EPA744-F-01-001
February 2001
ur
Design for the Environment
Gravure Partnership
The  Effect of  Ink Temperature
On  Solvent  Losses  and  Print  Quality
GAA
  WESTERN
  MICHIGAN
  UNIVERSITY
    U.S. EPA
Background—The U.S. Environmental
Protection Agency's (EPA) Design for the
Environment (DIE) Program, the University of
Tennessee (UT) Center for Clean Products
and Clean Technologies, and Western
Michigan University (WMU) partnered with
the Gravure Association of America (GAA),
gravure printers from the packaging and prod-
uct sectors, and other industry experts to iden-
tify  1) common environmental issues for
gravure printers, especially small- and medi-
um-sized businesses in the packaging and
product sectors; and 2) potential risk reduction
and pollution prevention opportunities for
addressing key issues.
    Packaging and product gravure printers are
particularly concerned about solvent losses
from ink during press operations—including
solvent losses from the ink sump and ink pan
areas—which might be reduced by controlling
ink temperatures.  Smaller gravure printing
operations generally use a press-side sump  to
pump ink to the press, where the ink may
                      absorb heat from
    U.S. Gravure Industry Statistics
Sector
Publication*
Packaging
Product
Total
Avg. employees
Annual sales ($/
#of plants
24
276
174
480
per plant**
'yr)**
Avg. presses
per plant
6.3
2.5
2.8
2.8
<20
>$18 billion
    Data from 1987-1993 (GAA Profile Survey of the U.S. Gravure
    Industry).
    * 2000 data from GAA.
    "Data for publication, packaging and product combined.
                      the ambient air or
                      from press opera-
                      tions. Large publi-
                      cation printers
                      generally have in-
                      line heat exchang-
                      ers and closed-
                      loop ink delivery
                      systems, which are
                      not  as subject to
                      solvent losses from
                      elevated ink tem-
                      peratures. The
                      Gravure Partner-
                      ship performed a
                      preliminary study
                      of the effect of ink
temperature on solvent losses and print quality,
which is summarized below. The results sug-
gest that packaging and product printers could
reduce solvent losses, and, in some cases,
improve print quality by controlling ink tem-
peratures. Further study by the industry is
needed to confirm these results.
Gravure Industry Statistics—The gravure
industry comprises three main sectors: publica-
tion, packaging, and product printing.
Publication gravure plants are generally large
operations that tend to be more automated,
with more advanced systems for addressing
environmental concerns. Packaging and prod-
uct gravure plants are often small- to medium-
sized printing facilities with fewer employees,
fewer presses, and more limited resources.
Risk Reduction Opportunities—The partner-
ship began with a scoping phase to identify
potential opportunities for packaging and
product printers to reduce emissions and risk
from printing operations. Project partners  con-
sulted with GAA and industry experts to
develop a preliminary list of risk reduction
opportunities (see box, page 2), which were
then verified through site visits to gravure
printers in the packaging and product sectors.
DfE project leaders chose to study the effect of
ink temperature on VOC emissions and print-
ability for the following reasons:
•  Ink temperature's effect on solvent losses
   and print quality are common problems
   among various packaging and product
   printers, in spite of different inks, number
   of colors,  and substrate.
•  By controlling ink  temperature, printers
   might gain print quality and cost benefits
   as well as environmental benefits.

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   Emissions from the ink sump and ink pan areas are
   not always captured by air pollution control equip-
   ment attached to presses.
   Reduction in the use of hazardous air pollutants
   (HAPs) and VOCs could  reduce adverse impacts on
   human health and the environment (due to direct tox-
   icity from HAPs and indirect effects of smog forma-
   tion from VOCs).
Risk Reduction Opportunities
Risk reduction opportunities identified by the DfE
Gravure Partnership include:
•  Volatile organic compound (VOQ/solvent emis-
   sions reduction
   - from floor cleaning
   - from press operations
•  Hazardous waste generation
•  Shop towel management

WMU Temperature Control Study
The WMU laboratory experiment met key objec-
tives of the DfE Gravure Partnership by:
•  Developing information on the effects of ink
   temperature on solvent consumption and print
   quality.
•  Determining that technologies to moderate or
   control ink temperatures are a worthy subject
   for further investigation by the industry.
Study Parameters
Controlled conditions
Press size:
Press speed:
Substrate:
Run length:
Ink type:
Solvent blend:
Initial ink vol.:
42" wide, 4-color press
300 ft/min
1.25 mil polyethylene film
3-hour production run
(samples taken every 20
minutes)
Type C (nitrocellulose),
magenta and cyan
50% n-propyl acetate,
50% n-propyl alcohol (by
volume)
60 Ib (solvent + ink)
Variable conditions
(average ink temperature)
66°F (cooled with cold water and ice)
79°F (ambient)
92°F (heated with hot water)
Measurements taken
Viscosity (adjusted every 5 minutes)
Solvent consumption
Ink consumption
Printability
•  Optical density
•  Gloss
•  Microstructure image analysis (dot
   structure)
•  Tonal response
•  Rub resistance (Sutherland Ink Rub
   Tester)
Gravure Partnership Purpose—The purpose of the DfE
Gravure Partnership was to 1) identify risk reduction and
pollution prevention opportunities for addressing key envi-
ronmental challenges in the gravure industry, 2) determine
whether promising risk reduction techniques might also
have cost and/or performance benefits, and 3) provide the
risk, performance, and cost data to the gravure industry for
further technology verification.
    Following scoping, a laboratory experiment was con-
ducted at WMU's Printing Pilot Plant to explore the rela-
tionships between ink temperatures, solvent losses,  and
print quality (Sosa, 1999). The results of the WMU tem-
perature control study, presented here, provide preliminary
information to the industry on the potential risk, perform-
ance, and cost benefits of ink temperature controls.


Temperature Control Study
Purpose
    The purpose of the preliminary laboratory study was to
evaluate the effects of temperature on solvent consumption
and print quality.
Method
    Two colors of nitrocellulose  (Type C) ink common to
packaging printers were used in 3-hour production runs on
a 42",  4-color gravure press at 300 ft/min. Type C  inks are
generally ester or ketone inks. The solvent blend used in
the temperature experiment was 50% normal propyl
acetate and 50% normal propyl alcohol  (by volume).
Samples were taken  for the two  inks at three different ink
                  temperatures: 66°F, 79°F, and 92°F.
                  The  cooler temperature was obtained by
                  using cold water and  ice to cool water
                  circulating through copper coils sub-
                  merged in the ink sump. The warmer
                  temperature was obtained by circulating
                  hot tap water through the copper coils.
                  No temperature controls were used for
                  the middle (ambient) temperature,
                  which increased by 3°F to 5°F during
                  the course of the 3-hour run.
                     During the runs, ink temperature
                  was measured and viscosity was  tested
                  and adjusted every 5 minutes. Print
                  quality measurements were taken every
                  20 minutes. Several measures of print-
                  ability were obtained. (See Study
                  Parameters Box.)
                              Gravure Partnership

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Solvent and Ink Consumption Results
   Colder ink needs more solvent to bring it to target
viscosity, but as temperature rises, the solvents in sol-
vent-based inks evaporate faster and require more sol-
vent to maintain viscosity (Sosa, 1999).
•  Total solvent consumption (solvent added during
   makeready plus solvent added during the print run)
   in the magenta ink increased with increasing tem-
   perature  (see Figure 1).
•  Total solvent consumption in the cyan ink was slight-
   ly greater at 66°F than 79°F due to the amount of
   solvent needed to reach target viscosity during make-
   ready Solvent consumption increased from 79°F to
   92°F (see Figure 1).
•  Total mass (ink plus solvent) consumption
   increased with increasing temperature: 9%-28%
   increase from 66°F to 79°F and 37%-56% increase
   from 79°F to 92°F.
•  Ink use (not including solvent added during make-
   ready or  the trial) also increased as temperature rose
   (see Figure 2). The increase in ink consumption at
   higher temperatures may be due to the higher pig-
   ment to solvent ratio  of warmer ink, which prints a
   thicker layer.
 Print Quality Results
   In the WMU study, printability and quality were
affected as ink temperature increased, with both print-
ed solids and tones affected (Sosa, 1999).
•  Reflection Density—dropped by 0.055% of reflected
   light for  every 5°F  temperature increase from 79°F
   to 92°F (see Figure 3). Theoretically, ink at higher
   temperatures should print darker colors, but
   reduced reflection densities at higher ink temper-
   atures have been reported elsewhere (Celio, 1998).
   Warmer inks evaporate faster, which can cause a
   wettability problem and screening. Screening is a
   print defect caused by uneven flow of inks between
   cells (GAA, 1991). In the WMU study, as ink tem-
   perature  rose to 92°F the ink dried before spread-
   ing adequately  on the substrate, thus reducing the
   overall printed  solid area and the reflection density
   (Sosa, 1999). Printed tone steps were most affected;
   the finest dots did not print at all.
•  Specular gloss—decreased by 20% from 66°F  to
   79°F, but increased by 3% from 79°F to 92°F (see
   Figure 4). Colder ink requires more solvent to reach
   target viscosity; lower pigment concentration leads
   to a thinner printed ink film. In the WMU study,
   the specular gloss measurements for the colder ink
Total Solvent Consumption
          12
                                                     Figure 1
    o
    Vj
    Q.
                         Magenta
                         Cyan
            -   3.5
                                   79°F
                             Ink Temperature
                                               92°F
Ink Consumption
                                                         Figure 2
    o
    c_3
                                                     7.E
                         Magenta
                         Cyan
                     4.5
Print Quality

          2.1

          2.0
          1.9
          1.8
          1.7
          1.6
          1.5
en
cc
                  66°F            79°F
                              Ink Temperature
             Reflection Density

                2.05
                                              92°F
                                                     Figure 3
                                   79°F
                              Ink Temperature
                                               92°F

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were influenced by the glossy polyethylene
substrate showing through the thinner ink
film. The increase in specular gloss seen
from 79°F to 92°F may be due to the
decreased wettability and increased screen-
ing observed at higher temperatures.
Screening may have caused more light to be
reflected from the polyethylene substrate.
Dot structure (see Figures  5 and 6)—hot
inks had deformed dot structure caused by
the "donut effect." As  ink fills the engraved
cells of a printing cylinder, it forms a con-
cave shape leaving an air bubble to be
trapped between the ink and the substrate.
The air prevents the ink from being trans-
ferred to the middle of the printed dot and
forces the ink to be spread outward, creating
a "donut." Warmer, less viscous ink pro-
duces a bigger concave meniscus as it lies in
the cylinder cells,  which results in more air
being trapped and a larger donut.  As  the
donut effect increases with temperature, the
amount of printed image decreases and the
printed dot becomes bigger (Sosa, 1999).
Deformed dots caused by the donut effect
also had bigger perimeters. As the dot
perimeter increases so  do the dot gain and
mottle,  causing a decrease in print quality.
Finally,  photographs taken in the solids
areas confirmed the reduced wettability of
the hotter ink; the white, non-printed areas
of the solids rose with increasing ink tem-
perature.
Haze—not a quantifiable variable  in the
WMU study, but  appeared to increase with
decreasing temperature. Decreasing efflux
time and/or doctor  blade pressure may
reduce haze.
Rub resistance—no change in rub resistance
at different temperatures. A Sutherland ink
rub tester was used to  rub the printed films
against a white surface for a specific amount
of time. The reflection density of the white
surface was measured before and after the
test to determine the amount of ink trans-
ferred from the printed film to the surface.
The difference in  the reflection densities of
the hottest temperature and the coldest tem-
perature inks  were within the resolution of
the densitometer.
Print Quality — Specular Gloss

         80 f   _73.5
         70
         60
    _   50
    ^o
    I   4°
    ^    30
    _ro
    §    20
    %   10
                                                    Figure 4
                                                Cyan
                                  79°F
                             Ink Temperature
                                                 92°F
Magenta elongated tone (25%)
        — 150 lines per inch
                                                    Figure 5

                                              y  9  9
           *  *   •  *
         **••*
               79°F
Cyan compressed tone (25%)
        — 150 lines per inch
       «  •  *
              79°F
Magenta solid —150 lines per inch
                                             92°F
                                                    Figure 6
                                             « V  <
                                          
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Conclusions
   The WMU study assessed the effects of
three ink temperatures (66°F, 79°F, and
92°F) on solvent consumption and print
quality of Type C inks under laboratory-con-
trolled conditions. The study was designed to
provide preliminary data on the potential
benefits of ink temperature controls to the
gravure industry for further technology verifi-
cation (see box on Study Limitations). The
results are promising.
•  Small- and medium-sized printers in the
   product and packaging sector may be able
   to reduce solvent consumption, improve
   print quality, and achieve cost reductions
   by implementing ink temperature con-
   trols.
•  Decreasing solvent consumption and sol-
   vent emissions could also reduce health
   risks because of reductions  in potential
   exposures to workers or the public.
•  The greatest benefits may occur when  ink
   temperature is maintained near a typical
   room temperature  rather than chilled to
   below typical room temperatures,  suggest-
   ing less chilling is needed to achieve opti-
   mal results.
Study Limitations
•  The WMU laboratory study was designed to evaluate the potential risk, perform-
   ance, and cost benefits of ink temperature controls for gravure printers. The
   study does not establish a definitive relationship between ink temperature, sol-
   vent emissions, and print quality.
•  The study evaluated the effects of ink temperature on Type C inks only. Results
   may differ with other ink types.
•  The range of test temperatures (66°F to 92°F) was selected to  represent the
   extreme of printing conditions that might be encountered in the industry. Smaller
   printers may have ink temperatures approaching the upper  limit in the summer
   months, but these higher temperatures are  not typical of year-round operating
   practices.
•  Many ink and solvent systems used in packaging and product gravure have an
   affinity for pressroom air moisture, particularly at low temperatures. Moisture
   pickup due to low ink temperature can cause blushing and ink kick-out. The
   study did not directly assess the moisture pickup of the colder inks, but no blush-
   ing and ink kick-out effects were seen.

Potential  Cost Savings
Parameter

Solvent emissions (Ib/yr)
Ink consumption (Ib/yr)
Annual solvent costs
Annual ink costs
Scenario 1

113,400
97,200
$56,700
$388,800
Scenario 2

86,400
86,400
$43,200
$345,600
Reductions
or savings
27,000
10,800
$13,500
$43,200
                                               Solvent & ink costs
                              $445,500
$388,800
$56,700
•  Ink temperature controls might also reduce
   overall ink consumption (up to 20%-30%)
   without adversely affecting print quality, but these
   results need to be confirmed on different substrates
   and in "real world" settings.
•  Ink temperature controls can also be expected to
   reduce solvent use (perhaps up to 50%), especially in
   the summer months  when ambient temperatures are
   higher.
Potential Cost Savings—Potential savings were estimat-
ed for two scenarios using the assumptions of the model
facility (see box at right) and the solvent and ink con-
sumption results  from the WMU study. Scenario 1
assumes a small printer operates at 92°F for three
months and 79°F for nine months a year. Scenario 2
assumes the printer implements temperature controls to
maintain a constant temperature of 79°F all year.
   Conditions will vary greatly by facility; many other
factors may also affect these estimates. Nonetheless, they
provide a starting point  for companies to estimate their
                         Example Model Facility
                         Press size:               23" wide
                         Printing units:            3
                         Annual operation time:     7200 hr/yr
                         Press speed:             300 ft/min
                         Solvent use rate:         9 Ib/hr at 92°F
                           (per color):             4 Ib/hr at 79°F
                         Ink use rate:             6 Ib/hr at 92°F
                           (per color):             4 Ib/hr at 79°F
                         Solvent cost:             $0.50/lb
                         Ink cost:                $4.00/lb

           own potential savings. Although these estimates do not
           account for the cost of cooling, any cooling solution and
           associated energy requirements that cost less than the
           estimated savings above could  result in payback after the
           first year.
           Industry Challenge—The results of the DfE Gravure
           Partnership suggest ink temperature controls may present

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 gravure printers with an excellent opportunity to prevent
 pollution at the source, while improving print quality
 and reducing costs. Small- and medium-sized printers
 that experience printing inefficiencies due to fluctuations
 in ink temperatures may benefit most from ink tempera-
 ture controls, but no  clear or commonly implemented
 solutions for addressing  these inefficiencies yet exist. The
 DfE Gravure Partnership challenges the industry to con-
 firm project findings  to  optimize printing operations. To
 meet  this challenge, gravure printers could:
 •   Independently evaluate the effects of ink temperature
     on solvent and ink consumption, print quality and
     cost.
 •   Assess and/or optimize current ink temperature  con-
     trol options, including
     - Submerged copper coils in the ink sump, including
      the cost and pollution implications of frequent
      cleaning.
     - In-line heat exchangers on the supply line.
     - Room temperature control  (air conditioning).
 •   Adapt a temperature control  option  from another
     industry.
 •   Develop a new, innovative method for controlling ink
     temperatures.
   Questions to consider when evaluating the use of
temperature control in a printing facility include:
•  How will less solvent consumption affect treatment
   systems such as oxidizers and recovery systems?
•  What is the cost of adding temperature controls on
   press and providing cooling water?
•  How do different colors and ink types behave, noting
   that in this study the two Type  C inks behaved differ-
   ently?
References
Celio, Tino (1998). Ink Temperature Control in Gravure
   Printing. Ambril, Swtizerland: Paper presented at the
   annual meeting of the Gravure Association of
   America conference, Memphis, TN.
GAA (1991).  Tone Reproduction. Gravure, Rochester, NY.
Sosa, Rodrigo (1999). Effects of Temperature Control on
   Gravure Packaging Ink: A Thesis Submitted to the
   Faculty of the Graduate College in partial fulfillment
   of the requirements for the Degree of Paper and
   Imaging Science, Western Michigan University,
   Kalamazoo, MI.
What is EPA's Design for the Environment
Program?
EPA's Design for the Environment (DfE) Program partners with stake-
holders to help businesses help the environment. DfE projects help
businesses design products, processes, and management systems
that are cost-effective, cleaner, and safer for workers and the public.
The DfE goals are to:
•  Encourage businesses to incorporate environmental information
   into their decision criteria.
•  Effect behavior change to facilitate continuous environmental
   improvement.
To accomplish these goals, DfE and its partners use several
approaches including cleaner technology and life-cycle assessments,
environmental management systems, formulation improvement, best
practices, and green supply chain initiatives.
To date, the DfE Program has brought environmental leadership to
over 2 million workers at over 170,000 facilities. Small- and medi-
um-sized businesses recognize DfE as a unique source of reliable
environmental (as well as performance and cost) information that
allows them to make better decisions.
How Can I Get More Information?
To learn more about EPA's DfE Program or the Gravure Partnership,
contact:

EPA's DfE Program
Phone:202-260-1678
Web site: www. epa.gov/dfe

The Gravure Association of America
Phone:716-436-2150
Fax:716-436-7689

UT Center for Clean Products and Clean Technologies
Phone: 865-974-9526
E-mail: socolofml@utk.edu

Rodrigo Sosa, RJR  Packaging (formerly of WMU)
Phone:336-741-4974
E-mail: sosar@rjrt.com

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