UntedSutM
Envwonmafltai Protection
AQ«ney
Offio»Of
Wat«r
(WH-6SOGJ
EPA57IVWI-010
ApriM991
A Review Of Methods For
Assessing Nonpoint Source
Contaminated Ground-Water
Discharge To Surface Water
                         Printed on.Recycled Paper

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 A Review of Methods for Assessing Nonpoint Source

Contaminated Ground-Water Discharge to Surface Water
                     April 1991
          Office of Ground-Water Protection
         U.S.  Environmental Protection  Agency

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!          J

                                                                                                                               i!      II
                                                                                                                               II  '   II
                                 ii!  a SB. I!

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                              Table of Contents
.A
                               .                      .....
I. '   Introduction  ......... .-.- • ; '.*'*• .....  '  '
    '.            "       .         /    •''.'        •       '   '        .'.... ~' 1
      A.    Purpose of -this report   .,.....•••  ......
        -'•'•''      .              •'''•-••         •                .  .   2
    .  B.    Organization of this report  ......•••••••••
II    Methods for Measuring or  Estimating Nonpoint  Source  Contaminated       ^
      Ground,- Water Discharge  to  Surface  Water  .  .......••••••
             Studies  involving use  of seepage meters or mini piezometers  ;     •
           •  to  measure ground-water discharge  to  surface water. .. ...  ..*.

       B-  -.'  Ground-water quality sampling and ^asurements^of ground- .
         '    water flow to estimate loading to surf ace . water ..... '  ' '
       C     Studies involving geophysical techniques to estimate ground-     ^
             water discharge to surface water  ......•>••••••
       D.    Studies involving hydrograph separation, regression^     :
           •.  analysis, or mass balance approaches to estimate  the
             contribution of  ground  water to stream flow .........
       E    ' Numerical models of surf ace -water/ground- water interactions .    54'
              use types
        G     studies 'using -environmental isotope methods ^ to estimate the
         '   '  contri'bution of ground water to stream flow . ...... ,  •  •


        Total Maximum Daily L6ad and Waste Load Allocations ......

        A.-   Statutory and Regulatory Mandate for Determining WLAs  and ^  ^    g&
              LAs under the TMDL process   .  . ......  ••.-••
                                                                               88
         B     Determining the  total maximum  daily load  ...  •  . .....  -..
               Waste Load Allocation
             '  .'. ,   :
         D.     Summary ..••••••.*'

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niiiiii	i1
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                                    Chapter  I

                                  Introduction
 A.    Purpose of this report

       This report presents a summary of methods that have been applied to
 measure or estimate nonpoint source contaminated ground-water discharge  to
 surface water.  The U.S. .Environmental Protection Agency (EPA) Office of
 Ground-Water Protection  (OGWP) developed this analysis as part of an effort  to
 broaden the understanding of the manner in which human activities can affect
 water quality in all phases of the hydrologic cycle within a watershed.  EPA
 undertook this project in response to the-growing awareness tha.t contaminated
 ground-water discharge is a significant source of nonpoint source contaminant
 Loading to surface waters in many parts of the country.  In particular,  this
 report is intended to stimulate understanding of the methods that may ~be
 applied to better account for nonpoint sources of contaminant  loading.
 'Improved characterization of nonpoint ^source loads  to surface  water may,' in
 turn lead to.more comprehensive approaches for setting  total  maximum daily
 loads for surface waters and waste, load allocation.1  This report provides an
 overview of  these methods,  rather  than a manual for employing  the methods
 presented.   Readers  who  intend  to  apply the methods summarized here should
 study the primary references cited.                        .   '   • .

       While  ground water and surface water are  generally thought of as
 separate  systems,  they are  highly  interdependent  components  of the  hydrologic
 cycle   The  hydrologic cycle refers  to  the circulation of water  among soil,
 ground  water,  surface water, and the atmosphere.   Within a watershed,  water
 may enter the basin through precipitation,  upstream inflow,  and ground-water
  discharge   Water leaves the watershed through downstream -outflow,     ,  •
  evaporation, and ground-water  outflow (see Figure 1-1).   Some,rainwater never
  reaches surface water due to the evaporation of intercepted rainfall from
  vegetative surfaces and the.soil matrix and transpiration of -water by.plants,
  returning water'vapor back into the atmosphere.                   .

        Rainfall that reaches surface water may travel to the stream or lake  as
  subsurface storm runoff, overland flow,  or ground water.  In most humid
  environments, about 80,  percent of rainfall will infiltrate into the s^oil '
  -ather than travel by overland flow.  Overland flow is more predominant in
  semi-arid rangelands, roadways, and*cultivated fields in regions with high
  intensity rainfall.  Rainfall that percolates into the soil matrix is held  by-
  capillary forc'es.  As the soil moisture increases, older, soil water is
  displaced and percolates laterally and/or vertically.  Lateral percolation  may
  eventually  enter streams as subsurface storm runoff, while vertical
  percolation generally enters the saturated ground-water zone.  Ground water
  moves more  slowly than  subsurface, storm runoff and will eventually discharge
'  and provide water to streams, wetlands, and lakes.
      .  i See Chapter  3  of  this document  for  a. discussion  of  total maximum  daily
   load  and' the waste, load allocation process.                          ,      r.

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      Host streams  and lakes' are surrounded by bank storage zones that
increase during  storm events.  During a rainstorm,  precipitation entering
increase Curing  "°™       content which are closer to the stream displaces
«•«. of *£*•?"• s^aeer ^ereby providing the  stream with water from bank
Che **fisr ^g^^^e topsoil is underlain by a less permeable
        ; waterlccumiateTabove that horizon and flows downhill through the
        This  represents a shorter route to the stream*.
          soil.
           surface water and the methods  that have been developed and applied for
           assuring this Kbnpdint source loading to surface water.

                 In preparing this report,  EPA contacted over 100 individuals who are



           proKssioniriiterature.  .This report represents a synthesis of the
           information collected from these sources .                .


           B.    Organization of this report

                 This report is organized in  three  chapters.   Following this








           • K companion volume  to this  document.   ,                       •
            ::":  "2  	 '	Dunne/Thomas	" and Luna B.  Leopold:  "tfnrff In Environmental
            ."Planning.  W.H. Freeman and Company,  1978,  pp.  255-277.
                  'See  "Ah Annotated Bibliography to  the            ^^
            Source Contaminated' Ground- Water  Discharge to Surface Water,  EPA
            006.
	il.taiS;;•;	iat	;•• i• «•	;, r,;:> .„•• •„:•.•» t j*'r	i' ;: ;"" •  • . • ..fi• ',.."j	 :-•. :.• •':;;;• - .• i, •: ;	  ,:••./ „
        ti	:::,,!i Illllli:!1!,	|:>!;	Ui!!!,:	luii!!,M1 •.';• ilIilil^i£'[:;>Er;lt^        X ,'i	tiH,	i:. •:	''H'^Hritii:",!:;	!i	''>iii1,';, <, ';]•>-!'i>':'t':	<

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                                        Figure 1-1
                         '•^•/-.V Cfcuria f«ttf to toil :.:/ji> v:V-V-:'"X'.>^t.v':i«V;'.:/SS
                      •..;./:.•/'.•'•/•; fyauna 
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Ill 1 1111
 1111
111 111   I I1 II1     111 I
111 111  I I III  II
II 111 111 111   I I
                                  Chapter II

Methods for Measuring or Estimating Nonpoint Source Contaminated Ground-Water
                          Discharge to Surface Water
 ill 11.     	    I I Hill  I           ill                !|       1     i1 . • > '••',.       •

Introduction

      Seven groups of methods have 'tee'n'identifiedin the literature for
measuring or estimating  contaminated  ground-water  discharge to surface water.
Each section of this chapter presents a  general  description of the method,
assumptionsand limitations for  the method,  summarizes the data inputs and
output^for the method,  describes the environmental settings and contaminant
types th"at"fiavebeen evaluated using  the method, and presents  a general
evaluation of  the suitability of the  method for  other applications.  Each
se'ctionalso" concludes with tables  summarizing  information presented in the
companion volume to thisdocument,^it Annotated Bibliography to the
LiteratureAddressing Nonpoint Source Contaminated Ground-Water Discharge to
Surface	Water,*	EPA	450/6-90-006". 	^	;	:   '            ,

  	 A1	:limiMionl':commdn::'l't'6	'"all	of the  methods	discussed in this report  is
the high"degree of uncertainty  inherent  in the  study of ground .water.  The
heterogeneity  of  geologic formations presents a major problem in ground-water
study   Fdr eicample,  hydraulic'conductivity values can range from 10   cm/s  to
less than  10"10 cm/s  in different geologic settings.  Furthermore, hydraulic
conductivities and other hydrogeologic  parameters  can vary significantly  over
even small distances.   Thus,  errors inherent in ground-water parameter
estimates  can  vary by 50 percent or more,  whereas  an acceptable error for
surface-water  work  is about 10  percent.   As a result, the reader should note
that the methods  described in this chapter may inherently encompass broad
ranges  of  uncertainty in their estimates.
            •=-•"••" "gtu:diei involving use of seepage meters or mini-piezometers to measure
                   ground-water discharge to surface water

                   The papers cited in this section are summarized in Section I of  "An
            ' Annotated Bibliography of the Literature Addressing Nonpoint Source^
             Contaminated Ground-Water Discharge to Surface Water," September 1990,  EPA
             440/6-90-006    	   ,'_  .'_'	[['''''.'	[	,  ". 	,"'"'''_	'II'''  "J  '    ''.'''


                   i.    General description of method  •

                      a.       Description of method or procedure

                   Seepage meters and mini-piezometers may beused  to measure  the  quantity
             and quality of ground water discharging to surface water.  These methods
             ieasurea"point-location" ground-water discharge rate  and allow  for  water-
             quality sapling  over a very  small area at the s»rface-wa"r/sedil!";*    . .
             interface.  In order to characterize  larger  areas,  several measuring/sampling
             pointsr';::muit:	be	selecteH:	Areas  with  different sediment types  maybe  mapped
             and several seepage meters/mini-piezometers  installed in each-sediment type.

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The  total  discharge and loading rate to the surface-water body as a result of
.ground-water discharge can be estimated by applying average measurements per
sediment type to the entire bottom area.  Alternatively, reconnaissance over a
large area may be used to identify areas where the greatest quantity of   ,
contaminants is entering the surface water body.   Seepage meters and mini-
piezometers may then be used to monitor and quantify discharge zones.       •

  '-.'' Seepage meters and mini-piezometers have been used to investigate  -
 ground-water discharge into lakes, streambeds, and marine environments   They
 are best suited for use in moderately permeable soils and relatively quiet
 waters  but adaptations allow successful use .under more adverse conditions.
 They may be used in combination with one another or with piston corers^to
 analyze soil permeability, ground-water quality,  "*• J«^-WJJJ "j^J"-
 An important function of these methods .is to provide field, verification  for
. geophysical techniques that may be used to estimate ground-water discharge to
 a surface water body  (see  Section II..C).                  '                . \
       Seepage Meter'
       In its simplest  form, a  seepage meter can be a  55-gallon  drum with  the
 bottom cut off and  a vent hole placed in  the closed end.  The open end pf.the
 drum  is pushed into the bottom sediments  of the surface-water body until  only  ,
 the closed top of the  drum  is  exposed (Lee, 1977),  The vent hole  remains
 unstoppered and  the seepage,meter  equilibrates with .the sediment environment.
 After several days, a  collection system consisting of a tube and a deflated
 bag is attached  to  the vent hole (see Figure 2-1).  One can use seepage meters
 to estimate discharge  velocity of  ground  water tq surface water. Dividing the
 collected volume of seepage by the duration of the collection period and  by
 che area of  the  seepage  meter produces  an estimate of ground-water; discharge
 •velocity:  Multiplying by. the surface area of the stream  or lake bottom
 estimates  the  total ground-water discharge rate  through that area.

        Provided that consideration is given to  chemical alteration, seepage.
  meters  might be used to determine ground-water, quality from collected seepage
  samples.   Multiplying the measured chemical constituent concentration in the
  seepage by .the calculated ground-water discharge rate to the surface-water
  body estimates the constituent's loading to the surface water  (Goodman et al.,
  1989).     .       .  ••       •'••'•-..     ' (                 -   '

        Mini-piezometer             .  •                   .

       '.  Description  and installation     •            .

   -    ' Piezometers  are devices consisting of pipes, with slotted tips  or well-
  points on £he end.  They are  used to measure hydraulic head in saturated
   geologic materials.   Piezometers  are usually installed: in  machine-drilled_
  boreholes.  Mini-piezometers  are  similar to piezometers,' but -are.*"!!«• »»~
   size and installed manually.  A mini-piezometer  consists of a  —"-«••£«;
   tube perforated over  a  short distance  .at ;one end.  Nylon mesh  covering the
   perforated tube keeps sediment  from clogging the mini-piezometerTo place a
   mini-piezometer,  a length  of thick-walled pipe,  with an  inside diameter
   slightly larger than the  tubing,is hammered into the sediment. A temporary
                                          5  :

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                                 Figure 2-1
                              water surface
                 Full section view of seepage meter showing proper
        placement m. the sediment.  A. 4 liter. 0.017 mm  memerane
        plastic Baggies Alligator bag  (open ,end was heat  sealed): B.
        rubber-oand wrap;  C.' 0.64 cm inside diameter. 6 cm long,.
        polyethylene tube:  D. 0.79 cm inside diameter. 4,5 cm long,
        amoer-tatex  tube: F.15 cm "x"5?"cm"diameter epoxy-coatea
        cylinder  (ena-sectidri  ofa"st'eei drum).
 	   Lee "David R.;  and John A.  Cherry:   "A Field Exercise on Ground-Water
Flow Using Seepage  Meters and Mini - Piezometers," Tnnmnl of Geo^^g.
Sducacion.. 1978. Volume 27:  p. 8.

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 plug attached to the end of the pipe keeps sediment from entering the pipe
 during placement. .  The plug is knocked free before the mini-.piezometer is
 inserted to the bottom of the pipe, perforated tip first   The mini-piezometer
 tube is held in place as the length of pipe is removed   .The pipe used in    •
 installation may be pulled back to expose the perforated section but left in
 See to providJ added protection to the tubing.  A collection system similar
 to the.seepage meter tube and collapsible bag system can be .used to.collect
 seepage samples  (see figure 2-2).

          Mini-piezometer variations                                .

       One difficulty often associated with the installation of mini-
 faiezometers  is  their tendency to move before the sediment collapses around the
 ' Ptubr« if the  tube is pulUd later on.  Lee and Welch  (1989) have  tested a
 harpoon piezometer which helps  to  alleviate this problem  (se^Figure  2-3)
 -Krbs" on the  tip of  the piezometer grip the sediment  and help  to  keep  the
 screen at the desired  depth  as  the driving rod, or pipe,  is.withdrawn or if     •
 the  screen in moved during use.                 _

        Another variation of  the  mini-piezometer  is  the bundle-type  mini-
 piezometer,  consisting of  several  small tubes placed within the  pipe  at  one
 time   The  tubes are  placed at selected depths  to  allow detailed vertical
 resolution of head and pore-water  chemistry at  the selected mini-piezometer
 location.  .If bundle-type  mini-piezometers' are  placed at selected  points along.
 a vertical  plane,  patterns of flow and geochemical processes in the subsurface
 are observable.                    .             .

           Mini-piezometer measurements

        An alternative to direct measurement of ground-water discharge is to use
  hydraulic conductivity and hydraulic head data obtained from mini-piezometers
  to calculate the ground-water discharge rate to surface water using Darcys
  Sw   Comparing the Hydraulic head in the mini-piezometer with the hydraulic
  htad of the surfac-e-water body determines the hydraulic gradient across bottom
  sediments.  Hydraulic head differential may be measured using a manometer (see.
  Figure 2-4) or  a continuous water level recorder (see  Figure 2-5).  Head
  differential is divided by  the depth of the piezometer screen below the      - ..
 . leolment-water  interface to obtain the vertical hydraulic gradient   Hydraulic
  conductivity of the bottom, sediments may be estimated  or be ^asured using
  either a constant head or  falling head test.  A constant head test has been
' developed using sections of sediment.cut directly from a thin-walled piston ,
  core  barrel (Munch  and Killey, -1985).   Once the hydraulic  gradient and^
  hydraulic  conductivity have been  determined, Darcy's Law may be used to
   determine  the  ground-water flux through the  sediment  (see  Section A.i d).
  Multiplying the calculated- flux by the surface area of the  surface-water
   bottom "yields.the ground-water discharge rate  to  the  surface-water body.

 'The  mini-piezometer yields  seepage samples  using a syringe  or  other   ^
   sampling device   Multiplying the measured chemical constituent concentration
  '•ItTSHround water by ?he calculated .ground-water "discharge rate yields the
   loading rate to surface water.                                 .

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                                               Figure 2-2
           II	Fill	I I,1., (":„;(•',,,"!	,	I'*
                              General fea'tures and method of installation of a mmi-
                     Diezorneter. A. casing driven into the^ sediment: B. plastic tube
                     with ""'screened1' tip	mserteci	'in	f^e"'casing;' C, plastic tube is"-a
                     '{Mzd'rn'eter arid iridi'dales differential .head -(h) with respect to the
                     surface water: 0. plastic bag attached to the piezometer collects
                     sediment-pprewster.	•„	.ci	'	,	•
           	  Lee, David R.,  andJohn A. Cherry:   "A Field  Exercise on Ground-Water
          Flow Using Seepage Meters and Mini-Piezometers," Journal'  of Geologic
          Education. 1978, Volume 27:  p. 7.
i	in 11 i
                           !•;, :tl ..... L 4: ..... M l..i' ...... lie ..... ....... IB; t'lii ..... ill ..... 'i l:> ::: »^!!iJ:::i
                                                          .ki!:!!1;, '
                                                                 i ££ i !», ...... V-ilU .'I.'.'!, '

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                                      Figure 2-3'.'
                           1/4" O.D.
                           polyethylene
                              Cubing

                     240 ayIon atsh
                        3/8" 0.0. polyethylene cub*
                                       groove  to,fit,.
                                       drive rod
                           polyethylene  tip
*t«inlt««-»tt«l wire
to secure  two tubes
            Harpoon piezometer tip, screen and tube.  Dimensions for the small
            type are shown here. The screen is 10 cm iong, has 8 1/4* diameter
            perforations and is covered with 3 layers of 240 M«D mesh tightly
            rolled around the 3/81 O.D. polyethylene tube to prevent entry of
            sediment.  The drive rod, not shown, fits loosely in groove.  The
            •barbs'  are folded back before driving in sediment to ensure that
            they grip in the sediment.                                   •
       Lee,  D.L.  and S.J. Welch;   "Methodology "for Locating and Measuring.
 Submerged Discharges:  Targeting  Tool,  Harpoon Piezometer arid  More,"  FOCUS
•Conference on Eastern Regional Ground Water  Issues,"  Kitchener,  Ontario,
 Canada. October  17-19, 1989.,,p. 8.   '    . •  •                          ' .•

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                                       Figure  2-4
                     •*•  -
                     •'".
                     '•K.
                                                     rubber bulb
                                                 B
                                              • ••I !••'
                                                clear »U«iie
                                                ••(•r slick
                                                  t» III
                    £•*
                    The manometer used to measure differential heads in
           miniDiezorneters.  A.  principle of  operation: B.- the field ap-
           paratus!	":	'" :'	'.'
  '';'''•;' "','"• Laa, ,',Davtd  %..,  and'John'. A,	'.Cherry:	"A'Field Exercise  on Ground-Water
,'F|,ow Using Seepage  Meters and Mini-Piezometers, M	journal of  Geologic
 Education.  1978	". "Volume' 27r	p".	.8".'	:	
                                           10

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                                   Figure 2-5
            wartr
            levti
            rtcoratrsv

                  Continuous measurement of head differences between
            piezometrjc level and river level using two water-level
            recorders.
      Lee,  David R.,  and Stephen J.  Welch:   "A Method for  Installing and"
Monitoring  Piezometers in Beds of Surface Waters," Ground  Water.  1989, Volume
27(1): ' p.  -89.        .     -,  "-       ..  '   '
                                        11-

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  ill	i M IM 11 «    11 nil
      In geologic units having permeabilities too low to allow  easy withdrawal
of waterfrom a piezometer tip, a piston corer may be used  to obtain  a
continuous vertical profile of sediment (Lee, 1988).  Munch and Killey  (1985)
have used a modified piston corer featuring a thin-wall core barrel and
wireline recovery to sample both cohesive and cohesionless  sediment frpm
depths up to 30 m below the watertable.  The porewater can then  be extracted
from the piston core for chemical analysis.                       .

         b.       Assumptionsinvolved in using  seepage meters  and mini-
  	       i     i .piezometers

          Flow  rate  is  uniform  through the  sampling interval

       Seepage  meters and mini-piezometer infer that  measured ground-water
quantity  and quality are representative .of  actual  conditions throughout the
stapling  interval.  The ground-water discharge rate  recorded using a  seepage
''meteror mini-piezometer represents the average  ground-water discharge  rate
for thecollection period.   If asingle discharge  measurement or  a series of
discharge  measurements recorded over a short time  period are used to  determine
the ground-water  discharge  rate to  a surface-water body,  the calculated
discharge rate may vary from actual rates.              •   .

          Sampled interval_is representative temporally

       A series of discharge measurements  taken over a short duration can vary.
 substantially due to tidal cycles,  storm events, and seasonal changes.
 Furthermore;seasonal variations within and between years' may be substantial.
 It is possible that a series of discharge measurements recorded over a  long
 duration may' hot be representative of actual conditions if  the measurements
 were recorded in excessively wet or dry years.          ,

          Sampling placement is representative spatially

       Seepage meters and mini-piezometers"provide ppint measurements that
 determine the ground-water discharge  rate and.loading rate  to a surface-water
 body through extrapolation (Goodman et al., '1989).  The representativeness of
 the sampling locations and the number of locations  influence the accuracy  of
 the"results.  For example, Belanger and Connor  (1980) not  only found
 decreasing seepage rates with increasing distance from shore, but also  that
 ground-water recharge occurred toward the center of East Lake Tohopekaliga.
 An overestimation of  ground-water  seepage would result if  seepage meters used
 in the study were all located near shore.  Conversely, if  all  the seepage
 dgters were located towardthe center of the lake,  one would erroneously
 conclude  thattheentirelake was  recharging ground water.

           Measured samples  are 'repres'enta^i've'bf ground-water dischar&e.
	  oUalitV      "     -           •                          '             ,
  	,	 „	Measured ground-water quality may not be representative of actual
  conditions' because of interactions "occurring at the sediment/surf ace .water
  interface   Belanger and Mikutel (1985) concluded that direct determination of
  water quality using seepage meters overestimated nutrient loading to lakes due
  to  the  enclosure of bottom sediments, which results in anaerobic conditions
                                        12
                                     1 S'i"'",,,' . II	i" •!,"!•

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and increased release rates of ammonium, nitrogen, and phosphate.  In
addition, seepage .meter or mini-piezometer samples from shallower, shoreline
locations may be influenced by bank storage water. •

         c.       Limitations of the methods            	              .

         Placement on different surface-water bottoms                   . .

      Not all bottom areas of a surface-water body are conducive  to
installation of seepage meters or mini-piezometers.  Because seepage meters
and mini-piezometers require insertion  into bottom sediments, ideal
installation locations-are areas with relatively soft, fairly thick,
moderately permeable sediments containing few cobbles or stones.  However,
German has successfully installed seepage meters in cobbles and rocks using
bentonite placement.* ,

         Deep  surface waters require additional expertise and equipment   ..

       Seepage meters and mini-piezometers_ located in deep water  require scuba
abilities and  equipment for installation, sampling,' arid maintenance.  Depths
that limit divers' safe performance control installation depths  (Woessner  and
Sullivan, 1983).  Additionally, some bottom locations are not suited to
installation of seepage meters and mini-piezometers.

         Strong currents and harsh  seasons

      Without  modification, mini-piezometers and  seepage meters  should  not be
used w-ith strong  currents.  Acceptable  installation locations vary with
seasons  in areas  due to wave and current action.  Additionally,  in colder
climates, ice  covering surface waters may limit seepage meters and mini-
piezomepers sampling and maintenance activities.    .

      Sklash has  overcome  some of these problems.5  In his investigation,
handles  placed on seepage  meters aided  divers  in  fast currents.   Also,  once
the seepage meter is placed, bolts  are  used to clamp  it.down 'and ensure its
stability.  To protect seepage bags  from  the elements;  Sklash used rapid
disconnects for .the bags and placed rigid containers  around'them.       .  .


          Maintenance       —               .  '•    ' •    •    '  '  .      •

       Seepage  meters  and mini-piezometers equipped with sample  collection
 devices  require" substantial.maintenance;  Without frequent  changes,  the
 increased pressure associated  with  a full catchment  device  reduces  the  amount
      4   German,  Dave,  personal  communication,  Nonpoint  Source Contaminated
 Ground-water Discharge to Surface Water Workshop,  Chicago, IL, November. 30,.
 1989.        '-"..'•"'•,'•        '''.".-.-'.

      5   Sklash,  Mike,  personal  communication,  Nonpoint  Source Contaminated
 Ground-water Discharge to Surface Water Workshop,  Chicago, IL, November 30,
 1989.   '            ,        ,                  •               -•-._.-'•.

        ','-.'         •   " .     -    ' '    13''   '  -     . - •       '           ' -   .

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          of ground-water flow into the seepage meter.  The  sample collection tubing for
          seepage1 ietersIhd mini-piezometers requires  regular cleaning or replacement
          co preventalgae growth.  There may be a need to periodically replace seepage
          meters and iinf-piezbmetersdue to wave and current action.

                   Anaerobic environment within equipment

                A final limitation of seepage meters and  mini-piezometers is that
          anaerobic conditions develop within the seepage meter,  altering the chemistry
          of the discharging ground water (Belanger and Mikutel,  1985).  As a result,
          calculated loading rates to surface water, determined using seepage meters,
          may not be representativeof actual seepage  from  the ground water.

                   d.       Representative  equations                                    .

                Darcy's Law is used to calculate  the ground-water discharge rate to
          surface water when using .mini-piezometers.   The form of Darcy's Law us.ed is:

	   ,  	        Q - K(dh/dl)A       /	 ,   	 •	\    '   _  |   '   .  '

          where         '                                               '

                Q   -       Ground-water  discharge  rate  [L3/T]
                K   -     "  Hydraulic  conductivity [L/T]
                dh/dl -     Hydraulic  gradient [L/L]              .
 *              A   _r       surface area  of the bottom of the surface-water body  [Lz] .

i;:.,.; ,^,;,,| r^^n ^^^'rVS "£o'" surlace"	water " as'"a	result "of ground-water  discharge is:    -
 '' ! W'i | j|f!J •,,''':•;* .nSIJ ' IJ  IliliV '' : '"„''!'"•' ,'l!! ,,N|1 '""!:!' ' '"« '!' »» ' ' 'lilli ,,'
llll1:1:1!'!" 1 », kJIni "i , "l,.i, ........ ..... 'JiUIHil, ' LJU ""• i ,, ..... !MM" ....... f *' 'TD  ^
          where                                      ,              .

                 LR  -       Loading rate [M/T]
                 Q   -       Ground-water discharge  rate  [L3/T].
                     „     '""Chemical cons'tituent coricentration  in ground water [M/L ]


          ' ''"'. .-:^"  .^ ...... ... e't ....... ""^""'"Description of field equipment     •

                 Equipment and materials often used  for  installation,  sampling, and
          maintenance of seepage meters include:.

                    open-ended 55-gallon drum with vent  hole,
                    tubing,
                 -  plastic  seepage bag,
                 - ' boat ,  and    •                                           '.        •
                 -  scuba  gear. ................ •  " •'

          .typical equipment and materials required  for  installation,  sampling, and
          maintenance^ of ............ mini-piezometers include:    _     •   _    , .   ,  •  ,

                    ffietal  pipe,

                                                " "u    '   •       ...... . '  ' '".'"'

-------
      -  end plugs,
      -  .tubing,
      -  nylon mesh,
         hammer,
         sample bag, and
      -  boat.
For a detailed description -of seepage meters installation -and- sampling,  see
Se (W7*   installation and sampling of seepage meters in deeper,  more
turbulent' water often requires additional equipment.

"-.;"•    f.        Expertise needed to apply method
      Sitine sampling locations  requires a sufficient understanding of.
reeionai geology  ^hydrology.   Extrapolating sampling results also requxres



 If «SI iLzometers may be made from a surface platform -as described by Welch
 !nd Se"a98?)   Se surface platform sits on top. of two -14 foot boats  ; and

                                                                                -
 intensive, especially with dive team involvement.


       ij_;         Data  inputs for  the method
                      of  sample  results  to  areas with  similar  sediment
                          Icnowledge  of  the spatial  ^$^&S
  discharge rate.
        iii.   Outputs from the method- • -

                meters and mini -piezometers provide a direct
  can provide estimates- of the.' total loading from ground^ater seepage
                                         15

-------
                                      figure 2-6
                   SIDE vi£W
plywood box  beam on
center joist" only
                            2x4  joist
                                                    platform
                                                    eye bolt (3/8 in x 8 m)
                                                    joists

                                                    aluminum boat
                                                    polypropylene
                                                    rope (5/6 in dial
                   PLAN VIEW
                                                    20  cm x .20 cm  hole
                                                   •joist (2x4 mx13 ft
                                                    13-4x8 ft  5/8 m  thick
                                                    T & G plywood)
                                                    •14 ft aluminum boat
                     Side and plan view. Working platform for installing
              piezometers and coring sediments from the water surface.
       Lee,  David R.,  and Stephen J.  Welch:   "A Method for Installing  and
Monitoring  Piezometers in Beds of Surface Waters," Ground.Water•.  1989.  Volume
27(1):   p.  87.
                                           16

-------
        a.-     Ground-water quantity discharge to surface water
       wide range of seepage rates can be measured using seepage meters and
           rl:;^^^
simple seepage meter described above  (Lee, 1977),
        b.      Ground-water quality discharge to surface water
      Seepage meters allow for the collection of samples for water quality
                                                                    -
•^SS^i^^S^^c..^^.^.^?^^^^.

    .  iv •        Settings in which the method has been applied and  _
                 contaminants .that have been measured using this method
      Summaries in Table A-1 describe some of the locations wher* seepage
      ,25mini-piezometers have.been' used successfully and the. contaminants
 met*rs
 measured using the- method.
      v.
            Evaluation of the method
    .  Seepage meters and mini -piezometers provide a simple  d








 .extrapolating results  to the points of discharge,                        ,

       vi         References to annotated bibliography   •

  '     References to the annotated bibliography presented in the accompanying
  volume to this document are provided in Table, A- 2.
                                     17

-------
                                                                                                                          11!  I In B Illi   • I*
                                                                                                                          ii  Hi I!   i!i
                                                                                                                                                               i  i i    i  « iliS! i
                                                                                                                                                               MI    II III !
                   j »T»UU A-l. ,S««ary of S«Ltl<.Sa In Ht.td« the Hatttod tin Beun Applied ami tin CoHlijiiJnaroU Hea»ur»d.
                              Location
                                                                                                                                                                  Author
 u i;
r:
fc-
I; -.;-
K
                      Oiilarlo

                      SILBS naar LsaralngLon.  .
                  '    Ontirto and «t Capa Cod
                  i:[ :i HasstchusatLs

                    •  Chalk River, Ontailo
                     . Douglas

                     ••: Key Largo National
                     - Marine Saucturay, Florida

                     1 Key Largo National
                   \  'Marine Sanctuary, Florida

                     : OsceoLa County,  Florida
                       Wisconsin
                       Michigan and Wisconsin
                       Btovard CouuLy, Florida
                       Belanger

                       Upper Great Lakes
                       Connecting Channels
                       Orlando, Florida
                       Brezonik

                       South Dakota
                       Colorado
                       Winter
                                                                        Floridan Aquifer
                                                                        Shallow glacial,
                                                                        glacial bedrock Inter-
                                                                        face and bedrock units.
                                                                                                                     Hltratei
                                                                                                                     (Ontario)
                                                                                                                     Pesticide*
                                                                                                                     Heavy M«lal«

                                                                                                                     Nitrates, selected
                                                                                                                     cations, total phosphates

                                                                                                                     .Phosphorous, Hltrogen
                                                                                                                     Hl.trate, Phosphorous,  '
                                                                                                                     Ammonia;
                                                                                                                      Chloride
Phosphorous,  Chromium,
Lead, Barium, Zinc,  Cobalt
Nickel. Phenols

Nitrate
                                                                                                                      Nitrogen,  Phosphorous,
                                                                                                                      Pesticides
                                    0. R. Lee, S. J. Welch

                                    D. R. Lee



                                    J. B. Hunch,  R.  W.
                                     G.  H.  Slnmons Sr.
                                     F.  G.  Love

                                     G.  M.  Simwmi Jr.
                                     J.  Hetherton

                                     T.  V.  Belanger
                                     D.  F.  Hlkutel

                                     I.  D.  Brock, 0. R. Lee,
                                     D.  Janes, D. Hinek

                                     D.  A.  Cherkauer.
                                     J.  M.  McBrlde

                                     J.  N.  Connor. T.V.
EPA Hon Point Source Work
Group •


C. R. Fellows, P. L.


J. Goodman at al.


J. H. LeBaugh, T.C.
                        Eastern Ontario
                                                                                                                                                           D. R. Lee, J. A. Cherry.
                                                                                                                                                           F. Plckens

-------
Table A--1.  Sunaary of Settings ID Which the Method B«» Been Applied and the Contaminants Measured.   (Continued)
        Location. •
                                                          Aquifer
                                                                                               Contasdnant
                                                                                                                                             Author
tu!.leiu Ontario

Minnesota, Wisconsin
North Carolina, Nova Scotia

Southern Ontario

Barbados, West Indies

SouLliuastern Virginia
Minnesota

Holbrook, Massachusetts  '
Ostyre,
 Mahantago Creek,  •
 Gburek,
 Pennsylvania

 Chicago,  Cook County,
 Demlssle,
 Illinois

 Virginia's Eastern Shorn
 Sault Ste. .Maria,. Ontario

 West tliorton, Hew Hampshire

 Lake Mead, Nevada
 Sullivan


 East Coast 'of Florida
Barbados Aquifer

Shirley. Yorktown,
and Tabb Formations
Manhantago Creek Basin



Cambrian and Ordovician

Aquifers
 Tertiary-Cretaceoug

 Gale-Hills Formation
    Tritium

Phosphate!, Nitrate*,
Ammonia, Chloride  •  '•

Nutrients  '

Nitrogen, Phosphorous

Inorganic Nitrogen.
Phosphorous, Nitrogen

Volatile Organlca and

Inorganics

Nitrogen, Phosphorous



E.P. Metals
                                          Hitrete,  Araoonla,  Total
                                          Phosphorous
                                          IDS, calciura-iulfate
                                          Phosphate
 D.  R.  Lee,  J.  A.  Cherry •

 D.  R.  Lee


 D.  R.  Lee.  H.B.N. Hynea

'j.  B.  Lewis

 W.  G.  Maclntyre,
• 0.  H.  Johnson-,
 H.  G.  Reay,
'6.  H.  Sinmons, Jr.

 J.  K.  Heel. R. M. Brlce

 H.  R.  Herman. D. P.

 J.  S.  Hobin

 H.  B.  Poinke, N: J.

 N.  J.  Gburek  et. al.

 M. S. Henabry, M.

 et el.

 G. M. Sinmons, Jr.


 S. J. Welch.  D.  R.  Lee

 T. C. Winter  .'

 W. H. Woessner,  K.    .
                                          C. F. Zlmnerman,
                                          J. R. Montgomery,
                                          P. R.. Carlson

-------
,  iij j  ]   I

  !, I  i   *
i,:!  I Nil!         ill!
jsri iilj         MI

I;;:.: js3         ^

              inj.ihi
                                                                                                                             !i!i       Hli 1
                                                                                                                             !i!l IP!  !i i
              A 2,  Ktil«rwic*s to AmiMtated
                  =            :  i
                 Autliur
                                                                                   Citation
                                                                                                        Reference to Annotated
                                                                                                              Bibliography
           V. B»l*ng«r. D. F. HikuHl
        R. Care.  T. C. Hlntur
      ;   D.  A.  CItarkouer,  J.  H.  HcDrlde
     ,    J.  H.  Connor,  T.  V.  Belanger
to
   "
       '  EPA tlon Point Source Hork  Group
         C.  R.  Fellows.  P.  L.  Brazonlk
         J,  Goodman'et at.
         J. H. LaBaugh, T. C. Hintar
                                            "On th« Us* ot S«»p«g» Haters  to Estl«*te                          pp.2-3'
                                            Ground-Witer HutrUnt Loading  to Likei,"
                                            Hater Resources Bulletin.  1985, Volume
                                            21(2)!  265-272.

                                           <"An Annotated Blbllogrephy of  Devices Developed          •         p.8 •
                                            'for Direct Measurement of  Seepage,"  U.S. Geological
                                            Survey Open File Report  00-344, I960.

                                            "A Remotely Operated Seepage Mater  for  Use in  Large.               pp.9-10
                                            Lakes and Rivers," Ground  Hater. 1988,  26(2):
                                            165-171.

                                            "Ground Hater Seepage in Lake  Washington  and the Upper            pp.11-12
                                            St. Johns River Basin, Florida," Hater  Resources Bulletin,
                                            1981, 17(5):  799-805,

                                            "Upper Great Lakes Connecting  Channel Study, Haste Disposal       pp.13-17
                                            Disposal Sites and Potential Ground Hater Contamination.
                                            St. Clalr River," Non Point Source  Hork Group Report,
                                            April. 1988.

                                            "Fertilizer Flux into Two  Florida Lakes Via Seepage,"              pp.18-19
                                            Journal ot Environmental Quality.  1980, Volume 10(2):
                                            174-177.                            .

                                            "Oakwood Lakes - Poinsett: Rural Clean Hater Program              pp.20-21
                                            Comprehensive Monitoring and  Evaluation Technical Report,
                                            Project 20," Rural Clean Hater Program Comprehensive
                                            Monitoring and Evaluation  Technical Report, Project  20,
                                            May, 1989.

                                            "In Impact of Uncertainties in Hydrologlc Measurement  on          pp.22-23
                                            Phosphorous Budgets and  Empirical Models  for Two Colorado
                                            Reservoirs," Limnology and Oceanography^  1984, Volume  29(2):
                                            322-339.

-------
 Table  A-2.. Kufuruncua  t.o Aiuiotateil Blbllogra|>hy  (Continued).
         Author
                                                                           Citation
                                                                     Baferenca to Annotated
                                                                           Bibliography
 D.  R.  Lee
 P.  R  Lee.  S.  J.  Match
 T. D.  Brock,  D.  R.  Lee,.
 David Janes,  David Hinek

'D. R.  Leu.  J. A. Cherry,  J. F. Pickens
 D. R. Lee, J. A. Cherry
 D. R. Lee
 D. R. Lee, II.B.H. Hynes '
 J. B. Lewis
"Six In-Sltu Methods for Study of Gcoundwatar Discharge,"
Proceedings of the International Symposium oh Interaction
Sympoiiura on Interaction Between Groundwatar and Surfaca
Hater. 30 May-3 Juna, 1988, Yitad. Sweden, edited by
Patar Dahlblom and Gunner Lindh, Department of Hater
Resource* Engineering, Lund University, Sweden.

"Methodology for Locating 'and Measuring Submerged
Discharges:  Targeting Tool, Harpoon Piezometer and
More," FOCUS Conference on Eastern Regional Ground Hater
Issues:  October 17-19, 1989, Kitchener, Ontario,
Canada, Co-sponsored by the Association of Ground Hater
Scientists end Engineers., Division of HHHA and Haterloo
Center for Groundwater Research, University of Hatarloo.

"Ground-Hater Seepage as a Nutrient Source to a Drainage
Lake; Lake Mandota, Hisconsln,"     .                  ,  •

"Ground-Hater Transport of a Salt Tracer through a
Limnology and Oceanography. 1980, Volume 25(1):
45-61.                               .

"A Field, Exercise on Ground-Hater Flow Using
Seepage Metara and Mini-piezometers," Journal'of
Geological Education. 1978, Volume 27:  6-10.

"A Device for Measuring Seepage Flux in Lakes
Lakes and Estuaries," Limnology and Oceanography.
1977, Volume 22(1):   1*0-147.

"Identification of Groundwatar Discharge Zones in a
Reach of Hi1 loan Creak In Southern Ontario," Hatar
Pollution Research Canada. 1976,  13:   121-133.

"Measurements of Ground-Hater Seepage Flux ontq a
Coral Reef:  Spatial  and Temporal Variations,"
Limnology and Oceanography. 1987, 32(5):
1165-1169.                                .         '
                                                                                                                                      pp.27-29
                                                                                                                                      pp.37-39
pp.6-7


pp.32-34



pp.30-31



pp.24-26



pp.35-36



pp.40-41

-------
                  S Ii ! i                      Mil
S!M!                                         MM
»,*-
3
aiBi
                     T»l)lo A 2.  Kaf«r*nea« to Ana«jL«t«J
                    ?!    . !    (i           :   M    !  I ,
                                                                      (Continue*!).
                                                                                                      i    t
                                                                                                                                                                i Ii
                                                                                                                                                                111
                                                                                                                                                                                          • III
                             Author
                                                                                              -, Citation)
                                                                                                                                                   Reference to Anraotated
                                                                                                                                                         Blbllogcaipby
      •*•
4s
iv-
  ! rt
  iiHi
             K>
             ,to
                     H  G. Haclntyre, G. II. Johnson,
                   !SH  G. Reay, G. M  Siwmni. Jr.
                    ; J. K  lluul , K. M. Uclce
                     U  K. Hoiniaci, D. P. Ostrye,
                     J. S. Hobin
                     II. U. Pionke. J. R. Hoover.
                     R. R. Schnabel, V. J. Gburek.
                     J, B, Urban, A. S. Rogowokl
                    '  P-  E» Ross, M. S. Hanebry.
                      J.  B, Risetli. T. J. Murphy,
                    :  M.  Demi55ie County, Illinois
                      G. M.  Simmons Jr..  F. G. Love
                      G.  M.  Sinmons  Jr.,  J.  Netherton
                                                                    "Ground-Hater Hon-Polnt Sources  of Hutrlants  to the
                                                                    Southern Chesapeake Bay," Proceedings of Ground
                                                                    Hater Issues and Solution* In the Potoaac River
                                                                    Bailn/Che»apeake Bay R«nlon.  Co-sponsored by  the
                                                                    Association of Ground Hater Scientists and Engineers,
                                                                    pp. OS-JO*.                  '

                                                                    •'Watershed and Point Source Enrichment and Lake
                                                                    State Index." US EPA, April 1979. EPA-600/3-79-046.

                                                                    "Use of Seepage Meters to Quantify Ground-Hater Discharge
                                                                    and Contaminant Flux Into Surface Hater at the Belrd and
                                                                    McGulre Site (HPL No. 1*),"  Proceeding of Third Annual
                                                                    Eastern Renlonal Ground Hater and Conference. 1986.
                                                                    p. 472-491.

                                                                    "Chemlcal-Hydrologic Interactions In the Near-Stream Zone,"
                                                                    Zone," Hater Resources Research. 1988, Volume 24(7X:
                                                                    .1101-1110.

                                                                    "A Preliminary Environmental Assessment of the Contamination
                                                                    Associated with Lake Calumet Cook Hazardous Haste Research end
                                                                    Information Center. Illinois State Hater Survey, 1988, HHR1C
                                                                    RR-019, 88/300.

                                                                    "Hater Quality of Newly .Discovered Submarine Ground Hater
                                                                    Discharge  Into a Deep  (Coral Reef Habitat," (JOA^ Symposium
                                                                    series for Undersea Research. Volume 2(2):  155-163.

                                                                    "Groundwater Discharge  In a Deep. Coral Reef Habitat:
                                                                    Evidence for e Hew Blogeochenlcel Cycle?."  Diving for
                                                                    Science...86, Proceedings of the Sixth Annual Scientific
                                                                    Diving Symposium (1986), Tallahassee, Florida, Charles t.
                                                                    Mitchell,  editor.
                                                                                                                                                          pp.42-43
                                                                                                                                                          pp.44-46


                                                                                                                                                          pp.47-49






                                                                                                                                                          pp.50-52



                                                                                                                                                          pp.53-55




                                                                                                                                                          pp.60-61



                                                                                                                                                          pp.62-64
       i :   r.

-------
        Table A-2.  References to Annotated Bibliography- (Continued).
                 Author
                                                                                   Citation
                                                                             Deference to Annotated
                                                                                   Bibliography
to
OJ
        G. M. Simmons, Jt:
        G. H, Slnmons,  Jr.
         S.  J.  Welch,  D.  R.  Lee
         I.  C.  Winter
         W.  M,  Moessner,  K.  Sullivan
         C. F. Zinroarraan, J. R. Montgomery.
         P'; R. Carlson
"Understanding the Estuary Advance* In Chesapeake
Research," Proceedings of a Conference-, March 29-3),
198, Baltimore, Maryland, Chesapeake Research Consortium •
Publication 129.  CBP/IHS 24/88.

"The Chesapeake Bay's Hldd.n Tributary:  Submarine Ground-
mt-rr P'-"hr''ll*." P™r.«.i»n»« nt Ground Hater Issuas and  .
Solutions In the Potoaac River Basln/Chesapaake Bay RaRJon.
Co-sponsored by the Association o{ Ground Hater Scientists end
Engineers, pp. 9-29.  t    '   '              '.

"A Method for  Installing and Monitoring Piezometers in Beds of
In Beds of Surface Haters." Ground Hater. 1989 27(1):  87r90.

•'Geohydrologlc Setting of Mirror Lake. West Thorton, Mew Hampshire,
1984, U.S. Geological Survey Hater Resources Investigation! Report,
84-4266, 61 pp.   .     •                .     •

"lisa of Soopage Maters and Mini-piazoneters for  Identifica-
tion of Reservoir - Groundwatar Interactions in  Lake Mead,
Nevede," Desert Research  Institute Hater Resources Canter,
1983. PB 83-22689*.   '

"Variability of Dissolved Reactive Phosphate Flux Rates in
Nearshora Estuarlne Sediments." Estuaries.  1985,8(26):  228-236.
pp.36-57




PP;58-59





pp.65-66


pp.67-68



pp.69-70




pp.71-72

-------
Ill
                   Ground-water quality samplingand measurements of ground-water  flow to
                   estimate loading to surface water
                       papers cited in thissectionare summarized in Section VIII  of "An
             Annotated Bibliography of the Literature Addressing Nonpoint Source
             Contaminated Ground-Water Discharge to Surface Water," September,  1990,  EPA
             440/6-90-006.                                         ,           ;

                   1.          General description of method

                               Description of procedures
                         a.
              I III     n       II II I Illl 1 1  I       I I ill! 1  I I I  } I II i   I       I II I    »      ' ,1 , i  " „ '   ,'"!,'„   :. ' i,   '    ' :
                   Water-level elevation measurements  from piezometers and ground-water
             wells provide an indication of the quantity  of ground water, discharging to
             surfacl water in a watershed.  This method uses water-level  measurements
             obtained from wells  located in the watershed to develop a water table contour
                   glrcy's^Law is then applied to  calculate the discharge rate of ground
             water to surface water by incorporating estimates of hydraulic conductivity
             and the cross -sectional area  of the aquifer.  By  assuming  the aquifer
             underlying the watershed is homogenous and isotropic, the  water-level contour
             map can be used  to  determine  flow directions and  horizontal gradients in the
             basin   In a homogeneous,  isotropic aquifer, flow lines will be perpendicular
              co equipotentials.   Hydraulic conductivity can be estimated for a particular
              rock or soil type or can be measured  in-situ via  aquifer tests.  Aquifer   ••
              geometry is' estimated by examining  lithologic logs of wells in the watershed.  .
              Ill I I I     I     I I II I III           I III      I I III    I II      I    lull ' ! " ,': Mill,"™". „'!, '' I,!,,," ..... ' j "''  ' ' ''.•   ' ,  '   ' "
                   This" method  is often used in  conjunction with other methods, such as
              mini-piezometers,  seepage  meters, tracer studies, isotopic studies, or water
              and mass balances  analyses to verify study results.  This method has been
              practiced  in loth marine  and fresh water environments and has been used on a
              large  scale, such as in Long Island  (Franks and McClymonds) and North Central
              Kansas  (Spruill) and on a smaller scale such as in South Farmingdale, New  York
              (Perlmutter and ; X£eber) and the Stockett-Sand Coulee coal field  Montana
              (Osborne,  et.'al.).   This method has been used for glacial and dolomite   .
              aquifers."   Contaminants studied include metals , nutrients, and some organic
              constituents.

                    Ground-water  samples taken from wells within  the basin can be used  to
              characterize the spatial distribution of  ground-water  quality  as a. means  of
              estimating nonpoint source contaminant load.  To  properly characterize  ground-
              water quality in a  drainage basin, potential  nonpoint  source loading  areas    •
              should be identified and the underlying  ground water sampled.  Agricultural
              areas located on soils allowing  rapid infiltration of precipitation  are of
              particular concern.  Such areas  are  identified from soil and land  use ">aps
              fHallbere et al. ,  1983).  Evaluation of  ground,wat«r quality beneath nonpoint
              source loading  areas, over time will  indicate qualitatively  whether the loading.
              tatfto sSpe water, as a  result of ground-water discharge,  will increase or-
              decreasej'iif tKe ^future :_
                                      _ .....     , _. ,.,,   .... ..... . , , ,  ,.. ....     . .       .,

                    Ground-water quality in wells adjacent to the s«fa";wat" ^J^"6  Bv
              assumed  to bi  repreVahfiielve of ground water discharging to surface water.  By
                    .....                ...... concenfr'ations and the calculated ground-water flux, the-
                 ng

             1(1! ..... .,!.",:• 'i1   Jlilllll  i." ..... . ,."" . "i;11: ;. I  ',, 1|,,!!l! ..... il  vti'l ....... liil'ii1!' I1.1'-"""
                                    .   .   '         Illl 111 Illlllll I II Mill III ||||I||||||||||||| ll I  II III Illl I  I  I   I I  II   	 III  III I     (III

-------
immediate  loading  rate  to  surface water from ground-water discharge can be
calculated.                    .                                           ,

            b.     Assumptions  involved in these methods               .

       To use  Darcy's Law to calculate ground-water discharge to surface water.
it is  assumed that the  aquifer is. homogeneous',  isotropic, of constant
thickness, and that flow is horizontal.  The assumption.that the aquifer is
homogeneous and isotropic is necessary to ensure that flow lines are
perpendicular to equipotentials (Perlmutter and Lieber, 1979).  _ By assuming a
constant aquifer thickness and horizontal flow, the one-dimensional version of
Darcy's Law can be used.  Additionally, .water quality in sampled: wells is
assumed to be representative of the quality of the water discharging to the
stream. ...'"-                       •

          •  c.    Limitations  of the-method           .

             Aquifer -characteristics

       The  limitations of this method reflect the natural; variability of
 aquifers and the availability of information on aquifer characteristics;  'In
 nature, considerable heterogeneity exists and few, if any, .aquifers are
 homogeneous, isotropic, and of constant thickness.  In a heterogeneous,
 anisotropic aquifer, ground-wafer flow is not perpendicular to equipotentials,
 and the angle between flow direction and equipotentials  is not constant.
 Because the predicted flow path length differs from the  actual flow path
 length, the calculated hydraulic gradients will not be representative of  the
 actual gradient.  Additionally, horizontal gradients determined using wells
 screened  at different depths below the water table or  in different'.geologic
 formations may not  represent the actual horizontal gradient.   Temporal  changes
 in the hydraulic  conductivity due to changes in seepage  face from
 precipitation events increase the difficulty of estimating  an  average ground-
 water discharge.  Hydraulic conductivity  also  varies spatially and
 directionally in  a  heterogeneous, anisotropic  aquifer.   It  would be difficult,
 if hot impossible,  to  determine an accurate  equivalent.hydraulic conductivity
 and aquifer  thickness  for the basin.   Because  of  the difficulties  in
 determining  horizontal  hydraulic gradient, hydraulic .conductivity, and  aquifer
• thickness, precise  determination of  ground-Water  discharge  to  surface water  is
 problematic  (Koszalka,  1983).                          .' .

         .  •  Well  installation

        Installing the number of wells needed to properly- characterize  ground-
 water quality in a watershed  is resource intensive.  As  an alternative  to
  installing costly monitoring  wells,  existing production, domestic, and stock
 wells may be sampled.   In many cases,  however, these wells.will not be  in
 optimum locations or open to  the geologic, formation of interest.
 Additionally, water-quality results can be altered by  well construction
- materials, faulty well construction, arid sampling procedures.   Consequently,
  ground-water quality in the basin may not be accurately characterized, due to
  the construction and lo'cation of the well.
                                        25

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                                                                      •	
                         d.   Representative equations

                  Darcy's Law is USed in determining the quantity of  flow entering surface
            water.   The fora of Darcy's Law used is:

              .................. ' ..... Q"'- .......... KCdh/dl)A ............... ; .........        " '  ' ......... ;

            where ................................................. ' _; ............................................. ,

                  Q           -     Ground-water discharge rate  (L3/T)
            '"  ............... ..... "' ....... ! '' £ ........ ' .......... '" ....... "i:i ........ ' ...... '' ' - ":  " "v '"Hydraulic conductivity (L/T)
                  dh/dL       -     Hydraulic gradient (L/L)
                  A           -     Cross  sectional area of the  aquifer (L2) .
            The loading rate 'to' ..... 'surface  a/S''rffadt of  ground-water discharge',  is
            determined by multiplying the ground-water discharge  rate by the concentrati
            of the constituent' in "the^ ground water. _ pie loading  rate equation is:

                         LR - Qc ................... ''   "" ...... """ ..... ............ ........... ....... '""•" ............ .
             where                       .                               '  .

             .,	,,:,,,;; ,.LR           -     Loading rate  (M/T)
              II,".,',! Q	"	 -	•	Ground-water "discharge rate (L3/T)
             : BS;ai;;£'6 ' "'	'  '	"'-1"11	"	Concentration in  ground-water (M/L3)
it III,,,,!	I'MJii;	;j]f '! i:;!!;1"'' iiitl. k!.^J'W\-
Jill1 iflilil !*', I 'Will,	i"1'1!1!1' liiJI, j,! ,  IlilEili JH,™ !	l!!lli«! ""
                         e.Description of field equipment
                        I'll	»l! Illlill '"!"",, "ill	'Ill1'',,," ' ,'    I II       	.1-	,',	 •, ," 	 "1!" .I',,!, .''I I',!,,-. './.' ,|	 !':
              ~ 'l"l After' the" wells 'have been installed,  equipment is required 'to"measure
             wacer levels and obtain ground-water  samples.   Suggested equipment includes:

                          steel tape and chalk or electric well sounder,
              	*•*	'submersible pump,
                     ,:,',;' " i; ^'pentrifugal pump,
lllilWIIIIIIE'l'iirli L iMni'li! mi/ ill Bii , ,  nllHIiiJ'!'', U,!",! »' ,',i,'~i, !
-------
 determining aquifer characteristics and geometry.   Aquifer tests are labor
 intensive  and sometimes difficult to interpret.   Additionally, aquifer
 characteristics determined for one portion of a watershed must be extrapolated
 to other portions of the watershed (Koszalka et al., 1985).


       ii.          Data inputs                          .    .

       To apply Darcy's Law and estimate the ground-water loading rate for a
 watershed, level elevations, hydraulic,conductivity, aquifer geometry, and
 chemical constituent concentrations in ground water are needed.  Well
 construction information is essential to determine the subsurface zones that
 .the hydraulic head and water quality measurements represent.


     '  iii.  Outputs from the method

         a.  Quantity of ground water

    "   A wide range of  ground-water discharge  to surface water rates  can be
 estimated using  this method.  The  factors controlling the  quantity of ground-
 water discharge  to surface  water are hydraulic conductivity  and gradient.   If
 the hydraulic  conductivity.of the  aquifer is  low,  and the  hydraulic  gradient
.- across  the  aquifer is  minimal, the  ground-water discharge  rate to surface
 water will  also  be low.  Conversely, a high.ground-water  discharge rate to
 surface water  will occur when the  hydraulic conductivity  and gradient for an
 aquifer are high.                         •       •

 ',        _b.   Quality  of ground water

      • A broad range  of loading  rates  to  surface'water'as-a result of ground-
 water discharge can be predicted using this :method. The  ability to  determine
 ground-water quality in sampled wells, is limited only by  the characteristics
 of the  well materials and the quantitation limits; for the individual
 constituents.


        iv          Settings in which the method has been applied and    .
                    contaminants that have been measured using this method

        Some of the locations where this method has been used and the
  contaminants  that have been measured using the method are summarized in Table
  B-l. -•     '. •      :.     .-              '            .        •.'-      .'.••'


        v.          Evaluation of the method

        Most watersheds contain observation  or water supply wells that can1be
  used to  obtain, water  level- elevations., and  water quality data  making this
  method applicable in  many  locations.  The  method  can qualitatively  determine
   the amount of -ground-water discharge  and the loading rate to surface water
  within a watershed.   Increasing  the number of sampling locations will improve
   the predictive  capabilities of  the method.                             :

         •  •   „  ••                        27   .          :     '•'•'••

-------
                 Because the method  is  often applied with limited knowledge of aquifer
           ch,r.cS*i«ics, a  large  number of sampling points will not necessarily result
           f !^Sate Quantification of ground-water discharge or loading rates to
           surfacfwate?!comparable qualitative indication of the loading rate to
           surface water as" a  result of ground-water discharge can be obtained by
           o^ervtnrvater-quality crends in the watershed.  If, within a watershed
           ^wtaB^er £     ^dentrations in ground water increase with time, the
           fuSre Lading  rate to surface water  as a result of ground-water discharge can
           .116 be  expected to increase.  In addition-to using the.method to
                      governing fertilizer and pesticide usage on ground-water


                  V£.         References to annotated bibliography

                  References to the accompanying annotated bibliography  are  located in
            Table "B-2.	'	.'.
                                11	'' j' ' ' ''

                           l ill I '..; '',"  I 	:nl: . i: I' f'.-.y
                                                    28
!!!!!!!!!'!!!!!!!! "!!''„,' ; T" it

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Table H-l.  Sunnary of Setting* |D Milcb the Method Baa Been Applied and the ContaaUnantB Maaaured.
        Location
                                           Aquifer
                                                                            Contaminant
                                                                                                                     Author
Patchogue.
Long Island, Hew "York

Penfield, Hew York

Upper Great Lakes
Connecting Channels
Long.Istand. Haw York
Clayton City, Iowa
Perth,-Australia

Niagara County,
Hew York

Stockett and Sand
Coulee, Montana

Hassau County,
New York

llorth Central Kansas
Lockport dolomite

Shallow glacial, •
glacial bedrock.   :
interface. & bid-
rock units

Upper Glacial, .
Magothy. and Lloyd

Galena
'Kootenai  Formation,
 Morrison  Formation

 Magothy
 Almena,
 Kansas  Bostwlck,
 Cedar Bluff Units
                                                                         .Nitrate Nitrogen
Sodium Chloride

Zinc, Phenol*,
Phoiphoroua
TDS, Inorganic
M«taU

Nitrates, Herbicide
Pesticides/Bacteria £
.turbidity

Nitrate

Inorganic t Organic
Constituents

Heavy Metals
Cadmium, Chromium
Sulfate," Sodium
Chloride, Calcium
                                                                      D. Capon*, H.  Bautista
L. R. Davis

EPA Hon-Point Source
Group
                                                                                                               0. L. Frank*.  H.  E.  McClyioonds
G. R. Hallberj. B. E.  Hoyer
E. A. Bettls,  III, R.  D.  Libra
R. E.- Johannes

E. J. Koazaifca.  J.  E.  Paschal
T. S. Miller. P.  B.  Duran

T. J. Osborn*, J. L. Sonneregger,
J. J. Donovan

N. M. PerLmitter.
H. Lleber

I.'B. Sprulll
 Butte. Mead  and
 Lawrence, South Dakota
 Arkansas  River  Basin
                                 Arsenic,
                                 Selenium
                                  TDS, Salinity.
                                  Chloride
                                      R.  L.  Stach,  R.  N.  Helgerson.
                                      R.  F.  Brett,  H.  J.  Tipton.
                                      D.  R.  Blessel, J. C.  Barksen •

                                      J.  D.  Stoner      •     '
 Schwatka Lake,  Yukon
 Territory, Canada
                                  Nitrogen, .
                                  Phosphorous
                                     P. H. Whlttield,  B. McHaughton.
                                     H. G. Hhltley

-------
I!
                     T«Mu U Z.  HuluruiiLU. lo AuiwUlud Bllil Iojt«|Jrjr
 a Guide to Hater-Management Alternatives," U. S. Geological
 Survey Professional Paper 627-F,  59p.

 "Hydrogoology. Hater Quality, and Land Management  In the Big
 Spring Basin, Clayton County, Iowa." Iowa Geological Survey,
 Open-File Report  83-3,  1983 Report on contract  82-5500-002.

 "The  Ecological Significance  of  the Submarine Discharge of
 Groundwater," Marine Ecolonv  —  Progress Series.  1980,
 3:  365-373.             •

 ••Preliminary Evaluation of Chemical Migration to Ground Hater
 and the  Niagara  River  from Selected Haite -  Disposal Sltea."
 USEPA. March  1985.  EPA 905/4-85-DOi:

  "Interaction between Groundwater and Surface Hater Regimes -
  and Mine-induced Acid - Mine Drainage in  the Stockett-Sand
 Coulee Coal Field," Montana  Jotnt.Hater Resources Research
 Center,  1983,  Project No. A-129MONI. Bozeman, Montana.

  "Dispersal of Plating Hastes and Sewage Contaminants  in Ground
  Hater and Surface Hater, South Faraiingdale  - Massapequa Area,
  Nassau County, Hew York," U.S.  Geological Survey Hater Supply
  Paper 1879-G.
                                                                     Reference to Annotated
                                                                           Blbllogtaphjr
pp.198-199


pp.200-201




pp.202-206



pp.207-209



pp.210-211



pp.212-213



pp.2U-216



 pp.217-219




 pp. 222-223
w ,

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Toblu U 2.  Huloruiiuea tu Aiuiotatud Blbl logra|J>y (Colillnuud)
       .Author
                                                                           Citation
                                                                             Reference to Annotated
                                                                                   Bibliography
T. B. Spruill
R. L. Stach, R. N. Helgerson.
R. F. Bretz. M. J. Tlpton,
D  R. BlesseL. J. C. Haiksen
J. D. Stoner
 f. II. Whitfieia.  B. McHaughton
"Statistical Evaluation of the Effect* of Irrigation on
Chemical Quality of Ground Hater and Ba»e Flow In Three
River Valley* In North Central Kansas." U,'S, GeoloKlcel
Survey Water Reaource Investigation Report 85-*156, 1985.

"Arsenic Level* in the Surface and Ground Haters' along
Hhltewood.Creek, Belle Fourche River, and a portion of
the Chtfyenna River. South Dekota," Completion Report,
Project Number A-OS4-SDAK. Agreement Number .U-3*-0101-60*3,
July. 1978.                                          '

"Disiblved Solid* in the Arkansas River Basin,." Rational,
Rational Hater Sunraary 198*:  HvdrolOKtc Eventt. Selected
Hater Quality Trends, and Ground-Hater Reaource*.. U.S.
Geological Survey Hater Supply Paper 2275.

"Indication* of Ground-Hater Influence* on Nutrient Transport
Through Schwatka Lake. Yukon Territory," Hater Resource* Bulletin.
.1982, 18(2):  197 - 203..
                                                                                                                                      pp.224-226
                                                                                                                                      pp.227-228
                                                                                                                                      p. 229
                                                                                                                                      pp.230-232

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   i!!1! linn 'i!!!!!!1:1)1:1!	iiiiiiiiiiiiiio1"1!: I'liiiiiiiggngiiiiii;;:;;!!1«' i iniig ;nfi VCTWWW w inwi	nnr WEHM1# f, ,^WWIE?I i!: iiiii'i'f'ii" I'liiini' in11"'!'' iii'iiiS!	r1  .     !iiiii!i!i; in	ifi • riiiiinnn11'' "' "'in ii'"  -', :;;•'' ;.<'i: ,< i^: :I: ii'!1'!''" n;; 'iiiii, i;:,,, ''. ,','., n ••' , ,1  , • s ,  i '••„.:,•    1|:,'L jMW'iiiii: J!'".; , ' '/''.'i;
C.    Studies  involving geophysical techniques to  estimate ground-water
      discharge  to surface vater
          papers  cited in this section are summarized in Section II of "An
Annotated Bibliography of the Literature Addressing Nonpoint Source
Contaminated Ground-Water Discharge to Surface Water," September 1990, EPA
440/6-90-006.                        .                      .

      i.     General description of method

             a.  Description of method or procedure

      Ground water discharging to surface water  is controlled by the hydraulic
properties  of the sediments of the surface-water body and the hydraulic
gradient across those sediments.  The sediment hydraulic properties of large  .
water bodies,  such as the Great Lakes or the  Chesapeake Bay, are difficult  to
measure due to the depth of the sediments in  open water,  Standard methods  of  '
drilling and sediment sampling become slow and costly endeavors in deep
aquatic. . environments .  Less costly shipboard  geophysical -systems offer a
method  that continuously characterizes bottom sediments along the ship's
track.  Combining seismic and electrical geophysical measurements provides
data to estimate  sediment ' type , thickness, and sequence, as well as relative
vertical hydraulic conductivity.  Based on this  information, one can calculate
the volume  of ground water discharging to surface water.
       Geophysical methods have primarily been applied to lakebeds.  Bradbury
and Taylor (l9"8~45 'collected' geophysical data at an offshore site in Lake
Michigan with sediment thicknesses ranging from 0.3 to 37 m and water depths
from  2.5 to' 27m.  Otherinvestigators have used geophysical techniques in
smaller lakes and in channels connecting the Great Lakes .(see Btadbury and
Taylor,  1984; Cherkauer and Taylor,  1987;  Lee,1989,  and Taylor and Cherkauer.,
1984).   Zektser and Bergelson (1989) have  used continuous measurements of
temperature and electricconductivity and  continuous  seismoacoustic profiling
to detect temperature and salinity anomalies in Lake-Issyk-Kul in the -
southeastern USSR.' One major difficulty associated with geophysical
techniques is the need for field  tests  to  verify the  results.  Field
verification can be. difficult to  obtain in- deep water.    ;             '

       Seismic         .               .                    .  •    '
                                                                        t
       Seismic exploration involves generating seismic waves arid measuring  the
time  required for the wavesto travel  to a series of receiving devices called
geophones.  In seismic studies of large, surface-water bodies, a shipboard
seismic profiling system can generate  and  receive the seismic waves.  Seismic
gWes ge'ifg'r'ate'd on board the ship travel downward through the lake bottom
sediment'untilthey reflect off a hard surface and back up through the
sediment to the "ship's geophones.  Information on sediment type, thickness,
and sequence can be inferred through interpretation of the travel'times, of the
seismic waves(Taylor and Cherkauer,  1984).
                                        32

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      Induced Pot?pttal or Electrical Charge

      This method involves charging the. sediment with a current, shutting off
the power source, and measuring the rate of current decay.  An electrical
array towed behind the boat charges bottom sediments and measures the rate of
current decay. . The relative clay content of bottom sediments can be
determined using this method.  These determinations are then used to estimate
the vertical hydraulic conductivity of the sediment.  Taylor and Cherkauer
(1984) describe the equations characterizing the use of electrical
conductivity and seismic readings used to estimate seepage (see Section
C.i.d).   ,                                       .'

      Resistivity      ' .                     ...        '                   .      .

      Resistivity methods also employ an artificial source of current which
enters the subsurface  through point-electrodes.  Receiving electrodes, measure
the potentials of the  electric flow field, which are influenced by the
composition of the subsurface materials.  An electrical array of source  and
receiving electrodes towed behind a boat (see Figure 2-7) measures the
resistivity of an induced electrical field in the sediments. -Sediment type,  ,
thickness, and sequence affect the configuration of the induced electrical
field.   Investigators  infer  the effective longitudinal conductance of the
bottom sediments through interpretation of the  resistivity "of the induced
electrical field.. The effective longitudinal conductance, combined with
sediment thickness information from seismic techniques and clay content
estimates  from electrical/resistivity techniques, provides data used  to
determine  the effective vertical hydraulic conductivity of the sediment
sequence.  The effective vertical hydraulic conductivity, the hydraulic
gradient over the sediment  sequence  (the change in hydraulic head over
distance,  measured at  various points over a large area or assumed constant
over  the study area),  and surface  area  of the water body  bottom provide  data
to assess the likelihood  and quantity of ground water discharging to  surface
water (Cherkauer and 'Taylor, 1984).

       Temperature  and Electrical  Conductance          ;

       Another indirect method  for locating  ground-water  discharge areas
 involves measuring temperature  and bulk electrical  conductance.  A  sediment
 probe with temperature and electrical  conductance sensors is  towed  behind a
'boat along, the bottom of a surface water body.   From the-continuous record of.
 temperature and conductance, anomalies  in temperature  and bulk electrical
 conductance are located.   These anomalies  indicate  the  likelihood of ground-
 water inflow.  Knowledge of the sediment.type,  water depth,  and other geologic
 or hydrologic information 'concerning the nature of the  possible discharge area
 may be needed for data interpretation,   Investigators  may,correlate measured
 temperatures and conductivities with other techniques  to better characterize
 the nature of sediment anomalies (Lee,  1989).
                                       33

-------
                                                   Figure  2-7
lirillLiii111, 
  • r S.qna, '• f* Block dicgrcrs. of i electriccl .'In'iiei'd"; Tjtvl,or, Robert W. , and Douglas- S. Cherkauer, "The Application of Combined'Seismic and Electrical Measurements to the Determination of the Hydraulic conductivity of a Lake Bed," Cround^Water Monitoring Review, 1984, Volume 4(4): p. 80. 3A

  • -------
              b.-  Assumptions involved in using these models
    
    
              geismjg
         «== ™ -
     seismic waves.  If the "^^ace  the seismic wave may be sufficiently
    . 1984) .
    
     bot-:^:^^W^sr^
    ' gradient  is often assumed for the entire body.        .        .
    
            '"  F.I metrical Charge ?T1H ***! stlvitV         .    •   ;      _
    
                                   eal- Conductance
      water discharge to the surface-water body (Lee, 198-5).
    
    
                c   Limitations of the methods
    
                                       35.
    

    -------
    • •liiiilillilllilli11 iini	(  ii   ill in	MM i	i, MI ,
            , ,1 ,:
    
    ana"
                    lytical results  derived from  these techniques.
                                  Representative equations
                                                                                             of
                  S -
    
     where:
                               Longitudinal  electrical conductance .[1/MLT]
                               Thickness of  layer ML]
                               Electrical  resistivity, of  layer i [1/MLT].
                        s            -
                        bl            -     Thickness of layer
                         l
    nil iiiiiii i in IP i i in
                                                                                                  .
    
                  (Gherkauer and Taylor):
                               Kv - (C0bT)/S
    
                  where:
                         y            -  '   Effective vertical hydraulic conductivity [L/T]
                         Cv           -     Total  thickness of sediment sequence  [L]
                         ST        "   .     Longitudinal electrical conductance  [1/MLT]
    
                         c            -     Scaling factor  [1/MLT2].
     	   ,	Law  is as follows:
    
    	        I, Q -  K.dh/dlA
    nun in i inn   i n   in     n n             mi mi
                   where:
                                       Grbuhd-water discharge rate  [L3/T]
                                       Effective  vertical hydraulic conductivity  [L/T]
                                     - Hydraulic  gradient across the sediment  sequence [L/L]
                                                             36
                 ikiV;:,*.!1?	i;ii.f':(i:i:i!;^:v:;;^                                            •'••.•:•/
                 , llflj||ln!j I i ii Ilin "I11,, ,':!|,il|.' - •!'  i • Jl ii, An Kjllj j, '"ll™1 ,'<';,' ' <	" i" "' .11'I Vlu! I ll«i '' A III '» i! i 1 |l,
    -------
             A      - Area on bottom of surface-water body with similar-
                      effective vertical hydraulic conductivity [L2] .
    
                e.  Description of field, equipment
    
          These methods usually require a boat, and sometimes a sizeable ship, to
    contain and deploy the geophysical instruments and support equipment used to
    characterize bottom sediments .  Shipboard seismic instrumentation, used to
    determine sediment thickness, consists of a high resolution sounder and
    rlcoSE?  Electrical resistivity and chargeability equipment  used to
    determine the electrical longitudinal conductance and clay content of a
    sedi^nt sequence consists of a long -Iticonductor <^%^f £*' S™~
    and/receivine electrodes.  The cable is .towed behind the ship.  A Lor an
    navigation system determines . the location of the ship's position for each
    ^1 urement ^ A computer stores the position and •-«««•£< f ^ ^
    assist  in the interpretation of the data (Taylor and Cherkauer, 1984).
    
        .-' '       f.   Expertise  needed to. apply  the methods
    
          The papers reviewed  for  this  report  suggest  that  geophysical  methods
    require considerable  expertise.  Prior  experience  helps., one  to properly
    coSigure  the instruction,  conduct .the tests,  and interpret  the results^
    Also  because a large boat must be used to house the  geophysical  system,  these.
    methods require navigational and piloting  skills.  , For a more complete
     dlsduslion of the expertise required to appLy geophysical methods readers are
     re?er«d ?o Taylor and Cherkauer (1984) .Bradbury and Taylor (1989),  Cherkauer
     and Taylor,  and Lee (1985, 1989) .        ,         ,                        _
           it.   Data inputs for the method
    The geophysically determined effective hydraulic conductivity °
                                       '                      e  uanti   of
             e geop
     sediments fs estimated for use with Darcy's Law to determine the quan
     ground water discharging to a surface-water body.  Addi ^al input data
     include a representative vertical hydraulic gradient for the .entire surface
     water body  and  the  area of the bottom of the Surface-water body.
    
        ,   When  bottom sediment temperatures and conductivities are used to predict
     -ground- water 'discharge .areas to  surface water, one^known source^of g«und    .
     water  seepage aids  in calibrating  the equipment.  This- technique  is limited  to.
     general  information^ about potential  ground-water  seepage .zones.
    
    
            iii .   Outputs from the method
    
      " '   .a. Ground-water quantity discharge  to surface water    ..
    
      -    ••  Geophysical methods estimate essentially any amount ' °J
      Taylor, 1984).                       .
    
                 "•                  :         37
    

    -------
     •'I
             b.   Ground-water quality discharge to, surface water
    
                  techniques ......... do ..... not' ......... Determine "'growid-water ...... quality, but.
                                               presence of
                                                        --
                    ; • x;. ••• ' :•; •;/; • ; ', ;. ;;; ; •: • > • ,,= ;. j i ' -ft "f. ;« ..... ,• < , : ' f y > >. ,: "i; M r si ..... .is- * v-j; ;:,; ,j* ft „
                    £n ^i£li • the ' ,iethod has" been" applied
    used.
         Table C-l summarizes some of the locations where  this method has been
    
              Contaminants that have been measured using the method
    
    
    
    measurement.               •  •                         .
    
          vi    General evaluation of the method
    
    
    
    
    
     5^^^^^^^r^r^r^^:«=s: »£
     (described in Section A o£ this chapter) .provide >     ^^ recharge zones
     SJ^ss: ss: » ssSLiTSi - ^ - "«^* Z°MS • -£«e-»""
     quality can be better protected.  .
    
          vii. References to annotated bibliography
          References to  the  accompanying annotated bibliography are provided in
     Table C-2.  "  ,     -             .        '       . •
                                    .  38
    

    -------
    Table C-l.  Suomary of Setting* in
                                      Which the Method Ba. Been Applied and the Contalnant. Measured.
    Ontario
    
    Green Bay, Mi
     Detroit Metropolitan
     Area,  HI
    
     Mequon/MI
     Great Lakes
     Hardwlck and Mew
     Braintree,- MA
     Dover, NJ
    
     Chalk River
     Nuclear - Laboratories,
     Ontario
    
     Southeastern
     U.S.S.R.
    Shallow glacial,
    glacial bedrock
    interface, bedrock
    units
                                                                                Contaminant
                                                                               organic solvents
                                                                                                                         Author
    D. R. Lee, S. J. Welch
    
    K. R. Bradbury,   .  •
    R. H. Taylor
    
    D. S. Cherkauer,
    R. H. Taylor
    
    D. S. Cherkauer,
    B. Zvibletnan
    
    EPA  Non Point
    Source  Group
                                                                                                                    H. H. Lajpham
                                                                           D. R.  Lee
                                                                         .•  I.  S.  Zek»ter
                                                                           G.  M.  Bergelton
    

    -------
    II
                                                                                               i« -I Illl          !   II!
                                                                                               111   •ban  i i i I  •  i   •• =
                  C 2.  K«tur*M«u« to AamtUt*!
    
                                                                        •            iilii!!  i!
                                                                        H            l!!l!l!  i!
                                                                                  - r  ": ' =       "i l»ISft= -"
                    Ati'Utor
                                                                                       Citation
                                                                                                                                           Ret«r«ic« to
    Mi »
            K. R  Bradbury
            R. H. Taylor
            U. S. Churkaiiui
            R. H. Taylor
             U.  S.  Cherkauer
             B.  Zvibleraan
             EPA Hon Point Source
             Work Group
             H. H.
             D. R. Lee
             R. M. Taylor
             D. S. Cherkauer
              I. S.  Zekster
    "Determination of llydrogaolojlc Ptoportles of
    Lakebtds Uilng Offshore Geophysical Surveys,"
    Ground Hater. 198* Volume 22(6):  690-695".
    
    "G«opliyslcally Determined Ground Hater Flow Into
    the Channels Connecting Lakes Huron and Erie."
    Proceedings of the Second National Outdoor Action
    Conference on Aquifer Restoration. Ground Hater
    (tonltorlnn and Geophysical HethpcU, Volume 2.
    Presented by the Association of Ground Hater
    Scientists and Engineers and EPA/EHSL - Las Vegas.
    pp. 779-799.
    
    "Hydraulic Connection between Lake Michigan and  a
    Shallow Ground-Hater Aquifer." GroundJIater,  1981,
    Volume  19(4):  376-381.
    
    "Upper  Great Lakes Connecting Channel Study,  Haste
    Disposal Sites and Potential Ground Hater Contamination
    St. Clalr River," Hon  Point Source Work Group Report,
    April,  1988.
    
    "Use  of Temperature Profiles beneath Streams  to  Determine
    Rates of Vertical Ground-Hater  Flow  and Vertical Hydraulic
    Conductivity," Draft Hater Supply Paper No.  2337.
    
     "Method for  Locating Sediment  Anomalies-in Lakebeda that
     that  can be  caused by  Ground-Hater Flow," Journal of
     Hydrology.  1985.  79:   187-193.
    
     "The  Application of Combined Sei.smlc. and Electrical Measurements
     to the Determination of the Hydraulic Conductivity of a Lake Bed,
     Ground-Hater Monitorinn Review. 198*.  Volume *(*):   78-85.
    
     "Effect of Ground Hater on Lake Hater Quality." Hater'Quality
     B..1I.H..  1r.n...ry.  1OBQ  pp  in-1"i	__	:	
                                                                                                                                                     74-75
                                                                                                                                                  pp.76-78
                                                                                                                                                   pp.79-80
                                                                                                                                                   pp.81-85
                                                                                                                                                   pp.86-87
                                                                                                                                                   pp.88-89
                                                                                                                                                   pp.92-93
                                                                                                                                                   pp.94-95
    

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     D     Studies  involving hydrograph separation,  regression analysis, or mass
           balance  approaches to estimate the contribution of ground water to
           istream flow
    
           The papers cited in this section are summarized in Section III of .''An
     Annotated Bibliography of the Literature Addressing Nonpoint Source      ;
     Contaminated Ground-Water Discharge to Surface Water," September, .1990, EPA
     440/6-90-006.             "            . r  .                      ,      :   :   .
                      /'                  ••-,"-''•     .     "       -           -
    
           i.    General description of method                ,
    
                 a.    Description of method or procedures
    
           The methods discussed in this section have been applied by investigators
      in areas throughout the U.S., in Ontario, Canada, and in the United Kingdom.
      Hydrograph separation has been used in conjunction with graphical  techniques
      to estimate the distribution of ground-water flux to areas of  the  Great
      Lakes 6  Other, investigators have used analysis of conservative tracers along
      with hydrograph separation data to estimate ground-water flux ;and  contaminant
     'loading   The regression analysis and soil moisture balance methods rely on
      equations developed for specific regions.  Arihood and Glatfelter  (1986) have
      developed regression equations for northern Indiana, while Beyans's (1986)
      work  was  in eastern Kansas.  Wilson and Ligon  (1979) applied a water balance
      model to  the  Piedmont  and  Sandhill Regions of  South Carolina.
    
            Hvdrograph  Separation    '     •  '           ,                       ,
    
            Precipitation entering a watershed travels to a  stream by three  main
      routes:   surface  runoff,  interflow (or  subsurface  storm flow),  and ground-
      water flow.   The  amount of water  contributed  to  the stream by. each of  the
      three processes is reflected in  the shape of  the stream hydrograph, a  graph  of
      stream discharge  at a particular  point  in the  watershed versus time.   The
      hydrograph for a single,  short  duration precipitation event,  occurring over
      the entire watershed,  follows a  general pattern (see  Figure  2-8).   The
    •  hydrograph shows a period of increasing stage, or  increasing discharge,  known
      as the rising limb,  that culminates in a peak or crest.   Following the" peak
      discharge,  the hydrograph shows  a period of decreasing discharge,  referred to
      as the recession limb.  Hydrograph separation techniques are applied to the
      recession limb to estimate contributions to stream flow from surface runoff,
      'interflow,.and ground-water flow.                     .
    
            When the hydrograph is plotted on semilogarithmic graph paper (discharge-
      on the semilogarithmic y-axis),  the recession limb has three identifiable line
      segments of different  slopes, (see Figure 2-9).  The slope of the line segment
      immediately after the  peak discharge is the steepest and represents
      contribution to stream flow as a result of surface runoff and subsurface
           -6  Pranckevicius, Pranas, personal communication, Nonpoint Source
       Contaminated Ground-water Discharge  to  Surface Water  Workshop, Chicago,  IL,
       November  30,  1989.  '                      .         '"_••'-
    

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    11 111
                                 111
                                                                                                           „	,, ';:::::':.  ;'„, ;:H
                                                       Figure 2-8
                            in/ill, i ' 
    -------
                                            Figure 2-9
                                                    •otot runoff
                                                    Surface runoff plus
                                                      subsurface runoff
                                                    Surface runoff
                                                      f    -.1   I
                                                 ^•Grounawoter runoff
    
                                                    Subsurface runoff
                                         i \      i \
                         28 29  30  31   I    23   4   5676
                                       August -Septemotr, 1951            .
    
              Senaiibgarithmic plotting of a hydrograph, showing separation of runoff com-
    ponents.  (Panther Creek at El Paso, Ulinoia.)
                Chow/ V.<  (ed.-)  --^QAA^
    Of Applied Hydrology.  New York:   McGraw-
       '•••Hill.
    

    -------
     runoff,  which includes interflow and ground-water storage depletion.  When
     surface  runoff storage is depleted, the slope of the recession limb flattens.
     This portion of the recession limb represents contribution to stream flow as a
     resultof interflow and ground-water storage depletion.  The slope of the
     recession limb of the hydrograph changes again when interflow storage is
     depleted and contribution to stream flow is a result of ground-water storage
     depletiononly.  The ground-water contribution to stream flow is referred to
     as baseflow (see Figure 2-8).   Surface runoff and interflow are often combined
     and'referred to as direct ruhoff.  The slope of the final segment of the
     recession limb is the ground-water recession constant, K^,  for the watershed.
     The line segment representing baseflow is extended back in time to a point
     under the hydrograph" peak to determine maximum ground-water discharge to the
     stream as a result of the precipitation event.  The ground-water recession
     constant for a watershed and the maximum ground-water discharge rate are used
     ^n an" empirical formula to estimate ground-water discharge to surface water at
     any time after a precipitation event.
    
           0/Brien  (1980) has developed a "dynamic method" of hydrograph .separation
    , which matches"the hydrograph of an index well with the stream hydrograph to
     •determine the moment of maximum ground-water discharge for two small wetland-
     controlledbasins in Massachusetts,  the advantage of the method is that it  is
     not rigidly tiedtoground-water stage, and it accommodates variations  in
     ground-water inflow and loss.in channel storage in response to temperature,
     vegetation, stream stage, and change in seasons,, causing shrinking and  • .
     swelling of the peat and muck in'the wetlands.
           Regression Analysis
           Equations  developed with  regression techniques  that relate basin
      characteristics  to  baseflow characteristics  in gaged  streams  can be  used to
      estimate baseflow in ungaged streams.   Examples of basin characteristics used
      £n the  regression"'analysisinclude  drainage  area of the  watershed  and flow
      duration ratio.   The flow' duration  for .a stream at a  given point in  the
      vaters'hed	is	the	proportion	of  time	that discharge is less than a  specific
      dl'scH'arge value. Flow duration is  commonly  expressed as a curve representing
      the percent of 'time discharge is less  than an indicated  value versus discharge
      pf afff gf Che  watershed,  (see Figure 2-10').   The flow  duration ratio  is the
      20-percent  flow  duration divided by the 90-percent flow  duration.. The
      drainage areas of the watersheds and the flow duration ratios are  transformed
      gp logarithmic units and a  regression equation is developed by backward
      elimination and  maximum R2  improvement procedures.  For  more  information on
      -™»^S"aSIisli	see'Trl^ooafana	Glatfelter	 (1986) and Bevans  (1985).
                ' Moisture Balance
            The ground-water discharge component to a stream can also be estimated
      using a soil moisture mass balance approach, where inflow-(precipitation)
      equals outflow (baseflow).  Soil moisture water balance methods for a
      watershed assume that any excess soil moisture below the root zone ultimately
      will contribute to baseflow.  The soil characteristics of the major soil types
      within the watershed are used tq estimate thewater-holding capacity of the
      different soil types.  Excess soil moisture content below the root zone is
                                            44
    

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                                       Figure 2-10
    2
    3
                  50
    
    
    
                   10
    
                    5
    i  i
                                               <
    
                                            •
                  .   Maaragua R. at   y     _-
                Maaragua* 138 sq mil./       ~-
                   •01 '      52~~i5  10  20   40  60   80 90 95    99
    
                      - Percent of time the flow is less than the indicated value
    
                            Flow duration curves for the River Maaragua in
                 humid, centrai Kenya (mean annuai rainfall 60 inchesrand
                 for the Uaso (River) Nviro in semi-arid, north-central Kenya
                 (mean annuai Tamfail 3*5 inches). Toe dasned lines indicate
                 the flow values betow which  discharge declines for 10 percent
                 of the time. The curves were constructed from  records for the
                 period 1956-1970.
        '   Dunne, T.  and L. Leopold.  (1978)  Uacer i'n Environmental  Planning.   San
    •Francisco:  W.H.  Freetaan  and Co.      _•'••;                                 .    ,
    

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               Ill III III III III 111 11 III I III IIII III I III 11 I III III
            predicted1 using precipitation  data,  the  evapotranspiration rate,  and estimates
         '!   of surface runoff  for  the watershed.   The  watershed is  divided into two zones
            based on a predetermined depth toground water from land surface.   In the zone
            where depth  to water from land.surface is  less than the predetermined depth,
            excess soil  moisture below  the root  zone is  assumed to  discharge immediately
           .".co the stream.  In the zone where  depth to water is greater than the
    i;!S^r''* ::''i:pr^tfetenKne"d	depth,	excess	soil moisture  below the root.zone is assumed to
            discharge to the stream.in  uniform increments, based on the time between •
            '^r^c'ipieatioh! events.   For  more information  on soil moisture balance methods,
            see Wilson and Ligon  (1979).
    
                         b.     Assumptions  involved in  using these methods
    
         	 Hvdrograoh  Separation	'	
    
                  Use of hydrograph separation techniques assumes that precipitation
            entering a watershed is evenly distributed and o.f the same intensity for the
            duration of  the  storm.  Additionally,  hydrograph separation techniques assume
            cfiicthe semilogarithmic plot of the recession limb of the stream hydrograph
            will have  three  identifiable'  segments""of different slopes.
                   Regression Analysis
                   An important assumption when usingregression equations to predict
             baseflow in unaged streams is that the basin- characteristics used in the
             regression analysis are similar to basin characteristics of the unaged stream.
             Basin characteristics of concern are (a) .the ground-water gradient, (b) the
             direction of theground-water'gradient, (c) the topography of the watershed,
             (d)theslopeof the stream channel, and (e) the length of overland flow.
             Also  the geologic material underlying the basin will influence the shape of
             the stream hydrograph (Arihood and Glatfelter, 1986, and Bevans, 1986).
                   Soil Moisture.Balance
    
                   The soil moisture water balance model assumes t'fiat any excess  soil
             moisture below the  root'zone ultimately contributes to baseflow.  Excess  soil
             moisture below the  root zone in the  zone nearest  the  stream is  assumed  to
             enter the stream  immediately following a precipitation event.   Excess soil
             moisturebelow the  root zone, in  the zone  farthest from the creek,  is assumed
             £6"	IfeScii the	stream."in uniform	increments;	based	on" the time between
             precipitation events.  Additionally, when  the water table.is below  the  root
             zone  it is assumed that  no evapotranspiration  occurs.  Ground-water
             boundaries	are"	aMumeV'cV'cVrreipond	to "surf ace-water boundaries, and there _
             are no  losses of  ground water  to  other watersheds (Wilson  and  Ligon, 1979).
    
                         c\     Limitations  of  the methods
    
                   Hvdroeraph  Separation
    
                   In theory,  it is straight  forward to separate  the  recession limb  of-a
              stream  hydrograph into thfie  segmentsof different -slopes  from which the
              quantity of water contributed to  the stream by surface runoff, interflow, and
              ground-water  flow can be determined.  In practice, separating the recession
    
                                                    46
    

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         of   .«..                                   oiven Sat
    arbT<7tnnCevents are not often o? constant intensity or evenly distributed
    precipitation events are not           t  ical watershed,, this is not
    and- considering the ^JJ"*™1^ ts o?bank storage will make separating
    surprising   Af^io5a^' ^orm hydro graph into three segments even more
    
    
    
    
    method.
           Regression Analysis
                                                          .
    
    
    basef low  redictions.
      resulting in inaccurate basef low predictions.
    
                 .Mo if f"^e Balance
                                                                        and
       may be  inaccurate.
               "    d.  :   Representative equations
            •„
                                             47
    

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                   N - A0-2
               1 1 1 II  I I
             where :
                                                •	!	i.1,!*;,,,,. ', -I
                    N -   Number of days after the peak when baseflow begins  [dimensionless]
                    A -   Watershed area in square miles. [L2].
    
              the equation to determine , the quantity 'of ground water discharging to surface
              water at any time after a precipitation event is: .
              where:
    n
    K°
                                Ground-water flow at  time  t  after the peak discharge'
                             ..........   [L3/T]          '              '   „*„,        '
                                Ground- water flow at  time  t  - 0 [L /T]
                                Ground-water recession constant (derived from the
                             ........ • ........ ''•"" hydro graph)
                                Time  [T] .       •       ,  '     •         '    .        '
              Equations for regression  analysis  and soil moisture balaftce methods are not-
              presented here,  as  the  equations are region specific and not universally
              applicable.  Readers  interested in these techniques are advised to read Wilson
              and Ligon (1979), Arihood and Glatfelter -(1986) ,  and Bevans (1.986).
                           e.
                                 Description of equipment needs
                     Stream stage data are obtained using a continuous-chart recorder.
               Ideally the recorder should be located in a controlled section of the  stream
               channel so a stream stage/discharge relationship can be developed.
    
                     For water balance methods, topographic maps are used to determine'the
               a"reaof a watershed.  A rain gage can be used to measure precipitati9n;  soil
               maps are used to determine soil types and to estimate soil properties.
    
                           f.     Expertise required to apply this method
    
                     The greatest difficulty in using this method is in selecting  .the portion
               Of the baseflow recession hydrograph to use in  determining  the  ground-water
               recession constant  (Kr) for the watershed.  Estimation, of Kr requires
               knowledge of basin  characteristics and the  temporal  distribution of
               precipitation  in  the basin as well as considerable professional judgement.
               bnce calculated,  Kr can be used in the empirical ground-water discharge
               formula to  determine the quantity of ground water  discharging to surface water
               in a watershed as a result of a precipitation event.
               I   I  I        I Illll     "I    III        II I III I  III  .        V" .III.	". ...' L ••  .  ',' "'' -j. v-i  '. ,_u'' «•
                      Computer programs, as  well as  PC-based  spreadsheets,  are available that
               determine  equations relating dependent  and independent variables tM-micrh
               regression analysis.   The  difficulty in using computer programs to^
               the relationship  of stream stage  to  basin characteristics is i
               Vhich  basin characteristics  are appropriate input parameters.
               It  may be  difficult to determine  the area over which a regression  equation is
                                                                I              '          ,
               	  '	'	 '  ";	  48
    111 ...... Ill illl
        ^^^    iilllll 111 i
                 llllllilillllll illllillillllllillii Iliililllillil 1 ll
                              lllll|i|||l||i|||lllillillilllililii T in
    

    -------
     applicable.  As with hydrograph separation, this method is best utilized by a
     hydrolqgist who is familiar with the subject basin.
    
          • A significant level of effort may be required to use soil moisture
     balance models to predict baseflow in a watershed.  The upper and  lower
     watershed zones must be delineated based on estimates of depth to  ground water
     below land surface.  Additionally, surface runoff and evapotranspiration rates
     must be estimated for the watershed.  Because of a-lack of representative
     precipitation measurements, the precipitation entering a watershed often must
     be: estimated from precipitation measurements.taken some distance, away.  Again,
     -familiarity with the hydrologic and geologic characteristics and the  temporal
     and spatial distribution of precipitation in the subject-basin as  well as
     surrounding basins.is highly recommended for the successful use of these
     models.                                         .
    
    
           ii.   Data inputs for the method
    
           Hydrograph separation techniques requires continuous record of stream
     stage or discharge to determine ground-water contribution to stream flow.
     Continuous stream  stage/discharge data are available for many watersheds .from
     the United States  Geological Survey.                   '  •
    
           The drainage area of the watershed must be known to use regression
    -equations  to determine baseflow in an ungaged stream  (Arihood and  Glatfelter,
     .1986).
    
           Soil moisture  balance models require the  following data:  precipitation
     records, water-holding  capacity of major soil classes  in the watershed, area
     of  the  watershed,  and drainable porosity measurements  (Wilson and  Ligon,
    ' 1979).
    
    
            iii.   Outputs  for the method
    
                  a..     Ground-water quantity  discharge  to  surface1 water      .
    
            Essentially any quantity of ground-water  discharge  to  surface water  can
     be  predicted using hydrograph separation techniques.   If the  time.between
      precipitation events is sufficiently long,, the  predicted ground-water
      discharge rate to surface water will decrease  over time.  The maximum ground-
      water discharge rate to surface water will be  a function of the  length and
      intensity of the precipitation event and the amount of ground water currently
      stored in the watershed.                   ...'.;•'
    
            As with hydrograph separation, any quantity of baseflow can be  predicted
      using, regression- equations and soil moisture water balance  models.
    
    
                  b.    Ground-water quality discharge to surface water
    
            'Hydrograph ,separation, regression equations, and soil moisture water
     .balance methods do not predict the quality of ground water discharging to
    
                    .           '-' '.      :      49                   -     ..'-••'
    

    -------
                surface water.   Baseflow determinedusingthese methods can be used in
                Conjunction with ground-water quality measurements obtained in wells located
                ^jicehtto the  surface-water body to estimate the ground-water loading rate
                to surface water.
    
    
                       iy.   Settings in which the method has been applied
    
                       Some of the settings in which this method has been used are presented in
                Table  D-l.
    
    
                       v.     Generalevaluation of the method
                       Hydrograph separation "techniques are an established method for
              •   estimating the ground-water discharge rate to surface water in a watershed.
                 The method is well understood, simple to apply, and continuous stream
                 stage/discharge data are readily available for many watersheds.  The key to
               '  approximating actual ground-water discharge rates to surface water using this
                 method involves correctly determining the slope of the baseflow portion of the
    I!,!!  I'1!11',; ,'  Secession" lin!b	of;	the	fiyarograpH;	Different slopes will produce markedly   .
                 different predictions of ground-water contributions to .stream flow.   •
    
                      ' Baseflow in ungaged streaii:'c'in'1 bV'estimated'"u'sTng'regression.equations..
                 The equations are developed using regression analysis,, relating drainage basin
                 characteristicstobaseflow, at gaging stations located  in  the same region.   ,
                 Because baseflow characteristics are  dependent on the geology and geographic
                 location of a drainage basin, a regression equation developed using drainage
                 basincharacteristicsfromoneregionshould not be used to predict baseflow
                 of screams io'cate'S"outside that region.  Therefore, accurate estimation of
    	bas'eHow	In	ungaged'" streams1" is dependent on the ability  of  the individual
                 applying the method  to Identify regions  having similar-basin characteristics.
                 Therein liesthe  problem-basin characteristics that influence baseflow are a
                 result ofa combination  of components,.some obvious,  such as geographic
                 location, and  some not so obvious,  such  as geology.   .Additionally,, the degree
                 ofihteractibnbetweenthe components affecting baseflow in a drainage basin
                 is  not well understood.'  Therefore,  the  potential  exists that regression
                 equations will be misapplied, resulting  in inaccurate baseflow predictions.
    
                       Soil moisture  balance  techniques  can be  used to estimate baseflow  in
                 unpaged watersheds.   Because  so  many of the  input  parameters  for  the  model
                 must be estimated,  the  error  associated with baseflow predictions, made using
                  this method may be large.
    
    
                       vi.    References	to	annotated'bibliography
    
    	 References to the accompanying bibliography are summarized in'Table D-2.
                                                        50
                          '                      	                      '     	v'^kjj!:^	".'. ..I;, •... ,      •  	ii jlilill
    

    -------
    Tablo U 1.  S.«i,«ry of Sittings  In HUUh  Uio MotlHMl Uau Uum, Applied and the Contaminant. Mua.urod.
            Location
                                               Aquifer
                                                                                Contaalnant
                                                                                                                         Author
    Lincoln, Massachusetts
    
    Northern and
    Central Indiana
    
    Upper Coastal Plain
    of South Carolina;
    North Carolina;
    Georgia
    
    United Kingdom
    
    Eastern Kansas
     Elliot :Lake,  Ontario
     Clayton County
     Iowa
     Clayton County
     Iowa
    
     Illinois
    
     Quebec and Ontario
    
     Cedar River Basin,
     Iowa-Minnesota
    
     Piedmont and
     Sandhill Regions,
     South Carolina
    Upper Coastal
    Plain Aquifer
    Galena
    Aquifer
     Galena
    •Aquifer
     Cedar River
     Basin
    Sulfate; Coal
    mine drainage
    
    Pyrite, Accessory.
    metals, Radlo-
    nuclides
    
    Herbicides,
    Pesticides", Nitrate.*
    and other agricultural
    inorganics
    
    Nitrate nitrogen;
    Pesticide*
                                      Herbicides
                                                                              A. L. O'Brien
    
                                                                              L. D. Arlhood,  D.  R.  Glatfelter
                                             H. R.  Aucott,  R.  S.  Meadows,
                                             G. G.  Patterson
                                                                               M.  D.  Bako, Ayodela Owoade
    
                                                                               Hugh E.  Bavaria
    
    
                                                                               D.  H.  Blowes, R. M. Gillhmm
    G. R. Hallberg. R. D. Libra,
    E. A. Bettis, III. B. E. Hoyer
    R. D. Libra. G. R. Hallberg-
    B. E. Hoyer, L. G. Johnson
    
    Michael O'Hearn.  James  P. Glbb
    
    M. G. Sklaih. R.  H.  Farvolden
    
    P. J. Squillaca,  E.  M.  Thurman
    
    
    T. V. Hllson, J.'T.  Llgon
    

    -------
    !  lill!  iii
    
      °
            -  Tublu U .i.  Rulai«wti.U'a to Aiuwtatud BII»U«nrai|Jn)r
    •  illII  i!|       Ml      !       '    	_
                                                                                             I   1
                                                                                             I   !
    I  M!Pi  ii*
                        AuUioc
        "" -   -   t.  0.  Arlhood,  D.  R.  Glatfelter
                M. R. Aucott, R. S. Meadows,
                G. G. Patterson
                H.D. Bako, Ayodele Owoade
                H. E. Bevans
                0. H. Blowes. R. H. Gillham
                 G. R.  Hallberg.  R.  D.  Libra,
                 E. A.  Bettis.  III.,  B.  E. Hoyer
                 R.  D.  Libra,  G.  R.  Hallberg,
                 B.  E.  Hoyer,  L.  G.  Johnson
                 A.  L-  O'Brien
                 H. O'Hearn. J. .P. Glbb
                 H. A. Pettyjon, R. J. Manning
                                                                                  Citation
                                                                         Reference to Annotated
                                                                               Bibliography
    "Method £or Estlnttinf Low-Flo« Ch«r«ctarl§tlci of
    Uiisagad Stcaana In Indiana," U.S. Gaolofical Sucvay,
    Op«n-Ftla Report 86-323. 1986.
    
    "Raglonal Ground-Hatar Dlicharga to Larga Strain In
    tho Uppar Coaatad Plain of South Carolina and GaorgU."
    USGS Hatar Raaourca Invaatlgatlons Report 86-4332,  1987.
    
    "Field Application of a Numerical Method for the Deviation
    of Dataflow Racaaalon Constant," Hvdro.loRtcal Process.  1988,
    2:  331-336.
    
    "Estimating Stream-Aquifer  Interactions  In  Coal Area»
    of Eastern Kansai by u«lng  Stremnflow Records," USGS
    Hater Supply  Paper 2290  (January,  1986).
    
    "The Generation end Quality of Streamflow on  Inactive
    Uranium Tellings Hear Elliot Lake,  Ontario,"  Journa}. of,
    HydrolQKY.  1988, 97:  1-22.
    
     "Hydrogeologlc and Hater .Quality Investigations In the Big
    Spring  Basin. Clayton County, Iowa," Iowa  Geological Survey.
     1984, Open-File Report  84-4.
    
     "Agricultural Impacts on Ground-Hater Quality," proceedings of
     the Aurlcultural I«pact» on Ground Hater.  1986, National Hat.r
     Hell Association.  Omaha, Nebraska, pp. 253-273.
    
     "The Role of Ground Hater in Stream Discharges from Two Small
     Hetland Controlled Basins In Eastern Massachusetts," Ground Hater.
     1980. Volume 18(4):   .          ,
    
     State Hater Survey Report Number 2*6. 1980 Illinois Institute of
     Natural Resources.
    
     "Preliminary Estimate of Regional Effective Ground Hater. Recharge
     Rates, Related Streamflow and Hater Quality in Ohio," Hater Resources
     Center, Preliminary Estimate of Regional Effective Ground Hatet
     Recharge Rates  in Ohio. Project Completion Report,  323 pp.. 1979.
    l>p.97-9B
    
    
    
    pp.99-101
    
    
    
    pp.102-103
    
    
    
    pp.104-105
    
    
    
    pp.106-107,
    
    
    
     pp.108-110
    
    
    
     pp.111-112
    
    
    
     pp.113-114
    
    
    
     pp.115-116
    
    
     pp.J17-119
    

    -------
           Tnlilu I) 2.  Hutuioncua
                   Author
                                  I.U Annotated Bllil lugraphy (Contlnuod)
           P. J. Squillace, E. M. Ttiurman
            t.  V.  Hilson,  J.  T.  Ligon
                                                                                      Citation
    "Surface-Hater Quality of the Cedar River Basin,
    Iowa-Minnesota, Hlth Emphasis on the Occurrence and
    Transport of Herbicides. May 198* through November
    1985." U,S.G.S. Tonic Substances HvdroloKY ProKram.
    Abstracts of Technical Heating. PHoenU. Arljtona.
    Septimber 26-30, 1968.
    
    "Prediction of Baseflow  for Piedmont Watersheds,"
    Office of Hater Research and Technology, Hater
    Resources Research  Institute. Report [lumber  80,
    1979, 47 pp.
                                                                                                                                           Refarcnc* to Annotated
                                                                                                                                                 pp:120-122
                                                                                                                                                  pp.123-125
    I/I  •
    CJ
    

    -------
    E.    Numeric*! models of surface-water/ground-water interactions
    
          The papers cited in this section  are  summarized  In  Sections  IV, V,  and
    VII of  "An Annotated  Bibliography of  the  Literature Addressing Nonpoint Source
    Contaminated Ground-Water Discharge to  Surface Water,"  September,  1990, .EPA
    MO/6 -90 -006.
           i.     General description of methods
    
                 a.     Description of method of  procedure
    
      ................... : " MathematicaF ground-water ..... modelling' simulates ....... an ....... [aquifer or watershed
     system using a series of equations governing flow and/or mass balance
     nronerties   When developing a model,  transport properties should be
     constructed using a framework of measured variables."  Modelling represents a.
     SSSSSv. procels of data gathering arid model verification to ensure an
     Curate depiction of real world phenomena  in the computer simulation   Models
     should not be used without field, data and ground truthing, and the transient
    'conditions of the study locations should be understood and incorporated into •
     the analysis.                                                •            .
    
           Mathematical ground-water models consist of sets of differential
     equations that describe or "govern" ground-water flow and/or contaminant
     transport.  These equations can be solved to develop an analytical solution
     however  field situations may be complex and difficult to solve exactly  and
     the assumptions that must be made to obtain the analytic solution are often
     unrealistic arid are not representative of the flow or transport problem under
     consideration.  In these situations, numerical methods can be used to solve
     the differential  equations and obtain an approximate solution that can be used
     to simulate relatively complex ground-water flow and contaminant transport.
     ^is process is presented in  Figure 2-11.  Two popular numerical methods used
     Co convert  differential equations  into algebraic equations are the finite
     difference  method and the' finite element method.        .
    
            To  utilize  a numerical  flow model, a  flow  system  is defined and      _
     discretized- into  a finite number of rectangular  blocks,  in-the case  of  finite-
     difference  models, or  triangles  or quadrilaterals, in the. case of finite-
     element models.   Figures  2-12 and 2-13, show finite difference  and finite
     element representations of  an aquifer .bounded on three  sides by  an
                                                         -d o  the fo "
    eement represen                      .
    boundary (i.e., no flow into or out of the aquifer) -d on the fo ""^ide by
    a river into which discharge from the aquifer occurs.  Each cell in the flow
    reeion is ass'igtwMts' own hydrologic properties based on measurements or
                                                      Boundary «'»•«• then
      obervations from the flow region being modeled   Boundary «££'£»•
      IScorporaTe'a Into the numerical model.   Typical boundary conditions are
      ground-water. divides (no flow), surface-water bodies (fixed head)^ and  .
      soecified flow.  The numerical model is run on a computer, and typically,  the
      calculated head-'field 'distribution at nodal .points (the intersections  of the
      Unes delineating the region or centers of the blocks) is compared to  the
      actual head,field distribution (obtained through measurement of water  levels
      Swells) in the flow region and, if available, the results »f «£**£"£
      Solution (see Figure 2-11).  If the predicted and actual head fields are not
        1      IfleSnt; 'the model  is adjusted by manipulating boundary conditions
                                            54
    

    -------
                                    Figure  2-11
       |    Set of differential
        equations tmatnemaucal
               model)
               Calculus
              tecriniques
    Method of finite
     differences or
     nnite elements
     Set of alzeonic
    equations (discrete
         model)
                 1
       I    Analytical solution
       !   i possible for a limited  •
       ":     numoer of casesi  .
       Compare if
        pojsiole
                             Iterative metnoos
                                   or  '
                              direct metnods
    Approximate soluuon
                  I
                                   i
               Compare
                                   *
                                Compare
                                          Reid'
                                       observations
         Relauonships between matneniaucai model, discrete algebraic model, analytical
         solution, approximate soluuon. and field observauons.
    Wang  H.. and M.  Anderson.   noa^  Tnt-T^duecion  to Ground water Modeling;'
    Finice  Difference and Finite  El*mgnc Methods.   San.  Francisco:   W.H.  •
    Freeman and Co., 237.p.           ,                        .    -                ,
                                            55
    

    -------
    mam UBBNEW .a ^:' IB •	w$ i	nswr dura rt: MB *;t :#* rk-^Kiiw'^sr t. tfa i:i? jf.PftjsHR^i'H^vt.iK w"' i- &•: im"1 vi!air'iii	t	i;: iKwr
    
    
    IIH       	liliis'. '''ii,  i»vJp*'! 111*,]::!!!!* '!iii:S,! 'i ,il h(«l'i'1 '''1''!	'::!'"..' V'1'^ "'";UJij^Wfr ':' '*"'.•>''L'"11' I!.!'"'•..':• iW(iif^rf •',Vjf.l.,4<','v-iii1. V^.'^'ilF,1'iiji'is?: -i 'WJ'i '
    
    iiiiiili iiliiii'itiiiv'l E'SiilSF' i i i','" !!,!»„ ii i:iiiii,, i; 'I :''': liiiiiiiiiiilNii „ \ I i!!"!	!," f::! iii!	i' ;li; ,'s ,,'il in< i' 'in'!!, iiui 'iiiiiiiii'": LJ,," l,» ».' !!!•' i' >''' i I1'  :,'',•!' I !„: ' ' i Ui'i ,i • >i it • ,„• „ I, ,i: ." l,;""'':;,..' i'lflt 4,!" •'"' ' 11	' ' 'ii;ii i,.'!1 \ • i, (, iif'1';"1'! iw i'i', j'lHifiii ' Ii i»'' !i! t, " • ,'flii Ii::,,
                                                                                                    ;'i;| .•,' •>.,  :ii-!1 •
    111 lllllll  I  II
    
    
    
    
    
    
     111 111	    I
    
    
    
    (111 lllllll    I ll
     111 111
    
    
    
    lllllll HI
                     ! ur ,I
                      iiiiiii
    
    
                      iiiiiii
                                       iiiiiii
                                                                • Figure 2-12
                                                                                                  Finm diffn
                                         ib)
                                                          • I • I •<••!• • I • i •'•*•* * '  * '  *   •><
    
    
                                                      Js±±±ii±>: :  :  :   :   •   ^
                                                       • V •  •• • «•••• «••'•••   •   •   •   •
                                                      ^TTjg^^^^m^^^^mM
    
    
    
    
    
    
    
    
    
    
                                                   i
    
                                                 :
    
    
    
                                                * 5
                                                                                .            Mlllln'ili     hl   '   '    ' '     I:!' .  '      '
    
    
    
    
    
    
    
    
    
    
                                          Ftmte diffeitnet and fimut ewntnt repraeaaaota of an aauifer. repon.
    
                                          ' laT Mao view of aa«Jitr snowan *«J fteki, obietvaooa weite. ana boundanea.
    
                                          ib» Fuusi 
    -------
                                   Figure 2-13
                  1C)
                id Finite diteenae ind w«h i
                id) Finite eteoeat mesa «mh mtafnttr eieaenu where 6 is the uuiier thiekaen.
                (Adaptea from Mercer ana Fmuit. J980e,»
     Wang,  H." and M. .Anderson.   (1982) Incroduetion  to Ground water ModelIrfg:
    '.Finite -Difference and' .Finite  Element Methods.   San Francisco:   W.H.  .-
     Freeman and Co. ,  237  p'.
                                         57
    

    -------
                             ilIiiniiilllfflliaiflllllN        	Ill	lI'IlliKJIilIliliniill	IllllllilillVllfin	inillllinil'IH	•  	EBSCflNilEnu  - 	:l!'l: I?1!!1 'I!'!!!|:::|":||'I:£.:"I>' "IT11	':'',!"	'!' I!1'
    i ,! ',!i|'i,!iill!ii' „„'Ihi,!1
    ill'llililllllllllllii	::' ' I'th.;,,1!!'!!!
             and/or	the	hydroTogic'properties  of the individual cells.  When close
            i1'ifglglgfigfi'e	IS"	reached	fietveen predicted and actual head-field distribution-,  the
            "nioHel	Is	considered calibrated.
     I, VH ,lf: 'S ; •',  •  'lillllillllljl: "I!;!!	I'mBSWIIIIInll'i;! 'MSii'l,,11 
    -------
           Chemical inputs to the flow region as a result of agricultural or other
     practices are assumed from generalized land use (Gburek et al., 1989)., The
     input is assumed constant, with time for a given land use for all contaminant
     source's within a study region.  Instantaneous mixing is assumed to occur in
     each cell for each time step.   Additionally, in the random walk process .of
     transport simulation, it is assumed that dispersion in porous media can be
     considered a random process having a normal distribution.
    
                 c.    Limitations of the models
    
           The major limitation of numerical models is the large amount of data
     required to accurately calibrate them.  To accurately calibrate a numerical
     model  information on the spatial and temporal distribution of land use;
     recharge, chemical input, hydraulic head, ground-water quality, and surface-
     water quality is needed.  Also of prime importance is the spatial distribution
     of aquifer characteristics.  Often, ground-water models do not take into
     account- the variable effects of near shore phenomena.  Generally, models will
     not simulate ground-water quality changes associated with seasons, or  reflect
     the hydraulic conductivity changes associated with seepage face growth and
     capillary response to precipitation.                    •            .
    
           Prior  to using a model, the scale and  the geographic conditions  of the
     study area must be incorporated into  the model.  For instance, fracture flow, .
     macropore flow, karst  terrain, and anthropomorphic effects on  the study area's
     ground  water may  require  that adjustments be made to the model's structure,.
     Few watersheds have  been  monitored sufficiently to provide the data needed to
     calibrate a.numerical  model.  Knowledge about  one watershed  in a region will
     assist  in characterizing  another watershed  in  the same  region, but additional
     data  probably will be  required before  the model is considered  calibrated and  .
     can be  used  for predictive  purposes.   Without  being  able  to  reproduce  flow-
     field conditions  or  chemical  concentrations, little  confidence can be  placed
     in a model's predictive capabilities.                                       •
    
            An additional  limitation of  numerical models results from  the
     uncertainty  associated with them.  This  uncertainty  is  a result  of numerical
     models being based on mathematical expressions that  are a simplification of.
    '  the real world and the measurement error associated with input data;   This
     uncertainty could result in predicted values that  deviate'significantly from
      the actual flow in the region being  modeled.  However,  proper  field data-
      collection techniques and the use  of well-tested models by experienced
      personnel combine to produce reliable predictions  in most cases.
    
                  d.    Representative equations
    
         .The partial-differential equation that describes time-variable .flow  in a
      heterogeneous, anisotropic two-dimensional aquifer (one in which hydraulic
      conductivity varies both in direction and space throughout the aquifer) is:
    
             a/SxdV Sh/8x) '+ a/8y(V 4h/5y)  -  Ss-6h/5t
    
      'where":              .        '       \ "••''"
    
      .-       K,     -     Hydraulic  conductivity in x direction  [L/T]              .
    
    
             ••              ;                 59
    

    -------
          v     -     Hydraulic conductivity in y direction [L/T]
          St    -     Specific storage  [L"1]
          h     -     Hydraulic head [L]
          x     -     x direction [L]
          y     -     y direction [L]                                     ,
          t     -     -Time  [T].                                         .
     ill     i i      i n in i ii ',,,"1,,, ,;, .Hi1 iir i '"Mi1 .•.:;-!•, siiH, ,:"..",:;• i' » :;, lif',	'Mt:,iii.i!iiiihi';i;:r '.; ''iivu,.	KS	i/^hji't^	u ;n •«": . H	lur „" iv,1'1,' • '^~''  n"   ,  *': '
    A finite-difference numerical model approximates the above  differential
    equation using  a  series  of finite-difference equations.  The two-dimensional
    finite-difference equation for a homogeneous, isotropic medium, where  the grid
    spacing* in the x- and y-  directions are the same and hydraulic conductivity
    is constant and isotropic  throughout the aquifer (K, - Ky),  is:.
    
    
    
    where:                                                 .
    
          h    -    Hydraulic  head.[L]
          T    -    Transmissivity [L2/T]'
           S    1     storativity [dimerisionless]           .     •          '
     	     ti	 ";	 "-	Time increment [T]    -.               '•',*•>'
           x     .     width of the  grid spacing, where  »x ?-*y  [L]
           i     J     Column number [dimensionless]
          "j  	  _	,  "ROW "number "•[dlmensionless]   '                 ^
           k     -     Time step or  iteration  index [dimensionless].
    
     Columnand row numbersinthis  equation correspond to those in the finite
     difference grid presented in  Figure 2-14.   Nodes  (intersections of grids) are
     spaced horizontally by *x and vertically  by *y.   For -the first ^ration  or
     solution of the equati6n, the modeler estimates  the value for  the hydraulic
     Jeal it eich node   The head values of the first  iteration (k-1) are used to
     calculate the  head values for the  second iteration (k-2)    The equation is
     Solvedseveraltimesinthis  manner until the difference between the h«-d
     values of the  final  iteration and.  the previous iteration is less than  a value
     specified by the modeler, called a convergence criterion.
    
           The partial-differential equation that describes solute  transport  in  a
     two-dimensional, homogeneous aquifer through dispersion and advection is:
                                   - Vx-»c/8x.- »e/«t
    
                   dispersion        advection
                                             60
    

    -------
                               Figure 2-14.
    
    
    j
    \
    
    1
    (1.
    
    f
    
    a
    1)
    
    
    
    .4)
    
    
    
    (i- "i,j'i
    L'-""
    U-jijc —
    
    
    M,;-i)
    •(/./)
    - •
    />n
    •
    
    
    
    (i-r I.;')
    (5
    
    •
    Av'
    I' :••
    » •
    .4)
    	 	 : 	 >
             Finite difference grid showing index numisering convenuon.
     Wang  H.  and M: Anderson.  (1982)  TnrrodurHon  co  Ground water 'Mode
       "'            ^d Tin!-. • ^ »m«r,r  Methods.-  San Franexsco:  W.H.-
    • Freeman, and Co. , 237 p..
                                     • 61
    

    -------
               where:           	 ,  	     ',   ,
    
                      p^     -     Longitudinal dispersion coefficient  [L2/T]
                      Ot     -     Transverse dispersion coefficient  [L2/T]
                      C     -     Concentration [M/L3]
                      V     -     Averageporevelocity in the x direction  [L/T]
                      x*     -   /'^"dj-rectipn (direction offlow)	[L]	.
                      y     -     y direction [L]
                      t     -     Time [T].
    
    Ill 111'  I"	I  i  111 I i n in the random'walk approach, solute transport  in a  porous medium is
    Illll      ii|i " represented by a	series"	of •equations'^	Dissolved chemical constituents are
    iIJII   ['   '  re'p'res'ented by a	finite number of discrete' particles each having  a mass
               representing a fraction of the total mass of the chemical constituent involved
                (Pricket et al.,1981).'The total distance a particle travels  between time
               steps is:                                             .   •             ' •
    
                      dx - d + d*                            .                  '            .     •
    
               where:                 '            ,             •
    
                      dj  	-	 Total	distance	traveled per 'time step {LJ
                      d.     _  •"   Distance traveled as a  result of advection per  time .step [L]
                      d"  	-	DTs*tance'	traveTe'd*	as	'a""result:"of dispersion per
                                        time step  [L].
                The equation representing the distancea particle  is  transported by advection:
    
                      d - vt",
    
                where:
    
                      d     -      Distance particle  travels for each  time- step [L]
                     •v     -      Ground-water  flow  velocity [L/T]
               :.'=:-,	v~:".'t:	 -	Time  step  duration [T] .         •             ';
    
                     •After the  particles have  been  moved advectively,  the position of.each
                -p-'greicle  is adjusted a  random amount in any direction to account for
                aispersion.  The one-dimensional equation representing the influence of
                dispersion oh  i" particle's position  is:
    
               rSii],;	r.4*	..^'pjdi/v-t)*"     '   .
    
                where:
                       d*     -  .   Distance traveled as a result of dispersion per
                                         time step [L] ......................... • ................................     ,
                         ...........   .....................           ''''''1  .............................
                      iiiyi     - ..................... •.Qrpund-water wlocity [L/T]      ^        .(
                       t     -     Time step duration [T]
                       N     -  -   A number between -6 and 6, drawn from a normal distribution
                                   of numbers having a standard deviation of 1 and  a mean  of
                                   zero [dimensionless] .
    
                               Hi                                       i i       i    1;
                                                       62
    

    -------
    The e'quacion determining individual cell concentration for each time step in a
    two-dimensional.model is:
    where:
                      Concentration per unit width of chemical constituent  [M/L3]
                      Number of particles  in a cell  [4imensionless]
                      Mass per particle  [M]
                      Cell length  in x direction  [L]
                      Cell length  in y direction  [L]
                      Column number  [.dimensionless]         ,    .    -•
                 -    Row number  [dimensionless].              .
    C
    n
                 e.
                       Description of computer hardware or software needs
                                                              55
                                                               ars
     •hardware includes:
                  a  PC  computer with math coprocessor chip and graphics card,
                  a  high resolution monitor  (for plotting results on the screen),
                  a printer,  and
                  a plotter.
      Numerous software packages,  both in the private  an^^ tranter"6
                                                                      Some of
      Lonnquist«,  Trescott •« al.9, and the International Ground-Water Modeling
      Center at Butler University -in Indiana.            .-
           7 vonikow -L  and J. Bredehoeft.'(1978)  Computer model of two-dimensional
      solute ^ans^'r^and dispersion in ground water   ^S-^^^^'
      Techniques of Water Resources Investigations Book 7, Chapter C2, 90 p.
    
           8 Prtckett  T  and C. Lonnquist.  (1971)  Selected digital computer
      techniques for 'groundwater resource evaluation.  Illinois State Water Survey
      Bulletin 55,  62  p..-.
    
            » Trescott, P., G.  Pinder, and S; Larson. (1976) Finite-difference model
       for aauifer  simulation in two  dimensions with results of numerical
       fxperSents.   U.S.  Geological  Survey Techniques  of  Water Resources
       Investigations,  Book 7,  Chapter Cl,  116 p.
                                             63
    

    -------
                             f .     Expertise needed to run the models
          To adeauately simulate1 flow situations  using numerical modeling
    
       u ,T°    S^^TlL! of
    techniques  knowledge of
                                                    ,  numerical methods,  computer language,  and
                                                    •   these skilUi  an intuitive sense,  derived
                                                                     determine if predicted
                 values are as expected and are correct.
                       ii.   Data inputs for the models                     •
    
                                               s for numerical models are the
                  required.
    
    
    
                        ill.'  Outputs  from the models
    
                              a.     Ground-water quantity discharge  to surface water
                  (cfs) have been simulated (Eddy and Doesburg,
    
                             "b.     Ground-water quality discharge .to surface water
    
    
                  :      Ae  W4ch Quantity of ground'-water discharge to surface water,  essentially
                  any  conLntratirofVemiLls in  both ground water and. surf ace  water can be
    
                  simulated.                                                                       •
    
    
                         ivl  iettingV'in  which the  methods have been applied and  contaminant
    
                               discharge that  has been modeled
    
                                                           ^ :': Y ^-dei :-'--an:" :'b'e'Calibrated to simulate
                         With enough information, a numerical m        •         enough input data,
    
                  -S            P? S.S^S S^:2^rii  Si»uX«ed.  8Con^iMnc
                   contaminants that have been transported
    !!!!B^^^^
    IlillilliiL'W^^^^^^^^^^^^^^ ' iii'll!':
    IllllijilllllU	l/illlllLliir:" , III ;llli'
    
    llllllllIK^^      	'!"
    lilllilllllllllbul!;"' ihnllFlllli	 , II	Ill1,,'
    •i inpip, < i1. iiiiim	M1 a]!,,,
       ,   ,	
                                                           64
                                                                                                   ;•'! '•«, ,3.:i'i , •• .'•' "iii
    

    -------
          v.    General evaluation of the method            _                 .
    
          Numerical models can be used to simulate various nonpoint source loading
    scenarios for complex aquifer conditions.  Before a numerical model can be
    used for predictive purposes,  however, a large amount of input data is often
    required to properly calibrate the model.  .The amount of data required will
    depend.on the type'of model used, the objectives of the study, and the level
    of accuracy required.  Acquisition of the needed data can require considerable
    time, expertise, and expense.   Because of these constraints, the numerical
    model may have limited usefulness in cases where data are scarce and funding
    is limited.       •         .                 '.  •
    
          The numerical model's strength is its usefulness as a screening tool.
    Numerical models calibrated to simulate watersheds in different'regions  of the
    country could be used to assess  the general effect of various regulatory
    scenarios on ground-water quality in those,watersheds located in those
    •regions...    •  •         .   ,   •   - -  /       •                 •   • .     -
    
    
          vi.   References to annotated bibliography
    
        •  References  to  the accompanying annotated bibliography are summarized in
    Table E-2.        '      .      '      . •   '              •  ' V  -.
                                           65
    

    -------
    • III II-
    i   mi     i       i
                - -   :  ] S I
       ijjjj     i  .    i
    •  i!l| 1   II
                                 Ml
                                 I  II
                     I S « I: • I   i  i»
                     Wisconsin
    
                     Kent, Washington
    
    
                     Pennsylvania
    
    
    
                     Junaau,  Alaska
    
                      Northwestern
                      Indiana
    
                      Central Sand Plain,
                      Wisconsin
    Trinmera Rock
    and CatskilL
    Formations
    
    HendenhalL Basin
    
    Calumet
    Aquifer
                            Organlca, chloroform and tri-
                            chloro«thyl«n«; zinc
    
                            Kitratas
                             Agricultural chemicals
                                                                             D. S. Ch«rkau»t, B. R., U»n§«l
    
                                                                             C. H. Eddy.  J.  H.  Doaiburg
                                                                                                                H.  J.  Gburak, R. R. Schnabal
                                                                                                                S.  T.  Pott»r
                                                                                                                D. I. Siagal
    
                                                                                                                L. R. Hatson, J. M. Fanalaon
                                                                                                                C. Zheng, K. R. Bradbury
                                                                                                                M. P. Anderson
            cr>
     isj:
    

    -------
     Tufcle  K-2.   Kofureuces  to Annotated Bibliography
             Author
                                                                       Citation
     V.  K.  Barwell,  D.  R.  Lee
     D. S. Cherkauer. B. R. Hansel
     V. T. Dubinchuk
     C. M. Eddy, .J. M. Doesburg
     W. J. Gburek. R. 'R. Schnabel
     S. I. Potter
    
     T. A. Prlckett,  T. G.  Nayroik
     C. G. Lonnqulst
      D.  I.  Siegel
      1. R. Watson,  J. M.  Fenelson
      C. Zheng. K. R. -Bradbury
      M. P. Anderson
      C. Zheng,: H. F. H«ng
    '  M. P. Anderson, K. R. Bradbury
     "Determination of Horizontal-to-Vertical  Hydraulic
     Conductivity Ratios  from Seepage Measurements  on  Lake
     Beds."  Hater Resources  Research.  1981.  17:   565-570.
    
     "Ground-Hater Flow  into Lake Michigan from Wisconsin."
     .Im.rn.l of Hydrology.  1986.  Volume 64:   261-271.
    
     "Radon and Radium Discharge  to Surface Streams,".
     Hater Resources.  1981,  8(1):  102-116,  translated
     from Vodnye Resursy.        •
    
     "Remedial Action Modeling Assessment Western Processing
     Site. Kent, Washington." Report prepared for U.S.
     Environmental Protection Agency,  Region X. Seattle,
     Washington  98101.  July 1985.
    
     "Modeling the Effect of the Shallow Weathered Fracture
     Layer on Nitrate Transport." Unpublished Draft Report.
    
     "A  'Random Walk* Solute Transport Model  for Selected Ground
     Quality Evaluations."  Illinois State Water Survey,
     Charapaiun. 1L. 1981. ISWS/BUL-65-81..
    
     "The Recharge-Discharge Function  of Wetlands  near  Juneau,
     Alaska:   Part I.  Hydrogeological Investigations." Ground
     Hater.  1988, 26(4).:  *27-«<..
    
     "Geohydrology of a  Thin Water-Table  Aquifer Adjacent  to Lake
    "Michigan/Northwestern Indiana/:  (in press).
    
     "Role  of  Interceptor Dilches-ln  Limiting the  Spread of
     Contaminants in Ground Water," Ground Water.  1988,
     Volume 26(6):   734-742.
    
      "Analysis of Interceptor Ditches  for Control  of Ground Water
      Pollution," Journal of Hydrology. 1988.  98:   67-81.    '
                                                                         Befarenca to Annotated
                                                                               Bibliography
    pp.173-174
    
    
    
    pp.175-177  .
    
    
    pp.178-179
    
    
    
    pp.180-181
    
    
    
    
    pp.182-184
    
    
    pp.185-187
    
    
    
     pp.188-189
    
    
    
     pp.190-191
    
    
     pp.192-193
    
    
    
     pp.l»4,-196
    

    -------
                                                 inn nil
                                                 i II I ill
               F     Studies involving the application  of  functions  estimating nonpoint
                     source loading to surface water  for various .land us.e types
    i illii  i HI  (i
    I! lil I Mil  1
         Ill	I,!  ^e" Up1.???1	cfted"	Jin	'this	section "are	summarized in Section VI of "An
        Annotated Bibliography of the Literature Addressing Nonpoint Source
        Contaminated Grofn^Witer^Dischargeto Surf ace 'Water," September, 1990, EPA
        440/6-90-006.   	'.	'	'"'	           ".
    
              I.    General description of method
    
                    a.    Description of method or procedure •
    
              Nonpoint source loading models combine surface runoff, sediment yield,
        aTld ground-water discharge with empirical loading rates to  obtain estimates  of
        nitrogen and phosphorous chemical.concentrations in surface water.  Runoff  in
        the watershed is calculated from daily weather data using  the U.S.  Soil
        donservatibn service's Curve Number Equation   Sediment yje"alf "^a*ed .
        using" the Universal Soil Loss Equation in conjunction  with, the  Richardson
        daily rainfall erosivity  index.  Ground-water discharge  is calculated  from
        daily waterbalances  for  the unsaeurated and saturated zones  in a watershed or
        by using hydrograph separation  techniques.  Loading  rates  for  runoff,  sediment
        yield   and ground-water discharge are  assigned based on ..land use.   Land use is
        divided into  residential,  commercial,  industrial,  and  agricultural  categories
        Agricultural  land  is  further  subdivided bksed on land  use   crop type   and land
        management practices.  The land use  loading rates  for  runoff, .sediment yield,
        and ground-water discharge are  summed and multiplied by. the total  area of
        similar land use in the watershed to  obtain the  empirical  loading rate as a
        result  of that  land use"  category".   The total nonpoint  source  loading rate for.
         the drainage basin rate  is obtained by summing  the calculated loading rates
         for each land use  category (Haith andShoemaker,1987, and Ritter,  1986).
    
               The estimation of ground-water" "discharge  from functions is best used in
         coniunction with verification methods such as  mass arid water balance
         ilcliites;ground-water monitoring,  piezometer sampling, and seepage-meter
         monitoring.   Functions'have been used to estimate discharges- in inland
         Satersheds  in Pennsylvania (Gburek, et.  .1.)  and Wisconsin (Uttormark, et
        •ml )   and in Inland Bays in Delaware  (Ritter)  and the Chesapeake Bay (Schnabel
         and Gburek).  Most of the studies utilizing this method have examined nutrient
         loadings into surface waters.       ;
    
                     b.     Assumptions  involved in using these models       .
    
                The inajor "assumption	Of "'nonpoint To'ading	models is'  that  the  empirical  .
         loading rates assigned a  land  use category for  runoff, sediment load  and
         ground-wateroTscharge are representative  of actual loading conditions.  The
         Assigned runoff ,and  ground-water discharge loading  rates  for a land us*
         category areassumed independent of  topography, soil  type, or  tillage methods
          (Schnabel and"Gburfik, 1983).                      '
    
    HJJI    '"'I1,1!      Another	assumption	'is	'tna'r'tne	transport	process'is not  scale dependent;
    1	lhat  is," the"'	SSp'SrScal	loidlng-rBSrCfor  land use «"
    -------
          •  .  .   c.   Limitations of the methods
    
           The ultimate purpose of loading models is to predict the impact various
     land management schemes will have on Surface-water quality in a watershed
     through use of empirical loading factors.  Ideally, loading factors for
     various land types, should only be representative of on-field processes, such
     as tillage and fertilization practices.  In reality, loading factors are a   .
     combination of on-field and off-field processes.  Off-field processes such as
     non-crop plant nutrient uptake, deposition of sediment in buffer strips near
     streams in the watershed, and mixing of interflow and baseflow components of
    'different chemical composition, are included in loading factors.
     Additionally, loading factors make no distinction between, flowpaths,
     effectively masking the processes which contribute to sediment and chemical
     loss from a watershed.  As a result, loading factors mask the interaction of
     on- and off-field processes and cannot be adjusted to account for individual
     changes in either on- and off-field management practices.  Thus, as a
     predictive tool, loading factors may have limited use.
    
           There was significant uncertainty associated with the input parameters
     for the model 'applications referenced  in  this review.  Precipitation and
     temperature data were, collected at one or two locations•in a watershed and
     were  assumed  to be representative for  the entire watershed (Haith and
     Shoemaker  19S7).  The  shallow ground-water  storage value and recession index
     were  assumed  to represent  the  entire watershed  even though several aquifers
     • may discharge  ground  water to  surface  water.  Because  of these uncertainties
     associated with input values  to  the model,  predicted loading rates to  surface
     water may  not be  representative.
    
                  d.     Representative  equations
    
            Ground-water discharge to  a surface water is determined using  a  lumped
     parameter water balance model based on daily water balances  from the
     unsaturated and shallow saturated zones (Haith and Shoemaker,  1987).   The
      equation describing ground-water discharge  is  as follows:
    
        •    Gt- St-r     .   :    .            •     •       _.        '        ...
    
      where: •            .              .' '        '              '               •
    
            Gt -  Ground-water discharge [L3/T]      .                     •
            St -  Shallow  saturated zone moisture content [L ]
            r  -  Ground-water-recession constant, [1/T].
    
       The  loading rate to  surface water as a result of ground-water discharge is:
    
            LR - Gt-C                 .                .         ••   .         '
     i        •.-..-•'         •                       '      :     J.
       where:• • •           .         .          '    '   .           -
    
         '    LR  -   Loading  rate  to  surface water  [M/T]
            ' Gt -   Ground-water  discharge rate  to  surface water [L /T]
         '   'c  -   Concentration of chemical constituent  in  ground water
                                             69
    

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                            e.    Description of equipment needs
    
                Equipment needed  for  the  methodincludes
     •
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    :::;  "  .....    i:1",;  ".     continuous' -chart recorder,
    Illllllll III • III I I I  I  I    III II  I  III    I II   I       . 'li"ii"J» ", MM I 111 I ...... II' " ...... !'|i,iii|iii':,' ........ II, V ........ in'l'i,"'! I.. ........... II 'I ..... '» , ''M ' ,, I*1! "i ..... "I ,!„: ,' ..... II' ,' ,: ...... HJIIIIU'I  • • ' I  , i.   , i         i1    "
                            soil maps,                       .         .
                      v     crop distribution maps, and
                      -     land-use distribution maps.
    
                      A  PC computer-based spreadsheet would be very useful  to  an application
                 of  the method.                                                ,
    
                             f.     Expertise needed  to use the method
    
                      A  significant amount of effort 'is  required to use  this method.   The
                 greatest iRel of effort is required  to  classify land  into  the various
               .  Stories  which involves correlating, soil  type distribution  with land use .
                 and crop distribution in the watershed.   Knowledge  of  relationships between
                 soil t^e  Land use, and crop distribution within the  watershed is usrful.
                 SSr Se'waSrshed'has been'sectioned  into  representative  land-use categories
                 and the recession constant has been determined,  the method becomes a
                 Sokkeeptng exercise.  A computer  spreadsheet can be utilized to multiply and
                 add the calculated  values  to estimate the loading rate to surface water.
    
    
                       ii,   Data inputs  for the  model
    
                       The model requires  data describing land use and soil type distribution
                 and daily precipitation.   The ground-water recession constant can be  estimated
                 using standard hydrograph separation techniques and stream gage data.
          iii.  Outputs from the model
    
          The" method'' estimates' ..... the" loa          ,
    ground^ater discharge, sediment  load,  and surface runoff for various land
                        The method'' estimates' ..... the" loading rate, to ' surface water  as "a result of
                  uses.
    
                              a.
                       Ground-water quantity discharge to surface water
                       "The amount of ground-water  discharge  to  surface  water predicted by this
                  method is Tfunction of the recession constant and the storage capacity of the
                                                                        and thsta    are
                                    "-•                                      vba«
                  small, the predicted discharge  rate will be small;  conversely, if both are
                  large, the predicted discharge  rate will be large.
    
                               b.    Ground-water  quality discharge to surface water
                         The  chemical  constituents commonly modeled using this methor
                  nitrogen and phosphorous (Haith and Shoemaker, 1987)   ThVCOM;n!"-t££ln|r
                  predicted  in surface water using these methods are a function of the  loading
                                                         70.
       III IIIB^^^ IIIIH i il	                          .                    	Jill	lililll	ill	iii	l!i^^^^^^^ 	             •       	-'-.ii.!.'..'!;!'	'
    

    -------
    rates assigned to the various land types and land use distribution.
    
                                               •'
          iv.   Settings in which the models have been applied and  contaminants
                that have been modeled
    
          The  settings  and the contaminants that have been modeled, using  this
    method are summarized in Table  F-l.
    
    
          v.    General evaluation  of the  method
    
          The  method has obvious  appeal  for many applications because information
    concerning land use, soil  type  distribution, precipitation and  temperature
    data, and  stream stage are readily available for iaost watersheds.
    Additionally,  the method  is  relatively easy to  use.  Once a  computer  spread.
    sheet containing the required inputs has been established for a given
    watershed, by inputting weather data,  the  loading  rate  to surface water can be
    estimated. However, ultimately any  model  used  for management decisions must
    be able  to predict  future  loading rates  as a result  of  changes  in management
    practices.  Because loading  models  rely  on a multicomponent  loading factor,
    the effect of changing one component of  the loading  factor on surface-water
    quality  may be difficult  to  determine, making  the  models .le;ss suited for
    ..management applications.      '                             •
    
    
           vi.    References to annotated bibliography                              •
    
           References to the accompanying annotated bibliography are 'summarized in
     Table F-2.
                                            71
    

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    -------
    Table V 2.  Kuforunces to Annotated Bibliography
            Author
                                                                      Citation
                                                                         Reference  to Annotated
                                                                                Bibliography
    W. J. Gburek, J. B. Urban
    R. R. Schnabel
    0. A. Haith, L. L. Shoemaker
     "Nitrate Contamination of 'Ground Hater  in  an Upland
     Pennsylvania Hatershed,"  Proceedings  of the  Agricultural
     Impacts on Ground Mater,  A  Conference,  Omaha,  Nebraska,
     August 11-13,  1986.  pp.  352-380.
    
     "Generalized Watershed Loading Functions for Stream  Flow
     Flow Nutrients," Hater Resources Bulletin.  1987,  23(3):
                                                                                                                                         pp. 160-162
                                                                                                                                         pp. 163-165
    W  F. HILLur
    R. R. Schnabel. H. J. Gburek
    P, 0. Uttormark, J. D. Chapln
    . "Nutrient Budgets for the Inland. Bays,"  Report  to Delaware
     Department of Natural Resources and Environmental Control,
     August,  1986.                         .
    
     "Calibration of NFS Model Loading Factors," Journal of
     Environmental Engineering. 1983.
    
     "Estimating Nutrient Loading of Lakes from Non  Point Sources,
     Office of Research and Monitoring, 1974, Environmental
     Protection Agency report number PA 660/3-74-020.
    pp. 166-167
    
    
    
    pp. 168- 169
    
    
    pp. 170-171
    

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                :]V^                           ^PBSflHIlJ-iflB!If Si|.?f ^OTTOT1?-IB?;;i!'^f • • \;'i•* A';'.• •' • \ <' • •''•':;• •'' •':':!:;i:! -i;i:.,I• '•'W': II1 '••' 1?!
               G.'='' ' Studies "us'ing environmental"'' Isotope" methods" to" estimate the' contribution
                     of ground water to stream flow
                         papers Sited  in this section are  summarized in Section XI of "An
                         «?KiLraphv  of the Literature Addressing Nonpoint Source
                             gSSt:* Discharge  to. Surface Water," September, 1990, EPA
               440/6-90-006.              ,                            :     .
                     i.    General description of method
                           a     Description of  method or procedure
                                «opes   . con-only used in           ,
                    t.           ,.„„,, is fiso^  deuterium (D  or  H) , ana tritium  {i  or  n; .
                Thlse^isTtope0* are all t ideal facers 'for runoff generation  studies,  due- to
                These  isotopes are aimos                          ^ T are constituent parts
                KP principal characteristics   Qi; sin      ,   ^                    L  ^ ?he
    are altered only by physical processes  such as:   mixing,  diffusion,
    dispersion, and radioactive decay.
          Both "0 and D are stable isotopes which occur naturally, accounting  for.
                                                                             -
                      °^£ -SiE^^JS^^^-^^M^ -ef
                      are about 2000 and 320 ppm, respectively.  T is a radiogenic  isotope ,  of
                      gen whose half -life is in the order of 12.4 years^ T atoms represent an
                 of thermonuclear devices in 1952, T produced as a by-product of this testing  .
                 has been the dominant source of T in precipitation.
                       The "tern" "hydrograph separation," discussed in section D of  this  report
                                              IS OS ve JLU^CVA do ^*»» »•«*«.*-» «-— —	   *      —
                                             different flow paths and have different residence
                 times".  	 •	, 	    .'      	      :
                                                        74
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    -------
                                                                                          •1
              tracer- based
    
                  any' ^during    ^Jf^le runoff event is a mixture of
               «     -new water," which is water from the current rain or snowmelt
               "old wat"- which is the subsurface water which existed in the
    catchment prior to the "current rain.
    
    
    
         '
            -old*-  and -nlw"' water  components  are chemically or  isotopically
             t  the stream water becomes  "diluted- by  the addition of  the  -new-    .-
    
     watr   The extent of this dilution  is a function of the relative
     contributions 'from the -old"  and "new" water  components,
    
    
           The precursor to using natural isotopes as  tracers  in the  simple  two-
    
    
    
    
    
     concentrations. of most chemical parameters than -new water? .
    
    
          • The major problem- associated with separating hydrographs on the basis of
    
    
    
    
    
    
    
      -oS".f r-  contribution  since  the  -new' water- P^«J— ^^ ^iTSat of
      solutes on its way to • the stream and its chemistry becomes more  like that
      the -old water".   One can, however, derive some valuable  information^
    
    
    
    '
      deposited particulates by overland flow.
    
    
    
            During the I960- s, hydrologists began to use- the separation equations
    
      with anthropogenically-produced radioisotopes.
    
    
    
                  b.    Assumptions involved in using the method
                                                                         - •- «
       snowmelt hydrograph can be determined.                                     .
                                             75
    

    -------
    illlllllllllli I I 111 I I   1(11   II ill	I 1111111
                annual sinusoidal cycle with the most  depleted values in  the  winter and the
                least depleted values in the summer.   Whether the "old" water del values are
                constant or cyclical is controlled by  the residence time  of the "old" water
          	 i, f^jf	|fte ,difpee of dispersive flow in the watershed.  The  "old" water tritium
          	concentrations,	in	small	watersheds	generally show a gradual decrease with
                Ctme, reflecting  the progressively lower tritium concentrations in recent
                (post-1963) precipitation and tritium  decay.
    
                      The isotopic signature of the "new" water component provides the
               ,co:E^?:as5 n??ded for the isotopic separation.   Although the general seasonal
          	Y^.Eif.'rlSB,?.	In	iS6,	"9,,«	PJ and. T. concentrations	in	precipitation and the
          ',,"«.«,,, '",;?,*£?£*?:	i£n,I,*,H?,,51	decline	in^ tritium	levels	are	documented, it must be  "
                emphasized that there is no guarantee  that the "new" water in  an  individual
    
      !^^                             	Ili^^^f^^^r"^^	..d-.Ipe."n^»-"?.,irh^e.'"?ld"  Wer-
                      Fourassumptions govern the reliability of hydrograph separations  using
                environmental  isotopes:
    
                  '    •     The "new" and "old" water  component can be characterized  by  a
                            single isotopic value for  each component or variations  in each
                                       3  Isotopic content  can  be  documented.
                      •     The isotopic  content of the "old water"  component is significantly
    Illililll  Ml  I in I     PI I ill  I i I  i different  from that of the "new water" component.
                                P                              »                 ,','!'
                      •     Vadose zone water contributions to  the stream are negligible
       .                    during the event or they must be accounted for (use an additional
                            tracer if  isotopically different from ground water) .•
                            Surface waterstorage (channel storage,  ponds,  swamps, etc.)
                            contributions  to  the stream are negligible  during the runoff
                            event.
                                                       76
         r
    
    iiiiiiiiii  in in  i  i     11           i ill
    Ulilllill	(H (i Ili    INI1     i       Mill
                            cJ    Limitations  of the method                ,
            I'll. ',.i in.,.!, iiiii.li!!1;. if i; M,	iiiniji.!!	ef'tix liiiiiiiiiii11 :-i M* «';>!**;	          •          sii ..:: ;'	fS1;.*!	".i	Kef,, »:;*»*: •I'j"-'!*	i. '•«•••„   ...  '  . ..';:::'. ;. •  ": 'ii
                      One major assumption in  using, environmental isotopes is that the
               baseflow represents the  "old"  water component and the source of ground-water
               flow to  the stream during  storm and snowmelt events  is  the same as the source
               during	baseflow	conditions.	However,,	ephemeral springs remote from 'the. stream
            ""'  "or'TC	'ground"-wafer	flow	sy'ste'as'	may 'contribute differently during events
               and  if their isotopic signatures differ from that of baseflow, the assumed
               ^old water" isotopic value may be- incorrect.  Although  the occurrence of such
               situations could be tested"by  hydrometrie monitoring and isotopic analyses of
    in mi Illililll MI i these features, qualification  could be difficult.
    ill1 ill in inii| in "i i    iiiii	i	i1  i i-   i in             I,  ,,       i    '      ".LI     ',:, '•;;•' •' "'•'  .: .,'.  .•  •.-.' "  '•  :»;.i* "i-\  •'**••'•
                      Catchments with significant surface storage cannot be accurately
               characterized using isotope  hydrograph separation methods.   Isotopic
               enrichment of surface water  in lakes, ponds, and swamps by evaporation may
               introduce complications  in the simple two component  model.
    II III 111 III HIM IIIII IIII III III    III IIII I    II II   I    IIII III III III    II   Illililll    IIIII   II    II    I     II   ... .... !,',.* '. . :i . .LI   ....   .:	 '.I1 ».. "iT.	III. '. .  ',..
                      During some events,  the  "old" and "new" water  isotopic contents may be
               too  similar for meaningful hydrograph separations.   .Considering that
               substantial time may be  spent  waiting for and then sampling an event and
        Illililll II III 111    IIIIIIIIII I
       111 11 Illlllllllllli 1111 Illililll II Illililll 111 III ill III III III I III II Illililll 1111III
    

    -------
     considerable costs "may be incurred for isotopic analyses, it is prudent to
     monitor  an event using chemical tracers as well as isotope analysis.  These
     other  methods may include:   (1) testing for other independent isotopes such as
     T  rather, than, 180  if 180 is  unsuitable and (2)  testing for a conservative
     chemical constituent,  such as silica, or other less conservative parameters
     such as  electrical .conductivity.
    
           Estimating the actual isotopic composition of the rainfall reaching the
     ground surface is complicated in forested catchments because of the
     interception loss (by evaporation) from the forest canopy during rainfall.
     Evaporation from water, stored on the forest canopy typically occurs at rates
     of 0.1-0.5 mm/hr and can account for the loss -of about 20X of the gross _
     rainfall.  Depending on the ambient relative humidity at the canopy level,
     evaporation of 20X of the rainfall could substantially enrich the D or 180
     composition of throughfall and net rainfall compared with that of the gross
     rainfall usually measured and sampled.  This is a po.tentially serious problem
    . only when the. gross rainfall is isotopically lighter (more negative in delta
     notation; equation [1] below) than the prestorm stream water.     ,           .^
    
                 d.    Representative, equations                ,
    
          ' Since D and 180  concentrations  in- natural waters .are  much smaller  than
     their  common light isotopes (:H and 160) , D and 180 concentrations are  _
     generally expressed in 'the conventional delta  (8). notation as per mil (0/00)  •
     differences relative to the international. standard, SMOW:
    
            5D or 5180 - (Rsamole - RSMOW)  X 1000   [1]
                              RSMOW               .
    
     Analytical precision for 5D and 5180 by mass spectrometry is better than  2 and
     0.2X,  respectively, with a confidence  level of 95Z.
    
           Between storm events-, stream base flow reflects the isotopic composition
     of the  "old"  (stored) water.   During storm runoff events, however, the
     isotopic character of  the  stream may be altered by the addition of "new"  water
     from rainfall^  The r old"  and  "new" .water contributions  at any specified .time
     can be  calculated by solving the "mass  balance  equations  for the water and
     isotopic fluxes  in the  stream.  These  equations  are expressed as:
       '    Q8 - Qo + Qn        .     .     .                    -
    
           C.Q. - C0Q0  +, CnQn        '       •               . -   ;•  [-3]-
    
           Oo  -  CCs  -  Cn)  x 0.      -         .                     [*]   '
                  (Co - Cn)
    
     where Q is  discharge, C expresses  tracer  concentration,  and the  subscripts  s,
     o,  and  n. refer  to the "stream,  "old water,"  and "new water," respectively.   The
     utility of  the  mass balance equations  for arty particular storm event is  -
     controlled  mainly by  the magnitude of  (C0 - C^) relative to .the analytical
     error and the recognition of areal and temporal variations in C0  and Cn.  The
     equations can also provide estimates of- "old" and "new"  water percentage
     contributions to' throughflow and overland flow.                             .
    
           -   '       '  .'     .                77
    o
    

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                    Environmental isotope data can also'used in estimating the  areal extent
              of overland  flow contributing areas and in calculating mean residence time of
              the "old" water in the catchment.  Assuming that overland flow  is generated
              entirely as  saturated overland flow, the overland flow contributing area is
              estimated by the following equation:
                           Y -
                                                                            •IS]
                where Y is  the  discharge area expressed"-'as  a fraction of the total  basin area,
                V  is the total volume  of "new water" which  leaves  the catchment and Vto is
                the total volume  of "new water" which  falls on the catchment.  The  mean
                residence time  of the "old water"  in a catchment can be estimated by  comparing
                the seasonal variations in del values  for the precipitation and*h* |«*fflow
                or by analyzing the tritium input  (precipitation) and output  (streamflow)
                functions.
    
                             e.     Description" of'" equipment'' 'heeds
    III || II11   || I ||     Ililllll I            Ml 111   " i ,11V" .in i "i": !'  , | •: 'I" ii	•»!' &, nih;' • u ;<;"" ;|i' iiru, a i, ,i;.,}; f,	a•• i;:: |!<: :,:"•' r $ 1 y ar"	h 'i y	;',, v, >.|	' „;: < •«; •:" || r I,'. i' i, "I, >...: ,: ; .   ,,,!.•    i •  ' i   • i, ', •' "i
    in iiiwini ii in 1    1  iiiiiii i  iii   i   ii iiiiiii   Af. *;.;-'iv'.'?a^tMi; -i''-^^^'^'^!!!'^*^ ^'i\\.i"^^^^i'Mvi.\ii^ $yKfi.'i-w '•'••' •>••• j	• '•>• • '  >•!  •• '
                      Stage or precipitation activated  time discrete automatic water  samplers are
                needed  to ensure sampling  at  the start of  an event,  .especially  for night-time
                storms  or for remote catchments.  Snowmelt lysimeters are needed  for sampling
                snowmelt.   To sample soil water, lysimeters  are required.   Ground-water samples
                are  obtained by  installing  piezometers.    Measurements  of  streamflow from
                catchments require weirs with stage recorders.
    
                       The concentration^  of "0 and D  in" a water sample- are  normally measured
                using a doubleTcoIIectih-g mass  spScCrofltoter which compares the concentration  of
                 18o «r n in the water sample to a standard water.  Water  samples for T analysis
                   or D in the water sampl
               are measured using a liquid scintillation counter.
    
                            f.     Expertise required  to  apply this method
    
                      The  method" requires knowledge "of basin characteristics and  the .temporal
               distributionof precipitation and  runoff in the basin as weU as  considerable
               professional judgement.'  Site water sampling requires a sufficient
               understanding of regional geology  and hydrology.         •
    ilw'rw ''
                        ii.    Data inputs for the method
    
                        To determine the "old"'water isotopic value, the samples  to  be obtained^
           « v-fincluoVthe following:  ground water at various sites (shallow
                               soil  mb'istiire'-ae1 "seveYal sites  (shallow or deep),  and
                            rier ..... stream ......... in ..... the catchment or baseflow  in a larger order stream.
                 ost IsotopiE studies have used either ground  water or baseflow to
                Characterize the  isotopic content of the "old" water.   The isotopic value of
                streak baseflow is- a good approximation of the isotopic -al-%of,Sround.water
              '  discharging into  the stream.  Soil moisture is also appropriate for the  "old
                water component in certain hydrologic environments.
                        i;,i ,'.' .ii iiiiiii .i*Hr«'.MHJiiMi»[*:Lffi'iii ..... ;.;' iii'i! ; j'''i ';(«:. iFyiiii ..... »iii:'ii::i":iw:;";iii:!iiiii<. ..... i ..... new ...... s. ..... i ..... -v -t, ...... ,1 ......... Kiiiimi1"!"' t ; • . "  •• • • •   '_*;.. in1 «.«'
                           simples are needed when conducting environmental isotope studies
                                    runoff ;  i.e., 'one must take  as many time discrete  samples
                     liS ;. . M"!,!,	,,; IHIIK I	" I" :., "", "ii'ipf !"J". . J • •' !1"!' .I1,!;,1 -IfJ1 (nlf	I a1"-;".™,!!>",	'."If	!,.,ll>'l
                                                       .78
                .                       .               	lirK              	M';!!,!;
    

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     of the precipitation (arid, snowmelt) and the stream as possible.  Depending on
     the nature of the study, sampling frequency may vary from minutes to day or
     loneer depending on the size of the catchment, type of sampling equipment
     type of event, and detail desired.  Through flow, overland and macropore flow
     sources can also be separated.using isotopic methods,
    
    
           iii.  Outputs for the method    .
    
                .a.    Ground-water quantity discharge to surface water
    
           Essentially any  quantity of  ground-water discharge - to surface water can
     be  estimated  using  isotopic tracer-based hydrograph  separation techniques
     Isotopes  leave  signatures of  stored water  (in the unsaturated and saturated
     zones)  that can be  detected at the discharge  points..  Environmental ^otope  _
     results can be  used .to test whether integrated water quality models represent
     catchment processes appropriately.
    
    '••''     .   b.    Ground-water quality discharge to  surface water   .
    
            Observed  contaminant  concentrations  in surface water can be  correlated
     with the  runoff components  Indicated  by the isotopic data.  For  example,  if   ;
     stream flow  is  found  to be  dominated  by "old" water  during a  precipitation   .
     event and observed contaminant concentrations rise above baseflow
    ' concentrations-, the increased contaminant  levels may presumably  arise from
     subsurface .discharge.
    
    
             iv.   Settings  in which the method .has been applied
    
             Some of  the  settings assessed and the isotopes analyzed in           _
      representative  studies are presented in Table G-l.   The predominant conclus-ion
      from these studies is  that "old" water components normally dominate storm and
      snowmelt  runoff in humid, headwater catchments.  These studies demonstrate how
      isotope  tracer studies.can improve the characterization of runoff processes
      beyond those findings based  upon  hydrometric and/or hydrochemical data,.
            v.
                   General evaluation of  the method
             Because isotopic tracers  are  constituent parts  of natural water  .   _
       molecules,  they can be used as  excellent tracers -of water  origin  and.movement^
       The long term and widespread application of these  tracers  analyses,  will allow
       researcLrs to study runoff generation on. scales ranging from »a«°P°5" |°
       portions of catchment slopes to first and higher order streams (Sklash 1990).
    
             Several disadvantages may arise, in the use of  isotopic tracers,  however.
       Conditions for  thai*  use  are not met  in every  event, arid  sample  «£y™  £
       expensive   In some catchments, the isotopic content of  "old" and "new  waters
       is not  distinguishable in  the  snowmelt, and variability in the  "new water"
       isotopic component may decrease the precision of the separation.
                                             79
    

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    in in  i i  in PHI  i   ill 11 in
    vi.   References  to  annotated bibliography
    ^^ — ^ ^'    o;anin  annocated bibliography are provided in Table
               G-2.
    Ill  I mi
                                                          80
    

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    C 1.    Suowary of Settings In Milch the Method Uaa Been Applied and the laotopea Heanured
            Location
                                     Catclunenl Size (km2)
    Isotope
    180          D
                                                                                                        Author(s)
    1       France
                                     2*
                             E. Crouiet,
                             P. Hubert,     -
                             P. Ollv.,     .
                             E. Sluertz.
                             A. Horc« (1970)
            United Kingdom
                                      1.0
                                                                                                        D.S. Blegln (1971)
            Mother lands
            Canada
                                      650 ha
                                      JO. 5.  >.24,  1.76
                             H.G. Hook.              .
                             O.J. Groanvald
                             A.E. Bouwn,
                             A.J. Van Ganswyk  (197*)
    <, Canada 22, 1.6
    
    
    5 Canada 73 to 700
    
    6 Canada 1. 1.2. 3.9
    * P. Fritz,
    • ' J.A.1 Charry,
    K.U. Heyer,
    H.G. Sklash (1976) .
    « H.G. Sfclash.
    . R.N. Farvolden,
    P. Fritz (1976)
    * H.G. Sklash.
    R.H. Farvoldan. (1976)
                              D.J.  Bottomley,
                              0.  Craig,
                              L.M.  Johnston (198
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    t
    

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    G 1.    S.«ai»ary of Setting lu Milcli th. MoU.od Uaa Boon Applied «nd the I.otope.. Ma.uured
    U Location Catchment Size (km2) Isotope Author(s)
    ' T 180 . D . '
    18 Canada ' • 368 * . *
    19 Canada . .2.8 * • * ;
    20 Sweden ' 4.0, 6.8 .
    •21 Swuden . several '
    22 . Canada . 10.5 . , *
    
    23 Norway 41 ha . • , • .
    ,' :•
    24 USA'. - *2'-2 . . . *
    25 Canada .60 *
    26 Canada 10.5 *
    
    
    P.M. Schwartz (1980)
    H.G. Sklash.
    R.N. F«rvolden (1980)
    A. Rodh* (1981)
    A. Rodhe (1984) ,
    D.J. Bottoraley, . .
    D. Craig,
    L.H.- Johnston (1984)
    N. Christophersen,
    S. Kjiernsrod,
    'A. Rodhe (1985)
    : R.P.- Hooper,
    C.A. Shoemaker (1986),
    H.H. Obradovic. .
    H.G. Sklash (1986)
    A.J. Bottoraley,
    0. Craig.
    L.M. Johnston (1986)
     27
             USA
                                                                                                           J.R. Lawrence  (1987)
    

    -------
    l!
          =>=  Author
    Ill B   ill
    Mil!* I
    
                                                                                Citation
                                                                                                                    Rafarttacv to
                                                                                                                    Annotated
    I i  !  Si
              H.  G.  Sklash
              M. G. Skiash,
              I. D. Moore,
              G. J. Burch
    R. P. Hooper,
    C. A. Shoemaker
    
    P. Maloszewskl,
    H. Rauert,
    H. Stlchler. ,H.  Herrmann
    
    M. G. Sklash,
    •R. H. Farvolden
                                          "EnvlroiwwntaL  Isotope Studies ot Storm and SnoMnelt
                                          and  Runoft Generation,"  In Surface  and Subsurface Processes
                                          in Hydrogeology, H. G. Anderson  and T. P.  Burt.  (ad.).
                                          Joint Hlley and  Suns Ltd., Sussex, England.  73  p.-, 1990,
                                          In print.
    
                                          "Environmental  Isotope Tracer Studies of  Catchment  Proceases:
                                          Tools for Verifying  Integrated Hater  Quality Models,"   In:  •
                                          Proceedings  of  the USDA, AIRS-B1,  pp. «,59-W.  International
                                          Symposium  on Hater Quality  Modeling of  Agricultural Non-point
                                          Sources.
    
                                          "A Comparison of Chemical and Isotoplc  Hydrograph Separation,"
                                          Separation," Hater RasouiVes Research.  1986,  pp. 1**4-1«5».
    
                                          "Application of Flow Models in an Alpine Catchment Area Using
                                          Tritium and Deuterium Data." Journal of Hydrology.  1983. 66:
                                                  319-330.
    
                                          "The Role of Groundwater in Storm Runoff," Journal of Hydrology.
                                          1979, O: *5-65.                           	
                                                                                                                                                           p. 289
                                                                                                                                                            pp.2B5-286 ;  ,  :
    
    
                                                                                                                                                            pp.287-288 -[•-  '
    

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                                      Chapter III
    
           The Impact of Nonpoint Source Contaminated Ground-Water Discharge
                to Surface Water in Water Quality-Limited Water Bodies:
    
            Determining Total Maximum Daily Load and Waste Load Allocations
     Introduction'
    
           This  chapter provides a general overview of the process for determining
     the Total Maximum Daily Load (TMDL)  for water quality-limited water bodies and
     the allocation of point source waste loads  and nonppint source- loads to
     achieve the TMDL.   .  \              ,     ,
    
     :      As,used in-this, chapter, TMDLs are'defined as the assimilative capacity.
     of a waterbody,  which! is the sum of the individual Waste Load'Allocations
     (WLAs) for  point sources and Load-Allocations (LAs) for nonpoint sources and
     natural background (see 40 CFR 130.2(h)),  plus a safety factor.  A Waste Load
     Allocation  is the portion of a receiving water's loading capacity that is
     allocated to one of its existing.or future point sources of -pollution (see 40
     CFR 130.2(g)).  Similarly, Load Allocations (LAs) are the portions of a
     receiving water's loading capacity.that is attributed either to one of its
     existing or future nonpoint sources of pollution or to natural background
     sources  (see 40 CFR 130.2(f)).. In sum, the TMDL should encompass the
    "contaminant waste loads from point sources and nonpoint sources.  However, the
     nonpoint source load allocation may be accounted for simply as a component of
     background contaminant concentrations.  This chapter provides a preliminary
     discussion of the rationale for applying the methods described under 2 above
     to better measure or estimate the nonpoint source component of the load
     allocation under a TMDL.                               .
    
           Under Section 319 of the Clean Water Act, by August 4, 1988 the States
     were  required to identify those water bodies that were not expected to attain
     •or maintain their respective water quality standards due to point or nonpoint
     source  loads.  In addition, the States were directed to develop a program to
     alleviate  these  problems, by describing how they will utilize the TMDL process
     to control nonpoint source pollution  in accordance with Section 319 (b) (2)
     (B) of  the Clean Water Act.   This Section calls for "an identification of
     'programs to achieve implementation of the best management practices (BMPs) by
     the categories,  subcategories, and particular nonpoint sources designated
     under subparagraph  (A)."   Subparagraph  (A) requires an identification of the
     BMPs  and measures which will.be undertaken to reduce pollutant loadings
     resulting  from  each category,, subcategory, or particular nonpoint source  .
     designated under Section  319  (a)  (1)  (B).  Presently, this requirement is the
     only  regulatory tool  available under  the Clean Water Act to promote nonpoint
     source controls.  To  date,  the Agency has prepared a variety of guidance
     documents  and models  to assist in determining TMDLs as part of the water
                                            85
    

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                quality-based permitting process.  l  This discussion  specifically addresses
                the manner  in which nonpbint source  loads  may be accounted for in this
                process.
    
                      The chapter is organized infour sections.  Following this introduction,
                Section 2 introduces the regulatory  concepts and statutory authorities
                          theTMDL aidloadallocation processes.  Section 2 also- provides a
                sumfflary of  the  status of WIA applications  and water quality-based permitting
                Section 3 discusses the theory behind the  TMDL process and the application of
                3?VJ!	wIS	regard to estimating	water	quality impacts 'from biochemical oxygen
                Demand, nutrients, and toxic substances and provides a limited overview of WIA
                modeling approaches.  Finally, Section 4 reviews .the applicability of the
                lethods described in  2 to supply the data needed to assess nonpoint source
                loads as part of a TMDL analysis.
                 A<     Statutory and regulatory, mandate for determining WLAs and LAs under  the
               	"	TMDL process       •       •
    
                            "Rationale behind waste load alioc'ffclon and water-quality fcased
                            i-p-grmitting     '                          -.'•.-
                                                                              .      ,  .  ,
                                     303ofeCeat,-'	IKS"States 'are  required to  set
                          !i"ty	standard's	^at-protecl	the "public -health or welfare,  enhance  the
                         ol	wfcef;	arid	serve "the purposes  of'the Act for all  waters  in the
                          These standards are based on water quality criteria developed by
                 U S  EPA3 and are to guarantee the achievement of a designated  use  for the
                 water body.  The State may not set a water body's  designated use at^less than
                 fishable/swimmable without performing a use  attainability analysis.   •
        Mill1 III' 111!  ti
    ill	Ill	
          1  EPA  is  in the process  of,preparing a series  of nine Waste Load
     Allocation guidance	aScumetiits":"	Several of those documents that are currently
    	SvaJiWe1	f?om	the	Monitoring and Data Support Division/U.S .  EPA are cited in
     this chapter.
    
     .     2See aiso 48 £E 51400  for the regulations implementing the water
     quality standard process.
    
                   water quality criteria are developed under Section 304(a) of the
                  ct;  ""^ ^ Criteria  for Water 1986.. published May 1987,  is the
     most recent EPA summary of water quality criteria.
     III II III I I I  III III I  III I II   III 111111  I II   II I  III   I  II   I I II II11  I  I III    I   I      II    I           ' ,     >'
    
          *  Use attainability analyses involve a determination of the level of
     aquatic  protection that can  beachieved  for a water body  The  analysis     -
     iSsKaei^n	assessment	of  (1) what  are the aquatic uses(s) currently being  .
     achieved in the water body,- (2) what are the potential  uses  that can be
     attained based on  the physical, chemical,  and Biological <*a""^e £j  Jf
     Chewater"body;and(3)what are the causes of  any impairment of the uses?
         T  Hn-igal Support Manual:   Water Body Surveys  and Aegaggmants for
     Conducting tTge Attainability Analyses. November 1983. USEPA/OW.
    
                                           .86
        HI ill
                              II IPl
    

    -------
          Sections 302 and 304(1) of the Clean Water Act require the States to
    identify those waters for which technology-based effluent limitations are not
    sufficiently stringent to attain the water quality standards.  The technology-
    based limits are mandated under Sections 301 and 307 of the Act and are
    implemented by the Agency through the promulgation of industry-specific.
    effluent guidelines.5  The States must rank their water quality-limited
    stretches for planning purposes and set total maximum daily -loads of
    pollutants in the stretches that will achieve the applicable standard.
    Finally, the TMDLs are to be converted to wasteload allocations through
    modeling and ultimately to water quality-based effluent limitations on
    individual point source dischargers in the limited stretch.
    
          ii.   Implementing waste load allocations and load allocation in water
                quality-limited water bodies
    
          Water quality-based controls are implemented for any stream segment in
    which it is know that water quality does not meet applicable water quality
    standards, and/or is not expected to meet applicable water quality standards,
    even after the application of the technology-based effluent-limitations
    required by Sections 301 (B). and 306 of the Clean Water Act (see 40 CFR
    130.2(i)).  For these segments, water quality-based effluent limits, may be
         5 Under Sections "301 and 307 of the Clean Water Act, as amended-in 1972',
    .EPA  is responsible  for promulgating technology-based effluent  guidelines,  and
    applying  these  guidelines  in permits to' industrial point source  dischargers.
    EPA  is to review  standards  annually and to revise them every three years.
    Equivalent technology based standards  also apply to municipal  discharges;
    these have been defined by  EPA  as secondary  treatment  of municipal wastewater.
    
          Under the 1972  amendments, industrial  point sources were required to
    apply the best  practicable  control technology currently available  (BPT) to
    their processes by  July 1,  1977.  BPT  was interpreted  as involving mainly",
    "end-of-pipe" controls that imposed control  costs and  economic impacts that.
    were not  "wholly, out  of proportion" with water  quality benefits.   In the
    second phase of pollution control,- the Act mandated that industries  were  to
    adopt best available  technology economically.achievable (BAT), or, if
    feasible, zero  discharge,  by July  1, 198.3.   In  contrast, to  BPT,  BAT  was
    thought of primarily  as  in-plant process changes that  had been or were capable
    of being  achieved.  Compliance  costs were considered  in setting  BAT,  but  no
    cost-benefit analysis was necessary as with  BPT.  Finally,  new sources were   •
    expected  to immediately,  comply  with strict standards of performance  based on
    best available  demonstrated control technology  (BACT), a standard  comparable
     to BAT  for existing sources.     .    '••'".'•                ' ,  '
    
          Under the 1977  amendments to  the Act,  Congress  modified  the  original
     technology-forcing approach somewhat  to include a new category of  control,.
    besf conventional pollutant control  technology  (BCT),  to be achieved by July
     1, 1984.   However,  EPA found the BCT  cost  tests difficult to apply and; as .a
    •result,  for most industry, categories  the BCT effluent limitations  are
    virtually equivalent to  BPT requirements.     .    •   ,  •
                                           87
    

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                                                                           rm	KV ; ilililii;,!!'11!'1":1!!!;!!!!!!
                  :;;)	liii;!:1:!*1'1!!!*;,;,	sir #;(„,;:
                               I .".MI.; ,„:•	is '"Si"* i tf	illM!'11 ii" ;	I; .'!
    Illlil1
    imposed on point source dischargers under  the  authority of Sections 302 and
    402 of the Clean Water Act.  Water quality-based effluent, limits are derived
    co protect water7qualityInthe  receiving  water regardless of cost or waste
    stream cfeaTabilitty.  In  addition, however,  Section 302 of the Act makes
    provision for permitees to apply for  variances from the water quality-based
    effluent limits based upon the  "relationship between the economic and social
    costsandthebei»:f£fstobeobtained from achieving such limitation."
    
        1  Control programs for nonpoint  sources are developed as .part of the
    planning processdescribed under Section 319 of the Clean Water Act.  In many
    cases  States do not have certified  or established techniques or procedures
    for completing  load allocations.In those cases, the State should present its
    overall schedule form implementing the TMDL process and a schedule with
    milestones  for  establishing  the appropriate load allocations.  Vntil the load
    allocation  is approved by EPA,  the State should pursue a technology-based
    approach.   Technology-based  controls are to be based upon water quality   .
    considerations  and not just  resource protection.  For example  while
    agricultural management  activities are directed at minimizing soil erosion for
    productivity purposes,  the  technology-based approach requires the
    landowner/operatortoinclude not only productivity based controls but offsite
    measures  such  a filter strips and sediment and water control structures, as
    well    If BMP  implementation is not adequate,  the State .-should develop an
    action plan to  develop additional BMPS, including a schedule to assess the
    waceY cjlillity conditions and determine if "standards are being met within an
     appropriate timeframe.
      ill i i i  w     in i  niiinii          n in  i i  i  i  n  11      i      i      i '  i      ,«.'
     B,    Determining the Total Maximum Daily Load
    
           This section presents a brief  description of  the scientific
     Understanding of the processes  underlying estimates of total maximum daily   .
     load   Because the  approach for assessing water quality impacts  from different
     categories of contaminants  varies, each of three classes- of substances,
     biochemical oxygen  demand,  nutrients,  and toxics is discussed separately.
    
    
           i.    Theory  behind Waste Load Allocation          '
                       Basic Principles              -                                . '
    
                        Qt^ ^— imum "D'aily "Load"assessments provide- information 'to assist in
                        iffective	decisions on levels of treatment required for *««"£•£
                         of pollutant load.  WLAs are water quality oriented and are ^rected^
        	:	~	'	•---::•; re-iJltiBlTsfeLni	a qualitative relationship between a particular waste load and
                 ics impact on water quality.  These relationships make it possible to compare
        £^	::"; Incremental changes in .concentrations of specific constituents in the
        	water "System;	One^is then able to.identify the maximum; waste load
                      can beDischarged without violating a water quality standard.
                                                    IIIH	ii	"PHI mi"» i iii	mi	
                      s  Technical Guidance Manual-for Performing Waste Load Allocations.
                         Guidance.
    
                                                        88
       '	 -	
      	I	
    

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         .Because of the array of variable elements (e.g:, temperature, stream
    flow  load level, reaction rates) that must be considered in WLAs,.
    computerized mathematical models are generally employed to make the necessary
    calculations.  Furthermore, the factors and model formats also differ
    depending on the water contaminant under investigation.  The approaches  taken
    for each of three-major classes of water contaminants assessed in  determining
    TljlDLs are discussed below.                                           .
    
          Biochemical Oxygen pemand/Diffiftlved Oxygen
    
          Biochemical oxygen demand  (BOP)  is a measure of the amount of oxygen
    used in stabilizing a biodegradable material.  Both  carbonaceous organic
    compounds  (CBOD) and nitrogenous forms (NBOD), such  as ammonia and "g-nlc^
    nitroeen   are  subject to bio-oxidation.  In most WLA applications, the  amount
    of  oxyge;  consumed for biodegradation  over a  five-day period  (BOD5) is used  as
    the standard measurement.  However,  fuU oxidation of organic compounds
    generally  requires in excess  of  twenty to  thirty days for completion.   ,
    
          When an  organic waste  is loaded  into a  water body,  it is  subjected to
    two processes  that  influence the transport of the waste:   (1) advection  which
    represents the downstream transport of the waste, load in stream flow,  ««M2>Q
    dispersion, which encompasses the  turbulent and eddying;processes  that tend to
    mix the waste  load with upstream and downstream waters.  .Under  steady-state
    conditions (i.e.,  constant waste load and stream flow),  the. advection and    -
    dispersion processes can be assumed to be constant.   In many WLA. applications,
    one may assume steady-state" conditions because critical low-flow conditions
     are modeled (e.g.,  the 7-day,- 10-year low flow period).   However,  if
     conditions vary, the transport processes will also vary.
    
           The biochemical oxygen demand and the resulting dissolved oxygen levels
     in the water body are a function of the ability of naturally occurring^
     bacteria to decompose the organic waste materials,  thereby utilizing the  .
     oxygen resources of the water body.   Replenishment of the oxygen resources  in
     the water body occurs either through  transfer of atmospheric oxygen into the
     water column  or, to a lesser extent,  through oxygen production by aquatic
     •plants.     .'   v  ''-.'.      ..'                            .     •   '
    
          -The  interaction of  these  processes produces the reduction in dissolved.
     oxygen levels which is  the  focus of WIA modeling.  The critical factor an the  .
    • protection of water quality is  an  understanding of  the rate at which  _
     reaeration takes place  and  the  magnitude of  this rate in relation to the rate
     of oxvgen consumption.:  This relationship is generally expressed  in terms of   ,
     an oxygen deficit,  which is defined as the difference in concentration, between
      the  saturation value  and the actual dissolved oxygen concentration.
                                                                  Allocation.   Book
      2: Streams and Rivers. Chanter 1,;  Biochemical
      PB86-178936. September 1983. p.. 2-13.
    
           8  Ibid,, p. 2-19 ^
    
                     '.   • •      ..:  .'       39:
    

    -------
                     i ..... fJutrients__and
                      The major water body impact associated with nutrient loading is
                eutrophication, or  enrichment of the biological productivity of the water
                •body.  Waste  load allocations for control of eutrophication are generally
                designed to reduce  nutrient inputs.   This strategy presumes that the nutrient
                to be controlled  limits  the rate of growth and subsequent population of
                phytoplankton.  It  further presumes that reducing the population level of
                ^_ISikcon win  provide the desired control of the complex process of
                eutrophication and  eliminate undesirable water quality situations such as
                algal blooms.  Therefore,  it should be noted' that WLAs to control
                eutrophication in water  bodies focus directly on nutrient reductions and
                indirectly  on phytoplankton and dissolved oxygen conditions that result from
                overs timulat ion by  nutrients.9
    
                      Nutrient levels  in water bodies are controlled by external and internal
                sources.  External  sources of nutrients include municipal and industrial point
                sources; stream  inputs,  atmospheric deposition, urban. runoff , ground-water  .
                discharge ", .......... agricultural ........... drainage", ....... and" other nonpoint sources.  Internal
                sources  include  sediment release, biological recycling, and -nitrogen fixation.
                       Chemicals and Toxic Substances
     j*j,|i ji., ._
    " .....    ' '"
                   *iswi!^|Je'':"pr'0!c!edu1re for developing realistic mathematical models for chemical.
                    S'lts ........ similar "to the mass-balance approach used for other measures of water
    ............................................  MalityT such' ............. as" ......... biochemical oxygen demand.  The main ......... differences involve the  .
                 modeling of processes affecting the chemical constituent.  These processes
                 include chemical partitioning between the soluble phase and adsorption onto
                 particuiate matter, chemical transfers and kinetics involved in the decay or
                 volatilization of the constituent, and sedimentation processes.  In conducting
                 WLA for toxic substances, all of these procesises are accounted for in a mass
                 balance equation.  The result is a prediction of chemical concentrations in
                 the water column, sediment, and, in some cases, in the biota present in the
    ................................. : ............................. water body.              .                                    '
    
                       The fundamental transfer and kinetic characteristics are known for a
                 wide variety of chemicals based upon laboratory analyses.  These
                 characteristics can be combined with other relationships, such as advection
      i          and dispersion predictions, to account for the manner in which. any material is
                 transported in a water body.10     .
    111111  I 111 ll'I1 Pli    111	_	!	                                 •..'..'.:!.  :-' :,",'.''-
    	J	    9- Technical Guidance Manual for Performing Waste Load Allocations.	Book
                 4:  Lakes  and Impoundments' I   cHap'ter 2:  Nutrient/Eutrophication Impacts.   PBS 6-
                 178928, August 1983.  p.  1-4.  ,
    
      i    '            1°  Technical Guidance Manual  for Performing Waste Load Allocations. Book
                 4:  Lakes.ReservoirsandImpoundments.  Chapter 3:  Toxic Substances Impact.
                 EPA 440/4-87-002. .December 1986.  p. 6.                      •
    

    -------
         "ii.   Waste Load Allocation models:  Steady-state conditions
    
          General Approach
    
          Conservation of mass is the fundamental principle which is used as the
    basis of all mathematical WLA models of real world processes.  All material
    must be accounted for whether transported, transferred, or transformed.  A
    rate equation which conforms to the requirements of mass balance is
    
         'V-dc/dt'- J + *T+. *R + *W
    
    where                                       ;
          c -   concentration of the chemical                      .
          J[ -   transport through the system
          f -   transfers within the system
          R -   transformation reactions within the system      •  .
          W -   chemical inputs      .                  .              ,     .
          V -   volume of water body.
     ••    t -   time.           •, '
    
          This  fundamental model forms  the basis for assessing pollutant load  to  a
    .water.system.  Most WLA applications also  assume steady-state conditions,
     thereby'eliminating the need to measure  changes in parameters over  time.   The
     simplified  steady-state framework for chemical WLA modeling  also assumes
     complete mixing  throughout the water body.
                                             *             ••         .        •    " '   v
          A  steady-state model requires single, constant  inputs  for effluent  flow,.
     effluent concentration, background  receiving water concentration, receiving
     water flow,  and  meteorologic conditions.   As a result,  the effects  of
     variability in nonpoint source  and  point source contaminant  discharge on
     receiving water  quality cannot  be predicted accurately  using these  steady-
     state techniques.   Nonetheless,  steady-state models provide  a relatively
     simple  and  conservative tool  for estimating water quality impacts from
     contaminant discharges.   The  specific  analytical  approaches  for steady-state
     WLA modeling for BOD,"  nutrients,  and  toxic substances are described below.
    
           Biochemical Oxygen  Demand and Dissolved Oxygen  Profile
    
          A dissolved oxygen profile for  a stream  reach  is  based upon a simple
     mass balance which accounts  for the mass of BOD  entering a stream reach,  the
     .mass leaving the reach,  and the biodegradation and reaeration processes that
     occur within the reach that result in the oxygen sag.  At steady-state,  the
     following mass .balance applies:11              .'                   •      .
          11  Technical Guidance Manual for Performing Waste  Load Allocation.  - Book
     2: Streams and Rivers. Chapter 1:  Biochemical Oxygen Demand/Dissolved Oxygen.
     September 1983; PB86-178936, p. 2-40.
                                           91
    

    -------
    I III II 11  II
                      MASS IN - MASS  OUT + SOURCES  -  SINKS - 0
    
                      QC. Q:(c+  ac/dx-*x) -*• K.-«VC)-V -  K.J-L-V - o
    
                             • if U - Q/A and V  - A-*x, then:
    
                      Q-dC/dx-AX - (Q-*x)-dC/dx - (U-A-*x)-dC/dx - U-V-dC/dx,  and'
    
                       -U-dC/dx + Km- (C.-C)  -  Kd-L - 0
    
                             • if  the oxygen concentration  (C)  is-expressed in terms
    j!!!!!!!!"!!!,,!,"!!',  '"[  ,	•»!,',«„ M«'!  ,!",„",!, of  oxygen deficit (D) and  the  saturated oxygen
                               concentration  (Cs) ,  then C - Cs - D,  and
    
          "   ,          -U-d(C,-D)/dx + K.-D -  Kd-L - 0
    iiiill'ii if!!!1, iijji  i   11111,1 iii.i, i  n,11 , i	iiiiiii	 i,,in  ill	i	I ,,i	, ,,       •    '        •. : i':
                  	"        j "if1 c, is constant over all x,  then
    
                       U/ dD/dx •«• K«- D - Kd- L - 0
                              •  the rate  of change in biochemical oxygen demand
                                concentration (L) is expressed as:         •
    
    
                                    L  - Lo-e'-*
    
                              •  therefore ,
    
                        U- dD/dx + K.-D -  Kd-Lo-
    
                              • integrating and  solving the equation for the condition
                                thatTD-pp at x-0 yields the following:
    iiiiiiiiiiii i i iiiii  in iiiiiii  i   iiiiiii MI  iiiiiii  ii j i  {-jf«-'jc/U} ji v / (Y -K ^-Ln' f e ' ~"E' */"' - g(-K»-x/U)y
    
    Illliilif illlili l ii ill  i'1  ill 1 1 I 1 ....... In 1 1  ...... 1 I ill ii      I      i       ' .....           •               .';, '  :  •, •    ::  "
    iiiiiiiiiiii 1 I ii nil  iiiii  i  i iiiiiiii i i in i     IN iiiiiii        4          .  .            i             i       •      ',''.•'
                  where                    .    ,       '                               ......
    
                        Q -          river flow  rate                             ••
                        C -          concentration of dissolved oxygen entering the segment
                        Cj »         saturation  concentration of dissolved oxygen
    .................................. [[[ " [[[ i ....... OC -         mass of oxygen entering the segment -                 _
                        dC/dx -      rate of change of oxygen (C)  with distance (x) ;  equivalent
                                  '.  to rate of  change with time (t) when converted by velocity
                                                                              '
                                                                         -
    ............. ' ............................... ' ...... F ............. !" ...... « .......... -"'^< • ............... • ....... '; ...... ...... '^ae/aBe;"*"* ...... - ........... change  in oxygen concentration during time of passage
    [[[ .............................................. ........................................... through segment of  length »x
               f"f» 'iSi'^iV/iit jja _    •    atmospheric reaeration rate coefficient .
              .......... : " "'.:: ..... •":1"^  „        BOD" removal" rate ........ coefficient (-K,j) .
        liajwMf.^ii •'ws'iik'.i^j n    ' ' id ii  i1    i  i  i  111 •           L '           *    '       •-;.. v ".r  	=	
        	iE.!''v.ilj;|l!if;(This is a steady-state solution for the oxygen deficit in a stream
             - ""• "igmiftic	"of	teng'tt	''xV'"'	The source  term for biochemical oxygen demand (L)
          ::,,:r:,':,,;,,'^SSieF«nES	the concentration of  BOD within the mixing zone below  a P°^
    

    -------
    ground- water discharge.
    
          Nutrients
          In lakes and estuaries, nutrient inputs may promote  increased biological
    productivity or eutrophication.  Such eutrophication processes  depend upon
    continual input of nutrients, as a net sedimentation of nutrients  occurs over
    time   This process can be expressed in a general steady-state,  mass balance
    equation which, assumes a completely mixed water body.   The removal rate of the
    nutrients is assumed  to be proportional to  their water  concentration,  which is
    expressed as follows12:
                V-dP/dt - EQi-Pi - K.-.p-V - Qp                           ,
    
           • where               '                                       •
    
           EQ --Pi       -      the sum  of all the  mass  rates  of total nutrients
                             discharged to the lake  from all sources (point source
                             and nonpoirit source)  [M/T] ;  Qt  - flow [L3/T]; and Pi -
                             the initial nutrient  concentration [M/L3]
    
           p -          lake  nutrient  concentration [M/L3]     .   ;
    
           V -          lake  volume  [L3]
    
           K,-          the net sedimentation rate  of the nutrient [1/T]
    
           Q -  '  ' •   .  lake  outflow [L3/T]                           .  •            "
                          *                    '
           •  assuming steady- state (dp/dt - 0),  and letting W - EQt-Pi:
    
                 p - W/(Q.+ K.-V)
    
           •  if V - A- z {where A- lake surface area and z - mean depth) , then:
    
                 p - W/[A-zUQ/V) > K,)]
    
           This expression provides a simple estimate of the ambient, lake water
     nutrient concentration  given. a loading rate of W.  However,  the equation does
     not provide any indication of the water quality impacts resulting from  the
     nutrient loading.  Such an estimate  could be made based upon the  ambient
     nutrient concentration.     .
    
        •  . . toxic Substances               •                   ' .
    
           As mentioned above,  the modeling approach for toxic substances  is
     similar to  that used for  BOD and  dissolved oxygen depletion  WLAs.   One  of  the
     principal differences  between the  approaches arises in the modeling of  the
           12  .Technical Guidance Manual for Performing Waste'Load Allocations.....
      Book 4:  Lakes-and Impoundments.   Chapter 2:  Nutrient/Eutroohication Impacts,.
      PB86-178928.  August 1983.  p.3-18.
                                            93
    

    -------
                various  fate processes  and reaction rates  affecting organic and heavy metal
                toxic  constituents.   Several references  list reaction  rates for toxic
                constituents."   If a first-order decay rate estimate for a particular
                constituent is available,  the following  equation for estimating the  downstream
                concentration of the  contaminant may be  used:
                           ••o
    
                where
                       e - c0-e-K<*/u)
                       C -   downstream concentration
                       C0-   concentration at the mixing zone
                       X -   distance downstream of mixing zone,
                       u -   river velocity
                       K -   measured decay rate.
                 However  the  fate of many toxic .constituentscurrently is not.well  understood
                 because of  the  confounding effects of varying temperature, pH,  and  other
        BK|»;!.:^>^vir6nnentaI conditions in a water body.  .            '              •
        Bll, III!: «i;' aW-HltHM.™ yil; 41111 <(»;•;	i'*lll; *'-	i: i!;'." i	i":" n? - K 1>	SKS, «:StT'ii/i»;- X OBSaE»l vsiiii It*.::,,;l t" • • •;; ;•.'.' ;«i ,  /.••.,'..-  ,  .
        MIS jf Mini ,i>"!i!!,i ,:B „	 n 111 in i  ii ii  n i i i  ii i i minium inn i i i '"lii'i'ihiii'iiiJiiiEi'ii,:. JH^iiHiyiai!!!1''11,,,!',»I'si rfi'ii"»!" i1 SIWIMIIM^^^     	'.i i^^wiJi^iiN!11'11*1'J1'1"111""!' "• •	s	v •	»   - *•   •  •'  '     ''__-i
                       FPA*c TMDL euidance for modeling  individual  toxicants  in  streams and
    :iillllllll||P|||l|i|	nilKllllii'	lii'lllllh, 'I*If",!!!: , llllllllllllllllll  I II  II C*ITA. & AiUJl^ ^V*j.Vfc&i*wy. ^.**          CT                                  /O«l.«.««w*
    	i	!	I.	!i	'	' 'r: ,f:-,	i'OL'rs1" r'ecoiJends	tine" "following steady-state models:   Simplified  Lake/Stream'
                 Analysis (SLSA),  Michigan River,Model (MICHRIV),  Chemical Transport and
                iSalyses Program  (CTAP),~ Exposure Analysis Modeling System  (EXAMS), and Metals.
                 Exposure Analysis Modeling System (MEXAMS).  All  of these models  except MEXAMS
                 can simulate  both organic chemical and  heavy metal fate and  transport in
                          EPA  also recommends  these steady-state models for modeling individual
                	CBXicants	in	laKe's "and""reservoirs .
    
                        In addition to  steady-state models,  research has continued on the
                 development of dynamic or continuous simulation models.  These modeling
                 approaches are discussed,below.  EPA recommends the following continuous
                 simulation models for rivers, streams,  and .lakes:  Estuary and Stream Quality
                 Model (WASTCX) , Chemical Transport and Fate  Model (TOXI^^.L,^a™ei.   „
                 'Transport  Model (CHNTRN), Finite Element Transport Model  (FETRA) ,  Sediment
                 Contaminant Transport Model  (SERATRA),  Transient One-dimensional Degradation
                 dnd MigrationModel (TODAM), and Hydrologic  Simulation Program-Fortran  (HSPF).
                 All of thesecontinuousmodels are designed for multiple  reach, multiple
                 Source analyses of  both ofganics arid heavy metals.
    
                        Detailed descriptions  of these  steady-state and dynamic models  are
                 provided  in several of the EPA guidance documents cited  in Chapter III  of  this
                 document.
       ^   ''''P!!;1!!1!!!!1! ' , i/nl ', IIUi'linK 'h 	 	FI'"':^ "IK, JIM,!!!"'!!,!"1' i llllllllllllllllt i«i'	M"'!1 l!i"'i" nil'i"!	!!"i|i'	iri'l'iVkli'liI 1UIIPIIPI1 Pn^iiAr'iti'PJIPPi'il'l'IS'lPnnPP <"	liu	li'l'W	^>-	L^	 	•"' 	'' f""^/io n«J^«.4«>*«v 13/^1
                        13  For example,  see Wager Related Fate of 129 Priority Pol
    
          aa:';:. ;i; JKr^umas	f "an? 'Ii::	EPA-440/4-81-014.
               ''  iiiP1'' * i
               :11,, Illliiraii'' \M • ii',; i	litK!	('"• m Wl •. ilHIIIIlli;;	LWiWfrl ihiPS	K^afWfiJfiBI»l /-, i^^ftfflWnp^j \WM\. ^t'\ •. U;.iS i ito iVir,'i: •: "'''JK '::i'i; '''Si	t' : i' ••'' r "i;, -'! •.,.. i  '  •:' .'   :' "' L"  \. •  ' .".•."'',: f.  I' I': • - ' ,:,, \ M
    

    -------
          Hi.  Dynamic tfasteload Allocation Modeling      ...  •
    
          At the present time, most States and EPA Regions use steady-state
    models  which assume the wastewater is completely mixed with the receiving
    water and the c6ntaminant source loads are constant, to calculate WIAs for
    pollutants   This -assumption may be adequate for conventional pollutants
    because the greatest environmental impact in the receiving water, such as
    severe oxygen depletion, is found downstream of the pollutant outfall.
    However  for toxic pollutants the highest concentration in the  receiving water
    (i e   near the pollutant outfall) may serve as the critical level  for
    determining the waste  load for the contaminant.  As a result, dynamic modeling
    approaches are increasingly being applied to better account for variations  in
    point source loads and variations in  ambient water conditions resulting from
    changes in nonpoint  source loads and  other factors.
    
          Dynamic TMDL models calculate an entire probability distribution for
    receiving water  concentrations rather than a single worst case  based on
    critical  conditions.   The prediction  of  complete probability- distributions.
    allows  the risks inherent  in  alternative treatment strategies to be
    quantified.  The dynamic modeling  techniques have an  additional advantage  over
    steady-state modeling in that they  determine the entire  effluent concentration
    distribution required to produce  the  desired frequency.of criteria compliance.
    
           Continuous or dynamic  simulation models  use  each .day's effluent flow
     (Q ) and  concentration data (C.) with each day's receiving water flow. (Q.)  and
    background concentration (C8)  to calculate downstream receiving water
     concentrations.   The model predicts these concentrations in chronological
     order with the same time sequence as the input variables.  The  daily receiving
    'water concentrations can then be ranked from the lowest to the  highest, without
     regard to time sequence.  A probability, plot can be constructed from these
     ranked values, and the occurrence frequency of any one-day concentration of
     interest can be obtained.15
    
           Several methods are available  to compute the probability that downstream
     toxicants (or effluent  toxicity) will exceed criteria.  These, approaches
    'include an approximate method of moments and numerical integration.   The
     method of moments is  based on the -following equation:
    
                 ct - c.- [Q./(Q.-KJ.)] >.c,- [l-(Q./(Q.-*5.»]'
    
     where Ct - downstream concentration of the contaminant- at time .t.   Estimates
     of  the mean and variance of  the effluent concentration,  effluent flow, and
     upstream concentration-can be made by regressing the natural log of  each of
     these variables against a standard lognormal random variable.  More  specific
     information concerning  the variation in each of these terms may also be
     applied.
           15  Technical  Support Document for Water Quality-based Toxics Control.
      September 1985, EPA-440/4-85-032. p.  40.
           16   Ibid,  p.  41.
    
                                            95
    

    -------
           An additional dynamic modeling approach involves the use of Monte Carlo
     simulation.   MoileCarlo combines probabilistic and deterministic analyses
     since ic uses a fate and transport mathematical model with statistically
     described inputs.  While MonteCarlo simulations require more input data and
     calibrationdata than steady-state modeling approaches, they can account for
     interactions of time-varying water quality, flow, temperature, and point and
     nonpoint source lo'ading terms.
    
           The above discussion presents a brief overview of modeling approaches
     for WLAs.  More detailed descriptions of the approaches outlined above are
     available in the documents summarized in the annotated bibliography which
     accompanies this SSport:The following section discusses how information
     characterizing nonpoint contaminated ground-water discharge to surface water
     may be incorporated in the WLA process.
    
    
     C     Assessment of nonpoint source contaminated ground-water discharge to
           surface-water analysis methods as components of waste load allocation
    
           i.    UPS  loading in current TMDL models
           In steady-state TMDL models, all source terms, including NFS loads, are
     assumed to be constant.  Therefore, one may conclude that NFS loading is
     accounted for as a component of ambient water quality conditions.  However,
     because the application of steady-state models typically focuses only on point
     source loads, the contribution of nonpoint source inputs within the water body.
     segment of concern may not be adequately assessed.  Furthermore, if the WLA  is
     determined for  other than low flow conditions, the NFS load may vary greatly
     and a significant contaminant source  term may be overlooked.
    
           The need  for a more thorough understanding of the change in ambient
     water body conditions brought about by contaminated ground-water discharge
     increases for dynamic WLA modeling applications.  This understanding should
     Include  an assessment of the magnitude of NFS loading throughout the water
    i, body segment  of concern and the  spatial  and  temporal variations  in that  -
     loading.
    
           The accuracy of the waste  load allocation process  is highly dependent  on
     the quality  of  the data used for simulation  modeling.  This  data includes
      Information concerning the  ambient conditions  in  the water body, spatial and
      temporal variations in the  source loading terms,  and a detailed  understanding
      of the kinetics of contaminant fate  and transport.  WLA  models should.also be •
      calibrated and verified prior to allocating  waste loads.   Sufficient
      historical"data to accomplish these objectives  are  often lacking, however, or
      of the wrong type.  Therefore,  improved data collection is  often needed to
      better quantify ambient conditionsand anticipated loadings.
    
            In addition tocharacterizingambient conditions,  a firm understanding
      of the contaminant  source terms should be obtained.  .For systems that are not
            "  See Stream Sampling for Waste Load Allocation Models.   EPA/625/6-
      86/013.
                                             96
    IIIPIll 1 1111 11 111 111 1
    
    '
    liilill n n 'Hill
    U II II III III
    	 \mm 	 iiiiiiivi 	 iiiiiiiiH
    1 i I in i i i 1 1 i ° in ' 'i,-: • , .• , '"; .;.;.;::) ;
    , i, •;: ' • . v , ,,
    i'i 11,1 liilill 	 1(11 1 1 . 11 1|| lllllli | 1 |l 111 1 1 1 111 111 (1 ' 1 (111 i1 11(1 111 ill 111 111 1111 1 1 i| II 1 1 1 III li l|il 111 1 1 111 1 1 III „. ;•£,: , . .• 1,; f • ;, •• >':'- :'• ': ' ,j 'I,!" 	 ' ' „
    i.n', " ' ',' ' ' '''Jliilli
    !l«
    il1 ill ill ,'',!< « 'ni'l
    

    -------
    in low flow  (i e.. near steady-state)  conditions,  this  understanding  includes
    a quantitative measure of source constituent  and concentration levels over
    time   For point  sources, this  information is readily available through
    analyses  of  permit conditions or past  operating practices.   For nonpoint
    sources,;  however, the amount of information available to characterize the
    source terms accurately typically  is limited.
    
          A sampling  program  to support a  WLA assessment should, at a. minimum,
    Include the  following sampling  locations within the stream segment:  upspream
    boundary, point, source, upstream of point source,  mouth of any tributaries
    entering  the segment,.upstream  of  the  tributaries, upstream of any nonpoint
    sources?  downstream of nonpoint sources, and downstream boundary of segment
    In areas  where significant  nonpoint source loadings are known to exist, both
     the flow rate and constituent concentrations  should be  measured.  If this area
     is not so large that other  water  quality changes are likely ^occur during
     the travel time through the area,  it is reasonable to assume that the^changes
     in concentrations are due to the  nonpoint sources and to use these differences
     as a basis for. estimating the loads."  However, if the leveL of nonpoint  •
     source loading is significant,  a. more thorough characterization of the
     nonpoint source term may be needed.
    
         •  The following section reviews the applicability of the methods described
     in  2 above  to better characterize nonpoint  source loading  as part of  the TMDL
     assessment process.
    
    
           ii    Analysis of contaminated  ground-water discharge to  surface water
              '    assessment methods as  sources  of data for  waste load allocation
    
    
           As described  above,  there is no single analytical approach  to  waste load
     allocation.   The TMDL analysis and the type  and amount of data required for an
     assessment  will  differ depending  upon the water body characteristics,  the
     point and nonpoint  source  contaminant loads, and  the level  of water  quality
      impairment.  Furthermore,  in many situations there may-be no  need to
      characterize the component of  the ambient water contaminant concentrations
      contributed by nonpoint  source loads.- Such  a circumstance  may arise if the
      nonpoint source  load is  minimal and limited  controls on the point sources
      within the  watershed will  achieve the applicable  water .quality standard^  On
      the other hand,  if nonpoint. sources- contribute a large portion of the ambient
      contaminant concentrations in a water body and stringent  controls on point
      source discharges will not achieve the water quality standard  there may be  a
    .  strong  incentive to characterize  the contaminant load  provided by ground-water
      discharge to support development of a nonpoint source  management strategy
      This section discusses the applicability of the various contaminated ground-
      water discharge to surface water analysis methods for  supporting such nonpoint
      source  load assessments.
    
          '  All  of the methods  described in Chapter II will provide an estimate of
      .      18  sr-ream Sampling for W^e Loa'd Allocation' Applications ..  EPA-625/6-
      86-013.  p.  2-7.                            ,                            -
                                             97
    

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                                                                                    •f
                                                                                                       "*»w, 1
    lllllllllliii I'lli'lllii  'llIKi  i
        ^
    the loading of nonpoint source contaminants to a water body.   However, the
    methods differ significantly in  the  level of effort required,  the degree of
    specificity ofthecollected data, and the ability to accurately assess
    ceiporlland spatial variations  in nonpoint source loads.   As  a result,
    different methods may be suitable for different levels of  analysis.  For
    exampleinwa£*rbodies that are severely water quality-limited and that have
    high nonpoint source loads, the  ability to accurately predict  changes in
    contaminated ground-water discharge  may be critical to support dynamic load
    allocation£b"aiirhg:In contrast,  for water bodies that are not as severely
    water  quality-limited, a fundamental understanding of the  component of the
    water  contaminant concentration  contributed by ground-water discharge at base
    flow or  steady-state conditions  may be sufficient for determining  >:.,:e TMDL.
    
           The following table summarizes four attributes of  the contaminated
    ground-water discharge to surface-water analysis methods.   The
    characterizations are very  general  in nature and are intended to provide only
    a "first-cut" assessment ofthevariousattributes of  the  methods.  Because
    the categorizationof the methods necessarily combines  several different
    approaches under onegeneral method heading, a more detailed review of each
    method application is needed to  better assess the relevance of the approach  to
    aparticular situation." Nonetheless, this summary- allows  one to compare and
    contrast the suitability of the  methods for  specific  applications.
    
           The  attributes  are as follows:  (1)-.resources  needed to implement  the
    method-   (2) ability  to  assess spatial variations  in  ground-water discharge to
    "i	gcreii	••segment	Sr	VSESS	body;  (3)  ability  to measure changes in  ground-water
    -fisj^iarge  levels over  time; and (4)  the  level of  confidence in the method  s   -
    iribifityto provide  data that accurately  reflects  the "true" level  of
     contaminated  ground-water  discharge  to a  water body.   The attributes  for each
     of the methods  are  ranked relative  to one another.   A more detailed analysis
           acific	method" Applications	would be  needed to  provide absolute measures
        	th'e	actr'lb'ute's	for each method.
                            Seepage Meter/
                            Mini-pjezometer
                             Hydrograph
                            • Separation
                                           Total Flux
                                           Measurement
                       Numerical
                       Models
                       Loading'
                      . Functioni
                                                      Geophysical
                                                      Methods
    Isotopic
    Metho
    ill iiiiiii
    lllllllllliii li
    .....
      •
                  Temporal
                  Change*;
      Data
      Specificity:
                            moderate
                                         low
                 Spatial
                 Variation:     pottfbjy. with     no
                 	multiple sample
                            points
                             yes
                                                   moderate
                                       no
                                       yes
                                                     high
    
    
                                                     yes
    
    
    
    
                                                     yes-
    samples
    
    
    high
                                                                      low
                                                          yes
                                                          no
                                                                   high
                                                                   yes
    moderate
    moderate
      ;IUI!I .,', 'I	I' .
                       moderate to  low
                                                    high
    
    
                                                  •  yes
                                          moderate.
                                          high
                        This analysis indicates thatno onemethod may be suitable for all
                  applications.   Nonetheless, one or more  of  the methods can provide
                  sufficient data to support load allocations formanyapplications and
                                                          98
    

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    environmental'settings.                               '      .
    
    D.    Summary
    
          The preceding discussions outlined"several methods that have, been
    applied in a varie.ty of environmental settings to assess nonpoint source.
    contaminated ground-water discharge to surface water.  Each of the methods
    is'suitable for different applications and settings and the resources
    required to implement each of the methods also differ.  An enhanced
    understanding of nonpoint source contaminated ground-water.loadings.to
    surface water may also improve the total maximum daily load assessment
    process in water quality-limited water bodies.  These methods can support
    point and nonpoint source load allocations by better characterizing the
    component of ambient water quality contamination contributed by nonpoint
    sources under steady-state conditions and by improving the ability to
    characterize and predict changes in-contaminated ground-water loading in
    dynamic simulation models.  The manner in which several of the methods
    described above can .be applied to better account for nonpoint source
    loading to a stream is the focus of a companiqn volume to this' document.
                                         •99
    

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