United States Environmental Protection Agency Risk Reduction Engineering Laboratory Cincinnati, OH 45268 Research and Development EPA/540/SR-95/505 May 1995 wEPA Project Summary Removal of RGBs from Contaminated Soil Using the CF Systems® Solvent Eixtraction Process: A Treatability Study Joseph Tillman, Lauren Drees, and Eric Saylor The United States Environmental Pro- tection Agency (EPA), through its Su- perfund Technical Assistance Re- sponse Team (START) and Super-fund Innovative Technology Evaluation (SITE) Programs, completed a treatabil- ity study to determine the effectiveness of solvent extraction in separating poly- chlorinated biphenyls (PCBs) from soil collected at the Springfield Township Dump (STD) Superfund site near Davisburg, Ml. The study consisted of a total of six runs, in which 100 Ib of dried soil was processed for each run. Based on pre- liminary analytical results, three 20-min extraction cycles were chosen as the most economical way to achieve the project objectives. Therefore, this three- extraction cycle condition was repeated twice to acquire data for three runs operated at the same condition. The other three runs consisted of two, four, and five 20-min extraction cycles. The results of the study indicated that on average approximately 98 per- cent removal of PCBs was achieved for the test runs using three extraction cycles. The four- and five-extraction cycle runs were the most effective in reducing the concentration of PCBs in soil, to 1.8 and 2.2 mg/kg, respec- tively. This indicated that the number of extraction cycles required for attain- ing the lowest concentrations of PCBs in product solids was greater than three but less than or equal to five since there was no discernible improvement in PCB removal from four to five ex- traction cycles. However, results from oil and grease analysis suggest that high&r removal efficiencies may be pos- sible with additional extraction cycles. Analysis of the filtered process wa- ter collected from all six runs indicated that PCBs were detected only in the filtrate from the two-cycle run [1.9 mi- crograms per liter [fig/L)]. PCBs were not detected (<1.0 ng/L) in the filtrate collected from the other five runs. This Project Summary was developed by EPA's START and SITE programs in Cincinnati, OH to announce key find- ings of a solvent extraction treatability study that is fully documented in a separate report of the same title (see Project Report ordering information at back}. Project Background EPA conducted a treatability study on soil collected from the STD Superfund site. The approximately 4-acre site is located near the town of Davisburg, Ml (Figure 1). Between 1966 and 1968 the STD was used for the disposal of drummed and liquid industrial waste. Primary contami- nants in the soil (a fine-to-coarse-grained sand) include: arsenic, lead, and barium; volatile organic compounds (VOCs); and semivolatile organic compounds (SVOCs), which include RGBs and the pesticide di- eldrin. Onsite incineration had been specified in the Record of Decision for remediating the soil at the site, but negative public opinion toward incineration has led to the consideration of treatment alternatives. Based upon preliminary bench-scale test- ing on soil samples taken from the site, Printed on Recycled Paper ------- SPRINGFIELD TOWNSHIP * DUMP Figure 1. Location of the STD Superfund site. the CF Systems® (CFS) solvent extrac- tion process was believed to be such an alternative. Therefore, a treatability study was conducted to determine whether the technology would be effective in treating soils at the STD to the desired cleanup standard. Approximately 1,158 Ib of soil were ob- tained directly from PCB "hot zones" at the STD site and then screened onsite to remove oversize material (>1/2-in. diam- eter), which was approximately 168 Ib (14.5 percent). Of the approximately 1,000 Ib of material screened to <1/2-in. diameter, CFS used approximately 150 pounds to conduct a series of bench-scale tests in order to establish basic operating conditions for the treatability study. The remaining volume was shipped to Hazen Research, Inc. in Golden, CO, which is the home base for CFS's Mobile Demon- stration Unit (MDU). The treatability study was conducted using CFS's pilot-scale MDU on a batch- mode. Liquified propane was the solvent chosen to extract the organic compounds from the STD soil. Figure 2 illustrates the basic CFS process and the sample loca- tions. At Hazen Research Inc., the feed mate- rial was air-dried, further screened to re- move oversize material (>1/4-in. diameter), and mixed to produce a homogenous test feed. Table 1 summarizes the results of the test soil screening for removal of over- size material. The contaminated soil was fed in 100-lb batches into the extractor and thoroughly mixed with approximately 150 Ib of sol- vent for each cycle. Following phase sepa- ration of the solvent and contaminants from solids, the solvent/contaminant mix- ture passes from the extraction system to the solvent recovery system. Once in the solvent recovery system, the solvent is vaporized from the contaminant, con- densed, and recycled back to the extrac- tion system as fresh solvent. After all ex- traction cycles are completed, water is added to the extractor and mixed with the solids to aid in removing any residual pro- pane. Product solids are discharged as a slurry in water and then filtered to form a filter cake. Test Objectives and Conditions The primary objectives for the treatabil- ity study were: • Determine the effectiveness of removing PCBs from STD soil to the remedial action standard (RAS) of <1 mg/kg. • Determine PCB concentrations in the filtrate water to ensure proper disposal. Secondary objectives of the treatability study included but were not limited to veri- fying the absence of PCBs in the pilot- scale unit prior to testing, determining re- sidual concentrations of dieldrin in the product solids, and determining mass bal- ance for total materials. The CFS pilot-scale treatability study was conducted in two phases, which in- cluded a total of five main process runs. Phase I consisted of three test runs, each consisting of a different number of extrac- tion cycles. The first run consisted of three 20-min extraction cycles, the second run consisted of four 20-min extraction cycles, and the third run consisted of five 20-min extraction cycles. Preliminary analytical results, using hex- ane as the extracting agent, indicated that the primary objective of producing solids having <1.0 mg/kg PCB concentration was met for the three-cycle run. Therefore, Phase II consisted of two additional test runs using three 20-min extraction cycles each, since this process condition was believed to be the most economically fea- sible in achieving the objective. It was later determined that these preliminary re- - -^- Process Path Used for Full-Scale System Only 0 Solid Sample Location £?; Liquid Sample Location Figure 2. CF3S Process Diagram. ------- Table 1. Percentage Of Screened Oversized Material Location Springfield Township Dump Hazen Research Inc. Starting Material (Ibs) 1,158 -626 Material Screened (Ibs) 168* 26» % Oversize ~ 14.5 -4.0 Total % oversize > 1/4nch ~18.Sc a Using plastic crating having approximately 1/2-inch openings. b Using an ASTM sieve having 1/4-inch openings. c Oversize material could be treated following size reduction (i.e., pulverizing) during a full-scale remediation. suits underestimated the concentration of PCBs in the treated soil. A sixth run consisting of two 20-min extraction cycles was added to test the limits of the pilot unit in treating soil to the desired levels. Table 2 summarizes the process condi- tions for all six runs. Analytical Results Sampling was performed in accordance with an EPA-approved Quality Assurance Project Plan. The critical process streams sampled for each of the six runs included: feed soil; product solids (filter cake); and filtrate water. Samples of the organic ex- tract were taken at the end of Run 6, in order to perform a mass balance on PCBs. Table 3 summarizes the MDU's PCB percent removal efficiencies for each run and as averages of all six runs and the three triple extraction cycle runs. Oil and grease (O&G) analysis was also conducted on feed and product solids for each test run to determine propane's capability in extracting semi- and nonvolatile organic compounds in addition to PCBs. Results of the O&G analyses are summarized in Table 4. PCBs were not detected in the filtrate samples collected for the five main test runs (<1.0 ng/L). However, for Run 6, which involved only two extraction cycles, PCBs were detected at 1.9 ng/L. The prod- uct oil collected at the end of the entire study (3700 g) contained a PCB concen- tration in excess of 11,000 mg/kg. This shows that the process was effective in concentrating the PCBs within the product oil fraction. Dieldrin was not detected in the feed soil nor product solids; therefore removal could not be evaluated. More detail of the analyses and measurements are dis- cussed in the Project Report. Mass Balance A total materials balance was conducted to account for all material loaded into the unit for each run and to ensure that the majority of the material was recovered and did not simply remain in one or more of the process components. Any material loaded into the unit or exiting the unit was examined in the total materials mass bal- ance. Table 5 summarizes the results of the total materials balance for each run and over the entire treatability study. Results indicate that approximately 98% of input material was accounted for in the product streams. The mass balance closure for PCBs was approximately 62%. The low recovery is believed to be at least partially attributable to the inability to drain all of the oil from the extract product tank and associated piping. Quality of the Data The data quality objectives established for this pilot-scale treatability study were based on project requirements and thus designed to ensure that the data gener- ated during the study would be of known and acceptable quality to achieve the project's technical objectives. There were several quality control analy- ses conducted to evaluate the laboratory performance. These results are discussed in detail in the full report. The critical Table 2. Process Conditions For All Test Runs Test Phase 1 II Run No. 1 2 3 4 5 Feed Loaded (Ibs) 100 100 100 100 100 No. of Extraction Cycles 3 4 5 3 3 Mixing Time Each Cycle (min) 20 20 20 20 20 Mixing Speed Full 0/FulP Full Full Full Solvent/ Feed Ratio (by weight each cycle) 1.5/1 1.5/1 1.5/1 1.5/1 1.5/1 Extraction Pressure (psi) Avg/Range 315/250-409 261/223-308 238/182-294 266/202-309 243/194-299 Extraction Temp (°F) Avg/Range 133/125-138 122/106-133 117/93-150 124/98-140 119/98-137 Added Run 6 100 20 Full 1.5/1 277/231-319 125/110-138 3 bottom. °ne °fthe f°Ur eXtraCt!°n CyCl8S' ^ miX6r WaS inoperable: however'a solvent «ow ™* established by recirculating propane from the top ofthe extractor into the 3 ------- Table 3. PCB Removal Efficiencies Run Number 1 2 3 4 5 6 No. of Extraction Cycles 3 4 5 3 3 2 Soil Feed Concentration1 (mg/kg) 210 240 340 3102 220 220 Product Solids Concentration1 (mg/kg) 4.9 1.8 2.2 4.& 5.8 19.0 Percent Removal 97.7 99.3 99.4 98.7 97.4 91.4 Average3 260/250 6.3/4.9 97.6/98.0 1 The test method used was SW-846 3540/8080; Aroclor 1254 was the only PCB identified. 2 Average concentration of analyses of field duplicate samples (see Table 7). 3 Two values are given; the first is the average of all six runs and the second is the average of the three extraction cycle runs (Runs 1,4, and 5). Table 4. O&G Removal Efficiencies Run Number 1 2 3 4 5 6 No. of Extraction Cycles 3 4 5 3 3 2 Soil Feed Concentration1 (mg/kg) 4480 4560 5870 5460 5140 7060 Product Solids Concentration1 (mg/kg) 112 73 <20 133 93 279 Percent Removal 97.5 98.4 >99.6 97.6 98.2 96.0 Average2 5430/5030 <118/113 >97.8/>97.8 1 Tho test method used was SW-846 9071. 2 Two values aro given; the first is the average of all six runs and the second is the average of the three extraction cycte runs (Runs 1,4, and 5). target analyte (PCB Aroclor 1254) was spiked into both a sample of the product solids and into a sample of the product water to determine the accuracy and pre- cision for these matrices. The results of these matrix spike/matrix spike duplicate (MS/MS D) samples (Table 6) show that accuracy and precision were obtained for both matrix types and that the project qual- ity assurance (QA) goals were met. Field duplicate samples of raw feed, product solids, product oil, and product water were collected and analyzed for RGBs. Field duplicates provide a mea- sure of precision for the combined samp- ling and analytical processes. Table 7 pre- sents these results, which show that the project relative percent difference (RPD) goal of 40 was easily met. It should also be mentioned that PCBs were not detected in any of the laboratory method blanks, nor in a rinsate sample collected from the pilot plant prior to the study, indicating that contamination was not a problem. Conclusions The analytical test data indicate that the primary goal of producing solids having a <1.0 mg/kg PCB concentration was not attained by the designated test method used. Of the five main test runs, the closest PCB concentration to the HAS was 1.8 mg/kg in Run 2 product solids, which was approximately a 99.3 percent removal efficiency. The average PCB removal ef- ficiency attained for the three-extraction cycle test runs was 98%. There is not enough PCB data to indi- cate whether the additional fifth extraction cycle conducted during Run 3 benefited Table 5. Total Materials Balance Run Number 1 2 3 4 5 6 Total Input (grams) Feed Soil1 45,400 45,800 45,800 45,800 45,800 45,800 274,400 Water 52,600 80,800 93,800 88,500 99,500 103,000 518,200 TOTAL 98,000 126,600 139,600 134,300 145,300 148,800 792,600 Output (grams) Oil Extract 3,700 3,700 Slurry 71,600 147,400 1 16,200 134,800 141,200 158,800 770,000 F-1 Filter Solids 485 485 485 640 640 640 3,380 Total3 72,090 147,900 116,700 135,400 141,800 163,100 777,000 (%) Recovery Material 73.6 1172 83.6 101 97.6 110 98 1 Runs 2-6 Includs the addition of 454g of sand to fill void space in the extractor. 2 Solids not flushed out In Run 1 exited at the end of Run 2. 3 Totals rounded to four significant digits. ------- Table 6. PCS Aroclor 1254 Matrix Spike/Matrix Spike Duplicate (MS/MSD) Results Sample Spike Sample Cone. MS MS%R MSD MDS % R1 RPD* Product Solids Filtrate 4.9 mg/kg 10.0 ug/L 4. 1 mg/kg < 1.0 ug/L 8.2 mg/kg 9.0 iig/L 84 90 9.1 mg/kg 7.8ng/l. 102 78 10 14 1 The OA objective for accuracy was a recovery of 50-150 percent. C'-C, % Recovery -- x 100 where, 2 The OA objective for precision was an RPD of<40. (Maximum Value - Minimum Value) C1 is the measured concentration in the spiked sample C0 is the measured concentration in the unspiked sample C, is the known concentration ofanalyte added to the sample HPD (Maximum Value + Minimum Value)/2 x 100 Table 7. PCS Aroclor 1254 Field Duplicate Results Sample Matrix Sample Result Result 2 RPD' Feed Product Solids Product Oil Filtrate 350 mg/kg 4.0 mg/kg 1 1,200 mg/kg < 1 ug/L 260 mg/kg 3.9 mg/kg 1 1,300 mg/kg < 1 ug/L 30 2.5 0.9 NC ' The project objective for precision was an RPD of<40. NC = Not calculated PCS removal beyond the four-extraction cycles conducted during Run 2. The two concentration values, for Run 2 (1.8 mg/ kg) and Run 3 (2.2 mg/kg), are essentially equal since they are within the range of field sampling and analytical error. How- ever the O&G analytical results can be used to supplement the interpretation of results, with respect to organics removal in general. As Table 4 indicates, when the O&G data is evaluated, the five-ex- traction cycles used for Run 3 appears to have performed the best for overall or- ganics removal. The performance of the runs relative to one another is illustrated in Figures 3 and 4. These show the removal of RGBs and O&G, respectively, for each test run as the decline in contaminant concentration from starting feed to product solids as sloped lines. Both figures show the dis- parity in performance between test runs for the respective parameters, which may not be as apparent when simply looking at percent removal values. Figure 3 clearly shows that Runs 2, 3, and 4 came closer to the test objective, assuming a feed concentration equal to the average of all runs (250 mg/kg). Their slopes essentially parallel one another. Figure 3 also shows that Runs 1 and 5 had an almost identical performance and that Run 6 had the poor- est performance. For O&G removal, Fig- ure 4 indicates that Run 3 produced the "cleanest" solids, while Runs 1, 2, 4, and 5 had similar performance. Again, Run 6 had the poorest performance, indicating that greater than two extraction cycles are required to achieve O&G removal efficien- cies > 96%. These results suggest that the extraction process operating condi- tions could be further optimized to yield higher removal efficiencies than were iden- tified in this study. Another important conclusion that re- sulted from the study regarded the vol- ume reduction of hazardous waste. Al- though the CFS solvent extraction pro- cess is not capable of destroying PCBs and other contaminants present in the STD soil (as is the case with solvent extraction technologies in general), it is a means of separating those contaminants from the soil, thereby reducing the volume of haz- ardous waste that must be treated. This in turn reduces the cleanup costs involved. The cumulative mass of the wet contami- nated feed soil for all six runs of the treat- ability study was approximately 274,000 g. The mass of the oily extract sampled at the completion of Run 6 was approximately 3,700 g. Therefore, the process reduced the overall mass of the contaminated material to 1.35% of its origi- nal waste mass. The volume of the feed soil [SG=1.34 g/mL and oil extract (SG=0.87 g/mL) were approximately 204 and 4.3 L, respectively. Therefore, the process reduced the overall volume"of the contaminated material to 2.1% of its origi- nal waste volume. The highly concen- trated oil extracted from the CFS process is either destroyed by incineration or chemical dechlorination. ~ The full report was submitted in fulfill- ment of Contract No. 68-CO-0048, Work Assignment No. 0-50, by Science Appli- cations International Corporation under the sponsorship of the U.S. Environmental Pro- tection Agency. ------- D) I If) CO o g g o O CD 400 300 200 100- MJ Run No. — — . Test Objective " 3 extraction-cycle runs —•— 4 extraction-cycle run —— 5 extraction-cycle run 2 extraction-cycle run 12345 i 1 — 10 15 Product Solids Concentration (PCBs in mg/kg) 20 Figure 3. PCB removal trend. 7000 - "55 E 6000 _c CD O 5000 | g 4000 § 8 0 3000 •o CD <9 2000 1000 *» *. ». ». •^ •» •. •. > •• \ \ "\ V\ \ r^ \ y&% "\ **••. IXX^S "-® I \\ \ X \ * \ \ (3) ^2) \\ 'T \ % ( 1 / '*'*** • * ^i^t. **"* l \ VN S 1 \ A7-N ** ** 1 , \ ®, \ \ . © Run Ho. ••""•• 3 extraction-cycle runs — «— 4 extraction-cycle run — — 5 extraction-cycle run • •• •• 2 extraction-cycle run »4 •» •. *. •» * » »» ». »» ». •• •. •. •» •. 30 50 100 150 200 250 Product Solids Concentration (O&G in mg/kg) 300 Figure 4. Oil & grease removal trend. ------- ------- Joseph Tillman, Lauren Drees, and Eric Say/or are with Science Applications International Corporation in Cincinnati, OH 45203. Mark Meckes is the EPA Project Officer (see below). The complete report (Order No. PB95-199030; Cost: $19.50, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Risk Reduction Engineering Laboratory U.S. Environmental Protection Agency Cincinnati, OH 45268 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati, OH 45268 Official Business Penalty for Private Use $300 BULK RATE POSTAGE & FEES PAID EPA PERMIT No. G-35 EPA/540/SR-95/505 ------- |