EPA-450/4-82-018
Northeast Corridor  Regional Modeling Project
               Description  of the 1980
                   Urban Field Studies
                           Norman C. Possier
                            Warren P. Freas
            On assignment from the National Oceanic and Atmospheric Administration
                      Air Management Technology Branch
                      Monitoring and Data Analysis Division
                   U.S. ENVIRONMENTAL PROTECTION AGENCY
                       Office of Air, Noise and Radiation
                    Office of Air Quality Planning and Standards
                   Research Triangle Park, North Carolina 27711

                             October 1982

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 This report has been reviewed by the Office of Air Quality
Planning and Standards, EPA, and approved for publication.
Mention of trade names or commercial  products is not intended
to constitute endorsement or recommendation for use.

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Table of Contents
— - -                                                          Page
1.0  Background  .............................    '
2.0  Introduction ............................    3
3.0  Surface Air Quality and Meteorological Measurements   ........    3
4.0  Aircraft Monitoring   ........................  ^
5.0  Upper Air Meteorological Measurements   ...............  16
     5.1  Rawinsonde  Sounding Operations   ................  20
     5.2  Sodar  Operations   .......................  20
     5.3  Pilot  Balloon  Observations   ..................  22
6.0 Hydrocarbon Species Measurement  Program  ..............  22
7.0 Quality  Assurance Program   .....................  24
     7.1  QA  -  Surface Monitoring ....................  25
          7.1.1   Systems Audits .....................  25
          7.1.2  Interlaboratory Calibration Verification ........  28
          7.1.3  Instrument Calibrations and Zero/Span
                  Precision Checks ....................  29
           7.1.4  Instrument Audits  ...................  30
           7.1.5  Reduction of Surface Data  ...............  30
      7.2  QA - Aircraft Monitoring  ...................  32
           7.2.1  Aircraft Instrument Calibrations ............  32
           7.2.2  Aircraft Audits  ....................  32
           7.2.3  Instrument Altitude Response ..............  37
           7.2.4  Data Reduction  ......................  37
      7.3  QA - Upper Air Meteorological Measurements   ..........  38
      7.4  QA - Hydrocarbon Species Measurement Program   .........  39
 8.0  Availability of NECRMP Data  Base  ..................  39
                                                                            dn
 9.0  References  .............................  HU
 Appendix A.  Air Quality/Meteorological Monitoring  Sites   ........  A-l
 Appendix B.  Special Measurement  Dates   .................  B-1
                                      m

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List of Figures


Figure                            Ti tle                                 Page


  1              NECRMP Regional/Urban Modeling Domain                     2

  2              Locations of NECRMP Ozone Sites                          5

  3              Locations of NECRMP NMOC Sites                           6

  4              Locations of NECRMP NOX Sites                            7

  5              Locations of NECRMP Surface Wind Sites                   8

  6              Locations of NECRMP Surface Temperature and
                Solar Radiation  Sites                                    9

  7              Conceptual  Plan  for Urban Corridor
                Monitoring  Flights                                      14

  8              Locations of Urban Corridor Upper Air
                Meteorological Measurement Sites                        19
                                     iv

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List of Tables


Table                               Title                               Page


  1               Participants in the Aircraft Measurement Program        11

  2              NECRMP Aircraft Measurements                            12

  3              Rawinsonde, Pibal, and Sodar Site Locations             17

  4              Rawinsonde Sounding Schedule                            21

  5              Fixed Hydrocarbon Species Sampling Locations            23

  6              Systems Audit Evaluation Items                          26

  7              Air Quality Control Tests Applied to NECRMP
                 Ozone and Nitrogen Dioxide Data                         31

  8              Procedures and Calibration Systems Used for
                 Aircraft Instruments                                    33

  9              Frequency of Calibrations and Zero/Span
                 Checks for Aircraft Systems                             35

 10              Audit Summary for Aircraft Instrumentation              36

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                  Northeast Corridor Regional Modeling Project
                   Description of the 1980 Urban Field Studies
1.0  Background
     The Northeast Corridor Regional Modeling Project (NECRMP) is being
conducted to support the development of effective and equitable control
strategies necessary to reduce ozone concentrations in the Northeast.   It
has been recognized that high ozone concentrations are pervasive throughout
the Northeast and that significant interurban pollutant transport can  occur
between Corridor cities.  In this regard, the project was designed as  a
joint venture between EPA, State/local agencies, and Metropolitan Planning
Organizations in the Northeast to take an uniform approach to the control
of ozone within this Region.  The focus of this approach is the development
of various control strategies through combined application of Regional and
urban scale photochemical models.  The Regional Oxidant Model1 to be used
in NECRMP is being developed by the EPA Environmental Sciences Research
Laboratory (ESRL).  The Airshed2 and/or the OZIPP/EKMA Model3 will be
applied as the urban model for the large Corridor cities.  The structure of
the NECRMP and the models selected for strategy development have been
described, in detail, elsewhere.'4'5
     The development, evaluation and application of the selected models
requires a rather extensive data base to describe the air quality, meteoro-
logy and pertinent emissions within the NECRMP modeling domain.  The NECRMP
Regional domain (large grids) and urban domain (small grids) are shown in
Figure 1.  Several large field monitoring programs were conducted during 1980
to gather the data base required for modeling this region.  One portion of
the NECRMP monitoring effort, the Northeast Regional Oxidant Study (NEROS),
was conducted to principally support the development and application of the
Regional model.  As part of the NEROS, various large scale monitoring  experi-
ments were conducted across the Regional domain, together with urban plume
experiments in Columbus, OH and Baltimore, MD.  The specific field programs
which comprise the NEROS are described in reports by Clarke, et a!. ,6  Vaughan,
et a!.,7 and Possiel, et al.^  The focus of this report is the NECRMP  Urban
Field Studies conducted to obtain the ambient data base necessary
for application of the urban model(s) to the major Corridor cities.   The
report describes, in detail, the design and procedures of these studies.

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2.0  Introduction
     The urban studies were conducted from June through mid-September
1980 to gather the ambient data base necessary for application of the Airshed
model to Washington, DC, Baltimore, New York, and Boston.  [Philadelphia,
which is also included in the modeling program, was subject to an intensive
data collection effort in 1979.]  The data base, although collected to run
Airshed, is more than sufficient for applying less complex models, such as
OZIPP/EKMA.
     In general, the ambient data requirements for applying Airshed include
specifying pollutant concentrations at the boundary of the modeling domain,
and initial concentrations in each grid cell.  Also, meteorological
measurements are needed to define the horizontal and vertical flux of the
pollutant species.  Verification of the model against ambient data requires
specification of pollutant concentration fields for each predictive time
step.  These broad data requirements led to the development of a four-part
monitoring program designed to collect the required data base.  The four
monitoring tasks included continuous surface air quality and meteorological
measurements, air quality measurements aloft (via aircraft), upper air
meteorological measurements, and hydrocarbon species measurements.  The
following sections describe each of the monitoring tasks and the associated
quality assurance program.
3.0  Surface Air Quality and Meteorological Measurements
     The urban air quality monitoring networks were designed to obtain
measurements of ozone  (03), nitrogen oxides  (NO/N02/NOX), nonmethane organic
compounds  (continuous  NMOC, and species) and carbon monoxide  (CO) at
locations upwind, within and downwind of the urbanized portion of each city.
In  the  strictest sense, this would  have required a series of monitoring
rings around each city, beginning  in the core  area and extending  outward  up
to  perhaps  100  km in  order to ensure that  the  pollutant  concentrations were
measured under  various wind regimes.  However,  since the highest  ozone
concentrations  in the  Corridor  are  typically associated  with  the  prevailing
summer  season wind  flow  (from south through west), the monitoring  networks
were oriented along a  general southwest to northeast axis.   A few measure-
ment sites  were  also  located in crosswind  directions to  provide  for  some
variation  in wind flow from the prevailing sector.  To supplement the  urban

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 area monitoring and to provide measurements in more remote portions of the
 Corridor, four remote, rural sites were established and included in the
 network.

      In designing the network for each urban area, existing State/local
 sites were used to the extent possible.   In some cases, new instruments  were
 added to existing sites,  and new sites were established to fill  in gaps
 between existing sites.   For each city,  03, NO/N02/NOX and NMOC  monitoring
 sites were situated to the south and west of the city  center  at  a distance
 of from 30 to 45 km in order to measure  pollutants being transported into
 the urban area at the  ground level  upwind boundary of  the  city.   Within  the
 urban core,  measurements  were made  principally  for NO/N02/NOX and NMOC in
 order to specify initial  concentrations  of ozone precursors.
      Measurements  of NO/N02/NOX and 03 were also made  in suburban areas on
 the fringe of each city to assess the  spatial distribution  of NOX and to
 measure peak 03  concentrations  during  near stagnation  conditions  or  recircu-
 lation  wind  flows.   To the north  and east  of each  city,  03  was measured
 at numerous  locations  to  record concentrations  downwind  within the urban
 plume,  and thus  provide verification data  for model estimates  of  peak 03
 concentrations.
      Surface  meteorological measurements of wind speed and  wind direction
 were  made  throughout the  network to help determine  surface  pollutant
 transport  and  to indicate  the occurrence of mesoscale surface wind regimes
 which affect  pollutant concentrations.  Temperature and  solar radiation
 (direct  plus  diffuse) measurements were made at a few locations to determine
 photochemical  rate constants needed by the  model.  These meteorological
 measurements,  obtained at  State/local agency and contractor sites, were
 collected  to  supplement data from National  Weather Service and auxiliary
 observation stations within the Corridor.
     The sites at which measurements were made for 03 are shown in Figure 2,
 NMOC  in  Figure 3, and NO/N02/NOX in Figure  4.  Sites at which  wind speed
 and wind direction were measured are in Figure 5, and temperature and solar
 radiation  in Figure 6.   A list of the specific air quality and meteorological
measurements at each of the NECRMP monitoring sites is  given in Appendix  A.

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 4.0  Aircraft Monitoring
      Air quality and meteorological  measurements  aloft were obtained from
 instrumented  aircraft operated  in  the  vicinity  of each of the  four cities
 during  a five week  period  from  July  14 through  August  15.   The intent of
 the monitoring flights  was  to describe the  horizontal  and vertical  distri-
 bution  of 03, NO/NQX,  and  NMOC  on  high 03 days  which might be  potentially
 suitable for  modeling.   The EPA groups and  contractors participating in
 this program  are listed in  Table 1,  along with  the  location  of each  field
 office.   The  aircraft  programs  in  Washington, DC,  New  York,  and Boston
 were part of  the Urban  Corridor Studies, whereas  the program in Baltimore
 was part of the NEROS.   The air quality and meteorological  variables
 measured from each  aircraft and the  type of aircraft used  in each city
 are listed in Table 2.
      In  all four cities, monitoring  flights were  conducted on  days when
 photochemical  activity  and  subsequent  widespread  high  ozone  concentrations
 would be  likely.  Three  types of meteorological scenarios were  sought for
 flight days:  (1)  southwest  wind  flows  favorable for interurban  transport
 (when pollutants  from one or several cities impact upon another  Corridor
 city); (2) wind  flows from  directions  not conducive to interurban transport
 (when the  impact  of emissions from individual cities can be more easily
 reconciled);  and  (3) near stagnation or recirculation  flows  (when a city's
 pollutant  effluents tend to remain in  the vicinity of  the urban area).
 The  conceptual  plan of daily flight emissions for all   cities, except
 Baltimore, is  shown in Figure 7.  The  plan includes three flights per day,
 with vertical   spirals and horizontal  transects designed to map the pollu-
 tant concentration fields aloft.  Transects  were flown at approximately
 750 m, with spirals from ^  150 m to ^ 2100 m over rural areas and ^ 300 m
 to ^ 2100 m over urban areas.   In Baltimore, aircraft monitoring flights
were conducted to investigate the interaction of the Washington, DC -
 Baltimore urban plumes and the blending of the urban plume(s) into the
 regional ozone burden.  F:or this, aircraft measurements were made at
 preselected distances upwind and downwind,  similar to flights in the
 other Corridor cities and,  in addition, an attempt was  made to  measure
 temporal  changes in pollutant concentrations within specific air parcels
that had crossed the Baltimore urban area  at specific  times during the day.
                                     10

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Table 1.   Participants in the Aircraft Measurement Progra
                 m
    Participant
Area of Operations
   Field Station
EPA Environmental Monitoring
 Systems Laboratory - Las Vegas
Washington, DC
Manassas, VA  Airport
Brookhaven National Laboratory
Washington State University
Baltimore
Middle River, MD
Glenn Martin Airport
Battelle Pacific Northwest
 Laboratories
New York City
Morristown, NJ Airport
Battelle Columbus Laboratories
Boston
Beverly, MA  Airport
                                        11

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 Table 2.  NECRMP Aircraft Measurements

 Washington, DC - EMSL/Las Vegas
 Aircraft:   UH/IH Bell  Huey Helicopter
 Measurements/Instruments:
 Ozone
 NO/NOx
 S02
 Bscat
 Temperature
 Dew-Point  Temperature

 Baltimore  -  Brookhaven
 Aircraft:  Britten Norman  Islander
 Measurements/Instruments:
 Ozone
 NO/NOx
 S02
 Bscat
 Temperature
 Relative Humidity
 Solar Radiation Total
Solar Radiation UV
Turbulence
 Bendix  8002
 Monitor Labs  8440
 TECO 43
 MRI  1550B  Integrating  Nephelometer
 Rosemont Platinum -  Type  Total  Temperature
 General  Eastern  Model  1011  Hygrometer
AID 560
TECO 14B
Meloy 160-2
MRI 1550
Yellow Springs 705
Weather Measures Model HM 111
Eppley Pyranometer Model 8-48
Eppley UV Radiometer Model 14168
MRI Model 1120
                                     12

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Table 2.  Continued
Baltimore - Washington State Univ.
Aircraft:  Cessna 402
Measurements/Instruments:
Ozone
NO/NOx
Bscat
Temperature
Dew Point Temperature
Condensation Nuclei
CSI 2000
Monitor Labs 8440 HP
MRI 1550
Metrodata M-8 (bead thermister)
Metrodata M-8 (carbon strip)
Environment One-Rich 100
 New  York  - Battelle  Pacific Northwest Labs.

 Aircraft:  Cessna 320  F
 Measurements/Instruments :
Ozone
NO/NOx
Bscat
Temperature
Dew  Point Temperature
Bendix 8000
Monitor Labs 8440 HP
MRI 1550  Integrating Nephelometer
Rosemont  Model 102U2U
EG & G Cambridge Model 137-C
 Boston  -  Battelle  Columbus  Labs

 Aircraft:   Cessna  411
 Measurements/Instruments :
 Ozone
 NO/NOx
 Bscat
 Temperature
 Dew Point Temperature
 Winds
 Bendix  8000
 Monitor Labs  8440 HP
 MRI  1550 Integrating  Nephelometer
 Rosemont 102U2U
 EG & G  Cambridge Model  137-C
 Global  VLF System
                                      13

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                 Vertical
                 Spiral
               Horizontal
               Transect
EARLY

MORNING
MID-MORNING
                                  AFTERNOON
  Figure  7.  Conceptual  Plan for Urban Corridor Monitoring Flights,
                            14

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     The early morning flights in Washington, DC, New York and Boston
were used to measure the 03 and precursor burden aloft prior to the break-
up of the surface stable layer in order to define pollutant levels either
transported into or remaining over the city from the previous day.  These
flights were concentrated on the upwind side of the city and included
vertical spirals to indicate the presence of vertical gradients in 03
aloft.  Mid-morning flights included spirals on the upwind and downwind
fringe and over the urban core to define the vertical distribution of
pollutants during the period of rapid change in atmospheric mixing and
possible fumigation from elevated plumes.  Afternoon flights consisted of
cross-wind traverse patterns and spirals downwind of each city to map the
dimensions of the urban plume, and thus provide verification data for
model predictions in areas between surface sites.  Vertical spirals were
made over several points downwind, including the area of estimated peak
ozone concentration.  In Washington, DC and Boston, afternoon flights
extended 60-100 km downwind.  In New York, measurements were obtained
downwind to 100-130 km.
     The conceptual flight plan just described was modified, depending
upon the configuration of the city, its position in the Corridor, and
the meteorological conditions on the flight day.  In addition, three major
alterations to the plan were: (1) after the first few flight days, the
mid-morning flight in New York was discontinued because of flight restric-
tions and the need to conserve pilot hours for extended afternoon flights;
(2) the afternoon flight in Boston included an upwind transect and spiral
on days with southwest winds to note any daytime transport from upwind
urban areas; and  (3) toward the end of the program, the two morning flights
in Washington, DC were consolidated in order to conserve flying time.
      In order to  provide meteorological  information to support the flight
programs, a temporary weather forecast center was established at Martin
State Airport near Baltimore.  The center was manned by Brookhaven
National Laboratories  (BNL) and equipped to receive National Weather
Service observations, and forecasts and  computer products  from the
National Meteorological Center in Washington, DC.   Forecasts of 12-hour
and  18-hour boundary layer winds, cloud  cover and precipitation for the
study cities were prepared daily and transmitted to  the field offices by
1600  EST.  The  forecasts were used in deciding whether or  not to  plan a
                                      15

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 flight for the following day.   Updated forecasts were provided at 0400 EST
 on flight days.   In addition to information received from the forecast
 center, real-time boundary layer winds were obtained by the field personnel
 from pilot balloon observations (pibals)  made at sites in the vicinity of
 each city.   These measurements  were used  to fine-tune the direction and
 distance of flight tracks  during the day.
      Flight days  in New  York and Boston were selected independently of each
 other,  since meteorological  conditions often differed between the two  areas.
 However,  flight days  and flight patterns  in Washington,  DC  and Baltimore
 were closely coordinated in  order  to maximize use  of the  aircraft assigned
 to both cities.   At the end  of  each  flight  day,  flight crews  were debriefed
 by EPA  field personnel on  the magnitude and distribution  of ozone
 concentrations observed aloft.   This  information was  used in  planning
 subsequent  flights.
 5.0   Upper  Air Meteoro1^gjcaj_jjte£sujr^ments-
      A  program of  upper air  meteorological  measurements was conducted  as
 part  of NECRMP to  obtain wind,  temperature  and mixing  height  information
 necessary for the  model to estimate  pollutant transport and vertical
 dispersion.  Three  types of  measurement, procedures were used:  (1)  rawin-
 sonde soundings for temperature  and  wind profiles; (2) pilot  balloon
 observations for wind profiles;  and  (3) sodars for low level mixing heights
 (data on the vertical distribution of  temperature are  also available from
 aircraft flights).  The upper air meteorological measurements  began on
 July  18 and  continued through September 12,   1980, except for the  pibals
which began July 14 and were terminated at  the end of  the aircraft measure-
ment program.  The days with upper air measurements are listed in Appendix B.
     Rawinsonde soundings were conducted by  Beukers Laboratories at six
 locations in the Corridor,  sodars were operated by AeroVironment at four
locations, and pibal observations were taken at six locations by those
responsible for the aircraft flights.  A list of pertinent information on
each measurement site is  given  in Table 3, and the locations of the sites
are shown in Figure 8.  These locations were selected in order to characterize
both the extent of vertical mixing and mesoscale wind regimes in the vicinity
                                      16

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Table 3  Rawinsonde, Pibal, and Sodar Site Locations
                                  Rawlnsonde Soundings
Site
Number
11
12
13
14
15
16
Site
Number
1
2
3
4
5
6
Sitei
Type
S
U
S
U
R
U
Sitei
Type
R
S
S
S
S
R
Site
Name
Baltimore
Boston
Derby, CT
Newark
Marlboro, NJ
Washington, DC
Pilot
Site
Name
Bel Aire, MD
Beverly, MA
Glen Cove, NY
Medfield, MA
Morristown, NJ
Manassas, VA
Location
Johns Hopkins
University
Mass. Inst. of
Technology
Derby High School
Rutgers University
Municipal Complex
National Airport
Balloon Observations
Location
NECRMP Monitoring
site
Municipal Airport
Lattington Beach
State Hospital
Municipal Airport
Municipal Airport
Lat./Long.
39°19'48"N
76°37I22"W
42021'41"N
71005'33"W
41°19'26"N
73°05'26"W
40°39'23"N
74°13'18"W
40°19'00"N
74°15'00"W
38°50'36"N
77°02'irw
Lat./Long.
39°37'37"N
76°19'46"W
42°35'10"N
70°55I20"W
40°53'30"N
73°35I55"W
42°12'44"N
71°20'08"W
40°47'50"N
74025'20"W
38°43I00"N
77°31 '00"W
Elevation
(m MSL)
73
35
78
5
55
3
Elevation
(m MSL)
10
33
24
84
57
57
1  U:  urban
  S:  suburban
  R:  rural
                                         17

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Table 3.  Continued
Site
Number
7
8
15
9
Site1
Type
R
S
R
R
                    Site
                    Name

                    Camp Upshur,
                     VA
Sodar Operations


Location
US Marine Base,
 Quantico

Goucher College
                                       Municipal  Complex
                                       Great Meadows
                                       National Wildlife
                                         Reserve
Lat./Long.
38°37'25"N
77°37'15"W

39°24'46"N
76°35'30"W

40°19'00"N
74°15'00"W

42°23'05"N
71°23'19"W
Elevation
 (m MSL)

    61


   113


    55


    37
  U:  urban
  S:  suburban
  R:  rural

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                                                        RAWINSONDE SITES
                                                      • PILOT BALLOON SITES
                                                      • SODAR SITES
                                                      ARAWINSQIMDE AND
                                                        SODAR SITE
Figure 8.  Locations of Urban Corridor Upper Air Meteorological
           Measurement Sites.
                             19

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  of  the  Corridor  cities.   In  addition,  upper  air  soundings were  obtained
  at  six-hour  intervals from National Weather  Service stations  (except
  New York City) within the Regional domain, as part of the NEROS.
  5.1  Rawinsonde  Sounding^ Op erations
      The NECRMP  rawinsonde soundings were obtained five days per week,
  typically Monday through Friday, although the schedule was adjusted to
  obtain soundings on weekend days when aircraft flights were planned.
  The daily schedule of soundings at each site is provided in Table 4.
  Basically,  soundings were conducted during (1) the early morning to
 provide an  estimate of low level  atmospheric stability at urban and rural
 locations prior to sunrise;  (2) the mid-morning period of rapid mixing
 height rise;  and (3)  the early afternoon when the vertical  extent of
 mixing reaches a maximum.  Slow rise  balloons were used  for  soundings
 to obtain a more detailed temperature  structure  within the  boundary layer
 than is  available from routine National  Weather  Service  soundings.   An
 average  ascent rate of 400  ft./min. was  achieved,  and  data were  recorded
 between  ground level  and 700  mb (^  3500  m) only.
     Temperature/dew  point temperature  and height  values  for  "mandatory"
 and  "significant" levels  (pressure altitudes)  were  determined  using
 standard  National  Weather Service data  reduction  procedures,8 except
 that a criteria  of  +  1/2°C was  used rather than +  i°c  for selecting
 "significant"  temperature points.  Wind  speed  and wind direction  values
 were determined at  30-second  intervals for the entire  sounding.   Standard
 National Weather  Service  radiosondes were used for the temperature and
 humidity measurements.
 5.2  Sodar Operations
     The AeroVironment model 300 monostatic acoustic radar (sodar) was
 used to provide a near continuous record of the thermal structure of the
 lower atmosphere  from 30 m to 1000 m AGL (the respective lower and upper
detectable limits of the  instrument).   Data from the sodar were reduced
into 30-minute average mixing height values determined  as the height of
the base of  the lowest stable layer detected  by the instrument.
                                     20

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 Table 4.    Rawinsonde  Sounding  Schedule
 Sounding  Site

 Washington,  DC
 Site  16
 Baltimore
 Site  11
 Marlboro
 Site  15
 Newark
 Site  14
Derby
Site 13
 Start/End Date

 July  24  - September 12
July  16 - September 12
July 17 - August 29
July 19 - September 12
July 16 - September 12
Launch Time (EST)

       0500
       0900
       1300

       0700
       0900
       lOOOa
       1200?
       1300
       1400a
       1500a
       1600a

       0500
       0700
       0900
       1300

       0500
       0900
       llOOb
       1300c
Boston
Site 12
July 18 - September 12
a...  soundings on July 16 and 31, and August 1,  5,  6,  7 and  14  only,

b.  sounding effective September 3.

c.  sounding discontinued September  2,

d.  winds only,  no temperature measurements.
      0500
      0700d
      0900
      llOOd
      1300
      1500d
                                        21

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 5 . 3  Pilot Balloon Observations
      Pilot balloon observations of wind speed and direction aloft were
 made almost daily during the period July 14 through August 15, 1980.
 Thirty-gram balloons were released hourly from 0400 EST through 1700  EST
 and tracked with a single theodolite.   Readings of azimuth and elevation
 were recorded every 30 seconds for a total  of 20 minutes.   A constant
 rise rate was assumed for reducing the  raw data into wind  speed and
 direction values.   The reduced wind data began at 110 m AGL and continued
 at  approximately 90 m intervals up to 3690  m AGL.
 6 . 0  Hydrocarbon Species
      Hydrocarbon  species  concentrations  were  obtained  at  various  locations
 in  the  vicinity of  the  study  cities  in order  to  define the  mix  of non-
 methane hydrocarbons  needed as  input  to  the model.   Species  concentrations
 were  identified by  gas  chromatographic (GC) analysis of both grab samples
 and one-hour  integrated samples of ambient air.  The collection of  these
 samples began on  July 14  and  continued through August  29.
      Integrated ground  level  samples  were collected  between  the hours of
 0500-0600 and 0700-0800 EST at two sites in the  urbanized portion of each
 city.   As time permitted, grab samples were collected  from  a  "roving van"
 at various  locations downwind of Washington,  DC  and  Baltimore.  The fixed
 sampling sites are  listed in Table 5.  Integrated samples were collected
 in Teflon or Tedlar bags  using an automated timer-pump  system.  The
 roving  van  grab samples were collected in stainless  steel  canisters.
     Ambient grab samples were also collected aloft  in  six-liter  stainless
 steel canisters during aircraft flights.   In Washington, DC, New  York
 and Boston, grab samples were obtained within and above the surface stable
 layer during vertical spirals on early morning flights.  In Washington, DC
 and Boston, two samples were also collected (at different altitudes) over
 the urban center during the mid-morning flights.   In New York, grab samples
were collected during the afternoon within the mixed layer over southern
 Connecticut (these samples were intended  to measure the composition of
 hydrocarbons remaining in the New York plume after the peak in photo-
chemical activity).   In Baltimore,  four grab samples were  collected on
each flight throughout the day.   These samples were used to characterize
                                22

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Table 5.   Fixed Hydrocarbon Species Sampling Locations
Urban Area
Washington, DC
Sampling Sites

West End Library
NECRMP site 9

University of Maryland Campus
non NECRMP site

Takoma Park
NECRMP site 10
Baltimore
Read Street
NECRMP site 13

Essex, MD
NECRMP site 20
New York City
Newark, NJ
New Jersey Inst0 of Technology
NECRMP site 46

Linden, NJ
NECRMP site 43
Boston
East Boston, MA
NECRMP site 27

Watertown, MA
NECRMP site 37
                                  23

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 hydrocarbons upwind, within and on either side of the Baltimore urban
 plume.  Not all collected samples were analyzed because of time limita-
 tions on the gas chromatographs.   However, those samples which were
 selected for GC analysis were analyzed within 48 hours of collection.
      Laboratories for GC analysis were established at Martin Airport
 near Baltimore and at the New Jersey Institute of Technology at Newark
 by Washington State University (WSU).   In the Boston area,  a GC
 laboratory was operated at Beverly Airport by Battelle Columbus
 Laboratories (BCL).   The specific chromatographs and peripheral data
 systems  are given in references  9 and  10  for WSU and BCL,  respectively.
 A  description of the species  data are  included in  reference 11.
 7.0  Quality Assurance Program
      A comprehensive Quality  Assurance (QA)  program  accompanied the
 various  NECRMP ambient measurement programs.   The  objectives  of the  QA
 program  were as follows:
      (a)   to obtain  a  data  base of measurements  as precise  and  accurate
 as  possible within  the limitations of  available  manpower and  funds;
      (b)   to obtain  a  high  percentage  (>_  90%)  recovery of data  during
 the  measurement program;
      (c)   to ensure  that  surface measurements  are  representative of  the
 desired  spatial  and  temporal  scales; and
      (d)   to  ensure  that  all  air quality measurements are traceable  to
 a single source  (National Bureau of Standards  [NBS])  in order to provide
 internal  consistency and  comparability among measurements made  by the
 various study participants.
     Assistance  in designing and implementing  the QA  program was provided
 by the Environmental Monitoring Systems Laboratory (EMSL) at Research
Triangle Park, North Carolina.  All of the air quality analyzers (except
 for those measuring NMOC) were operated using  EPA designated reference
or equivalent methods.  The NMOC analyzers (MSA model 11-2) were selected
by EMSL-RTP for use in this study, based upon  the results of their evalu-
ation of several state-of-the-art  instruments.  The specific QA activities
are described below for each NECRMP measurement program.
                                 24

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7.1  QA - Surface Monitoring
     The QA activities conducted during the surface monitoring program
were developed from requirements for National  Air Monitoring Stations (NAMS),
as specified in 40 CFR Part 58, Federal Register, May 10, 1979.12  Guidance
for implementing the QA plan is contained in Volume II of the "Quality
Assurance Handbook for Air Pollution Measurement Systems."13  The specific
QA elements of the NECRMP surface measurement  program included:
     (a)  systems audits of monitoring sites;
     (b)  verification of calibration procedures;
     (c)  instrument calibrations and zero/span and precision checks; and
     (d)  instrument performance audits.
7.1.1  Systems Audits
       Systems audits were conducted by Research Triangle Institute (RTI),
under contract to EMSL-RTP.  As part of this effort, 24 of the designated
NECRMP sites were evaluated during the period  May 22 through June 11, 1980.
These sites were selected to represent monitoring operations by  each of the
agencies and contractors participating in the  surface monitoring portion of
the study.  The general items checked at each  site included the  following:
       (a)  suitability of the location and exposure for 03 and  NO/N02/NOX
monitoring;
       (b)  the sample inlet system leading into the site, including the
placement and height of the probe:
       (c)  the analyzer set up (e.g., gas connections, power connections);
       (d)  the calibration systems (including zero air and standards); and
       (e)  the record keeping and documentation of site operations.
       Other more specific items checked by RTI are listed in Table 6.
Meteorological systems were also checked to ensure that the instrument had
an unobstructed exposure and that the systems  were operating normally.
The results of the systems audits are documented in a report by
                                     25

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Table 6.  Systems Audit Evaluation Items


A-  Ambient Air Analyzer Checks

    Ozone -

          Equivalency designated analyzer

          Calibration system (ozone source, dilution source, UV photometer,
          or transfer standard)

          Ethylene purity

          Flowmeter range and accuracy; flowmeter calibration

          Repair parts available

          Proper electrical  and pneumatic installation

    Oxides of Nitrogen -

          Equivalency designated analyzer

          Suitable calibration system

          NBS-traceable NO in nitrogen cylinder and/or NBS-traceable
          N02 permeation tube

          Suitable flowmeters; flowmeter calibration

          Proper electrical  and pneumatic installation


B.  Pollutant Standards Delivery System

    Availability and adequacy of dilution and/or gas phase titration equipment

    Proper grade and traceability of pollutant standards

    Stability of ozone generator; proper plumbing

    Calibration and precision checks accomplished by delivering pollutant
    to analyzer while it is  in its normal  ambient sampling configuration


C.  Site Location

    Unobstructed airflow

    Sited according to current EPA criteria

    Security

    Distant from sources of  oxides or nitrogen or hydrocarbons
                                     26

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Table 6.  (continued)




D.  Site Facilities



    Cleanliness



    Sufficient workspace



    Safety



    Temperature control



    Adequate voltage



    Inlet probes, manifolds, blowers; their cleanliness and integrity





E.  Site Operation



    Calibration procedures, schedule



    Zero and span check  procedures, schedule



    Precision check procedures, schedule



    Data transmittal  and reduction to concentration units



    Audit procedures, schedule



    Documentation control  charts,  operating and  reporting  procedures



    Corrective action procedures



    Strip chart annotation, data forms



    Routine  maintenance  procedures, schedule
                                      27

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Recommendations were made by EPA to the site operators for correcting any
deficiencies found by the audits.  All serious problems were resolved by
the agencies as soon as possible.
7.1.2  Inter!aboratory Calibration Verification (ICV)
       An audit system verification center was established to verify the
accuracy of the 03 and NO/N02/NOX audit systems used by audit teams during
the summer field program.  The center was operated from April 23 through
May 1, 1980, by RTI, at the EPA Region II laboratory.  Participating in the
ICV were representatives from the following agencies:
       EPA Region I,
       EPA Region II,
       Massachusetts Department of Environmental  Quality Engineering,
       Connecticut Department of Environmental  Protection,
       New York Department of Environmental Conservation, and
       New Jersey Bureau of Air Pollution Control.
The center was equipped with the following analyzers:
       Bendix Ozone Analyzer, Model  8002A,
       Monitor Labs Ozone Analyzer,  Model  8410,
       Bendix Total Oxides of Nitrogen Analyzer,  Model  8440,  and
       Bendix Carbon Monoxide Analyzer, Model  3501C5A.
       The following approach was taken to maintain a chain of traceability
in the NECRMP audit program.  Prior  to establishing the ICV,  RTI's cali-
bration systems were taken to EMSL-RTP for verification against NBS
certified standards.  RTI then set up and calibrated the above analyzers
at the ICV center in Region II.   The verification of the participants was
accomplished by having each team generate concentrations from their audit
systems.   These were compared to the predicted  concentrations, as calculated
from the instrument response and calibration equation established by RTI.
The slope (m) and intercept (b)  of the linear regression of the two sets of
concentrations were used to evaluate the performance of each  team for each
pollutant.  The following criteria were used to judge the performance of
the participants:
                                 28

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 Excellent Performance Levels
. Slope:         0.95  <  m _< 1.05; and
 Intercept:     -1% FS <  b _<  +1% FS (FS = full scale range of analyzer).
 Satisfactory Performance Levels
 Slope:         0.90 _<  m < 0.95 or 1.05 > m _<  1.10;  and
 Intercept:     -2% FS _<  b < -1% FS or 1% > b _<  2% FS.
 Unsatisfactory Performance Levels
 Slope:         m  < 0.90  or m  >  1.10;  and
 Intercept:     b  < -2% FS or  b  > +2%  FS.

        For those  systems  which  gave an  unsatisfactory response,  the
 operating  procedures  and  analyzers  were checked by  RTI and  the operator
 in  order to  identify  the  source  of  the  discrepancies.  Appropriate cor-
 rections/adjustments  were subsequently  made  by  the  operator.  The results
 of  the ICV are  documented in a  report by  RTI.15
 7.1.3   Instrument Callbrations  and  Zero/Span  and Precision  Checks
        The 03 analyzers operated  at the  surface monitoring  sites were
 calibrated by UV photometry or Gas  Phase Titration  (GPT), according to
 requirements in Appendix  A of reference  11.  The NO/N02/NOX analyzers
were calibrated by GPT, according to requirements in Appendix A of this
 reference.  The zero/span and precision checks were conducted for 03 and
NO/N02/NOX analyzers, according  to guidelines in reference  13.  The
specific,  routine QA procedures  used by Battelle Columbus at their sites
in New  York and New Jersey, and  by Engineering Science in Maryland,  are
documented in references  16 and  17, respectively.  The NMOC analyzers
were calibrated by PEDCo, using EPA certified methane and propane cali-
bration gases, according to procedures described in reference 18.  The
procedures used for zero/span and precision checks for the NMOC analyzers
are also described in that report.
       The following schedule was prescribed by EMSL for calibrations and
for zero/span and precision checks at surface sites:
                                  29

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                Calibrations         Zero/Span  Checks          Precision  Checks
 OS  and           monthly              twice  per week            twice  per week
 NO/N02/NOX

 NMOC             once  every           daily                     three  times
                 two weeks                                     per week

       The above frequency of  zero/span  checks was recommended  to detect
 drift in  instrument response and  thereby permit  the  correction  of a problem
 before data would have to be invalidated.  The relatively frequent  precision
 checks were recommended because of  the short  term nature of  the study  and
 the need  to provide sufficient data  to evaluate  statistically the performance
 of each analyzer during the three month  study.   This schedule was followed by
 most of the monitoring agencies and  contractors.  However, a  somewhat  less
 stringent schedule was adopted by a  few  agencies at  particular  sites,  due to
 limited personnel and/or calibrators.
 7.1.4  Instrument Audits
       Audits of the  03, NO/N02/NOX, and NMOC analyzers operated at the
 designated NECRMP monitoring sites were  performed twice during  the field
 program.  The agencies participating in  the ICV, together with  RTI, shared
 the responsibility for auditing these sites.  Instruments found to give an
 unsatisfactory response to the audit ( >_ 15% difference between audit  output
 and instrument response) were recalibrated by the operating agency or
 contractor.  The  results of the two audits conducted during the field
 program are summarized in reference 19.
 7.1.5  Reduction  of Surface Data
       The continuous measurements made at surface monitoring sites were
 reduced into hourly arithmetic averages,  except for wind measurements at
 sites in New York State which were reduced as vector averages.  The precision
and audit data collected for each air quality analyzer were used in validating
measured values.  Each agency/contractor was responsible for judging the
precision of its own instruments.   However, EMSL-RTP provided an evaluation
of precision data for the NMOC analyzers.
       The 03 and N0£ data were assembled and submitted to the appropriate
 EPA Regional  Office,  where they were run  through the automated Quality
Control  (QC)  screening tests  listed in Table 7.20  These screening  tests
                                 30

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 Table 7.   Air Quality Control  Tests Applied to NECRMP
           Ozone and Nitrogen Dioxide Data
           Tests                                   Flag  Values  (pom)
 1.   Maximum  Value  Test:

     flags  unexpectedly  high  values.         >  0.50  (1000-1700)
                                            >  0.38  (1800-0900)         >  0.64

 2.   Adjacent Value Test:

     flags  an unexpected fluctuation         +0.15  (day)
     in concentration between two            +0.10  (night)             ±0.27
     consecutive hours.                      ~

 3.   Spike  Test:

     flags  the middle vaiue of three         +_  0.10  (day)
     consecutive hourly values if it;         +0.05  (night)             -   -11
     is much higher or lower than the        ~  or                         or
     two adjacent hours.                      +_  300%                     + 30o%

4.  Consecutive Four Hour Test:

    flags short term clusters of            > 0.25                    > 0 53
    unexpectedly high values.

5.  Gap Test:

    flags unexpectedly high values
    by checking for gaps in the
    frequency distribution.
                                    31

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flagged potentially invalid data points.  Agencies and contractors were
notified of any flagged values identified at their sites.  These data were
then verified as valid, or deleted if determined to be invalid.  No auto-
mated screening tests were run for the NO, NOx, NMOC, or surface meteoro-
logical data; only manual spot checks were made of these data.  However,
all of the surface air quality and meteorological data will be run through
additional screening checks prior to the creation of the modeling data
base in 1983.
7.2    QA - Aircraft Monitoring
       Quality Assurance activities associated with the aircraft monitoring
program included calibrations, zero/span checks and audits of the monitoring
systems.  The types of monitors operated on board each aircraft are listed
in Table 2.
7.2.1  Aircraft Instrument Calibrations
       The systems and procedures used to calibrate the air quality
instruments operated on board the five aircraft are described in Table 8.
For all aircraft systems, the calibration equipment was assayed against
NBS-SRM certified equipment prior to the start of the measurement program.
Meteorological equipment were also calibrated at that time.  The general
schedules of calibrations and zero/span checks adopted by each aircraft
operator are listed in Table 9.  The specific QA procedures followed are
in references 21, 22, 23, 24, and 25 for the aircraft in Washington, DC,
Baltimore (BNL), Baltimore (WSU), New York and Boston, respectively.
7.2.2  Aircraft Audits
       Audits of the air quality instruments were conducted by RTI for
each aircraft system during the initial days of the program.  Instruments
found to give an unsatisfactory response were recalibrated following any
necessary instrument repairs or modifications to operating procedures.  A
summary of the audit results is provided in Table 10.  Details of the
audits are available in reference 19 for aircraft in Washington, DC,
New York and Boston, and in reference 26 for the two aircraft in Baltimore.
                                  32

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 Table 8.  Procedures and Calibration Systems Used for Aircraft  Instruments
 Urban Area:
 Washington, DC
 Aircraft Operator:  EMSL-Las Vegas
 Ozone:
 NO/N02/NOX:
 S02:
 Calibrations were performed using a TECO 101 dilution
 system equipped with an ozone generator, the output of
 which was monitored with a Dasibi 03 monitor referenced
 to a long-path UV photometer.

 Calibrations were performed using a cylinder of NO in
 nitrogen (Np) tertiary standard.  The span calibration
 was performed by dilution, using a Bendix Dynamic
 calibration system with zero air from an Aadco pure
 air generator.  The pure air generator also provided
 for the zero air calibration.

 Calibrations were performed using a cylinder of S02
 (secondary standard) certified by comparison to an NBS
 permeation tube.   The span calibration was  performed
 using a direct span gas bottle and zeroed using the
 Aadco pure air generator.
 Urban  Area:
 Baltimore,  MD
 Aircraft  Operator:   Brookhaven National  Laboratory
 Ozone:
NO/N02/NOX:
S02:
 Calibrations were  performed  using  an  AID  ozone  generator,
 the  output of which was verified by Gas Phase Titration
 with  an  NBS standard cylinder of NO in N2.

 Calibrations were  performed  using  a Monitor Labs 8500
 calibrator equipped with an  NO dilution system  and a
 46 ppm NBS NO in a N2 cylinder.

 Calibrations were  performed  using  a Monitor Labs 74447
 calibrator and NBS traceable S02 permeation tube.
Urban Area:

Aircraft Operator:

Ozone:



NO/N02/NOX:
Baltimore, MD

Washington State University

Calibrations were performed using a MEC 1000 ozone
generator, the output of which was verified by UV
(Dasibi 1008-PC).

Calibrations were performed using a Meloy Model CN 020
calibrator with an NBS cylinder of 52 ppm NO in N2.
Span checks were made with a 0.93 ppm NO in N2 cylinder,
the concentration of which was verified by GPT prior to'
the study.
                                     33

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Table 8.  (continued)


Urban Area:          New York City, NY and Boston, MA

Aircraft Operator:  Battelle Northwest and Battelle Columbus

Ozone:              Calibrations were performed using a CSI 1700 Gas Phase
                    Titration calibration system referenced to an NBS
                    certified UV photometer.

NO/NQ2/NOx:          Calibrations were performed using the CSI 1700 with an
                    NBS cylinder of NO in N2.
                                     34

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 Table  9.   Fr^guenc^_o^ajj^r_at_1ons  and  Zero/Span  Checks  for  Aircraft Systems


 Washington, JK

 o   Multipoint calibrations were  conducted  prior  to and  following  the  study.

 o   Zero/span checks were  conducted prior to and  following  each  flight day.

 o   Zero air calibrations  were conducted  in flight.


 Baltimore  (BNL)

 o   Multipoint calibrations were  conducted three  times on the  N0/N02/N0x analyzer,
    two times on the 03 analyzer, and once on the S02 analyzer.

 o   In-flight zero air calibrations ^or SO? were  conducted  at  each flight altitude

 o   In-flight zero air calibrations were conducted  for 03 and  NO/N02/NOX.

 o   Span checks were performed twice on the 03 analyzer  and once each  on the
    NO/N02/NOX and S02 analyzers  during the program.


 Baltimore  (WSU)

 o   Multipoint calibrations were  conducted four times on the 03 analyzer and
    once, prior to the study, on  the NO/N02/NOX analyzer.

 o   Zero/span checks were conducted on the NO/N02/NOX analyzer four times during
    the study.


 New York City

o  Multipoint calibrations were conducted weekly.

o  Zero/span checks were conducted daily between morning and afternoon flights.


Boston
o  Multipoint calibrations were conducted weekly.

o  Zero/span checks were conducted daily between early morning and mid-morninq
   flights.
                                    35

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 Table 10.   Audit Summary for Aircraft
 Washington,  DC
 03
 NO/NOx
 S02
 Bscat

 Baltimore  (WSU)
 03
 NO/NOx
 S02
 Bscat

 Baltimore  (BNL)
 03
 NO/NOx
 S02
 Bscat
                                       Ratings1
 S
 S/E
 S
 within + 10%
 S
 S/E
 S
 within  + 10%
 S
 E/E
 S
 +  19.4%
New York City
03
NO/NOX
Bscat
 E
 S/S
within + 10%
Boston
03
NO/NOX
Bscat
E
E/E
within + 10%
 1 E = Excellent
   S = Satisfactory
   U = Unsatisfactory
                                     36

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  7.2.3  instj^uiront^

         Corrections  to  measured  data  for  variations  in  instrument  response
  with  altitude were  made  for  03  measurements  obtained in  Boston.   For  these
  data,  Battelle  used relationships described  by White.27  According  to
  these  relationships, not adjusting the 03 data for  variations  in  response
  due to  altitude could  result in concentrations too  low by 15-25%  at 2,000 m,
  which was about the highest altitude of  the  aircraft spirals during NECRMP.
  This is on the order of 0.02 ppm, considering typical values observed at
  this altitude during the program.   In Baltimore, altitude response relation-
  ships were developed by BNL and WSU for the particular ozone analyzers
 operated aboard their aircraft,  however,  the data have not been adjusted.
 No altitude corrections were deemed necessary for the other analyzers.
        In general, there were no major  difficulties  with  the operation of
 the on board instrumentation.   However,  BNL  did  have some problems main-
 taining their NOX  analyzer  in calibration,  due to high  cabin temperatures
 h 35°C) at the  ground  and  aloft.  As a  result, multi-point  calibrations
 were  performed  on  this  instrument  on  several  occasions  during  the  study.
 Also,  problems with  the NOX  zero were encountered by BNW  in  the New  York
 area.   This  occasionally  resulted  in  slightly negative  NO/NOX  values at  a
 few points  on vertical  spirals.   In addition,  apparent  imprecision in  the
 humidity instrument  operated  by  BNW resulted  in the  dew-point  temperature
 slightly exceeding the  ambient air temperature when  high  humidity  was
 encountered.
 7.2.4  Data Reduction

       The continuous measurements recorded on magnetic tape from  the  on
 board analyzers were reduced from raw voltages into  scientific  units,  using
 the calibration equations and zero/span data, according to procedures
 described in  the reports prepared by each aircraft operator.21,22,23,2^,25
 Quality Control  checks conducted by the aircraft operators were accomplished
 by visually screening time versus concentration plots of the reduced data or
 the original strip chart trace as recorded in flight.  Unusual fluctuations
 in air quality or meteorological  parameters were checked for physical
consistency.  The data were  also checked against flight logs to note any
                                  37

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 instrument problems, zero checks, times when the aircraft passed through
 plumes, and the height of inversion layers.  Data determined to be invalid
 were deleted from the data base.  In addition, the aircraft data will be
 subject to more intensive screening prior to the creation of the modeling
 data base in 1983.
 7.3    QA - Upper Air Meteorological Measurements
        The instrument systems used by Beukers Laboratories for tracking
 and recording data  from the radiosondes were calibrated prior to the start
 of  the field program, as were the acoustic radar units deployed by
 AeroVironment.   These systems have been found to be fairly stable during
 routine field operations and require recalibrations only after major
 repair.   All  of the radiosondes  used during the  study were purchased from
 VIZ and subject to  QC by the manufacturer.
        Most of  the  QA activities in  the program  were  conducted during the
 data compilation and reduction phase.   Quality Control  checks  of the upper
 air sounding  data consisted  of (1)  a point-by-point review of  each  sounding
 in  the  field;  (2) a check of each sounding  while the  data  were being
 processed  on  the computer;  and (3)  a review of the  temperature and  wind
 sounding  data for meteorological  reasonableness  and spatial  and temporal
 continuity.  Any soundings  or individual  data points  which appeared suspect
 of  being  invalid were reprocessed,  verified,  and corrected or  deleted, as
 appropriate.
       The  QC procedures  for the  sodar-derived mixing  height data began
 in  the  field, when  the measured  values  were  reduced from the strip  chart
 records.   This  enabled the technician to  spot any readings  indicative of
 possible  instrument malfunctions.  The  strip charts were reevaluated  and
 reviewed by AeroVironment at  their Pasadena, CA  facility,  prior  to  being
 entered onto magnetic tape.   In  addition  10% of  the values were  spot  checked
 by  supervisory  personnel.
       No rigorous QC procedures  have as yet been applied  to the pilot
balloon wind observations.   However, the data were  spot checked  against
the original data records, and all winds were reviewed for meteorological
reasonableness and consistency, both between successive pibal observations
and against rawinsonde wind data.  No suspect data were identified.
                                  38

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        In addition to the above QC checks, the upper air data will be
 further screened prior to the creation of the modeling data base in 1983.
 7•4    QA - Hydrocarbon Species Measurement Program
        Quality Assurance procedures during the collection and analysis of
 hydrocarbon species measurements included:
        (1)   analysis of all  samples within 48 hours of collection;
        (2)   checking chromatograms for evidence of container contamination
             of samples;
        (3)   calibration  of chromatographic columns with known standards;
        (4)   precision checks  with  artificial  hydrocarbon mixtures; and
        (5)   a  "round robin" analysis  of specific  samples by each  laboratory.
        A  report describing the  results  of  the "round  robin" analyses  is
 being  prepared by  the EPA  Environmental  Sciences  Research  Laboratory  (ESRL).
 In  addition, ESRL  will be  screening the  species data  to identify  possible
 invalid data prior to the  creation  of  the  modeling data base  in 1983.
 8.0     Availability of NECRMP Urban Corridor  Data  Base
        The data  described  in  the preceding sections have been assembled into
 a data  base available on magnetic tape.  The  surface air quality  and meteoro-
 logical data are recorded  in SAROAD hourly data card image  format.  These  data
 have been converted  to a standard set of reporting  units for  each  pollutant
 and meteorological  parameter and to local  standard  time  (LST).  The special
 NECRMP  rawinsonde  and pilot balloon wind speed and  direction  data  have been
 merged  into a  single  data  set.  The rawinsonde temperature  sounding data
 comprise another separate  data set.  The mixing height  data obtained with  the
 monostatic acoustic  radar  (sodar) were also place  in SAROAD hourly data card
 image format.  Since  these mixing heights  represent 30 minute values, there
 are four, rather than two, cards for each  day.  The aircraft data obtained in
 Washington, DC, New York, and Boston complete the Urban Corridor data base.
 A description of the NECRMP Urban Corridor data base, including data formats,
 reporting units, and  tape specifications is contained in the report entitled:
 "Northeast Corridor Regional  Modeling Project - Urban Corridor Data Base
 Description."28  The entire NECRMP  data base, including Urban Corridor data,
 Baltimore aircraft data, and other  data sets obtained as part of the NEROS
will be available from ESRL in 11983.
                                  39

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 9.0  References


  1.  R. G. Lamb, "A Regional Scale (1000 km) Model of Photochemical Air
      Pollution, Part 1: Theoretical Formulation," U.S. Environmental
      Protection Agency Technical Report, in press.

  2.  S  D  Reynolds and L. E. Reid, "An Introduction to the SAI Airshed Model
      and Its Usage,1 Systems Applications, Inc., Report EF 78-53R, May 1978.

  3.  U.S. Environmental Protection Agency, "Uses, Limitations and Technical
      Basis of Procedures for Quantifying Relationships Between Photochemical
      Oxidants and Precursors," EPA-450/2-77-021a, Research Triangle Park
      North Carolina, November 1977.

  4.  N. C.  Possiel, J.  F.  Clarke,  T.  L. Clark,  J. K.  S.  Ching, and
      E. L.  Martinez, "Recent EPA Urban and Regional  Scale Oxidant Field
      Programs in the Northeastern  U.S.," Preprint, 75th  Annual Meeting
      of the Air Pollution  Control  Association,  New Orleans, Louisiana
      June 20-25, 1982.

  5.  U.S.  Environmental  Protection Agency,  "Northeast Corridor Regional
      Modeling Project  - Study Protocol," Office of Air Quality Planning
      and Standards, Research Triangle  Park,  North Carolina, September  1980.

  6.  J.  F.  Clarke,  J.  K. S.  Ching,  R.  M.  Brown, H.  Westberg,  and
      J.  H.  White,  "Regional  Transport  of Ozone,"  Preprint Volume,  Third
      Joint  Conference on Application of Air  Pollution Meteorology
      San Antonio, Texas, January 15-21,  1982.

  7.   W.  M.  Vaughan, M.  Chan,  B.  Cantrell, and F.  Pooler,  "A Study  of
      Persistent  Elevated Pollution  Episodes  in  the Northeastern United
      States,"  Bulletin  of  the American  Meteorological  Society, 63  (3)-
      258-266,  March 1982.                                          V  ''

 8.   Federal Meteorological  Handbook No.  3,  "Radiosonde Observations "
      Circular  P, U.S. Department of Commerce, January  1 ,  1969.
 9"  i'Son1?,^ Assurance Report, Detailed Hydrocarbon Analysis - NEROS/NECRMP
     an ^0^°^ Kepa!:ed by Washin9ton State University for EPA Grant No.
     oU-oooo, July ^7, 1981.
10.  "The Collection and Analysis of Ground Level and Aircraft Samples for
     Hydrocarbons in the Boston Area," Report prepared by Battelle Columbus
     Laboratories for EPA Grant No. 80-6683, November 21, 1980.

11.  H. G. Richter, "Analysis of Organic Compound Data Gathered During 1980
     in Northeast Corridor Cities," EPA Report in press.

12.  Federal Mister ,  Volume 44, No.  92, Pages 27558-27604, May 10,  1979.

13.  "Quality Assurance Handbook for Air Pollution Measurement Systems "
     Volume II,  EPA-600/4-77-027a,  Research Triangle Park,  North Carolina
     May 1977.
                                    40

-------
14.   W.  C.  Eaton and R.  S.  Wright, "Site Evaluations of Air Monitoring
     Stations of the 1980 Summer Northeast Corridor Regional  Modeling
     Project," Report prepared by Research Triangle Park Institute for
     EPA Contract No. 68-02-3222, TD-75, November 1980.

15.   R.  W.  Murdoch and F. K.  Arey, "Region II Northeast Corridor Regional
     Modeling Project Side-by-Side Verification," Report prepared by
     Research Triangle Institute for the U.S. Environmental Protection
     Agency, May 1980.

16.   J.  E.  Howes, Jr., "Air Quality and Meteorological  Measurements for
     the New York Metropolitan Area," Report prepared by Battelle Columbus
     Laboratories for EPA Contract No.  68-02-3529, October 10, 1980.

17.   "Report for Ambient Monitoring near the Town of Rising Sun,
     Cecil  County, Maryland,  and the town of Hickory, Hartford County,
     Maryland," Report prepared by Engineering-Science for EPA Contract
     No. 68-02-2537, November 1980.

18.   "Northeast Corridor Regional Modeling Project Continuous Nonmethane
     Organic Compound Data Collection," EPA-450/4-80-034, November 1980,
     Report prepared by PEDCo for EPA Contract No. 68-02-3519.

19.   W.  C.  Eaton, F. K.  Arey, and R. W. Murdoch, "Summary Report for
     Northeast Corridor Regional Modeling Project Performance Audits,"
     Report orepared by Research Triangle Institute for EPA Contract
     No. 68-02-3431, TD-11, November 1980.

20.   U.S. Environmental  Protection Agency, "Aeros Software Documentation -
     NAE67F, NAE67G," Office of Air Quality Planning and Standards, National
     Aerometric Data Branch, Research Triangle Park, North Carolina,
     June 1, 1979.

21.   J.  Wengert and R. Rutherford, "1980 Aircraft Monitoring in Washington, DC,"
     Report prepared by Northrop Services for EPA Contract No. 68-03-2591,
     April  1981.

22.   J.  Tichler, R. Brown, P. Daum, and D. Leahy, "Data Collected Aboard
     the BNL Aircraft and Van During NEROS 1980," Report prepared by
     Brookhaven National Laboratory for EPA Contract No. 79-DX-0533,
     August 1981.

23.   "Quality Assurance Document, Baltimore - Washington, DC Plume Study,
     NEROS-1980," Report prepared by Washington State University for
     Grant No. 80-6683, November 20, 1981.

24.   A.  Alkezweeny,  K. M. Busness, R. C.  Easter, and J. S. Wetzel,
     "Northeast Corridor Regional Modeling Project, Aircraft Measurements -
     New York and Vicinity," EPA-450/4-81-012, March 1981, Report prepared
     by Battelle Northwest Laboratories for  EPA Contract No. 68-03-2958.

25.   C.  W. Spicer,  G. M. Sverdrup, P. R.  Sticksel, J. R. Koetz, and
     G.  F. Ward, "Northeast Corridor Regional Modeling Project, Aircraft
     Measurements -  Boston and  Vicinity," EPA-450/4-81-013, March 1981,
     Report prepared  by  Battelle  Northwest Laboratories for EPA Contract
     NO. 68-03-2958.
                                      41

-------
26.  F. K. Arey, R. C. Schores, and R.  W. Murdoch, "Performance Audits of
     the NEROS/PEPE Sites," Report prepared by Research Triangle Institute
     for EPA Contract No. 68-02-3222, TD-98, March 1981.

27.  J. H. White, R. Strong, and J. B.  Tommerdahl, "Altitude Characteristics
     of Selected Air Quality Analyzers," Report prepared by Research Triangle
     Institute for NASA (NASA - CR - 159165), November 1979.

28.  W. P. Freas, "Northeast Corridor Regional Modeling Project - Data Base
     Description," Report being prepared by U.S.  Environmental  Protection
     Agency, Research Triangle Park, North Carolina.
                                    42

-------
        APPENDIX  A
AIR QUALITY / METEOROLOGICAL



      MONITORING SITES
             A-l

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-------

-------
      APPENDIX   B
SPECIAL MEASUREMENT DATES
           B-l

-------
Washington, DC


M
T
W
T
F
S
S











Date
July
14
15
16
17
18
19
20
21
22
23
24
25
26
27
28
29
30
31
Aircraft Pibals

x
x x
x x
x
x
x x
x
x x
x x
x
x
X X
X
X
X
X
X
X X
Rawinsondes Sodar
W T

-
-
-
-
- x
- x
- x
- x
- x
- x
X
XX
- x
- x
XX X
- x
X
XX X
Species
A Y_ K,

x
X X
X X
X
X
X
— —
X X
X X
X
X
X X
_ _
_ _
X
X
X
X X

X
X
X
X
X
-
_
X
X
X
X
X
_
_
_
-
-
_
_u

_
_
-
-
-
-

_
_
_
-
_
_
_
X
X
X
X
       B-2

-------
Washington, D.C.
Date
August
1
2
3
4
5
6
7
8
9
10
11
12
13
14
15
16
17
18
19
20
21
22
23
24
25
26
27
28
29
30
31
Aircraft Pibals
X X
X X
X
X
X
X
X X
X X
X X
X
X
X
X X
X
X
-
-
-
-
-
-
-
-
-
-
-
-
-
-
-
-
Rav/insondes
W T
X
X
X
X
X
X
X
X
-
X
X
X
X
-
X
X
X
X
X
-
-
X
X
X
X
X
-
-
X
X
X
X
X
X
X
X
-
X
X
X
X
-
-
X
X
X
X
X
-
-
X
X
X
X
X
-
-
Sodar
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
Species
A 1 K U.
X X
X
- X
- X
- X
X X
X X
X
- X
- X
X X
- X
- X
-
- -
- X
- X
- X
- X
- X
-
- X
- X
- X
-
- X
_
_ _
- X
- -
-
- X
- -
- X
- X
- X
- '-
- X
- X
- X
- X
- X
_
- X
- X
- X
- X
- X
-
- X
- X
- X
- X
- X
-
_ _
      B-3

-------
                               Washington, DC
Date

September
 1
 2
 3
 4
 5
 6
 7
 8
 9
 10
 11
 12
Aircraft
Pibals
Rawinsondes
W       T
                                            Sodar
                                               Species
                                            A   Y   K   U
 W:  Winds
 T:  Temperature
                A:  Aircraft
                Y:  West  End  Library
                K:  Takoma  Park
                U:  Univeristy of  Maryland
                                      B-4

-------
Baltimore


M
T
W
T
F
S
S











Date
July
14
15
16
17
18
19
20
21
22
23
24
25
26
27
28
29
30
31
Ai
S_
-
X
X
-
X
X
-
X
-
-
X
X
X
X
-
-
-
X
rcraft
IB
-
X
X
-
X
X
-
X
-
-
X
X
X
X
-
-
-
X
Pibal

X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
Rawinsondes
W
_
-
X
X
X
-
X
-
-.
-
-
X
-
-
X
-
-
X
T
_
-
X
X
X
X
X
-
-
-
-
X
-
-
X
-
-
X
Sodar
A
— —
X
X
-
X
X X
X
X X
-
-
X
X
X
X
_
X
- X
X X
Species
R
X
X
X
X
X
X
X
X
_
X
X
_
X
X
X
X
X
X

I
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
   B-5

-------
Baltimore
Date Aircraft
Sn
D
August
1 x
2 xx
3 xx
4 xx
5 xx
6 xx
7 xx
8 -
9
10
11
12 xx
13 xx
14 x x
15
16 -
17
18
19 -
20
21
22
23
24 -
25 - -
26 -
27 -
28 -
29 -
30 -
31 -
Pibal
x
x
x
X
X
X
X
X
X
X
X
X
X
X
X
-
-
-
-
-
-
-
-
-
-
-
-
-
-
-
Rawinsondes
W T
x
X
-
X
X
X
X
X
X
-
X
X
X
X
-
X
X
X
X
X
-
-
X
X
X
X
X
-
-
X
X
-
X
X
X
X
X
X
-
X
X
X
X
-
X
X
X
X
X
-
-
X
X
X
X
X
-
-
Sodar
x
x
x
x
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X •
X
X
X
X
X
X
X
Species
A R. I
X
X
X
-
X
X
X
X
-
X
X
X
X
-
-
-
-
-
-
-
-
-
-
-
-
-
-
-
_
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
-
_
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
_
_
    B-6

-------
                                    Baltimore
Date

September
  1
  2
  3
  4
  5
  6
  7
Aircraft
S     B
Pibal
Rawinsondes
Sodar
                                              Species
                                              ARE
  9
  10
  11
  12
  13
 S: Washington State University
 B: Brookhaven National  Laboratory

 W: Winds
 T: Temperature
X
X
X
X
X
-
-
X
X
X
X
X




X
X
X
X
X
-
-
X
X
X
X
X
""
A: Aircraft
R: Read St.
E: Essex
X
X
X
X
X
X
X
X
X
X
X
X
X



                                      B-7

-------
New York City
M
T
W
T
F
S
S











Date
July
14
15
16
17
18
19
20
21
22
23
24
25
26
27
28
29
30
31
Aircraft

X
-
X
-
-
X
X
-
X
X
X
X
X
-
-
X
Pibals Rawinsondes
GO W I
D N^ M D N_ M
X Y
X
/\
X
X
X
X
-
X
X
X
X
X
-
-
X
X
X
X

X x - X X - -
X x - X X - -
X X X X X X X
x x x x x x x
XXX XXX
x x x x x x x
X X X X X X X
V _ _ _ _

x - x x - x x
X X X X X X X




X X X X X X X
X— _



X X X X X X X
Sodar

_
-
-
-
X
X
X
X
X
X
X
X
X
-
-
X
Species
A L. N_

X X
X
X X
X X
X
X X
X X
X
X X
X X
X
_ _
X X
X
X
X X

X
X
X
X
X
X
X
X
X
X
X
_
X
X
X
X
       B-8

-------
New York City
Date
August
1
2
3

4
5
6
7
8
9
10
11
12
13
14
15
16
17
18
19
20
21
22
23

24

25
26
27
28
29
30

31
Aircraft Pibals Rawinsondes Sod
£ 0 W T
ID
x xxx
x xxx


x xxx
X XXX
x xxx
x xxx
x xxx
X


X XX
*» s\ /\
X x
- x
X
X




X
X
X
- - x
X




X
X
X
- - x
X


-
N
X
X


X
X
X
X
X
X




X
X
X
X




X
X
X
X
X




X
X
X
X
X



M
X
X


X
X
X
X
X
X




X
X
X
X




X
X
X
X
X




X
X
X
X
X



p.
X
X

X
X
X
X
X
X




X
X
X
X




X
X
X
X
X




X
X
X
X
X



N.
X
X

X
X
X
X
X
X




X
X
X
X




X
X
X
X
X




X
X
X
X
X



M
X
X

X
X
X
X
X
X




X
X
X
X




X
X
X
X
X




X
X
X
X
X




X
X

X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X
X

X

X
X
X
X
X
X


X
                                              Species
                                              A  L  N
                                              -xx
                                              xxx

                                              XXX
                                              xxx
                                              xxx
                                              xxx
                                              xxx
                                              -XX

                                              -XX
                                              -XX
                                              -XX
                                                X  X
                                                X  X
                                                X  X
                                                X  X
                                                X  X
                                                -  X

                                                X  X
                                                X  X
                                                X  X
                                                X  X
                                                X  X
      B-9

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                            New York City
Date
Aircraft
September
Pibals
G    0
Rawinsondes
  W      T
D N M  D N" M
                                                        Sodar
                                                                   Species
                                                                   A  L  N
  1
  2
  3
  4
  5
  6
  7_
  8
  9
  10
  11
  12
  13
                            XXX  XXX
                            XXX  XX-
                            XXX  XX-
                            - x x  - x -
                            - x x  - x -

                            X - -  - - -
                            - x x  - x -
                            - x x  - x -
                            -XX  - X X
                            - x x  - x x
                            XXX  XX-
                                  X

                                  X

                                  X
                                  X

                                  /\

                                  X

                                  X
                                  X
                                  X
                                  X
                                  X
                                  X

                                  X
 W: Winds
 T: Temperature
              G: Glen Cove
              0: Morristown
              D: Derby
              N: Newark
              M: Marlboro'
                            A: Aircraft
                            L: Linden
                            N: Newark
                                    B-10

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Boston
Date Aircraft Pibals
E M

M
T
W
T
F
S
S























July
14 x
15 x
16 x
17 x
18
19 x
20
21 -
22
23
24 x
25 x
26
27
28 x
29
30
31 x
August
1 x
2
3

4
5 x
6 x
7
8 x
9 x
10

x
X
X
X
-
X
-
X
X
-
X
X
-
-
X
-
-
X

X
X


-
X
X
X
X
X
-

X
X
X
X
-
X
-
X
X
-
X
X
-
-
X
-
-
X

X
X


-
X
X
X
X
X
-
Rawinsondes
_W T

..
-
-
-
X X
X X
x x
x x
X
-
x x
x x
_
_
x x
-
-
x x

x x
x x

™ •"
x x
x x
X X
x x
x x
X X
-
Sodar Species
A E: R

XX
XX
XX
XX
- X
XX
- X
_
X - -
x - x
X XX
X XX
x - x
x - x
X - -
X -
- X
X X
.
XX
- X

- X
- X
XX
- x
- X
x xx
x xx
x - x

X
X
X
X
X
X
X
X
_
X
X
X
X
X
_
X
X
X

X
X

x
X
X
X
X
X
X
X
   B-ll

-------
Date
August
11
12
13
14
15

16
17
18
19
20
21
22
23
24
25
26
27
28
29
30
31
Aircraft Pibals Rawinsondes Sodar Species
B M W I - - -
X - X X
- - XX X - X X
- - XX X - X X
x _-xx x - x x
--xx - -xx
-XX

x - x x
- - x x x - x x
- - xx x - x x
- - xx x - x x
- - xx x - x x
- - X X X '-XX
X - X X
X -XX
- - xx x -xx
- - xx x -xx
- - x x x -xx
- - xx x -xx
xx x - - -
x x x - - -
x x x - - -
September
  1
  2
  3
  4
  5
  6
  7
  __.

   9
   10
x
x
X
X
X
X
X
X
X
X
                                   B-12

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                                 Boston
Date      Aircraft    Pibals      Rawinsondes        Sodar           Species
September             B.   M       W       T_                          A  L  R

  11         -        --xx            x             _  _  .
  12         -        --xx            x             -  .  .
  13         -        -__-            x             ...
  14_        -        ....            x             _  .  .
  15         -        -   -       -       -            x             -  -  -
  16         .....                          	
W: Winds              B: Beverly Airport
T: Temperature        M: Medfield
A: Aircraft           E: East Boston
                      R: Watertown
                                   B-13

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|1 REPORT NO.

   EPA-450/4-82-018
                                     TECHNICAL REPORT DATA
                              (Please read Instructions on the reverse before completing}
                              1 .   —	—	•	'   I  5"c7
                               2.
|4. TITLE AND SUBTITLE
   Northeast Corridor Regional  Modeling Project

   Description  Of The 1980  Urban Field Studies
 7. AUTHOR(S)

   Norman  C.  Possiel and  Warren P.  Freas
 9. PERFORMING ORGANIZATION NAME AND ADDRESS

   Monitoring and Data  Analysis  Division
   Office  of Air Quality Planning  and Standards

   Office  of Air, Noise and Radiation
   U.S.  Environmental  Protectionj\gency	
 Il2. SPONSORING AGENCY NAME AND ADDRESS
  15. SUPPLEMENTARY NOTES
  16. ABSTRACT
             RECIPIENT'S ACCESSION NO.
             REPORT DATE
             October  B82
            . PERFORMING ORGANIZATION CODE
            13. TYPE OF REPORT AND PERIOD COVERED
                                                                14. SPONSORING AGENCY CODE
           »p  .




       (A data base for modeling Philadelphia  was acquired in 1979.    The IVBurie a
        tudies incLded continuous  surface measurements  of ozone   nxtrogen oxides,
   18 DISTRIBUTION STATEMENT
                                    KEY WORDS AND DOCUMENT ANALYSIS
                                                   b. IDENTIFIERS/OPEN ENDED TERMS
19. SECURITY CLASS (This Report)
  Unclassified
                                                    20. SECURITY CLASS (This page)

                                                      Unclassified
                                                                                  COSATI Field/Group
                                                                                       66
   EPA Form 2220-1 (Rev. 4-77)    PREV.OUS  ED.T.ON .s OBSOLETE

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