&3WFR 83
Monday
Aprif 4, 1183
Hazardous Waste
Proposed Rule
               Agency.
Management System;

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  14514
federal Register / Vol. 48, No. 65 / Monday, April 4,1983 / Proposed Rules
  ENVIRONMENTAL PROTECTION
  AGENCY

  40 CFR Parts 261, 264, 265, and 775

  ISWH-FRL 2315-5]

  Hazardous Waste Management
  System: Identification and Listing of
  Hazardous Waste; Standards for
  Owners and Operators of Hazardous
  Waste Treatment, Storage, and
  Disposal Facilities; Interim Status
  Standards for Owners and Operators
  of Hazardous Waste Treatment,
  Storage, and Disposal Facilities;  and
  Storage and Disposal of Waste
  Material: Prohibition of Disposal  of
  Tetrachlorodibenzo-p-Dioxin

  AGENCY: Environmental Protection
  Agency.
  ACTION: Proposed rule and request for
  comments.

  SUMMARY: The Environmental Protection
  Agency (EPA) is today proposing to
  amend the regulations for hazardous
  waste management under the Resource
  Conservation and Recovery Act
  (RCRA), by listing additional hazardous
 wastes containing certain chlorinated
 dioxins, -dibenzofurans, and -phenols,
 and by specifying certain management
 standards for these wastes. These
 wastes are being listed as acutely
 hazardous. EPA is also proposing to
 delete several commercial chemical
 products from the list of hazardous
 wastes since these listings are
 duplicated in today's proposal. In
 addition, EPA is proposing to list these
 material!! as solid wastes when they are
 recycled by being used or reused, so that
 these wastes remain subject to
 regulation when recycled in this manner.
 EPA also is proposing to revoke its
 regulation concerning the disposal  of
 2,3,7,8-letrachlorodibenzo-p-dioxin
 (TCDD)-contaminated wastes under the
 Toxic Substances Control Act (TSCA),
 when  this regulation under RCRA
 becomes effective. This action extends
 regulatory control to certain hazardous
 wastes not covered by the existing
 regulation. It requires handlers of such
 wastes to comply with the appropriate
 regulatory standards.
 DATE: EPA will accept public comment
 on this amendment until June 3,1983.
ADDRESSES: Comments should be sent
 to the Docket Clerk, Office of Solid
Waste (WH-562), U.S. Environmental
Protection Agency, 401M Street S.W.,
Washington, B.C. 20460.
Communications should identify the
regulatory docket numbers "Section
3001/Dioxin" or "OPTS 62007".
                       . Pursuant to provisions of RCRA and
                      TSCA, requests for a hearing should be
                      addressed to Eileen Claussen, Director,
                      Office of Management, Information, and
                      Analysis, Office of Solid Waste (WH-
                      562),.U.S. Environmental Protection
                      Agency, 401M Street, S.W., -
                      Washington, D.C. 20460.
                       Public Docket: The public docket for
                      40 CFR Parts 261, 264, and 265 is located
                      in Room S-269C, U.S. Environmental
                      Protection Agency, 401M Street, S.W.,
                      Washington, D.C. 20460, and is available
                      for viewing from 9:00 a.m. to 4:00 p.m.,
                      Monday through Friday, excluding
                      holidays.
                       .The public docket for 40 CFR Part 775
                      is located in Room E-107 at the same
                      address, and is available for viewing
                      during the same hours.

                      FOR FURTHER INFORMATION CONTACT:
                      RCRA Hotline, toll free at (800) 424-9346
                      or at (202) 382-3000 or Judy Bellin (202) ,
                      382-4770.

                      SUPPLEMENTARY INFORMATION:

                     Outline
                     I. Background
                     II. Summary of the Proposed Listing
                     III. Basis for Listing
                       A.-Toxicity of Contaminants of Concern
                       B. Contaminant Concentration Levels in
                         These Wastes
                       C. The Wastes' Potential to Cause
                         Substantial Harm if Mismanged
                       D. Listing as Acutely Hazardous Wastes
                     IV. Removal of Certain Commercial Chemical
                        Products Listed in 40 CFR 261.33[f)
                     V. Regulatory Status of These Materials
                        When Recycled by Being Used or Reused
                     VI. Relation of Today's Proposal to
                        Regulation of TCCD—Contaminated
                        Wastes Under the Toxic 'Substances
                        Control Act
                     VII. Proposed  Management of These Wastes
                       A. Management at RCRA Interim Status
                        Facilities
                       B. Management at Fully Permitted Facilities
                       C. Other Management Options Considered
                        For These Wastes
                     Vin. Analytical Method for tetra-, penta-,  and
                        hexachlorodibenzo-p-idoxins and -
                        dibenzofurans
                     IX. Questions for comment
                     X. Economic, Environmental, and Regulatory
                        Impacts          •       :
                      A. Regulatory Impact Analysis
                      B. Regulatory Flexibility Act
                      C. Paper Reduction Act of 1980 ,  ,
                     XI. Rulemaking Record         ••£*»•'
                     XII. List of Subjects        >

                     I. Background                    "

                       On May 19,1980, as part of the final
                     and interim final regulations         -  .
                     implementing Section 3001 of RCRA,
                     EPA published a list of hazardous
                    wastes that included hazardous wastes
                    generated from non-specific sources.
                     (See 40 CFR 261.31.) This list has been
                    amended several times. In today's '
  action, EPA is proposing to amend this
  section to add particular wastes
  containing certain contaminants that
  are, for certain animal species, among
  the most toxic known; these wastes  '
  consequently are of particular
  environmental concern, EPA has
  evaluated these wastes  against the
,  criteria for listing acutely hazardous and
  hazardous wastes (40 CFR 261.11 (a) (2)
  and (a) (3)), and has determined that
.. they: (1) Are capable of causing or
  significantly contributing to an increase
  in serious irreversible or incapacitating
  reversible, illness, and (20) also pose a
  substantial present or potential 'threat tr
  human health or the environment when
  improperly treated, stored, transported,
  disposed of, or otherwise managed, and
  therefore are acutely hazardous wastes.'

  II. Summary of the Proposed Listing 2

   This proposed regulation covers
  principally wastes from the production
  of certain chlbrophenols and of
  chlorophenoxy pesticides, as well as
  discarded unused formulations
  containing tri-, tetra-, or
, pentachloropheriol and their derivatives.
 Specifically, this proposed regulation
 designates as hazardous certain wastes
 (including reactor residues, still bottoms,
 brines, spent filter aids, spent carbon
 from product purification, and sludges
 from wastewater treatment, but not
 including  untre.ated wastewater or spent
 carbon from hydrogen chloride
 purification) resulting from the following
 processes:3' *  •
   1 The RCRA definition of acutely hazardous waste
 is set forth at 40 CFR 261.11(a)(2). Under'that
 definition, such a material is not necessarily
 "acutely toxic" in the way that term is used by
 toxicologists. Rather, the term is intended by EPA to
 identify wastes which are'so hazardous that they
 inay, either through acute or chronic exposure,"
 "cause, or significantly contribute to an increase in
 serious irreversible, or incapacitating reversible,
 illness",.regardless of how they are managed.
   2The following acronyms and definitions are used
 in this document (and in the background document
 for this regulation):
  PCDDs = all isomers of all chlorinated dibenzo-jp-
 dioxins.                       >
  PCDFs=allisbmersofall chlorinated dibenzo-
 furans
  CDDs and CDFs=all isomers o£the tetra-, penta-,
 and hexachlorodibenzo-p-dioxins and -
 dibenzofurans, repectively.
  TCDDs and TCDFs = alI isomers of the
 tetrachlorodibenzo-p-dioxins and -dibenzofurans,
 respectively.
  TCDD and TCDF=the respective 2,3,7,8-isomers-,
  The prefixes D, Tr, T, Pe, and Hx denote the di-,
 tri-, tetra, penta-, and  hexachloro-congeners,
 respectively.
  3 Not all of these wastes are generated by every
 process discussed in the text.
  4 We are not proposing to list untreated
 wastewaters or spent  carbon from hydrogen
 chloride purification because these wastes are not
 expected to contain CDDs or CDFs at levels of
 concern. "                     ' '       '

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                   Federal Register / Vol. 48. No. 65  / Monday,. April 4;  1983 /  Proposed Rules            14515
  (a) The production and. manufacturing
use 5oftri-, tetra-, or pentachlorophenol
and intermediates used to produce their
derivatives;017       '
  (b) The manufacturing use of tetra.-,
penta-s or hexachlorbbenzenes under
alkaline conditions;
  (c)  the production of materials, onu
equipmentpreviously used for the
production or manufacturing use of  '
materials liatedJunder (a) and (bj above;
and        -.  '••
  (d) discarded unused formulations,
containing tri-,tetra-,r or .
pentachlorophenols, or discarded
unused formulations, containing
compounds, derived from,these
chlorophenols.8                 -    .
  5 In the context of this listing, "manufacturing
use" means the use of the named chemical as a
reactant or chemical interme,diate (for instance; as.
in the usecof 2,4,5,-tfichlorophenol (2,4,5,-TCB}:as a
feedstock for theisynthesis of 2,4,5,-T),,or as a*
component in a formulating process (as, for
instance; in the formulation of a mixture^of-2,4,5,-
TCP and,l,2,4,5,-TeGP, irt which these components
retain their chemical identity). In the present
context,,the term "manufacturing use" does,nat
include residues from, the use ofchlorophenoxy
pesticide formulationsi.e.g., in wood preservation.
  °The principal manufacturing use of
chlorophenols is: in. the synthesis of chlorophenoxy
acids, esters, and amines. They are. also'used in the
synthesis o£ phenolic resins, and of dye and pigment
intermediates. However, only wastes from
chlorophenoxy'synthesis are listed as hazardous  . -
wastes, because the Agency has no data on the  •
conditions of synthesis, generation of wastes, and
the leyelof chlorinated dihenza-p-dioxin or -
dibenzofuran contamination of wastes from the
synthesis of phenolic resins, dyes, and pigments:
The Agency solicits1 data on the extent of CDD/CDF!
contamination of the latter wastes; We also;are?
presently initiating sampling of some of these
wastes in the course of'our ongoing Industry Studies
program.
  'The 2,4,5;7TCP derivative Hexachlorophene:is
now synthesized from a purified 2,'4,5,-TCP in an
acid-catalyzed condensation reaction. Because the
reaction occurs at rather low temr)eratures,.and at
acidpH, no CDD or CDF formation.is expected to
occur.-Earlietproduction techniques resulted_in
TCDD contamination. Wastes.resulting-from
Hexachlorophene production therefore are not
included in this listing unless prepurified 2,4',5; TCP
was not used, or the process took place on
equipment contaminated with.CDDs or CDFs,
  aThis category .of listed wastes:includes   , *
discarded pesticides and formulations, containing
tri-, tetrar, or pentachlorophenol as ingredients.
Some of these materials, namely EPA Hazardous,
Wastes U212, 230,231, 242, and the chlorophenoxy
pesticides U232 and U233 already are hazardous
wastes under-40 CFR 261.33(f) when discarded'in
commercial grade, technical grade, oroff—
specification form, or wh'en present as the sole
active ingredient ura»formulation. However,
discarded'formulations containing these
chlorophenols or chlorophenoxy compounds as one
of a numberof ingredients (for example, hi a
mixture of 2,4;54-T, and.2,4;-D)"are not presently
consideredito be hazardous wastes (unless;they
exhibit a^characteristic ofhazardouawaste).These
multi-ingredient formulations nevertheless are likely
to-be,just as toxic an sole active'ingredfent mixtures,
since the concentration of toxic ingredients,isrthe1
same or higher. Today's action thus would remedy
this gap in regulatory coverage by listing the multi-'
ingredient formulations containing the discarded
III. Basis for Listing
       .   -    •   .                * -     -. ~
A. Toxicity of: contaminants of concern
  1. Toxicity of chlorinated dioxins. and
-dibenzofurans, The contaminants of;
concern in these wastes ana CDDs and
CDFS, tri-, tetra-, and
pentachlorophenols, and the
chlorophenoxy derivatives of these
chlorophenols. CDDs and CDFs are,,for
certain animal species.'among the most
potent toxic substances known. 9T,CDD
and two HxCDD isomers are' among the
most potent animal carcinogens tested.
Since each of these, substances are
carcinogenic in well-conducted tests hi ,
both rats and mice, they are also
considered by the Agency to be   .
potential human- carcinogena (see 4tFR
39858-39879 (Juiy-6,1979)).,Ittlaboratory
studies, TCDD haa-also been shown to
be tera'togenic; fetotoxic; and
embryotoxic at extremely low doses
(ng/kg/dayJ.'Based on structure-activity
relationships; TCDF also may have
reproductive effects at'extremely low •
doses. Many CDDs and7 CDFs are acute
toxicants as tested inJaboratory
animals at the ftg/kg/day dose rate,
and, even at these  very low
concentrations, have-many observable,
physiologic effectsi Although" an EPA
Scientific Advisory':Panel determined 1
ng/kg body weight to be "for-all
practical purposes" a no. observed, effect
level in rodents (44, FR 72337  (December
13, JL979)),. several other scientists have
Concluded that ariNOEL has not been
conclusively demonstrated-Mpreoveu,
the Scientific Advisory Panel concluded
that a NOEE had not been demonstrated
for primates. In addition, the  U.S. Food
and Drug Administration has
established a guideline suggesting,
limitation of human consumption of fish
containing TCD0 concentrations greater
than 25-50 ng/kg (ppt). Furthermore^ in .
severalenforcement actions and in two
site-specific risk assessments conducted-
by the Agency regarding Tunes Beach
and Imperial hi Missouri, environmental
concentrations in the ppt to ppb range1
were determined to be levels of concern,
and were used to define clean-up levels.
  The Agency emphasizes that,  for
purposes of this regulation.jt considers
all CDDs arid CDFs as toxicants of
concern hi these  wastes. Many
biochemical, and toxicology studies have
listed compounds. In addition, we are amendihg.the
basis for^h'sting these commercial chemical products
to include certain chlorinated dioxins and -
dibenzofurans as toxicants of concern.
  'The statements on toxicity, persistence, and
environmental contamination outlined in this
preamble are more fully, explained and
substantiated in the background document for this  ,
listing which is available for review in the public
docket.
 demonstrated that there; areFwell-
 defuied structure/activity correlations
 defining;the acute and chronic-toxic
 effects: of PCPDs and PCDFs. Those
 isomers that have halogens in at least
 three of the fqur lateral ring positions
 (numbers 2,3,7, or 8), and  that have at
 least one ring hydrogen atom, are the
 most toxic isamers. All the CDDs and
 CDEs substituted irr this manner have
 extremely higji acute, toxicity, bind
 strongly to  a eytosolic. protein receptor,
 and are potent inducers.of sey.eral liver.
 enzymes. The;Agency recognizes that,
 everLwithui such congenericrgroupnigs,
 there are. differences in toxicity; There
 is, for instance, a 370-fold difference  hi
 acute.! toxicity between, the I,2i3,7,8<~and
 me l,2,4,7,8-P.(iCDD iscaners;: however,
 even the. less 1;oxic:isomer has extremely
 high acute toxicity (oral LD50 in the
 guinea pig=l.l mg/kg).
  Only limited toxicity information is
 available on certain of the CDD and1
 CDF isomers. However,, many are  •-
 structurally similar^tootheECDD:and
 CDF isomers-.that are^potent toxicants.
 The- Agency maypermissibly- infer that
 certain waste constituent's are-toxic;
 based upon structural similaritjrto:
 known toxicants. -See EDFv. EPA, 598 F;
 2d 62^, 7&-S3 (D.C. Cir. 1978)" (prohibition
 of discharge* to navigable;waters ofless
 chlorinated:PGBs is permissible: hi;the
 absence of specific toxicolbgic data due
 to their structural similarityto7the: more
 chlorinated PCBs)V
  Consequently, because  most of the
•isomers of the listed GDDs and GDFs
 are toxic; albeit to different degrees,, .
 because Identification of ^individual
 isomers-in the waste would be an
 excessive-regulatory burden, and
 becausethe Agencybelieves thafrthese
 wastes would'contain a certaui
 percentage of the more toxic component,
 the Agency ha!s determhied that it is  a
 cohservative-public-health assumption
 that all the  isamers- of TCDD' should be
 considered in estunating its toxicity.  We
 have therefore!, determhied that all' the
 CDDs and CDFs identified or proposed
 to be identified in,Appendix VIII should
 be considered, as toxicants of concern, in
 these wastes. This decision is analogous
 to the finding adopted by the Agency in
 the case- of muinicipal waste resource
 recovery facilities.10
  2. Toxicity opchlorophBnois-and their
 chlorophenox'jrderivatives.  The other
 toxicants of concern hi these wastes
 also havepserious adverse effects. EPA's
 Carcinogen Assessment Gro.up has-   .
  10 See Interim evaluation of the health risks
associated with emissions of tetracBlorinated
dioxins from municipal waste resource recovery.
facilities. U.S. EPA, Office.of the Administrator, ,
November 16,1981L.      .

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 14516
Federal  Register / Vol. 48, No.  65 / Monday, April 4, 1983  / Proposed Rules
 determined that 2,4,6-TCP is a potential
 human carcinogen."In addition,
 ehlorophcnols may cause liver and
 kidney damage. Some chlorophenoxy
 compounds are also known or potential
 human carcinogens, and may have
 reproductive and teratogenic effects. •
 Water Quality Criteria have been
 established for many of these
 compounds. For example, for 2,4,6-TCP,
 the criterion for the protection of people
 from excess risk of developing cancer
 (10'8risk level) from the lifetime
 consumption of contaminated fish and'
 water is 12 ppb. The criterion for 2^,5-
 TCP (based on its chronic systemic toxic
 effects) is 2.6 ppm.
   For several other chlorophenols, the
 organoleptic water quality criteria are at
 the ppb level (see 45 FR 79318 November
 28,1980).
 B, Contaminant concentration levels in
 tliese wastes
   The toxicants of concern are likely to^
 be present in the listed wastes at
 concentrations many orders of
 magnitude greater than the levels which,
 as cited above, are of concern in terms
 or human health. In some cases, the
 Agency has inferred the presence of
 these contaminants from knowledge of
 reaction chemistry and process
 operating conditions. In other cases, the
 contamination of chemical,
 intermediates and commercial chemical
 products is analytically established. For
 example, analysis of distillation bottoms
 from manufacturing processes making or
 using trichlorophenols can contain
 several hundred ppm CDDs, filter aids
 may contain up to 6000 ppm TCDDs, and
 cooling pond muds were shown to
 contain as much as 1200 ppm CDDs. Still
 bottoms from 2,4,5-TCP and 2,4,5-T
 production generated by the Vertac
 Chemical Corporation contained up to
 111 ppm TCDDs. (U.S v. Vertac
 Chemical Corp., 489 F. Supp. 870, 879 (D.
 Ark. 1980)) (improper storage and
 disposal of dioxin-containing wastes
 results in imminent and substantial
 cndangerment warranting injunctive
 relief).
   Some process wastes may be
 contaminated with CDDs or CDFs
 because they were generated in the
 course of a manufacturing process
 performed on equipment that was
.previously used for a  CDD or CDF-
 goncrnting process. In the manufacture
 of chemicals on a production tram.
 previously used for a process generating,
 e,g., CDDs, both the product and the
 wastes generated can be contaminated
 with CDDs. This was  shown to be the
                      case, for instance, for wastes resulting
                      from the manufacture of 2,4-D. These
                      wastes contained TCDDs at the ppb
                      level, presumably because the
                      equipment, used previously to produce
                      2,4,5-T, remained contaminated with
                      TCDD after production shifted to 2,4-D'
                      (45 FR 32677, May 19,1980).
                        The.contamination-of tri-, tetra-, and
                     , pentachlorophenols, and their phenoxy
                      derivatives with CDDs  (30-100 ppm) and
                      CDFs (50-140 ppm) also results in the
                      contamination of biocides and their
                      formulations.
                        The concentration of higher   .
                      chlorinated phenols and chlorophenoxy
                      derivatives in these wastes also is likely
                      to be considerable. In the case of wastes
                      from cholorophenol production,
                      cholorophenols (because of their
                      solubility characteristics) are likely to
                      be present in reactor residues, in still- .
                      bottoms, and in the sludges from
                      wastewater treatment. Wastes from the
                      manufacturing use of these compounds
                      likewise will  contain these
                      chlorophenols—since they are the
                      principal raw material in the process^—
                      as well as various chlorophenoxy
                      derivatives. Because of the nature of the
                      purification and precipitation processes,
                      the latter compounds will occur
                      principally in reactor residues, on
                      adsorbents used for product purification,
                      and on filter aids. These compounds are
                      known to be present in'the wastes from
                      these processes. For example, a study of
                      the aqueous waste of one herbicide
                      manufacturing facility found that it
                      contained 13.5 kg/day of mixed
                      chlorophenols, and about 32.7 kg/day of
                      phenoxy acid. These are discharged in
                      fairly concentrated form: a typical  ,
                      untreated aqueous waste stream from
                      phenpxy acid manufacture contains 112
                      ppm of mixed chlorophenols and 235
                      ppm of chlorophenoxy acids.
                        Discarded pesticides  and pesticide
                      formulations containing these
                      chlorophenols as active ingredients
                      obviously will contain these toxicants in
                      high (percent) concentrations.-

                      C. The wastes'potential to cause
                      substantial harm if mismanaged

                        Not only are the contaminants of
                      concern present in significant
                      concentrations, but they are capable of
                      migrating from waste matrices and
                      reaching environmental receptors in
                      potentally dangerous concentrations.
                      These contaminants are persistent12—
  " U.S. EPA, Ambient water quality criteria for
cblorophcnols. EPA 440/5-80-032.
                        "CDDs (and presumably CDFs] are highly
                      resistant to microbial degradation. The Agency thus
                      believes that these toxicants will be present in
                      wastewater treatment sludges. The listed
                      chlorophenols and their chlorophenoxy derivatives
                      are biodegradable, but where overloading and
 CCDs and CDFs extremely so—and
 several can accumulate in the food
 chain. The measured bioaccumulation
 factor (BCF) for TCDD is species
 dependent, and varies from 2,000 to
 48,000; structure/activity considerations
 make it reasonable to assume that the
 BCF for other CDDs and CDFs are
 within the same range. The calculated
 BCF for the chlorophenols ranges from
 290 for 2,4,5-TCP to 610 for 2,4,6-TCP
 (however, the measured, steady state
 BCF for PGP is only 13). Thus, if these
 toxicants migrate from these wastes,
 even in extremely low concentrations,
 they can accumulate in biological
 organisms at much higher levels,
 increasing the likelihood of substantial
 harm to human health and the
 environment.
  _ These toxicants, moreover, are mobile
 in the environment, particularly as a
 result of water run-off or wind
 dispersion of contaminated particles,
 and can migrate from these wastes if
 they are improperly managed. Although
 CDDs and CDFs are relatively water
 insoluble, and bind strongly to organic
 .soil constituents, improper land disposal
 could cause substantial harm to
 environmental receptors. Pollution of air
 and surface waters can occur, perhaps
, as a result of windblown dust, water
 run-off or erosion, or flooding of waste
 disposal sites. All of these scenarios
 have occurred. In the Vertac case cited
. earlier, improper storage and disposal of
 wastes from the manufacture of 2,4,5-
 TCP, 2,4-D,  and 2,4,5-T resulted in
 significant environmental
" contamination. Fish and other aquatic
 life  in a local stream accumulated TCDD
 at levels as high as 600 ppt. The court
 concluded:
  Dioxins * * * can and have been
 transported off the Vertac site on dust, by the
 action of landfill areas and equalization
 basin area, and when people and equipment
 move to and from the Vertao  site. Samples
 show that dibxin has been transported off the
 Vertac site into fish and sediment in [a local
 stream), and also into the Jacksonville
 sewage treatment plant. (489 F..Sjipp. at 879)

 TCDDs also h*ive been detected at
 levels of concern in the sediments of
 streams, public sewers, and home'sumps
 at other sites, including Love Canal.
 TCDD has been reported in fish and
 crayfish living in contaminated streams,
 in concentrations (600 ng/kg) up to
 fifteen times higher than that at which
 FDA advises that human consumption
 be limited. High ppt concentrations have
 been reported for. other CDDs and CDFs
 in fish. Because of their insolubility in
 inadequate treatment occur, and in the anaerobic
 environment.of sludge disposal, they may persist.

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                  Federal-Register /Vol.  48, No; 65  /-Monday, April  4, 1983 / Proposed Rules
                                                                         14517
 water, and,their strong binding to
 organic soil constituents, CDDs. and
 CDEs are not ordinarily expected to
 leach, to ground water if proper    '    ;
 precautions are, taken.' However, if these
 wastes are co-disposed'with solufailizing,
 solvents, or disposed in situations where,
 soil binding site are exhausted, ground
 water dontamination.could,result:
   Although: chlorophenolsr and
 .chlorophenoxy compounds are subject
 to environmental degradation,^including
 blodegradaiion by adapted. .-
 communities, environmental pollution
 from,these, constituents haa occurred
 where wastes from the production  and
 manfuacturing usaof cMorophenols
 were mismanaged. More than.twenty-
 five, years after, the improper disposal of
 chloraphenolic wastes. at.Lova Canal,
 tri-, tetrar, and pentachlorophenols were,
 identified in'soil, waters and atorm
 sewer sediments at concentrations,
 ranghig from 14s ppb (PGP kksump
 waten) to. 496 ppm (TCPain atorm.sewer
 sediment).       ,
   A further risk ta human healthumay ba
 posed by, improper incineration;of these
 wastes: Impropen incuieration, of
 chlorophenola- are'prediced to form
 CDDs and GDEs as products, of
 incomplete combustion,.13 posing'a
 further riskof.substaniiaLhaEm. Indeed,
 as discusseilatermthiapreambletthe.
 Agency is studying whether different
 criteria or management standards (e.g.,
 higher destructioiuand removal
 efficiency for the incineration^ of these
 wastes), are>appropriate- and practical.,
   D. Listing: as-acutely hazardous
 wastes.
 •  It is: clear front this: discussion, that.
 these wastes have; the potential: to: cause;
 substantial-harmi, if:mismanaged. The
 Agency is further, convinced that these
 are  acutely hazardous wastes?under4Q.
 CFR 261.H(a)(2),, sinca they contain
 contaminants which;, when:teated hx
 animals,t are among the mast toxic
 contaminants kno.wn,, and thus:, are,
 capable of causing,, or significantly -
 contributing to: serioua irreversible;, or
 incapacitating, reversible;, illness; ^This
 standard is taken; directly front Section
 1004(5) of RCRA,. and. is reservedfor
 wastes;partic.ularly likely to pass a
 substantiaL'risk to human health.;and the.
   13Shaub,.W,,M. and-W. Tsang, SBhysicaland
 chemical, pr.operties;of dioxinaan relation- ta their
 disposaLPraceedings 2nd. International Symposium
 onDioxins. Arlington, VA. October 1981.
   "By means.of a site-speoifictexoiusibn petition, a
 generator may beiablettb show, that a;was.le:daes •
 not contain CDDs and/or CDFs at levels sufficient,
 to sustain regulatory concern as. acutely hazardous:
. waste; Such levelstliowever; as well as the-
 presence of cKlprophenols; or. chlorophenoxy
 compounds; may, still render,such wastes
 hazardous.
environment (see; preamble to Part 261,,.-
45 FR 33106, May 19,1980).
  Additional rea'sqna for listing these.
waates as acutely hazardous ane, that
the wastes have^beeatimplicated' in a1
series of damage, incidents, among.them
the. incidents of Eove Canal and Times
Beach. The Agency also, has been
compelled to exert regulatory control
over many of these'wastes under the
Toxic Substances Control'Act in the
face of the unreasonable risk posed'by
ongoing and contemplated waste
management practices (see further
discussion in Part VI. below),
  .The practical consequences of such*a
listing are two-fold":. First, these;wastes
will be subject to the 1 kg/month, small
quantity generator limitation contained
in40CFK'261;5(e).15   •      -
  The Agency deems-1kg to be
equivalent, for all practical purposes; to
total control of the management of these
wastes since, they are,genera±edJn
amounts far. greater than 1 kg. The
Agency solicits comments on.the  .  :
appropriateness, of'this limitation,       f
however; Second,, the residues in empty.
containers,'that contain.these1 listed'
wastes are subject to control under
Subtitle C of RCRA, unless the container"
has been triple-rinsed using a solvent
capable o£cleaning the containeri.or,the
container has been otherwise, cleaned
by a method-thai has- been shown to
achieve equivaleirfTemoval. In addition,
as explained more fidlybelow, we are
proposing that;tfrese wastes be managpd;
only, at treatment,., storage; and disposal
facilities that"have been fullypermitted
under RCRA (except as. diacussed; in
Section Vn.). tt the-Agency's-judgment,
these wastes shoufd.be managed
pursuanttb the most stringent
appropriate standards that are: '
contained-in theRGRA hazardous-waate.
management regulations.           ;

IV. Remo.vaL of Certain Commercial
ChemicaLPEoductSiListediin 4D GFR,
261.33J;f)     ,
  As-discussedin. the1 previous section,
the Agency is proposing tcplist-as
acutely hazardous those^unused
discarded* formulations1 containing tri-,
tetra-, or pentachlorophenol and
discarded forotnulations containing as
  15 The Agency is proposing today ta amend this*
provision to apply hxalliaeutely/Kazardousiwastes,.-.'
notjustto.the, acutely, hazardous. wastes;listed,ini4D
CFR'2ai.33(ej: At the time §.261.5 waa written,, there
were no acutely-hazardous wastes-otherthan those
in § 261.33(e). Now. that we-are proposing:to.list
wastes in §261.31 aar'acutely, hazardous, weare:
proposing to,confornvthe.reference,to,acutely
hazardous waste in I 261.5. For theisame reason, we
are proposing to make the samer type":of conforming ,
change to § 261.!'(bJ^—the provision statingtwhen
containers, that hay Kheld:acutely: hazardous wastes'
are "empty." -...•'          •  ,   "
 ingredients: co;mpounds derivedrfrom.
 these Ghlorophenols.,Some of these
 materials akeady are hazardous wastes
 under 40 CFR ,261.33(f) when discarded
 or intended for discard;in commercial
 grade, technical grade> or off-
 specification form, or when the toxicant
 is present in formulations as the sole
. active uigredienL They were originally
 listed as toxic, (rather, than acutely
 hazardous) because the Agency djd not
 at that time consider, the presence of
 CDDs and GDFs. However, as?shown
 above,: these formulations will contain ,
 chlorinated dioxins and -dibenzofurans,
 because the chlorophenol or
 chlorophehoxy derivatives will
 themselves be contaminated with GDDs
 and CDFs. For thia reason, we. are now
 listmg them asVactutely hazardous: under'
 40 CFR:261.11(a)(2).
   Ta avoid lis;ting'the:samawaste?under
 two different'(andihconsistent)
 provisions, we are proposing to remove
 EPA Hazardous Wastes U212, U230,
. U231, U232, U233, and U242"from 40 CFR
 261.33(f). As a consequence; there
 should:be no confusion that these  •
 wastes will be subject to a small
 quantity generator exclusion of 1 kg/mo.

 V. Regulatory  Status of These Materials
 When Recycled by Being Used or
 Reused       }__ '        •              ;

  . Qn May 19, l9ao,,EPA promulgated- a
 definition, of, sijh'd, waste, which,, among
 other things, slates, which materials are
 solid wastes; when recycled.. In
 promulgating. 1niarule,:EPAJestafalished
 broad, jurisdiction over, recycled      -v
 materials. andLrecycling,pperations.,EPA
 ia today proposing.in a separate, notice'
 to revise thia rulato, state. that,certaih
 types- of activitiea involving secondary
 material use:a:adlreuse, do, not constitute
 solid waste,m
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 14S1»
Federal Register / Vol. 48, No.  65 / Monday, April 4, 1983  /  Proposed Rules
 They also contain significant levels of
 hazardous constituents—CDDs and
 CDFs—not ordinarily found in raw
 materials or analogous commercial
 products, nor would these toxicants
 contribute to the efficacy of the
 recycling practice. In addition, in light of
 their toxicity and their environmental
 persistence, these wastes could pose the
 same potential for causing substantial
 harm when used or reused as when
 disposed. Since use or reuse would be
 unregulated, the potential for harm in
 fact 5s probably greater.16
   Accordingly, we are proposing
 elsewhere in today's Federal Register to
 list these materials as solid wastes
 when they are used or reused. As a
 result, these wastes will remain subject
 to regulation when transported and
 stored under the Subtitle C regulations
 even when recycled by being used or
 reused as ingredients in new products,
 or by being used or reused directly as
 products.
 VI. Relation of Today's Proposal to
 Regulation of TCDD-Contaminated
 Wastes Under the Toxic Substances
 Control Act

   Many wastes containing TCDD are
 presently regulated under 40 CFR Part
 775, a regulation issued under Section 6
 of the Toxic Substances Control Act
 (TSCA)." This regulation, promulgated
 on May 19,1980 (45 FR 32676), prohibits
 the Vertac Chemical Company from
 disposing of certain wastes containing
 TCDD, and requires the company to
 store and monitor these wastes until a
 long-term management solution can be
 determined. The regulation also requires
 other persons intending to dispose of
 TCDD wastes (defined as those resulting
 from the production of 2,4,5-TCP or its
 pesticide derivatives, or substances
 produced on equipment that was
 previously used for the production of
 2,4,5-TCP or its pesticide  derivatives) to
 notify the Agency 60 days in advance of  •
 such disposal. The regulation does not
 apply, however, "to persons disposing of
 wastes containing TCDD  at facilities
 permitted for disposal of TCDD under
  '*Wo note, however, that when secondary
miiloriiili that are derived from commercial
pesticides (such as rinse waters from pesticide
containers) are put to use as pesticides, they are not
considered to bo RCRA solid wastes. The Agency
constderti this activity to constitute continued use of
the pesticide, and so not to Involve waste
management. Any such use, of course, would have
to comply with requirements for-use of the pesticide
Imposed under the Federal Insecticide, Fungicide,
nnd Kucic nlicidc Act.
  "The hazardous waste listings proposed today
are more inclusive than those  regulated under
TSCA, including for example,  wastes from the
production of certain letrachlorophcnols and
eftlorobcnzcnes.
                      Section 3005(c) of RCRA." (See 40 CFR
                      775.197.)
                        On January 5,1982, EPA issued an
                      Advance Notice of Proposed
                      Rulemaking (ANPRM) (47 FR 193),
                      anriouncing the Agency's intent to
                      review the TCDD disposal rule (40 CFR
                      775), and solicited comment to aid the
                      Agency in determining the most
                      appropriate long-term solution for
                      TCDD-contaminated wastes. Several
                      comments received on this ANPRM
                      stated that the regulation of treatment
                      and disposal of hazardous wastes
                      properly belongs under RCRA, and that
                      the Agency should avoid overlapping
                      and potentially contradictory
                      approaches to the same problem under
                      different regulatory authority, e.g., TSCA
                      and RCRA. Section 1006(b) of RCRA in
                     ' fact provides that, in implementing the
                      Act, EPA "Shall avoid duplication" with
                      other statutes administered by the
                      Agency. Section 9(b) of TSCA provides
                      that the Agency must utilize its authority
                      under the other environmental laws it
                      administers where these laws are
                      adequate to prote'ct against
                      unreasonable risk, and where  there is no
                      stong public interest in taking  action
                      under TSCA.
                        EPA agrees that RCRA provides the
                      appropriate long-term solution for
                      controlling the management of TCDD-
                      contaminated wastes. The disposal rule
                      under TSCA was only meant as a
                      temporary solution. See 45 FR 32682.
                      EPA, in fact, acknowledged the
                      advantages of using RCRA, by providing
                      that final permits issued under RCRA
                      for disposal of TCDD-contaminated '
                      wastes would supersede  the TSCA rule.
                      The rule proposed today  under RCRA
                      will provide the safeguards of a final
                      permit, and will, therefore, render the
                      TSCA rule unnecessary.
                      .  Accordingly, only the RCRA rule
                      becomes effective, EPA proposes to
                      revoke the TSCA rule that applies to
                      disposal of TCDD-contaminated wastes.
                      The basis for this revocation.js stated in
                      the following paragraphs.
                        EPA promulgated the TSCA rule
                      under Section 6(a) of that Act.  Section  ,
                      6(a) provides that EPA may prohibit or
                      otherwise regulate any manner or  >
                      method of disposal of chemical
                      substances or mixtures if the Agency
                      finds that there is a reasonable basis to
                      conclude that such activities present or
                      will present "an unreasonable  risk of
                      injury to health or the environment."
                      Determining unreasonable risk involves
                      an administrative judgment which is
                     reached by balancing "the probability
                      that harm will occur and the magnitude
                      and severity of that harm against the
                      effect of proposed regulatory action on
 the availability to society of the benefits
 of the substance or mixture, taking into
 account the availability of substitutes ,
 for the substance or mixture which do
 not require regulation, and other
 adverse effects which such proposed
 action may have on society." {TSCA
 Legislative History at 422).
   In the May 19,1980 regulation, EPA
 determined that removal for disposal of
 certain TCDD wastes at Vertac's
 Jacksonville, Arkansas site would
 present unreasonable risks. The Agency
 found that maintaining drummed wastes
 on-site, with monitoring, presented a
 relatively, known and correctable risk,
 while disposing of the wastes, as,
 proposed by Vertac, posed a
 substantially greater risk, particularly
 where a case-spe'cific assessment on the
 management of these wastesjiad not
 been performed. (See Preamble to Final
 Rule  at 45 FR 32680; Preamble to
 Proposed Rule at 45 FR 15595.) Similar
 considerations led EPA to determine
 that disposal of TCDD wastes by other
 persons without prior notification to
 EPA would present unreasonable risks. _
 The. minimal costs of notifying EPA sixty
 days  before disposal,  so that EPA could
 evaluate the management scheme
 proposed by the notifier, was
 determined to be outweighed by the
 risks  of harm that could occur from
 exposure to TCDD disposed of
 improperly.
   We now propose to regulate these
 wastes under RCRA. On May 19,1980,  •
 EPA believed that the then existing :
 RCRA regulations for treatment and
 disposal of hazardous waste were not
 appropriate for TCDD-contaminated
 waste because EPA had not yet
 developed  final permit standards for
 land disposal or incineration of
 hazardous  wastes. Thes,e final
 regulations are not effective, and
 provide a means of properly evaluating
 the various management alternatives for
 TCDD-contaminated wastes to ensure
 that these wastes are managed in a
manner that does not present an '
unreasonable risk. Thus, when the rules
proposed today under RCRA become
final,  it will no longer present an
unreasonable risk for these wastes to be
treated and disposed of in RCRA
facilities, and this will be the only legal
waste management option. Since
promulgation of these  RCRA regulations
will vitiate the unreasonable risk finding
under TSCA, we will at the same time
revoke the  TSCA May 19,1980
regulation.
  It should be noted that,by doing this,
we are eliminating the 60-day
notification requirement under TSCA for
waste disposed at facilities not

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                     *.        •-                    -           •  " ' .       '     •     "           ,  ' '    ,
                   Federal Register /  Vol. 48,  No. 65- '[ Monday,  April 4, 1983 /Proposed Rules
                                                                       14519
  permitted under Section 3005(c) of
  RCRA. However, when this rule
  becomes effective, it will be illegal to
  dispose of these wastes at facilities that
  have not been fully permitted,
-  Therefore, we believe the TSCA 60-day
  notification requirement is unnecessary;
  in addition, notification .under Section
  3010(b) will still be required and thus,
  the Agency will still be informed of who
  is handUng these types of wastes.
     We also believe that it will be less
  confusing for the regulated community,
  and more cost effective, both with
  respecfto compliance and regulatory
  enforcement, for waste'disposal to be
  regulated under RCRA alone, rather
  .than under both statutes! Moreover, the
  technical expertise needed to issue
  permits for these wastes is chiefly
  within the Agency's office administering
  RCRA. We consequently believe that
  the public interest warrants rescission of
  the TSCA rule once this RGRA
 , regulation becomes effective.

  VII. Proposed Management of These
  Wastes

  A. Management at RCRA Interim Status
  Facilities     "

    As noted, the TSCA rule presently
  does not allow these wastes to be
  disposed or treated at interim status
  facilities without prior approval,
  bebause management of such waste at
 • unscrutinized interim status facilities
  ordinarily presents an unreasonable risk
  (45 FR 32682). To avoid a decrease in
  regulatory coverage, and in light of the
  waste contaminants' high toxicity,
  persistence, and potential to
  bioaccumulate, we are proposing to
  amend the RCRA regulations, except as
  noted below, for landfills, waste piles,
  surface impoundments, land treatment
  facilities, and incinerators, to require
  that these wastes be managed only at
  fully permitted facilities. The reasons for
  the unreasonable risk finding still hold.
  Interim status incinerators need not
  perform at 99,99% destruction and
  removal efficiencies, or meet the other
  performance standards contained in
  Subpart O of Part 264. Interim status
  landfills, waste piles, surface
  impoundments, and land treatment
  facilities need not meet the monitoring
  requirements in Subpart F or many of
  the design and operating standards of
  Subparts K, L, M, and N of Part ,264 until
  they are permitted. In addition, we
  believe that any facility that manages
  these wastes should be evaluated
  individually by EPA before accepting
  them in order to ensure that the facility
 ,is designed and operated properly. The
  proposed regulation consequently
 prohibits interim status facilities from
 managing these wastes.
   We have proposed three exceptions to
 this prohibition. The first applies to
 surface impoundments in which
 wastewater treatment sludges .are
 generated. The Agency has the authority
 to prohibit interim status surface
 impoundments from leceiving these  .
 wastes. If we propose this action,
 however, .the facilities now generating
 the listed wastewater treatment sludges
 would probably have to close down
 until they obtain permits for their
• impoundments, or build alternative
 treatment facilities that can efficiently
 tr-eat these wastes. The Agency is not
 proposing this course of action; and
 notes that Section 3004  of RCRA [as
 amended by the Solid Waste Disposal
 Act Amendments of 1980) specifically
 allows the Administrator, in setting
 standards for hazardous waste
 management facilities, to distinguish    :
 between new and existing facilities.The
 legislative history indicates that      .'-
 Congress was concerned with the costs
 of.modifying existing wastewater
 treatment impoundments installed to
 meet Clean Water Act requirements
 (although the Agency has the authority
 to require  such modification where
 appropriate). See S. Rep. NO.  96-172,  '.
 96th Cong. 1st Sess., laf 3. We are
 drawing this distinction in today's
 proposal.  -.        .-'•'•
   Allowing these wastewater treatment
 sludges at hiterim status surface
 impoundments in which they are
 generated should be environmentally
. acceptable for the period until a permit
 is issued. These sludges are expected to
 contain lower concentrations of CDDs,
 CDFs, and chlorophenols than the other
 waste we  are listing. The CDDs and
 CDFs present also will be adsorbed to
 the organic matter present; 'in addition,
 we believe, that there  should be little
 chance that solubilizing solvents, -such,
 as benzene, toluene, xylene, or
 halogenated benzenes, will be present in
 significant cdncentrations (since these
 solvents have very limited water
 solubility). This situation therefore
 should not present a significant risk of
 leaching. Risk of wind dispersal, one of  .
 the principal exposure pathways for
 CDD and CDF-containing wastes which
 are stored in open piles  or disposed in
 landfills, is not present for these
 wastewater treatment sludges when
 they are in an impoundment.       "
  . We are not proposing to allow other
 interim status surface impoundments to
 manage these sludges, however, because
 other impoundments could contain
 CDD- or CDF-solubilizing residues from
 processes  not related to chlorophenol or
  chlorophenoxy manufacture. In addition,
  manufacturing operations will not be
  curtailed if these impoundments have, to .
•  obtain permits before receiving these
  wastes.    -  '  .  .  -   '',-•-
   For all of these reasons, therefore, we
  are proposing to allow the listed
  wastewater treatment sludges to be
  managed .at the interim status surface
  impoundments in which they are
  generated. However, we expect, as a
  first priority,  ;to evaluate the Part B
  permit applications* of those interim
  status surface! impoundments that
  manage these wastes, in order to
  minimize any potential risk. In addition,
  if monitoring data, or a review of site
  management make it apparent that the
  wastes cannot be prevented from
  migrating, the. owner'or operator of the
  facility will be required to remove the
  waste from the surface impoundment.
   The second exception is for interim "'
  status tank arid container facilities,  '
-  which will be allowed to accept these
" wastes. These facilities, although not
  providing maximum protection, do
  provide control of these wastes to
  prevent them from posing a substantial
  environmental hazard or an
  unreasonable risk since tanks or
  containers at interim status facilities,
  must meet most of the requirements
  (e.g., storage  in non-leaking units,
  periodic inspections) required for fully
  permitted tank and container facilities.
  Therefore, theise facilities should
  provide adequate management of these
  wastes in the short term. However, we
  do expect to give highest priority to
  examining thei Part B'permit applications
  of those interim status tank and
  container storage' facilities that store
  these wastes, in order to minimize any
  potential risk.
   The final exception is for  enclosed
  waste piles. An "enclosed waste pile" is
  defined in this proposed rule as a pile
  that meets the: requirements of
  § 264.250(c)—namely, that the pile is
  inside a structure that provides
  protection from run-on, precipitation,
  and wind dispersal; does not generate
  leachate, and does-not contain free
  liquids. Under existing regulations, •
  waste piles meeting these requirements
  are exempt from the otherwise-
  applicable permitting provisions of
  Subpart L of Part 264 relating to ' •.
  containment.  (See 46 FR 55112,
  November 6,1981.)
   We are proposing that enclosed waste
  piles be allowed to accept these wastes
'  without first obtaining a permit because
  enclosure of t]ais type will guard in the
  short-term against ihe means of
  exposure of concern—run-off,jwind
  dispers'al, and leaching. In addition,

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 14520
Federal Register / Vol. 48, No. 65 / Monday, April 4,  1983 / Proposed Rules
 allowing this type of interim status
 facility to accept these wastes should
 help provide management capacity until
 disposal facilities receive permits to
 manage these wastes.
   We are proposing that interim status
 enclosed waste piles accepting these
 wastes still must meet the remaining
 applicable requirements of Subpart L of
 Part 265: waste analysis, special
 requirements for ignitable, reactive, or
 incompatible wastes, and closure
 requirements. (Post-closure
 requirements would not be applicable
 because we are assuming that these
 wastes will be removed from these
 piles.) We note, in addition, that to be
 eligible for interim status, the facility
 must have been fa existence on
 November 19,1980, submitted a Part A
 permit application, and (if required)
 submitted a notification of hazardous
 waste activity. (See § 122.23(a) and 45
 FR 76836, November 19,1980.) Enclosed
 piles added at interim status facilities
 after November 19,1980, or accepting
 these wastes after that date, may be
 eligible for interim status provided they
 meet the requirements for adding waste,
 increasing design capacity, and
 (possibly) adding a new management
 process. (See § 122.23(c) (1), (2), and (3)
 (permissible changes during interim
 status)).
 B. Management at Fully Permitted
 RCRA Facilities
  1, Management at fully permitted
 landfills, waste piles, surface
 impoundments, lagoons, and land
 treatment facilities. Except as described
 in the previous sections, the storage,
 treatment, and disposal of these wastes
 will be allowed only at fully permitted
 RCRA landfills, surface impoundments,
 waste piles that are not enclosed, and
 land treatment facilities. Enclosed waste
 piles that are permitted under Part 264
 would not require a waste management '
 plan prior to accepting these wastes.
 (The Agency made this determination
 because it judged that the means of
 enclosure satisfies the concerns the plan
 would address.)
  In addition, before any of these
 particular facilities can obtain a permit
 and, thus, before it can accept any of the
 wastes proposed to be listed today, it
 must have a "waste management plan"
 that is approved by the Regional
 Administrator. EPA believes that the
inherent hazard of these wastes,  and
 their mismanagement history, warrants
regulatory controls on potential
migration above those contained in the
 existing permit requirements. The
management plan will be the vehicle for
assuring individualized consideration
 that the wastes will be managed  safely.
                       The plan must be submitted by the
                       owner or operator "of the facility as part
                       of the permit application; it must
                       describe the potential for migration of
                       toxicants from the site via any media,
                       and, where migration is possible, it must
                       address measures to,be taken, over and
                       above the applicable permitting
                       requirement, to reduce migration of the
                       wastes or waste constituents.
                        At a minimum, the proposed plan
                       must address the volume and toxicant
                      'concentrations in the wastes to be
                       managed at the facility, the propensity
                       of toxicants to be emitted to the air
                       through volatilization or as aerosols or
                       dusts during placement of the wastes,
                       whether toxicants may migrate from or
                       with the wastes, whether the wastes
                       will be co-disposed with other materials
                       having mobilizing properties, and the
                       potential for soils to attenuate migrating
                       toxicants if the liner system (when one
                       is required by the regulations) is
                       damaged and breached. Where a"
                       potential for migration is identified, the
                       proposed plan must identify design
                       provisions  and/or operating practices to
                       be adopted to prevent that migration.  ' -
                       These design and operating features are
                       in addition to those that would-
                       otherwise be required by the
                       regulations. For example, if the facility
                       also disposes of dioxin solubilizing
                       solvents, the applicant may propose to
                       segregate the wastes to prevent contact.  •
                      If leaching is possible, the applicant
                      might propose lining the unit or mixing
                      the waste with activated carbon, organic
                      sorbents, or other materials designed to
                      immobolize the migrating toxicants.
                      Whatever is proposed by the applicant
                      must be supported by data or  a
                      technical rationale. The Regional
                      Administrator will evaluate whether
                      these additional management and
                      design features are adequate to prevent
                      migration.
                        As a general matter, the additional  '
                      measures required under a waste
                      management plan will focus on control
                      measures not currently specifically
                      required by the Part 264 land disposal
                      regulations. For example, the plan may
                      include specific waste treatment      •
                      processes that will reduce th&likelihood
                      that dioxin will migrate out of the unit.
                      In addition, the plan may include a
                      demonstration that siting factors (e.g.,
                      the attenuative properties of the soil
                      beneath the site) would operate to
                      control migration of dioxin. In most
                      cases, EPA does not believe that it will
                      be necessary to impose additional
                      structural requirements [e.g., liner
                      specifications) for the unit. The Agency
                      intends to provide detailed guidance for
                      the preparation of a waste management
 plan for managing these wastes prior to
 issuing this regulation in final form.
   Waste management plans''will be  ,
 considered in.the normal course of the
 permitting process, so that no special
 EPA review probedures are required.
   2. Management at fully permitted-
 incinerators. As stated, we also are
' .proposing-to allow incineration of these
 wastes only at fully permitted
 incinerators. It is the Agency's view that
 incineration often is a preferred ••
 management option for these wastes,
 because high temperature destorys the ,
 chlorinated dioxins and -dibenzofurans.
 If incineration is not properly performed,
 however, the original toxicants may be
 released,undestroyed, or chlorinated
 -dioxins, -dibenzofurans, biphenyls,  and
 -phenols can be formed from precursors
 such as chlorinated biphenyls,
 benzenes, and -phenols.
   The proposed regulation, therefore,
 allows these wastes to be burned only
 at fully permitted RCRA incinerators
 which have proven capability to assure
 99.99??; DRE for principal organic
 hazardous constituents (POHCs) which
 are as difficult, or more difficult to   -
 incinerate than CDDs or CDFs.ls The
 Agency judges that such a
 demonstration of DRE is sufficiently
 rigorous to ensure the proper
 management of these wastes, and
 therefore feels that it is not necessary to
 require an additional management plan
 for incinerator facilities treating these
 wastes.  ,          •   '  •
   3. Management at fully permitted tank
 and container storage facilities. We  also
 have tentatively decided against
 requiring fully permitted tank and
 container storage facilities to have a
 waste management plan approved by
 the Regional Administrator, before
' storing these wastes. The current
 storage regulations provide the Agency
 with sufficient information to evaluate
 the storage facility's ability to contain
 these  wastes. Therefore, an additional
 management plan for tank and container
 storage facilities storing'these wastes
 appears unnecessry.

 C. Other Management Options
 Considered or These Wastes
   1. Standards for Interim Status
 Landfills, Waste Piles, Surface      >
 Impoundments, Land Treatment
 Facilities, and Incinerators. The Agency
 considered proposing a regulation that
 would allow interim status land disposal
 and.incineration facilities to manage
 these wastes if they obtained prior
   18 The requirements for trial burn permits are
 described in 40 CFR 122.27. See also, "Guidance
 manual for hazardous waste incinerator permits;
 "U.S. EPA, Office of Solid Waste, November 1982.

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                  Federal  Register / Vol. 48, No. 65 / Monday, April  4, 1983 / Proposed Rules
                                                                        14521
 approval from the Regional             •.
 Administrator. It was felt that the
 Agency could provide interim.status
 facilities the same opportunities to
 handle these wastes as are provided to
 fully permitted facilities if the Agency
 can be assured that such management
 can be accomplished safely. The vehicle
 to be used to assure individualized
 consideration of prospective waste
 management would be a waste
, management plan that would address
 the factors outlined in the previous
 section as well as other design and
 operating conditions contained in the
 Part 264 regulations, as deemed
 appropriate by the Regional or State
 officials.            '  ."
   The procedures we considered for '
 approving a waste management plan
 would be the same as, or similar to,
 those for approving a closure plan. They
 would allow for public participation on
 the plan submitted by the facility, and
 on a tentative decision (and a rationale
 therefor) of the Regional Administrator.
 The Regional Administrator could hold a
 public hearing if he believed it would
 aid in elucidating the issues.
   However, the Agency .believes that
 most interim status facilities probably
 could not adequately manage these
 wastes without significant changes. In
 addition, the amount and detail of
 information to be provided in the
 'management plan could be almost
 equivalent to the-information needed to
 obtain a permit. For example, as part of
 the waste management plan for
 incineration,, the owner or operator of •
 the incinerator would need to conduct a
 trial burn to ensure that destruction and
 removal efficiencies could be met. EPA
 thinks it is unlikely that interim status
 facilities would go  to the expense of
 preparing and receiving approval on a
 plan, only to have to go through a later
 permit proceeding when their Part B
 application is processed.
   However, the Agency solicits
 comments on the desirability of allowing
• disposal and treatment of these wastes
 at interim status facilities ,having an
 approved management plan for these
 wastes.
   2. Additional Standards for Container
 and Tank Storage Facilities. The •
 Agency believes that container storage
 facilities storing these wastes should
 meet the moststringent requirements
 under Part 2641 Present regulations
 (Subpart I) do not require secondary
 containment for non-liquid wastes [e.g,
 tarry materials) if the storage area
 slopes, or the container is elevated.
 However, the A.gency believes that
 secondary containment might
 appropriately be required for container
 storage areas that store all non-liquid   •
 CDD and CDF-contaminated wastes,,
 due to the toxicity of these wastes, their
 potential to ooze and to spill, and the
 long time periods tfiese wastes may be
 stored before a disposal or incinerator
 treatment facility can be found that is
 willing to accept these,wastes. (For
 example, the wastes at the Vertac site
 have been stored for many years",
 despite the repeated attempts by the
 company to find a disposal site.) This
 requirement may be necessary to ensure
 that any spillage or release of these
 wastes is contained and not released
 into the environment. The Vertac
 damage incident, where improper
 storage of these wastes was responsible
 .for considerable harm, serves as an
, example of these wastes' potential for
 harm if stored improperly. The Agency
 therefore is considering a provision that
 would require secondary containment at
 container storage facilities that store
 non-liquid CDD- and CDF-contaminated
 wastes.'                        •
   The Agency is also considering a
 provision that would require secondary
 containment at tank storage facilities
 that stpre CDD- and CDF-contaminated
 wastes, due to the wastes' toxicity and
 the long periods of time they might be  .•
 stored. The damage incident .at Neosho,
 Missouri, when a concrete tank holding
 chlorophenolproductionstill bottoms (a
 waste covered by this proposal) and
 wastewater cracked, and caused
 considerable contamination, illustrates
 the potential for harm that s'econdary
 containment could address. The Agency
 solicits comment on the suitability of.-,
 these two provisions.                  ,
   3. Optional Standards Considered for
 Permitted Incinerators. Under current
 regulations, a facility which has shown
 that it can achieve 99.99% ORE for .   '
 POHC's  which are more resistant to
 thermal degradation than are CDDs or
 CDFs (such as carbon tetrachloride or
 pentachlorophenol), may be permitted to
 incinderate CDD or CDF-containing
 .wastes without conducting an additional
 trial burn or modifying its permit (40
 CFR 264.342 and 264.343). Because of
 theiriiazardousness, the Agency is
 considering proposing that a facility
 burning  these wastes notify the Regional
 Administrator of that fact. We are
 -considering this requirement because it
 is felt that Regional authorities might
 wish to prioritize compliance monitoring
 for facilities incinerating these wastes.
    The Agency solicits comments 'on the
 desirability of requiring notification to
 the Regional Administrator on the part
 of a facility that is burning CDD or CDF
 wastes.                   •••;,..
    4. Development of Special
 Management Standards.  The Agency is
 considering the development of special
management standards for CDD/CDF-
contaminated wastes. For some wastes,
high temperature incineration might be
the preferre'd method of treatment,
whereas for other wastes lane! disposal
might be a better alternative, For the
latter, disposal at sites having particular
. hydrogeological iand topographic or
surface water characteristics might be   •*
needed. The Agency is presently
reviewing these problems, arid may, for
example, propose incineration standards
that could require levels of destruction
and removal efficiency (DRE's) for these
wastes that ari» greater than the 99.99%"
DRE presently Required .under RCRA.
For some wastes, land disposal controls
ensuring the prevention of dust
formation could be imposed,, and for
some wastes the Agency could prescribe
the application of special technologies,   ,
such as photodechlorination, or molten
salt or critical water oxidation, which
are known to cause the destruction of
chlorinated aromatics. such as CDDs.
   The Agency solicits comment with
respect to the regulatory alternatives
discussed above, as well as any other  ,
approaches which might realistically be
considered,  j.-          .
             -• '•           - •*  '• '   '   •  '
YHI. Analytical Method foETetra-,  .
Penta-, and H«xachIoro-Dibenzo-p-
Dioxins and -Bibenzofurans     .

   In order to assist generators in the
determination of the contamination of
wastes with the above compounds, [e.g.,
for delisling purposes under §§260.20
and 260.22 of the RCRA regulations), the
Agency is proposing a method of
analysis for tetra-, penta-, and
hexachlorodibenzo-p-dioxinsjirid-   «-...-
-dibenzofurans (see Appendix A). The
method proposed in this regulation was
largely developed by!the workers at
Wright State University,; arid lias been
used for the analysis of TCDDs in. a
variety of wastes.19 If adopted, this ,-'
method will replace the method for
 analysis of ,TCDD presently listed in the
 solid waste test manual ("Test Methods
 for Evaluating  Solid Waste Physical/
 Chemical Methods", EPA publication
 number SW-846). The present method is
 inappropriate because it is not       -.
 sufficiently -sensitive, and.does not
 sufficiently eliminate interfering,
 substances. It also 'does not specify the
 procedure -to lie followed for the
   ""Analytical protocol for determination of'
 TCDDs in phenolic chemical wastes and soil
 samples obtained from the proximity of chemical .
 dumps", and "Analytical protocol for determination
 of chlorinated .dibisnzo-p-dioxins and chlorinated
 dibenzofurans in liver water", Brehm Laboratory,
 Wright State University, Dayton, OH,45435, January
 7,1982. These protocols are available in the Docket
 for this listing.   i       .. »  —  .:,     ,


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 14522
Federal Register / Vol. 48, No. 65 / Monday,  April 4,  1983 / Proposed Rules
 analysis of the chlorinated
 clibenzofurans.
   The proposed method subjects the
 sample to extraction with petroleum
 ether (waste not amenable to petroleum
 ether as an extractant, such as tar-like
 or carbonaceous wastes, will require
 extraction with other organic solvents,
 such as toluene, hexane, or
 dichloromethane).20The extract is
 successively washed with alkali and.
 acid, subjected to fractionation on
 alumina, and the eluate is analyzed by
 high-resolution gas chromatography,
 using a capillary glass column, and by
 low-resolution mass spectrometry. In
 case ofmterference, the alumina eluate
 is subjected to further cleanup with high
 pressure liquid chromatography (HPLC).
   The Agency has chosen the proposed
 method because it is the one that has
 been most successfully applied to
 chemical wastes. In addition, its
 originators have indicated to the Agency
 that it can be used for the analysis of
 both CDDs and CDFs.2*-24For example,
 the proposed method has been used for
 the analysis of TCDD in chlorophenol
 still bottoms, reactor residues, oxidation
 pond sediments, cooling pond muds,
 contaminated soils, and sludge samples.
 The detection limit for TCDD
 established in these different matrices
 varied from 15 ppt (soils, 0.5 ppb
 (cooling pond muds), and 1 ppb     •;
 (sludges) to 0.1-1300 ppb (still bottoms,
 highly variable). The recovery of added
 TCDD varied from 14-111 percent,
 averaging 76 percent. In incinerator
 stack effluents, the minimum detectable
 quantity was 3.8 ng for CDDs and 3.5 ng
 for CDFs, and the recovery of added
 CDDs or CDFs averaged 80 percent.
 IX. Questions for Comment
  The Agency welcomes public
 comment on all aspects of this proposed
rule. However, public comment is
 especially solicited with respect to the
 following questions.
  1. Should EPA develop, for ODD or
 CDF-containing wastes, a
  ""Capabilities on methodology for the analysis
of tclracJilorodibcnzo-p-dloxin", Baltelle Columbus
Laboratories, Columbus, OH 43201, August 10,1981.
  " Dr. M. Taylor, Wright State University, to C.
Corcln, U.S. EPA, Report of analytical data
(December 8,1979).
  *»Dr. T, O. Tieman. Wright State University, to D.
L, Rosengrcn. Viar and Company, Inc., Report on
sample analyses (Juno 1,1982].
  **Dr. T, O. Tieman, Wright State University, to L.
Unas, Viar and Company, Inc., Report on sample
analyses (August 6,1982),
  *4T. O. Tieman et al. Incineration of chemical
wastes containing polychlorinaled biphenyl;
assessment of tests conducted at Rollins
Environmental Services. Deer Park, Texas, and
Energy Systems Company, El Dorado, Arkansas. In:
Dcloxlcnlton of Hazardous Waste.}. H. Exner, Ed.,
Ann Arbor Science. 1982. pp 143-183.
                       "characteristic " definition of
                       hazardousness under Subpart C of
                       Section 261 of the RCRA regulations?
                       Instead of listing CDD/CDF-containing
                       wastes as hazardous under Subpart D of
                       the Part 261 regulations, EPA considered
                       an alternative approach, namely,
                       identifying such wastes as
                       "characteristic" hazardous wastes under
                       Subpart C of Part 261. This approach
                       would oblige the  Agency to make a
                       generic determination as to the lower
                       level of concern regarding CDD/CDF
                       contamination, and would then require
                       generators to either analyze or estimate
                       the amount of CDD's or CDF's in a
                       waste (by actual  analysis  or, for
                       example,  from a knowledge of reaction  :
                       chemsistry, process technology, and
                       chemical  engineering principles).
                        The Agency judged that this approach,
                       although at first glance appealing
                       because of its apparent simplicity,
                       would not be a suitable regulatory
                       alternative. It would require that the
                       Agency set a concentration (as in the EP
                       hazardous waste  characteristic) defining
                       the level at which CDD's and CDF's
                       constitute a minimum level of concern.
                       Heretofore, EPA has not attempted to
                       set a lower limit for the concentration of
                       a toxicant of concern in a waste, except
                       in a limited manner. Instead, EPA has
                       made qualitative  assessments in
                       determining-that certain wastes should
                       be listed in the RCRA regulations
                       because they present a potential threat
                       to human  health and the environment, if
                       mismanaged.
                        Because of the high^acute and chronic
                       toxicity properties of many of the CDD's
                       and CDF's, as evidenced in animal
                       studies, the Agency considered that, if a
                       lower limit of concern were to be
                       developed it would be very low.
                      Additionally, because biological
                       availability of these toxicants is
                       expected to be dependent  on waste
                      matrix characteristics, it was felt that a
                      generic risk estimation for all wastes
                      would be  extremely difficult-to. perform.
                       One alternative was to set thg lower
                      limit at the limit of detection of CDD's <
                       and CDF's in the waste. However, this is
                      not a fixed concentration. As outlined
                      above, the limit of detection is'sample
                      and matrix-dependent.  Since industrial
                      wastes are' highly variable, it may not be
                      realistic to establish generally
                      applicable standards for the level of
                      detection, recovery, and reproducibility
                      for the analytical  determination of
                      CDD's and CDF's in these wastes.
                       • Within the above limitations, the
                      Agency could nevertheless set a lower
                      level of concern for the concentration of
                      CDD's and CDF's  in these wastes. The
                      Agency solicits comment on the
 advisability, practicality, and
 desirability of doing so. If a lower level
 of concern is to be established, at what
 level should it be set, and how .could this
 level be justified?
  2. Analytical Methodology—The •
 Agency solicits comment on the
 proposed method of analysis for CDD's
 and CDF's; in particular, evidence that
 some extraction media may be more
 efficacious than others for particular
 wastes. The Agency considered whether
 it might be useful to develop a method of
 analysis that would be less detailed,
 and therefore less expensive, than that
 proposed, since a high degree of
 specificity with respect to isomeric,
 content is not necessary in the present
 instance. For delisting purposes, for
 instance, it might be sufficient for,a
 petitioner to show that a waste does not
 contain any CCD's or CDF's—even
 though, for example,- dichloro- or hepta-
 and octachlorodioxins are present. The
 Agency solicits comments with respect
 to the usefulness, practicability, and
 cost, for instance, of a GC/MS
 analytical method which would detect
 total CDD's and CDF's at low levels in a
 waste in one analytical determination.
  3. Wastes resulting from
 manufacturing processes conducted on
 equipment contaminated with CDD's or
 CDF's—The Agency is proposing to list
 as hazardous, wastes resulting from
 processes conducted on equipment
 previously used for  a manufacturing
 process that generated CDD's or CDF's,
 A generator could legitimately question
 how this regulation  can be enforced:
 how can they know whether the
 equipment in question was previously
 used for these processes? The Agency
 considers that a  demonstration of
 historical knowledge would be deemed
 sufficient for this purpose (45 FR 32678
 (May 19,1980); see also the Listing
 Background Document). If historical
 records are not available, or inaccurate,
 analysis of .the listed wastes on several
 occasions for total CDD'S and CDF's
would be sufficient to establish their
 absence. The Agency solicits comments
 on the appropriate historical records
 and time periods to  be used,  and the
 appropriate analytical detection limit to
 be used if historical records are not
 available.
  4. Identification of commercial
chemical products subject to this listing.
The Agency is concerned that some
users of commercial chemical products
may not be able to identify which
commercial chemical products contain
tri-, tetra-, or pentachlorophenol, or their
chlorophenoxy derivative acids, esters,
 and amine salts,  and which, therefore,
would be regulated (when discarded) as

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                  Federal Register  / Vol. 48,  No. 65 /  Monday,  April 4,  1983 /Proposed Rules
                                                                       44523
 EPA Hazardous Waste Nos. F023.
 Although the FIFRA regulations (40 CFR
 162) do require that active ingredients
 be identified by their chemical name or
 by a usual common name, and an EPA
 publication ("Accepted common names
 and chemical names for the ingredient
 statement on pesticide labels", EPA 540/
. 9-7-017) is available to aid in their
 chemical identification, these aids may
 not convey sufficient information to the
 unsophisticated user. Non-pesticide
 products may also be hard to identify.
 Therefore, the Agency is considering
 various mechanisms to solve this
 potential problem (i.e., labeling
 requirements for manufacturers,  . - ..
 publishing a list of all products which
 contain these compounds, etc.).The
 Agency solicits comment on this      "
 potential problem.
    5. Wastes which may contain CDDs
 and CDFs but which are not covered by
 the present regulation. The Agency has
 some data indicating that wastes, other
 than those covered by this proposal,
 may contain CDDs and CDFs. This may
 be the case, for instance for residuals
 such as fly ash from low temperature
 combustion of certain industrial wastes
 (especially of wastes containing
 chlorophenols, or chlorobenzenes);
 residuals from dichlorophenol
 manufacture; and sludges from wood
 preserving using pe'ntachlorophenols. In
 the case of the first two wastes,
 although the Agency, on the grounds of
 knowledge of reaction chemistry and
 process technology, believes this may be
 the case, it lacks sufficient data to
 support this supposition. For this reason,
 studies are being conducted in order to
 gather more data. These "wastes may be
 listed at a future date if further evidence
 demonstrates that they indeed are
 hazardous.                          "
   With regard to waste from wood
 preserving, we are presently
 investigating whether additional wastes
 from this process should be listed as
 hazardous, and whether CDDs and
 CDFs should be constituents of concern
 in the process wastes already listed
 (EPA Hazardous Waste K001,
 Wastewater treatment sludges). Pending
 completion of those studies we may take
 further regulatory action.  •
 X. Economic, Environmental, and
 Regulatory Impacts
 A. Regulatory Impact Analysis
   Under Executive Order 12291, EPA
 must "determine whether a regulation is
 "major" and therefore subjept to the
 requirement of a Regulatory Impact •
 Analysis. The effect of the present
 amendment is judged not to be major,
 since it in part replaces regulation under
 a different statute (Section B(d) of the
 Toxic Substances ControlAct), and
 imposes an additional regulatory burden
 only on three manufacturers, of'  '•':
 chlorophenols, and five manufacturers
 of chlorophenols and their
 chlorophenoxy derivatives. In addition,
 some number of manufacturers who use
 equipment that may be contaminated
 with CDDs or CDFs may also have
 additional regulatory burden. However,
 we presume that this part of the
 regulation is unlikely to affect many
 additional manufacturers ;other than the
 eight referred to above. La addition, this
 regulation imposes a regulatory burden
 on perspns or entities discarding some
 unused formulations containing tri-,
 te{ra-, or pentachlorophenol or unused
"formulations containing compounds
'derived from these phenols. The
 disposal of many of these formulations,
 however, is already regulated under
 § 261.33 of RCRA. Additionally, because
 of their inherent value, we do not
 believe that the regulated community
 will usually discard substantial
 quantities of these materials, further
 minimizing any.impact.
   In addition, we believe that there will
 be no adverse impact on the ability of
 U.S.-based enterprises to compete with
 foreign-based enterprises in domestic or
 export markets. Therefore, since the
 Agency does'not expect that the
 proposed action will result in either an
 effect oh the^economy of $100 million or
 more, or an adverse impact on U.S.
 based enterprises, this "proposed
 regulation is not considered to be a"
 major action. Because this proposed
 amendment is not a major regulation, no
 Regulatory Impact Analysis has been
 conducted.          •       '-.-..."
   This amendment was submitted to the
 Office of Management and Budget
 (OMB) for review as required by
 Executive Order 12291. Any comments
 from OMB to EPA, and any EPA   ,
 responses to those comments are
 available for public inspection in Room
 S-269CatEPA.   ,

 B. RegulatoryFlexibility Act

   Pursuant tq the Regulatory Flexibility.
 Act, 5 U.S.Gy§ 601 etseq., whenever an"
 agency is required to publish a general  ~"
 notice of rulemaking for any proposed or
 final rule, it must,prepare and make
 available for public comment a
 regulatory flexibility analysis that
 describes the impact of the rule on small
 entities (i.e., small businesses, small.
 organizations, and small governmental
 jurisdictions). No regulatory flexibility
 analysis is required, however, if the
 head of the agency certifies that the rule
 will  not have a significant economic
 impact on a substantial number of small
 entities.      (•'   ,
 '  Only one of the hazardous wastes"
 proposed to b« listed in § 261.31 is,
 expected to be generated by small
 entities. The Agency anticipates that
 pesticide aerial applicators will
 constitute the main segment/of small
 business entitj.es affected by this
 regulation.25However, these.persqns are
 probably already regulated under RCRA
 since a large number of pesticides (both
 acutely hazardous and toxic) are
 currently covered by existing        '
 regulations. Therefore; we would riot
 expect any aerial applicators to be
 newly regulateid as a result of this rule..
 In addition, thie Agency does not believe
 that small entities will dispose of
 significant quantities of the commercial
 chemical products proposed for   ;
 regulation. Thus, today's amendment is
• unlikely to have a significant economic
 impact on a substantial number of small
 entities. This regulation therefore does
 not .require a regulatory flexibility
 analysis.  •  ,',"               '     •

 C. Paper Reduction Act of1980

   The reporting orrecordkeeping        ;
 (information) provisions in this rule will
 be submitted for approval to the Office
 of Management and Budget (OMB)
 under Section 3504(h) of the Paperwork
 Reduction Act of 1980, U.S.G. 3501 et
 seq. Any final rule will explain.how its
 reporting or rebordkeeping provisions
 respond to any OMB or public
 comments.   ii '               •

 XII. Rulemaking Record

   The public docket for 40 CFR Part 775
 is located in Room E-107 at the address
 listed for the U.S. Environmental
 Protection Agency in the address section
 of this preamble. The entire rulemaking
 docket for the'rale being proposed today
 is included in ihe record for 40 CFR Part
 775. EPA will identify the complete
 rulemaking record for 40" CFR part 775
 on or before the date of repeal. EPA will
 consider any time between the  ~
 publication of this notice and the date
 the Agency ideintifies'thelinal record.

 XII List of Subjects
 40 CFR Part 261
          '  • .1               .'.'-,
   Hazardous materials, Waste
 treatment and disposal, Recycling.   -
  25 Farmers may also generate some of these
 wastes—discarded unused fonnulations—however,
 farmers are exempt from regulation provided the
 waste pesticides are from their own.use and are
 disposed of on their own farm rn a manner '
 consistent with the disposal instructions on the
 pesticide label. Therefore, we,do not expect farmers
•to. be severely impacted.

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14524
Federal Register /  Vol.  48, No. 65"/ Monday, April  4,  1983  / Proposed Rules
40 CFR Part 264
   Hazardous materials, Packaging and
containers, Reporting requirements,
Security measures, Surety bonds, Waste
treatment and disposal.

40 CFR Part 265
   Hazardous materials, Packaging and
containers, Reporting requirements,
Security measures, Surety bonds, Waste
treatment and disposal, Water supply.

40 CFR Part 775
   Environmental protection, Hazardous
materials, Pesticides and pests, Waste
treatment and disposal.
  Dated: March 21,1983.
John W. Hernandez,
Acting Administrator.
   For the reasons set out in the
preamble, it is proposed to amend Title
40 of the Code of Federal Regulations as
follows:

PART 261—IDENTIFICATION AND
LISTING OF  HAZARDOUS WASTE
   3. The authority citation for Part 261
reads as follows:
  AuUiority: Sees. 1006, 2002(a), 3001, and   .,
3002 of the Solid Waste Disposal Act, as
amended by the Resource Conservation and
Recovery Act of 1976, as amended [42 U.S.C.
6905,0912(a), 6921, and 6922).
   2. In § 261.5, paragraphs (e)(l) and
(e)(2) are revised to read as follows:
§ 261.S   Special requirements for
hazardous waste generated by small
quantity generators
*     *     *    *°    *
   (e) * * *
   (1) A total  of one kilogram of acutely
hazardous wastes listed in §§261.31,
281.32, or 261.33(e).
   (2) A total  of 100 kilograms of any
residue or contaminated soil, waste or
other debris resulting from the cleanup
of a spill, into or on any land or water,
of any acutely hazardous wastes listed
in §§261.31,261.32, or 261.33(e).
   3. In §261.7, the introductory text of
paragraphs (b)(l) and(b)(3) is revised to
read as  follows:                 -"

§261.7  Residues of hazardous waste in
empty containers.
*     *     *    *     *

   (b)(l) A container or an inner liner
removed from a container that has held
any hazardous waste, except a waste
that is a compressed gas or that is
identified as  an acutely hazardous
waste listed in §§261.31  261.32, or
261.33(e) of this chapter is empty if:
*****
   3. A container or an inner liner
removed from a container that has held
an acutely hazardous waste listed in
§§261.31 261.32, or 261.33(e) is empty if: -
                            4. In §261.31, add the following waste
                          streams:

                          §261.31   Hazardous waste from
                          nonspecific sources.
                         Industry and EPA
                         hazardous waste
                             .' no.
       Hazardous waste
Hazard
 code
                         Generic:
                           F020....
                           F021..
                           F022....
                           F023		
 . Wastes (except wastewater , (H).
    and spent carbon from hy-
    .drogen chloride purification)
    from  the  production  or
    manufacturing  use  (as a
    reactant, chemical interme-
    diate, or component in a
    formulating process) of tri-,
    tetra-.   or  'pentachloro-
    phenol, or of intermediates
    used to  produce their de-
    rivatives. (This listing does
    not include wastes from the
    production of  Hexachloro-
    phene from highly purified
    2,4,5-trichlorophenol.:
 . Wastes " (except wastewater  (H).
    and spent carbon from hy-
    drogen chloride purification)
    from the manufacturing use
    (as a reactant, chemical in-
    termediate,  or component
    in a formulating process) of
    tetra-, penta-, or hexachlor-
    obenzenes  under  alkaline
    conditions.
 .  Wastes (except  wastewater  (H).,
    and spent carbon from hy-
    drogen chloride purification)
    from the  production of ma- ,
    terials on equipment previ-
    ously used for the produc-
    tion  or manufacturing use
    (as a reactant,  chemical in-  ,
    termediate or. component in
    a formulating  process)  of
    materials listed under F020 .
    and F021..
   Discarded  unused  formula- '(H).
    tions containing tri-, tetra-,
    or  pentachlorophenot  or
    discarded unused formula-
    tions containing compounds
    derived from these chloro-
    phenols.
                           5. In § 261.33(f), remove the following
                         waste streams:

                         § 261.33   Discarded commercial chemical
                         products, off-specification species,
                         container residues, and spill residues
                         thereof.
                           Hazardous
                           waste No,
            Substance
                         U212	
                         U212	
                         U230	
                         0530.
                         U231.
                         U231.
                         U232.
                         U232.
                         U233.
                         U233.
                         U242.
                         U242,
2,3,4,6-Tetrachlorophenol.
Phenol, 2,3,4,6-tetracholorq'-.  -
2,4,5-Trichlorophenol.   V
Phenol, 2.4,5-trichloro-.
2.4,6-lrichlorophenol.
Phenol, 2,4,6-trichlorq-.
2,4,5-Trichlorophenoxyacetic acid.
2,4,5-T.
'Silvex.
Proptonic acid, 2-(2,4,5-trichlorophenoxy)-.
Pentachlorophenol.
Phenol, pentachloro-.    -       '    ,
                           6. Amend Table I in Appendix III of
                         Part 261, by removing the entry
                         "chlorinated dibenzodiqxins", and
                         adding the following entries in
                         alphabetical order:

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                     Federal  Register  / Vol. 48,  No. 65 /  Monday, April  4, 1983  /^Proposed Rules
                                                                                                                    14525
                     Appendix III—Chemical Analysis Test Methods
                   * .    ~        *       '      * /           *     "••-       *            ' *

                TABLE 1 .—ANALYTICAL CHARACTERISTICS OF ORGANIC CHEMICALS

                                                    \                    Measurement, techniques
            Compound
                                   Sample handling class/fraction
                                               Non-GC
                                               methods   GC/jyS
                                                                                Conventional -
                                                                               GC
                                                                                     Detector
 Chlorinated dibenzo-p-dioxins.'.	 Extractable/BN..,
 Chlorinated dibenzofurans	:	 Extractable/BN...
                                                         8280
                                                         8280
     7. Add the following  entries in numerical  order to  Appendix VII  of Part 261:

                  Appendix VII—Basis for Listing Hazardous Wastes   -
     EPA
   hazardous
   waste No. .
Hazardous constituents for which listed
   EPA_
hazardous
. waste No.
                                              Hazardous constituents for which listed
            . tetra-i  penta-, and  hexachlorodibenzo-p-
               "dioxins; tetra-, penta-, and- hexachlorodi-
               benzofurans; and tri-, tetra-,  and penta-
               chlorophenols and  their  chlorophenoxy.
               derivative acids, esters, .and amine salts..
             tetra-,  penta-, 'and  hexachlorodibenzo-p-
               dioxins; tetra-, penta-, and hexachlorodi-
               benzofurans; and trK tetra-,  and penta-
               'chlorophenols and  their  chlorophenoxy
               derivative acids, esters, and amine salts.
                                             tetra-, penta-,  and  hexachlbrodibenzo^-
                                              dioxins; tetra-, • penta-, and hexachlorodi-
                                              benzofurans; and tri-, tetra^,'and  penta:
                                             • chlorophehols and their  chlorophenoxy
                                             ' .derivative acids,  esters, and amine salts.
                                             tetra-, penta-,  and  hexachlorodibenzo-p-
                                              dioxins; tetra-, penta-; and hexachlorodi-
                                              benzofurans; and tri-, tetra-, and  penta-
                                            - chlorophenols and their  chlorophenoxy
                                              derivative acids,  esters, and amine salts.
     8, Add the  following constituents in alphabetical  order  to Appendix VIII of
 Part 261:         -                  .                            •               -

                      .  Appendix VIH—Hazardous Constituents
                       •*           *           *           *          * .         '    '
 hexachlorodibenzp-p-dioxins        ~"   ."                  "'...-'..'•••
 hexachlorodibenzofurans                                          .
 pentachlorodibenzo-p-dioxins         -     .              -
 pentaehlorodibenzofurans
 tetrachlorodibenzo-p-dioxins             '                         ...
 tetrachlorodibenzofurans                                            ,                    .
   9! Appendix IX is added to Part 261 to
 read as follows:

 Appendix IX—Method of Analysis for
 Chlorinated dibenzo-p-dioxins and -
 dibenzofurans1234 '-            -
-Method 8280
   1t  Scope and Application.        •
   'This method is appropriate for the analysis of
 tetra-, penta-, and hexachlorinated dibenzo-p-
 dioxins' and -dibenzofurans,
   2Analytical protocol for determination of TCDDs
 in'phenolic chemical wastes and soil samples
 obtained from the proximity of chemical dumps.
 T.O. Tiernan and M. Taylor. Brehm Laboratory,
 Wright State University, Dayton, OH 45435.
   Analytical protocol for determination of
 chlorinated dibenzo-p-dioxins and chlorinated
 dibenzofurans in river water. T.O. Tiernan and M. •
 Taylor. Brehm Laboratory, Wright State University,
 Dayton, OH 45435.
   ••In general, the techniques that should be used to
 handle these materials are those which are followed
 for radioactive .or infectious laboratory materials.
 Assistance in evaluating laboratory practices may
 be obtained from industrial hygienists and persons
 specializing in safe laboratory practice. Typical
                                  1.1  This method covers the determination
                                of chlorinated dibenzo-p-dioxins and
                                chlorinated dibenzofurans in chemical
                                wastes including still bottoms, filter aids,  .
                                sludges, spent carbon, and reactor residues,
                                and'in soils.                      ,
                                  1.2  The sensitivity of this method is
                                dependent upon the level of interferences.
                                  1.3  This method is recommended for use
                                :ohly by analysts experienced with residue
                                analysis and skilled in mass spectral"
                                analytical techniques.
                                  1.4  Because of the extreme toxicity of
                                these compounds, the analyst must take
                                necessary precautions to prevent exposure to
                                himself, or to others, of materials known or
                               •beleved to contain CDDs or CDFs.
                                infectious waste'incinerators are probably not
                                satisfactory devices for disposal of materials highly
                                contaminated with GDDs or CDFs. A laboratory
                                planning to use these compounds should prepare a
                                disposal plan to be reviewed and approved by
                                EPA's Dioxin Task Force [Contact Conrad Kleveno,
                                WH-548A, U.S. EPA, 401 M Street, S.W.,
                                Washington, D.C. 20460).
    2.  Summary of the Method.
    2.1  This method is an analytical
  extraction cleanup procedure, and capillary
  column gas chromatographty-low resolution
  mass spectrometry method, using capillary
  column GC/MS conditions and internal
" standard techniques, which allow for the
  measurement of PCDDs and PCDFs in the '
  exjract.     j . :    '   .   ,  .
    2.2 ' If interferences are encountered, the *
  method provides selected general purpose  -'
  cleanup procedures to aid the analyst in, their
  elimination. ,;';  •''-.'''
    3.  Interferences.
   •3.1  Solvents, reagents, glassware, and
- other sample processing hardware may yield
  discrete artifacts and/or elevated bas*eljnes
  causing misinterpretation of gas             .
  chrdmatograms. All of these materials must -
  be'demonstated to be free from interferences
  under the conditions  of .the analysis by
  running method blanks.. Specific selection of
 , reagents and purification of solvents by
  distillation in all-glass systems may be
  required.   ;      '       '     •     '.  ••  '
    3.2  Interferences co-extracted from  the
  samples will vary considerably from source
  to^source, depending  upon the diversity of the
  industry being sampled. PCDD is often
  associated with other interfering chlorinated
  compounds such as PCB's which may be at
  concentrations several orders of magnitude
  higher than that of PCDD. While general
  cleanup techniques are provided as part of
  this method, unique samples'may require
  additional cleanup approaches to.achieve the
  sensitivity stated in Table 1.
    3.3  The other isomers of
  tetrachlorodibenzo-prdioxin may interfere
  with the measurement of 2,3,7,8-TCDD. •"
  Capillary column gas chrpmatography is
  required to resolve those isomers that yield /
  .virtually identical mass fragmentation
  patterns.   !i      •
 •- 4.  Apparatus and Materials.   . .  •.
    4.1  Sampling equipment for discrete or
  composite sampling.                      '
    4.1.1   Grab sample bottle—:amber glass, 1-
  liter or 1-quart volume. French or Boston   _
  Round design is recommended. The container
  must be washed and  solvent rinsed before
  use to minimize interferences.  *
    4.1.2   Bottle caps—threaded to screw on to'
  the sample bottles. Caps must be lined  with
  Teflon. Solvent washed foil, used with the
  shiny side towards the sample, may be
  substituted for the Teflon if sample is not
  corrosive.   -.             : '  •
    4,1.3   Compositing equipment—automatic
  or manual compositing system. No tygon>or •
  rubber tubing may be. used, and the system
  must incorporate glass sample containers for
  the collection of a minimum of 250 ml. Sample
  containers must be kept refrigerated after •
  sampling.   ."   .    •          .   '
    4.2  Water bath—heated, with concentric
  ring cover, caipable of temperature control (±
  2° C). The bath sho.uld be use'd in a hood.
    4.3  Gas cliromatograph/mass
  spectrometer data system                •
    4.3.1   Gas chromatograph: An analytical
  system with a temperature-programmable gas
  chromatograph and all required accessories
  including syringes, analytical columns,  and

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14526
Federal  Register / Vol. 48, No.  65 /  Monday,  April  4,  1983  / Proposed  Rules
  4.3,2  Column: SP-2250 coated an a 30 m
 long x 0,25 mm LD. glass column [Supelco No.
 2-3714 or equivalent). Class capillary column.
 conditions; Helium carrier gas at 30 cm/sec
 linear velocity run spliUeas. Column
 temperature ia 210* C.
  4.3.3  Mass spectrometer: Capable of
 scanning from 35 to 450 amu every 1 sec or
 lass, utilizing 70 volts (nominal) electron
 energy in the, electron impact ionization mode
 and producing a mass, spectrum which meets
 all the criteria in "table 2 when 50 ng. of
 decafluorotriphenyl-phosphme (DFIPP) is
 injected through the GC inlet The system
 must also be capable of selected ion
 monitoring (SIM] for at least 4 ions
 simultaneously, with, a cycle time of 1 sec or
 less. Minimum integration time for SIM is 100
 ms. Selected ion monitoring ia verified by
 injecting .015 ng of TCD0 Cl" to give a
 minimum signal to noise ratio of 5 to 1 at
 mass 320.
  4.3.4  GC/MS interface: Any GC-to-MS
 interface that gives acceptable calibration
 points at 50 ng per injection for each
 compound of interest and achievea
 acceptable tuning performance criteria [see
 Sections O.t-6.3) may be used. GC-to-MS
 interfaces constructed of alt glass or glass-
 lined materials are recommended. Glass can
 be deactivated by silanizing with
 dichlorodimethyfsilane. The interface must be
 capable of transporting at least 10 ng of the
 components of interest from the GCto the
 MS.
  4.3.5  Data system: A computer system
 must be interfaced to the mass: spectrometer.
 The system, must allow the continuous
 acquisition and storage on machine-readable
 media of all mass spectra obtained
 throughout the duration of the
 chromatogiaphic program. The computer
 must have software that can search any GC/
 MS data file for ions of a- specific mass and
 that can, plot such ion abundances versus
 time or scan number. This type of plot is
 defined as an Extracted Ion Current Profile
 (EICP), Software must also be abler to
 integrate the abundance, to any EICP,
 between specified time or scan number
 limits.
  4.4  Pipettes-Disposable, Pasteur, 150-mm
 long x 5 mia ID (Fisher Scientific Co., No. 13-
 678-6A oruqulvalent).
  4.5  Flint glass bottle- (Teflon-Kned screw'
 cap).
  4.0  Reaoti-vital (sllanfaed} (Pierce
 Chemicat Co.).
  5. Reagents.
  5.1  Potassium- hydroxide-(ACSI, 2 percent
 in distilled water.
  5.2 Sulfuric acid-{ACS), concentrated.
  5.3 Methylcne chloride, hexane, benzene,
 petroleum either, methenol, tebradecane-
 pcsticide quality or equivalent.
  5.4  Stock standards in a glovebox,
 prepare stack standard solutions- of TCDD
 and Ct-TCDD (molecular weight 328), The
 slock solutions are stored in a glovebox, and
 checked frequently for signs of degradation
 or evaporation, especially fust prior to the
 preparation: of working' standards.
  5.5  Aluinina-basic, Woelm; 80/200 mesh.
Before use activate overnight at 600'C, cool to
room temperature in a dessicator.
  5.0  Prepurified nitrogen gas
                           6.0  Calibration.
                           6.1  Before using any cleanup procedure,
                         the analyst must process a series of
                         calibration standards through the procedure
                         to validate elution patterns and the absence
                         of interferences fronr reagents.
                           6.2  Prepare GC/MS. calibration standards
                         for the internal standard technique that will
                         allow for-measurement of relative response
                         factors of at least three TCDD/a7Cl-TCDD
                         and TCDF/3'C1-TCDF ratios.5 The 3'C1-
                         TCDD./E concentration in the standard
                         should ba fixed and selected to yield a
                         reproducible response at the most sensitive
                        . setting of the mass spectrometer.
                           &.3  Assemble the necessary GC/MS
                         apparatus  and establish operating
                         parameters equivalent to those indicated in
                         Section 11.1,of this method. Calibrate the
                         GC/MS system according to Eichelberger» et
                         al. (19Z5J by tha use of decafluorotriphenyl
                         phosphine (DFTPP). By injecting calibration
                         standards, establish the response factors for
                         CDDs vs. S4C1-TCDF. The detection, limit
                         provided in Table 1 should be verified by   '
                         infecting jQ15 ng of '"Cl-TCDD which should
                         give a minimum signal to noiae ratio of 5 to 1
                         at mass 320.
                           7.  Quality Control.
                           7.1  Before processing any samples, the
                         analyst should demonstrate through the
                         analysis of a distilled water method blank,
                         that all glassware and reagents are
                         interference-free. Each time a set of samples
                         is extracted or thera is a change ia reagents,
                         a method blank should be processed as a
                         safeguard against laboratory contamination.
                           7.2  Standard quality assurance practices
                         must be used with this method. Field
                         replicates must be  collected to validate the
                         precision of the sampling technique.
                         Laboratory replicates must be analyzed to
                         validate the precision of the analysis.
                         Fortified samples must be analyzed to
                         establish the assuracy of the analysis.
                           8.  Sample Collection, Preservation, and
                         Handling.                      ' ,
                           8.1  Grab and composite samples must be
                         collected in glass containers. Conventional
                         sampling practices should be followed,
                         except that the bottle must nnt heprewashed
                         with sample-before collection^ Composite
                         samples should be collected in glass -
                         containers, ia accordance with, the
                         requirements of the RCRA program. Sampling
                         equipment must be free of tygon and other
                         potential sources of contamination.
                           8.2  The samples must be iced of,
                         refrigerated from the time, of collection, until
                         extraction. Chemical preservatives siould
                         not be used in. the field unless more, than 2.4:
                         hours will elapse before delivery to the
                         laboratory. If an aqueous sample is faken and
                         the sample will not be extracted within 49
                         hours of collection, the sample should be
                         adjusted to a: ptf range of 6.0-S.O with sodium
                         hydroxide  or sulfuric; acid.
                          5 "'Cl-labelled TCDD and TCDF are available
                         from K.O.R. Isotopes, Cambridge, MA. Proper
                         standardization requires tbff tree of a specific
                         labelled iaomer for each congener to be determined.
                         However, the only labelled fsomers readily-
                         available are a7Gt-2;3,Z,8-TCDDand37Cl-2,3,?,8-
                         TCDF. Tints method therefore uses ffieseisomere as
                         surrogates for the CDDs ancf CDFs. Wfieir labelled
                         CDDs and CDFs are airailabre, their use^will be
                         required.
   8.3  All samples must be extracted with 7
 days and completely analyzed within 30 days
 of collection.
   9.  Extraction, and Cleanup Procedures.
   9.1  Use an aliquot of 1-10 g sample of the
 chemical waste or soil to be analyzed. Soils
 should be dried using a stream of prepurified
 nitrogen and pulverized in a ball-mill or
 similar device. Transfer the sample to a tared
 125 ml flint glass bottle (Teflon-lined screw
 cap] and determine the weight of the sample..
 Add an  appropriate quantity of 37Cl-lahelled
. 2,3,7,8-TCDD (adjust the quantity according
 to the required minimum detectable '
 concentration), which is employed aa an
 internal standard.
   9.2  Extraction.,
   9.2.1  Extract chemical waste samples by
 adding-10" ml methanol, 40" ml petroleum
 ether, Sttml doubly distilled water, and then.
 shaking the mixture for 2 minutes. Tars-
 should be completely dissolved in any of the
 recommended neat solvents. Activated
 carbon samples rouat he extracted with
 benzene usingmathad 3540, in SW-846 (Test
 Methods for Evaluating Solid Waste—
 Physical/Chemical Methods, available from,
 G.P.O. Stock #055-Q02r810Ql-2).
 Quantitatively; transfer the organic extract or
 dissolved sample, to a. clean. 250. ml flint glass
 bottle (Teflon lined screw cap), add 50 ml
 doubly distilled water and shakefor 2
 mmutes. Discard tha aqueous layer and
 proceed" with Step 9.3.
   9.2.2  Extract soil samples by adding 40 ml
 of petroleum ether, to the sample, and then
 shaking for 20 minutes. Quantitatively
 transfer the organic extract to a clean 250 ml
 flint glass bottle (Teflon-lined screw cap)v   •
 add 50 ml doubly distilled water and shake
 for 2 minutes. Discard the aqueous: layer: and
 proceed with Step 9.3.
   9.3  Wash the organic layer with 50 ml; of  -
 20% aqueous potassium hydroxide by shaking1
 for 10 minutes and then remove and discard
 the aqueous layer.
   9.4  Wash the organic layer with 50 ml of
 doubly, distilled water by shaking for 2
 minutes and discard the aqueous layer.
   9.5  Cautiously add 50. ml concentrated
 sulfuric  acid and shake for 10 minutes'. Allow
 the mixture to stand until layers- separate
 (approximately 10 mmutes), and remove and
 discard the acid layer. Repeat acid washing
 until no  color is visible lathe acid layer.
   9.6  Add 50 ml of doubly distilled' water to
 the organic extract and shake for 2 minutes-.
 Remove and discard the aqueous layer and
 dry the organic layer by- adding; lOg of
 anhydrous sodium sulfate.       '
   9.7  Concentrate the extract tot incipient
 dryness by heating in a 50,° C water bath and
 simultaneously flawing, a. atream of
 prepurified: nitrogen aver/ the extract.
 Quantitatively transfer the residue taan
 alumina microcolumn1 fabricated as follows:
   9.7.1  Cat off the top-section of a 10 ml
 disposable Pyrex pipette at the 4.0 ml mark
 and insert a plugof silanized.glasa wool inta •
 the tip of the lower, portion of the pipette.
   9.7.2  Add 2.8g of Waelnt basic alumina
 (previously activated at 600* C, overnight and
 then cooted tO-room temperature in a
 desiccator just prior to use).

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                    Federal Register /  Vol.  48, No. 65 /Monday, April 4,  1983  / Proposed Rules •
                                                                                   14527
   9.8  Elute the microcolumn with 10 ml o.f
 3% methylene chloride-in-hexane followed by
 15 ml of 20% methylene chloride-in-hexane
 and discard these effluents. Elute the column
 with 15'ml of 50% methylene chloride-in-
 hexane and concentrate this effluent [55° C
 water bath, stream of prepurified nitogren) to
 about 0.3-0.5 ml,
-  9.9.   Quantitatively transfer the residue   '
 (using methylene chloride to rinse the
 container) to a silanized Reacti-Vial (Pierce
 Chemical Co.). Evaporate, using a stream of
 prepurified nitrogen, almost to dryness, rinse
 the walls of the vessel with approximately 0.5
 ml methylene chloride, evaporate just to
 dryness, and tightly cap the vial. Store the
 vial at 5°C until analysis, at which time the
 sample is reconstituted by the addition of
 tridecane.                   "
   9.10  Approximately 1 hour before GC—MS
 (HRGC-LRMS) analysis, dilute the residue in
 the micro-reaction vessel with an appropriate
-quantity of tridecane. Gently swirl the
 tridecane on the lower portion of the vessel
 to ensure dissolution of the CDDs and CDFs.
 Analyze a sample by GC/EC to provide
 insight into the complexity of the problem,
 and to determine the manner in which the
 mass spectrometer should be used. Inject an
 appropriate aliquot of'the sample into the
 GC-MS instrument, using a syringe.
   9.11  If, upon preliminary GC-MS analysis,
 the sample appears to contain interfering
 substances which obscure the analyses for
 CDDs and CDFs, high performance liquid
 chromatographic (HPLC) cleanup of the
 extract is accomplished, prior to further GG-
 MS analysis.
 "  10.  HPLC Cleanup Procedure.
   10.1  Place approximately 2 ml of  hexane
 in a 50 ml flint glass sample bottle fitted with
 a Teflon-lined cap.
   10.2  At the appropriate retention time,
 position sample bottle to collect the required
fraction.              '                  ,
  10.3   Add 2 ml of 5% (w/v) sodium
carbonate to the 'sample fraction collected
 and shake for one minute.
  10.4  Quantitatively remove the hexane
layer (top layer) and transfer to a micro-
reaction vessel.
  10.5   Concentrate the fraction to .dryness
and retain for further analysis.
  11.  GC/MS Analysis
  11.1   The following column  conditions are
recommended: Glass capillary column
conditions: SP-2250 coated on a 30 m long X
0.25 mm I.D. glass column (Supelco No. 2--
3714, or equivalent) with helium carrier gas'at
30 cm/sec linear velocity, run splitless.
Column temperature is 210°C. Under these
conditions the retention time for TCDDs is
about 9.5 minutes. Calibrate the system daily
with, a minimum, three injections of standard
mixtures.      ,
  11.2   Calculate response factors for
standards relative to 37C1-TCDD/F (see
Section 12).
  11.3   Analyze samples with selected ion
monitoring of at least two ions from Table 3.
Proof of the presence of CDD or CDF exists if
the following conditions are met;
   11.3.1  The retention time of the peak in
 the sample must match that in the standard,
 within the performance specifications of the
 analytical system.           -   •
   11.3.2  The ratio df ions must_agree within
 10% with that of the standard.
   11.3.3  The retention time of the peak
 maximum for the ions of interest must
 exactly match that of the peak.
   11.4  Quantitate the CDD and CDF peaks
 from the response relative to the 37C1-TCDD/
 F internal standards. Recovery of the internal
: standard should be greater than 50 percent.
   11.5  If a response is obtained for the
 appropriate set of ions, but is outside the   :
 expected ratio, a co-eluting impurity may be
 suspected. In this case, another set of ions  •
" characteristic of the GDD/CDF molecules
 should be analyzed. For TCDD a~good choice •
 of ions is m/e 257 and m/e 259. For TCDF a
 good choice of ions is m/e 241 and 243. These
 ions are useful in .characterizing the
 molecular structure of TCDD or TCDF. For
 analysis of TCDD good analytical technique
 would require using all four ions, m/e 257,
 320, 322, 328, to verify detection and signal to
 noise ratio of 5.to 1. Suspected impurities
 such as DDE, ODD, or PCB residues can be
 confirmed by checking for their major
 fragments. These materials can be removed
 by the cleanup columns. Failure to meet
 criteria should be explained in the report or
 the sample reanalyzed.
   11.6 If broad background interference
 restricts the sensitivity of the GC/MS
 analysis, the analyst should' employ cleanup
^procedures and reanalyze by GC/MS.
 ^11.7.  In those circumstances where these
 procedures do not yield a,definitive ..
 conclusion, the use of high resolution mass
 spectrometry is suggested.
   12.  Calculations               •
   12.1  Determine the concentration of
 individual compounds according to-the
 formula:            --   •  '      '•_'••
     Concentration, ug/gm = •
          A x As

       G x Ais x R{
 Where:   '-    . \
 A=ug of internal standard added to the
     sample.6               '          ;
 G=gm of sample extracted           '
 As=area of characteristic ion of the
     compound being quantified
 Als=area-of characteristic ion of the internal.
     standard;
 Rt=response factor
   Response factors are calculated using data.
     obtained from the analysis of standards •
     accord^S to'the formula:          .   .. .
               'Rf = •
 s x Cte

AisxC,
   6 The proper amount'of standard to be used is  '
 determined from the~calibration curve (See Section
 6.0).         ...
                          Where:    .  /|-...      /            '•..    •'..
                          CjS=concentration of the internal standard
                          C5=concentration of the standard compoun'd
                            12.2  Report results in micrograms per
                          gram without uorrection.for recovery data
                          When duplicate and spiked samples are
                          analyzed, all data obtained should be
                          reported.     :               " '    .
                            12.3  Accuracy and Precision. No data are
                          available at this time^          '           :
                             TABLE 1—Gas Chromatography of TCDD.
Column
Glass Capi
ary. '! ' • '

• Retention
time (rain.)
95

Detection
limit (ug/
kg)'
0.003
                            •Detection limit for liquid samples is 0.003. ug/l. This Is
                          calculated from the minimum detectable GC'.response being
                          equal to five times the GC background noise assuming a I ml.
                          effective final volume of the 1 liter sample.extract; and a GC
                          injection of 5  microliters.  Detection levels apply to  both'
                          electron capture and GC/MS detection. For further details
                          see 44 FR 69526 (December 3, 1979).'   .    .    "   .  '

                               TABLE 2.--DFTPP KEY IONS'AND ION
                                     ABUNDANCE CRITERIA '
                             Mass
                          51	•:.	,
                          68	
                          70	
                          127	
                          197	......:	
                          198	
                          199	:.....;.:
                          275	
                          365.....	.".......,
                          441	„„.„„•	
                          442...',:	
                          443..:.	..-.	
                                              Ion abundance criteria
            30 to 60 percent of mass.198.
            Less than 2 percent of mass 69;
              .Do.
            40; to 60 percent of mass 198.
            Less than 1 percent of mass 198.
            Base peak, 100 percent relative abundance.
            5 'to 9 percent of mass 198.
            Id to 30 percent of mass 198.
            Greater than 1 percent of mass 198.
            Present but less than mass 443....
            Greater than 40 percent" of mass 198.
            17. to 23 percent of mass 442.         '
  >J. W. Bch'elbarger, L. E. Harris, and W. L. Budde. 1975.
Reference compound to -calibrate 'ion abundance measure-
ment in' gas chrpmatography-mass spectrometry. Analytical
Chemistry 47:9951 \      -..   .           ....

TABLE 3.—LIST OF ACCURATE MASSES MONI-
  TORED USING  GC  SELECTED-ION  MONITORT
 " ING, Low RESOLUTION,  MASS SPECTROM-
  ETRY  FOR SIMULTANEOUS DETERMINATION
  OF  TETRA-, PENTA-, AND HEXACHLORINATED
  DiBENZO-p-Dioxins  and Dibenzofurans

CJass of -
chlorinated
dibenzodioxin
or
dibenzofuran


Tetra
.



Penta

Hexa 	 	 	


Number
'of
chlorine
sijbsti-
tuents
(xj


4

_!•*.


, 5

'• .''6


Moni-
tored M/
. z for
dibenzo-
furans
Coc\-


'319.897
'321.894
2327.885
3256.933
=258.930
'353 858
' 355.855
389816
391.813

Moni-
tored m/
z for
dibenzo-'
dioxins


'303 902
321.899



"337863
339.860
373 821
' 375.818
Approxi-
mate
theoreti-
cal ratio
expect-
ed on
Basis of
isotopic
ab'un- .
dance
0 74
1.00

21
-> .20
57
1.00
• 1 00
,. .87
                           1 Molecular ion peak.
                           2Cl4^1abelled sta dard pi
                           3 Ions whict) can
                          confirmation purposi
                  . leaks.          .   ""',_.
               be monitored in TCDD analyses  for*

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 14528
Federal Register / Vol. 48. No.  65 / Monday* April f, 1983 / Proposed  Rules
 PART 264—STANDARDS FOR
 OWNERS AND OPERATORS OF
 HAZARDOUS WASTE TREATMENT,
 STORAGE, AND DISPOSAL
 FACILITIES
   10. The authority citation for Part 264
 reads as follows:
   Authority: Sees, 1006,. 2002la)t 3004, and
 3005 of the Solid Waste Disposal Act. as
 Amended by tho Resource Conservation and
 Recovery Act of 1976, as amended (42 U.S.C.
 6905, 0912;n}, 0024, and 6925).
   11. In Subpart K of Part 264, add: the
 following § 284.231:

 § 264.231  Special requirements for
 hazardous wastes F020, F021, F022, and
 F023.
   (a) Hazardous Wastes F020, F021,   .
 F033, and F023 must not be placed in a
 surface impoundment unless the owner
 or operator operates the- surface
 impoundment in accordance with a
 management plan for these wastes that
 !s approved by the Regional
 Administrator pursuant to- the standards
 set out in this paragraph, and in accord
 with all other applicable requirements of
 this Part. The factors to be considered
 are:
   (1) the volume, physical* and chemical
 characteristics of the wastes,, including
 their potential to migrate through soil or
 to volatilize or escape into the
 atmosphere;
   (2) the attenuative properties of
 underlying and surrounding s"oils or
 other materials;
   (3) the mobilizing properties of other
 materials co-disposed with these
 wastes;
   (4) the effectiveness of additional
 treatment, design, or monitoring
 techniques.
   (b) The Regional Administrator may
 determine that additional design,
 operating, and monitoring requirements
 are necessary for surface impoundments
 managing hazardous wastes F020, F021,
 F022, and F023 in order to reduce the -
 possibility of migration of these wastes
 to ground water, surface "water, or air so
 as to protect human health and the
 environment.
  12. In Subpart L of Part 264, add the
 following § 264.259:

§ 264.259  Special requirements for
hazardous wastes F020, F021, F022, and
F023.
  (a) Hazardous Wastes F020, F021,
F022, and F023 must not be placed in
waste piles that are not enclosed [as
defined in § 284.250(c)l unless the owjier
or operator operates the waste pile in
accordance with a management plan for
these wastes  that is approved by the
Regional Administrator pursuant to the
standards set out in this paragraph, and
                      in accord with, all other applicable
                      requirements of this Part. The factors to
                      be considered are:
                         (1) the volume, physical, and chemical
                      characteristics of the wastes, including
                      their potential to migrate through soil or
                      to volatilize or escape into the
                      atmosphere;
                         [2) the attenuative properties of
                      underlying and surrounding soils, or
                      other materials;
                         (3)' the mobilizing properties of other
                      materials co-disposed with these
                      wastes;
                         (4) the effectiveness of additional
                      treatment, design, or monitoring
                      techniques,
                        (bj The Regional Administrator may
                      determine that additional design,
                      operating, and monitoring requirements
                      are necessary for piles managing
                      hazardous wastes F020, FQ21, F022, and
                      F023 in order to reduce the possibility of
                      migration of these wastes to ground
                      water, surface water, or air so as to
                      protect human: health and the
                      environment
                        13^ In Subpart M of Part 26.4, add the
                      following § 264.283:

                      § 264.283 Special requirements for
                      hazardous wastes F020, F021, F022,and
                      F023.
                        (a} Hazardous wastes F020j F021,
                      F022, and F023 must not be placed hi a
                      land treatment facility unless the owner
                      or operator operates the facility in
                      accordance with a management plan for
                      these wastes, that is approved by the
                      Regional Administrator pursuant to the
                      standards set out hi this paragraph, and
                      in accord witkall other applicable
                      requirements of the Part. The factors to-
                      be considered are:
                        (1) the volume, physical, and chemical
                      characteristics of the wastes, including
                      thek potential to migrate through soil or
                      to volatilize or escape into the
                      atmosphere;
                        (2) the attenuative properties of
                      underlying and surrounding soils or
                      other materials;
                        (3) the mobilizing properties of other
                      materials co-disposed with these
                      wastes;
                        (4) the effectiveness of additional
                      treatment, design, or monitoring
                      techniques.
                        (b) The Regional Administrator may
                      determine that additional design,
                      operating, and monitoring requirements
                      are necessary for land treatment
                      facilities managing hazardous wastes
                      F020, F021, F022, and F023 in order to
                      reduce the possibility of migration of
                      these wastes to ground water, surface
                      water, or air so as  to protect human
                      health and the environment.
    14.. In Subpart N of Part 264, add the
  following § 264.317:

  §264.317  Special requirements for
  hazardous wastes F020, F021, F022, and
  F023.
    fa) Hazardous wastes F020, F021,
  F022, and F023 must not be placed in
  landfills unless the; owner or operator
  operates the landfill in accordance with
  a management plan for these wastes
  that is approved by the Regional
  Administrator pursuant to the standards-
  set out in this paragraph, and in accord
  with all other applicable requirements of
  this Part. The factors to be considered  .
  are:
    PL) the volume, physical, and chemical
  characteristics of the wastes, including
  their potential" to migrate through the
  soil or to volatilize or escape into the
  atmosphere;
    (2) tha attenuative properties of
  underlying and surrounding soils or
  other materials;
    (3} the mobilizing properties of other
  materials co-disposed with these
  wastes;
    [4] the effectiveness of additional
  treatment, design, or monitoring
  requirements.
    [b) The Regional Administrator, may
  determine that additional design^
*" operating, and monitoring requirements,
  are necessary for landfills managing
  hazardous wastes F020,.FQ21-, F022, and
  F023 in order to reduce the possibility of
  migration of these wastes, to ground
  water,  surface water, or air so as to
  protect human health and the
  environment.'

  PART 265—INTERIM STANDARDS
  FOR OWNERS AND OPERATORSOF
  HAZARDOUS WASTE TREATMENT,
  STORAGE, AND DISPOSAL
  FACILITIES

   15. The authority citation for Part 265
  reads as.follows:
   Authority: Seca. 1006, 2Q02(a), 300,4, and
  3005 of the Solid Waste Disposal Act, as
 ' amended by the  Resource Conservation, and
 Recovery Act of 1976, aa amended (42 UJS.C., •
 6905, 6S12(a), 6924, and 6925). -

   16.. § 265.1" ia amended by adding
 paragraph (d).

 § 2S5.1  Purpose, scope and applicability.
  *    *     *     *   *  r

   (d) The following hazardous wastes
 must not be managed at facilities
 subject tcr regulation under this Part.
   (1) EPA Hazardous Waste Nos. F020,
 F021, F022, and.F023 unless:
   (i) The waste is generated in a surface .
 impoundment as part of the plant's
 wastewater treatment  system.

-------
                  Federal Register  /  Vol. 48, No.  65 /Monday, April 4,  1983 / Proposed Rules
14529
 , (ii) The waste is stored in tanks or
 containers.
   (in) The waste is stored or treated in
 waste piles that meet the requirements
 of § 264.250(0)" as well as all other
 applicable requirements of Subpart L of
 this Part. "      -

 PART 775 [REMOVED]

,17. The authority citation for Part 775
 jeads as follows:  .      •
   Authority. Sec.  6 of the Toxic Substances  .
 Control Act (TSCA) Pub. L. 94-469, 90 Stat.
 2020 [15 U.S.C. 2605].
   18. Title 40 is  amended by removing
 Part 775. .-•••'
 [FR Doc. 83-7930 Filed 4-1-83; 8:45 am]
 BILLING CODE 6560-50-M

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