebel, K.,
Draft  Copy  Treatment Methods for Acidic  Wastewater  Containing
Potentially Toxic Metal Compounds,  Report by Radian Corporation,
Austin,  TX, submitted to USEPA Industrial Environmental Research
Laboratory, Cincinnati, OH  (1978).

91.  Bettler,  C. R., "Lime Neutralization of Low-Acidity Waste-
water,"  Proceedings of 32nd Industrial Waste Conference,  Purdue
University (1977), p. 830.

92.  Permuitt Co.,  Inc.,  Proceedings of seminar on metal waste
treatment featuring the Sulfex process, Paramus, NJ, undated.

93.  Larson, H. P., Shou, K. P., Ross, L. W., "Chemical Treatment
of Metal Bearing Mine Drainage,"  Journal Water Pollution Control
Federation,  45, 8, 1682 (1974) cited by Coleman, R. T., et. al.,
Draft  Copy  Treatment Methods for Acidic  Wastewater  Containing
Potentially Toxic Metal Compounds,  Report by Radian Corporation,
Austin,  TX, submitted to USEPA Industrial Environmental Research
Laboratory, Cincinnati, OH  (1978).

94.  Murao,  K.  and Sei, N., "Recovery of Heavy Metals from the
Wastewater of Sulfuric Acid Process in Ahio Smelter," Proceedings
of  Joint  MMIJ  AIME Meeting on World Mining  and  Metallurgical
Technology,  Denver, September, 1976, Volume 2, pp. 808-16 (1976)
cited by Coleman,  R.  T.,  et. al., Draft Copy Treatment Methods
for   Acidic  Wastewater  Containing  Potentially   Toxic   Metal
Compounds, Report by Radian Corporation, Austin, TX, submitted to
USEPA  Industrial Environmental Research Laboratory,  Cincinnati,
OH (1978).

95.  LaPerle,  R.  L.,  "Removal  of  Metals  from  Photographic
Effluent by Sodium Sulfide Precipitation," Journal Appl. Photogr.
Eng.  2, 134, (1976) cited by Coleman, R. T., et. al., Draft Copy
Treatment  Methods for Acidic Wastewater  Containing  Potentially
Toxic Metal Compounds,  Report by Radian Corporation, Austin, TX,
submitted  to USEPA Industrial Environmental Research Laboratory,
Cincinnati, OH (1978).
                               476

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XV
 96.  Scott,  M. (Senior Marketing Specialist, Permutit Company),
 Private communications with R.  Klausmeier (November, 1977) cited
 by^Coleman,  R.  T.,  et.  al.,  Draft Copy Treatment Methods for
 Acidic  Wastewater Containing Potentially Toxic Metal  Compounds,
 Report  by Radian Corporation,  Austin,  TX,  submitted to  USEPA
 Industrial  Environmental  Research  Laboratory,  Cincinnati,  OH
 (1978) .

 97.  Development Document for Interim Final and Proposed Effluent
 Limitations  Guidelines and New Source Performance Standards  for
 the Ore Mining and Dressing Industry,  EPA-440/1-75-061, Environ-
 mental Protection Agency (1975) cited by Coleman, R. T., et. al.,
 Draft  Copy  Treatment Methods for Acidic  Wastewater  Containing
 Potentially Toxic Metal Compounds,  Report by Radian Corporation
 Austin,  TX, submitted to USEPA Industrial Environmental Research
 Laboratory, Cincinnati, OH (1978).

 98.  Coleman,  R.  T.  and Malish, D. A.,  Trip Report to Paul Bergoe
 and Son,  Boliden Aktiebolag and Outokumpu as  part to EPA Contract
 68-02-2608, Radian Corporation (November, 1977)  cited by Coleman,
 R.   T.,   et.  al.,  Dragt Copy Treatment Methods  for Acidic Waste-
 water  Containing  Potentially Toxic Metal  Compounds,  Report  by
 Radian Corporation,   Austin,   TX,  submitted to USEPA Industrial
 Environmental  Research Laboratory, Cincinnati, OH (1978).

 99.   Maltson,   M.   E.,  "Membrane Desalting Gets  Big Push," Water
 and Wastes  Engineering (April,  1975), p.  35.
 100. Cruver,  J.  E.,   "Reverse Osmosis  for Water Reuse,"
 Environmental System  (June,  1973).
               Gulf
 101.  "Water  Renovation  of  Municipal  Effluents  by  Reverse
 Osmosis," Gulf Oil Corporation, San Diego  (February, 1972).

 102.  Spatz, D. D., "Methods of Water Purification," Presented to
 the  American Association of Nephrology Nurses and Technicians at
 the  ASAIO AANNT Joint Conference,  Seattle,  Washington   (April,
 j- y / £ / •
103.  Donnelly,  R. G., Goldsmith, R. L., McNulty, K. J. , Grant,
D. C., and Tan, M. , Treatment to Electroplating Wastes by Reverse
Osmosis,   EPA-600/2-76-261,   Environmental  Protection   Aqencv
(September, 1976).                                          ^   •*
104.  Rook,  J.  J.,  "Haloforms  in  Drinking  Water,"  Journal
American Water Works Association, 68:3:168 (1976).

105.  Rook, J. J., "Formation to Haloforms During Chlorination of
Natural  Waters,"  Journal Water  Treatment  Examination,  23:234
( iy 74 ) . .

106.  Trussell,  R.  R,   and Umphres,  M.  D., "The Formation of
Trihalomethanes,"   Journal  American  Water  Works   Association
70:11:604 (1978).
                               477

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           GENERAL DEVELOPMENT DOCUMENT
                   SECT - XV
107.  Nebel, C., Goltschlintg, R. D., Holmes, J. L., and Unangst,
p.  C.,  "Ozone  Oxidation of Phenolic Effluents," Proceedings of
the 31st Industrial Waste Conference,  Purdue University  (1976),
pp. 940-951.

108.  Rosen, H  M., "Wastewater Ozonation:  a Process Whose Time
Has Come," Civil Engineering, 47, 11, 65 (1976).

109.  Hardisty,  D.  M. and Rosen, H. M., "Industrial Wastewater
Ozonation," Proceedings of the 32nd Industrial Waste  Conference,
Purdue University (1976), pp. 940-951.

110.  Traces  of  Heavy  Metals in Water Removal  Processes  and
Monitoring,  EPA-902/9-74-D01,  Environmental  Protection  Agency
(November, 1973).

111.  Symons,  J.  M.,  "Interim Treatment Guide for Controlling
Organic  Contaminants in Drinking Water Using Granular  Activated
Carbon," Water Supply Research Division,  Municipal Environmental
Research Laboratory,  Office of Research and Development,  USEPA,
Cincinnati, OH  (January, 1978).

112.  McCreary,  J.  J.  and V. L. Snoeyink, "Granular Activated
Carbon   in  Water  Treatment,"  Journal  American  Water   Works
Association, 69, 8, 437 (1977).

113.  Grieves,  C.  G.  and Stevenson,  M. K.,  "Activated Carbon
Improves Effluents," Industrial Wastes  (July/August,  1977),  pp.
30-35.

114.  Beebe,  R. L. and Stevens, J.  I.,  "Activated  Carbon System
for   Wastewater   Renovation,"  Water  and  Wastes   Engineering
(January,  1967), pp. 43-45.

115.  Gulp, G. L. and Shuckrow, A. J.,  "What lies ahead  for PAC,"
Water and  Wastes Engineering  (February,  1977),  pp.  67-72, 74.

116.  Savinelli, E. A. and Black, A.  P.,  "Defluoridation of Water
With   Activated   Alumina,"   Journal   American   Water   Works
Association, 50, 1, 33  (1958).

117.  Paulson,  E.  G.,   "Reducing Fluoride  in  Industrial Waste-
water," Chemical Engineering,  Deskbook  Issue  (October 17, 1977).

118.  Bishop,   P.  L.  and Sansovey,  G.,  "Fluoride Removal from
Drinking   Water  by  Fluidized  Activated  Alumina   Adsorption,"
Journal American Water Works  Association,  70,10,554 (1978).

119.  Harmon,   J.  A.  and Kalichman,   S.  G.,  "Defluoridation of
Drinking   Water   in Southern  California,"  Journal  American  Water
Works Association, 57:2:245  (1965).
 120.   Maier,   F.   J.,
 Works, 91:90  (1960).
"Partial Defluoridation of Water," Public
                                478

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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - XV
121.  Bellack, E.,  "Arsenic Removal from Potable Water," Journal
American Water Works Association, 63, 7 (1971).

122.  Gupta,  S. K. and Chen, K. Y., "Arsenic Removal by Adsorp-
tion," Journal Water Pollution Control Association  (March, 1978),
pp. 493-506.

123.  Johnson,  D.  E. L., "Reverse Osmosis Recycling System for
Government Arsenal," American Metal Market (July 31,  1973) cited
in Draft Development Document for Effluent Limitations Guidelines
and  New  Source  Performance  Standards  for  the  Miscellaneous
Nonferrous  Metals   Segment,   EPA-440/1-76-067,   Environmental
Protection Agency (March, 1977).

124.  Nachod,  F.  C. and Schubert, J., Ion Exchange Technology,
Academic Press, Inc. (1956).

125.  Volkert,  David,  and Associates, "Monograph on the Effec-
tiveness and Cost of Water Treatment Processes for the Removal of
Specific  Contaminants," EPA 68-01-1833,  Office of Air and Water
(1974) cited by Contaminants Associated with Direct and  Indirect
Reuse of Municipal Wastewater, EPA-600/1-78-019 (March, 1978).

126.  Clark,  J.  W.,  Viessman,  W., Jr., and Hammer, M., Water
Supply and Pollution Control, (3rd ed.) IEP, New York (1977).

127.  AWARE (Associated Water and Air Resources Engineers, Inc.),
Analysis  to National Industrial Water Pollution Control  Costs,"
(May 21, 1973) .

128.  AWARE,  "Alternatives for Managing Wastewater in the Three
Rivers Watershed Area," (October, 1972).

129.  Bechtel,  "A  Guide  to  the Selection  of  Cost-Effective
Wastewater Treatment Systems," EPA 430/9-75-002 (July, 1975).

130.  Smith  R., "Cost of Conventional and Advanced Treatment of
Wastewater," Journal Water Pollution Control Federation,  40,  9,
1546 (1968).

131.  Icarus,  "Capital and Operating Costs of Pollution Control
Equipment  Modules," Vols.  I and II,  EPA-R5-73-023a & b  (July,
1973).

132.  Monti,  R.  P.  and Silberman,  P.  T.,  "Wastewater System
Alternatives:   What Are They .   .   .  and What Cost," Water  and
Waste Engineering (May, 1974), p. 40.

133.  Process Design Manual for  Removal of Suspended Solids, EPA-
625/175-003a (January,  1975).
134.  Process Design Manual for Carbon Adsorption, EPA
71-002a (October, 1973).
                                                          625/1-


135.   Grits,  G.  J.,  "Economic  Factors  in Water  Treatment,"
                               479

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
Industrial Water Engineering (November, 1971), p. 22.

136.  Barnard, J. L. and Eckenfelder, W. W., Jr., "Treatment Cost
Relationships for Industrial Waste Treatment,  Environmental  and
Water Resources Engineering, Vanderbilt University (1971).

137.  Grits,  G.  J.  and Glover,  G.  G.,  "Cooling Slowdown in
Cooling Towers,"  Water and Wastes Engineering (April,  1975), p.
45.

138.  Kremen,  S.  S.,  "The  True  Cost  of  Reverse  Osmosis,"
Industrial Wastes (November/December, 1973), p. 24.

139.  Cruver,  J.  E. and Sleigh, J. H.,  "Reverse Osmosis - The
Emerging  Answer  to  Seawater  Desalination,"  Industrial  Water
Engineering (June/July, 1976), p. 9.

140.  Doud,  D.  H., "Field Experience with Five Reverse Osmosis
Plants," Water and Sewage Works (June, 1976), p. 96.

141.  Lacey,  R. E. and Loed, S., (eds.), "Industrial Processing
with Membranes," in The Cost of Reverse Osmosis,  John Wiley  and
Sons (1972).

142.  Disposal  of  Brines Produced in Renovation of  Industrial
Wastewater, FWPA Contract #14-12-492 (May, 1970).

143.  Process  Design Manual for Sludge Treatment and  Disposal,
EPA 625/1-74-006 (October, 1974).

144.  Black & Veatch, "Estimating Cost and Manpower Requirements
for  Conventional Wastewater Treatment Facilities," EPA  Contract
#14-12-462  (October, 1971).

145.  Osmonics,  Inc.,  "Reverse  Osmosis  and  Ultrafiltration
Systems Bulletin No. G7606," (1978).

146.  Buckley,  J.  D.,  "Reverse Osmosis  Moving from Theory.to
Practice,"" From Fluid Systems  Div.,  UOP,  Inc.  (Reprint  from
Consulting Engineer), 45, 5, 55 (1975).

147.  Process Design Manual for Nitrogen Control, EPA-Technology
Transfer  (October, 1975).

148.  Rizzo  and Shepherd,  "Treating Industrial Wastewater with
Activated Carbon," Chemical Engineering  (January 3, 1977).

149.  Richardson,   "1978-79  Process  Equipment,"  Vol.  4  of
Richardson Rapid System.

150.  Thiansky, D. P., "Historical Development of Water Pollution
Control   Cost  Functions,"  Journal  Water   Pollution   Control
Federation, 46, 5, 813 (1974).

151.  Zimmerman, O. T., "Wastewater Treatment," Cost Engineering
                               480

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XV
 (October,  1971),  p.  11.

 152.   Watson,   I.  C.,   (Control   Research,   Inc.)   "Manual   for
 Calculation of  Conventional  Water  Treatment Costs,"   Office  of
 Saline Water  (March,  1972).

 153.   Gulp,  R.   L.,  Wesner,   G.  M.,   Gulp,  G.  L., Handbook of
 Advanced Wastewater  Treatment,  McGraw Hill  (1978).

 154.   Dynatech  R/D  Company,   A Survey  of Alternate Methods   for
 Cooling Condenser   Discharge   Water Large-Scale  Heat  Rejection
 Equipment,  EPA  Project No. 16130 DHS (July,  1969).

 155.   Development Document for  Steam Electric Power  Generating,
 EPA 440/1-73/029  (March,  1974).

 156.   "Cooling   Towers   - Special   Report,"   Industrial  Water
 Engineering (May, 1970).

 157.   AFL  Industries, Inc.,  "Product Bulletin  #12-05.Bl (Shelter
 Uses)," Chicago, IL  (December  29,  1977).

 158.   Fisher Scientific Co., Catalog 77  (1977).

 159.   Isco,  Inc.,  Purchase  Order  Form,  Wastewater  Samplers
 (1977).

 160.   Dames & Moore,  Construction Cost  for Municipal Wastewater
 Treatment Plants:   1973-1977,  EPA-430/9-77-013, MCD-37 (January,
 1978).

 161.   Metcalf & Eddy, Inc., Wastewater Engineering:  Collection,
 Treatment, Disposal, McGraw-Hill, New York (1972).

 162.   Obert,  E. F. and Young, R. L., Elements of Thermodynamics
 and Heat Transfer, McGraw-Hill  (1962), p. 270.

 163.   Paulson,  E.  G.,   "How  to  Get Rid of  Toxic  Organics,"
 Chemical Engineering,  Deskbook Issue (October 17, 1977),  pp. 21-
 ^ / •

 164.   CH2-M-Hill,  "Estimating Staffing for Municipal Wastewater
 Treatment Facilities," EPA #68-01-0328 (March, 1973).

 165.   "EPA Indexes Reflect Easing Costs," Engineering News Record
 (December 23,  1976),  p. 87.

 166.  Chemical Marketing Reporter,   Vol.  210, 10-26 (December 6
and December 20, 1976).

 167.  Smith, J.  E.,  "Inventory of Energy Use in Wastewater Sludge
Treatment    and   Disposal,"   Industrial   Water    Engineering
 (July/August,  1977).

168.  Jones,  J.  L.,  Bomberger,   D. C., Jr.,'and Lewis,  F.  M.,
                               481

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
"Energy Usage and Recovery in Sludge Disposal, Parts 1 & 2, "Water
and Sewage Works (July and August, 1977), pp. 44-47 and 42-46.

169.  Hagen,  R. M. and Roberts, E. B.-, "Energy Requirements for
Wastewater Treatment,  Part 2," Water and Sewage Works (December,
1976), p. 52.

170.  Banersi, S. K. and O'Conner, J. T., "Designing More Energy
Efficient   Wastewater  Treatment  Plants,"   Civil   Engineering
(September, 1977),'p. 76.

171.  "Electrical  Power  Consumption for  Municipal  Wastewater
Treatment," EPA-R2-73-281 (1973).

172.  Hillmer, T. J., Jr., "Economics of Transporting Wastewater
Sludge," Public Works (September, 1977), p. 110.

173.  Ettlich, W. F., "Economics of Transport Methods of Sludge."
Proceedings  of  the Third National Conference on Sludge  Manage-
ment, Disposal and Utilization  (December 14-16, 1976), pp. 7-14.

174.  NUS/Rice  Laboratory,  "Sampling Prices,"  Pittsburgh,  PA
(1978) .

175.  WARF  Instruments,  Inc.,  "Pricing Lists  and  Policies,"
Madison, WI (June, 15, 1973).

176.  Orlando  Laboratories,  Inc.,  "Service  Brochure and  Fee
Schedule #16," Orlando, FL (January 1, 1978).

177.  St.  Louis  Testing  Laboratory,  "Water  and  Wastewater
Analysis - Fee Schedule," St. Louis, MO (August, 1976).

178.  Ecology Audits,  Inc.,  "Laboratory Services  - Individual
Component Analysis," Dallas, TX  (August, 1976).

179.  Laclede  Gas  Company,  (Lab  Div.),   "Laboratory  Pricing
Schedule," St. Louis, MO  (August, 1977).

180.  Industrial Testing Lab,   Inc., "Price List," St. Louis, MO
(October, 1975).

181.  Luther,  P.  A.,  Kennedy,  D.  C.,  and Edgerley, E., Jr.
"Treatability   and  Functional  Design  of  a  Physical-Chemical
Wastewater  Treatment System for a Printing  and  Photodeveloping
Plant,"  31st  Purdue Industrial Waste  Conference,  pp.  876-884
(1976).

182.  Hindin,  E.  and Bennett,  P.  J.,  "Water Reclamation  by
Reverse Osmosis," Water and Sewage Works,  116,  2, 66  (February,
1969).

183.  Cruver,  J.  E.  and Nusbaum,  I., "Application of Reverse
Osmosis to Wastewater Treatment," Journal Water Pollution Control
Association,  476,  2, 301  (February, 1974).
                               482

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XV
184.  Cruver,  J. E., "Reverse Osmosis - Where It Stands Today,"
Water and Sewage Works, 120, 10, 74 (October, 1973).

185.  Vanderborght,  B. M. and Vangrieken, R. E., "Enrichment of
Trace  Metals  by  Adsorption  on  Activated  Carbon,"  Analytic
Chemistry, 49, 2, 311 (February, 1977).

186.  Hannah,  S.  A., "Jelus, by Physical and Chemical Treatment
Processes," Journal Water Pollution Control Federation,  50,  11,
2297 (1978).

187.  Argo,  D.  G.  and Gulp,  G.  L., "Heavy Metals Removed in
Wastewater Treatment Processes - Parts 1 and 2," Water and Sewage
Works, August, 1972, pp. 62-65, and September, 1972, pp. 128-132.

188.  Hager, D. G., "Industrial Wastewater Treatment by Granular
Activated  Carbon,"  Industrial  Water  Engineering,   pp.  14-28
(January/February,   1974)  189.    Rohrer,   K.   L.,  "Chemical
Precipitants  for  Lead-Bearing  Wastewaters,"  Industrial  Water
Engineering, 12, 3 13 (1975).

189.  Brody,  M.  A.  and Lumpkins, R. J., "Performance of Dual-
Media Filters," Chemical Engineering Progress (April, 1977).

190.  Bernardin, F. E., "Cyanide Detoxification Using Absorption
and   Catalytic  Oxidation,"  Journal  Water  Pollution   Control
Federation, 45, 2 (February, 1973).

191.  Russel, D. L., "PCB's:  The Problem Surrounding Us and What
Must be Done," Pollution Engineering (August, 1977).

192.  Chriswell,  C.  D., et. al., "Comparison of Macroreticular
Resin  and Activated Carbon as Sorbents," Journal American  Water
Works Association (December, 1977).

193.  Gehm, H. W. and Bregman, J. I., Handbook of- Water Resources
and Pollution Control, Van Nostrand -Reinhold Company (1976).

194.  Considine,   Douglas  M.,   Energy  Technology  Handbook,
McGraw-Hill Book Company, New York, c.1977, pp. 5-173-5-181.

195.  Absalom,  Sandra T.,  Boron,  U.S.  Dept. of the Interior,
Bureau of Mines, Washington, D.C., May, 1979.

196.  Rathen,  John A.,  Antimony,  U.S. Dept. to the Interior,
Bureau of Mines, Washington, D.C., June, 1979.

197.  Harris,  Keith L.,  Cesium,  U.S.  Dept.  of the Interior,
Bureau of Mines, Washington, D.C., May, 1979.
                               483

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GENERAL DEVELOPMENT DOCUMENT    SECT - XV
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                   484

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            GENERAL DEVELOPMENT DOCUMENT
SECT - XVI
                            SECTION XVI

                             GLOSSARY
 This section is  an  alphabetical  listing  to  technical  terms   (with
 definitions)   used  in  this  document  which may  not be  familiar   to
 the   reader.

 4-AAP Colorimetric  Method

 An   analytical  method for  total phenols and total phenolic  com-
 pounds that  involves reaction with the color developing agent   4-
 aminoantipyrine.

 Acidity

 The   quantitative   capacity  to aqueous solutions to  react  with
 hydroxyl   ions.   It   is measured by titration  with  a  standard
 solution   to   a  base  to a specified end point,  and  is  usually
 expressed  as milligrams per liter to calcium carbonate.

 The  Act

 The   Federal   Water Pollution Control Act Amendments of  1972   as
 amended by the Clean Water Act to 1977 (PL  92-500).

 Amortization

 The   allocation  of a  cost or account according  to  a  specified
 schedule,  based  on the principal,  interest and period of  cost
 allocation.

 Analytical Quantification Level

 The  minimum concentration at which quantification of a specified
 pollutant  can  be reliably measured.

 Anglesite

 A mineral occurring in crystalline form or as a compact mass.

Antimonial Lead

An alloy composed of lead and up to 25 percent antimony.

Backwashinq

The  operation  of cleaning a filter  or column by  reversing  the
 flow  of  liquid  through it and washing  out  matter  previously
 trapped.
                               485

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XVI
Baghouses

The area for housing bag type air filters, an air pollution control
equipment device.
Ball Mill

Pulverizing equipment for the grinding of raw material
is done by steel balls, pebbles, or rods.

Barton Process
              Grinding
A  process  for  making  lead  oxide to  be  used  in  lead  acid
batteries.   Molten lead is fed, agitated, and stirred in  a  pot
with the resulting fine droplets oxidized.  Material is collected
in  a settling chamber where crystalline varieties of lead  oxide
are formed.

Batch Treatment

A  waste  treatment method where wastewater is collected  over  a
period of time and then treated prior to discharge.  Treatment is
not continuous, but collection may be continuous.

Bench Scale Pilot Studies

Experiments  providing  data  concerning the  treatability  of  a
wastewater  stream or the efficiency of a treatment process  con-
ducted using laboratory-size equipment.

Best Available Demonstrated Technology  (BDT)

Treatment technology upon which new source performance  standards
are to be based as defined by Section 306 to the Act.

Best Available Technology Economically Achievable  (BAT)

The   selected  technology  applicable  to  control   toxic   and
nonconventional  pollutants  on  which effluent  limitations  are
established.   These  limitations are to be achieved by  July  1,
1984  by  industrial discharges to surface waters  as  defined  by
Section 301(b)(2)(C) of the Act.

Best Conventional Pollutant Control Technology  (BCT)

The   selected  technology  applicable  to  control  conventional
pollutants used to develop effluent limitations  to be achieved by
July  1,  1984  for industrial discharges to  surface  waters  as
defined in Section 301(b)(2)(E) of the Act.

Best Management Practices  (BMP)

Regulations  intended to control the release of  toxic and hazard-
ous pollutants from plant  runoff,  spillage,  leaks,  solid waste
disposal, and drainage from raw material storage.
                                486

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           GENERAL DEVELOPMENT  DOCUMENT
SECT - XVI
 Best  Practicable Control Technology Currently Available  (BPT)

 The   selected  technology applicable to develop  effluent  limita-
 tions  to  have been achieved by July 1,  1977  (originally)  for
 industrial  discharges  to surface waters as defined  by  Section
 301(b)(l)(A) of the Act.

 Betterton Process

 A  process used to remove bismuth from lead by adding calcium and
 magnesium.   These compounds precipitate the bismuth which floats
 to  the top of the molten bath where it can be skimmed  from  the
 molten  metal.

 Billet

 A  long,  round  slender  cast product used as  raw  material  in
 subsequent forming operations.

 Biochemical Oxygen Demand (BOD)

 The   quantity  of  oxygen used in the  biochemical  oxidation  of
 organic matter under specified conditions for a specified time.

 Blast Furnace

 A furnace for smelting ore concentrates.   Heated air is blown in
 at the  bottom to the furnace, producing changes in the combustion
 rate.

 Blister Copper

 Copper  with 96 to 99 percent purity and appearing blistered; made
 by forcing air through molten copper matte.

 Slowdown

 The  minimum discharge to circulating water from a unit operation
 such  as  a  scrubber for the purpose  of  discharging  dissolved
 solids  or other contaminants contained in the water,  the further
 buildup  of which would cause concentration in amounts  exceeding
 limits  established by best engineering practice.

 Building Block

 The  smallest  sub-unit or segment of a subcategory for  which  a
 specific effluent limitation is established.  Building blocks are
 directly usable in defining the processes used in a plant and  in
 developing the discharge allowances for that plant.
Calcining

Heating  to  a high temperature without fusing so
material or make other changes.
       as   to   remove
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           GENERAL DEVELOPMENT DOCUMENT
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Carbon Reduction

The  process of using the carbon of coke as a reducing agent  in
the blast furnace.

Cementation

A  process  in which metal is added to a solution to initiate  the
precipitation of another metal.   For example,  iron may be added
to a copper sulfate solution to precipitate Cu:

             -F Cu +
Cerussite

A  mineral  occurring  in  crystalline form  and  made  of  lead
carbonate.

Charge

Material that has been melted by being placed inside a furnace.

Charging Scrap

Scrap material put into a furnace for melting.

Chelation

The  formation  to coordinate covalent bonds  between  a  central
metal  ion and a liquid that contains two or more sites for  com-
bination with the metal ion.

Chemical Oxygen Demand (COD)

A  measure  of the oxygen-consuming capacity to the  organic  and
inorganic matter present in the water or wastewater.

Cold-Crucible Arc Melting

Melting  and purification of metal in a cold refractory vessel or
pot.

Colloid

Suspended  solids whose diameter may vary between less  than  one
micron and fifteen microns.

Composite Samples

A  series of samples collected over a period of time but combined
into a single sample for analysis.  The individual samples can be
taken  after a specified amount of time has passed  (time  compo-
sited) ,  or after a specified volume of water has passed the sam-
pling  point (flow composited).   The sample can be automatically
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 collected   and   composited   by   a   sampler   or   can   be  manually
 collected  and combined.

 Consent  Decree  (Settlement Agreement)

 Agreement  between EPA and various  environmental  groups,  as  insti-
 tuted  by   the  United States District Court  for  the   District   of
 Columbia,   directing EPA to  study  and promulgate regulations   for
 the  toxic  pollutants (NRDC,  Inc.   v.  Train,  8 ERC  2120  (D.D.C.
 1976), modified March 9, 1979,  12  ERC 1833,  1841).

 Contact  Water

 Any  water  or oil that comes into  direct contact with the   metal,
 whether  it  is raw material,  intermediate product, waste product,
 or finished product.

 Continuous  Casting

 A casting process that produces  sheet,  rod, or  other  long  shapes
 by   solidifying the  metal  while  it is being poured   through   an
 open-ended  mold using little or  no contact cooling water.   Thus,
 no restrictions are placed on the  length of  the  product  and it  is
 not  necessary to stop the process  to remove  the  cast  product.

 Continuous  Treatment

 Treatment   of   waste streams operating  without   interruption   as
 opposed  to  batch  treatment.   Sometimes referred to   as  flow-
 through  treatment.                 ,  .

 Contractor Removal
Disposal
firm.
of oils,  spent solutions,  or sludge by  a  commercial
Conventional Pollutants

Constituents  of wastewater as determined by Section 304(a)(4) of
the  Act,  including but not limited to pollutants classified  as
biological-oxygen-demanding>  oil and grease,  suspended,  solids,
fecal coliforms, and pH.

Converting

The  process  of  blowing  air through molten  metal  to  oxidize
impurities.

Cooling Tower

A  hollow,  vertical structure with internal baffles designed  to
break up falling water'so that it is cooled by upward-flowing air
and the evaporation of water.
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           GENERAL DEVELOPMENT DOCUMENT
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Copper Matte

An impure sulfide mixture formed by smelting the sulfide ores  in
copper.

Cupelled

Refined  by means of a small shallow porous bone cup that is used
in assaying precious metals.

Cupola Furnace

A  vertical cylindrical furnace for melting materials on a  small
scale.   This  furnace is similar to a reverberatory furnace  but
only on a smaller scale.

Cyclones

A  funnel-shaped  device for removing particulates  from  air  or
other fluids by centrifugal means.

Data Collection Portfolio (dcp)

The  questionnaire  used in the survey of the  nonferrous  metals
manufacturing industry.

Degassing

The  removal of dissolved hydrogen from the molten metal prior to
casting.  This process also helps to remove oxides and impurities
from the melt.

Direct Chill Casting  s

A  method  of  casting where the molten metal is  poured  into  a
water-cooled  mold.   The  base  of this mold is  the  top  of  a
hydraulic  cylinder  that lowers the aluminum first  through  the
mold and then through a. water spray and bath to cause solidifica-
tion.  The vertical distance of the drop limits the length of the
ingot.  This process is also known as semi-continuous casting.

Direct Discharger

Any point source that discharges to a surface water.

Pore

Gold  and  silver bullion remaining in a cupelling furnace  after
oxidized lead is removed.

Dross

Oxidized impurities occurring on the surface of molten metal.
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           GENERAL DEVELOPMENT DOCUMENT
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Drying Beds

Areas for dewatering of sludge by evaporation and seepage.

Effluent

Discharge from a point source.

Effluent Limitation

Any standard (including schedules of compliance) established by a
state or EPA on quantities,  rates,  and concentrations of chemi-
cal,  physical,  biological, and other constituents that are dis-
charged from point sources into navigable waters,  the waters  of
the contiguous zone, or the ocean.

Electrolysis

A  method  of  producing chemical reactions by  sending  electric
current through electrolytes or molten salt.

Electrolytic Refining

A purification process in which metals undergo electrolysis.

Electrolytic Slime

Insoluble  impurities removed from the bottom of an  electrolytic
cell during electrolytic refining.

Electron Beam Melting

A melting process in which an electron beam is used as a  heating
source.

Electrostatic Precipitator  (ESP)

A  gas  cleaning  device that induces an electrical charge  on  a
solid  particle which is then attracted to an oppositely  charged
collector  plate.    The  collector  plates  are   intermittently
vibrated to discharge the collected dust to a hopper.

End-of-Pipe Treatment

The reduction of pollutants by wastewater treatment prior to dis-
charge or reuse.

Film Stripping

Separation  of  silver-bearing material from  scrap  photographic
film.
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 Fluid Bed Roaster

 A  type  of  roaster in which the material is  suspended  in  air
 during roasting.

 Fluxes

 Substances  added  to molten metal to help remove impurities  and
 prevent excessive oxidation, or  promote the fusing of the metals.

 Galena

 A bluish gray mineral occurring  in the form of  crystals,   masses,
 or grains;   it constitutes  the principal ore of lead.
 Gangue

 Valueless  rock  and mineral mined  with  ore.
 ore,  the material is  known as  "slag."

 Gas Chromatography/Mass  Spectroscopy  (GC/MS)
  When  separated  from
Chemical analytical  instrumentation used  for quantitative  organic
analysis.

Grab Sample

A  single  sample of wastewater taken without  regard  to  time  or
flow.

Hardeners

Master alloys that are added to a melt to control hardness.

Harris Process

A  process in which sodium hydroxide and sodium nitrate are added
to molten lead to soften or refine it.  These ,.two compounds react
with impurities in the molten metal forming a  slag that floats to
the top  of the molten metal.

Humidification Chamber

A chamber in which the water vapor content of  a gas is increased.

Hydrogenation

The addition of hydrogen to a molecule.

Hydrometallurgical

The use of wet processes to treat metals.
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           GENERAL DEVELOPMENT DOCUMENT
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Indirect Discharger

Any  point source that discharges to a publicly  owned  treatment
works.

Inductively-Coupled Argon Plasma Spectrophotometer (ICAP)

A laboratory device used for the analysis of metals.

Ingot

A large, block-shaped casting produced by various methods. Ingots
are intermediate products from which other products are made.

In-Process Control Technology

Any  procedure or equipment used to conserve chemicals and  water
throughout the production operations, resulting in a reduction of
the wastewater volume.

Litharge                                        «

A  yellowish  lead oxide compound with a crystalline  form;  also
known as lead monoxide.

Matte

A metal sulfide mixture produced by smelting sulfide ores.

Mischmetal

A  rare  earth metal alloy comprised of 94 to 99 percent  of  the
natural  mixture of rare earth metals.   The balance of the alloy
includes traces of other elements and 1 to 2 percent iron.

Mitsubishi Process

A  process  used in primary copper  refining  which  incorporates
three furnaces to combine roasting, smelting, and converting into
one  continuous  process.   The  Mitsubishi  process  results  in
reduced smelting rates and heating costs.

New Source Performance Standards (NSPS)

Effluent  limitations for new industrial point sources as defined
by Section 306 of the Act.

Nonconventional Pollutant

Parameters  selected  for use in performance standards  that  have
not  been  previously designated as either conventional or   toxic
pollutants.
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            GENERAL DEVELOPMENT DOCUMENT
SECT - XVI
 Non-Water Quality Environmental Impact

 The_ecological impact as a result to solid,  air, or thermal pol-
 lution due to the application to various wastewater  technologies
 to achieve the effluent guidelines limitations.    Also associated
 with  the non-water quality aspect is the energy impact of waste-
 water treatment.

 NPDES Permits

 Permits  issued  by EPA or an approved state  program  under  the
 National  Pollutant  Discharge Elimination System as required  by
 the Clean Water Act.

 Off-Gases

 Gases,   vapors, and fumes produced as a result of a metal forming
 operation.

 Oil and Grease (O&G)

 Any  material that  is extracted by freon from an acidified sample
 and that is  not volatilized during the analysis,   such as  hydro-
 carbons, fatty acids, soaps,  fats, waxes,  and oils.

 Outokumpu Furnace
A  furnace  used  for  flash  smelting,   in which hot  sulfide  concen-
trate   is fed  into a reaction  shaft along with preheated air   and
fluxes.   The  concentrate roasts and smelts itself  in  a   single
autogeneous process.
Parke's Process

A_process in which zinc is added to molten lead to form insoluble
zinc-gold  and zinc-silver compounds.   The compounds are skimmed
and the zinc is removed through-vacuum de-zincing.

Pelletized

An  agglomeration  process  in which an unbaked  pellet  is  heat
hardened.   The  pellets increase the reduction rate in  a  blast
furnace by improving permeability and gas-solid contact.

El

The  pH is the negative logarithm of the hydrogen ion activity of
a solution.

Platinum Group Metals

A  name  given  to  a group  of  metals  comprised  of  platinum,
palladium, rhodium, iridium,  osmium, and ruthenium.
                               494

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           GENERAL DEVELOPMENT DOCUMENT
SECT - XVI
Pollutant Parameters

Those  constituents  of wastewater determined to  be  detrimental
and, therefore, requiring control.

Precious Metals

A generic term referring to the elements gold,  silver, platinum,
palladium, rhodium, iridium, osmium, and ruthenium as a group.

Precipitation Supernatent

A liquid or fluid forming a layer above precipitated solids.

Priority Pollutants

Those  pollutants  included in Table 2 of Committee Print  number
95-30 of the "Committee on Public Works and Transportation of the
House of Representatives," subject to the Act.

Process Water

Water used in a production process that contacts the product, raw
materials, or reagents.

Production Normalizing Parameter  (PNP)

The  unit  to  production specified in the  regulations  used  to
determine  the  mass  of  pollution  a  production  facility  may
discharge.
PSES

Pretreatment   standards  (effluent  regulations)  for
sources applicable to indirect dischargers.

PSNS
              existing
Pretreatment  standards  (effluent regulations) for  new  sources
applicable to new indirect dischargers.

Publicly Owned Treatment Works (POTW)

A  waste  treatment  facility  that  is  owned  by  a  state   or
municipality.

Pug Mill

A  machine  for  mixing and tempering a plastic material  by  the
action to blades revolving in a drum or trough.
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           GENERAL  DEVELOPMENT  DOCUMENT
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Pyrometallurgical

The use to high-temperature processes  to  treat metals.

Raffinate

Undissolved liquid mixture not  removed during solvent refining.

Rare Earth Metals

A name given to a group of elements  including scandium,  yttrium,
and lanthanum to lutetium, inclusive.

Recycle

Returning treated or untreated  wastewater to the production  pro-
cess from which it originated for use  as process water.

Reduction

A  reaction  in  which there is a decrease in  valence  resulting
from a gain in electrons.

Reuse                         ....  ...;.'.

The use of treated or untreated process wastewater in a different
production process.

Reverberatory Furnaces                     :

Rectangular furnaces in which the fuel  is burned above the  metal
and the heat reflects off the walls and into the metal.

Roasting                        .....-.,     ,

Heating  ore to remove impurities prior to smelting.   Impurities
within  the  ore are oxidized and leave the  furnace  in  gaseous
form.

Rod                              ,  "•

An  intermediate  metal  product  having  a  solid,  round  cross
section 9.5 mm (3/8 inches) or more in diameter.

Rotary Furnace

A circular furnace which rotates the workpiece around the axis of
the furnace during heat treatment.

Scrubber Liquor

The  untreated wastewater stream produced by wet scrubbers clean-
ing gases produced by metal manufacturing operations.
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           GENERAL DEVELOPMENT DOCUMENT
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Shot Casting

A  method  of  casting in which molten metal  is  poured  into  a
vibrating  feeder,  where  droplets  of molten metal  are  formed
through perforated openings.  The droplets are cooled in a quench
tank.

Sintering

The  process  of forming a bonded mass by heating  metal  powders
without melting.

Skimmings

Slag removed from the surface of smelted metal.

Slag

The product of fluxes and impurities resulting from the smelting
of metal.

Smelting

The process of heating ore mixtures to separate liquid metal and
impurities.

Soft Lead

Lead produced by the removal of antimony through oxidation.  The
lead is characterized by low hardness and strength.

Spent Hypo Solution

A solution consisting of photographic film fixing bath and  wash
water which contains unreduced silver from film processing.

Stationary Casting

A  process  in which the molten metal is poured into  molds  and
allowed to air-cool.  It is often used to recycle in-house scrap.

Subcategorization

The process of segmentation of an industry into groups of plants
for which uniform effluent limitations can be established.

Supernatent

A liquid or fluid forming a layer above settled solids.
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           GENERAL DEVELOPMENT DOCUMENT
                                           SECT - XVI
Surface Water

Any visible stream or body of water,  natural or man-made.   This
does not include bodies of water whose sole purpose is wastewater
retention or the removal of pollutants,  such as holding ponds or
lagoons.

Surfactants

Surface  active chemicals that tend to lower the surface  tension
between liquids.

Sweating

Bringing  small globules of low-melting constituents to an  alloy
surface during heat treatment.

Total Dissolved Solids (TDS)

Organic  and inorganic molecules and ions that are in true  solu-
tion in the water or wastewater.

Total Organic Carbon (TOG)

A measure of the organic contaminants in a wastewater.   The  TOC
analysis  does not measure as much of the organics as the COD  or
BOD tests, but is much quicker than these tests.

Total Recycle

The  complete  reuse  of a stream,  with make-up water  added  for
evaporation losses.   There is no blowdown stream from a  totally
recycled  flow and the process water is not periodically or  con-
tinuously discharged.
                                             or treated effluent.
Total Suspended Solids (TSS)

Solids in suspension in water,  wastewater,
Also known as suspended solids.

Traveling Grate Furnace

A  furnace with a moving grate that conveys material through  the
heating  zone.   The feed is ignited on the surface as the  grate
moves  past the burners;  air is blown in the charge to burn  the
fuel  by  downdraft  combustion as it moves  continuously  toward
discharge.

Tubing Blank

A sample taken by passing one gallon to distilled water through a
composite sampling device before initiation of actual  wastewater
sampling.
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           GENERAL DEVELOPMENT DOCUMENT
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Tuyere

Openings  in the shell and refractory lining of a furnace through
which air is forced.

Vacuum Dezincing

A  process for removing zinc from a metal by melting  or  heating
the solid metal in a vacuum.

Venturi Scrubbers

A  gas  cleaning device utilizing liquid to remove dust and  mist
from process gas  streams.

Volatile Substances

Materials   that  are  readily  vaporizable  at  relatively   low
temperatures.

Wastewater Discharge Factor

The ratio between water discharged from a production process  and
the mass of product of that production process.  Recycle water in
not included.

Water Use Factor

The  total  amount  of contact water or oil  entering  a  process
divided  by the amount of product produced by this process.   The
amount of water involved includes the recycle and make-up water.

Wet-Scrubbers

Air pollution control devices used for removing pollutants as the
Igas passes through the spray.

Zero Discharger

Any  industrial  or municipal facility that  does  not  discharge
wastewater.

The  following  sources  were  used for  defining  terms  in  the
glossary:
Gill,  G.  B.,  Nonferrous  Extractive Metallurgy.
Sons, New York, NY, 1980.
          John Wiley &
Lapedes, Daniel N., Dictionary of Scientific and Technical Terms,
2nd edition.  New York, NY, McGraw-Hill Book Co., 1978.

McGannon,  Harold E., The Making, Shaping, and Treating of Steel,
9th edition.  Pittsburgh, PA, U.S. Steel Corp., 1971.
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