United States
Environmental Protection
Agency
Office of Water
Engineering and Analysis Division (4303)
Washington, DC 20460
EPA821-B-94-005
October 1994
Revision B
Method 1613: Tetra-Through Octa-
Chlorinated Dioxins and Furans by
Isotope Dilution HRGC/HRMS
                                    > Printed on Recycled Paper

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                     Acknowledgments


This method was prepared under the direction of William A. Telliard of the
   Engineering and Analysis Division within the EPA Office of Water.
   This document was prepared under EPA Contract No. 68-C3-0337 by
       DynCorp Environmental Services Division with assistance
                  from its subcontractor Interface, Inc.
                           Disclaimer

This method has been reviewed by the Engineering and Analysis Division,
   U.S. Environmental Protection Agency, and approved for publication.
        Mention of trade names or commercial products does not
           constitute endorsement or recommendation for use.

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 Introduction
   i

 Method 1613 was developed by the United States Environmental Protection Agency's Office of
 Science and Technology for isomer-specific determination of the 2,3,7,8-substituted, tetra- through
 octa-chlorinated, dibenzo-p-dioxins and dibenzofurans in aqueous, solid, and tissue matrices by isotope
   ution, high resolution capillary column gas chromatography (HRGQ/high resolution mass spectrom-
di
 etry (HRMS).
   i
 Qi|estions concerning this method or its application should be addressed to:

 W-A. Telliard
 US EPA Office of Water                                            '
 Analytical Methods Staff                                            j
 Mail Code 4303
 40 j M Street, SW
 Washington, D.C. 20460                                             ''
 202/260-7120
Requests for additional copies should be directed to:
   i  ,
Water Resource Center
Ma'il Code RC-4100
401 M Street, SW
Washington, D.C. 20460
202/260-7786 or 202/260-2814

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                       Method  1613,  Revision  B
             Tetra- through  Octa-Chlorinated Dioxins and Furans
                         by Isotope Dilution HRGC/HRMS
1.0  Scope and Application
 1.1  This method is for determination of tetra- through octa-chlorinated dibenzo-p-dioxins (CDDs)
      and dibenzofurans (CDFs) in water, soil, sediment, sludge, tissue, and other sample matrices by
      high resolution gas chromatography/high resolution mass spectrometry (HRGC/HRMS). The
      method is for use in EPA's data gathering and monitoring programs associated with the Clean
      Water Act, the Resource Conservation and Recovery Act, the Comprehensive Environmental
      Response, Compensation  and Liability Act, and the Safe Drinking Water Act. The. method is
      based on a compilation of EPA, industry, commercial laboratory, and academic methods
      (References  1-6).
 1.2  The seventeen 2,3,7,8-substituted CDDs/CDFs listed in Table 1  may be determined by this
      method. Specifications are also provided for separate determination of 2,3,7,8-tetrachloro-
      dibenzo-p-dioxin (2,3,7,8-TCDD) and 2,3,7,8-tetrachloro-dibenzofuran (2,3,7,8-TCDF).
 1.3  The detection limits and quantitation levels in this method are usually dependent on the level of
      interferences rather than instrumental limitations. The minimum levels (MLs) in Table 2 are the
      levels at which the CDDs/CDFs can be determined with no interferences present. The Method
      Detection Limit (MDL) for 2,3,7,8-TCDD has been determined  as 4.4 pg/L (parts-per-
      quadrillion)  using this method.
  1.4  The GC/MS portions of this  method are for use only by analysts experienced with HRGC/HRMS
      or under the close supervision of such qualified persons. Each laboratory that uses this method
      must demonstrate the ability to generate acceptable results using the procedure in Section 9.2.
  1.5  This method is "performance-based". The analyst is permitted to modify the method to overcome
       interferences or lower the cost of measurements, provided that all performance criteria in this
       method are  met. The requirements for establishing method equivalency are given in Section
       9.1.2.
  1.6   Any modification of this method, beyond those expressly permitted, shall  be considered a major
       modification subject to application and approval of alternate test procedures under 40 CFR 136.4
       and 136.5.

 2.0   Summary of Method
       Flow charts that summarize procedures for sample preparation, extraction, and analysis are given
       in Figure 1  for aqueous  and solid samples, Figure 2 for multi-phase samples, and Figure 3 for
       tissue samples.

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Method 1613
2.1
2.2
2.3
Extraction                                                         ;
  2.1.1   Aqueous samples (samples containing less than one percent solids)—Stable isotopically
        labeled analogs of 15 of the 2,3,7,8-substituted CDDs/CDFs are  spiked into a one-liter
        sample, and the sample is extracted by one of three procedures;
       2.1.1.1  Samples containing no visible particles are extracted with rnethylene chloride in a
               separatory funnel or by the solid-phase extraction technique summarized in
               Section 2.1.1.3. The extract is concentrated for cleanup.
       2.1.1.2  Samples containing visible particles are vacuum filtered through a glass-fiber
               filter. The filter is extracted in a Soxhlet/Dean-Stark (SDS) extractor (Reference
               7), and the filtrate is extracted with methylene chloride ;in a separatory funnel.
               The  methylene chloride extract is concentrated and  combined with the SDS
               extract prior to cleanup.
       2.1.1.3  The  sample is vacuum filtered through a glass-fiber filter on top of a solid-phase
               extraction (SPE) disk. The filter and disk are extracted in an SDS extractor,  and
               the extract is concentrated for cleanup.
  2.1.2   Solid, semi-solid, and multi-phase samples (but not tissue)—The labeled compounds are
        spiked  into  a sample containing 10 g (dry weight) of solids. Samples containing multiple
        phases  are pressure filtered and any aqueous liquid is discarded.  Coarse solids are ground
        or homogenized. Any non-aqueous liquid from multi-phase samples is combined with the
        solids and extracted in an SDS extractor. The extract is concentrated for cleanup.
  2.1.3   Fish and other tissue—The sample is extracted by one of two procedures:
       2.1.3.1  Soxhlet or SDS extraction—A 20-g aliquot of sample is homogenized, and a 10-g
               aliquot is spiked with the labeled compounds. The sample is mixed with sodium
               sulfate, allowed to dry for 12 - 24 hours, and extracted for 18-24 hours  using
               methylene chloride:hexane (1:1) in a Soxhlet extractor. The extract is evaporated
               to dry ness, and the lipid content is determined.        i
       2.1.3.2  HC1  digestion—A 20-g aliquot is homogenized, and a  10-g aliquot is placed in a
               bottle and spiked with the labeled compounds. After equilibration, 200 mL of
               hydrochloric acid and 200 mL of methylene chloride:hexane (1:1) are added, and
               the bottle  is agitated for 12-24 hours. The extract is evaporated to dryness, and
               the lipid content is determined.
After extraction, 37Q4-labeled 2,3,7,8-TCDD is added to each extract to measure the efficiency of
the cleanup process. Sample  cleanups may include back-extraction  with acid and/or base, and gel
permeation, alumina, silica gel, Florisil and activated  carbon chromatography. High-performance
liquid chromatography (HPLC) can be used for further isolation of the 2,3,7,8- isomers or other
specific isomers or congeners. Prior to the cleanup procedures cited above, tissue extracts are
cleaned up using an anthropogenic isolation column, a batch silica  gel adsorption, or sulfuric
acid and base back-extraction, depending  on the tissue extraction procedure used.
After cleanup,  the extract is concentrated  to near dryness. Immediately prior to injection, internal
standards are added  to each extract, and an aliquot of the extract is injescted into the gas

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                                                                                      Method 1613
        chromatograph. The analytes are separated by the GC and detected by a high-resolution
        (£10,000) mass spectrometer. Two exact m/z's are monitored for each analyte.
  2.4   An individual CDD/CDF is identified by comparing the GC retention time and ion-abundance
        ratio of two exact m/z's with the corresponding retention time of an authentic standard and the
        theoretical or acquired ion-abundance ratio of the two exact m/z's. The non-2,3,7,8 substituted
        isomers and congeners are  identified when retention times and ion-abundance ratios agree within
        predefined limits. Isomer specificity for 2,3,7,8-TCDD and 2,3,7,8-TCDF is achieved using GC
        columns that resolve these  isomers from the other tetra-isomers.
  2.5   Quantitative analysis is performed using selected ion current profile (SICP) areas, in one of three
        ways:
        2.5.1  For the fifteen 2,3,7,8-substituted CDDs/CDFs with labeled  analogs (see Table 1), the
              GC/MS system is calibrated, and the concentration of each compound is determined
              using the isotope dilution technique.
        2.5.2  For 1,2,3,7,8,9-HxCDD, QCDF, and the labeled compounds, the GC/MS  system is
              calibrated and the concentration of each compound is determined using the internal
              standard technique.
        2.5.3  For non-2,3,7,8-substituted isomers and for all isomers at a given level of chlorination
              (i.e., total TCDD), concentrations are determined using response factors from calibration
              of the CDDs/CDFs  at the same level of chlorination.
  2.6   The quality of the analysis is assured through reproducible calibration and  testing of the
       extraction, cleanup, and GC/MS systems.

3.0   Definitions
  Definitions are given in the glossary at the end of this method.

4.0   Contamination and Interferences

  4.1   Solvents, reagents, glassware, and other sample processing hardware may yield artifacts and/or
       elevated baselines causing misinterpretation of chromatograms (References 8-9). Specific
       selection of reagents and purification of solvents by distillation in  all-glass  systems may be
       required. Where possible, reagents are cleaned  by extraction or solvent rinse.
  4.2   Proper cleaning of glassware is extremely important, because glassware may not only
       contaminate the samples but may also remove the analytes of interest by adsorption on the glass
       surface.
        4.2.1  Glassware should be rinsed with solvent and washed with a detergent solution as soon
             after use as is practical. Sonication of glassware containing a detergent solution for
             approximately 30 seconds may aid in cleaning. Glassware with removable parts,
             particularly separatory funnels with fluoropolymer stopcocks, must be disassembled prior
             to detergent washing.

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   Method 1613
  4.$
 4.4
4.5i
4.61
    4.2.2  After detergent washing, glassware should be rinsed immediately, first with methanol
          then with hot tap water. The tap water rinse is followed by .another methanol rinse then
          acetone, and then methylene chloride.                     ;
    4.2.3  Do  not bake reusable glassware in an oven as a routine part of cleaning. Baking may be
          warranted after particularly dirty samples are encountered but should be minimized as
          repeated baking of glassware may cause active sites on the  glass surface that will  '
          irreversibly adsorb CDDs/CDFs.
    4.2.4  Immediately prior to use, the Soxhlet apparatus should be pre-extracted with toluene for
          approximately 3 hours (see Sections 12.3.1-12.3.3). Separatoty funnels should be shaken
          with methylene  chloride/toluene (80/20 mixture) for 2 minutes, drained, and then shaken
          with pure methylene chloride for 2 minutes.
  All materials used in the analysis shall be demonstrated to be free from interferences by running
  reference matrix method blanks initially and with each sample batch (samples started through the
  extraction process on a given 12-hour shift, to a maximum of 20 samples).
   4.3.1  The  reference matrix must simulate, as closely as possible, the sample matrix under test
         Ideally, the reference matrix should not contain the CDDs/CDFs in detectable amounts
         but should contain potential interferents in the concentrations expected to be found in the
         samples to be analyzed. For example,  a reference  sample of  human adipose tissue
         containing pentachloronaphthalene can be used to exercise the cleanup systems when
         samples containing pentachloronaphthalene are expected.
  4.3.2  When a reference matrix that simulates the sample matrix under test is not available
         reagent water (Section 7.6.1) can be used to simulate water samples; playground sand
         (Section 7.6.2) or white quartz sand (Section 7.3.2) can be used to simulate soils; filter
         paper (Section 7.6.3) can be used to simulate papers and similar materials;  and corn oil
         (Section 7.6.4) can be used to simulate tissues.
 Interferences  coextracted from samples will vary considerably from source to source, depending
 on the diversity of the site being sampled. Interfering compounds may be present at
 concentrations several orders of magnitude higher than the CDDs/CDFs. The most  frequently
 encountered interferences are chlorinated biphenyls, methoxy biphenyls, hydroxydiphenyl ethers
 benzylphenyl  ethers, polynuclear aromatics, and pesticides. Because very low levels of
 CDDs/CDFs  are measured by this method, the elimination of interferences is essential. The
 cleanup steps  given in Section 13 can be used  to reduce or eliminate  these interferences and
 thereby permit reliable determination of the CDDs/CDFs at the levels shown in Table 2.
 Each piece of reusable glassware should be numbered to associate that glassware with the
 processing of a particular sample. This will assist the laboratory in tracking possible sources of
 contamination for individual samples, identifying glassware associated with highly contaminated
 samples that may require extra cleaning, and determining when glassware should be discarded.
Cleanup of tissue—The natural lipid content of tissue can interfere in  the analysis of tissue
samples for the CDDs/CDFs.  The lipid contents of different species and portions of tissue can
vary widely. Lipids are soluble to varying degrees in various  organic  solvents and may be
present in sufficient quantity to overwhelm the  column chromatographic cleanup procedures  used

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                                                                                       Method 1613
       for cleanup of sample extracts. Lipids must be removed by the lipid removal procedures in
       Section  13.7, followed by alumina (Section 13.4) or Florisil (Section 13.8), and carbon (Section
       13.5) as minimum additional cleanup steps. If chlorodiphenyl ethers are detected, as indicated by
       the presence of peaks at the exact m/z's monitored for these interferents, alumina and/or Florisil
       cleanup  must be employed to eliminate these interferences.

5.0   Safety

 5.1   The toxicity or carcinogenicity of each compound or reagent used in this method has not been
       precisely determined; however, each chemical compound should be treated as a potential health
       hazard. Exposure to these compounds should be reduced to the lowest possible level.
        5.1.1 The 2,3,7,8-TCDD isomer has been found to be acnegenic, carcinogenic, and teratogenic
             in laboratory animal studies. It is soluble in water to approximately 200 ppt and in
             organic solvents to 0.14%. On the basis  of the available toxicological and physical
             properties of 2,3,7,8-TCDD,  all of the CDDs/CDFs should be handled only by highly
             trained personnel  thoroughly familiar with handling and cautionary procedures and the
             associated risks.
        5.1,2 It is recommended that the laboratory purchase dilute standard solutions of the analytes
             in this method.  However, if primary solutions are prepared, they shall be prepared in a
             hood, and a NIOSH/MESA approved toxic gas respirator shall be worn when high
             concentrations are handled.
 5.2  The laboratory is responsible for maintaining a current awareness file of OSHA regulations
      regarding the safe handling of the  chemicals specified in this method. A reference file of
      material  safety data sheets (MSDSs) should also be made available to all personnel involved in
      these analyses. It is also suggested that the laboratory perform personal hygiene monitoring of
      each analyst  who uses this method and that the results of this monitoring be made available to
      the analyst. Additional information on laboratory safety can be found in  References  10-13. The
      references and bibliography at the  end of Reference 13 are particularly comprehensive in dealing
      with the  general subject of laboratory safety.
 5.3  The CDDs/CDFs and samples suspected to contain these compounds are handled using
      essentially the same techniques employed in handling radioactive or infectious materials. Well-
      ventilated, controlled access laboratories are required. Assistance in evaluating the health hazards
      of particular laboratory  conditions  may be obtained from certain consulting laboratories and from
      State Departments of Health or Labor, many of which have an industrial health service. The
      CDDs/CDFs are extremely toxic to laboratory animals. Each laboratory must develop a strict
      safety program for handling these compounds. The practices in References 2 and 14 are highly
      recommended.
       5.3.1  Facility—When finely divided samples (dusts, soils, dry chemicals) are handled, all
             operations (including removal of samples from sample containers, weighing, transferring,
             and mixing) should be performed in a glove box demonstrated to be leak tight or in a
             fume hood demonstrated to have adequate air flow. Gross  losses  to the laboratory
             ventilation system must not be allowed. Handling of the dilute solutions normally used in

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Metnoa
            analytical and animal work presents no inhalation hazards except in the case of an
            accident.

      5.3.2  Protective equipment—Disposable plastic gloves, apron or lab coat, safety glasses or
            mask, and a glove box or fume hood adequate for radioactive work should be used.
            During analytical operations that may give  rise to aerosols or dusts, personnel should
            wear respirators equipped with activated carbon filters. Eye protection equipment
            (preferably full face shields) must be worn  while working with exposed samples or pure
            analytical standards. Latex gloves are commonly used to reduce exposure of the hands.
            When handling samples suspected or known to contain high  concentrations of the
            CDDs/CDFs, an additional set of gloves can also be worn beneath the latex gloves.
      5.3.3  Training—Workers must be trained  in the proper method of removing contaminated
            gloves and clothing without contacting  the exterior surfaces,   i
                                                                      ,1
      5.3.4  Personal hygiene—Hands and  forearms should be washed thoroughly after each
            manipulation and before breaks (coffee, lunch, and shift).     '
      5.3.5  Confinement—Isolated work areas posted with signs, segregated glassware and tools, and
            plastic absorbent paper on bench  tops will aid in confining contamination.
      5.3.6  Effluent vapors-The effluents of sample splitters from the gas chromatograph (GC) and
            from roughing pumps on  the mass spectrometer (MS) should pass  through either a
            column of activated charcoal or be bubbled  through a trap containing oil or high-boiling
            alcohols to condense CDD/CDF vapors.
     5.3.7  Waste Handling—Good technique includes minimizing contaminated waste. Plastic bag
            liners should be used in waste cans. Janitors and other personnel must be trained in the
            safe handling of waste.
     5.3.8  Decontamination.
                                                                      |
          5.3.8.1  Decontamination of personnel—Use  any mild soap with! plenty of scrubbing
                  action.                                              ;
          5.3.8.2  Glassware, tools, and surfaces—Chlorothene NU Solvent is the  least toxic solvent
                  shown to be effective. Satisfactory cleaning may be accomplished by rinsing with
                 .Chlorothene, then  washing with any detergent and water. If glassware is first
                  rinsed with solvent, then the dish water may be disposed of in the sewer. Given
                  the cost of disposal, it is prudent to minimize solvent wastes.
     5.3.9 Laundry—Clothing known to be contaminated  should be collected in plastic bags.
          Persons who convey the bags and launder the clothing should  be advised of the hazard
          and trained in proper handling. The clothing  may be put into a washer without contact if
          the launderer knows of the potential problem. The washer should be run through a cycle
          before being used again for other clothing.
          Wipe tests—A useful method of determining cleanliness of work surfaces and tools is to
          wipe the surface with a piece of filter paper.  Extraction and analysis by  GC  with an
          electron capture detector (BCD)  can achieve a limit of detection of 0.1 ug per wipe;
          analysis using this method  can achieve an even lower detection limit. Less than 0.1 ng
          per wipe indicates acceptable cleanliness; anything higher warrants further cleaning.
5.3.10

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                                                                                      Method 1613
              More than 10 ug on a wipe constitutes an acute hazard and requires prompt cleaning
              before further use of the equipment or work space, and indicates that unacceptable work
              practices have been employed.
       5.3.11  Table or wrist-action shaker—The use of a table or wrist-action shaker for extraction of
              tissues presents the possibility of breakage of the extraction bottle and spillage of acid
              and flammable organic solvent. A secondary containment system around the shaker is
              suggested to prevent the spread of acid and solvents in the event of such a breakage. The
              speed and intensity of shaking action should also be adjusted to minimize the possibility
              of breakage.

6.0   Apparatus  and  Materials

    Note:  Brand names, suppliers, and part numbers are for illustration purposes only and no
    endorsement is implied. Equivalent performance may be achieved using apparatus and materials
    other than those specified here. Meeting the performance requirements of this method is the
    responsibility of the laboratory.                        	

 6.1   Sampling equipment for discrete or composite sampling.
        6.1.1  Sample  bottles and caps.
              6.1.1.1  Liquid samples (waters, sludges and similar materials containing 5 percent solids
                     or less)—Sample bottle, amber glass, 1.1-L minimum, with screw cap.
              6.1.1.2  Solid samples (soils, sediments, sludges, paper pulps, filter cake, compost, and
                     similar materials that contain more than 5 percent solids)—Sample bottle, wide
                     mouth, amber glass, 500-mL minimum.
              6.1.1.3  If amber bottles are not available, samples  shall be protected from light.
              6.1.1.4  Bottle caps—Threaded to fit sample bottles. Caps shall be lined with
                     fluoropolymer.
              6.1.1.5  Cleaning.
                     6.1.1.5.1  Bottles are detergent water washed, then solvent rinsed before use.
                     6.1.1.5.2  Liners are detergent water washed, rinsed with reagent water (Section
                              7.6.1) followed by solvent, and baked at approximately 200°C for a
                              minimum of 1 hour prior to use.
        6.1.2  Compositing equipment—Automatic or manual compositing system incorporating glass
              containers cleaned per bottle cleaning procedure above. Only glass or fluoropolymer tub-
              ing shall be used. If the sampler uses a peristaltic pump, a minimum length of
              compressible silicone rubber tubing may be used in the pump only.  Before use, the
              tubing shall be thoroughly rinsed with methanol, followed by repeated  rinsing with
              reagent  water to minimize sample contamination. An integrating flow meter is used to
              collect proportional composite samples.
 6.2   Equipment for glassware cleaning—Laboratory sink with overhead fume hood.

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Melkod 1613
6.3
6.4
Equipment for sample preparation.
  6.3.1  Laboratory fume hood of sufficient size to contain the sample preparation equipment
        listed below.
  6.3.2  Glove box (optional).
  6.3.3  Tissue homogenizer—VirTis Model 45 Macro homogenizer (American Scientific
        Products H-3515, or equivalent) with stainless steel Macro-shaft and Turbo-shear blade.
  6.3.4  Meat grinder—Hobart, or equivalent, with 3- to 5-mm holes in inner plate.
  6.3.5  Equipment for determining percent moisture.
       6.3.5.1  Oven—Capable of maintaining a temperature of 110 ±'5°C.
       6.3.5.2  Dessicator.
  6.3.6  Balances.                                                   '
       6.3.6.1  Analytical—Capable of weighing O.I  mg.
       6.3.6.2  Top loading—Capable of weighing 10 mg.            <
Extraction apparatus.
 6.4.1  Water samples.
       6.4.1.1  pH meter, with combination glass electrode.
                                                                   !
       6.4.1.2  pH paper, wide range (Hydrion Papers, or equivalent).
       6.4.1.3  Graduated cylinder, 1-L capacity.
       6.4.1.4  Liquid/liquid extraction—Separatory funnels, 250-, 500v, and 2000-mL, with
               fluoropolymer stopcocks.
       6.4.1.5  Solid-phase extraction.                               j
               6.4.1.5.1   1-L filtration apparatus, including glass funnel, glass frit support, clamp,
                        adapter, stopper, filtration flask, and vacuum tubing (Figure 4). For
                        wastewater samples, the apparatus should accept 90 or 144 mm disks.
                        For drinking water or other samples containing low solids, smaller disks
                        may be used.
              6.4.1.5.2   Vacuum source capable of maintaining 25 in. Hg, equipped with shutoff
                        valve and vacuum gauge.                  .  |
              6.4.1.5.3   Glass-fiber filter—Whatman GMF  150 (or equivalent), 1 micron pore
                        size, to fit filtration apparatus in Section 6.4.1,5.1.
              6.4.1.5.4  Solid-phase extraction disk containing octadecyl (Clg) bonded silica
                       uniformly enmeshed in an inert matrix—Fisher Scientific 14-378F (or
                       equivalent), to fit filtration apparatus  in Section 6.4.1.5.1.
 6.4.2  Soxhlet/Dean-Stark (SDS) extractor (Figure 5) for filters and solid/sludge samples.
       6.4.2.1  Soxhlet—50-mm ID, 200-mL capacity with 500-mL flask (Cal-Glass LG-6900, or
              equivalent, except substitute 500-mL round-bottom flask for 300-mL flat-bottom
              flask).                                               ,

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                                                                                    Method 1613
            6.4.2.2  Thimble—43 x  123 to fit Soxhlet (Cal-Glass LG-6901-122, or equivalent).
            6.4.2.3  Moisture trap—Dean Stark or Barret with fluoropolymer stopcock, to fit Soxhlet.
            6.4.2.4  Heating mantle—Hemispherical, to fit 500-mL round-bottom flask (Cal-Glass
                   LG-8801-112, or equivalent).
            6.4.2.5  Variable transformer—Powerstat (or equivalent), 110-volt, 10-amp.
      6.4.3  Apparatus for extraction of tissue.
            6.4.3.1  Bottle for extraction (if digestion/ extraction using HC1 is used)—500- to 600-mL
                   wide-mouth clear glass, with fluoropolymer-lined cap.
            6.4.3.2  Bottle for back-extraction—100- to 200-mL narrow-mouth clear glass with
                   fluoropolymer-lined cap.
            6.4.3.3  Mechanical shaker—Wrist-action or platform-type rotary shaker that produces
                   vigorous agitation (Sybron Thermolyne Model LE "Big  Bill" rotator/shaker, or
                   equivalent).
            6.4.3.4  Rack attached to shaker table to permit agitation of 4-9  samples simultaneously.
      6.4.4  Beakers—400- to 500-mL.
      6.4.5  Spatulas—Stainless steel.
6.5  Filtration apparatus.
      6.5.1  Pyrex  glass wool—Solvent-extracted by SDS for 3 hours minimum.
      i
   Note:  Baking glass  wool may cause active sites that will irreversibly adsorb CDDs/CDFs.	

      6.5.2 Glass  funnel—125- to 250-mL.
      6.5.3 Glass-fiber filter paper—Whatman GF/D (or equivalent), to fit glass funnel in Section
            6.5.2.
      6.5.4 Drying column—15- to 20-mm ID Pyrex  chromatographic column equipped with coarse-
            glass frit or glass-wool plug.
      6.5.5 Buchner funnel—15-cm.
       6.5.6  Glass-fiber filter paper—to fit Buchner funnel in Section 6.5.5.
       6.5.7  Filtration flasks—1.5- to 2.0-L, with side arm.
       6.5.8  Pressure filtration apparatus—Millipore YT30  142 HW, or equivalent.
 6.6   Centrifuge apparatus.
       6.6.1  Centrifuge—Capable of rotating 500-mL  centrifuge  bottles or 15-mL  centrifuge tubes at
             5,000 rpm  minimum.
       6.6.2  Centrifuge bottles—500-mL,  with screw-caps, to fit centrifuge.
       6.6.3  Centrifuge tubes—12- to 15-mL, with screw-caps, to fit centrifuge.
 6.7   Cleanup apparatus.

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Method 1613
        t                                                                  i
       6^7.1  Automated gel permeation chromatograph (Analytical Biochemical Labs, Inc, Columbia,
        i    MO, Model GPC Autoprep 1002, or equivalent).                 '|
        :    gj.1.1   Column—600-700 mm long x 25 mm ID, packed with 70 g of SX-3 Bio-beads
        i            (Bio-Rad Laboratories, Richmond, CA, or equivalent).
        ;    6.7.1.2  Syringe—10-mL, with Luer fitting.                       ;
        i    6.7.1.3  Syringe filter holder—stainless steel, and glass- fiber or fluoropolymer filters
        '            (Gelman 4310, or equivalent).                           '
        i                                                     "             •'
        ;    6.7.1.4  UV detectors—254-nm, preparative or semi-preparative flow cell (Isco, Inc.,
        ;            Type 6; Schmadzu, 5-mm path length; Beckman-Altex 152W, 8-uL micro-prep
        I            flow cell, 2-mm path; Pharmacia UV-1, 3-mm flow cell; LDC Milton-Roy UV-3,
        j            monitor #1203; or equivalent).                          ,i
       61.7.2  Reverse-phase high-performance liquid chromatograph.           !
        i    6.7.2.1  Column oven and detector—Perkin-Elmer Model LC-65T (or equivalent)
        i            operated at 0.02 AUFS at 235 nm.
            6.7.2.2  Injector—Rheodyne 7120 (or equivalent) with 50-uL sample loop.
        >    6.7.2.3  Column—Two 6.2 mm x 250 mm Zorbax-ODS columns in series (DuPont
        i            Instruments Division, Wilmington, DE,  or equivalent), operated at 50°C with 2.0
        ;            mL/min methanol isocratic effluent.
        !  .   6.7.2.4  Pump—Altex  110A (or equivalent).
       6.7.3  Pipets.                                                       ;
        i     6.7.3.1  Disposable, Pasteur,  150-mm long x 5-mm ID (Fisher Scientific 13-678-6A, or
        !            equivalent).
        |     6.7.3.2  Disposable, serological, 10-mL  (6-mm ID).               ,
        6.7.4 Glass chromatographic columns.
        ;     6.7.4.1   150-mm long x 8-mm ID, (Kontes K-420155, or equivalent) with coarse-glass
        i            frit or glass-wool plug and 250-mL reservoir.            ;
        !     6.7.4.2 200-mm long x 15-mm ID,  with coarse-glass frit or glass-wool plug and 250-mL
                     reservoir.
        ;     6.7.4.3  300-mm long x 25-mm ID,  with 300-mL reservoir and glass or fluoropolymer
        :             stopcock.                                             i      -      '
        16.7.5  Stirring  apparatus for batch silica cleanup of tissue extracts.      j
              6.7.5.1  Mechanical stirrer—Corning Model 320, or equivalent.   ,
              6.7.5.2 Bottle—500- to 600-mL wide-mouth clear glass.
        J6.7.6  Oven—For baking and storage of adsorbents, capable of maintaining  a constant
        I      temperature (±5°C) in the range of 105-250°C.                 i
        i
  6.8  Concentration apparatus.
        
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                                                                                    Method 1613
            6.8.1.1  Vacuum source for rotary evaporator equipped with shutoff valve at the
                    evaporator and vacuum gauge.
            6.8,1.2  A recirculating water pump and chiller are recommended, as use of tap water for
                    cooling the evaporator wastes large volumes of water and can lead to inconsistent
                    performance as water temperatures and pressures vary.
            6.8.1.3  Round-bottom flask— 100-mL and 500-mL or larger, with ground-glass fitting
                    compatible with  the rotary evaporator.
       6.8.2  Kuderna-Danish (K-D) concentrator.
            6.8.2.1  Concentrator tube—10-mL, graduated (Kontes K-570050-1025,  or equivalent)
                    with calibration verified. Ground-glass stopper (size 19/22 joint) is used  to
                    prevent evaporation of extracts.
            6.8.2.2  Evaporation flask—500-mL (Kontes K-570001-0500,  or equivalent), attached to
                    concentrator tube with springs (Kontes K-662750-0012 or equivalent).
            6.8.2.3  Snyder column—Three-ball macro (Kontes K-503000-0232, or equivalent).
            6.8.2.4  Boiling chips.
                    6.8.2.4.1  Glass or silicon carbide—Approximately 10/40 mesh, extracted with
                             methylene chloride  and baked at 450°C for one hour minimum.
                    6.8.2.4.2 Fluoropolymer (optional)—Extracted with methylene chloride.
            6.8.2.5  Water bath—Heated, with concentric ring cover, capable of maintaining a
                    temperature within ±2°C, installed in a fume hood.
       6.8.3  Nitrogen blowdown apparatus—Equipped with water bath controlled in the range of 30 -
             60°C (N-Evap, Organomation Associates, Inc., South Berlin,  MA, or equivalent),
             installed in a fume hood.
       6.8.4  Sample vials
             6.8.4.1  Amber glass, 2- to 5-mL with fluoropolymer-lined screw-cap.
             6.8.4.2  Glass, 0.3-mL, conical, with fluoropolymer-lined screw or crimp cap.
 6.9   Gas chromatograph—Shall have splitless or on-column injection port for capillary column,
      temperature program with isothermal hold, and shall meet all of the performance specifications
      in Section 10.
       6.9,1  GC column for CDDs/CDFs and for isomer specificity for 2,3,7,8-TCDD—60±5-m long
             x 0.32±0.02-mm  ID; 0.25-um 5% phenyl, 94% methyl, 1% vinyl silicone bonded-phase
             fused-silica capillary column (J & W DB-5, or equivalent).
       6.9.2  GC column for isomer specificity for 2,3,7,8-TCDF—30±5-m long x 0.32±0.02-mm ID;
             0.25-um bonded-phase fused-silica capillary column (J & W  DB-225, or equivalent).
6.10   Mass spectrometer—28- to 40-eV electron impact ionization, shall be capable of repetitively
      selectively monitoring 12 exact m/z's minimum at  high resolution (>10,000) during a period of
      approximately 1 second,  and shall meet all of the performance specifications in Section 10.
                                                                                              11

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    Method 1613
                                                          be interfaced
         electron or ion beams.  "	~"	'" ' ™ °* ™ ^ S°UrCe but *«* not interce'p7th7
   6.12|  Data system-Capable of collecting, recording) ^ storing M, ^

  7.0 \  Reagents and Standards
   7.1  pH adjustment and back-extraction.
       |   7.1.1  Potassium hydroxide—Dissolve 20 g
          7.1.2  Sulfuric acid-Reagent grade (specific gravity&L84)!
         7.1.3  Hydrochloric acid—Reagent grade, 6N.

  7.2


       i 7.2.3
 7.3   Extraction.
7.4
7.5   Adsorbents for sample cleanup.
      7.5.1  Silica gel.



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                                                                               Method 1613
             a stirring rod until a uniform mixture is obtained. Store in a bottle with a
             fluoropolymer-lined screw-cap.
      7.5.1.3  Basic silica gel—Thoroughly mix 30 g of IN sodium hydroxide with 100 g of
             activated silica gel  in a clean container. Break up aggregates with a stirring rod
             until a uniform mixture is obtained.  Store in a bottle with a fluoropolymer-lined
             screw-cap.
      7.5.1.4  Potassium  silicate.
             7.5.1.4.1  Dissolve 56 g of high purity potassium hydroxide (Aldrich, or
                      equivalent) in 300 mL of methanol in  a 750- to 1000-mL flat-bottom
                      flask.
             7.5.1.4.2  Add 100 g of silica gel and a stirring bar, and stir on a hot plate at 60-
                      70°C for  1-2 hours.   .
             7.5.1.4.3  Decant the liquid and rinse the potassium silicate twice with 100-mL
                      portions of methanol, followed by a single rinse with 100 mL of
                      methylene chloride.
             7.5.1.4.4  Spread the potassium silicate on solvent-rinsed aluminum foil and dry
                      for 2-4 hours in a hood.
             7.5.1.4.5  Activate overnight at 200-250°C.
7.5.2  Alumina—Either one of two types of alumina, acid or basic, may be used in the cleanup
      of sample extracts, provided that the laboratory can meet the performance specifications
      for the recovery of labeled compounds described in Section 9.3. The same type of
      alumina must be used for all samples,  including those used to demonstrate initial
      precision and recovery (Section 9.2) and ongoing precision and recovery (Section  15.5).
      7.5.2.1  Acid alumina—Supelco 19996-6C (or equivalent). Activate by heating to 130°C
             for a minimum of 12 hours.
      7.5.2.2 Basic alumina—Supelco 19944-6C (or equivalent). Activate by heating to 600°C
             for a minimum of 24 hours. Alternatively, activate by heating in a tube furnace at
             650 to 700°C under an air flow rate of approximately 400 cc/minute. Do not heat
             over 700°C, as this can lead to reduced capacity for retaining the analytes. Store
             at 130°C in a covered flask. Use within five days of baking.
7.5.3  Carbon.
      7.5.3.1 Carbopak C—(Supelco  1-0258, or equivalent).
      7.5.3.2 Celite 545—(Supelco 2-0199,  or equivalent).
      7.5.3.3 Thoroughly mix 9.0 g Carbopak C and 41.0 g Celite 545 to produce an 18% w/w
              mixture. Activate the mixture at 130°C for a minimum of 6 hours. Store in a
              dessicator.
7.5.4 Anthropogenic isolation column—Pack the column in Section 6.7.4.3 from bottom to top
      with the following:
      7.5.4.1  2 g silica gel (Section 7.5.1.1).
                                                                                         13

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Methofi 1613
 7.6
 7.7
  7.8
       7.5.4.2  2 g potassium silicate (Section 7.5.1.4).
       7.5.4.3  2 g granular anhydrous sodium sulfate (Section 7.2.1).
       7.5.4.4  10 g acid silica gel (Section 7.5.1.2).
       7.5.4.5  2 g granular anhydrous sodium sulfate.
 7.5.5  Florisil column
       7.5.5.1  Florisil—60-100 mesh, Floridin Corp (or equivalent). Soxhlet extract in 500-g
              portions for 24 hours.
       7.5.5.2  Insert a glass wool plug into the tapered end of a graduated serological pipet
              (Section 6.7.3.2). Pack with 1.5 g (approx 2 mL) of Florisil topped with approx 1
              mL of sodium sulfate (Section 7.2.1) and a glass wool plug.
       7.5.5.3  Activate in an oven at 130-150 °C for a minimum of 24 hours and cool for 30
              minutes. Use within 90 minutes of cooling.             ;
Reference matrices—Matrices in which the CDDs/CDFs and interfering compounds are not
detected by this method.
 7.6.1   Reagent water—Bottled water purchased locally, or prepared by passage through
        activated carbon.                                            ;
 7.6.2   High-solids reference matrix—Playground sand or similar material. Prepared by -
        extraction  with methylene chloride and/or baking at 450°C for a minimum of 4 hours.
 7.6.3   Paper reference matrix—Glass-fiber filter, Gelman type A, or equivalent. Cut paper to
        simulate the surface area of the paper sample being tested.
 7.6.4   Tissue reference matrix—Corn or other vegetable oil. May be prepared  by extraction
        with methylene chloride.                                    \
 7.6.5   Other matrices—This method may be verified  on any reference matrix by performing the
        tests given in Section 9.2. Ideally, the matrix should be free of the CDDs/CDFs, but in
        no case shall the background level of the CDDs/CDFs in the reference matrix exceed
        three times the minimum levels in Table 2. If low background levels of the CDDs/CDFs
        are present in the reference matrix, the spike level of the analytes used  in Section 9.2
        should be increased to provide a spike-to-background  ratio in the range of 1:1  to. 5:1
        (Reference 15).
 Standard solutions—Purchased as solutions or mixtures with certification to their purity,
 concentration, and authenticity,  or prepared from materials of known purity and composition.  If
 the chemical purity is 98% or greater, the weight may be used without correction to compute the
 concentration of the standard. When not being used, standards are stored in the dark at room
 temperature in screw-capped vials with fluoropolymer-lined caps. A mark is placed on the vial at
 the level of the solution so that solvent loss by evaporation can be detected. If solvent loss has
 occurred, the solution should be replaced.
 Stock solutions.
  14

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                                                                                      Method 1613
        7.8.1  Preparation—Prepare in nonane per the steps below or purchase as dilute solutions
              (Cambridge Isotope Laboratories (CIL), Wobum, MA, or equivalent). Observe the safety
              precautions in Section 5, and the recommendation in Section 5.1.2.
        7.8.2  Dissolve an appropriate amount of assayed reference material in solvent. For example,
              weigh 1 to 2 mg of 2,3,7,8-TCDD to three significant figures in a 10-mL ground-glass-
              stoppered volumetric flask and fill to the mark with nonane. After the TCDD is
              completely dissolved, transfer the solution to a clean 15-mL vial with fluoropolymer-
              lined cap.
        7.8.3  Stock standard solutions should be checked for signs of degradation prior to the
              preparation of calibration or performance test standards. Reference standards that can be  '
              used to determine the accuracy of calibration standards are available  from CIL and may
              be available from other vendors.
 7.9  PAR stock solution.
        7.9.1  All CDDs/CDFs—Using the solutions in Section 7.8, prepare the PAR stock solution to
              contain the CDDs/CDFs at the concentrations  shown in Table 3. When diluted, the
              solution will become the PAR (Section 7.14).
        7.9.2  If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be determined, prepare the PAR stock
              solution to contain these compounds only.
7.10  Labeled-compound spiking solution.
      7.10.1  All CDDs/CDFs—From stock solutions, or from purchased mixtures, prepare this
              solution to contain the labeled compounds in nonane at the concentrations shown  in
              Table 3. This solution is diluted with acetone prior to use (Section 7.10.3).
      7.10.2  If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be determined, prepare the labeled-
              compound solution to contain these compounds only. This solution is diluted with
              acetone prior to use (Section 7.10.3).
      7.10.3  Dilute a sufficient volume of the labeled compound solution (Section 7.10.1  or 7.10.2) by
              a factor of 50 with acetone  to prepare a diluted spiking solution. Each sample requires
              1.0 mL of the diluted solution, but no more solution should be prepared than can  be used
              in  one day.
7.11  Cleanup standard—Prepare 37Cl4-2,3,7,8-TCDD in nonane at the concentration shown in Table 3.
      The cleanup standard is added  to all extracts prior to cleanup to measure the efficiency of the
      cleanup process.
7.12  Internal standard(s).
      7.12.1  All CDDs/CDFs—Prepare the internal standard solution to contain I3C12-1,2,3,4-TCDD
              and I3C)2-l,2,3,7,8,9-HxCDD in nonane at the concentration shown in Table 3.
      7.122  If  only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be determined, prepare the internal
              standard solution to contain 13C12-1,2,3,4-TCDD only.
7.13  Calibration standards (CS1 through CSS)—Combine the solutions in Sections 7.9-7.12 to
      produce the five calibration solutions  shown  in Table 4 in nonane. These solutions permit the
      relative response (labeled to native) and response factor to be measured as a function of concen-

                                                                                               15

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  Method
       tration. The CSS standard is used for calibration verification (VER). If only 2,3,7,8-TCDD and
       2,3,7,8-TCDF are to be determined, combine the solutions appropriate to these compounds.
 7.141  Precision and recovery (PAR) standard—Used for determination of initial (Section 9.2) and
     |  ongoing (Section 15.5) precision and recovery. Dilute 10 uL of the precision and recovery
     I  standard (Section 7.9.1 or 7.9.2) to 2.0 mL with acetone for each sample matrix for each sample
     i  batch. One mL each are required for the blank and OPR with each matrix in each batch.
 7.15!  GC retention time window defining solution and isomer specificity test standard	Used to define
     i  the beginning and ending retention times for the dioxin and furan isorners and to demonstrate
       isomer specificity of the GC columns employed for determination of 2,3,7,8-TCDD and  2,3,7,8-
     I  TCDF. The standard must contain the  compounds listed in Table 5 (CIL EDF-4006, or
     I  equivalent), at a minimum. It is not necessary to monitor the window-defining compounds if
     i  only 2,3,7,8-TCDD and 2,3,7,8-TCDF are  to be determined. In this case, an isomer-specificity
     I  test standard containing the most closely eluted isomers listed in Table 5 (CIL EDF-4033, or
     j  equivalent) may be used.
 7.16 i  QC Check Sample—A QC Check Sample  should be obtained from a source independent of the
       calibration standards. Ideally, this check sample would be a certified reference material
       containing the CDDs/CDFs in known concentrations in a sample matrix similar to the  matrix
       under test.
 7.17   Stability of solutions—Standard solutions used for quantitative purposes (Sections  7.9 through
     |  7.15) should be analyzed periodically,  and  should be assayed against reference standards (Section
     ;  7.8.3) before further use.
     i   .       "
8.01  Sample Collection, Preservation, Storage, and Holding  Times.
     I
 8.1  i  Collect samples in amber glass containers following conventional sampling practices (Reference
     !  16). Aqueous samples that flow freely  are collected in refrigerated  bottles using automatic
     I  sampling equipment. Solid samples are collected as grab samples using wide-mouth jars.
 8.2 !  Maintain aqueous samples in the dark at 0-4°C from the time of collection until receipt at the
     I  laboratory. If residual chlorine is present in aqueous samples, add 80 mg sodium thiosulfate per
     i  liter of water. EPA Methods 330.4 and 330.5 may be  used to measure residual chlorine
     ;  (Reference 17). If sample pH is greater than 9, adjust to pH 7-9 with sulfuric acid.
     ;  Maintain solid, semi-solid, oily, and mixed-phase samples in the dark at <4°C from the time of
     !  collection until receipt at the laboratory.                             I
     |  Store aqueous samples in the dark at 0-4°C. Store solid, semi-solid, oily, mixed-phase,  and tissue
       samples in the dark at <-10°C.
 8.3  I  Fish and tissue samples.
        8.3.1 Fish may be cleaned, filleted, or processed in other  ways  in the field, such  that  the
             laboratory may expect to receive whole fish, fish fillets, or other tissues for analysis.
        8.3.2 Fish collected in the field should be wrapped in aluminum foil, and must be maintained
             at a temperature less than 4°C from the time of collection until receipt at the laboratory.
 16

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                                                                                       Method 1613
        8.3.3  Samples must be frozen upon receipt at the laboratory and maintained in the dark at <-
              10°C until prepared. Maintain unused sample in the dark at <-10°C.
 8.4   Holding times.
        8.4.1  There are no demonstrated maximum holding times associated with CDDs/CDFs in
              aqueous, solid, semi-solid, tissues, or other sample matrices. If stored in the dark at 0-
              4°C  and preserved as given above (if required), aqueous samples may be stored for up to
              one year. Similarly, if stored in the dark at <-10°C, solid, semi-solid, multi-phase, and
              tissue samples may be stored for up to  one year.
        8.4.2  Store sample extracts in the dark at <-10°C until analyzed. If  stored in the dark at <-
              10°C, sample extracts may be stored  for up to one year.

9.0   Quality Assurance/Quality  Control

 9.1   Each laboratory that uses this method is required to operate a formal quality assurance program
       (Reference 18). The minimum requirements of this program consist of an initial demonstration of
       laboratory capability, analysis of samples spiked with labeled compounds to evaluate and
       document data quality, and analysis of standards and  blanks as  tests of continued performance.
       Laboratory performance is compared to established performance criteria to determine if the
       results of analyses meet the performance characteristics of the method.

       If the method is to be applied to sample matrix other than water (e.g., soils, filter cake, compost,
      'tissue) the most appropriate alternate matrix (Sections 7.6.2-7.6.5) is substituted for the reagent
       water matrix (Section 7.6.1) in all performance tests.
        9.1.1  The  analyst shall make an initial demonstration of the ability to generate acceptable
              accuracy and precision with this method. This ability is established as described in
              Section 9.2.
        9.1.2  In recognition of advances that are occurring  in analytical technology, and to allow the
              analyst to overcome sample matrix interferences, the analyst is permitted certain options
              to improve separations or lower the costs of measurements. These options  include
              alternate extraction, concentration, cleanup procedures, and changes in columns and
              detectors. Alternate determinative techniques, such as the substitution of spectroscopic or
              immuno-assay techniques, and changes that degrade method performance, are not
              allowed. If an analytical technique other than the techniques specified in this method is
              used, that technique must have a specificity equal to or better than the specificity of the
              techniques in this method for the analytes of  interest.
              9.1.2.1  Each time a modification is made to this method, the analyst is required to repeat
                     the procedure in Section 9.2. If the detection limit of the  method will be affected
                     by the change, the laboratory is required to demonstrate that the MDL (40 CFR
                     Part 136, Appendix B) is  lower than one-third the regulatory compliance level cl-
                     one-third the ML in this method, whichever is higher. If calibration will be
                     affected  by the change,  the analyst must recalibrate  the instrument per Section 10.
                                                                                               17

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Method 1613
 18
             9.1.2.2  The laboratory is required to maintain records of modifications made to this
                    method. These records include the following, at a minimum:
                    9.1.2.2.1  The names, titles,  addresses, and telephone numbers of the analyst(s)
                             who performed  the analyses and modification, and of the quality control
                             officer who witnessed and will verify the analyses and modifications.
                    9.1.2.2.2  A listing of pollutant(s) measured, by name and CAS Registry number.
                    9.1.2.2.3  A narrative stating reason(s) for the modifications.
                    9.1.2.2.4  Results from all quality control  (QC) tests comparing the modified
                             method to  this method, including:
                             a)   Calibration (Section  10.5-10.7).         j
                             b)   Calibration verification (Section  15.3).
                             c)   Initial precision and recovery (Section 9.2).
                             d)   Labeled compound recovery (Section 9.3).
                             e)   Analysis of blanks (Section 9.5).
                             f)   Accuracy assessment (Section 9.4).
                    9.1.2.2.5  Data that will allow an independent reviewer to validate each
                             determination by tracing the instrument output (peak height, area, or
                             other signal) to  the final result. These data are to include:
                    a)     Sample numbers and other identifiers.
                    b)     Extraction dates.                             '
                    c)     Analysis dates and times.
                    d)     Analysis sequence/run chronology.            \
                    e)     Sample weight or volume (Section 11).
                    f)     Extract volume prior to each  cleanup step (Section 13).
                    g)     Extract volume after each cleanup step (Section 13).
                    h)     Final extract volume prior to  injection (Section 14).
                    i)     Injection volume (Section  14.3).
                    j)     Dilution data, differentiating between dilution of a sample or extract
                           (Section 17.5).
                    k)     Instrument and operating conditions.          :
                    1)     Column (dimensions, liquid phase, solid support, film thickness, etc).
                    m)    Operating conditions (temperatures, temperature program, flow rates).
                    n)     Detector (type, operating conditions, etc).      ;
                    o)     Chromatograms, printer tapes, and other recordings  of raw data.
                    p)     Quantitation reports, data system outputs, and other data to link the raw
                           data to the results reported.
       9.1,3  Analyses of method blanks are required to demonstrate freedom from contamination
             (Section  4.3). The procedures and criteria for analysis of a method  blank are described in
             Sections 9.5 and 15.6.
       9.1.4  The laboratory shall spike all samples with labeled compounds to monitor method
             performance. This test is described in Section 9.3. When results of these spikes indicate

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                                                                                     Method 1613
             atypical method performance for samples, the samples are diluted to bring method
             performance within acceptable limits. Procedures for dilution are given in Section  17.5.
       9.1.5  The laboratory shall, on an ongoing basis, demonstrate through calibration verification
             and the analysis of the ongoing precision and recovery aliquot that the analytical system
             is in control. These procedures are described in Sections 15.1 through 15.5.
       9.1.6  The laboratory shall maintain  records to define the quality of data that is generated.
             Development of accuracy statements is  described in Section 9.4.
9.2  Initial precision and recovery (1PR)—To establish the ability to generate acceptable precision and
     recovery, the analyst shall perform the following operations.
       9.2.1  For low solids  (aqueous) samples, extract, concentrate, and analyze  four 1-L aliquots of
             reagent water spiked with the  diluted labeled compound spiking solution (Section 7.10.3)
             and the precision and recovery standard (Section 7.14) according to the  procedures in
             Sections 11 through 18. For an alternative sample matrix, four aliquots of the alternative
             reference matrix (Section  7.6) are used. All  sample processing steps that are to be used
             for processing samples, including preparation  (Section  11),  extraction (Section 12), and
             cleanup (Section  13), shall be included  in this test.
       9.2.2  Using results of the set of four analyses, compute the average concentration (X) of the
             extracts in ng/mL and the standard deviation of the concentration (s) in ng/mL for each
             compound, by isotope dilution for CDDs/CDFs with a labeled analog, and by internal
             standard for 1,2,3,7,8,9-HxCDD, OCDF, and the labeled compounds.
       9.2.3  For each CDD/CDF and labeled compound, compare s and X with the corresponding
             limits for initial precision and recovery  in Table 6. If only 2,3,7,8-TCDD and 2,3,7,8-
             TCDF are to be determined, compare s  and  X with the corresponding limits for initial
             precision and recovery in Table 6a. If s and X for all compounds meet the acceptance
             criteria, system performance is acceptable and analysis of blanks and samples may begin.
             If, however, any individual s exceeds the precision limit or any individual X falls outside
             the range for accuracy,  system performance  is unacceptable for that compound. Correct
             the problem and repeat the test (Section 9.2).
9.3  The laboratory shall spike all samples with the  diluted labeled compound spiking solution
     (Section 7.10.3) to assess method performance  on the sample matrix.
       9.3.1  Analyze each sample according to the procedures in Sections 11 through 18.
       9.3.2  Compute the percent recovery of the labeled compounds and the cleanup standard using
             the internal standard method (Section 17.2).
       9.3.3  The recovery of each labeled compound must be within the limits in Table 7  when all
             2,3,7,8-substituted CDDs/CDFs are determined, and within the limits in Table 7a when
             only 2,3,7,8-TCDD and 2,3,7,8-TCDF are determined. If the recovery of any  compound
             falls outside of these limits, method performance  is unacceptable for that compound in
             that sample. To overcome such difficulties,  water samples are diluted and smaller
             amounts of soils, sludges, sediments, and other matrices are reanalyzed per Section 18.4.
9.4  Recovery of labeled compounds from samples should be  assessed and records should be
     maintained.

                                                                                              19

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Method 1613	        	

   :   9.4.1   After the analysis of five samples of a given matrix type (water, soil, sludge, pulp, etc.)
   :          for which the labeled compounds pass the tests in Section 9.3, compute the average
   i          percent recovery (R) and the standard deviation of the percent recovery (SR) for the
   \          labeled compounds only. Express the assessment as  a percent recovery interval from R -
   •          2SR to R + 2SR for each matrix. For example, if R = 90% and SR = 10% for five
             analyses of pulp, the recovery interval is expressed as 70 to 110%.
   :   9.4.2  Update the accuracy assessment for each  labeled compound in each matrix on a regular
   :          basis (e.g., after each five to ten new measurements).
9.5 i  Method blanks—Reference matrix method blanks are analyzed to demonstrate freedom from
   I  contamination (Section 4.3).
   I   9.5.1  Prepare, extract, clean up, and concentrate a method blank with each  sample batch
   i          (samples of the same matrix started through the extraction process on the same 12-hour
   j          shift, to a maximum of 20 samples). The  matrix for the method blank shall be similar to
   \          sample matrix for the batch, e.g., a 1-L reagent water blank (Section  7.6.1), high-solids
   i          reference matrix blank (Section 7.6.2), paper matrix blank (Section 7.6.3); tissue blank
   '          (Section 7.6.4) or alternative reference matrix blank (Section 7.6.5). Analyze the blank
   !          immediately after analysis of the OPR (Section  15.5) to demonstrate  freedom from
   |          contamination.
   i   9.5.2  If any 2,3,7,8-substituted CDD/CDF (Table 1) is found in the blank at greater than the
             minimum level (Table 2) or one-third the regulatory compliance level, whichever  is
   >          greater; or if any potentially interfering compound is found in the blank at the minimum
   !          level for each level of chlorination given  in Table 2 (assuming a response factor of 1
   '          relative to the I3C12-1,2,3,4-TCDD internal standard for compounds not listed in Table 1),
   ;          analysis of samples is halted until the blank associated with the sample batch shows no
   |          evidence of contamination at this level. All samples must be associated with an
   !          uncontaminated method blank before the  results for those samples may be reported for
   i          regulatory compliance purposes.                             ;
9.6   QC Check Sample—Analyze the QC Check Sample (Section 7.16) periodically to assure  the
   !   accuracy of calibration standards and the overall  reliability of the analytical process. It is
      suggested that the QC Check Sample be analyzed at least quarterly.
9.7   The specifications contained in  this method can be met if the  apparatus used is calibrated
   i   properly  and then maintained in a calibrated state.  The standards used for calibration (Section
   i   10), calibration verification (Section 15.3), and for  initial (Section 9.2) and ongoing (Section
   i   15.5) precision and  recovery should be identical, so that the most precise results will be
   '   obtained. A GC/MS  instrument will provide the  most reproducible  results if  dedicated to  the
   !   settings and conditions required for the analyses  of CDDs/CDFs by this method.
9.8   Depending on specific program requirements, field replicates may be collected to  determine the
      precision of the sampling technique, and spiked  samples may be required to  determine the
      accuracy of the analysis when the internal standard method is used.
 20

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                                                                                       Method 1613
10.0   Calibration

  10.1   Establish the operating conditions necessary to meet the minimum retention times for the internal
        standards in Section  10.2.4 and the relative retention times for the CDDs/CDFs in Table 2.
        10.1.1  Suggested GC operating conditions:
                        Injector temperature:    270°C
                        Interface temperature:   290°C
                        Initial  temperature:      200°C
                        Initial  time:            2 minutes
                        Temperature program:   200 to 220°C, at 5°C/minute
                                              220°C for 16 minutes
                                              220 to 235°C, at 5°C/minute
                                              235°C for 7 minutes
                                              235 to 330°C, at 5°C/minute
     Note:  All portions of the column that connect the GC to the ion source shall remain at or
     above the interface temperature specified above during analysis to preclude condensation of less
     volatile compounds.

             Optimize GC conditions for compound separation and sensitivity. Once optimized, the
             same GC conditions must be used for the analysis of all  standards, blanks, IPR and OPR
             aliquots, and samples.
        10.1.2  Mass spectrometer (MS) resolution—Obtain a selected ion current profile (SICP) of each
               analyte in Table 3 at the two exact m/z's specified in Table 8 and at >10,000 resolving
               power by injecting an authentic standard of the CDDs/CDFs either singly or as part of a
               mixture in which there is no interference between closely eluted components.
              10.1.2.1  The analysis time for CDDs/CDFs may exceed the long-term mass stability of the
                      mass spectrometer. Because the instrument is operated in the high-resolution
                      mode,  mass drifts of a few ppm (e.g., 5 ppm in mass) can have serious adverse
                      effects on instrument performance. Therefore, a mass-drift correction is
                      mandatory and a lock-mass m/z from PFK is used for drift correction. The lock-
                      mass m/z is dependent on the exact m/z's monitored within each descriptor, as
                      shown in Table 8. The level 6f PFK metered into the HRMS during analyses
                      should be adjusted so that the amplitude of the most intense selected lock-mass
                       m/z signal (regardless of the descriptor number) does not exceed 10%  of the full-
                      scale deflection for a given set of detector parameters. Under those conditions,
                      sensitivity changes that might occur during the analysis can be more effectively
                       monitored.

     Note:  Excessive PFK (or any other reference substance) may cause noise problems and
     contamination of the ion source necessitating increased frequency of source cleaning.
                                                                                               21

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   ]          10.1.2.2  If the HRMS has the capability to monitor resolution during the analysis, it is
   |                  acceptable to terminate the analysis when  the resolution falls below 10,000 to
   I                  save reanalysis time.
   !          10.1.2.3  Using a PFK molecular leak, tune the instrument to fneet the minimum required
   i                  resolving power of 10,000 (10% valley) at rn/z 304.9824 (PFK) or any other
   j                  reference signal close to m/z 304 (from TCDF).  For each descriptor (Table 8),
   |                  monitor and record the resolution and exact m/z's of three to five  reference peaks
   j                  covering the mass range of the descriptor.  The resolution must be  greater than or
   \    .              equal to 10,000, and the deviation between the exact rn/z and  the theoretical m/z
   I                  (Table 8) for each exact m/z  monitored must be  less than 5 ppm.
10.2   Ion abundance ratios, minimum levels, signal-to-noise ratios, and absolute retention times—
   i    Choose an injection volume of either 1 or 2 uL, consistent with  the capability  of the
       HRGC/HRMS instrument. Inject a 1  or 2 jiL aliquot of the CS1  calibration solution (Table 4)
       using the GC conditions from Section 10.1.1. If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be
       determined, the operating conditions  and specifications below apply to analysis of those
       compounds only.
       10.2.1  Measure the SICP areas for each analyte, and compute the ion  abundance  ratios at the
             exact m/z's specified in Table 8. Compare the computed ratio  to the theoretical ratio
             given in Table 9.
            10.2.1.1  The exact m/z's to be monitored in each descriptor are  shown in Table 8. Each
                     group or descriptor shall be monitored in succession as a function  of GC
                     retention time to ensure that all CDDs/CDFs are  detected. Additional m/z's may
                     be monitored in each descriptor, and the m/z's  may be divided among  more than
                     the five descriptors listed in Table 8, provided that the laboratory is able to
                     monitor  the m/z's of all the CDDs/CDFs that may elute from the GC in a given
                     retention-time window. If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be
                     determined, the descriptors may be modified to include only the exact m/z's for
                     the tetra- and penta-isomers, the diphenyl ethers,  and the lock m/z's.
            10.2.1.2  The mass spectrometer shall be operated in a mass-drift correction  mode, using
                     perfluorokerosene (PFK) to  provide lock m/z's. The lock-mass  for  each group of
                     m/z's is  shown  in Table  8. Each lock mass shall  be monitored and shall not vary
                     by more than ±20% throughout its respective retention time window. Variations
                     of the lock mass by more than 20% indicate the presence of coeluting
                     interferences that may significantly reduce  the sensitivity of the mass
                     spectrometer. Reinjection of another aliquot of the sample extract will not resolve
                     the problem. Additional cleanup of the extract may be required to remove the
                     interferences.
       10.2.2  All CDDs/CDFs and labeled compounds in the CS1 standard shall be within the QC
             limits in Table 9 for their respective ion abundance ratios; otherwise, the mass
             spectrometer shall be adjusted and this test repeated until the m/z ratios fall within the
             limits specified.  If the adjustment alters the resolution of the mass spectrometer,
             resolution shall be verified (Section 10.1.2) prior to repeat of the test.

22

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                                                                                     Method 1613
       10.2.3 Verify that the HRGC/HRMS instrument meets the minimum levels in Table 2. The
             peaks representing the CDDs/CDFs and labeled compounds in the CS1 calibration
             standard must have signal-to-noise ratios (S/N) greater than or equal to 10.0. Otherwise,
             the mass spectrometer shall be adjusted and this test repeated until the minimum levels in
             Table 2 are met.
       10.2.4 The absolute retention time of I3C,2-1,2,3,4-TCDD (Section 7.12) shall exceed 25.0
             minutes on the DB-5 column, and the retention time of 13C12-1,2,3,4-TCDD shall exceed
             15.0 minutes on the  DB-225  column; otherwise, the GC temperature program shall be
             adjusted and this test repeated until the above-stated minimum retention time criteria are
             met.
10.3    Reicntion-time windows—Analyze the window defining mixtures (Section 7.15) using the
       optimized temperature program in Section  10.1. Table 5 gives the elution order (first/last) of the
       window-defining compounds. If 2,3,7,8-TCDD and 2,3,7,8-TCDF only are to  be analyzed, this
       test is not required.
10.4    Isomer specificity
       10.4.1 Analyze the isomer specificity test standards (Section 7.15) using the procedure in
             Section 14 and the optimized conditions for sample analysis (Section 10.1.1).
       10.4.2 Compute the percent valley between the GC peaks that elute most closely to the 2,3,7,8-
             TCDD and TCDF isomers, on their respective columns, per Figures 6 and 7.
       10.4.3 Verify that the height of the valley between the most closely eluted isomers and the
             2,3,7,8-substituted isomers is less than 25% (computed as 100 x/y in Figures 6 and 7). If
             the valley exceeds 25%, adjust the analytical conditions and repeat the test or replace the
             GC column and recalibrate (Sections 10.1.2 through 10.7).
10.5    Calibration by isotope dilution—Isotope dilution calibration is used for the fifteen 2,3,7,8-
       substituted CDDs/CDFs for  which labeled  compounds are added to samples prior to extraction.
       The reference compound for each CDD/CDF compound is shown in Table 2.
       10.5.1 A calibration curve encompassing the concentration range is prepared  for each compound
             to be determined. The relative response (RR)  (labeled to native) vs. concentration in
             standard solutions is plotted or computed using a linear regression. Relative response  is
             determined according to the procedures described below. Five calibration points are
             employed.
       10.5.2 The response of each CDD/CDF relative to its labeled analog is determined using the
             area responses of both the primary and secondary exact m/z's specified in Table 8, for
             each calibration standard, as follows:
                                          _ (Aln  + A2n) C,
                                            (41,  + A2) Cn
  Where:
  Aln  and A2n = The  areas of the primary and secondary mfz!s for the CDDfCDF.
  Alt and A2l = The  areas of the primary and secondary m/z's for the labeled compound.
            C{ - The  concentration of the labeled compound in the calibration standard (Table  4).
            Cn = The  concentration of the native compound in  the  calibration standard (Table 4).

                                                                                              23

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  Method 1613
 10.6
  10.5.3 To calibrate the analytical system by isotope dilution, inject a volume of calibration
        standards CS1 through CSS (Section 7.13 and Table 4) identical to the volume chosen in
        Section 10.2, using the procedure in Section  14 and the conditions in Section 10.1.1 and
        Table 2. Compute the relative response (RR) at each concentration.
  10.5.4 Linearity—If the relative response for any compound is constant (less than 20%
        coefficient of variation) over the  five-point calibration range, an averaged relative
        response may be used for that compound; otherwise, the complete calibration curve for
        that compound shall be used over the five-point calibration range.
 Calibration by internal standard—The internal standard method is  applied to determination of
 1,2,3,7,8,9-HxCDD (Section 17.1.2), OCDF (Section 17.1.1), the non-2,3,7,8-substitute
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                                                                                         Method 1613
   10.8   Data storage—MS data shall be collected, recorded, and stored.
         10.8.1  Data acquisition—The signal at each exact m/z shall be collected repetitively throughout
                the monitoring period and stored on a mass storage device.
         10.8.2  Response factors and multipoint calibrations—The data system shall be used to record
                and maintain lists of response factors (response ratios for isotope dilution) and multipoint
                calibration curves. Computations of relative standard deviation (coefficient of variation)
                shall be used to test calibration linearity. Statistics on initial performance (Section 9.2)
                and ongoing performance (Section  15.5) should be computed and maintained, either on
                the instrument data system, or on a separate computer system.

11.0   Sample Preparation

  11.1   Sample preparation involves modifying the physical form of the sample so that the CDDs/CDFs
        can be extracted efficiently.  In general, the samples must be in a liquid form or in the form of
        finely divided solids in order for efficient extraction to take place. Table 10 lists the phases and
        suggested quantities for extraction  of various sample matrices.
        For samples known or expected to contain high levels of the CDDs/CDFs, the  smallest sample
        size representative of the entire sample should be used (see Section 17.5).
        For all samples, the blank and IPR/OPR aliquots must be processed through the same steps as
        the sample to check for contamination and losses in the preparation processes.
      t 11.1.1  For samples that contain particles, percent solids and particle size are determined using
               the procedures in Sections  11.2 and 11.3, respectively.
        11.1.2  Aqueous samples—Because CDDs/CDFs may be bound to suspended particles, the
               preparation of aqueous samples is dependent on the solids content of the sample.
             11.1.2.1  Aqueous samples visibly absent particles are prepared per Section 11.4 and
                      extracted directly using the separatory funnel or SPE techniques in Sections 12.1
                      or 12.2, respectively.
             11.1.2.2  Aqueous samples containing visible particles and containing one percent
                      suspended solids or less are prepared using  the procedure in Section 11.4. After
                      preparation, the sample is extracted directly using the SPE technique in 12.2 or
                      filtered per Section  11.4.3. After filtration, the particles  and filter are extracted
                      using the SDS procedure in Section  12.3 and the filtrate is extracted using the
                      separatory funnel procedure in Section  12.1.
             11.1 A3  For aqueous samples containing greater than one  percent solids,  a sample aliquot
                      sufficient to provide 10 g of dry solids is used, as described in Section 11.5.
       11.1.3  Solid samples are prepared using the procedure described in Section 11.5 followed by
           .   extraction via the SDS procedure in Section 12.3.
       11.1.4  Multiphase samples—The phase(s) containing the CDDs/CDFs is separated from the non-
              CDD/CDF phase using pressure filtration and centrifugation, as  described in Section
              11.6. The CDDs/CDFs will be in the organic phase in a multiphase sample in which an
              organic phase exists.
                                                                                               25

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 Method 1613
       11.1.5  Procedures for grinding, homogenization, and blending of various sample phases are
              given in Section 11.7.
       11.1.6  Tissue samples—Preparation procedures for fish and other tissues are given in Section
    \          11.8.
11.2;   Determination of percent suspended solids.

    Note:   This aliquot is used for determining the solids content of the sample, not for
    determination of CDDs/CDFs.
    l
    i
       11.2.1   Aqueous  liquids and multi-phase samples consisting of mainly an aqueous phase.
             11.2.1.1  Dessicate and weigh a GF/D filter (Section 6.5.3) to three significant figures.
             11.2.1.2 Filter 10.0 ± 0.02 mL of well-mixed sample through the filter.
             11.2.1.3 Dry the filter a minimum of 12 hours  at 110 ± 5°C arid cool in a dessicator.
             11.2.1.4 Calculate percent solids  as follows:

               ,-j     weight of sample aliquot after drying (g) - weight of filter (g)    inn
          % solids  =	—	=	—. x  1UU
                                                   10 g

       11.2.2  Non-aqueous liquids, solids, semi-solid samples, and multi-phase samples in which the
              main phase is not  aqueous; but not tissues.
             11.2.2.1 Weigh 5 to 10 g of sample to three significant figures in  a tared beaker.
             11.2.2.2 Dry a minimum of 12 hours at 110 ± 5°C, and cool in a  dessicator.
             11.2.2.3 Calculate percent solids  as follows:                 ;
                                                                        i
                      _,    ...     weight of  sample aliquot after drying
                      %  so lias =	—:	—;—  x
                                  weight of sample aliquot before drying
11.3   Determination of particle size.                                     ;
       11.3.1  Spread the dried sample from Section 11.2.2.2 on a piece of filter paper or aluminum foil
    i          in a fume hood or glove box.
    I   11.3.2  Estimate the size of the particles in the sample. If the size of the largest particles is
    i          greater than  1 mm, the particle size must be reduced to 1 mm or less prior to extraction
    i          using the procedures in Section 11.7.
11.4   Preparation of aqueous samples containing one percent suspended solids or less.
    !   11.4.1  Aqueous samples visibly absent particles are prepared per the procedure below and
              extracted directly using the separatory funnel or SPE techniques in Sections 12.1  or 12.2,
              respectively. Aqueous samples containing visible particles and one percent suspended
              solids or less are prepared using the procedure below and extracted using either the SPE

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                                                                                       Method 1613
             technique in Section 12.2 or further prepared using the filtration procedure in Section
             11.4.3. The filtration procedure is followed by  SDS extraction of the filter and particles
             (Section 12.3) and separatory  runnel extraction of the  filtrate (Section 12.1). The SPE
             procedure is followed by SDS extraction of the filter and disk.
      11.4.2  Preparation of sample and QC aliquots.
            11.4.2.1  Mark the original level of the sample on the sample bottle for reference. Weigh
                     the  sample plus bottle to  ±1 g.
            11.4.2.2-  Spike 1.0 mL of the diluted labeled-compound spiking solution (Section 7.10.3)
                     into the sample bottle. Cap the bottle and mix the sample by careful shaking.
                     Allow the sample to equilibrate for 1 to 2 hours,  with occasional shaking.
            11.4.2.3  For each sample or  sample batch (to a  maximum of 20 samples) to be extracted
                     during the same 12-hour  shift, place two 1.0-L aliquots of reagent water in clean
                     sample bottles  or flasks.
            11.4.2.4  Spike 1.0 mL of the diluted labeled-compound spiking solution (Section 7.10.3)
                     into both reagent water aliquots. One of these  aliquots will serve as the method
                     blank.
            11.4.2.5  Spike 1.0 mL of the PAR standard (Section 7.14) into the remaining reagent
                     water aliquot. This aliquot will serve as the OPR (Section 15.5).
            11.4.2.6  If SPE is to be used, add 5 mL of methanol to the sample, cap and shake the
                     sample to mix thoroughly, and proceed to Section 12.2 for extraction. If SPE is
                     not to be used,  and  the sample is visibly absent particles, proceed to Section 12.1
                     for  extraction.  If SPE is not to be used and the sample contains visible particles,
                     proceed to the following  section for filtration of particles.
      11.4.3  Filtration of particles.
            11.4.3.1  Assemble a Buchner funnel (Section 6.5.5) on top of a clean filtration flask.
                     Apply vacuum  to the  flask, and pour the entire contents of the sample bottle
                     through a glass-fiber filter (Section 6.5.6) in the Buchner funnel, swirling the
                     sample remaining in the bottle to  suspend any particles.
            11.4.3.2  Rinse the sample bottle twice with approximately 5-mL portions of reagent water
                     to transfer any  remaining particles onto the  filter.
            11.4.3.3  Rinse any particles  off the sides of the Buchner funnel with small quantities of
                     reagent water.
            11.4.3.4  Weigh the empty sample bottle to ±1  g. Determine the weight of the  sample by
                     difference. Save the bottle for further use.
            11.4.3.5  Extract the filtrate using  the separatory funnel procedure in Section 12.1.
            11.4.3.6  Extract the filter containing the particles using the SDS procedure  in  Section
                     12.3.
11.5  Preparation of samples containing greater than one percent solids.
                                                                                                27

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   \Method1613
 11,6
11.7
   11.5.1  Weigh a well-mixed aliquot.of each sample (of the same matrix type) sufficient to
          provide 10 g of dry solids (based on the solids determination in Section 11.2) into a
          clean beaker or glass jar.
   11.5.2  Spike 1.0 mL of the diluted labeled compound spiking solution (Section 7.10.3) into the
          sample.
   11.5.3  For each sample or sample batch (to a maximum of 20 samples) to be extracted during
          the same 12 hour shift, weigh two  10-g aliquots of the appropriate reference matrix
          (Section 7.6) into clean beakers or glass jars.
   11.5.4  Spike  1.0 mL of the diluted labeled compound spiking solution (Section 7.10.3) into each
          reference matrix aliquot. One aliquot will serve as the  method blank. Spike  1.0 mL of the.
          PAR standard (Section 7.14) into the other reference matrix aliquot. This aliquot will
          serve as the OPR (Section 15.5).                        (
  11.5.5   Stir or tumble and equilibrate the aliquots for  1 to 2 hours.
  11.5.6   Decant excess water. If necessary to remove water, filter the sample through a glass-fiber
          filter and discard the aqueous liquid.
  11.5.7  If particles >1 mm are present in the sample (as determined in Section  11.3.2), spread the
         sample on clean aluminum foil  in a hood. After the sample is dry, grind to reduce the
         particle size (Section 11.7).                              !
  11.5.8  Extract the sample and QC aliquots using the SDS procedure in Section 12.3.
•  Multiphase samples.
  11.6.1  Using the percent solids determined in Section 11.2.1 or 11.2.2, determine the volume of
         sample that will  provide 10 g of solids, up to 1 L of sample.
  11.6.2  Pressure filter the amount of sample determined in Section 11.6.1 through Whatman
         GF/D glass-fiber filter paper (Section 6.5.3). Pressure filter the blank and OPR aliquots
         through  GF/D papers also. If necessary to separate the phases and/or settle the solids,
         centrifuge these aliquots prior to filtration.
  11.6.3  Discard any aqueous phase (if present). Remove any non-aqueous liquid present and
         reserve the maximum amount filtered from the  sample (Section 11.6.1) or 10 g,
         whichever is less, for combination with the solid phase  (Section 12.3.5).
  11.6.4  If particles >1  mm are present in the sample  (as determined in Section  11.3.2) and the
         sample is capable of being dried, spread the sample and QC aliquots on clean aluminum
         foil in a hood. After the aliquots  are dry or if the sample cannot be dried, reduce the
        particle size using the procedures in  Section 11.7 and extract the reduced particles using
        the SDS procedure in Section 12.3.  If particles  >1  mm are not present, extract the
        particles and filter in the sample and QC aliquots directly using the SDS procedure in
        Section  12.3.
 Sample grinding, homogenization, or blending—Samples with particle sizes greater than 1 mm
 (as determined in Section 11.3.2) are subjected to grinding, homogenization, or blending. The
 method of reducing particle size to less than 1 mm is matrix-dependent. In general, hard particles
 28

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                                                                                      Meuioa
      can be reduced by grinding with a mortar and pestle. Softer particles can be reduced by grinding
      in a Wiley mill or meat grinder, by homogenization, or in a blender.
      11.7.1  Each size-reducing preparation procedure on each matrix shall be verified by running the
             tests in Section 9.2 before the procedure is employed routinely.
      11.7.2 The grinding, homogenization, or blending procedures shall be carried out in a glove box
             or fume hood to prevent particles from contaminating the work environment.
      11.7.3 Grinding—Certain papers and pulps, slurries, and amorphous solids can be ground in a
             Wiley mill or heavy duty meat grinder. In some cases, reducing the temperature of the
             sample to freezing or to dry ice or liquid nitrogen temperatures can aid in the grinding
             process. Grind the sample aliquots from  Sections 11.5.7 or 11.6.4 in a clean grinder. Do
             not allow the sample temperature to exceed 50°C. Grind the blank and reference matrix
             aliquots using a clean grinder.
      11.7.4 Homogenization or blending—Particles that are not ground effectively, or particles
             greater than  1 mm in size after grinding, can often be reduced in size by high speed
             homogenization or blending. Homogenize and/or blend the particles or filter from
             Sections  11.5.7 or 11.6.4  for the sample, blank, and  OPR aliquots.
      11.7.5 Extract the aliquots using the SDS procedure in Section 12.3.
11.8  Fish and other tissues—Prior to processing tissue samples, the laboratory must determine the
      exact tissue to be analyzed. Common requests for analysis of fish tissue include whole fish-skin
      on, whole fish-skin  removed, edible fish fillets (filleted in the field or by the laboratory),
      specific organs, and other portions. Once the appropriate tissue has been determined, the sample
      must be homogenized.
      11.8.1 Homogenization.
            11.8.1.1  Samples are homogenized while still frozen, where practical. If the laboratory
                     must dissect the whole fish to obtain the appropriate tissue for analysis, the
                     unused tissues may be rapidly refrozen and stored in a clean glass jar for
                     subsequent use.
            11.8.1.2  Each analysis requires 10 g of tissue (wet weight). Therefore, the laboratory
                     should homogenize at least 20 g of tissue to allow for re-extraction of a second
                     aliquot of the same homogenized sample, if re-analysis is required. When whole
                     fish  analysis is  necessary, the entire fish  is homogenized.
            11.8.1.3  Homogenize the sample in a tissue homogenizer (Section 6.3.3) or grind in a
                     meat grinder (Section 6.3.4). Cut tissue too large to feed into the grinder into
                     smaller pieces.  To assure homogeneity, grind three times.
            11.8.1.4  Transfer approximately  10 g (wet weight) of homogenized tissue to a clean,
                     tared, 400- to 500-mL beaker. For the alternate HC1 digestion/extraction, transfer
                     the tissue to a clean, tared 500- to 600-mL wide-mouth bottle. Record the weight
                     to the nearest 10  mg.
                                                                                                29

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    Method 1613
               11.8.1.5  Transfer the remaining homogenized tissue to a clean jar with a fluoropolymer-
                        lined lid. Seal the jar and store the tissue at <-10°C. Return any tissue that was
                        not homogenized to its original container and store at <-10°C.
         11.8.2  QC aliquots.                                          i
               11.8.2.1  Prepare a method  blank by adding approximately 10 g of the oily liquid reference
                        matrix (Section 7.6.4) to a 400- to 500-mL beaker. For the alternate HC1
                        digestion/extraction, add the reference matrix to a 500- to 600-mL wide-mouth
                        bottle. Record the weight to the nearest 10 mg.
               11.8.2.2  Prepare a precision and recovery aliquot by adding approximately 10 g of the
                        oily  liquid reference matrix (Section 7.6.4) to a separate 400- to 500-mL beaker ,
                        or wide-mouth bottle, depending on the extraction procedure to be used. Record
                        the weight to the nearest 10 mg. If the initial precision and recovery test is to be
                        performed, use four aliquots; if the ongoing precision and recovery test is to be
                        performed, use a single aliquot.
         11.8.3  Spiking.                                              \
              11.8.3.1  Spike 1.0 mL of the labeled compound spiking solution (Section 7.10.3) into the
                       sample, blank, and OPR aliquot.
              11.8.3.2  Spike 1.0 mL of the PAR standard (Section 7.14) into the OPR aliquot.
         11.8.4  Extract the aliquots using the procedures in Section 12.4.

12.0    Extraction  and  Concentration
   Extraction procedures include separatory funnel (Section 12.1) and solid phase (Section 12.2) for
   aqueous liquids; Soxhlet/Dean-Stark (Section 12.3) for solids, filters, and SPE disks; and Soxhlet
   sxtraction (Section  12.4.1) and HC1 digestion (Section 12.4.2) for tissues. Acid/base back-extraction
   [Section 12.5) is used for initial cleanup of extracts.

   Macro-concentration procedures include rotary evaporation (Section 12.6.1), heating mantle (Section
   12.6.2), and Kudema-Danish (K-D) evaporation (Section 12.6.3). Micro-concentration uses nitrogen
   jlowdown (Section  12.7).
  12.1   Separatory funnel extraction of filtrates and of aqueous samples visibly absent particles.
        12.1.1  Pour the spiked sample (Section 11.4.2.2) or filtrate (Section  11.4.3.5) into a 2-L
               separatory  funnel. Rinse the bottle or flask  twice with 5 mL of reagent water and add
               these rinses to the separatory funnel.
        12.1.2  Add 60 mL methylene chloride to the empty sample bottle (Section 12.1.1), seal, and
               shake 60 seconds to rinse the inner surface. Transfer the solvent to the separatory funnel,
               and extract the sample by shaking the funnel for 2 minutes with periodic venting. Allow
               the organic layer to separate from the aqueous phase for a minimum of 10 minutes. If an
               emulsion forms and  is more than one-third  the volume of the solvent layer, employ
               mechanical techniques to complete the phase separation (see note below). Drain the
               methylene chloride extract through a solvent-rinsed glass funnel approximately one-half
  30

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                                                                                       Method 1613
              full of granular anhydrous sodium sulfate (Section 7.2.1) supported on clean glass-fiber
              paper into a solvent-rinsed concentration device (Section 12.6).

    Note:  If an emulsion forms, the analyst must employ mechanical techniques to complete the
    phase separation.  The optimum technique depends upon the sample, but may include stirring,
    filtration through glass wool, use of phase separation paper, centrifugation, use of an ultrasonic
    bath with ice, addition ofNaCl, or other physical methods. Alternatively, solid-phase or other
    extraction techniques may be used to prevent emulsion formation. Any alternative technique
    acceptable so long as the requirements in Section 9 are met.
is
       Experience with aqueous samples high in dissolved organic materials (e.g., paper mill effluents)
       has shown that acidification of the sample prior to extraction  may reduce the formation of
       emulsions. Paper industry methods suggest that the addition of up to 400 mL of ethanol to a 1-L
       effluent sample may also reduce emulsion formation. However, studies by EPA suggest that the
       effect may be a result of sample dilution, and that the addition of reagent water may  serve the
       same function. Mechanical  techniques may still be necessary to complete the phase separation.  If
       either acidification or  addition of ethanol is utilized, the laboratory  must perform the  startup tests
       described in Section 9.2 using the same techniques.
       12.1.3  Extract the water sample two more times with 60-mL portions of methylene chloride.
              Drain each portion through the sodium sulfate into the concentrator. After the third
              extraction, rinse the separatory funnel with at least 20 mL of methylene chloride, and
              drain this rinse through the sodium sulfate into the concentrator. Repeat this rinse at least
              twice. Set aside the funnel with sodium sulfate if the extract is to be combined with the
              extract from the particles.
       12.1.4  Concentrate the extract using one of the macro-concentration procedures in  Section 12.6.
             12.1.4.1  If the extract is from a sample visibly absent particles (Section  11.1.2.1), adjust
                     the final volume of the concentrated extract to approximately 10 mL with hexane,
                     transfer to a 250-rnL separatory funnel, and back-extract using the procedure in
                     Section 12.5.
            12.1.4.2 If the extract is from the aqueous filtrate (Section 11.4.3.5), set aside the
                     concentration apparatus for addition of the SDS extract from the particles
                     (Section 12.3.9.1.2).
12.2  SPE of samples containing less than one percent  solids. (References 19-20).
       12.2.1   Disk preparation.
            12.2.1.1  Place an SPE disk on the base of the filter holder (Figure 4) and wet with
                     toluene. While holding a GMF 150 filter above the SPE disk with tweezers, wet
                     the filter with toluene and lay the filter on the SPE disk, making sure  that air is
                     not trapped between the filter and disk. Clamp the filter and SPE disk between
                     the 1-L glass reservoir and the vacuum filtration flask.
            12.2.1.2 Rinse the sides of the filtration flask with approx 15 mL of toluene  using a
                     squeeze bottle or syringe. Apply vacuum momentarily until a few drops appear at

                                                                                               31

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Method 1613
12
                  the drip tip. Release the vacuum and allow the filter/disk to soak for approx one
                  minute. Apply vacuum and draw all of the toluene through the filter/disk. Repeat
                  the wash step with approx 15 mL of acetone and allow the filter/disk to air dry.
          12.2.1.3  Re-wet the filter/disk with approximately  15 mL of rnethanol, allowing the
                  filter/disk to soak for approximately 1 minute. Pull the rnethanol through the
                  filter/disk using the vacuum, but retain a layer of methanol approximately 1 mm
                  thick on the  filter. Do not allow the disk to go  dry from this point until the  end
                  of the extraction.
          12.2.1.4  Rinse the filter/disk with two 50-mL portions of reagent water by adding the
                  water to the  reservoir and pulling most through, leaving a layer of water on the
                  surface of the filter.
    12.2.2  Extraction.
          12.2.2.1  Pour the spiked sample (Section 11.4.2.2), blank (Section 11.4.2.4), or IPR/OPR
                  aliquot (Section 11.4.2.5) into the reservoir and turn on the vacuum to begin the
                  extraction. Adjust the vacuum to complete the extraction in no less than 10
                  minutes. For samples containing a high concentration of particles (suspended
                  solids), filtration times may be  8 hours or longer.
          12.2.2.2 Before all of the sample has been pulled through the filter/disk, rinse the sample
                  bottle with approximately 50 mL of reagent water to remove any solids, and pour
                  into the reservoir. Pull through  the filter/disk. Use additional reagent water  rinses
                  until all visible solids are removed.                 .[
          12.2.2.3 Before all of. the sample  and  rinses have been pulled through the filter/disk, rinse
                  the sides of the reservoir with small  portions of reagent water.
          12.2.2.4  Allow the filter/disk to dry, then remove the filter and disk and place in a glass
                  Petri dish. Extract the filter and disk per Section 12.3.
,3   SDS extraction of samples containing particles, and of filters and/or disks.
    12.3.1   Charge a clean extraction thimble (Section 6.4.2.2) with 5.0 g of 100/200 mesh silica
            (Section 7.5.1.1) topped with 100 g of quartz sand (Section 7.3.2).
    Note:  Do not disturb the silica layer throughout the extraction process.
       12.3.2  Place the thimble in a clean extractor. Place 30 to 40 mL of toluene in the receiver and
              200 to 250 mL of toluene in the flask.                     <
       12.3.3  Pre-extract the glassware by heating the flask until the toluene is boiling. When properly
              adjusted, 1 to 2 drops of toluene will fall per second from the condenser tip into the
              receiver. Extract the apparatus for a minimum of 3 hours.
       12.3.4  After pre-extraction, cool and disassemble the apparatus. Rinse the  thimble with toluene
              and allow to air dry.
       12.3.5  Load the wet sample, filter, and/or disk from Sections  11.4.3.6,  11.5.8, 11.6.4,  11.7.3,
               11.7.4, or 12.2.2,4 and any nonaqueous liquid from Section 11.6.3 into the thimble and
  32

-------
                                                                                        Method 1613
              manually mix into the sand layer with a clean metal spatula, carefully breaking up any
              large lumps of sample.
       12.3.6  Reassemble the pre-extracted SDS  apparatus, and add a fresh charge of toluene to the
              receiver and reflux flask. Apply power to the heating mantle to begin refluxing. Adjust
              the reflux rate to match the rate of percolation through the sand and silica beds until
              water removal lessens the restriction to toluene flow. Frequently check the apparatus for
              foaming during  the first 2 hours of extraction. If foaming  occurs, reduce the reflux rate
              until  foaming subsides.
       12.3.7  Drain the water from the receiver at 1 to 2 hours  and 8 to 9 hours, or sooner if the
              receiver fills with water. Reflux the sample for a  total of 16 to 24 hours.  Cool and
              disassemble the apparatus. Record the total volume of water collected.
       12.3.8  Remove the distilling flask. Drain the water from the Dean-Stark receiver and add any
              toluene in the receiver to the extract in the flask.
       12.3.9  Concentrate the extract using one of the macro-concentration procedures in Section 12.6
              per the following:
             12.3.9.1  Extracts from the particles in an aqueous sample containing less than  one  percent
                      solids (Section 11.4.3.6).
                     12.3.9.1.1   Concentrate the extract to approximately 5 mL using the rotary
                               evaporator or heating mantle procedures  in Sections 12.6.1 or 12.6.2.
                     12.3.9.1.2   Quantitatively transfer the extract through the sodium sulfate (Section
                               12.1.3) into the apparatus that was set aside (Section 12.1.4.2) and
                               reconcentrate to the level of the  toluene.
                     12.3.9.1.3   Adjust to approximately 10 mL  with hexane, transfer to a 250-mL
                               separatory funnel, and proceed with back-extraction (Section 12.5).
             12.3.9.2  Extracts from particles (Sections 11.5-11.6) or from the SPE filter and disk
                      (Section 12.2.2.4)—Concentrate to approximately 10 mL using the rotary
                      evaporator or heating mantle (Section 12.6.1 or  12.6.2), transfer to a 250-mL
                      separatory funnel, and proceed with back-extraction (Section  12.5).
12.4   Extraction of tissue—Two procedures are provided for tissue extraction.
       12.4.1  Soxhlet extraction (Reference 21).
             12.4.1.1  Add 30 to 40 g of powdered anhydrous sodium sulfate to each of the beakers
                      (Section 11.8.4) and mix thoroughly. Cover the beakers with aluminum foil and
                      allow to equilibrate  for 12-24 hours. Remix prior to extraction to prevent
                      clumping.
             12.4.1.2  Assemble and pre-extract the Soxhlet apparatus per Sections 12.3.1-12.3.4, except
                      use the methylene chloride:hexane (1:1) mixture for the pre-extraction and rinsing
                      and omit the quartz sand. The Dean-Stark moisture trap may also be omitted, if
                      desired.
             12.4.1.3  Reassemble the pre-extracted Soxhlet apparatus and add a fresh charge of
                      methylene chloride:hexane to the reflux flask.

                                                                                                33

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Method 1613
           12.4.1.4  Transfer the sample/sodium sulfate mixture (Section 12.4.1.1) to the Soxhlet
                    thimble, and install the thimble in the Soxhlet apparatus.
           12.4.1.5  Rinse the beaker with  several portions of solvent mixture and add to the thimble.
                    Fill the thimble/receiver with solvent. Extract for 18 to 24 hours.
           12.4.1.6  After extraction, cool and disassemble the apparatus.
           12.4.1.7  Quantitatively transfer the extract to a macro-concentration device (Section 12.6),
                    and concentrate to near dryness. Set aside the concentration apparatus for re-use.'
           12.4.1.8  Complete the removal  of the solvent using the nitrogen blowdown procedure
                    (Section  12.7)  and a water bath temperature of 60°C. Weigh the receiver, record
                    the weight, and return the receiver to the blowdown apparatus, concentrating the  <
                    residue until a constant weight  is obtained.
           12.4.1.9  Percent lipid determination— The lipid content is determined by extraction of
                    tissue with the same solvent system (methylene chloriderhexane) that was used in
                    EPA's National Dioxin Study (Reference 22) so that lipid contents are consistent
                    with that study.
                  12.4.1.9.1   Redissolve the residue in the receiver in hexane and spike  1.0 mL of
                             the cleanup standard (Section 7.1 1) into the solution.
                  12.4.1.9.2   Transfer the residue/hexane to the anthropogenic isolation column
                             (Section 13.7.1) or bottle for the acidified silica gel batch cleanup
                             (Section 13.7.2),  retaining the boiling chips in the concentration
                             apparatus.  Use several rinses to assure that all material is transferred. If
                             necessary,  sonicate or heat the receiver slightly to assure that all
                             material  is re-dissolved. Allow the receiver to dry. Weigh the receiver
                            and boiling chips.
                  12.4.1.9.3  Calculate the lipid content to the nearest three significant figures as
                            follows:
                         Percent lipid =  w^Sht of residue (g)  x m
                                           Weight of tissue (g)


                 12.4.1.9.4  It is not necessary to determine the lipid content of the blank, DPR, or
                            OPR aliquots.
    12.4.2  HC1 digestion/extraction and concentration (References 23-2(5).
          12.4.2.1  Add 200 mL of 6 N HC1 and 200 mL of methylene chloride:hexane (1:1) to the
                  sample and QC aliquots (Section 11.8.4).
          12.4.2.2  Cap and shake each bottle 1 to 3 times. Loosen the cap in a hood to vent excess
                  pressure. Shake each bottle for 10 to 30 seconds and vent.
          12.4.2.3  Tightly cap and place on shaker. Adjust the shaker action and speed so that the
                  acid, solvent, and tissue  are in constant motion. However, take care to avoid such

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                                                                                         Method 1613
                       violent action that the bottle may be dislodged from the shaker. Shake for 12 to
                       24 hours.
              12.4.2.4  After digestion, remove the bottles from the shaker. Allow the bottles to stand so
                       that the solvent and acid layers separate.
              12.4.2.5  Decant the solvent through a glass  funnel with glass-fiber filter (Sections  6.5.2-
                       6.5.3)  containing approximately 10 grams of granular anhydrous sodium sulfate
                       (Section 7.2.1) into a macro-concentration apparatus (Section  12.6). Rinse the
                       contents of the bottle with two 25-mL portions of hexane and pour through the
                       sodium sulfate into the apparatus.
              12.4.2.6   Concentrate the solvent to near dryness using a macro-concentration procedure
                       (Section 12.6).
              12.4.2.7  Complete the removal of the solvent using the nitrogen  blowdown apparatus
                      (Section 12.7) and a water bath temperature of 60°C. Weigh the receiver,  record
                      the weight, and return the receiver to the blowdown apparatus, concentrating  the
                      residue until a constant weight is obtained.
             12.4.2.8  Percent lipid determination—The lipid content is determined in the same solvent
                      system [memylene chloride:hexane (1:1)] that was used  in EPA's National Dioxin
                      Study (Reference 22) so that lipid contents are consistent with that study.
                     12.4.2.8.1  Redissolve the residue in the receiver in hexane and  spike 1.0  mL of
                               the cleanup standard (Section 7.11) into the solution.
       '              12.4.2.8.2  Transfer the residue/hexane to the narrow-mouth 100- to 200-mL bottle
                               retaining the boiling chips in  the receiver. Use several rinses to assure
                               that all material is transferred, to a maximum hexane volume of
                               approximately 70 mL. Allow the receiver to dry. Weigh the receiver
                               and boiling chips.
                    12.4.2.8.3  Calculate the percent lipid per Section 12.4.1.9.3. It is not necessary to
                               determine the lipid content of the blank, IPR, or OPR aliquots.
             12.4.2.9  Clean up the extract per Section 13.7.3.
12.5   Back-extraction with base and acid.
       12,5.1  Spike 1.0 mL of the cleanup standard (Section  7.11) into the separately funnels
              containing the sample and QC extracts from Section 12.1.4.1, 12.3.9.1.3, or 12.3.9.2.
       12.5.2  Partition the extract against 50 mL of potassium hydroxide solution (Section 7.1.1).
              Shake for 2 minutes with periodic venting into  a hood. Remove  and discard the aqueous
              layer. Repeat the base washing until no color is visible in the aqueous  layer, to a
              maximum of four washings. Minimize contact time between the  extract and the base to
              prevent degradation of the CDDs/CDFs. Stronger potassium hydroxide solutions  may  be
              employed for back-extraction, provided that  the laboratory meets the specifications for
              labeled compound recovery and demonstrates acceptable performance using the
              procedure in Section 9.2.
                                                                                                35

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 Method 1613
       12.5.3  Partition the extract against 50 mL of sodium chloride solution (Section 7.1.4) in the
              .same way as with base. Discard  the aqueous  layer.
       12.5.4  Partition the extract against 50 mL of sulfuric acid (Section 7.1.2) in the same way as
              with base. Repeat the acid washing until no color is visible in  the aqueous layer, to a
              maximum of four washings.
       12.5.5  Repeat the partitioning against sodium chloride solution  and discard the aqueous layer.
       12.5.6  Pour each extract through a drying column containing 7  to  10  cm of granular anhydrous
              sodium sulfate (Section 7.2.1). Rinse the separatory funnel with 30 to 50 mL of solvent,
              and pour through the drying column. Collect  each extract in a  round-bottom flask. Re-
              concentrate the sample and QC aliquots per Sections 12.6-12.7, and clean up the samples
              and QC aliquots  per Section 13.
12'.6   Macro-concentration—Extracts in toluene are concentrated using a rotary evaporator or a heating
       mantle; extracts in methylene chloride or hexane are  concentrated using a rotary evaporator,
       heating mantle, or Kuderna-Danish apparatus.
       12.6.1  Rotary evaporation—Concentrate the extracts in separate round-bottom flasks.
            12.6.1.1  Assemble the rotary evaporator according to manufacturer's instructions, and
                     warm the water bath to 45°C. On a daily basis, preclean the rotary evaporator by
                     concentrating 100 mL of clean extraction solvent through the system. Archive
                     both the concentrated solvent and the solvent in  the catch flask for a
                     contamination check if necessary. Between samples, three 2- to 3-mL aliquots of
                     solvent should be rinsed down the feed  tube into a waste beaker.
            12.6.1.2  Attach the round-bottom  flask containing the sample extract to the rotary
                     evaporator. Slowly apply vacuum to the system,  and begin rotating the sample
                     flask.
            12.6.1.3  Lower the flask into the water bath, and adjust the speed of rotation  and the
                     temperature as required to complete concentration in 15 to 20 minutes. At the
                     proper rate of concentration, the flow of solvent  into the receiving flask will be
                     steady, but no bumping or visible boiling of the  extract will occur.
    Note:   // the rate of concentration is too fast, analyte loss may occur.
             12.6.1.4  When the liquid in the concentration flask has reached an apparent volume of
                     approximately 2 mL, remove the flask from the water bath and stop the rotation.
                     Slowly and carefully admit air into the system. Be sure not to open the valve so
                     quickly that the sample is blown out of the flask. Rinse the feed tube with
                     approximately 2 mL of solvent.
             12.6.1.5  Proceed to Section 12.6.4 for preparation for back-extraction  or micro-
                     concentration and solvent exchange.               \
       12.6.2  Heating mantle—Concentrate the extracts in separate round-bottom flasks.
 36

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                                                                                Method 1613
      12.6.2.1  Add one or two clean boiling chips to the round-bottom flask, and attach a three-
               ball macro Snyder column. Prewet the column by adding approximately 1 mL of
               solvent through the top. Place the round-bottom flask in a heating mantle, and
               apply  heat as required to complete the concentration in  15 to 20 minutes. At the
               proper rate of distillation, the balls of the column will actively chatter, but the
               chambers  will not flood.
      12.6.2.2  When the  liquid has reached an apparent volume of approximately 10 mL,
               remove the round-bottom flask from the heating mantle and allow the solvent to
               drain and cool for at  least  10 minutes.  Remove the  Snyder column and rinse the
               glass joint into the receiver with small portions of solvent.
      12.6.2.3  Proceed to Section 12.6.4 for preparation for back-extraction or micro-
               concentration and solvent exchange.
12.6.3  Kudema-Danish (K-D)—Concentrate the extracts in separate 500-mL K-D flasks
       equipped with 10-mL concentrator tubes. The K-D technique is used for solvents such as
       methylene chloride and hexane. Toluene is difficult to concentrate using the K-D technique
        unless a water bath  fed by a steam generator is used.
      12.6.3.1  Add 1 to 2 clean boiling chips to the receiver. Attach a three-ball macro Snyder
               column. Prewet the column by adding approximately 1 mL of solvent through the
               top. Place  the K-D apparatus in a hot water bath so that the  entire lower rounded
               surface of  the flask is bathed with steam.
      12.6.3.2  Adjust the vertical position of the apparatus and the water temperature as
               required to complete the concentration in 15 to 20 minutes. At the proper rate of
               distillation, the balls of the column will actively chatter but the chambers will not
               flood.
      12.6.3.3  When  the  liquid has reached an apparent volume of 1 mL, remove the K-D
               apparatus from the bath and allow the solvent to drain and cool for at least 10
               minutes. Remove the Snyder column and rinse the flask and its  lower joint into
               the concentrator tube with  1 to 2 mL of solvent. A 5-mL syringe is recommended
               for this operation.
      12.6.3.4  Remove the three-ball Snyder column, add  a fresh boiling chip, and attach a two
               ball micro  Snyder column to the concentrator tube.  Prewet the column by adding
               approximately 0.5 mL of solvent through the top. Place  the apparatus  in the hot
               water bath.
      12.6.3.5  Adjust the vertical position and the water temperature as required to complete the
               concentration in 5 to  10 minutes. At the proper rate of distillation, the balls of the
               column will actively chatter but the chambers will not flood.
     ' 12.6.3.6  When  the liquid reaches an apparent volume of 0.5  mL, remove the apparatus
               from the water bath and allow to drain and cool for at least 10 minutes.
      12.6.3.7  Proceed  to 12.6.4 for preparation for back-extraction or  micro-concentration and
               solvent exchange.
12.6.4  Preparation for back-extraction or micro-concentration and solvent exchange.

                                                                                         37

-------
 Method 1613
            12.6.4.1  For back-extraction (Section 12.5), transfer the extract to a 250-mL separatory
                     funnel. Rinse the concentration vessel with small portions of hexane, adjust the
                     hexane volume in the separatory funnel to 10 to 20 mL, and proceed to back-
                     extraction (Section 12.5).
            12.6.4.2  For determination of the weight of residue in the extract, or for clean-up
                     procedures other than back-extraction, transfer the extract to a blowdown vial
                     using 2-3 rinses of solvent. Proceed with micro-concentration and solvent
                     exchange (Section  12.7).
127   Micro-concentration and solvent exchange.
      12.7.1   Extracts to be subjected to GPC or HPLC cleanup are exchanged into methylene
              chloride. Extracts to be cleaned up using  silica gel, alumina, carbon, and/or Florisil are
              exchanged into hexane.
      12.7.2   Transfer the vial containing the sample extract to a nitrogen blowdown  device. Adjust the
              flow of nitrogen  so that the surface of the solvent is just visibly disturbed.

   Note:  A large vortex in the solvent may cause analyte loss.
       12.7.3  Lower the vial into a 45°C water bath and continue concentrating.
            12.7.3.1  If the extract is to be concentrated to dry ness for weight determination (Sections
                     12.4.1.8, 12.4.2.7, and  13.7.1.4), blow dry until a constant weight is obtained.
            12.7.3.2  If the extract is to be concentrated for injection into the GC/MS or the solvent is
                     to be exchanged for extract cleanup, proceed as follows:
       12.7.4  When the volume of the  liquid is approximately 100 uL, add 2 to 3 mL of the desired
              solvent (methylene chloride for GPC and HPLC, or hexane for the other cleanups) and
              continue  concentration to approximately 100 uL. Repeat the addition of solvent and
              concentrate once more.
       12.7.5  If the extract is to be cleaned up by GPC, adjust the volume of the extract to 5.0 mL
              with methylene chloride. If the extract is to be cleaned up by HPLC, further concentrate
             - the extract to 30 uL. Proceed with GPC or HPLC cleanup (Section 13.2 or 13.6,
              respectively).
       12.7.6  If the extract is to be cleaned up by column chromatography (alumina, silica gel,
              Carbopak/Celite, or Florisil), bring the final volume to 1.0 mL with hexane. Proceed with
              column cleanups (Sections 13.3 - 13.5 and 13.8).
       12.7.7  If the extract is to be concentrated for injection into the GCfMS (Section  14),
              quantitatively transfer the extract to a 0.3-mL conical  vial  for final concentration, rinsing
              the  larger vial with hexane and adding the rinse to the conical  vial. Reduce the volume to
              approximately 100 yL. Add 10 uL of nonane to the vial, and evaporate the solvent to the
              level of the  nonane. Seal the vial and label with the sample number. Store in the dark at
              room temperature until ready for GC/MS analysis. If GC/MS analysis will not be
              performed on the same day, store the vial at <-10°C.

-------
                                                                                        Method 1613
13.0   Extract Cleanup

  13.1   Cleanup may not be necessary for relatively clean samples (e.g., treated effluents, groundwater,
        drinking water). If particular circumstances require the use of a cleanup procedure, the analyst
        may use any or all of the procedures below or any other appropriate procedure. Before using a
        cleanup procedure, the analyst must demonstrate that the requirements of Section 9.2 can be met
        using the cleanup procedure. If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be determined, the
        cleanup procedures may  be optimized for isolation of these two compounds.
        13.1.1  Gel permeation chromatography (Section  13.2) removes high molecular weight
               interferences that cause GC column performance to degrade. It should be used for all soil
               and sediment extracts and may be used for water extracts that are expected to contain
               high molecular weight organic compounds (e.g., polymeric materials, humic acids).
        13.1.2  Acid, neutral, and basic silica gel (Section 13.3), alumina (Section 13.4), and Florisil
               (Section 13.8) are used to remove nonpolar and polar interferences. Alumina and Florisil
               are used to remove chlorodiphenyl ethers.
        13.1.3  Carbopak/Celite (Section 13.5)  is used to  remove nonpolar interferences.
        13.1.4  HPLC (Section 13.6) is used to provide specificity for the 2,3,7,8-substituted and other
               CDD and CDF isomers.
        13.1.5  The anthropogenic isolation column (Section  13.7.1), acidified silica gel  batch adsorption
               procedure (Section 13.7.2), and sulfuric acid and base back-extraction (Section 13.7.3)
               are used for removal of lipids from tissue samples.
  13.2   Gel permeation chromatography (GPC).
        13.2.1  Column packing.
              13.2.1.1   Place 70 to 75 g of SX-3 Bio-beads (Section 6.7.1.1) in a 400- to 500-mL
                       beaker.
              13.2.1.2  Cover the beads with methylene chloride and allow to swell overnight (a
                       minimum of 12 hours).
              13.2.1.3  Transfer the swelled beads to the column (Section 6.7.1.1) and pump solvent
                       through the column, from bottom to top, at 4.5 to 5.5 mL/minute prior to
                       connecting the column to the detector.
              13.2.1.4  After purging the column with solvent for 1 to  2 hours, adjust the column head
                       pressure to 7 to 10 psig and purge for 4 to 5 hours to remove air. Maintain a
                       head pressure of 7 to  10 psig. Connect the column to the detector (Section
                       6.7.1.4).
        13.2.2  Column calibration.
              13.2.2.1   Load 5  mL of the calibration solution  (Section 7.4) into the sample loop.
              13.2.2.2  Inject the calibration solution and  record the signal from the detector. The elution
                       pattern will be corn oil, bis(2-ethyl hexyl)phthalate, pentachlorophenol, perylene,
                       and sulfur.
                                                                                                39

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                                                                               •,
                                                                         corn o,l and >85% collection
         13.2
^3.3   Silica
r
       13.3.1
       13.3.2


       13.3.3

      13.3.4

      13.3.5
   13.2.2.3  Set the "dump time" to allow >85% removal of
           of the  phthalate.        all°W >85% removal of

   13.2.2.4  Set the "collect time" to the peak minimum between perylene and sulfur
   13.2.2.5  Verify the calibration with the calibration solution after every 20 extracts
           Calibration is verified if the recovery of the pentachlorophenol is greater than
           85%. If calibration ,s not verified, the system shall be recalibrated using the
           calibration solution, and the previous 20 samples shall be re-extracted and
           cleaned up using the calibrated GPC system.
.3  Extract cleanup-GPC requires that the column not be overloaded. The column specified
   m this method  is designed to handle a maximum  of 0.5 g of high molecular weiS
   material in a 5-mL extract If the extract is known or expected to I^     0.5
   ^ the extract ,. split into ahquots for GPC, and the aliquots are combined after elution
   from the column. The residue content of the extract may be obtained gravimetrical'y by
   evaporating the solvent from a 50-uL aliquot.                           metncai.y oy
 13.2.3.1  Filter the extract or load  through  the filter holder (Section 6.7. 1 .3) to remove the
          particles. Load the 5.0-mL extract onto the column.
 13.2.3.2  Elute the extract using the calibration data determined in Section 13 2 2 Collect
          the eluate in a clean 400- to 500-mJL beaker.     j
 13.2.3.3  Rinse the sample loading tube thoroughly with methylene chloride between
         extracts  to prepare  for the next sample.
 13.2.3.4 If a Particularly  dirty extract is encountered, a 5.(jLmL methylene chloride blank
         shall be  run through the system to check for carry-over.
 13.2.3.5  Concentrate the eluate per Section 12.6 and Section  12.7 for further cleanup or
         injection into the GC/MS.
gel cleanup.

 Place a glass-wool plug  in a 15-mm ID chromatography column (Section 6.7 4 2)  Pack
  he column bottom to top with:  1 g silica gel (Section 7.5.1.1), 4 g basic silica gel
 (Section 7.5. 13),  1 g silica  gel, 8  g acid silica gel (Section 7.5.1.2), 2 g silica gel, and 4
 g granular anhydrous sodium sulfate (Section 7.2.1). Tap the column to settle the
 adsorbents.

 Pre-elute the column with 50 to 100 mL of hexane. Close the stopcock when the hexane
 is w,thm 1 mm of the sodium sulfate. Discard the eluate. Check the column for
 channeling. If channeling is  present, discard the column and prepare another.
 Apply the concentrated extract to the column. Open the stopcock until the extract is
 within  1 mm of the sodium sulfate.

 Rinse the receiver twice with 1-mL portions of hexane, and apply separately to the
 column. Elute the CDDs/CDFs with 100 mL hexane, and collect the eluate.
40

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       13.3.6  For extracts of samples known to contain large quantities of other organic compounds
              (such as paper mill effluents), it may be advisable to increase the capacity of the silica
              gel column. This may be accomplished by increasing the strengths of the acid and basic
              silica gels. The acid silica gel (Section 7.5.1.2) may be increased in strength to as much
              as 44% w/w (7.9 g sulfuric acid added to 10 g silica gel). The basic silica gel (Section
              7.5.1.3) may be increased in strength to as much as 33% w/w (50 mL  IN NaOH added
              to 100 g silica gel), or the potassium silicate (Section 7.5.1.4) may be used.,

    Note:  The use of stronger acid silica gel (44% w/w) may lead to charring of organic
    compounds in some extracts. The charred material may retain some of the analytes and lead to
    lower recoveries of CDDs/CDFs.  Increasing the strengths of the acid and basic silica gel may
    also require different volumes of hexane than those specified above to elute the analytes off the
    column. Therefore,  the performance of the method after such modifications must be verified by
    the procedure in Section  9.2.

13.4   Alumina cleanup.
       13.4.1  Place a glass-wool plug in a 15-mm ID chromatography column (Section 6.7.4.2).
       13.4.2  If using acid alumina, pack the column by adding 6 g acid alumina (Section 7.5.2.1). If
              using basic alumina, substitute 6 g basic alumina (Section 7.5.2.2). Tap the column to
              settle the adsorbents.
       13.4.3  Pre-elute the column with 50  to 100 mL of hexane: Close the stopcock when the hexane
              is within 1  mm of the alumina.
       13.4.4  Discard the eluate. Check the column for channeling. If channeling is present, discard the
              column and prepare another.
       13.4.5  Apply the concentrated extract to the column. Open the stopcock until the extract is
              within  1 mm of the alumina.
       13.4.6  Rinse the receiver twice with  1-mL portions of hexane and apply separately  to the
              column. Elute  the interfering compounds with  100 mL hexane and discard the eluate.
       13.4.7  The choice of  eluting solvents will depend on the choice of alumina (acid or basic) made
              in Section 13.4.2.
            13.4.7.1  If using acid alumina, elute the CDDs/CDFs from the column with 20 mL
                     methylene chloride:hexane (20:80 v/v). Collect the eluate.
            13.4.7.2  If using basic alumina, elute the CDDs/CDFs from the column with 20 mL
                     methylene chloride:hexane (50:50 v/v). Collect the eluate.
       13.4.8  Concentrate the eluate per Section  12.6 and 12.7 for further cleanup or injection into the
              HPLC or GC/MS.
13.5  Carbon column.
       13.5.1  Cut both ends  from a 10-mL disposable serological pipet (Section 6.7.3.2) to produce a
              10-cm column. Fire-polish both ends and flare  both' ends if desired. Insert a glass-wool
              plug at one end, and pack the column with 0.55 g of Carbopak/Celite (Section 7.5.3.3) to

                                                                                              41

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                ml      t     T« T               ene  0OWe   y   mL * me'Mene chloride:
                m thanol.-toluene (5:4:1 v/v), 1  mL of methylene chloridexyclohexane (1:1 v/v), and 5
                mL of hexane. If the flow rate of eluate exceeds 0.5 mL'minute, discard the column
         13.5.3  When the solvent is within 1  mm of the column packing; apply the sample extract to the
                column. R,nse the sample container twice with  1-mL portions of hexane and apply
                separately to the column. Apply 2 mL of hexane to complete the transfer.
         13.5.4  Elute the interfering compounds with two 3-mL portions of hexane, 2 mL of methylene
                chlonde:cyclohexane (1:1 v/v), and 2 mL of methylene c}iloride:methanol:toluene (15-4-1
                v/v).  Discard the eluate.                               ;                          '  '
                                                                                                 r
         13.5.5  Invert the column, and elute the CDDs/CDFs with 20 mL of toluene. If carbon particles
                are present in the eluate, filter through glass-fiber filter paper.
        13.5.6   Conc^ntra^the eluate per Section 12.6 and  ,2.7 for further cleanup or injection into the

 113.6   HPLC (Reference 6),,
 |       13.6.1  Column calibration.

              13.6.1.1  Prepare a  calibration standard containing the 2,3,7,,8-substituted isomers and/or
                      other isomers of interest at a concentration of approximately 500 pg/uL in
                      methylene chloride.
             13.6.1.2  Inject 30 pL of the calibration solution into the  HPLC and record the signal from
                      the detector. Collect the eluant for reuse.  The elution order will be the tetra-
                      through octa- isomers.
             13.6.1.3   Establish the collection time for the tetra-isomers and for the other isomers of
                      interest. Following calibration, flush the injection system with copious quantities
                     of methylene chloride, including a minimum of five 50-uL injections while the
                     detector is  monitored, to ensure that residual CDDs/CDFs are removed from the
                     system.
             13.6.1.4  Verify the  calibration with the calibration  solution after every 20 extracts
                     Calibration is verified if the recovery of the CDDs/CDFs from the calibration
                     standard (Section  13.6.1.1) is 75 to 125% compared to the calibration (Section
                     13.6.1.2). If calibration is not verified, the system shall be  recalibrated using the
                     calibration  solution, and the previous 20 samples shall be  re-extracted and
                     cleaned up  using the calibrated system.
      13.6.2  Extract cieanup-HPLC requires that the column not be overloaded. The column
             specified in this method is designed to handle  a maximum of 30 uL of extract If the
             extract cannot be concentrated to less than 30 ui,,  it is split into fractions and the
             fractions are combined after elution  from the column.
            13.6.2.1   Rinse the sides of the vial twice with 30 uL of methylene chloride and reduce to
                    30 uL with  the evaporation apparatus (Section 12.7).
42

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                                                                                        Metnoa
             13.6.2.2  Inject the 30 uL extract into the HPLC.
             13.6.2.3  Elute the extract using  the calibration data determined in Section 13.6.1. Collect
                      the fraction(s) in a clean 20-mL concentrator tube containing 5 mL of
                      hexane:acetone  (1:1 v/v).
             13.6.2.4  If an extract containing greater than 100 ng/mL of total CDD or CDF is encoun-
                      tered, a 30-uL methylene chloride blank shall be run through the system to check
                      for carry-over.
             13.6.2.5  Concentrate the eluate per  Section 12.7 for injection into the GC/MS.
13.7  Cleanup of tissue lipids—Lipids are removed from the Soxhlet extract using either the
      anthropogenic isolation column (Section 13.7.1) or acidified silica gel (Section 13.7.2), or are
      removed from the HC1 digested extract using sulfuric acid and base back-extraction (Section
      13.7.3).
      13.7.1  Anthropogenic isolation column (References 22 and  27)—Used for removal of lipids
              from the Soxhlet/SDS extraction (Section  12.4.1).
             13.7.1.1  Prepare the column as given in Section 7.5.4.
             13.7.1.2  Pre-elute the column with 100 mL of hexane. Drain the hexane layer to the top
                     of the column, but do not expose the  sodium sulfate.
             13.7.1.3  Load the sample and rinses (Section 12.4.1.9.2) onto the column by draining each
                     portion to the top of the bed. Elute the CDDs/CDFs from the column into the
                     apparatus used for concentration (Section 12.4.1.7) using 200 mL of hexane.
             13.7.1.4  Concentrate the  cleaned up extract (Sections  12.6-12.7) to constant weight per
                     Section  12.7.3.1. If more than 500 mg of material remains, repeat the cleanup
                     using a fresh anthropogenic isolation column.
             13.7.1.5  Redissolve the extract in a  solvent suitable for the additional cleanups to be used
                     (Section  13.2-13.6 and 13.8).
             13.7.1.6  Spike 1.0 mL of the cleanup standard (Section 7.11) into the residue/solvent.
             13.7.1.7  Clean up the extract using the procedures in Sections  13.2-13.6 and 13.8.
                     Alumina (Section 13.4)  or Florisil (Section 13.8)  and carbon (Section 13.5) are
                     recommended as minimum additional cleanup steps.
            13.7.1.8  Following cleanup, concentrate the extract to 10 uL as described in Section 12.7
                     and proceed with the analysis in Section  14.
      13.7.2 Acidified silica gel (Reference 28)—Procedure alternate to the anthropogenic isolation
             column (Section  13.7.1) that is used for removal of lipids from the Soxhlet/SDS
             extraction (Section 12.4.1).
            13.7.2.1  Adjust the volume of hexane in the bottle (Section 12.4.1.9.2) to approximately
                     200 mL.
            13.7.2.2  Spike 1.0 mL of the cleanup standard (Section 7.11) into the residue/solvent.
            13.7.2.3  Drop the stirring bar into the bottle, place the bottle on the stirring plate, and
                     begin stirring.

                                                                                               43

-------
              13.7.2.4  Add 30-100 g of acid silica gel (Section 7.5.1.2) to the bottle while stirring,
                       keeping the silica gel  in motion. Stir for 2 to 3 hours.
     Note:  30 grams of silica gel should be adequate for most samples' and will minimize
     contamination from this source.
              13.7.2.5  After stirring, pour the extract through approximately 10 g of granular anhydrous
                      sodium sulfate (Section 7.2.1) contained in a funnel with glass-fiber filter into a
                      macro contration device (Section 12.6). Rinse the bottle and sodium sulfate with
                      hexane to complete the transfer.
              13.7.2.6  Concentrate the extract per Sections 12.6-12.7 and clean up the extract using  the'
                      procedures in Sections 13.2-13.6 and 13.8. Alumina (Section  13.4) or Florisil
                      (Section 13.8) and carbon (Section  13.5) are recommended as minimum
                      additional cleanup steps.
        13.7.3  Sulfuric acid and base back-extraction—Used  with HC1 digested extracts (Section
               12.4.2).
             13.7.3.1  Spike 1.0 mL of the cleanup standard (Section 7.1
1) into the residue/solvent
                      (Section  12.4.2.8.2).
             13.7.3.2  Add 10 mL of concentrated sulfuric acid to the bottle. Immediately cap and
                      shake 1 to 3 times.  Loosen cap in a hood to vent excess pressure. Cap and shake
                      the bottle so that the residue/solvent is exposed to the acid for a total time of
                      approximately 45 seconds.
             13.7.3.3  Decant the  hexane into a 250-mL separately funnel making sure that no acid is
                      transferred. Complete the quantitative transfer with several hexane rinses.
             13.7.3.4  Back extract the solvent/residue with 50 mL of potassium hydroxide solution per
                      Section 12.5.2, followed by two reagent water rinses.
             13.7.3.5  Drain the extract through a filter funnel containing approximately 10 g of
                      granular anhydrous sodium sulfate in a glass-fiber filter into a macro
                      concentration  device (Section 12.6).
             13.7.3.6  Concentrate the cleaned up extract to a volume suitable for the additional
                      cleanups given in Sections 13.2-13.6 and 13.8. Gel permeation chromatography
                      (Section 13.2), alumina (Section  13.4) or Florisil (Section 13.8), and
                      Carbopak/Celite (Section  13.5) are recommended  as minimum additional cleanup steps.
             13.7.3.7  Following cleanup, concentrate the extract to 10 uL as described in Section 12.7
                      and proceed with analysis per Section 14.          i
13.8   Florisil cleanup (Reference 29).
      13.8.1  Pre-elute the activated Florisil column (Section 7.5.3) with 10 mL of methylene chloride
              followed by 10 mL of hexane:methylene chloride (98:2 v/v) and discard the solvents.
 44

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                                                                                      Method 1613
         13.8.2  When the solvent is within 1 mm of the packing, apply the sample extract (in hexane) to
                the column. Rinse the sample container twice with 1-mL portions of hexane and apply to
                the column.
         13.8.3  Elute the interfering compounds with 20 mL of hexane:methylene chloride (98:2) and
                discard the eluate.
         13.8.4  Elute the CDDs/CDFs with 35 mL of methylene chloride and collect the eluate.
                Concentrate the eluate per Sections 12.6-12.7 for further cleanup or for injection into the
                HPLC or GC/MS.

14.0    HRGC/HRMS  Analysis

  14.1    Establish the operating conditions given in Section 10.1.
  14.2    Add IO uL of the appropriate internal standard solution (Section 7.12) to the sample extract
         immediately prior to injection to minimize the possibility of loss by evaporation, adsorption, or
         reaction. If an extract is to be reanalyzed and evaporation has occurred,  do not add more
         instrument internal standard solution. Rather, bring the extract back to its previous volume (e.g.,
         19 pL) with pure nonane  only (18 uL if 2 uL injections are used).
  14.3    Inject 1.0 or 2.0 uL of the concentrated extract containing the internal standard solution, using
         on-column or splitless injection. The volume injected must be identical to the volume used for
         calibration (Section  10). Start the GC column initial isothermal hold upon injection. Start  MS
         data collection after the solvent  peak elutes. Stop data collection after the OCDD and OCDF
         have eluted. If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are to be determined, stop data collection
         after elution of these compounds. Return the column to the initial temperature for analysis of the
         next extract or standard.

15.0    System and Laboratory Performance

  15.1   At the beginning of each  12-hour shift during which analyses are performed, GC/MS system
        performance and calibration are  verified for all CDDs/CDFs and labeled compounds. For  these
        tests, analysis of the CS3  calibration verification (VER) standard (Section 7.13 and Table  4) and
        the isomer specificity test standards (Section 7.15 and Table 5) shall be used to verify all
        performance criteria. Adjustment and/or recalibration (Section 10) shall be performed until all
        performance criteria are met. Only after all performance  criteria are met may samples,  blanks,
        IPRs, and OPRs be analyzed.
  15.2   MS resolution—A static resolving power of at least 10,000 (10% valley  definition) must be
        demonstrated at the  appropriate m/z before any analysis is performed. Static  resolving power
        checks must be performed at the beginning and at the end of each 12-hour shift according to
        procedures in Section  10.1.2. Corrective actions must be implemented whenever the resolving
        power does not meet the requirement.
  15.3   Calibration verification.
         15.3.1  Inject the VER standard  using the procedure in Section 14.
                                                                                              45

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 Method 1613
       15.3.2  The m/z abundance ratios for all CDDs/CDFs shall be within the limits in Table 9;
              otherwise, the mass spectrometer shall be adjusted until the m/z abundance ratios fall
              within the limits specified, and the verification test shall be repeated. If the adjustment
              alters the resolution of the mass spectrometer, resolution shall be verified (Section 10.1.2)
              prior to repeat of the verification test.
       15.3.3  The peaks representing each CDD/CDF and labeled compound  in the VER standard  must
              be present with  S/N of at least  10; otherwise, the mass spectrometer shall be adjusted and
              the verification  test repeated.
       15.3.4  Compute the concentration of each CDD/CDF compound by isotope dilution (Section
              10.5)  for those compounds that have labeled analogs (Table 1). Compute the concentra- '
              tion of the labeled  compounds by the internal standard method  (Section 10.6).  These
              concentrations are computed based on the calibration data in Section 10.
       15.3.5  For each  compound, compare the concentration with the calibration verification limit in
              Table 6. If only 2,3,7,8-TCDD  and 2,3,7,8-TCDF are to be determined, compare the
              concentration to the limit in Table 6a. If all compounds meet the acceptance criteria,
              calibration has been verified and analysis of standards and sample extracts may proceed.
i              If, however, any compound fails its respective limit, the measurement system is not
|              performing properly for that compound. In this event, prepare a fresh calibration standard
j              or correct the problem causing  the failure and repeat the resolution (Section 15.2) and
i              verification (Section 15.3) tests, or recalibrate (Section 10).
15.4  Retention times and GC resolution.                             ;
;       15.4.1  Retention times.                                       :
            15.4.1.1 Absolute—The absolute retention times of the 13C,2-1,2,3,4-TCDD and I3C12-
                     1,2,3,7,8,9-HxCDD GCMS internal standards in the  verification test (Section
                     15.3) shall be within ±15 seconds of the retention times obtained during
                    calibration (Sections  10.2.1  and  10.2.4).
            15.4.1.2 Relative—The relative retention times of CDDs/CDFs and labeled compounds in
                    the verification test (Section 15.3) shall be within the limits given in Table 2.
       15.4.2  GC resolution.
            15.4.2.1 Inject the isomer specificity standards (Section 7.15) on their respective columns.
            15.4.2.2 The valley  height between 2,3,7,8-TCDD and the other  tetra-dioxin isomers at
                    m/z 319.8965, and between 2,3,7,8-TCDF and the other tetra-furan isomers at
                    m/z 303.9016 shall not  exceed 25% on their respective columns (Figures 6 and
                    7).
       15.4.3  If the absolute retention time of any compound is not within the limits  specified or if the
              2,3,7,8-isomers  are not resolved, the GC is not performing properly. In this event, adjust
              the GC and repeat  the verification test (Section 15.3) or recalibrate (Section 10), or
              replace the GC column and either verify calibration or recalibrate.
      Ongoing precision and recovery.
 46

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                                                                                      Method 1613
        15.5.1  Analyze the extract of the ongoing precision and recovery (OPR) aliquot (Section
               11.4.2.5, 11.5.4, 11.6.2, 11.7.4, or 11.8.3.2) prior to analysis of samples from the same
               batch.
        15.5.2  Compute the concentration of each CDD/CDF by isotope dilution for those compounds
               that have labeled analogs (Section 10.5). Compute the concentration of 1,2,3,7,8,9-
               HxCDD, OCDF, and each labeled compound by the internal standard method (Section
               10.6).
        15.5.3  For each CDD/CDF and labeled compound, compare the concentration to the OPR limits
               given in Table 6. If only 2,3,7,8-TCDD and 2,3,7,8-TCDF are  to be determined, compare
               the concentration to the limits  in Table 6a. If all compounds meet the acceptance criteria,
               system  performance is acceptable and  analysis of blanks and samples may proceed. If,
               however, any individual concentration falls outside of the range given, the
               extraction/concentration processes are  not being  performed properly for that compound.
               In this event, correct the problem, re-prepare, extract, and clean up  the sample batch and
               repeat the ongoing precision and recovery test (Section 15.5).
        15.5.4  Add results that pass the specifications in Section 15.5.3 to initial and previous ongoing
               data for each compound in each matrix. Update  QC charts to form  a graphic
               representation of continued laboratory  performance. Develop a statement of laboratory
               accuracy for  each CDD/CDF in each matrix type by calculating the average percent
               recovery (R)  and the standard deviation of percent recovery (SR). Express the accuracy as
               a recovery interval from R - 2SR to R + 2SR. For example, if R = 95% and SR = 5%, the
               accuracy is 85 to 105%.
  15.6   Blank—Analyze the  method blank extracted with each sample batch immediately following
        analysis of the  OPR aliquot to demonstrate freedom from contamination and freedom from
        carryover from  the OPR analysis.  The results of the analysis of the blank must meet the
        specifications in Section 9.5.2 before sample analyses may proceed.

16.0   Qualitative Determination
   A CDD, CDF, or labeled compound is identified in  a standard, blank, or sample  when all of the
   criteria in Sections 16.1 through 16.4 are met.
  16.1   The signals for the two  exact m/z's in Table 8 must be present and must maximize within the
        same two seconds.
  16.2   The signal-to-noise ratio (S/N) for the GC peak at each  exact m/z must be  greater than or equal
        to 2.5 for each  CDD or CDF detected  in a sample extract, and greater than or equal to 10  for all
        CDDs/CDFs in the calibration standard (Sections 10.2.3 and 15.3.3).
  16.3   The ratio of the integrated areas of the two exact m/z's  specified in Table 8 must be within the
        limit in Table 9, or within ±10 percent of the  ratio in the midpoint (CS3) calibration or
        calibration verification (VER), whichever is most recent.
  16.4   The relative retention time of the peak for a 2,3,7,8-substituted CDD or CDF must be within the
        limit in Table 2. The retention time of peaks representing non-2,3,7,8-substituted CDDs/CDFs
        must be within  the retention time  windows established in Section 10.3.

                                                                                               47

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   Method 1613
  1615   Confirmatory analysis—Isomer specificity for 2,3,7,8-TCDF cannot be achieved on the DB-5
    I    column. Therefore, any sample in which 2,3,7,8-TCDF is identified by analysis on a DB-5
    1    column must have a confirmatory analysis performed on a DB-225, SP-2330, or equivalent GC
    I    column. The operating conditions in Section  10.1.1  may be adjusted to optimize the analysis on
    i    the second GC column, but the GC/MS must meet the mass resolution and calibration
    :    specifications in Section 10.
  1616   If the criteria for identification in Sections 16.1-16.5 are not met, the CDD or CDF has not been
        identified and the results may not be reported for regulatory compliance purposes. If
        interferences preclude identification, a new aliquot of sample must  be extracted, further cleaned
        up, and analyzed.                                              ;
17.0
Quantitative Determination
  17.1   Isotope dilution quantitation—By adding a known amount of a labeled compound to every
        sample prior to extraction, correction for recovery of the CDD/CDF can be made because the
        CDD/CDF and its labeled analog exhibit similar effects upon extraction, concentration, and gas
        chromatography. Relative response (RR) values are used in conjunction with the initial cali-
        bration data described in Section 10.5 to determine concentrations directly, so  long as labeled
        compound spiking levels are constant, using the following equation:

                                                  (Aln + A2J C,
                                    Ca (rig/ml) =  —1	"-—I-
                                     "            (Al,+A2l)RR
                   where'.
                   Ca = The concentration of the CDD/CDF in the extract, and the
                         other terms are  as defined in Section 10.5.2
                                                                      i
                                                                      •i
        17.1.1  Because of a potential interference, the labeled analog of OCDF is not added to the
               sample. Therefore, OCDF is quantitated against labeled OCDD. As a result, the
               concentration of OCDF is corrected for the recovery of the labeled OCDD. In instances
               where OCDD and OCDF behave differently during sample extraction, concentration, and
               cleanup procedures, this may decrease the accuracy  of the  OCDF results. However,  given
               the low toxicity of this compound relative to the other dioxins and furans, the potential
               decrease in accuracy  is not considered significant.
        17.1.2  Because 13C12-l,2,3,7,8,9-HxCDD is used as an instrument internal standard (i.e., not
               added before extraction of the sample), it cannot be used to quantitate the 1,2,3,7,8,9-
               HxCDD by strict isotope dilution procedures. Therefore, 1,2,3,7,8,9-HxCDD is
               quantitated using the  averaged response of the labeled analogs of the other two 2,3,7,8-
               substituted HxCDD's: 1,2,3,4,7,8-HxCDD and 1,2,3,6,7,8-HxCDD. As  a result, the
               concentration of 1,2,3,7,8,9-HxCDD is corrected for the average recovery of the other
               two HxCDD's.
   48

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                                                                                     Method 1613
       17.1.3  Any peaks representing non-2,3,7,8-substituted CDDs/CDFs are quantitated using an
              average of the response factors from all of the labeled 2,3,7,8-  isomers at the same level
              of chlorination.
17.2   Internal standard quantitation and labeled compound recovery
       17.2.1  Compute the concentrations of 1,2,3,7,8,9-HxCDD, OCDF, the  l3C-Iabeled analogs and
              the  37C-labeled cleanup standard in the extract using the response  factors determined from
              the  initial calibration data (Section 10.6) and the following equation:
                                                 (41, +  A2J Ch
                                 C  (ng/ml) =  —-1	——
                                   " ' *'       (41 u - A2J RF
                      where:
                      C^  = The concentration of the compound in the extract.
                            The other terms are  defined in  Section 10.6.1
    Note:   There is only one m/z. for the 37Cl-labeled standard.

       17.2.2  Using the concentration in the extract determined above, compute the percent recovery of
              the I3C-Iabeled compounds and the 37C-labeled cleanup standard using the following
              equation:

      ,                 o       /a^    Concentration found (wr/mL)   1An
                       Recovery (%) = —	——J     ™  /x  100
                                       Concentration spiked  (/jg/mL)
17.3  The concentration of a CDD/CDF in the solid phase of the sample is computed using the
      concentration of the compound in the extract and the weight of the solids (Section 11.5.1), as
      follows:
                           Concentration in solid (ng/kg) =
                     where:
                     Ca - The concentration of the compound in the extract.
                      Va - The extract volume in mL.
                      Ws - The sample weight (dry weight) in kg.
                                                                                             49

-------
  Method 1613
 17.4   The concentration of a CDD/CDF in the aqueous phase of the sample is computed using the
       concentration of the compound in the extract and the volume of water extracted (Section 11 4 or
       11.5), as follows:

                                                                (C  x  V )
                        Concentration  in aqueous phase (pg/L) = ——	—

                       where:
                       Ca =  The concentration of the compound in  the extract.
                       Va =  The extract volume in mL.                \
  ;                      Vs -  The sample volume in liters.
  i
  i
  i                                                                   ;
  i
 17.5   If the SICP area at either quantitation m/z for  any compound exceeds the calibration range of the
  !     system, a smaller sample aliquot  is extracted.                     i
  i     17.5.1  For aqueous samples containing 1% solids or less, dilute 100 mL, 10 mL, etc., of sample
  I            to 1 L with reagent water and re-prepare, extract, clean up, and analyze per Sections 11-
  !            14.
  !
  i     17.5.2  For samples containing greater than 1% solids, extract an amount of sample equal to
              1/10, 1/100, etc., of the amount used in Section 11.5.1. Re-prepare, extract, clean up, and
              analyze  per Sections 11-14.                              :
  |   .  17.5.3  If a smaller sample size will not be representative of the  entire sample, dilute the sample
  ••            extract by a factor of 10,  adjust the concentration of the instrument internal standard to
  •            100 pg/uL in the extract, and analyze an aliquot of this diluted extract by the internal
              standard method.
  [                                                                   j
17|.6  Results are reported to three significant figures for the CDDs/CDFs and labeled compounds
  i    found in all standards, Blanks, and samples.
  j     17.6.1   Reporting units and levels.
  !
  |        - 17.6.1.1  Aqueous samples—Report results  in pg/L (parts-per-quadrillion).
  |          17.6.1.2 Samples containing greater than 1%  solids (soils,  sediments, filter cake,
  J                  compost)—Report results  in ng/kg based on the dry weight of the sample. Report
  i                  the percent solids  so that the result may be corrected.
  ;          17.6.1.3 Tissues—Report results in ng/kg of wet tissue, not on the basis of the lipid
                    content of the sample. Report the percent lipid content, so that the data user can
                    calculate the concentration on a lipid basis if desired.
            17.6.1.4 Reporting level.
                   17.6.1.4.1   Standards (VER, IPR, OPR) and samples—Report results at or above
                              the minimum level (Table 2). Report results below the minimum level
                              as not detected or as required by the regulatory authority.
                   17.6.1.4.2   Blanks—Report  results above one-third the ML.
 50

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                                                                                       Method 1613
        17.6.2  Results for CDDs/CDFs in samples that have been diluted are reported at the least dilute
               level at which the areas at the quantitation m/z's are within the calibration range (Section
               17.5).
        17.6.3  For CDDs/CDFs  having a labeled analog, results are reported at the least dilute level at
               which  the area at the quantitation m/z is within the calibration range (Section 17.5) and
               the labeled compound recovery is within the normal  range for the method (Section 9.3
               and Tables 6, 6a, 7, and 7a).
        17.6.4  Additionally, if requested, the total concentration of all isomers in an individual level of
               chlorination (i.e.,  total TCDD, total TCDF, total PeCDD, etc.) may be reported by
               summing the concentrations of all isomers identified in that level of chlorination,
               including both 2,3,7,8-substituted and non-2,3,7,8-substituted isomers.

18.0   Analysis of Complex Samples

  18.1   Some samples may contain high levels (>10  ng/L; >1000 ng/kg) of the compounds of interest,
        interfering compounds, and/or polymeric materials. Some extracts will not concentrate to 10 uL
        (Section  12.7); others may overload the GC column and/or mass spectrometer.
  18.2   Analyze a smaller aliquot of the sample (Section  17.5) when the extract will not concentrate to
        10 uL after all cleanup procedures  have been exhausted.
  18.3   Chlorodiphenyl ethers—If chromatographic peaks are detected at the retention time of any
        CDDs/CDFs in any of the m/z channels being monitored for the chlorodiphenyl ethers  (Table 8),
        cleanup procedures must  be employed until these interferences are removed. Alumina (Section
        13.4) and Florisil (Section 13.8) are recommended for removal of chlorodiphenyl ethers.
  18.4   Recovery of labeled compounds—In  most samples, recoveries of the labeled compounds will be
        similar to those from reagent water or from the alternate matrix (Section 7.6).
        18.4.1  If the recovery of any of the  labeled  compounds is outside of the normal range (Table  7),
               a diluted sample shall be analyzed (Section 17.5).
        18.4.2  If the recovery of any of the  labeled  compounds in the diluted sample is outside of
               normal range, the calibration  verification standard (Section 7.13) shall be analyzed and
               calibration  verified (Section 15.3).
        18.4.3  If the calibration  cannot be verified, a new calibration must be performed and the
               original sample extract reanalyzed.
        18.4.4  If the calibration  is verified and die diluted sample does not meet the limits for labeled
               compound  recovery, the method does not apply to the sample being analyzed and the
               result may  not be reported  for regulatory compliance purposes. In this case, alternate
               extraction and cleanup procedures in this method must be employed to resolve  the
               interference. If all cleanup  procedures in this method have been employed and  labeled
               compound  recovery remains outside of the normal range, extraction and/or cleanup
               procedures that are beyond this scope of this method will be required to analyze these
               samples.
                                                                                               51

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   Method 1613
        Pollution Prevention
   I
  1J9.1   The solvents used in this method pose little threat to the environment when managed properly.
        The solvent evaporation techniques used in this method are amenable to solvent recovery, and it
        is recommended that the laboratory recover solvents wherever feasible.
   i
  19.2   Standards should be prepared in volumes consistent with laboratory use to minimize disposal of
   i     standards.                                                   [
   i
   :

20.0   Waste Management

  2&.1   It is the laboratory's responsibility to comply with all federal, state, and local regulations
        governing waste management, particularly the hazardous waste identification rules and land
        disposal restrictions, and to protect the air, water, and land by minimizing and controlling all
        releases from fume hoods  and bench operations. Compliance is also required with any sewage
        discharge permits and regulations.
  2ID.2   Samples containing HC1 to pH <2 are hazardous and must be neutralized  before being poured
   i     down a drain or must be handled as hazardous waste.
  20.3   The CDDs/CDFs decompose above 800°C. Low-level waste such as absorbent paper, tissues,
        animal remains, and plastic gloves may be burned in an appropriate incinerator. Gross quantities
        (milligrams) should be packaged securely and disposed of through commercial or governmental
   :     channels that are capable of handling extremely toxic wastes.
  2d.4   Liquid or soluble waste should be dissolved in methanol or ethanol and irradiated with
      •  ultraviolet light with a wavelength shorter than 290 nm for several days. Use F40 BL or
        equivalent lamps. Analyze liquid wastes, and dispose of the solutions when the CDDs/CDFs can
        no longer be detected.
  20.5   For further information on waste management, consult "The Waste Management Manual for
        Laboratory Personnel"  and "Less is Better-Laboratory Chemical Mianagement for Waste
        Reduction," available from the American Chemical Society's Department  of Government
        Relations and Science Policy, 1155 16th Street N.W., Washington, D.C. 20036.

21.0   Method  Performance
   Method performance was validated and performance specifications were developed using data from
   EPA's  international interlaboratory validation study  (References 30-31) and the  EPA/paper industry
   Long-Term Variability Study of discharges from the pulp and paper industry (58 FR 66078).
22.0
References
    1   Tondeur, Yves, "Method 8290: Analytical Procedures and Quality Assurance for Multimedia
        Analysis of Polychlorinated Dibenzo-p-dioxins and Dibenzofurans by High Resolution Gas
        Chromatography/High Resolution Mass Spectrometry," USEPA EMSL, Las Vegas, Nevada, June
        1987.
   52

-------
                                                                                 Method 1613
 2  "Measurement of 2,3,7,8-Tetrachlorinated Dibenzo-p-dioxin (TCDD) and 2,3,7,8-TetrachIorinated
    Dibenzofuran (TCDF) in Pulp, Sludges, Process Samples and Wastewaters from Pulp and Paper
    Mills," Wright State University,  Dayton, OH 45435, June 1988.
 3  "NCASI Procedures for the Preparation and Isomer Specific Analysis of Pulp and Paper Industry
    Samples for 2,3,7,8-TCDD and 2,3,7,8-TCDF," National Council of the Paper Industry for Air
    and Stream Improvement Inc., 260 Madison Avenue, New York, NY 10016, Technical Bulletin
    No. 551, Pre-Release Copy, July 1988.
 4  "Analytical Procedures and  Quality Assurance Plan for the Determination  of PCDD/PCDF in
    Fish," USEPA, Environmental Research Laboratory, 6201 Congdon Boulevard, Duluth,  MN
    55804, April 1988.
 5  Tondeur, Yves, "Proposed GC/MS Methodology for the Analysis of PCDDs and PCDFs in
    Special Analytical Services  Samples," Triangle Laboratories, Inc., 801-10  Capitola Dr, Research
    Triangle Park, NC 27713, January 1988; updated by personal communication September 1988.
 6  Lamparski, L.L., and Nestrick, T.J., "Determination of Tetra-, Hexa-, Hepta-, and
    Octachlorodibenzo-p-dioxin Isomers in Paniculate Samples at Parts per Trillion Levels,"
    Analytical Chemistry,  52: 2045-2054,  1980.
 7  Lamparski, L.L., and Nestrick, T.J., "Novel Extraction Device for the Determination of
    Chlorinated  Dibenzo-p-dioxins (PCDDs) and Dibenzofurans (PCDFs) in Matrices Containing
    Water," Chemosphere, 19:27-31, 1989.
 8  Patterson, D.G., et. al. "Control  of Interferences in the Analysis of Human Adipose Tissue for
    2,3,7,8-Tetrachlorodibenzo-p-dioxin,"  Environmental lexicological Chemistry, 5: 355-360, 1986.
 9  Stanley, John S., and Sack,  Thomas M., "Protocol for the Analysis of 2,3,7,8-
    Tetrachlorodibenzo-p-dioxin by  High  Resolution Gas Chromatography/High  Resolution  Mass
    Spectrometry," USEPA EMSL, Las Vegas, Nevada 89114, EPA 600/4-86-004, January  1986.
10  "Working with Carcinogens,"  Department of Health, Education, & Welfare, Public Health
    Service, Centers for Disease Control,  NIOSH, Publication 77-206, August 1977, NTIS PB-
    277256.
11  "OSHA Safety and Health Standards,  General Industry," OSHA 2206, 29  CFR 1910.
12  "Safety in Academic Chemistry  Laboratories," ACS Committee on Chemical Safety, 1979.
13  "Standard Methods for the Examination of Water  and Wastewater,"  18th edition and later
    revisions, American Public  Health Association, 1015 15th St, N.W., Washington,  DC 20005, 1-
    35: Section  1090 (Safety), 1992.
14  "Method 613—2,3,7,8-Tetrachlorodibenzo-/7-dioxin," 40 CFR 136 (49 FR 43234), October 26,
     1984, Section 4.1.
15  Provost, L.P., and Elder, R.S., "Interpretation of Percent Recovery Data,"  American Laboratory,
     15: 56-83, 1983.
16  "Standard Practice for Sampling Water," ASTM Annual Book of Standards, ASTM, 1916 Race
    Street, Philadelphia, PA 19103-1187,  1980.

-------
Method 1613
j!7   "Methods 330.4 and 330.5 for Total Residual Chlorine," USEPA, EMSL, Cincinnati, OH 45268,
|     EPA 600/4-79-020, March 1979.                               ;
18   "Handbook of Analytical Quality Control in Water and Wastewater Laboratories," USEPA
;     EMSL, Cincinnati, OH 45268, EPA-600/4-79-019, March 1979.
JI9   Williams, Rick, letter to Bill Telliard, June 4,  1993, available from the EPA Sample Control
>     Center operated by DynCorp  Viar, Inc., 300 N Lee St, Alexandria VA  22314, 703-519-1140.
120   Barkowski, Sarah, Fax to Sue Price, August 6, 1992, available from the EPA Sample Control
     Center operated by DynCorp  Viar, Inc., 300 N Lee St, Alexandria VA  22314, 703-519-1140.
!                                                 .               . '
21   "Analysis of Multi-media, Multi-concentration Samples for Dioxins and Furans, PCDD/PCDF
     Analyses Data Package", Narrative for Episode 4419, MRI Project No. 3091-A, op.cit. February
     12, 1993, Available from the  EPA Sample Control Center operated by DynCorp Viar Inc, 300 N
     Lee St, Alexandria, VA 22314 (703-519-1140).                  I
[                                                                 '
22   "Analytical Procedures and Quality Assurance Plan for the Determination of PCDD/PCDF in
I     Fish", U.S. Environmental Protection Agency, Environmental Research Laboratory, Duluth  MN
i     55804, EPA/600/3-90/022, March 1990.
23   Afghan, B.K., Carron, J., Goulden, P.D., Lawrence, J., Leger, D., Onuska, F., Sherry, J., and
     Wilkenson, R.J., "Recent Advances in Ultratrace Analysis of Dioxins  and Related Halogenated
     Hydrocarbons", Can J. Chem., 65: 1086-1097, 1987.
i
J24   Sherry, J.P., and Tse, H., "A  Procedure for the Determination of Polychlorinated  Dibenzo-p-
!     dioxins in Fish", Chemosphere, 20: 865-872, 1990.               \
!25  • "Preliminary Fish Tissue Study", Results of Episode 4419, available from the  EPA Sample
     Control Center operated by DynCorp Viar, Inc., 300 N Lee St, Alexandria, VA 22314, 703-519-
     1140.                                                       ;
26   Nestrick, Terry L., DOW Chemical Co.,  personal communication with D.R. Rushneck, April 8,
     1993. Details available from the U.S. Environmental Protection Agency Sample Control Center
     operated by DynCorp Viar Inc, 300 N  Lee St, Alexandria, VA  22314, 703-519-1140.
27   Barnstadt, Michael, "Big Fish Column", Triangle Laboratories of RIP, Inc., SOP 129-90, 27
     March 27,  1992.
28   "Determination of Polychlorinated Dibenzo-/?-Dioxins (PCDD)  and Dibenzofurans (PCDF) in
     Environmental Samples Using EPA Method 1613", Chemical Sciences Department, Midwest
     Research Institute, 425 Volker Boulevard, Kansas City, MO 44110-2299, Standard Operating
     Procedure No. CS-153, January 15, 1992.
;29   Ryan, John J., Raymonde Lizotte and William H. Newsome, J. Chwmatog. 303 (1984) 351-360.
J30   Telliard, William A., Harry B. McCarty, and Lynn S. Riddick, "Results of the Interlaboratory
i     Validation  Study of USEPA Method 1613 for the Analysis  of Tetrai- through Octachlorinated
     Dioxins and Furans by Isotope Dilution GC/MS," Chemosphere, 27, 41-46 (1993).
|31   "Results of the International Interlaboratory Validation Study of USEPA Method 1613", October
!     1994, available from the EPA Sample Control Center operated by DynCorp Viar, Inc., 300 N
1     LeeSt, Alexandria, VA  22314,703-519-1140.                  i
54

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                                                                                          Method 1613
23.0   Tables and Figures
   Table 1:    Chlorinated  Dibenzo-p-dioxins and Furans Determined by Isotope Dilution
                and Internal Standard High Resolution Gas Chromatography (HRGC)/High
                Resolution Mass Spectrometry (HRMS)
CDDs/CDFs1 CAS
2,3,7,8-TCDD
Total TCDD
2.3,7.8-TCDF
Tolal-TCDF
1.2,3.7.8-PeCDD
Tolal-PeCDD
1,2,3,7,8-PeCDF
2.3,4,7,8-PeCDF
Total-PeCDF
1.2,3,4,7.8-HxCDD
1,2.3,6,7,8-HxCDD
1,2,3,7,8,9-HxCDD
Tolal-HxCDD
1,2.3,4,7,8-HxCDF
1,2,3,6,7,8-HxCDF
1,2,3,7,8,9-HxCDF
2,3,4,6,7,8-HxCDF
Total-HxCDF
1,2,3,4,6,7,8-HpCDD
Total-HpCDD
1,2,3,4,6,7,8-HpCDF
1,2,3,4,7,8,9-HpCDF
Total-HpCDF
OCDD
OCDF
Registry
1746-01-6
41903-57-5
51207-31-9
55722-27-5
40321-76-4
36088-22-9
57117-41-6
57117-31-4
30402-15-4
39227-28-6
57653-85-7
19408-74-3
34465-46-8
70648-26-9
57117-44-9
72918-21-9
60851-34-5
55684-94-1
35822-46-9
37871-00-4
67562-39-4
55673-89-7
38998-75-3
3268-87-9
39001-02-0
1 . Chlorinated dibenzo-p-dioxins and chlorinated dibenzofurans
TCDD s Tetrachlorodibenzo-p-dioxin
PeCDD s Pentachlorodibenzo-p-dioxin
HxCDD = Hexachlorodibenzo-p-dioxin
HpCDD » Heptachlorodibenzo-pKlioxin
OCDD = Octachlorodibenzo-pKlioxin
TCDF
PeCDF
HxCDF
HpCDF
OCDF
                                                        Labeled analog
                                                        13C12-2,3,7,8-TCDD
                                                        37CI4-2,3,7,8-TCDD

                                                        13C,2-2,3,7,8-TCDF

                                                        '3C12-1,2,3,7,8-PeCDD

                                                        "Cl2-1,2,3,7,8-PeCDF
                                                        13Cl2-2,3,4,7,8-PeCDF

                                                        "0,2-1,2,3,4,7,8-HxCDD
                                                        13C12-1,2,3,6,7,8-HxCDD
                                                        "C,2-1,2,3,7,8,9-HxCDD

                                                        13C12-1,2,3,4,7,8-HxCDF
                                                        "C,2-1,2,3,6.7,8-HxCDF
                                                        13C12-1,2,3,7,8,9-HxCDF
                                                        13C12-2,3,4,6l7,8-HxCDF

                                                        '3C,2-1,2,3,4,6,7,8-HpCDD

                                                        "0^1,2,3,4,6,7,8-HpCDF
                                                        13C12-1l2l3,4l7,8,9-HpCDF
                                                       "C12-OCDD
                                                       not used
                                                             Tetrachlorodibenzofuran
                                                             Pentachlorodibenzofuran
                                                             Hexachlorodibenzofuran
                                                             Heptachlorodibenzofuran
                                                             Octachlorodibenzofuran
CAS Registry
     76523-40-5
     85508-50-5
     89059-46-1

    109719-79-1

    109719-77-9
    116843-02-8

    109719-80-4
    109719-81-5
    109719-82-6

    114423-98-2
    116843-03-9
    116843-04-0
    116843-05-1

    109719-83-7

    109719-84-8
    109719-94-0

    114423-97-1
                                                                                                   55

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Method 1613
Table 2: Retention Time References, Quantitation References,
Times, and Minimum Levels for CDDs and CDFs
Relative Retention



Minimum level1
Retention time Relative
and quantitation retention
CJDD/CDF reference time
Compounds using "0^-1 ,2,3,4-TCDD as the injection internal standard
2,3,7,8-TCDF "C,2-2,3,7,8-TCDF 0.999-1.003
2,3,7,8-TCDD 13C,2-2,3,7,8-TCDD 0.999-1.002
1,2,3,7,8-PeCDF "C,2-1,2,3,7,8-PeCDF 0.999-1.002
2,3,4,7,8-PeCDF 13C12-2,3,4,7,8-PeCDF 0.999-1.002 I
1,2,3,7,8-PeCDD "Cl2-1,2,3,7,8-PeCDD 0.999-1.002
13Cl2-2,3,7,8-TCDF "C12-1 ,2,3,4-TCDD 0.923-1.103 \
"C12-2,3,7,8-TCDD "C,2-1 ,2,3,4-TCDD 0.976-1.043
37CI4-2,3,7,8-TCDD 13C12-1 ,2,3,4-TCDD 0.989-1.052
"{V1,2,3,7,8-PeCDF "0,2-1 ,2,3,4-TCDD 1.000-1.425 '
13012-2,3,4,7,8-PeCDF 13C,2-1,2,3,4-TCDD 1.011-1.526
13fe12-1,2,3,7,8-PeCDD "C,2-1 ,2,3,4-TCDD 1.000-1.567 ;
Compounds using °C1f 1,2,3, 7,8,9-HxCDD as the injection internal standard ;
1,2,3,4,7,8-HxCDF "C,2-1,2,3,4,7,8-HxCDF 0.999-1.001
1,J2,3,6,7,8-HxCDF 13C,2-1 ,2,3,6,7,8-HxCDF 0.997-1.005
1,2,3,7,8,9-HxCDF "C,2-1 ,2,3,7,8,9-HxCDF 0.999-1.001
2,p,4,6,7,8-HxCDF "C12-2,3,4,6,7,8,-HxCDF 0.999-1.001
1,2,3,4,7,8-HxCDD "0,2-1 ,2,3,4,7,8-HxCDD 0.999-1.001
1,2,3,6,7,8-HxCDD "C,j-1 ,2,3,6,7,8,-HxCDD 0.998-1.004
1,|2,3,7,8,9-HxCDD — 2 1.000-1.019
1,2,3,4,6,7,8-HpCDF "C,2-1 ,2.3,4,6,7,8-HpCDF 0.999-1.001
1,b,3,4,7,8,9-HpCDF "C,2-1 ,2,3,4,7,8,9-HpCDF 0.999-1.001
1,b,3,4,6,7,8-HpCDD "C,2-1 ,2,3,4,6,7,8-HpCDD 0.999-1.001
obDF "0,2-OCDD 0.999-1.008 \
OCDD "0,2-OCDD 0.999-1.001 ;
"0,2-1 ,2,3,4,7,8-HxCDF "0,2-1 ,2,3,7,8,9-HxCDD 0.944-0.970
"0,2-1 ,2,3,6,7,8-HxCDF "C,2-1 ,2,3,7,8,9-HxCDD 0.949-0.975
"0,2-1 ,2,3,7,8,9-HxCDF "0,2-1 ,2,3,7,8,9-HxCDD 0.977-1.047 :
"0,2-2,3,4,6,7,8,-HxCDF "C,2-1 ,2,3,7,8,9-HxCDD 0.959-1.021
"0,2-1 ,2,3,4,7,8-HxCDD "C,2-1,2,3,7.8,9-HxCDD 0.977-1.000
"0,2-1 ,2,3,6,7,8-HxCDD "C,2-1 ,2,3,7,8,9-HxCDD 0.981-1.003
13£,2-1,2,3,4,6,7,8-HpCDF "C,2-1 ,2,3,7,8,9-HxCDD 1.043-1.085
"C,2-1,2,3,4,7,8,9-HpCDF "C,2-1 ,2,3.7,8,9-HxCDD 1.057-1.151 j
"0,2-1, 2,3,4,6,7,8-HpCDD "C,,-1 ,2,3,7,8,9-HxCDD 1.086-1.110
"JVOCDD "C,2-1,2,3,7.8,9-HxCDD T.032-1.311
Water
(P9/L;
ppq)

10
10
50
50
50







50
50
50
50
50
50
50
50
50
50
100
100










Solid
(ng/kg;
Ppt)

1
1
5
5
5







5
5
5
5
5
5
5
5
5
5
10
10










Extract
(pg/^L;
ppb)

0.5
0.5
2.5
2.5
2.5







2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
5.0
5.0










I.,   The Minimum Level (ML) for each anaiyte is defined as the level at which the entire analytical system must give a
  |   recognizable signal and acceptable calibration point. It is equivalent to tie concentration of the lowest calibration
  •   standard, assuming that all method-specified sample weights, volumes, and cleanup procedures have been employed.
2.1   The retention time reference for 1,2,3,7,8,9-HxCDD is 13C,2-1,2,3,6,7,8-HxCDD, and 1,2,3,7,8,9-HxCDD is quantified
  :   using the averaged responses for "C,2-1,2,3,4,7,8-HxCDD and "C,2-1,2,3,6,7,8-HxCDD.

5(5                                                                               i

-------
                                                                                     Method 1613
                                         spiking
                                        solution2
                          (ng/mL)      (ng/mL)
    "C,i!-1,2,3,4,6l7,8-HpCDF
    "Cl2-1,2,3,4,7,8,9-HpCDF
    "C12-OCDD
            100
            100
            100
            100
            100
            100
            100
            100
            100
            100
            100
            100
            100
            100
            200
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             2
                                             4
                                     PAR stock  PAR spiking
                                     solution3     solution4
                                      (ng/mL)
                                          40
                                          40
                                         200
                                         200
                                     .    200
                                         200
                                         200
Table 3:    Concentration of Stock and Spiking Solutions Containing CDDs/CDFs and
             Labeled Compounds
                               Labeled      Labeled
                             compound   compound
                                stock
                              solution1
    CDD/CDF
    2,3,7,8-TCDD
    2,3,7,8-TCDF
    1,2,3,7,8-PeCDD
    1,2,3,7,8-PeCDF
    2,3,4,7,8-PeCDF
    1,2,3,4,7,8-HxCDD
    1,2,3,6,7,8-HxCDD
    1,2,3,7,8,9-HxCDD               -            -            200
    1,2,3,4,7,8-HxCDF               -            -            200
    1,2,3,6,7,8-HxCDF               -            -            200
    1,2,3,7,8,9-HxCDF               -            -            200
    2,3,4,6,7,8-HxCDF               -            -            200
    1,2,3,4,6,7,8-HpCDD             -            -            200
    1,2,3,4,6,7,8-HpCDF             -            -            200
    1,2,3,4,7,8,9-HpCDF             -            -            200
    OCDD                         —            —            400
    OCDF                         -            -            400
    "0,2-2,3,7,8-1000
    "0,.,-2,3,7,8-TCDF
    13C12-U3,7,8-PeCDD
    \3C12-1,2,3,7,8-PeCDF
    uC12-2,3,4,7,8-PeCDF
    "0,2-1,2,3,4,7,8-HxCDD
    1JC12-1,2l3l6,7l8-HxCDD
    13C,2-1,2,3l4,7,8-HxCDF
    "C,2-1,2,3,6,7l8-HxCDF
    "C,2-1l2,3,7,8l9-HxCDF
    "C12-213,4,61718-HxCDF
(ng/mL)
   0.8
   0.8
    4
    4
    4
    4
    4
    4
    4
    4
    4
    4
    4
    4
    4
    8
    8
Cleanup Standard
3TCI,-2,317,8-TCOD
Internal Standard^
"0,2-1,2,3,4-1000
"C,j-1,2,3,7,8,9-HxCDD
       Concentration
          (ng/ml)

            0.8

            200
            200
1.Section 7.10—
2.Section 7.10.3—
S.Section 7.9—
4.Section 7.14—
5.Section7.11—
B.Section 7.12—
prepared jn nonane and diluted to prepare spiking solution.
prepared in acetone from stock solution daily.
prepared in nonane and diluted to prepare spiking solution.
prepared in acetone from stock solution daily.
prepared jn nonane and added to extract prior to cleanup.
prepared in nonane and added to the concentrated extract immediately prior to injection into the GC
(Section 14.2).
                                                                                              57

-------
Method 1613
I
Table 4: Concentration of CDDs/CDFs in Calibration and Calibration Verification
i Solutions

'
CbD/CDF
2,3,7,8-TCDD
2,3,7,8-TCDF
1,2,3,7,8-PeCDD
1,2,^,7,8-PeCDF
2,3,4,7,8-PeCDF
1,2,13,4,7,8-HxCDD
1,2,3,6,7,8-HxCDD
1,2,3,7,8,9-HxCDD
1,2,J3,4,7>HxCDF
1,2,3,6,7,8-HxCDF
1,2,3,7,8,9-HxCDF
2,3,!t,6,7,8-HxCDF
1,2,3,4,6,7,8-HpCDD
1,2,|3,4,6,7,8-HpCDF
1,2,j3,4,7,8,9-HpCDF
OCDD
OCDF
"C12-2,3,7,8-TCDD
"0,2-2,3,7,8-TCDF
"C,2-1,2,3,7,8-PeCDD
"0,2-PeCDF
"0,2-2,3,4,7,8-PeCDF
"C,2-1,2,3,4,7,8-HxCDD
"0,2-1 ,2,3,6,7,8-HxCDD
"0,2-1 ,2,3,4,7,8-HxCDF
"0,2-1 ,2,3,6,7,8-HxCDF
"0,12-1,2,3,7,8,9-HxCDF
"C,!2-1,2,3,4,6,7,8-HpCDD
"C,2-1 ,2,3,4,6,7,8-HpCDF
13C,2-1,2,3,4,7,8,9-HpCDF
"CJj-OCDD
Clebnup Standard
37CI4-2,3,7,8-TCDD
Internal Standards
"C^-l ,2,3,4-TCDD
"C,L-1,2,3(7,8,9-HxCDD

CS1
(ng/mL)
0.5
0.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
2.5
5.0
5.0
100
100
100
100
100
100
100
100
100
100
100
100
100
200

0.5

100
100

CS2
(ng/mL)
2
2
10
10
10
10
10
10
10
10
10
10
10
10
10
20
20
100
100
100
100
100
100
100
100
100
100
100
100
100
200

2

100
100
VER1
CS3
(ng/mL)
10
10
50
50
50
50
50
50
50
50
50
50
50
50
50
100
100
100
100
100
100
100
100
100
100
100
100
100
100
100
200

10

100
100

CS4
(ng/mL)
40
40
200
200
200
200
200
: 200
200
200
200
200
200
200
200
400
400
100
100
100
: 100
100
; 100
100
100
100
100
100
!• 100
100
200

; 40
i
100
! 100

CSS
(ng/mL)
200
200
1000
1000
1000
1000
1000
1000
1000
1000
1000
1000
1000
1000
1000
2000
2000
100
100
100
100
100
100
100
100
100
100
100
100
100
200

200

100
100
1.    Section 15.3, calibration verification solution.
581

-------
Table 5:    GC Retention Time Window Defining Solution and Isomer Specificity Test
            Standard (Section 7.15)

DB-5 Column GC Retention-Time Window Defining Solution
 CDD/CDF
 TCDF
 TCDD
 PeCDF
 PeCOD
 HxCDF
 HxCDD
 HpCDF
 HpCDD
First eluted
        1,3,6,8-
        1,3,6,8-
      1,3,4,6,8-
      1,2,4,7.9-
     1,2,3,4,6,8-
     1,2,4,6,7,9-
    1,2,3,4,6,7.8-
    1,2,3,4,6,7,9-
Last eluted
       1,2,8,9-
       1,2,8,9-
      1,2,3,8,9-
      1,2,3,8,9-
    1,2,3,4,8,9-
    1,2,3,4,6,7-
   1,2,3,4,7,8,9-
   1,2,3,4,6,7,8-
                      DB-5 Column TCDD Specificity Test Standard
                                     1,2,3,7+1,2,3,8-TCDD
                                        2.3.7,8-TCDD
                                        1,2,3.9-TCDD
                 DB-225 Column TCDF Isomer Specificity Test Standard
                                        2,3,4.7-TCDF
                                        2,3,7,8-TCDF
                                        1,2,3,9-TCDF

-------
Method 1613
Table 6: Acceptance
Tested1



CDP/CDF
2,3,7,8-TCDD
2,3,7,b-TCDF
1,2,3J7,8-PeCDD
1,2,3,k8-PeCDF
2,3,4,7,8-PeCDF
1,2,3,4,7,8-HxCDD
1,2,3,6,7,8-HxCDD
1,2,3,k8,9-HxCDD
1,2,3,4,7,8-HxCDF
1,2,3,6,7,8-HxCDF
1,2,3,17,8,9-HxCDF
2,3,4,6,7,8-HxCDF
1,2,3,4,6,7,8-HpCDD
1,2,3,4,6,7,8-HpCDF
1,2,3,'4,7,,8,9-HpCDF
OCDD
OCDF
13C12-2,3,7,8-TCDD
13C12-S,3,7,8-TCDF
'3C12-il,2,3,7,8-PeCDD
l3C12-1,2,3,7,8-PeCDF
13C12-2,3,4,718-PeCDF
13C12-1,2,3,4,7,8-HxCDD
13C12-1,2,3,6,7,8-HxCDD
13C,2-1,2,3,4,7,8-HxCDF
13C,2-1,2,3,6,7,8-HxCDF
13C12jl.2,3,7,8,9-HxCDF
13C12-2,3,4,617,8,-HxCDF
13C12-1,2,3,4,6,7,8-HpCDD
13C12-1,2,3,4,6,7,8-HpCDF
13C12-1,2,3,4l7,8,9-HpCDF
13C12bCDD
37CI«^,3,7,8-TCDD
1. All specifications are given
Criteria for Performance Tests When


Test
I V9H •
cone
(ng/mL)
10
10
50
50
50
50
50
50
50
50
50
50
50
50
50
100
100
100
100
100
100
100
100
100
100
100
100
100
100
100
100
200
10


All CDDs/CDFs

are
.,-
IPR2-3

s
(ng/mL)
2.8
2.0
7.5
7.5
8.6
9.4
7.7
11.1
8.7
6.7
6.4
7.4
7.7
6.3
8.1
19
27
37
35
39
34
38
41
38
43
35
40
37
35
41
40
95
3.6
as concentration in the final extract

X
(ng/mL)
8.3-12.9
8.7-13.7
38-66
43-62
36-75
39-76
42-62
37-71
41-59
46-60
42-61
37-74
38-65
45-56
43-63
89-127
74-146
28-134
31-113
27-184
27-156
16-279
29-147
34-122
27-152
30-122
24-157
29-136
34-129
32-110
28-141
41-276
3.9-15.4
!
OPR
(ng/mL)
6.7-15.8
7.5-15.8
. 35-71
40-67
; 34-80
35-82
38-67
! 32-81
36-67
42-65
39-65
35-78
' 35-70
' 41-61
; 39-69
78-144
63-170
20-175
22-152
| 21-227
! 21-1 92
13-328
21-193
25-163
19-202
21-159
I
* 17-205
'• 22-1 76
i 26-1 66
| 21-158
20-186
. 26-397
'3.1-19.1

VER
(ng/mL)
7.8-12.9
8.4-12.0
39-65
41-60 ;>
41-61
39-64
39-64
41-61
45-56
44-57
45-56
44-57
43-58
45-55
43-58
79-126
63-159
82-121
71-140
62-160
76-130
77-130
85-117
85-118
76-131
70-143
74-135
73-137
72-138
78-129
77-129
96-415
7.9-12.7
assuming a 20-^L volume.
2. is = standard deviation of the concentration
3. X = average concentration.
60











-------
                                                                                    Method 1613
Table 6a.  Acceptance Criteria for Performance Tests When Only Tetra Compounds
            are Tested1
CDD/CDF
2,3,7,8-TCDD
2,3,7,8-TCDF
"0,2-2,3,7.8-7000
"C12-2,3,7,8-TCDF
"CI4-2,3,7,8-TCDD
1.   All specifications are given as concentration in the final extract, assuming a 20-nL volume.
2.   s = standard deviation of the concentration
3.   X = average concentration
Test
cone
(ng/mL)
10
10
100
100
10
IF
(ng/rnL)
2.7
2.0
35
34
3.4
'FT-
X
(ng/mL)
8.7-12.4
9.1-13.1
32-115
35-99
4.5-13.4
OPR
(ng/mL)
7.3-14.6
8.0-14.7
25-141
26-126
3.7-15.8
VER
(ng/mL)
8.2-12.3
8
6-11.6
85-117
76-131
8.3-12.1
                                                                                            61

-------
     Table 7:   Labeled Compound Recovery in Samples When All
               Compound

               13Cl2-2,3,7,8-TCDD  ,
               )3C,2-2,3,7,8-TCDF
              13C,2-1,2,3,7,8-PeCDD
              faC«-1,2,3>7,8-PeCDF
              '3C,2-2,3,4,7,8-PeCDF
              13C«-1,2,3l4,7,8-HxCDO
              "0,2-1,2,3,6,7,8,-HxCDD
              13Cl2-1,2,3,4,7,8-HxCDF
              13C12-1,2,3,6l7,8-HxCDF
              '3C,2-1,2,3,7,8l9-HxCDF
              13C12-2,3,4,6,7,8,-HxCDF
             13C,2-1,2,3,4,6l7,8-HpCDD
             '3C,2-1,2,3,4,6,7,8-HpCDF
             13C«-1,2,3,4,7I8l9-HpCOF
             13C,2-OCDD
             37CI4-2,3,7,8-TCDD
                                                             Labeled compound
                                              Test cone         Recovery
                                               (ng/mL)    (ng/mL)1
  1.
Soe
100
100
100
100
100
100
100
100
100
100
100
100
100
100
200
10
25-164
24-169
25-181
24-185
21-178
32-141
28-130
26-152
26-123
29-147
28-136
23-140
28-143
26-138
34-313
3.5-19.7
25-164
24-169
25-181
24-185
21-178
32-141
28-130
26-152
26-123
29-147
28-136
23-140
28-143
26-138
17-157
35-197
Specification given as concentration in the final extract, assuming a 20-nL volume.
           Compound
           13C12-2,3,7,8-TCDD
           13C12-2,3,7,8-TCDF
           37CI4-2,3,7,8-TCDD
                                    Ra°°V"y '" Samp'eS When Onl* Tetra Compounds
                                                 Test cone
                                                          Labeled compound
                                                               recovery
                                                               * 1      ._ .
                                                	_          icwx/very
                                            (ng/mL)    (ng/mL)1      (%)
       I

 1.   Specification given as concentration in the final extract, assuming a 20-ML volume.
       i
       i
100
100
10
31-137
29-140
4.2-16.4
31-137
29-140
! 42-164
62

-------
Method 1613
Table 8: Descriptors, Exact
CDDs and CDFs
Descriptor Exact m/z1
1 292.9825
303.9016
305.8987
315.9419
317.9389
319.8965
321.8936
327.8847
330.9792
331.9368
333.9339
375.8364
2 339.8597
341.8567
351.9000
353.8970
354.9792
355.8546
357.8516
367.8949
369.8919
409.7974
3 373.8208
375.8178
383.8639
385.8610
389.8157
391.8127
392.9760
401.8559
403.8529
430.9729
445.7555
m/z's, m/z Types, and Elemental Compositions of the

m/z type
Lock
M
M+2
M
M+2
M
M+2
M
QC
M
M+2
M+2
M+2
M+4
M+2
M+4
Lock
M+2
M+4
M+2
M+4
M+2
M+2
M+4
M
M+2
M+2
M+4
Lock
M+2
M+4
QC
M+4

Elemental composition
CjF,,
CttH^O
C)2H43SCI337CIO
13C,2H4MCI40
'3C,2H4M(V7CIO
CK.H^Q,
C12H435CI337CI02
C,2H437CI402
C7F13
XH.^CI.O,
13C12 H4 "Clj 37CI 02
C,2H435CI537CIO
CnHt*CAttrQO
C12HIS8CI1SIC!20
"C^Hj^CI/'CIO
XHs'VCIjO
C9F13
C^Hj^CI^CIOj
C12H3MCI337CI202
XHa^CI^CIOj
XH.^'CI.Q,
C^Hj^Clg^CIO
C12H235CI537CIO
C^H^^CIjO
XHj^O
"C^HZ^IJ^CIO
C,2H235CIS37CI02
C12H2MCI437CI202
C,F15
"CvU^C^ClOt
»C12H235CI437CI202
C,F17
CuHj^CI.^O

Substance2
PFK
TCDF
TCDF
TCDF3
TCDF3
TCDD
TCDD
TCDD4
PFK
TCDD3
TCDD3
HxCDPE
PeCDF
PeCDF
PeCDF
PeCDF3
PFK
PeCDD
PeCDD
PeCDD3
PeCDD3
HpCDPE
HxCDF
HxCDF
HxCDF3
HxCDF3
HxCDD
HxCDD
PFK
HxCDD3
HxCDD3
PFK
OCDPE
63

-------
* ' 1. '
Method 1613
Table 8: Descriptors, Exact m/z's, m/z
CDDs and CDFs (continued)
Descriptor Exact m/z1 m/z type
4 407.7818 M+2
409.7789 M+4
417.8253 M
419.8220 M+2
; 423.7766 M+2
425.7737 M+4
430.9729 Lock
435.8169 M+2
437.8140 M+4
479.7165 M+4
5 441.7428 M+2
442.9728 Lock
443.7399 M+4
457.7377 M+2
459.7348 M+4
469.7779 M+2
471.7750 M+4
513.6775 M+4
1. Nuclidic masses used:
H = 1.007825 C = 12.00000
0 = 15.994915 *C\ = 34.968853
2. TCDD = Tetrachlorodibenzo-/xlioxin
PeCDD = Pentachlorodibenzo-p-dioxin
HxCDD = Hexachlorodibenzo-p-dioxin
HpCDD = Heptachlorodibenzo-p-dioxin
OCDD = Octachlorodibenzo-pKlioxin
HxCDPE = Hexachlorodiphenyl ether
OCDPE = Octachlorodiphenyl ether
DCDPE = Decachlorodiphenyl ether
Types, and Elemental Compositions of the
Elemental composition Substance2
C18 H "CIs 37CI 0 HpCDF
C12 H MCI5 "CI, 0 HpCDF
XH^O ! HpCDF3
13C12 H ^Clg 37CI 0 HpCDF3
C,2 H "Gig 37CI 02 HpCDD
CttH^^O, HpCDD
C, F17 PFK
"C,2 H "Clg 37CI 02 : HpCDD3
1'C1,Ha8CI537Clj-Of HpCDD3
C,2 H "Clj 37Clj 0 NCDPE
^"C^CIO OCDF
C10F17 : PFK
Cu^Clg^CljO OCDF
C12MCL37CI02 OCDD
Ct^Clg^O, OCDD
^^"CIO, i OCDD3
13C12 ^Cl, "CIj O2 OCDD3
C12 ^Cl, "Clj 0 , DCDPE
1
13C = 13.003355 I F = 18.9984
37CI = 36.965903
TCDF = Tetrachlorodibenzofuran
PeCDF = Pentachlorodibenzofuran
HxCDF = Hexachlorodibenzofuran
HpCDF = Heptachlorodibenzofuran
OCDF = Octachlcfodibenzofuran
HpCDPE = Heptachlorodiphenyl efrier
NCDPE = Nonachlorodiphenyl ether
PFK = Perfluorcikerosene
3.   ; Labeled compound



4.   j There is only one m/z for 37CI4-2,3,7,8,-TCDD (cleanup standard).
64

-------
                                                                                   Method 1613
Table 9:    Theoretical Ion Abundance Ratios and QC Limits
      Number of
   chlorine atoms
           4a
           5
           6
           6J
           7
           f
           8
1.   QC limits represent ±15% windows around the theoretical ion abundance ratios.
2.   Does not apply to "CI^.S.T.e-TCDD (cleanup standard).
3.   Used for "C12-HxCDF only.
4.   Used for "C,2-HpCDF only.
m/z's
forming ratio
M/(M+2)
(M+2)/(M+4)
(M+2)/(M+4)
M/(M+2)
(M+2)/(M+4)
M/(M+2)
(M+2)/(M+4)
Theoretical
ratio
0.77
1.55
1.24
0.51
1.05
0.44
0.89
XIV 1
Lower
0.65
1.32
1.05
0.43
0.88
0.37
0.76
IIDII
Upper
0.89
1.78
1.43
0.59
1.20
0.51
1.02

-------
Method 1613
Table 10:    Suggested Sample Quantities to be  Extracted for Various Matrices1
Sample matrix2

Single-phase
Aqueous
Solid
   i
   j
   l

Organic




Tissue
Multi-phase
Liquid/Solid
Aqueous/Solid
Organic/solid
   i
Liquid/Liquid
Aqueous/organic


Aqilieous/organic/solid
Example
Drinking water
Groundwater
Treated wastewater
Dry soil
Compost
Ash
Waste solvent
Waste oil
Organic polymer
Fish
Human adipose
Wet soil
Untreated effluent
Digested municipal sludge
Filter cake
Paper pulp
Industrial sludge
Oily waste


In-process effluent
Untreated effluent
Drum waste
Untreated effluent
Drum waste
Percent
 solids
   Phase
   >20
    Solid


   Organic


   Organic
  1-30
    Solid
  1-100
   >1
     Both



   Organic


Organic & solid
 Quantity
extracted
  1000 ml



    10g



    10g



    10 g
    10 g
    10g



    10 g


    10 g
1.  i The quantity of sample to be extracted is adjusted to provide 10 g of solids (dry weight). One liter of aqueous samples
   i containing one percent solids will contain 10 grams of solids. For aqueous samples containing greater than one percent
   ! solids, a lesser volume is used so that 10 grams of solids (dry weight) will be extracted.
2.  : The sample matrix may be amorphous for some samples. In general, when the CDDs/CDFs are in contact with a
   | multiphase system in which one of the phases is water, they will be preferentially dispersed in or adsorbed on the
   ! alternate phase because of their low solubility in water.
3.  | Aqueous samples are filtered after spiking with the labeled compounds. The filtrate and the materials trapped on the filter
   j are extracted separately, and the extracts are combined for cleanup and analysis.
66\

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                                                                                                      Method 1613

Determine % solids
§11.2



Determine particle size
§11.3

   Prep per §11,5
                                             WillSPE
Visible
<
/Par
'size>
\Hrom
tele \ No
1mm?>— -,
§11. Y
Yes
>
Grind per §11. 7




SDS extraction
per §12.3


Concentrate
per §12,6.1 or
§12.6.2'
l


\ be used? /
JYes
SPE extraction per §12.2
i

SDSextracfon
ofSPEdisk
per §12.3

>
Concentrate
per §12.6.1 or
§12.6.2*




N. particles? /
jMfes
Filter per §11. 4.3
1
>

AND
i
SDS extraction
of filter per
§12.3
\

Concentrate
per §12.6.1 or
§12.6.2'
1
Transfer
through
sodium sutfate











Sep. funnel
extraction of
filtrate per §12.1
i

Sep. funnel
extraction per
§12.1

Concentrate per
§12.6.1, §12.6.2
or §12.6.3
1
Mix sep. funnel
extract & SDS
extract together
per §12.3.9.1 .2
\
Back-c
per§


sxtract
12.5

Concentrate per
§12.6.1, §12.62
or §12.6.3



' The K-D concentration procedure in §12.6.3 can be
 used if the water bath is fed by a steam generator.
                     Rgure 1.  Flow Chart for Analysis of Aqueous and Solid Samples
                                                                                                    52-028-1A
                                                                                                              67

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    Method 1613   .
                            Aqueous
         Discard
                                                          Determine %
                                                         solids per §11,2
                                                     Determine particle size
                                                           per§11.3
                                                         Pressure filter
                                                       aliquot per §11.6.2
                                                                                Macro-concentrate per
                                                                                   §12.6.1- §12.6.2*
                                                                                                             Reserve 10g
                                                                                                             or maximum
                                                                                                            amount from 1 -L
                                                                                                               sample,
                                                                                                           whichever is less
       Particle  \  yes
     size < 1mm?
* The' K-D concentration procedure in §12 6 3
 can|be used if the water bath is fed by a steam
 generator.
                                                       Concentrate
                                                     per §12.6-§12.7
                                                      Clean up per
                                                   §13.2-§13.6, §13.8
 Reconcentrate
per §12.6-§12.7
                                                                                Back-extract per §12.5
                                Transfer thru
  Analysis
per§14-§i8
                           Figure 2. Flow Chart for Analysis of Multi-Phase Samples
                                                                                                                    52-028-2A

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                                                                                                                                  *   I-
                                                                                                            Method 1613
                                                     Homogenize
                                                    tissue per §11.8
                                                     Remove 10g
                             Soxhlel Extraction
                                                        OR
                   Mix Na2S04
               Extract per §12.4.1
                   Decant thru
                    Na2S04
              Concentrate to dryness
                per §12.6-§12.7
              Determine % liptds per
                   §12.4.1.9
   Column Cleanup      |
       Batch Cleanup
   Remove Kpids
    per §13.7.1
                      OR
                                    _L
Redissolve and spike
    cleanup std
  Concentrate per
   §12.6-§12.7
 Remove liptds per
      §13.72
Redissolve and spke
    cleanup std
   Transfer thai
                              Concentrate per
                               §12.6-§12.7
                                                                  Ctean-up per §13.2-
                                                                     §13.6, §13.8
                                                                    Concentrate per
                                                                     §12.6-§12.7
                                                                 Analyze per §14-§18
                                                                 HC! Digestion
                                                                      HCI digest per §12.4.2
                                                                        Decant thru Na £0t
                                                                        Macro-concentrate
                                                                            per §12.6
                                                                         Micro-concentrate
                                                                        to dryness per §12.7
                                                                        Determine % lipids
                                                                           per §12.4.2.8
Redissolve and spike
    cleanup std
 Back-extract with
 H2S04 per§13.7.3
  Back-extract per
      §12.5.2
                                                                       Transfer thru Na2S04
                                                                                                      Concentrate per
                                                                                                       §12.6-§12.7
                                                                                                                52-028-3A
                              Figure 3. Flow Chart for Analysis of Tissue Samples

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Method 1613
70
                                                           90-mmGMF 150 Filter
                          Figure 4. Solid-Phase Extraction Apparatus
                                                                                           52-027-1A

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                                                                 Method 1613
                                                                    52-027-2A
Figure 5. Soxhlet/Dean-Stark Extractor
                                                                       71

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      (QIJ
              3B  DBS Column
         100n
         80
         60
         40-
         20-
                         24:00
              25:30



Retention Time (minutes)
27:00
            Figure 6.  Isomer-Specific Separation of 2,3,7,8?TCDD on DB-5 Column
                                                                                             52-027-03
72

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                                                                                 Method 1613
               6-May-88       Sir: Voltage 705       Sys: DB5US
  Sample 11njection 1         Group 1      Mass 305.8987
  Text: Column Performance
100-n
 80-
 60-
 40-
 20-
  0-L-T
                                          2,3,4,8-TCDF
Norm: 3466
                                                         1,2,3,9-TCDF
    16:10 16:20 16:30  16:40 16:50 17:00  17:10  17:20  17:30  17:40  17:40  18:00
                              Retention Time (minutes)
Figure 7.  Isomer-Specific Separation of 2,3,7,8-TCDF on DB-5 Column
                                                                                    52-027-4A
                                                                                        73

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   Method 1613
24.0   Glossary of Definitions and Purposes

   These definitions and purposes are specific to this method but have been conformed to
   common usage as much as possible.
     !

 24.1 |Units of weight and measure and their abbreviations
   24J1.1     Symbols
     i°C     degrees Celsius
            microliter
t
L
.m
   24.h.2
micrometer
less than
greater than
percent

Alphabetical abbreviations
ampere
centimeter                                            ;
gram
hour
inside diameter
inch
liter
Molecular ion                                         ,
meter
milligram
minute
milliliter
millimeter                                            !
mass-to-charge ratio
normal; gram molecular weight of solute divided by hydrogen equivalent of solute,
per liter of solution
outside diameter
picogram
part-per-billion
part-per-million
part-per-quadrillion
part-per-trillion
pounds-per-square inch gauge
volume per unit volume
weight per unit volume
 24.2 Definitions and acronyms (in alphabetical order).
     i
     Analyte—A CDD or CDF tested for by this method. The analytes are listed in Table 1.
     I
     Calibration standard (CAL)—A solution prepared from a secondary standard and/or stock
     solutions and used to calibrate the response of the instrument with respect to analyte
     concentration.                                               ;
     ;m
     3
     i
     D
     n.

     M
     Tl
     Tig
     nin
     mL
     mm
     (n/z
     N

     |DD
     pg
     Ppb
     ppm
     jjpq
     ppt
     psig
     y/v
     j/v/v
   74

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                                                                          Method 1613
Calibration verification standard (VER)—The mid-point calibration standard (CS3) that is
used in to verify calibration. See Table 4.

ODD—Chlorinated dibenzo-p-dioxin. The isomers and congeners of tetra- through octa-
chlorodibenzo-p-dioxin.

CDF—Chlorinated dibenzofuran. The isomers and congeners of tetra- through octa-
chlorodibenzofuran.

CS1, CS2, CSS, CS4, CSS—See Calibration standards and Table 4.

Field blank—-An aliquot of reagent water or other reference matrix that is placed in a
sample container  in the laboratory or the field, and treated as a sample in all respects,
including exposure to sampling site conditions, storage, preservation, and all analytical
procedures. The purpose of the field blank is to determine if the field or sample transporting
procedures and environments have contaminated the sample.

GC—Gas chromatograph or gas chromatography.

GPC—Gel permeation chromatograph or gel permeation chromatography.

HPLC—High performance liquid chromatograph or high performance liquid chromatography.

HRGC—High resolution GC.

HRMS—High resolution MS.
   t
IPR—initial precision and recovery; four aliquots of the diluted  PAR standard analyzed to
establish the ability to generate acceptable precision and accuracy. An IPR is performed
prior to the first time this method is used and any time  the method or instrumentation is
modified.

K-D—Kuderna-Danish concentrator; a device used to concentrate the analytes in a solvent.


Laboratory blank—See Method blank.

Laboratory control sample (LCS)—See Ongoing precision and recovery standard (OPR).

Laboratory reagent blank—See Method blank.

May—This action, activity, or procedural step is neither required nor prohibited.

May not—This action, activity, or procedural step is prohibited.

Method blank—An aliquot of reagent water that is treated exactly as a sample including
exposure to all  glassware, equipment, solvents, reagents, internal standards, and
surrogates that are used with samples. The method blank is used to determine if analytes
or interferences are present in the laboratory environment, the reagents, or the apparatus.
                                                                                 75

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Method 1613
  Minimum level (ML) — The level at which the entire analytical system must give a
  recognizable signal and acceptable calibration point for the analyte. It is equivalent to the
  concentration of the lowest calibration standard, assuming that all method-specified sample
  weights, volumes, and cleanup procedures have been employed.  :
  i
  MS — Mass spectrometer or mass spectrometry.
  i
  i
  Must— This action, activity, or procedural step is required.

  
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                                                                            Method 1613
SPE—Solid-phase extraction; an extraction technique in which an analyte is extracted from
an aqueous sample by passage over or through a material capable of reversibly adsorbing
the analyte. Also termed liquid-solid extraction.

Stock solution—A solution containing an analyte that is prepared using a reference material
traceable to EPA, the National Institute of Science and Technology (NIST), or a source that
will attest to the purity and authenticity of the reference material.

TCDD—Tetrachlorodibenzo-p-dioxin.

TCDF—Tetrachlorodibenzofuran.

VER—See Calibration verification standard.
                                                                                   77

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