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United States          Municipal Environmental Research   EPA-600/9-80-014
Environmental Protection   Laboratory                June 1980
Agency             Cincinnati OH 45268


Research and Development                     	
                    Report
                    of
                    Progress
                     This document has not been
                     submitted to NT.S, therefore ft
                     should be retained.

-------
                                    EPA-600/9-80-014
                                    June 1980
Report
of
Progress
                     U.S. Environmental Protection Agency
                     Region 5, Library (PL-12J)
                     77 West Jackson Boulevard. 12th Ftocr
                     Chicago, IL 60604-3590

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                          FOREWORD

  The chief aim and primary purpose of our laboratory is to develop technol-
ogy, systems, processes and improved management practices to prevent,
control and treat pollutants that affect communities and municipalities. We
develop and demonstrate cost-effective methods in the areas of sewage and
wastewaters, solid and hazardous wastes, and public drinking water supplies.
  We recognize our responsibility to help establish and maintain communica-
tions with our user community. We are also aware that every effort must be
made to reduce the time it takes to move research findings from the laboratory
to the user. This publication is one way for us to share with you our research
results.  It briefly outlines our progress during 1979. Should you have any
comments about this publication, or suggestions for its improvement, please
take the time to write to  me.

                           Francis T. Mayo
                              Director
             Municipal Environmental Research Laboratory

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                         TABLE OF CONTENTS
OFFICE OF THE DIRECTOR 	 1
SOLID AND HAZARDOUS WASTE RESEARCH DIVISION	6
WASTEWATER RESEARCH DIVISION	26
DRINKING WATER RESEARCH DIVISION	57
INTERNATIONAL ACTIVITIES	"71

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                            OFFICE  OF THE  DIRECTOR
MANAGEMENT
  The Municipal Environmental Research Laboratory is composed of the Office of the Director and
three operating divisions. In 1980 it has a budget of almost $26,000,000 and a permanent staff of 160
scientists, engineers and support personnel. The Office of the Director (O.D.) has three major purposes,
the most important of which is to provide direction and leadership to the operating divisions. Program
planning and review, resources management, the timely execution of projects and programs, manage-
ment reporting, and information management are some of the major functions performed within the
O.D.  In 1979, the office developed procedures for implementing a new output planning procedure,
began work on a highly visible and intensive system of peer review, implemented a highly successful
final  report mailing list system, and mechanized their word processing function.

COORDINATION

  The second major purpose of the Office of the Director is to establish effective  communications
between the Laboratory and its user community.  The Director has devoted much of the office's effort to
strengthening ties between the MERL and the EPA Program Offices and Regional Offices. Additionally,
a mid-year reorganization moved the laboratory from the Office of Air, Land and Water Use to the Office
of Environmental Engineering and Technology, and new  channels of communication were quickly
developed to expedite the exchange of information and ideas between  and among the ORD Headquar-
ters Office and our new sister Industrial Laboratories in Cincinnati and RTR Another area of increased
effort is with the research committees that provide an effective planning forum for ORD, the Program
and Regional offices.

                       TABLE 1. MERL BUDGET FOR FY 1979 (In $1000's)

  PE#                 AREA OF WORK             PFTE POSNS.*  IN-HOUSE $     XM $      TOTAL

1BC821   Urban Systems, Toxics & Residuals Mgmt.      52     $2,170.9   $3,989.1   $6,160.0
1BC822  Wastewater Systems Control Technology       45      1,940.1     11,060.0    13,000.1
1CC824  Drinking Water Treatment                    47      1,925.2     5,360.1     7,285.3
1DC818  Solid Wastes Control Technology              16      1,055.8     4,638.4     5,694.2
1NE827  Environmental Impact of Energy Systems       —          —      265.0       265.0
1AD712  Carbon Fiber Research                       —          —      350.0       350.0
XM1627 Reimbursable Agreements                   —     	—      186.3       186.3
             Total MERL                            160     $7,092.0   $25,848.9   $32,940.9
*PFTE stands for Permanent Full-Time Equivalent


ADMINISTRATION

  The third major purpose of the O.D. is to provide our line managers and supervisors with the
resources they need to accomplish their mission. At the MERL, this translates into the nuts and bolts of
moving the paper necessary to recruit personnel, purchase supplies and materials, maintain commit-
ment records of expenditure, provide for adequate space,  provide editorial and publications support
for reports and technical information,  processing research contracts, cooperative  agreements arid
grants, and all of the other chores necessary to keep a laboratory on the move.

                                           1

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                           Where The MERL Dollars Were Spent in FY-79
                                          In-House
                                          $7092.0 K
                                            21.5%
                                   Extramural
                                   $25,848.9 K
                                     78.5%
                                                Total MERL FY-79
                                                  Expenditures
                                                    $32,940 K
              Extramural Costs
                                                      In-House Costs
    lAG'S - 3.5%
Contracts - 21.4%
                                           Personnel
                                             Costs
                                             73.4%
                          All Others - 7.7%

                          Printing - 5.2%

                          Equipment - 6.6%

                          Supplies - 4.4%

                          Travel - 2.7%
     PE#

   36B1C
   35B1C
   61C1C

   73D1C
   07A1D
   1MH1E
                         TABLE 2. MERL BUDGET FOR FY1980 (In SIOOO's)
             AREA OF WORK
PFTE POSNS.ซ  IN-HOUSE $
                                                              XM$
Urban Systems, Toxics & Residuals Mgmt.
Wastewater Systems Control Technology
Drinking Water Treatment & Groundwater
Prot.
Solid Wastes Control Technology
Carbon Fiber Research
Acid-Rain Anticipatory R&D
    Total MERL
                                                    159.1
TOTAL
55.1
41.0
r
47.0
16.0
—
—
$2,438.8
1,690.0
1,981.1
1,025.9
—
—
$ 4,825.3
3,966.2
4,648.8
4,565.0
600.0
100.0
$ 7.264.1
5,656.2
6,629.9
5,590.9
600.0
100.0
            $7,135.8   $18,705.3   $25,841.1
   *PFTE stands for Permanent Full-Time Equivalent

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                    COMPOSITION OF MERL WORKFORCE BY DISCIPLINE
                                Biological
                               and Physical
                              Sciences - 30% I Engineers - 34%
                                                  Clerical
                                               Support - 12%
  Technical
Support - 17%
                                Administrative    N   Other
                                 Support - 4%  Professionals - 3%
           PROFESSIONAL POSITIONS

Chemical Engineer                         8
Environmental Engineer                   45
Mechanical Engineer                       1
Microbiologist                            10
Soil Scientist                               3
Chemist                                  29
Environmental Scientist                     2
Physical Scientist                           5
Economist                                 1
Operations Research Analyst                3
Systems Analyst                           1
                                  Totals 108
                                                           SUPPORT POSITIONS
                Secretary
                Biological Aid/Tech.
                Engineering AioYTech.
                Equipment Mechanic
                Physical Sci. Aid/Tech.
                Administrative Officer
                Administrative Tech.
                Program  Analyst
                Management Analyst
                Editorial Assistant
                Extramural Assistant
      20
       4
       7
       1
      15
       1
       1
       1
       1
       1
       1
Totals 53

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Composition and Size of MERL Workforce by Organization
                   (December 1979)
       DWRD
      SHWRD
          OD|
                 3PROFESSIONAL STAFF
                 ]TECHNICIANS AND AIDS
                 3 ADMINISTRATIVE SUPPORT
     18
  11
                   20
               44
            40
60
80
                   MERL Resource Trends
       $30M-


       $25M


       $20M


       $15M


       $10M


        $5M
FY-77
$20.0
                              -FY-79-
                               $32.9
        FY-78
        $23.9
   FY-80
   $25.8

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                   PERSON YEARS OF EFFORT FOR MERL IN FY 79
Person-Years
  100
Permanent Person-Years
Constitute 74% of the
Total Work Effort, While
Temporary Person-Years are
26% of the Total Effort
                                              Shaded Area = Permanent Person-Years
                                             Unshaded Area =Temporary Person-Years
                                                                                  100
                                                                                   90
                                                                                   80
                                  70
                                                                                   60
                                                                                   50
                                                                                   40
                                                                                   30
                                                                                   20

PERM P.Y.
TEMP. P.Y
TOTAL P.Y.
WRD
862
24.7
110.9
DWRD
424
16.1
58.5
SHWRD
17.2
7.9
25.1
OD
11 0
47
15.7
MERL
156 8
534
210.2

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           SOLID AND HAZARDOUS WASTE RESEARCH DIVISION

  The Solid and Hazardous Waste Research Division (SHWRD) conducts research in three major
functional areas: disposal technology, hazardous wastes, and resource recovery. In the past, solid
waste research was concentrated on problems associated with municipal solid waste. With present
efforts directed primarily toward the environmental effects of hazardous waste disposed onto or into
the land, research has concentrated  on disposal or  treatment technologies that will  minimize or
prevent harmful effects.
  The problems of solid waste disposal are interrelated with those of air and water pollution. Incinera-
tion, grinding, the use of water either for transportation of solids or as a solid  waste sink - these
impinge upon the concurrent attempts to purify the  air and water environments. Additionally, the
elimination of impurities from air or water effluents by such processes as separation, drying or
compaction, results in the generation of solid wastes - solids that, in turn, require disposal. Measures
to reduce pollution or disposal of waste material must, therefore, betaken with full consideration of the
effect on the overall environment - air, water, and land.
  The solid waste problem is concentrated in densely populated urban areas. Refuse storage, collec-
tion, transportation, and processing directly and intimately affect some 80 percent of the population.
The costs of waste handling,  already severe, are rising. The loss of billions of tons of material to
unreclaimed waste each year indirectly affect each consumer.
  Even more threatening in terms of public health and environmental effects are the present disposal
practices for hazardous wastes. Current estimates indicate that 30 to 35 million tons of hazardous
wastes are disposed  of to the ground with no controls, no records as to location, and quantity and
composition. At the  present time,  proven  techniques for large-scale disposal of most, if not all,
hazardous wastes are not available and generators of these wastes have little incentive to expend
resources for adequate managment.
  Municipalities  and other governmental  agencies need new and improved systems for storage,
collection, and transportation of solid waste; improved technology or methodology for waste reduc-
tion; and criteria for site selection, design, and operation of landfills.

WASTE  DISPOSAL
                                                 2. Pollutant Transport
  Increasing  amounts of waste resjduals are      3. Pollutant Control
being directed to the land for disposal by landfill-      4. Co-disposal
ing. The waste disposal program of SHWRD has      5. Pollutant Treatment
been designed to document and evaluate the po-      6. Environmental Assessment
tentially adverse environmental  and public      7. Remedial Action for Inoperative Sites
health effects that could result if precautions are      8. Landfill Alternatives
not taken for handling the environmental degra-      9. Economic Analysis
dation produced in the course of landfilling. The
SHWRD research - encompassing state-of-the-   Waste Characterization/Decomposition
art documents, laboratory analysis, bench  and     Studies in this area involve collecting composi-
pilot studies, and full-scale field verification stud-   tion data on municipal and  hazardous wastes
ies - will result in research reports, criteria, guid-   from individual waste residuals and landfill  dis-
ance documents for user communities, and in a   posal sites. The study objectives are to (1) quan-
criteria data base for  the development of stand-   tify the gas and leachate production from current
ards mandated by the recently enacted "Re-   best-practice sanitary landfilling and (2) modify
source Conservation and Recovery Act of 1976."   the landfill method to reduce  the environmental
The current research activities classified and dis-   impact of gas and leachate production in a posi-
cussed here are:                                tive and predictable manner. These objectives are
    1. Waste Characterization/Decomposition     to  be achieved by construction  and long-term

-------
monitoring of typical and simulated landfill cells
and  investigation, development, and optimiza-
tion of those factors that control gas and leachate
production. Results are expected only after long-
term monitoring, due to the extremely slow reac-
tion rates.

Standard Techniques

  Procedures for analyzing contaminants in
leachate samples are being developed, both spe-
cific to the wastes being studied and for general
use. In studying the potential environmental im-
pact  of contaminants, a standard test is being
planned to assess contaminants  leached from a
waste by water and other solvents, both initially
and over time.
Waste Leachability

  The leachability of municipal refuse has been
the subject of several  studies. One involves the
determination of long-term gas and  leachate
generation  characteristics by leaching 395 Mkg
(thousands of kilograms) of municipal refuse and
comparing the results to those from monitoring
106 Mkg and 2.7 Mkg experimental landfills at the
Boone County Field Site (BCFS)  of USEPA. The
volume of leachate collected from the 395 Mkg
landfill has been 15 percent greater than pre-
dicted using the USEPA water balance method.
Composition of the leachate seems to have
reached a stable rate of contaminant release (Fig-
ure 1 - total dissolved solids or chemical oxygen
demand vs. time). Gas composition, at 50 percent
O)
E

O 50,000
u
  40,000
< 30,000
oc
ฃ 20,000
  10,000
Q
LU
H
X
O
       O O O
         O O
O
O
'CO
8888
00    O    CN    
-------
w
Q
_l
O
co
euoo
50.00
40.00
3000
2000
10.00
0.00

-
- .
- • ••.
'-•• •
•.••'• ••
i i i i i i i
        O PJ'
                  T—  LO   oo
        CUMULATIVE LEACHATE VOLUME,
           LITERS/kg OF DRY REFUSE
                                                   to
                                                   Q
                                                   _l
                                                   O
                                                   C/3
                                                                    TIME DAYSxIO
  Figure  3. Total solids concentration from experimental refuse landfill leached at 813 mm/yr.
ling, on enhanced methane production. In addi-
tion, several landfills will be used to indicate how
methane may be enhanced at old sites where the
refuse is partially decomposed.
  Another ongoing leachability study deals with
inorganic industrial waste in which  there is no
appreciable biological activity. Consequently, the
chief mode of decomposition and pollutant re-
lease issolubilization and other strictly chemical/
physical changes rather than the  biological de-
composition  that takes place as the waste is
leached with water. Accordingly, the testing pro-
gram is designed to evaluate leaching and pollu-
 D)
 E
Q 60,000
"Z.
LU
CD
>
X
o
^40,000
o
LU
I
CJ
 ; 20,000
Q
LU
I—
I
CD
                                 e-k,v-e-V
maX-e~k2Vma,
o—o TEST CELL 2A - BCFS
D—n PREDICTION

      C_
      C>max
      Cmax = 55,4000 m/l
      Vmaป = 200 mm
      k, = 0.00098
      k2 = 00145
                 EQUIVALENT TIME = 4.25 YR-
                400      800      1200    1600
        CUMULATIVE LEACHATE VOLUME, mm
Figure 4. Empirical curve fit by wigh for Boone
          County Field Site Test Cell 2A.
                                             tant release through time under a variety of
                                             leaching conditions encountered in one or more
                                             disposal situations.
                                               Results to date  are consistent with findings
                                             from other projects that leachability of inorganic
                                             wastes is a function not only of the constituent of
                                             interest, but also the surface area per unit weight
                                             of waste  and the stability of the compounds
                                             formed during waste treatment. The variability in
                                             degree of buffering against solvent-induced
                                             changes indicates that the time dependent leach-
                                             ability also be considered.

                                             Waste Decomposition

                                               The several research projects underway are
                                             intended to document the rates and gaseous and
                                             liquid releases of decomposing refuse and to
                                             control  these processes so they may occur in a
                                             predictable and desireable manner. One tech-
                                             nique to accelerate the rate of decompsotion
                                             which has been under development  by the
                                             SHWRD is leachate recycle. Pilot scale evaluation
                                             of a batch operated recycle system was recently
                                             completed and  indicated that  stabilization of
                                             readily  available organic materials in shredded
                                             refuse and transferred to recycled leachate was
                                             essentially completed within six months. Daily
                                             gas production during the period of rapid stabil-
                                             ization was as high as 50.5 ml/kg of dry refuse
                                             which then dropped to 0.79 ml/kg of dry refuse
                                             after stabilization. The total quantity of gas col-
                                             lected was approaching 3.0 I/kg dry refuse, with
                                             approximately 2.76 I/kg dry refuse produced in a
                                             six month period (Figure 5). Additional work is
                                             intended to resolve the long-term environmental
                                             effect if the stabilized waste is allowed to leach in
                                             a traditional manner.
                                               Processing of refuse has also been viewed as a
                                             means of controlling waste decomposition rates.
 8

-------
       C/3
            54.0
             450
      O
       O)
      _^
      \
       E
       O)
      >
      O
      c/)
      Q
      _l
      O
      C/5
             36.0
             270
180
              90
                                  A
                                •o*
                                                  0
                            ฐ
                                 +
          :o
          'ฐ
         •o
  .  MUNICIPAL REFUSE LEACHED a 813 mm/yr
 -+  MUNICIPAL REFUSE LEACHED a 406 mm/yr
 O  MUNICIPAL REFUSE SLUDGE AND SEWAGE
 ฃ    LEACHED a 406 mm/yr.
    MUNICIPAL REFUSE AND 3% BY WEIGHT
 4    of CaCo3 AND LEACHED a 406 mm/yr
    MUNICIPAL REFUSE PLACED a FIELD CAPACITY
 v   AND LEACHED a 406 mm/yr
    MUNICIPAL REFUSE AND INORGANIC PIGMENT
 _   WASTE LEACHED a 406 mm/yr
 T  MUNICIPAL REFUSE LEACHED a 406 mm/yr
      a 21 ฐC (7ฐC WARMER THAN OTHERS)

J	I	
                                     1.0
                                                          30
                                                                  20
                                  CUMULATIVE LEACHATE VOLUME,
                                      LITERS/kg OF DRY REFUSE

            Figure 5. Total solids  removed from different experimental landfills.
The effect of baling on refuse leachability and gas
production was the object of a contractual study
located in Franklin, Ohio. The treatments were
placed in pilot scale (10 Mkg) experimental land-
fills and were subjected to seasonal rainfall ap-
plication of 600 mm/year. Interim results indicate
that baled refuse still is microbiologically active
and yields gas composition typical  of un-
processed refuse: 50 percent CH4 and 50 percent
C02. Thus gas migration, which is driven by diffu-
sional rather than total pressure differentials,
presents as much of a hazard at  balefill  as at a
traditional landfill. Comparison of leachate com-
position and production, however, indicates that
baled refuse may release less of a contaminant to
the environment than unprocessed refuse (Fig-
ure 6) over a four year period. It appears that the
bulk of the refuse is not subjected to the surface
leaching of each bale of refuse in an above the
ground water table  balefill, however, when the
                                 bales are allowed to saturate, then there is very
                                 little difference in leaching characteristics of the
                                 baled and  unprocessed refuse (Figure 7). It is
                                 uncertain how long the internal volume of each
                                 bale will remain  isolated from the  percolating
                                 water of an above the ground water table balefill.

                                Pollutant Transport
                                  Recent pollutant transport studies have
                                focused on organic compounds that present dis-
                                posal/toxicity problems. Work has  been com-
                                pleted on polychlorinated  biphenyls (PCB), is
                                under way on polybrominated biphenyls (PBB),
                                hexachlorobenzene (HCB), and hexachlorocyclo-
                                pentadiene (HCCPD).
                                  A recent publication entitled "Attenuation of
                                Water-Soluble Polychlorinated Biphenyls by
                                Earth Materials" (EPA-600/2-80-027) reported the
                                results of a laboratory study of the aqueous sol-

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solvents by the Ambersorb.
  PBBs and HCB remain immobile in soils when
leached with water or landfill leachate but are
high mobile when leached with organic solvents.
Mobility is directly proportional to the solubility
of the compounds in the leaching solvents and to
the soil organic matter content.
  PBBs and HCB are resistant to microbial degra-
dation. Both compounds  presisted in soils in ex-
periments  lasting 6 months and in solution
culture experiments lasting for 4 weeks with no
measurable degradation.

Pollutant Control

  The pollutant control  studies determine the
ability of in-situ soils, ranging from sands to
clays, and  natural soil processes to limit the
transport of leachate contaminants as the leach-
ate migrates from landfill sites through the soil.
The studies also determine how various syn-
thetic and admixed materials can be utilized as
liners to prevent leachate migration. The overall
objective is to enable minimization of sub-sur-
face pollution, particularly of groundwater.

Liners/Membranes/A dmixtures

  The test  program is evaluating, in a landfill
environment, the chemical  resistance  and du-
rability of liner materials over 12-, 24-, and 52-
month exposure periods to leachates derived
from hazardous wastes, SOX wastes, and munici-
pal solid wastes. The liner materials being inves-
tigated for municipal solid wastes include six
admixed materials.
    2 asphalt concretes (varying in permeability),
    1 soil asphalt,
    2 asphalt membrances (one based on an
      emulsified asphalt and the other on cata-
      lytically-blown asphalt),
    1 soil cement;
and six flexible  membranes:
    butyl rubber,
    ethylene propylene rubber (EPDM),
    chlorinated polyetheylene (CPE),
    chlorosulfonated polyethylene (HYPALON),
    polyethylene (PE), and
    polyvinyl chloride (PVC).
  Results of the first 12 month's exposure to mu-
nicipal solid  wastes produced  only minor
changes on the physical properties of the liner
materials exposed to landfill leachate. Subex-
periments within this  project have started pro-
ducing  results. In an  experiment designed to
investigate accelerated  testing,  samples that
were exposed on both sides in immersion tanks
produced one year exposure results in approx-
imately eight months. Results of the testing indi-
cated minor changes in the physical properties.
Results of the ASTM E-96, Method  BW water
vapor permeability has been reported (X). These
results rank polyvinyl chloride as having the
highest permeability to water vapor and butyl
rubber and elasticized polyolefin the lowest.
There was some indication that permeability in-
creased with test time, probably due to the mem-
branes swelling caused by the water. An osmotic
bag test was developed which shows promise of
assessing membranes under a variety of ex-
posure conditions. The advantage of using this
test is its small size, ease of handling and poten-
tial for producing results on a timely basis.
  The dismantling of the exposure cells con-
taining hazardous wastes and various liner mate-
rial candidates was delayed  so that a longer
exposure data  base could be developed.
However, monitoring of the cells continued in
order to detect any failures that may have oc-
curred. No failures or leakages occurred during
this time period. Sub-experiments of the project
were performed to increase the potential cause
and effect of liner failures. The effect of immer-
sion is shown  in  Table 3, which presents the in-
crease in weight during the exposure period. As
with the  results from the first year's data the
effects vary considerably with liner type and
waste. In addition, significant variation in effects
occurs between liners made of the same  poly-
mer. This is particularly true among, the three
PVC liners.
   Hanging the samples in the wastes allows the
various phases of the waste to contact the speci-
mens. The effects of this exposure on the top and
bottom sections of the samples are shown in
Table 4.

Water Adsorption of Polymeric Liners

   Results of the water adsorption tests run on the
same polymeric  membrane liners at room tem-
perature and at 70ฐC are presented in Table 5. The
immersion time for this- experiment was 308
days. These results show a great difference in
ultimate swelling of these lining materials by
water. Of particular interest is the low water swell
of the elasticized polyolefin membrane of the
PVC membranes at room  temperature.

Membrane Bags Containing Water

   This test of the liner membranes which ran up
to 337 days, showed them to be very impermea-
ble. A slight increase occurred in the conductivity
of the deionized water outside the bags, indicat-
ing that some ions do pass through the mem-

-------
      TABLE 3. SWELLING OF MEMBRANE LINING MATERIALS ON IMMERSION IN WASTES
Liner Vulcan- Acidic Wastes Alkaline Wastes Lead

Immersion time, days
Butyl rubber
Chlorinated polyethylene
Chlorosulfonated polyethylene

Elasticized polyolefin
Ethylene propylene rubber

Neoprene
Polyester Elastonar
Polyvinyl Chloride


No.
—
44
77
6-R
55
36
83
91
90
75
11
59
88
TABLE 4. RETENTION
ized
—
Yes
No
No
No
No
Yes
?
Yes
No
No
No
No
OF
HP
250
2.7
9.4
6.8
5.4
0.3
3.1
16.1
9.6
0.6
10.2
2.3
7.5
HNO3 Slop- Spent Waste
water caustic
193
1.4
9.3
10.3
7.5
2.7
2.6
18.3
10.9
4.2
16.8
-2.8
193
2.0
1.5
3.8
3.8
17.3
2.7
3.1
0.4
35.1
13.5
-6.4
19.8 -13.5
238 236
0.4 20.1
0.6 70.9
3
2
0
1
0
0
0
0
-3
0
.3 83.0
.2 69.6
.5 18.2
.3 23.0
.2 29.3
.8 45.6
.6 7.6
.1 4.4
.0 8.8
.1 2.2
Oily Wastes
Aro- Pond
matic 104
257 248
32
59
51
53
21
15
35
60
.3 96.5
.5 31.6
.1 75.1
.2 58.4
.3 33.5
.8 35.4
.3 80.1
.7 25.3
17.1 7.9
10,
11,
7,
.7 -7.7
.3 -1.5
,2 -10.3
Weed
252
70.8
116.7
202.3
210.5
44.2
73.4
79.4
94.8
16.3
10.0
33.4
18.1
Pest-
icide/
Herb-
icide
242
0.8
9.6
13.1
12.3
0.0
3.7
8.1
3.5
2.4
4.0
0.5
2.9
TENSILE STRENGTH OF MEMBRANE LINER
MATERIALS ON IMMERSION
(Percent of
original
IN "WEED OIL""
value)



Original
Polymer

Butyl rubber
Chlorinated polyethylene
Chlorosulfonated polyethylene

Elasticized polyolefin
Ethylene propylene rubber

Neoprene
Polyester elastomer
Polyvinyl chloride












































Liner
No.
44
77
6-R
55
36
83
91
90
75
11
59
88




























Value,
psi
1520
2235
1730
1715
2595
970
1865
1940
6770
2955
2555
3155




Retention
Top
of specimen












16
(b)
7
(b)
26
(b)
30
18
90
72
50
63
Bottom
of specimen
55
4
43
45
32
39
40
32
81
84
42
68












a Immersion time, 252 days.
(b) Too soft to test
R = Fabric reinforced
branes.  On the  other hand, the bags  have
generally increased in weight, showing that the
water has moved into the bags as a result of
osmotic pressure. Table 6 illustrates this effect for
the bags containing strong acid.
Chemical Stabilization

  Chemical stabilization is achieved by incor-
porating the solid and liquid phases of the waste
in a relatively inert matrix that protects the com-
ponents of the waste from dissolution by rainfall
 72

-------
              TABLE 5. SWELLING OF POLYMERIC MEMBRANE LINERS IN WATER*
                                  (Percent weight increase)
Polymer
Butyl rubber
Chlorinated polvethylene
Chlorosulfonated polyethylene
Elasticized polyolefin
Ethylene propylene rubber

Neoprene

Polyester elastomer
Polyvinyl chloride

Liner
No.
57-R
77
6-R
36
8
26
43
82
75
10
59
Room
Temp.
4.5
10.2
10.9
0
1.6
1.5
37.8
18.5
10.2
0.7
2.4
70ฐC
53.9
140.0
245.6
0.6
10.8
11.2
240.0
191.4
140.0
39.2
24.0
a Immersion time 308 days.
R = Fabric reinforced.
 TABLE 6. SEALED BAGS CONTAINING STRONG ACID WASTE IMMERSED IN DEIONIZED WATER*
Deioriized water
Polymer

Chlorinated polyethylene
Chlorosulfonated polyethylene
Elasticized polyolefin
Polybutylene
Polyvinyl chloride

Liner
No.

86
85
36
98
19
88
—
pH

4.0
7.7
5.9
3.1
2.5
2.4
4.9
Conductivity
/u mho

132
306
25
296
1970
2285
7
Increase in
weight of bag
containing waste
g.
6.1
8.9
0.5
0.6
5.0
11.3
—
"Immersion time, 337 days.
or other water in the soil.
  If this slows the rate of contaminant leaching
sufficiently to render the waste essentially harm-
less, then restrictions on disposal  site  location
can be minimal.  The test program consists of
investigating five industrial wastes, in both the
raw and fixed states. Each waste was treated in
five separate fixation processes and subjected to
physical testing for leachability. Results to date
indicate that leaching of fixed wastes is a function
of physical,  chemical, and biological mecha-
nisms and principally occurs in the following two
ways:
    1. External leaching which occurs primarily
      as surface washing and/or as  diffusion
      into surface flow.
    2. Internal leaching which  is primarily a
      function of the solubility of the material.
  Since most fixed wastes are characterized as
being highly impermeable; then in a field dis-
posal situation the internal leaching contributes
an insignificant mass of contaminants to the en-
vironment. External leaching is the predominant
mechanisms for contaminant mobility stated,
this external leaching is a combination of surface
washing and/or diffusion to surface flow.
  Fixation of sludges will generally result in an
improvement in leachate quality  because of the
inherent physical and chemical properties of the
fixed wastes as compared to the raw sludges. The
                                                                                       13

-------
primary factor contributing to improvement in
leachate quality from fixed wastes is the reduc-
tion in raw waste surface exposed to leaching.
This fact generally results, not only in lower
leachate concentrations, but also in a significant
improvement in the total mass of contaminants
released to the environment.
  Co-disposal of the fixed waste with municipal
refuse is also being investigated. Chemically sta-
bilized industrial sludges have been loaded into
large lysimeters with  municipal solid waste.
These lysimeter systems will simulate landfill
conditions. Differences in leachate quality be-
tween untreated sludges, stabilized sludges, and
MSW without sludges are being determined.

Pollutant Treatment

  The treatability  of landfill leachate  has been
evaluated in the laboratory; a summary of the
pertinent processes and results was prepared by
Chian and DeWalle. A critical problem impeding
the full scale implementation of  leachate treat-
ment is the flow and compositional variation. The
long-term trend  toward decreasing con-
centration (Figure 8) has caused at least one
treatment facility to be  grossly over-designed.
The composition had decreased between field
sampling/pilot-scale testing and  completion of
the treatment facility. One means of dealing with
large flow and composition  variation is to use a
large equalization pond and bleed directly into a
 0!
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4.
<                    0.3               0.6
O            LEACHATE PRODUCTION,
               liters/kg of dry refuse

Figure 8.  Flux of total solids from experimental
          landfills.
 municipal sewerage system. Toward this end,
 and as a follow-up of laboratory studies, the co-
 treatment of leachate and municipal wastewater
 at an activated sludge facility will be performed at
 the MERL Test & Evaluation Facility.

 Co-disposal

  Wastewater treatment plant sludges and  in-
 dustrial wastes are often co-disposed with muni-
 cipal refuse at  landfills, but there is very little
 quantitative information available concerning
 the environmental effects of such practices. The
 addition  of municipal or industrial sludges may
 affect the rate and  amount of contaminants
 leached from refuse by modifying the type and/
 or duration of bacterial activity within the refuse.
 The introduction of industrial wastes may also
 yield new contaminants not usually found in sig-
 nificant concentrations in leachate from refuse.
 The ability of the  landfill and  the surrounding
 environment  to accept increases in types and
 quantities of contaminants is not understood. It
 was also considered plausible that the rate and
 amount  of contaminants leached from refuse
 may be reduced.
  Interim results from a project started in 1975 at
 our Center Hill Facility to evaluate the leaching
 characteristics of several selected wastes co-dis-
 posed with municipal refuse have not provided
 consistent conclusions. The addition of refinery
 sludge has generally reduced the leaching  of
 contaminants; copper and lead release, however,
 has been greater than the municipal refuse con-
 trol. Addition of sewage sludge has not signifi-
 cantly  affected the leaching characteristics  of
 municipal refuse, even at per capita production
 rates. Large differences in the contaminant  re-
 lease rates were not noticable for inorganic pig-
 ment wastes. Heavy metal and salt flux were
noticeably greater when chlorine production
brine sludge was added to refuse. Despite the
initial alkaline nature of the electroplating sludge,
an increase in the  heavy metals, organics, and
chloride was noticed when disposed with muni-
cipal refuse. The addition of battery production
waste showed a similar response. The addition of
organic pigment sludge indicated a general sup-
pression of metal release and an enhancement of
the  leading of other materials such as COD, total
solids, and alkalinity. Those results fail to show
any consistent trend but instead indicate that the
landfill response to co-disposal of specific wastes
is unique.
  Another project designed to assess the poten-
tial effects of co-disposal involves the leaching of
industrial wastes with municipal landfill leachate
14

-------
as well as water. Leachatefrom a municipal solid
waste (MSW) landfill was used to extract the five
industrial wastes and to study movement of their
components in the soil columns. MSW leachate
dissolved much greater amounts of substances
from the wastes and  apparently increased the
mobility of these substances in the soil columns
relative to the dissolution and mobility observed
when deionized water was used as a leaching
solution. The municipal  landfill leachate is a
highly odorous  material containing  many
organic acids and  is  strongly buffered at a pH of
about 5. Consequently, it has proved to be a very
effective solvent. A sequential batch leaching and
soil adsorption  procedure has been developed
that provides information comparable to that
from soil column studies  but in  a much shorter
time.
  Another experimental landfill project involves
a study of the effects of co-disposal of chemically
stabilized sludges in a municipal refuse landfill.
The stability, weatherability, pollutant leach-
ability, and leaching rate of raw and fixed sludges
will be determined. Test results show that fixing
can cause significant changes in the properties of
sludge, that fixed sludges  are similar to soil, soil-
cement, or low strength concrete, and that prop-
erties are process dependent.

Environmental Assessment

  Disposal of municipal solid waste to the land is
a common  practice  and is likely to be the pre-
dominant disposal mode  for  most communities
for many years in the future. This research area is
concerned with the impacts on the environment
due to this landfilling of solid wastes.
  The impacts of different disposal practices are
assessed along with the response of vegetation
to landfill environments. Studies on the effects of
land application of waste on vegetation have also
been conducted. Economic analyses will be per-
formed on both municipal solid waste and flue
gas cleaning sludge disposal.
  During the past dozen years, many attempts to
revegetate completed sanitary landfills have
been undertaken throughout the United  States,
with varying degrees of success. This has been
evaluated in a recent nationwide field survey of
vegetation growth on completed sanitary land-
fills. Based on the  results of this survey, literature
reviews and other field experiences, a study was
undertaken to determine which species, if any,
can  maintain themselves in  a landfill environ-
ment; to investigate the feasibility of preventing
landfill gas from  penetrating the root zone of
selected species by using gas barrier techniques;
and to identify the factors which are most impor-
tant  in maintaining adequate plant growth on
completed sanitary landfills. Ten replicates of
nineteen woody species were planted on a ten-
year old completed sanitary landfill and five gas
barrier systems were constructed. The experi-
ment was replicated on nearby old forest land to
act as a control. Of the nineteen species planted
on the landfill for the past two years, certain spe-
cies  have tolerated the  landfill conditions better
than others. Where the gas barrier technique kept
landfill gases from the root zone the trees grew
best.
  A  research program to  determine effects of
milled refuse particle  size on landfilled solid
waste has also been initiated. Four experimental
test plots were constructed using four different
particle size distributions. Each pit representing a
specific milled refuse particle size will be evalu-
ated in an  attempt to correlate particle size with
different parameters. The parameters  under
study are: wind displacement of milled refuse,
differential  settlement of compacted milled re-
fuse, and attraction of vectors, rodents, birds and
wildlife to the milled refuse. Monitoring  of the
test  pits has  just  been initiated so preliminary
results are not available to  date.

Remedial Action for Waste Disposal Sites

  A recent  House Commerce Investigative Sub-
committee report on the waste disposal practices
of 53 of the nation's largest chemical manufac-
turers identified 3,383 sites that were used for
disposal operations since 1950. Of the 3,383 sites
identified 1,099 are no longer in use. The report
states that among these closed sites a substantial
portion, have probably been abandoned with no
company or person identifiable as responsible
for cleaning up the areas. These abandoned sites
contain an estimated 100 million tons of chemical
wastes. The members of the House Subcommit-
tee cautioned that the study only addressed the
53 largest chemical manufacturers, while smaller
companies with less resources  for proper dis-
posal are still unidentified.
  The EPA has estimated that 379 million tons of
waste were generated in 1977 by all industry not
just  chemical manufacturers. There are an esti-
mated 50,000 hazardous waste sites in the U.S.,
over 34,000 of which may pose potential environ-
mental  problems and 2000 of which may pose
very serious environmental problems.
  In 1976 SHWRD was requested by the Office of
Solid Waste to initiate a definitive research and
development program in  the area of remedial
action. Subsequent to this request the Resource
Conservation and Recovery Act (RCRA), Public
Law 94-580, Section 4005,  Part C designated the
                                                                                       75

-------
SHWRD  to assist in solving the Army Creek
(Llangollen) hazardous waste landfill problem.
  As a result of these mandates SHWRD awarded
its first contract in remedial action research dur-
ing October of 1976. This initial award resulted in
a full-scale remedial action research project as a
municipal landfill in Windham, Connecticut. This
municipal landfill remedial action will soon be
monitored to determine its effectiveness in re-
ducing the discharge of contaminants into a
drinking water reservoir. An interim report of the
potential remedial actions that were studied  in
preparation for this field verification is available
as an EPA publication (EPA-600/2-78-142) entitled
"Guidance Manual for Minimizing Pollution from
Waste Disposal Sites." Work is expected to be
completed by the Spring of 1980.
  During the  period of 1976 to the  present,
SHWRD has been called upon to providefunding,
task force support and technical advice on re-
medial action sites located throughout the United
States from Iowa to Rhode Island. Some of these
sites include:
    Love Canal, New York
    Saltvill, Virginia (Chloroalkali plant site)   '
    Army Creek Landfill, Deleware
    Kin Buck Landfill, New Jersey
    La Bounty Landfill, Iowa
    Earthline Corporation Landfill, Illinois
    Clermont Environmental, Ohio
    Stringfellow Landfill, California
    Rollins Environmental, Texas
    Mesita del Buey Landfill, New Mexico
    Li Pari Landfill, New  Jersey
    Valley of the Drums,  Kentucky
    Candy Box Farm, Rhode Island
  At the present time SHWRD is in the process of
issuing two new contracts in remedial action
technology. One will be for remedial action at a
hazardous waste disposal site and the other for
remedial action at a surface impoundment. The
purpose of the remedial  action programs being
conducted by SHWRD is to provide a  data base
for other federal agencies, state agencies, local
communities  and private industries in solving
their needs for the selection of viable, econom-
ical and environmentally protective remedial ac-
tions at any type of polluting waste disposal site.

Landfill Alternatives

  The promulgation of air  and  water  pollution
control regulations has resulted in more effective
removal  of contaminants from  waste streams,
especially the  hazardous constituents in many
industrial effluent streams. These cleanup ac-
tivities have resulted in an increased quantity  of
concentrated hazardous wastes that must be dis-
posed of. Growing concern over possible degra-
dation of the environment from current disposal
methods has led  government to seek more ac-
ceptable ways for industry to dispose of its haz-
ardous wastes.
  Many disposal techniques have been utilized
or proposed,  none of which is problem free.
Problem areas encountered have included  ad-
verse enviromental impacts, excessively high
costs and a scarcity of acceptable sites. Current
research activities on landfill alternatives con-
cern such methods as deep-well injection, land
cultivation, and disposal in saline/marshland en-
vironments. Some of these methods are cur-
rently being practiced in the United States.

Deep-Well Injection

  Available information has been compiled on
the injection of industrial hazardous wastes into
deep wells. The planning and operation of a deep
well system is a multi-disciplinary effort involv-
ing geological, engineering, chemical, biological
and legal expertise.
  Deep-well injection systems for nearly all types
of non-hazardous and hazardous industrial
waste are a safe method of handling if the sys-
tems are properly located, designed, operated,
maintained and regulated.

Land Cultivation

  The disposal technique  of land cultivation,
whereby specific  waste residues have been di-
rectly applied or admixed into soils, has been an
alternate disposal option for many years by phar-
maceutical, tannery, food processing, paper  and
pulp, and oil  refinery  industries. To assess  this
concept,  various research efforts have been
initiated.
  Land cultivation practices were observed at six
sites disposing of industrial residuals. The sites
were selected to  permit identification and  ver-
ification of parameters that contribute to the en-
vironmental acceptability of land cultivation for a
variety of industrial wastes under markedly dif-
ferent hydrogeological, meteorological, and land
use conditions. Landfarming at each site investi-
gated was characterized as a physical/chemical/
biological waste treatment process. Accordingly,
information was obtained on the physical  and
chemical  composition  of the waste  fed to  the
surficial soil treatment system; characteristics of
the treatment system;  operational procedures;
effectiveness  of treatment; potential environ-
mental  impacts; and costs. To assess the effec-
tiveness of treatment, samples of waste, soil  and
waste-soil mixtures were collected and analyzed
for organic compound classes; pH; S04 and Cl;

-------
electrical conductivity;  cation exchange capac-
ity; total Kjeldahl nitrogen; As, B, Ca, Cd, Cr, Cu,
K, Mg, Mo, Na, Ni, P, Se, V, and Zn. To access the
extent of uptake of inorganic waste constituents,
vegetation was collected at most sites, and ele-
mental analysis was carried out. Waste inputs to
a landfarming system can be characterized quite
precisely;  output stream can  be  determined in
principle by comparing the composition of waste
application areas with the composition of suita-
bly chosen control areas. Treatment processes
occurring in the soil system for particular wastes
in particular locations can, at the present time,
only be inferred from observed  compositional
changes. This points up the need  for long-range
research on fundamental mechanisms of waste
treatment  in soil systems; and short-range re-
search on  monitoring protocol for landfarming
operations.
  Preliminary studies of the effects of amending
soils with API oil-water  separator sludge on the
germination and yield of ryegrass were initiated
to generate data on acceptable sludge  loading
rates and to elicit mechanisms which affect plant
responses.
  A petrochemical and  refinery waste were uti-
lized and each waste was mixed with each of four
soils in varying ratios by volume. The mixtures
were planted with ryegrass, and emergence and
dry matter yields were  determined. Eight plant
harvest cycles were completed over a 17 month
test period. Soil wettability was also determined
periodically.
  Concentrations of petroleum hydrocarbons as
low as 2 percent by volume depressed ryegrass
emergence and yields, apparently through at
least two mechanisms. Phytotoxic waste constit-
uents initially acted to severly diminish plant re-
sponse. Long term  yield reductions  largely
resulted from impaired water, air, and nutrient
relations associated with recalcitrant hydro-
phobic hydrocarbons.
  The petrochemical sludge suppressed the
emergence and yield over a longer period of
time. The suppression was proportional to the
amount of each waste applied.

Economic Analysis

  The use of scrap futures markets as a means for
encouraging resource recovery from solid waste
was investigated. As a  result of  a preliminary
feasibility study, the Solid and Hazardous Waste
Research Division sponsored a symposium in
May 1979 in New Orleans, Louisiana for persons
interested in implementation of futures markets
for ferrous scrap and wastepaper. A follow-up
symposium, limited to  discussions on futures
markets for wastepaper, was held in November
1979 in Washington, D.C. These symposiums
provided forums for informal discussions among
persons in industry, government, and research
on the potential advantages and  disadvantages
of scrap futures markets in private industry. As a
result of these meetings, a major stock exchange
has developed  plans to submit  model trading
contracts  to the Commodity Futures Trading
Commission for approval.
  A number of case studies were undertaken to
identify and quantify the economical, technologi-
cal, and other impediments which affect the suc-
cessful operation of resource recovery facilities
receiving municipal solid waste. Preliminary re-
sults at the end of the year indicated that none of
the eight  selected facilities  had  been able to
achieve a  breakeven  financial record in  recent
years. The financial analyses were based pri-
marily on actual operating data in contrast to past
studies which relied mainly on engineering esti-
mates, and other preliminary  or hypothetical
data. The  study indicated that a  significant  im-
pediment to successful operation  of the facilities
(i.e. revenues equal to or in excess of costs) was
the competitive advantage held by landfilling of
municipal  solid waste.

RESOURCE RECOVERY
  SHWRD is charged with the responsibility for
(1) resource recovery research and development
(including materials and energy recovery), (2)
waste reduction,  and (3)  hazardous materials
treatment and processing. The multifaceted re-
source recovery programs involve research to
determine and develop the best  techniques for
the recovery and reuse of the material and energy
values contained in municipal solid waste. Cur-
rently, the program involves research in seven
basic areas:
    1. Refuse derived fuels
    2.  Evaluation of resource recovery facilities
    3. Technology assessment
    4.  Process equipment evaluations
    5. Economic and institutional studies
    6.  Environmental impacts
    7. Special studies under the  Resource Con-
      servation and Recovery Act (PL 92-580).

Refuse Derived Fuel

  This research involves  extracting the  com-
bustible organic fraction of municipal solid
waste, processing it into an easily handled form,
and investigating its combustion  characteristics
in industrial, institutional, and utility boilers. Re-
search priorities include co-firing of refuse de-
rived fuels (RDF) and coal; investigating chemical
                                                                                      17

-------
and thermal processes for improving RDF fuel
quality; onsite combustion tests to determine en-
vironmental emissions, plant modifications, and
equipment requirements, development of stand-
ard sampling  and testing procedures, and speci-
fications for standardized RDF and d-RDF (densi-
fied). With increasing experience the knowledge
the marketability and acceptability of RDF should
improve, making it a promising resource recov-
ery alternative.
  SHWRD is cooperating with others to help in-
crease the acceptability of the concept. Joint pro-
jects  were implemented with the Industrial
Environmental Research Laboratory (IERL) in
Cincinnati  to evaluate special aspects of the
Madison and  Milwaukee, Wisconsin resource re-
covery systems dealing with the use of RDF Addi-
tionally, IERL  and SHWRD are cooperating with
the State of Maryland in a project to use RDF as a
fuel in cement kilns. The State of Maryland was
involved in the first combustion test of densified
refuse derived fuels in the Maryland Correctional
Institute's stoker boiler located near Hagertown,
Maryland.  Industry is also  participating in the
second phase tests of d-RDF in  an  industrial
boiler located in Erie, Pennsylvania. SHWRD
provided 60 tons of d-RDF to be tested at a state
boiler in New York. Approximately 2000 tons of d-
RDF were burned in the GE Boiler at Erie,  Penn-
sylvania. Test data are still  being  analyzed, but
tests  were successful. Much valuable informa-
tion was obtained on the combustion  and  boiler
operating characteristics, emissions characteris-
tics, and the  storage, handling, and transporta-
tion of d-RDF

Resource Recovery Facilities
   Several  research  projects  are  directly con-
cerned with the design, implementation, testing,
and evaluation of planned or existing resource
recovery facilities.
   The City of Ames, Iowa, received a grant from
SHWRD  to evaluate the city resource recovery
system. Research includes statistically designed
experiments  to  investigate air emissions from
RDF combustion boiler corrosion, burnouts, and
boiler and plant operations.
   The project is providing the first long-term data
available on the effects of RDF on the corrosion of
boiler tubes. Tubes placed in situ  have been re-
moved after 1,000 hours and one year  of ex-
posure to the combined combustion of RDF and
coal.  Analyses have indicated virtually no corro-
sion for  the 1,000 hour samples for the year-ex-
posed samples. Based upon the detailed analysis
of these samples, the investigators  concluded
that burning RDF with coal does not alter the
basic mechanism of corrosion found to exist on
superheater and waterwall  tubes when coal is
burned alone. There is no evidence to suggest
that the presence of RDF causes an  acceleration
of the rate of attack. This work will provide signifi-
cant information to the industry and should help
to reduce concerns that RDF will corrode boiler
tubes.
  SHWRD has conducted several projects to de-
velop facility design and operating data, includ-
ing alternative disposal systems and methods for
predicting waste composition and quantity. A
study of  the Palos Verdes, California landfill in-
volved optimizing methane production from the
landfill and testing biodegradation processes
and rates.
  An additional study further defined the state-
of-the-art of methane recovery from  landfills and
assessed the technical and economic feasibility
of the concept. The concept is technically feasi-
ble, but economically dependent on  local market
conditions. Off-site sales of raw (low BTU) gas to
industrial customers  in profitable under current
market conditions if a minimum production vol-
ume can be guaranteed. Sales  of cleaned gas
(medium to high BTU) to utilities is economical
only in specific cases. With the  deregulation of
natural gas, however, this concept will likely be
attractive in most cases.
  A current study involves the evaluation of dif-
ferent molecular sieves for gas cleanup. The ob-
ject  is  to improve the BTU yield by increased
C02  removal.
   (g)
Technology Assessments

  In  addition to the data being  generated from
evaluation of available resource recovery facili-
ties, studies are being conducted to assess the
feasibility of alternative technologies for re-
source recovery.
  The biological conversion of cellulosic wastes
to methane studies have been completed at three
commercially constructed, intermediate-sized di-
gesters. Materials handling presented the great-
est obstacle to satisfactory operation of farm-
scale anaerobic digesters. Conversion of biogas
to electricity via standard engine-generator sets
is capital and maintenance intensive. Combining
wastes from several  forms and/or communities
could provide economics of sale provided man-
agement and social barriers are overcome.
   Research was continued on  optimization of
acid hydrolysis technology for  industrial-scale
conversion  of waste cellulose to glucose. This
one ton/day plant utilizes hydropulped refuse
and sawdust  as feedstock. The Werner &
Pfleiderer is used as the reactor devise for contin-
 18

-------
                                     Seven Access Ports
                                     1  acid injection
                                     1  steam injection
                                     4  temperature measurement
                                     1  pressure measurent
                              1       2345      6
                                                              Flushing^
                                                                Drain

              Figure 9. Schematic of the twin screw and hydrolysis system.
uously reacting cellulose in dry or aqueous slurry
at suitability evaluated temperatures. Figure 9 is
a schematic of the Werner & Pfleiderer twin-
screw extruder (reactor), selected because of its
capacity for conveying and  mixing the
feedstocks. This equipment allows accurate con-
trol of temperatures, pressure and resident time
and temperature during intensive mixing. Cur-
rently, plans are being developed for a cellulose-'
glucose pilot  plant capable of producing 10-50
tons/day of glucose.
  Three techniques have been developed and
evaluated  on  the pilot scale for utilization and
stabilization of pyrolytic oils produced from mu-
nicipal solid waste.  Physical and chemical pro-
cessing steps are being investigated to maximize
the value of the oils produced and to maintain
their consistency during storage. Evaluations of
three processes are continuing for the 50 pounds/
day continuous process selection.
 • Related studies have identified and verified
chemical treatments for cellulose embrittlement.
As a result, the basic requirements were defined
for  producing a fine powdered  RDF from the
organic fraction of municipal solid waste. This
work is continuing to further evaluate the com-
bustion characteristics of powder fuel obtained
from processed MSW. Additionally, work will
evaluate techniques for preparing stabilized mix-
tures of the powder RDF and oil, and to determine
the mixtures' combustion characteristics.

Process Equipment Evaluations
  Several projects are being conducted to evalu-
ate the operating performance of selected types
of resource recovery process equipment. Nine
shredders at several large-scale solid waste pro-
cessing facilities were evaluated to determine
their performance characteristics as well as  to
verify basic theoretical relationships developed
in laboratory  research on the size reduction  of
solid waste.
                                                                                       19

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  Seven horizontal hammermills, one vertical
hammermill, and one vertical ring shredderwere
evaluated. Also, two stage-size reduction and sin-
gle-stage size reduction were studied. The work
has resulted in the development of analytical re-
lationships among the size reduction parameters
and established levels of shredder performance
with respect to energy  consumption and  ham-
mer wear.
  Another study is evaluating the operating per-
formance of large-scale air classifiers (AC). Pri-
mary emphasis is placed upon parameters that
can be determined from the testing of air classi-
fiers operating the field. Parameters such as the
air/solids ratios, light fraction quality, fuel quality
index,  and  operation efficiency will be deter-
mined. Seven air classifiers  with  operation
ranges of 5  to 50 tons per hour will be tested.
  Other evaluations at Recovery I in New Orleans
are continuing on the use of froth flotation for gas
recovery and  the use  of  the  trommel rotary
screen to separate MSW prior  to shredding. In
conjunction with this, SHWRD is providing tech-
nical assistance  to the  Department of Energy's
large research and development study on the use
of trommel  screens for resource recovery.
  A more basic research project in investigating
the densif ication of solid waste to produce d-RDF.
Attempts are being made to develop the  basis
data required to design proper equipment and
processes for the production of d-RDF Prelimin-
ary results  have shown a relationship between
pellet quality  and temperature, moisture, die
taper, and the level  of  compaction of the light
MSW prior to entering the pelletizer chamber.
The effect of temperature is unclear and the effect
of moisture content is  counter to  observations
made during the actual  production of d-RDF for
the field combustion tests.
  Explosions in resource recovery facilities have
been a problem. While many have gone  unre-
ported, there is documentation  for well over a
hundred in  only a few years. Some have caused
very extensive facility damage and some have
caused personnel injury. In an effort to minimize
this  problem, SHWRD initiated  a  project to
provide the data necessary to design explosion
venting systems for solid waste shredders, the
one piece of equipment causing the most explo-
sions. The project will adopt information avail-
able for explosion venting of  other industrial
equipmentthrough conduct of actual explosions
in a mock-up full-scale shredder.

Economic and Institutional Studies

  An economic analysis has shown the feasibility
of employing scrap futures markets  for ferrous
and waste paper. Establishment of the concept
could aid the trading of these secondary mate-
rials and  encourage the flow of capital to the
scrap industry. The results of this study were
presented at a symposium on scrap futures in
New Orleans. As a result of this symposium,
COMEX  decided to recommend the establish-
ment of a futures market for ferrous scrap. An-
other symposium is being conducted to provide
the latest information on futures markets to the
paper industry.
  A study of user charges for solid waste man-
agement was inconclusive regarding the  rela-
tionships of user charges' effects on the quantity,
composition, and rate  of resource recovery of
solid waste. Additional work is required to estab-
lish these relationships.  Results did  show,
however, that there was a significant relationship
between the user charges  and the frequency of
solid waste pick up service demanded.

Environmental Impact

  Several continuing projects involve investiga-
tions of the emissions and needed controls to
make  resource recovery systems environmen-
tally acceptable. One study involves emissions
from preprocessing and bioconversion systems.
Investigators  are characterizing  pollutants,  de-
veloping assessment criteria and pollution mea-
surement techniques, and performing a trade-off
analysis of cost and performance  of pollution
control equipment. Another study involves selec-
tion and on-site testing of  various air pollution
control devices, with a determination of unit ac-
ceptability and needed improvements. This work
is being  conducted in cooperation with IERL-
Cincinnati.
  Potential methods available for removing  lead
and other metals from solid waste are being in-
vestigated. The presence of lead in solid waste
has resulted in potentially unacceptable levels of
lead in the emissions from facilities  combusting
RDF with coal. Emphasis is being placed  on po-
tential lead emissions to the air from current and
planned incinerators and RDF plants over  the
next several years.
  A study to assess the environmental impact of
resource recovery was completed. It  showed that
the net environmental impact of RR from MSW
will be primarily beneficial. Emissions from most
air pollutants will be reduced. Discharge of some
pollutants to surface waters will increase. Less
landfill capacity will be  required for disposal of
MSW. Energy savings will  be  realized from en-
ergy conservation in materials production and
energy  recovery from  MSW. The analysis is
based on specific scenarios selected from MSW
20

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disposal in 1990 with and without resource
recovery.


Special Studies

  SHWRD is responding to mandates of RCRA by
conducting several special studies. These studies
are designed to provide status reports to the Con-
gress on various  aspects of resource recovery.
Studies include assessments of selected small-
scale, low technology resource recovery meth-
ods, evaluation of the compatability of source
separation with centralized resource recovery fa-
cilities, and techniques for forecasting the quality
and  composition of municipal solid waste. In
other special studies,  research priorities for re-
source recovery are being assessed as are  the
impediments to the economical operation  of re-
source recovery facilities. The status of glass and
plastics resource recovery, and the impediments
to passenger tire recycling are the subjects of
other special studies.
  The study of forecasting the quantity and com-
position  of MSW showed that, based on the
model assumptions, per capita generation of
waste will increase at a rate less than the rate of
increase projected for the GNP through  1990.
This is largely accounted for  by the projected
substitution of light materials  (plastics, alumi-
num, etc.) for glass and steel. The study of eco-
nomic impediments to resource recovery facili-
ties indicates that large MSW to RDF plants  are
uneconomical from a market point-of-view. Mod-
ular  incinerators with  heat recovery appear to
hold promise. These are preliminary findings
only.
  In the assessment of small-scale and low tech-
nology, the study showed that modular incinera-
tion  with heat recovery and source separation
were the most feasible  at this time. Scaled
downed versions  of other technologies or sys-
tems appear unacceptable.
  Results of the study to determine the  com-
patibility of source separation and centralized
processing  (high technology) are still being  re-
viewed, however, they tend to show that neither
source separation and centralized processing
(high technology) are still  being  reviewed,
however, they tend to show that neither source
separation nor mixed-waste processing alone
would provide maximum benefits to the Nation
and to the hypothetical community analyzed. A
combination was judged to provide the greatest
benefits. The study identified various combina-
tions and their relative value for providing  max-
imum benefit to a community from resource
recovery.
TOXIC AND HAZARDOUS WASTE TREATMENT

  Under the  mandates  of the Resource Con-
servation and Recovery Act and the Toxic Sub-
stances  Control Act, the EPA is in the process of
identifying hazardous and toxic materials man-
ufactured or generated by industrial operations
which, if not properly controlled, pose significant
environment and public health problems. Muni-
cipal waste disposal facilities are generally not
capable of treating and managing such materials
and their release in certain instances from unac-
ceptable disposal  sites  has led to highly un-
desirable environmental contamination. Accord-
ingly, SHWRD's research program  is concerned
with the identification/assessment of effective
techniques for treatment and control of toxic and
hazardous waste materials.
  These techniques involve biological processes,
incineration, and chemical/physical treatment, as
well as  the corresponding  economic and en-
vironmental impacts of such activities. The pro-
gram is  designed  to eliminate or reduce the
hazardous nature of wastes and to protect the
environment. The research program includes:
    1. Techno-economic  assessments
    2. Environmental impacts
    3. Treatment technologies

Techno-Economic Assessment

  A study has been completed which quantified
the amount  of industrial hazardous waste dis-
posed of in public sector facilities. This analysis
determined industrial waste types and disposal
method of generators' Standard Industrial Classi-
fication  (SIC)  Code. Five SIC codes were exam-
ined. These were chemicals and allied products,
petroleum refining and related industries, rubber
and  miscellaneous plastic products, leather and
leather  products, and electrical and electronic
machinery, equipment and supplies. These five
codes were found to account for 50 percent of the
hazardous waste generated in the  country; with
approximately 10 percent of this waste entering
the municipal sector.
  Other assessments being performed involve
the relevancy and adequacy of existing and de-
veloping processing techniques for selected haz-
ardous  wastes. Processes examined include
chlorinolysJs, deep-well injection, catalysis, con-
centration techniques for heavy metal waste, as-
sessment of techniques for treatment of selected
hazardous waste, biodegradation treatment pro-
cesses,  and state-of-the-art processes for
pesticide disposal.
  Economic evaluations of the interrelationships
between control costs and regulations for haz-
                                                                                       21

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                              Figure 10.  Unit Cost Calculator.
                                Subtotal Capital Costs
                              Subtotal Direct O & M Costs
     Xo/
 ^^^ซ /o
y    o/
X    %
     Xz
 	%
                                Amount Funds Needed During Construction

                                Working Capital   	
                   F-
                   "-^X	
   =  Administrative Overhead
   =  Total Capital Costs    -*—

   =  Debt Service/Amortization
%  =  Allowance for R E. Taxes & Insurance
                      X Inflation Factor = Direct Operating Costs
                   Admin. Overhead X Inflation Factor + Debt Service/Amotization
                   + R.E Taxes & Insurance  = Indirect Operating Costs 	
                           I  =  Total Annuahzed Costs
                      X Present Value Factor  =  Present Value Annual Costs
                   Divided by Annual Throughpart
                   Simple Averages.
                                • Life Cycle
                                         Unit Cost
ardous waste treatment and disposal are being
conducted. For example, a study to evaluate the
cost-effectiveness of available treatment and dis-
posal alternatives for hazardous wastes to meet
proposed RCRA regulations is  underway. Some
16 treatment and  5 disposal unit processes ap-
plicable to  selected industries  are  being  evalu-
ated for life cycle and simple average costs
(Figure 10. Unit Cost Calculator) using a compu-
ter-assisted cost/performance program. Pre-
liminary indications are the flotation, filtration,
and hydrolysis rank among the more cost-effec-
tive treatment options, while encapsulation and
land disposal are most cost-effective among the
disposal options.

Environmental Impact

  Pollution levels associated with the processing
of hazardous waste are being  studied to deter-
mine the environmental impacts. One project is
evaluating both toxicity of  by-products and the
                    associated health and environmental hazards of
                    air emissions from selected hazardous waste
                    management facilities. Sampling and analysis
                    are underway at several locations. Thus far, no
                    hazardous  levels of emissions have been de-
                    tected at any of the test sites.
                      A second newly initiated project will assess the
                    nature and magnitude of hazardous pollutants
                    discharged into the environment from the barrel/
                    drum reconditioning industry. To date, there is
                    little  information on the nature and extent of air,
                    land, and water pollution caused by improper
                    reconditioning of barrels and drums.

                    Treatment Technologies

                      To  effectively process the diverse hazardous
                    wastes generated, many treatment technologies
                    have been evaluated. A study to assess new haz-
                    ardous waste treatment technologies is ongoing.
                    The objective  of this study is to identify and eval-
                    uate  technologies that are  more cost-effective
22

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than the treatment method now being used.
  Microwave plasma detoxification of various
forms of hazardous wastes was successfully
tested at 5-7 pounds per hour in the laboratory. A
larger 15 kilowatt,  10-12 pounds  per hour unit
effectively destroyed  several complex chlori-
nated gases, but liquids and solids were  in-
completely treated because of  undeveloped
evaporation techniques. Two to five years of addi-
tional research and development may be needed
to perfect the technology for wide ranges of ma-
terials at larger scales. Meanwhile, tests with real
nerve gases (U.S. Army) and PCB's (Canadian
Electrical Association)  are continuing. The U.S.
Environmental Protection Agency plans to dem-
onstrate a new pesticide laboratory unit around
1982.

BIOLOGICAL/CHEMICAL/PHYSICAL
TREATMENT

  A specially constructed pesticide pit has been
evaluated for three years and has proven to be an
effective method for containment of excess
pesticides and rinse waters generated by farmers
and applicators. Monitoring of air and water in
the surrounding  area  has  shown no pesticide
contamination. Study of the pit content has  re-
vealed that microorganisms are present and  ca-
pable of destroying many of the pesticides
discharged into the pit. In areas where pesticide
pit disposal will have limited application, filtra-
tion/adsorption techniques are being developed.
Identification of filtration/adsorption for effective
treatment of pesticide waste water will provide
for pesticide removal  and safe discharge of
treated water to sewers.
  Treatment of  hazardous  wastes by con-
centration of technologies is being evaluated. In-
dividual unit processes under going evaluation
are chemical coagulation'and precipitation, bio-
logical  treatment of activated sludge, activated
carbon adsorption,  resin adsorption, reverse os-
mosis, ultrafiltration, and air or steam stripping.
Using the above  unit processes and developed
process trains, bench and pilot scale treatability
studies will be performed on hazardous wastes
and leachates. The leachate from Love Canal is a
prime example. The objective of the study is to
develop concentration technologies for the  re-
moval of hazardous constituents and enable the
majority of the waste to be discharged to existing
municipal treatment plants. As a result, the con-
centrated wastes can be cost-effectively treated,
incinerated or disposed of in secure landfills.
  Techniques to control inorganic  chemical
wastes, especially heavy metals, have been iden-
tified and evaluated. Three techniques that have
broad application for hazardous inorganic con-
stituents are high gradient magnetic separation,
solvent extraction, and chemical precipitation.
Demonstration and verification of these selected
techniques for treatment of inorganic pollutants
from municipal landfills, surface impoundments,
and  hazardous waste treatment facilities are
ongoing.
  A chemical method is  being developed  and
evaluated for detoxification of halogenated  haz-
ardous chemical wastes. The active reagent is for
treatment  of molten sodium  and polyethylene
glycol. Thus far, the method has proven effective
for decomposition of hexachlorocyclohexane,
tricholorobenzene, Kepon, DDT, and more impor-
tantly, PCB-contained dielectric fluids. Fields ver-
ifications  are planned  at the conclusion of
laboratory studies.
  Encapsulation techniques have been  de-
veloped for safe storage and/or disposal of  haz-
ardous waste. This project has researched and/or
evaluated the use of cement for encapsulating
small containers of waste; the use of large ce-
ment containers, i.e., culverts, missile silos, etc.
for the disposal of waste; and the four polymeric
techniques which include encapsulation of 55-
gallon drums or other containers. Encapsulating
materials formed with the polymeric techniques
are unique in their capabilities to resist physical


                                  CYLINDER
                                     CLAMP
                                   FLATTEN
                                     COVER
                                     VALVE
                                    HEATER


                                      PUMP




                               RECEPTACLE
                               	—"

                              55-GAL DRUM
  Figure 11. Apparatus for encapsulating
             55- gallon  drums holding
             hazardous wastes.
                                                                                      23

-------
and chemical stresses. They are tough, flexible   laboratory scale for three processes, while full-
coatings which prevent leaching of materials into   sca|e Work is proceeding for the fuse welding
or from the matrix.  Process development and   process for encapsulating 55-gallon containers.
product evaluations have been conducted on a   (Figure 11)

RELATED RESEARCH PUBLICATIONS

 1. Abeles, T.R et al. ENERGY AND ECONOMIC ASSESSMENT OF ANAEROBIC DIGESTERS AND
   BIOFUELS FOR RURAL WASTE MANAGEMENT. EPA-600/7-78-174, December 1978.
 2. SCS Engineers. SELECTED BIODEGRADATION TECHNIQUE FOR TREATMENT AND/OR ULTIMATE
   DISPOSAL OF ORGANIC MATERIALS. EPA-600/2-79-006, March 1979.
 3. Oberacker, D.A. AIR POLLUTION SAMPLING AND MONITORING AT HAZARDOUS WASTE MAN-
   AGEMENT FACILITIES. Paper presented at 72nd APCA Annual Meeting and Exhibition, Cincinnati,
   Ohio, June 1979.
 4. Carnes, R.A. CURRENT STATUS OF USEPA INVOLVEMENT IN CARBON FIBER RESEARCH. Paper
   presented at a technical  information exchange seminar for various agencies involved in carbon
   fiber management, Hampton, Virginia, May 1979.
 5. Carnes, R.A. CURRENT USEPA/SHWRD ACTIVITIES IN HAZARDOUS WASTE INCINERATION AC-
   TIVITIES. Paper presented in a  five state regional symposium on  hazardous waste research,
   Chicago, Illinois, May 1979.
 6. Wiles, C.C. FEDERAL SUPPORT FOR DEVELOPING DESIGN CRITERIA FOR SOLID WASTE SHRED-
   DER EXPLOSION VENTS. Paper presented at Explosion Protection for Solid Waste Shredders
   Seminar, New Castle, Pennsylvania, June 1979.
 7. Carnes,  R.A. HAZARDOUS WASTE INCINERATION AND GASEOUS WASTE POLLUTION CON-
   TROL. Paper presented at 72nd APCA Annual Meeting and Exhibition, Cincinnati, Ohio, June 1979.
 8. Carnes, R.A. PARAMETRIC EVALUTION OF A FIELD SCALE HAZARDOUS WASTE INCINERATOR.
   Paper presented at 72nd APCA Annual Meeting and Exhibition, Cincinnati, Ohio, June 1979.
 9. Roulier, M.H. and N.B. Schomaker. RESEARCH ON POLLUTANT TRANSPORT. Paper presented at
   NATO/CCMS meeting, Vancouver, British Columbia, June 1979.
10. Carnes, R.A. THE THERM AL DECOMPOSITION ANALYTICAL SYSTEM (TDAS): ITS DEVELOPMENT
   AND APPLICATION. Paper presented at 72nd APCA Annual Meeting and Exhibition, Cincinnati,
   Ohio, June 1979.
11. Carnes, R.A. UDRI EFFORT. Paper presented at 72nd APCA Annual Meeting and Exhibition, Cincin-
   nati, Ohio, June 1979.
12. Ham, R.K., et al. RECOVERY, PROCESSING, AND UTILIZATION OF GAS FROM SANITARY LAND-
   FILLS. EPA-600/2-79-001, February 1979.
13. Roulier, M.H. FIELD VERIFICATION OF GAS MIGRATION. Paper presented at SHWRD Fifth Annual
   Research Symposium, Orlando, Florida, March 1979.
14. Brunner, D.R. FORECASTING PRODUCTION OF LANDFILL LEACHATE. Paper presented at SHWRD
   Fifth Annual Research Symposium, Orlando, Florida, March 1979.
15. Carnes,  R.A. A HAZARDOUS WASTE INCINERATION PROGRAM. Paper  presented at  Second
   National Conference on Hazardous Materials Management, San Diego, California, March 1979.
16. Roulier, M.H. MODELING POLLUTANT MOVEMENT IN SOIL Paper presented at SHWRD Fifth
   Annual Research Symposium, Orlando, Florida, March 1979.
17. Klee, A.J. AN OVERVIEW OF RESOURCE RECOVERY ACTIVITIES. Paper presented at SHWRD Fifth
   Annual Research Symposium, Orlando, Florida, March 1979.
18. Wiles, C.C. PRODUCTION AND USE OF DENSIFIED RDF Paper presented at SHWRD Fifth Annual
   Research Symposium, Orlando, Florida, March 1979.
19. Leone, I.A., FB. Flower, E.F Gilman and J.J. Arthur. ADAPTING WOODY SPECIES AND PLANTING
   TECHNIQUES TO LANDFILL CONDITIONS. EPA-600/2-79-128, August 1979.
20. Fletcher, M.W. and D.E. Fiscus. ANALYSIS OF AIRBORNE VIABLE BACTERIA AT SOLID  WASTE
   PROCESSrNG FACILITIES. EPA-600/2-79-131, August 1979.
21. Fiscus, D.E., RG. Gorman, M.R Schrag, and L.J. Shannon. ASSESSMENT OF BACTERIA AND VIRUS
   EMISSIONS AT A REFUSE DERIVED FULL PLANT AND OTHER WASTE HANDLING FACILITIES;
   EXECUTIVE SUMMARY. EPA-600/8-79-010, August 1979.
22. Gorman, RG., D.E. Fiscus,  M.R  Schrag, and L.J. Shannon. COMPARISON OF METHODS FOR
   SAMPLING BACTERIA AT SOLID WASTE PROCESSING FACILITIES. EPA-600/2-79-090, August
   1979.

24

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23. U.S. Army Engineer Waterways Experiment Station. EFFECTS OF FLUE GAS CLEANING WASTE
   ON GROUNDWATER QUALITY AND SOIL CHARACTERISTICS. EPA-600/2-79-164, August 1979.
24. Styron, C.R. Ill and Z.B. Fry, Jr. FLUE GAS CLEANING SLUDGE LECHATE/LINER COMPATIBILITY
   INVESTIGATION; INTERIM REPORT. EPA-600/2-79-136, August 1979.
25. Efaw, F and W.N. Lanen. IMPACT OF USER CHARGES ON MANAGEMENT OF HOUSEHOLD SOLID
   WASTE. EPA-600/5-79-008, August 1979.
26. Fungaroli, A.A. and R.L Steiner. INVESTIGATION OF SANITARY LANDFILL BEHAVIOR; VOLUME I.
   FINAL REPORT. EPA-600/2-79-053a, July 1979.
27. Fungaroli, A.A. and R.L Steiner. INVESTIGATION OF SANITARY LANDFILL BEHAVIOR; VOLUME II.
   SUPPLEMENT TO THE FINAL REPORT. EPA-006/2-79-053b, July 1979.
28. Copenhaver, E.D. and B.K. Wilkinson. MOVEMENT OF HAZARDOUS SUBSTANCES IN SOIL: A
   BIBLIOGRAPHY; VOLUME 1. SELECTED METALS. EPA-600/9-79-024a, August 1979.
29. Copenhaver, E.D. and B.K. Wilkinson. MOVEMENT OF HAZARDOUS SUBSTANCES IN SOIL: A
   BIBLIOGRAPHY; VOLUME 2. PESTICIDES. EPA-600/9-79-024b, August 1979.
30. MUNICIPAL SOLID WASTE: LAND DISPOSAL. In:  Proceedings of the Fifth Annual Research
   Symposium, M.R Wanielista and J.S. Taylor, eds. EPA-600/9-79-023a, August 1979.
31. Gordon, J.G. ASSESSMENT OF THE IMPACT OF RESOURCE RECOVERY ON THE ENVIRONMENT.
   EPA-600/8-79-011, August 1979.
32. Wigh, R.J. BOONE COUNTY FIELD SITE INTERIM REPORT;  TEST CELLS 2A, 2B, 2C, 2D.
   EPA-600/2-79-058, July 1979.
33. Ham,  R.K., M.A. Anderson, R. Stegman and  R. Stanforth. COMPARISON OF  THREE WASTE
   LEACHING TESTS. EPA-600/2-79-071, July 1979.
34. Ham,  R.K., M.A. Anderson, R. Stegman, and  R. Stanforth. COMPARISON OF  THREE WASTE
   LEACHING TESTS; EXECUTIVE SUMMARY. EPA-600/8-79-001, May 1979.
35. Lutton, R.J., G.L Regan and L.W. Jones. DESIGN AND CONSTRUCTION OF COVERS FOR SOLID
   WASTE  LANDFILLS. EPA-600/2-79-165, August 1979.
36. Thompson, D.W. ELUTRIATE TEST EVALUATION OF CHEMICALLY STABILIZED WASTE MATE-
   RIALS. EPA-600/2-79-154, August 1979.
37. Haxo, H.E. Jr., R.S. Haxo, and T.F Kellogg. LINER MATERIALS EXPOSED TO MUNICIPAL SOLID
   WASTE  LEACHATE; THIRD  INTERIM REPORT. EPA-600/2-79-038, July 1979.
38. Van Noordwyk, H., L Schalit, W. Wyss, and H. Atkins. QUANTIFICATION OF MUNICIPAL DISPOSAL
   METHODS FOR INDUSTRIALLY GENERATED HAZARDOUS WASTES. EPA-600/2-79-135, August
   1979.
39. Rogers,  C.J. RESEARCH  ON THE IN-SITU  TREATMENT OF TOXIC ORGANIC LANDFILL CON-
   TAINMENTS. Paper presented at Office of Science & Technology and ISETAP workshop, Biological
   Treatment for Wastes Contained in Existing Non-Nuclear Hazardous Waste Dumpsites, Wash-
   ington, D.C., August 1979.
40. James, S.C. METHANE GAS PRODUCTION BY MIXING MSW-MSS IN LARGE SCALE ANAEROBIC
   DIGESTERS. Paper presented at Conference on Land Disposal of Municipal and Industrial Waste,
   Madison, Wisconsin, September 1979.
41. James, S.C. and C. Rhyne.  METHANE RECOVERY FROM THE CITY OF MT. VIEW, CALIFORNIA.
   Paper presented at Conference on Land Disposal of Municipal and Industrial Waste, Madison,
   Wisconsin, September 1979.
42. James, S.C. RECOVERY OF LANDFILL GAS AT MT. VIEW. Paper presented at Engineering Founda-
   tion Conference on Resource Recovery, Henniker, New Hampshire, July 1979.
43. Landreth, R.E. UPDATE ON EPA ACTIVITIES. Paper presented at 87th AlChE  National Meeting,
   Boston, Massachusetts, August 1979.
44. Carnes, R.A. USEPA CARBON FIBER RESEARCH PROGRAM. Paper presented to Office of Science &
   Technology, White House, Washington, D.C., September 1979.
                                                                               25

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                      WASTEWATER RESEARCH DIVISION
  The Wastewater Research Division (WRD) was formed in July of 1975 from the Advanced Waste
Treatment Research Laboratory which  had been initiated in Cincinnati in  1960. Advanced waste
treatment work had been carried out under both the U.S. Public Health Service and the Department of
the Interior before the establishment of the U.S. Environmental Protection Agency in 1970. With the
passage of Public Law 92-500 in 1972, with changes in the national perception of municipal research
problems, and with a consolidation of USEPA municipal wastewater pollution research within MERL,
the range of topics expanded beyond those formerly addressed. Wastewater Research Division had
become a more accurate description of the program.
  Following the special topics is a description of the work and of important accomplishments in the
Division.
SPECIAL TOPICS

Urban and Rural Communities
Cooperate In Land Utilization of Sludge

  When a municipality decides that land applica-
tion of sludge is economically and environmen-
tally desirable, it is generally faced with the need
to convince the  potential recipients or the com-
munity at large that sludge reuse is a good thing.
Strategic plans are laid to choose the optimum
sites, keep the community informed, and estab-
lish a "climate of trust."
  The "climate  of trust" is often very hard to
establish. If the proposed recipient is a farmer, he
is asked to stake his farm and his livelihood on
the claims of "honest-looking" municipal offi-
cials, who clearly have their own reasons for en-
couraging sludge use on land, that sludge is safe
for  his crops, is not hazardous to his family's
health, and is a profitable replacement for much
of his fertilizer needs. The farmer knows that his
farm must still  be profitably producing crops
long after municipal authorities have left office,
engineering firms have  gone on to other jobs,
and those sewage treatment operators who were
so reassuring have transferred to some other
treatment plant. The farmer often concludes that
his safest course is to reject the sludge option.
  Another approach, hard at first, but more prof-
itable in the long run, is for the municipality to
surrender to the agricultural community some of
the decision-making authority about the use of
sludge, and let the farmer make up his own mind,
using his own information sources. The mecha-
nism to use is the unique intercommunication
web that provides the farmer with the informa-
tion he needs to do the best thing possible with
his land. Partners in the effort are private organi-
zations such as the Farm  Bureau Federations,
State and Federal agricultural extension services,
and the research programs of State and Federal
agricultural agencies. These organizations do not
produce all the information that a farmer needs,
but they are his reliable counselors that assess
the claims of equipment manufacturers, fertilizer
producers, and seed  suppliers,  and give the
farmer the good advice he needs.
  The conventional intercommunication channel
from sludge producer to receiver is not used. A
measure  of control  by the city  must be relin-
quished to the rural residents. The agricultural
community decides  what is safe,  what sludge
application rates are  appropriate, and even what
sludges should or should  not be used on land.
When this is done, the farm community reverses
itself,  and a  difficult struggle for acceptance is
turned into an enlightened program, where
knowledgeable people who have the trust of the
farmer make key decisions.
  In Ohio, the nearly traditional confrontation be-
tween farm and city has been encountered and
reversed. Cooperation between  State,  Federal,
and farm organizations has produced a model
program that may point the way nationally to the
resource-conserving utilization of all the sludge
that should be reused. With support of an EPA
demonstration grant to the Ohio Farm Bureau
Federation, Ohio is showing how city and coun-
try people can work together harmoniously to
use municipal sludge on farms to benefit both the
rural and urban communities.  Involvement of
concerned  residents of both  communities in
planning  and implementation of the sludge-use
project has enabJed  them to avoid the distrust
                                          26

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and strife that has plagued so many prior efforts
to recycle urban wastes on agricultural land.
  Although sludge use on land is common in this
country, there is still a general lack of understand-
ing among participating farmers and  munici-
palities of the  management procedures neces-
sary to assure the optimal benefits and minimal
health and environmental risks. Residents of the
communities involved in this project were invited
to educational  meetings where agricultural and
medical scientists discussed the use of sludge as
fertilizer- its benefits and risks. Thus, the nega-
tive attitudes associated with lack of information
have been avoided.
  Who is carrying out a project is often more
important than what is done, or how, in determin-
ing its acceptability. This demonstration was initi-
ated by the Ohio Farm Bureau  Federation,  an
organization of farmers dedicated to  the ad-
vancement of farmers. The Farm Bureau is one of
the oldest and largest farmer organizations in
America with County Farm Bureau Federations
combining to form the Ohio Farm Bureau Federa-
tion which in turn combines with other state
Farm Bureau Federations to comprise the Amer-
ican Farm Bureau Federation. The confidence
that the farmers have in the sponsoring organiza-
tion is  important in gaining  acceptance of, and
participation in such projects.
  The Ohio Farm Bureau Federation's interest in
a project to learn how to use sludge beneficially
developed out of its activities in defense of some
of its members who were threatened with loss of
their farms to a city for use as a municipal sludge
farm. With the assistance of The Ohio State Uni-
versity, College of Agriculture, the Federation
submitted an application for an EPA grant to sup-
port a large demonstration of safe beneficial use
of sewage sludge on privately owned farm  land.
The grant application was submitted at a conven-
ient time, because EPA was searching for a model
demonstration of a successful way to plan, im-
plement,  and conduct a sludge use program  on
farm land. Such a demonstration would involve
resolution of legal and institutional  obstacles,
following the best available site  management,
and  educational  programs to  publicize the
project.
  A grant was extended to the Farm Bureau De-
velopment Corporation in 1977. The scope of the
project was significantly expanded by addition of
an epidemiological study to assess the effects
upon the health  of animals and humans from
careful use of  sludge on farms.  The project is
funded jointly by EPA's Health Effects and Munic-
ipal Environmental  Research Laboratories in
Cincinnati.
  One of the important aspects of the project that
distinguishes it from most previous efforts to
apply urban wastes on rural  land is the great
number of participating agencies, organizations
and individuals that have cooperated in the plan-
ning and implementation of it. They represent.
the rural communities, the urban communities,
and the local, state, and federal government. The
Ohio Farm Bureau Development Corporation ac-
cepted the EPA grant, contributed 25 percent of
the funds, and provided overall supervision and
direction. The Ohio State University and the Ohio
Agricultural Research and  Development Center
serve as subcontractor and perform most of the
scientific research work. The College of Agricul-
ture participates through three departments and
the Cooperative Extension  Service. The Depart-
ment of Agronomy tests soils and sludges and
recommends sludge application rates and other
soil and crop management practices to be fol-
lowed. Soils and crops are  periodically sampled
and analyzed to determine changes caused  by
use of sludge. The Department of Agricultural
Engineering  advises in  matters concerning
sludge handling and application and studies the
effect of sludge on soil density and compaction.
The Department of Agricultural Economics as-
sesses the economic impact of various sludge
handling and application systems on the farm
enterprise. The Extension Service is the leader in
information dissemination and in obtaining
farmer cooperators. They also set up field days
and collect soil and plant samples.
  The College of Medicine, The Ohio State Uni-
versity, participates in the epidemiological stud-
ies through two departments. The Department of
Medical Microbiology analyzes sludge for patho-
genic bacteria and viruses, and evaluates sludge-
treated soil to determine the rate of survival of
these pathogens. They also examine the cooper-
ating farm families to determine any evidence of
bacterial or viral infections  from sludge applica-
tion. The Department of Preventive Medicine co-
operates in design of the epidemiological study
and in analyzing the data.
  The College of Veterinary Medicine cooperates
in the study of the effect of sludge use on human
health and monitors the effect of sludge on the
health of domestic animals. They evaluate the
effects of metals, Salmonella, and parasites.
They also perform the Tuberculin sensitivity test
on farm animals.
  All of the  participating departments of The
Ohio State University (OSU) and the Farm Bureau
have cooperated under the  leadership of the Co-
operative Extension Service in conducting meet-
ings to inform both rural and urban residents of
                                                                                     27

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the objectives and plans of the project and  in
obtaining cooperation of farmers. Volunteers  to
receive and use sludge and their neighbors have
been fully informed of benefits and risks involved
in sludge use on farms. Thus, enlightened deci-
sions are made possible by publicity and educa-
tional programs. By involving  affected residents
in both  the  rural and urban  communities, the
volatile  reaction that sometimes accompanies
the initiation of waste disposal projects has been
avoided.
  Some of the other participants in the project
include  the Ohio Municipal League, State and
County  Health  Departments and the municipal
officials of the cities that furnish sludge for the
project.  Wastewater treatment officials transport
and apply sludge on farms, sample sludge for
analyses, and participate in educational phases
of the program. The Ohio EPA is responsible for
regulating sludge disposal  within the  state,  so
they not only approve sites but also participate in
planning and implementation  of the project.
  The four communities that were originally se-
lected for participation in the project were chosen
because of geographical distribution and be-
cause of the soil and cropping patterns that were
found there. In the meantime, one community,
Montgomery County, withdrew because person-
nel changes in the Sanitary District resulted  in
loss of interest in the project. They were replaced
by Columbus. Defiance elected not to participate
in the health  effects studies, but they have ap-
plied sludge on a few farms and the environmen-
tal effects are being measured. Zanesville had  to
withdraw because they could not produce sludge
of desirable quality. The cadmium concentration
was higher than desirable and efforts to control
the influent to the treatment plant were not suc-
cessful.  Springfield replaced Zanesville and is in
the process of conducting educational meetings,
obtaining  participating farmers, and planning
the sludge application schedule. Medina County
was the first community to get started in sludge
application and with the epidemiological studies.
They have nine farms receiving sludge and par-
ticipating in the health studies. In addition, seven
farms that receive no sludge are participating in
the epidemiological studies. Columbus entered
into the study late but have 21  farms that receive
sludge  and 20 farms that have  not  received
sludge  participating in the  epidemiological
studies.
   The plan for sludge application and site man-
agement is a  responsibility of the  OSU Agron-
omy Department. Acid soils are limed as need is
indicated by a soil test. Sludge is being applied to
supply the phosphorus needs  of the crop as indi-
cated by the soil test. Therefore, the application
rates, which range from 1 to 5 tons per acre of
sludge solids, are lower than they would be if
they were determined by the crop's nitrogen re-
quirements. These low  application  rates assure
that the risk of environmental or health problems
will be very low.  Supplementary nitrogen and
potassium are usually needed.
  Tours and field days are very important for
publicizing the project. The Ohio State University
established plots  on  the demonstration site of
The Ohio State University's Farm Science Review,
an annual  three-day exposition of the  latest
methods and  materials used in agriculture.
About  100,000 people attended  the exposition.
Several thousand viewed the plots where sludge
had been applied  at several rates and heard the
investigators discuss the benefits and risks of
sludge use.
  The epidemiological study is an important as-
pect of the study because it provides assurance
to participants that no adverse effect on their
health, if it  does occur, will be untreated. These
studies  began in Medina  County and  in
Zanesville and  Columbus vicinities in 1978. A
total of 1304 questionnaires were completed and
checked.  Each examination and  interview was
conducted with a physician and nurse. Blood and
stool samples are collected and analyzed in addi-
tion  to the physical examination to determine
general health. To date, no differences in rate of
illness or other indicators between sludge  users
and the non-users have been detected. Sixteen
calves we re tested prior to sludge application and
at the time  of slaughter with no adverse effects
being detected. Sludge and fertilizer have been
equally effective in enhancement of crop growth
and yields.The value of the nutrients in oneton of
sludge varies from about $7.00  to $46.00,  de-
pending upon the composition of the sludge.
  Although results of the project are preliminary
and  no conclusions  can  be drawn concerning
eventual environmental or health effects, it is ap-
parent that publicity,  educational programs and
cooperative planning can do  much to alleviate
the suspicion and  fear that often accompany the
disposal of urban  wastes in a rural community.
  An average sludge  applied to a crop that uses
the nutrients efficiently, at a rate of 3 tons  per
acre, is worth $75.00  per acre.

Tertiary Wastewater Filtration

  Filtration is considered to be the most impor-
tant  tertiary process in the implementation of
the Federal Water Pollution Control Act Amend-
ments of 1972 and 1977. Many existing secondary
wastewater treatment  plants cannot meet the
 28

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minimum monthly average effluent standard of
30 mg/l for suspended solids and biochemical
oxygen demand (BOD)  established by the En-
vironmental Protection Agency in  1973. This is
particularly true for small plants where removal
efficiency is usually less than that achieved for
large plants. The addition of tertiary filters will
enable many plants to meet the standard and
higher treatment levels for water quality limited
streams. A survey conducted in 1974 identified
only 77 operating U.S. tertiary filters treating sec-
ondary effluents with flows greater than 0.3 mgd
(1,136 m3/day). Based on tertiary filtration needs
compiled in 1974, tertiary filters will be required
at over 1500 plants to achieve water quality stand-
ards established by the 1972 Act. Approximately
94 percent of the plants will  be smaller than 5
mgd  (18,925 m3/day) and  80  percent will  be
smaller than 1 mgd (3,785 m3/day).
  Research  on  tertiary wastewater filtration in
the United States began in the mid-1960's. Since
then numerous pilot-scale studies have been
conducted  to evaluate the effect of media size,
media depth, and flow rate on process perfor-
mance. It is generally recommended that pilot-
scale studies be conducted at each site to develop
design parameters for full-scale plants since fil-
tration models cannot be used to reliably predict
performance. The classical  mechanisms for in-
depth filtration, that were developed from stud-
ies of potable water filtration and from laboratory
studies using suspensions with controlled prop-
erties do not adequately describe suspended sol-
ids  removal for direct filtration of secondary
effluents due to straining of large particles at or
near the surface of the filter medium. In previous
wastewater filtration studies, insufficient atten-
tion  has been given to the effect of secondary
effluent suspension properties on particle collec-
tion mode and clarification efficiency.
  A study has recently been completed at North-
western University with objectives to gain  a
clearer understanding of parameters affecting
the  clarification efficiency of full-scale granular
media wastewater filters and to develop opera-
tional mathematical models to describe primarily
this clarification efficiency. Operating and perfor-
mance data were collected  on tertiary filters at
eight small treatment plants in the Chicago met-
ropolitan area. The treatment plants had design
flows between 0.8 and 2.5 mgd (3028 and 9462
m3/day) and used 2-7 filters.  Products from six
filter manufacturers were represented. Filter de-
sign flows  ranged 1.0-4.3 gpm/ft2 (41-175 1/min-
m2). Five plants had filter configurations shown in
Figure 12 with a backwash storage tank located
above the sand and anthracite dual filter media.
 FILTER
 INFLUENT
               INFLUENT
               SPLITTER BOX
EFFLUENT
    WEIR.
              BACKWASH
              STORAGE
              TANK
                                   FILTER
                                   EFFLUENT
              UNDERDRAINS
 BACKWASH
 DISCHARGE
            Figure  12.  Filter design.

The other plants included either trimedia filters
or single media sand filters of  unique design.
Typical filter installations are shown in Figures 13
and 14.
Figure 13. Picture of tertiary filter installation.

  Filter clarification efficiency was characterized
using conventional design and operating param-
eters, and the statistical properties of secondary
effluent and filter effluent parameters were deter-
mined. Averaged secondary effluent suspended
solids varied from  28 to  62 mg/l for the eight
plants and average filter effluent suspended sol-
ids from 5 to 20 mg/l. The average  removals of
suspended solids varied from 47 to 83 percent for
the eight plants. Average secondary efluent BOD
                                                                                       29

-------
                                             percent of the data for three plants.
                                              The most important single design considera-
                                             tion for small tertiary filtration plants that are not
                                             staffed 24 hours per day is the ability to handle
                                             secondary process upsets. This consideration
                                             appears to favor dual-media designs with rela-
                                             tively large media and high terminal headloss.
                                             Regular inspections should be made to detect
                                             problems in operation and preventive and cor-
                                             rective maintenance should be promptly sched-
                                             uled, this applies  particularly to accessories
                                             such as control valves which were observed to
                                             stick frequently in the open position.
                                              In summary, tertiary filters provide a very effec-
                                             tive means for upgrading secondary effluent to
                                             meet water quality standards  if proper design
                                             criteria are followed.

                                             TREATMENT PROCESS DEVELOPMENT
                                             BRANCH
                                              The Treatment Process Development Branch is
                                             responsible for the development of technology
                                             and processes  in the areas of biological treat-
                                             ment, physical-chemical treatment, and the ulti-
                                             mate disposal of solids.
                                              Full-scale evaluations completed this year in-
                                             cluded  the activated bio-filter  system, the Max
                                             Plank Institute trophic system, and three types of
                                             fine bubble submerged air aeration systems. The
                                             first municipal Deep Shaft System in the United
                                             States was placed on stream at Ithaca, New York.
                                             A 16-month experimental program has  been
                                             designed.
                                              A study was completed on analyzing the oper-
                                             ating and performance data from tertiary filters at
                                             eight small treatment plants. The data showed
                                             that tertiary filters provide a very effective means
                                             for upgrading secondary effluents if proper de-
                                             sign criteria are followed.
                                              Cost  effectiveness is an important considera-
                                             tion of  any sludge treatment process. Cost esti-
                                             mates are being prepared on  three interesting
                                             processes: hot acid extraction to remove metals
                                             and improve dewaterability, vericomposting, and
                                             aerobic digestion that will pasteurize the sludge.
                                              A sizable portion of the Branch research effort
                                             has been  devoted  to determining the  fate and
                                             effects of nutrients and trace elements in sludge-
                                             treated soils. Copper, nickel and zinc have been
                                             identified as metals that are most likely to cause
                                             phytotoxicity. Cadmium is the element of most
                                             concern because of its adverse effect on human
                                             beings.
Figure 14. Picture of tertiary filter installation.

varied from 9 to 44 mg/l and average filter effluent
BOD varied from 3 to 25  mg/l. The average re-
movals of BOD varied from 18 to 87 percent for
the eight plants depending largely on the soluble
BOD content of the secondary effluent. Limited
tests at two plants showed that a significant frac-
tion  of the soluble BOD  was removed by the
filters.
  For plants where flow to individual filters was
varied, average clarification efficiency decreased
linearly with average flow rate. Correlation coeffi-
cients between filter solids removal efficiency
and  operating parameters such as flow, solids
loading and run length were poor for data ob-
tained over long time frames, improved correla-
tions were, however, obtained for data analyzed
over shorter time periods which minimized the
effect of seasonal and other variations in second-
ary plant effluent suspension characteristics. Dif-
ferences in characteristics of secondary effluent
suspended solids rather than media  grain size
and  depth are most likely the major reason for
variations in clarification efficiency between
plants.
  The following semiempirical  model was de-
veloped for in-depth filtration: C = 0.40C0086Q034
where:  C =  filter effluent suspended solids
              - mg/l
        C0 =  secondary effluent suspended
               solids- mg/l, and
        Q =  filtration rate - gpm/sf
In testing with independent data, the in-depth
model was able to predict C within  ฑ 25 to 85
RELATED RESEARCH PUBLICATIONS

Bunch, R.L. PILOT PLANT DEVELOPMENT OF OZONE DISINFECTION.  Presented at Conference on
Physical Methods for Water and Watewater Treatment, Lublin, Poland, June 7-9,1979 (Proceedings
published by Pergamon Press).
30

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Ultimate Disposal Section

  The primary responsibility of the Ultimate Dis-
posal program is to find environmentally accept-
able and cost-effective approaches for treatment
and disposal  of municipal wastewater sludges.
Frequently, toxic and pathogenic substances are
either not  present or can be neutralized so that
constructive use can be made of the sludge. It is
the program's responsibility to develop  the po-
tential for reuse to a maximum while at the same
time safeguarding the environment from possi-
ble harm.
Sludge Processing and Treatment

  Sludge processing and treatment include all of
the steps from the first appearance of sludge until
it enters the disposal step. A determined effort is
underway to scrutinize quantitatively the cost-
effectiveness of processes under development. A
Boston-based engineering firm  is completing
cost estimates of three processes: hot acid treat-
ment of sludge to remove metals and upgrade
sludge dewaterability, vermicomposting - the
use of earthworms to process sludge into a high
grade potting soil, and  aerobic digestion of
sludge under conditions such that self-heating
occurs and pasteurizes the sludge. If the proc-
esses  prove competitive, the next step will be
either large-scale  pilot plant construction or
demonstration.
  The LA/OMA (Los Angeles, Orange County
Metropolitan Area) project - an areawide study
supported by EPA, is aimed at developing the
best options for sludge processing and disposal
in this geographical area. Experimental and engi-
neering studies are completed and recommen-
dations have been made. Public documentation
of this project is now underway with  MERL
support.
  Energy reduction in all aspects  of wastewater
treatment is of  primary  concern;  however, if
sludge is properly treated and utilized, it is possi-
ble not merely to reduce energy use but even to
generate a major part of the energy needed in
other parts of the plant. The Wilton, Maine, plant
- an energy self-sufficient facility using solar en-
ergy and the methane generated in sludge diges-
tion - was dedicated in the Fall of 1979. The plant
was built with EPA funds and an evaluation is
being financed by a joint EPA-Department of En-
ergy grant. MERL will also be supporting along
with DOE and the State of California a project, in
which a modular turbine is bieng developed to
generate heat and electricity from sludge gas.
The development of a low-cost modular turbine
is expected to make recovery of energy from
methane cost-effective in smaller plants than is
possible now.
  The pathogen content of sludge is a major con-
cern if sludges are to be reused for agricultural
purposes or soil renovation. It is important to
determine the effect of conventional treatment
processes on pathogen densities, and if possible
develop cost-competitive methods that pasteur-
ize the sludge.  Disinfection of sludge by ther-
moradiation is being studied at Sandia Laborato-
ries in a project jointly funded with the Depart-
ment of Energy. Previous excellent results show-
ing inactivation of all pathogenic forms at bench
scale in sludge by thermoradiation will soon be
demonstrated at pilot scale. In a study  at the
University of Florida, inactivation of virus  and
bacteria in  sludges during aerobic digestion is
being investigated. Demonstration of a two-step
thermophilic aerobic-anaerobic digestion pro-
cess for sludge stabilization, developed by Union
Carbide Corporation, has reached the operating
stage. In  this process, sludge is aerobically di-
gested with oxygen for about one day,  which
causes it to self -heat to over 55ฐC. The sludge is
then processed in a mesophilic digester  for an
eight-day stabilization period. The sludge is ex-
pected to be pathogen-free.
  In-house evaluations of modern  dewatering
equipment are  underway at the new Test  and
Evaluation Facility at Cincinnati's Mill Creek plant.
An  important study is  underway to determine
whether a high-metals fraction of sludge can be
"scalped off" by passing liquid sludge through a
solid-bowl "classifying" centrifuge. The small
high-metals fraction could be separately  dis-
posed of, whereas the bulk of the sludge could
now be constructively reused on the land.

Sludge Conversion

  Sludge conversion is any process that changes
the nature  of the  sludge so that it is no  longer
perceived as sludge. The static-pile forced- aera-
tion process, developed by the U.S.  Department
of Agriculture with MERL and other EPA assis-
tance, continues to provide  answers  to the
sludge problems  of many communities. Com-
posting has provided a major relief valve for
communities with no  other acceptable sludge
disposal  options.  Our research efforts on  this
process now are concentrated  improvement of
the process and of our understanding of its fun-
damental nature.
  Composting sludge within vessels makes the
process even more acceptable to communities
than  unconfined processes. MERL  has funded
studies of  the economics  of European within-
vessel methods, as well as methods developed
                                                                                      31

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by United States firms. MERL will also be spon-
soring a test of composting in a barge-mounted
plant.
  Thermal conversion techniques, particularly
those utilizing a low-grade fuel to supplement the
thermal deficiency of dewatered sludge cake, are
the object of high  interest for sludge disposal.
MERL is evaluating acoincineration plant (sludge
and  refuse-derived fuel - RDF) at Duluth, Min-
nesota. At this plant,  solid waste is processed
into  metal and RDF fractions, the  RDF is burned
with sludge, and surplus steam is generated for
plant use. About 100 acres of scarce landfill space
will be saved annually by using this process.
  Two innovative processes that form sludge into
briquettes with another  fuel are  being  investi-
gated and show great promise. At the University
of California (at Davis),  sludge and RDF have
been pelletized and burned in a down-flow gas
producer. A grant application for a larger demon-
stration is in preparation.  In New York City at
Columbia University,  the Sanoplex process is
being evaluated with MERL support. In this proc-
ess, a low value caking coal is pelletized with RDF,
sludge, and a black liquor binder. The pellets are
partially  combusted with oxygen to produce a
medium  heating value fuel gas. Economic eval-
uations have been extremely encouraging. These
novel processes may provide the solution to the
sludge problem when  logistics and/or high met-
als content of sludge preclude constructive reuse
of sludge on land.

Beneficial Utilization and Disposal

  Beneficial utilization includes any constructive
use of sludge. The options for selection of sys-
tems for treatment, handling, and disposal of
sewage sludge are numerous; however, land is
the only acceptable ultimate  receiver of sludge.
Sludge may be utilized in or near the surface to
enhance soil productivity or it  maybe se-
questered beneath the surface. The former offers
the opportunity to consume some of the useful
constituents of sludge while disposing of it eco-
nomically in an  energy-use  efficiency manner.
Sequestering sludge in landfills, basins, or
trenches offers the possibility of economical dis-
posal where sludge quality  or site conditions
make landspreading unfeasible. More informa-
tion is needed for development of technology for
utilizing or disposing of sludge under the multi-
tude of sludge-soil-climate-land use conditions
that  may be encountered in  planning and con-
struction of public  wastewater treatment
facilities.
  Plant nutrients, inorganic components,  and
organic components of sludge can be beneficial
to soil and make it more productive, or they can
be harmful to the environment or hazardous to
public health,  depending  upon the amounts
added to the soil and their environmental fate.
The amount of each component that is accept-
able is dependent  upon site characteristics and
management.
  A sizable portion of MERL's research effort has
been devoted to determining the fate and effects
of the nutrients and trace elements in sludge-
treated soils.  Copper, nickel, and zinc have been
identified  as  metals that are more likely to ac-
cumulate to phytotoxic levels in  sludge-treated
soils.  Cadmium is the element of most concern
because of its potential adverse effects on human
health. It is assimilated by growing plants and is
accumulated in the  human liver and  kidneys.
Lead  is of concern if sludge-contaminated for-
ages are ingested by humans or animals. Nitrates
can leach  into ground water,  and both  nitrates
and phosphates can be  transported by surface
runoff into streams and reservoirs. Progress has
been made in identifying acceptable sludge ap-
plication rates and appropriate site management
techniques for application of specific sludges on
specific soil-climate-crop combinations. A grant
to Chicago is supporting a study of the accumula-
tive effects of annual sludge applications over a
long period of time. After 10 years, cadmium con-
centration ingrain does not appear to be increas-
ing. No phytotoxicity from metals has been
encountered. Corn yields from  sludge-treated
soils  are equivalent to, or superior to, con-
ventionally fertilized plots. With  MERL support,
the Science and Education Administration of the
U.S. Department of Agriculture at St. Paul, Min-
nesota, is developing site management technol-
ogy to enable the beneficial use of sludge as a soil
amendment. Diversion terraces, contour cultiva-
tion, and appropriate cropping systems are being
used to minimize runoff and leaching of soluble
and suspended sludge constituents. Animal
feeding of sludge-produced corn silage is being
used to determine the effect  of the cadmium-
enriched feed on animal health, carcass com-
position, and  milk composition.
  Toxic organic substances that may find their
way into sludge are of increasing interest. The
principal known organic constituents of sludge
are polychlorinated biphenyls (PCBs)  and
pesticides, but concentrations  of persistent
pesticides  in  sludge  are usually  lower than in
soils to which they are applied, so sludge applica-
tion should be  of concern only if sludges with
unusually  high concentrations of pesticides are
used.  PCBs are  adsorbed on soils and have low
solubility, plant  uptake is negligible, but surface
32

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contamination of crops could be significant. The
lack of data on the environmental fate of  the
priority organic compounds has led to the  de-
velopment of a grant with North Carolina State
University to determine their fate, and whether
they are taken up by plants.
  Pathogens in sludge and their possible trans-
mission to humans when sludge is used on soil
continue to be of concern. Technical support is
being provided to EPA's Office of Solid Waste for
the preparation of landfill criteria as required by
the Resource Conservation and Recovery Act of
1976. One of the issues  is the potential disease
risk from landspreading of sludges. At the Uni-
versity of Illinois, studies are continuing to deter-
mine whether worm-free pigs housed in pens
located on sludge-treated soils became infected
with parasites. Evidence  is accumulating that the
pigs can be infected by parasites (e.g., Ascaris
suum) by  either  direct feeding of sludge  or
through foraging on some sludge-treated soils. It
appears that the degree of exposure, which gov-
erns the opportunity for ingestion and parasite
density, must be very high to produce a signifi-
cant degree of infection.
  Laboratory studies are beginning at the Univer-
sity of Cincinnati to determine the rate of inactiva-
tion of helminth  eggs under sludge  lagoon
environments.  Eggs of parasitic  species  of
nematodes and cestodes known to be resistant to
conventional sludge stabilization will be seeded
in sludges before and after mesophilic anaerobic
and aerobic digestion.
  Studies on the  uses of sludge  for non-food
chain crops produced a final^eport on "Effects of
Sludge Irrigation on Three Pacific Northwest For-
est Soils," a grant project with Seattle, Wash-
ington. The results showed that liquid sludge (1
to 3 percent solids) applied at optimum rates of
20 to 30 metric-tons/hectar/year (Mt/ha/yr) (dry
solid basis) was beneficial for growth of existing
forest stands in a coniferous forest and will not
cause  environmental  problems. Peer Con-
sultants, Inc. is seeking the most feasible non-
food chain crops for sludge  use. The most prom-
ising non-food chain crops and crop categories
for sewage sludge use application appear to be:
    1. Monoculture timber tract operations
    2. Forest nurseries
    3. Horticulture specialties
    4. "New" crops such as Jojoba, Guayule,
      and Eurphorbia.
  Cotton is also being evaluated, though the use
of cottonseed oil and meal is being eliminated
because it is a food chain crop. A 3-year grant to
the Ohio Agricultural Research and Development
Center will "Demonstrate the Feasibility of Using
Sludge to Produce a Valuable  Non-Food Chain
Crop." The purpose of the study is to elucidate
the effects of digested sludge on:
    (a) container-produced conifer and hard-
       wood trees in the greenhouse
    (b) conventional nursery production of for-
       est tree seedlings
    (c) mycorrhizal fungi (which are important in
       tree nourishment)
    (d) plantation production of Christmas trees.
  A four-year survey of the background  con-
centrations of selected trace elements in the prin-
cipal soils and crops of major food chain crop-
producing areas of the United  States is being
conducted under a cooperative agreement with
the U.S. Department of Agriculture and the Food
and Drug Administration.
RELATED RESEARCH PUBLICATIONS

 1. Bingham, FT, R.J. Mahler, and G. Sposito. EFFECTS OF IRRIGATION WATER COMPOSITION ON
   EXCHANGEABLE SODIUM STATUS OF A FIELD SOIL So/7 Science 127:248-252, 1979.
 2. Hyde, H.C., A.L. Page, FT. Bingham, and R.J. Mahler. EFFECT OF HEAVY METALS IN SLUDGE ON
   AGRICULTURAL CROPS. Journal of Water Pollution Control Federation 51:2475-2486, 1979.
 3. Kienholz, FW., G.M. Ward, D.E. Johnson, J. Baxton, G. Braude, and G. Stern. METROPOLITAN
   DENVER SEWAGE SLUDGE FED TO  FEEDLOT STEERS. Journal Animal Science 48(4):735-741,
   1979.
 4. Kraemar, D.F, J.B. Lucas, H.R. Pahren, J.A. Ryan, and N.E. Kowal. CADMIUM TOXICITY. The Lancet
   1979:1242.
 5. Mahler, R.J.,  FT Bingham, A.L  Page, and J.A. Ryan. COMPOSITION OF CROPS  GROWN ON
   SLUDGE-AMENDED SOILS. Agronomy Abstracts 1979, p. 33.
 6. Ryan, J.A.,  and J.B. Lucas. THE  CADMIUM CONNECTION: FACT OR FANTASY. Agronomy Ab-
   stracts 1979, p. 37.
 7. Ryan, J.A., L.D. Grant, J.B. Lucas, R.E. Marland, H.R. Pahren, W.A. Galke, and D.J. Ehreth. CADMIUM
   HEALTH EFFECTS; IMPLICATIONS FOR ENVIRONMENTAL REGULATIONS. July 1979. (To be
   published.)
                                                                                     33

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 8. Wall, H.O., and J.B. Farrell. PARTICULATE EMISSIONS FROM MUNICIPAL WASTEWATER SLUDGE
   INCINERATORS. In: Proceedings of Mid-Atlantic States Section, Semi-Annual Technical Con-
   ference on Air Quality Impact of Ocean Disposal Alternatives, Air Pollution Control Association,
   Newark, New Jersey, April 27,1979.
 9. Wall, H.O., and R. Olexsey. COMBINED INCINERATION OF  SOLID WASTES AND MUNICIPAL
   WASTEWATER SLUDGE. Department of Energy Conference on Water and Wastewater Manage-
   ment, New Orleans, Louisiana, December 10-13,1979.
10. REVIEW OF TECHNIQUES OF TREATMENT AND DISPOSAL OF PHOSPHORUS LADEN CHEMICAL
   SLUDGES. SCS Engineers. EPA 600/2-79-083.
11. CHEMICAL PRIMARY SLUDGE THICKENING AND DEWATERING. Envirotech. EPA-600/2-79-055.
12. EVALUATION OF DEWATERING DEVICES FOR PRODUCING HIGH-SOLIDS SLUDGE CAKE. Blue
   Plains, District of Columbia. EPA-600/2-79-123.
13. THE CODISPOSAL OF SEWAGE SLUDGE AND REFUSE IN THE  PUROX SYSTEM. Union Carbide
   Corportion, Linde Division, Tonawanda, New York 14150. EPA-600/2-78-198.
Biological Treatment Section

  New developments in wastewater control tech-
nology for municipal applications must be evalu-
ated on a continuous basis. A large portion of the
Section's activity is thus devoted to field scale
studies  of innovative unit'processes that are
monitored under carefully defined scopes of
work. Results are published in EPA reports, tech-
nical journals, and seminars.
  Technical assistance is provided to EPA re-
gions, municipalities, and consultants on short
term projects. Committee and workshop assign-
ments are also considered  an effective way to
assist the technical community by transferring
research information rapidly into practice.

Disinfection of Wastewater

  The program on development of alternative
disinfection  technology has continued in the
areas of ozonation, ultraviolet irradiation, and
chlorine dioxide treatment.

Ozonation

  A comparison of a bubble diffuser ozone con-
tactor and a stirred turbine reactor on filtered and
unfiltered municipal effluent revealed superior
transfer efficiency and coliform reduction effi-
ciency in the bubble diffuser. Factors affecting
final coliform numbers in ozonated effluent were
total chemical oxygen demand, nitrate, total sus-
pended  solids, and the absorbed ozone dose. A
model was developed to predict final coliform
density as a function of the absorbed ozone dose.

Ultraviolet Light

  Demonstration of ultraviolet light (UV) as a via-
ble, cost-effective alternative to chlorine was suc-
cessful at Northwest Bergen County. A number of
small treatment plants have already committed
themselves to this technology as a result of the
study. Data from the project provided  sufficient
information to formulate a design theory for UV
equipment, and the theory will be tested  in a
second generation study planned in the upcom-
ing year. A thin-film design will be compared with
a thicker water wall design on a secondary stand-
ard municipal effluent.

Chlorine Dioxide

  In  a study conducted by Stanford University
personnel, chlorine dioxide was found to be
equally effective  as chlorine on a mass dose
basis, using a conventional secondary effluent.
However, on a nitrified filtered secondary
effluent, chlorine dioxide was clearly superior to
chlorine, requiring only about 20 percent of dose
to effect the same coliform reduction. Using the
same nitrified effluent but without filtration, the
two disinfectants were equally effective. Appar-
ently, one or  more critical components in the
effluent were removed by the filter.
  A commercial, field scale chlorine dioxide gen-
erator was evaluated for product yield. The gen-
eration technique was the acid  activation of
sodium chlorite. The chlorine dioxide yield was
approximately 80 percent, compared with the 90
to 95 percent  obtainable in the laboratory.  The
lower yield in the commercial unit could signifi-
cantly affect costs, because of the relatively high
cost of sodium chlorite. A complete cost evalua-
tion is being conducted, based on all data  col-
lected in the laboratory and in the field.

Pre-Conference Workshop at Houston, Texas

  The Water Pollution Control Federation Disin-
fection  Committee sponsored a state-of-the-art
workshop on  wastewater disinfection alterna-
tives. The workshop provided a forum for the
exchange of practical  information on chlorina-
tion/dechlorination, ozonation, chlorine dioxide
treatment, ultraviolet  irradiation, and bromo-
chlorination. Case  histories were also presented,
34

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as well 'as discussions on the need  for waste-
water disinfection and methods for assessing the
relative risks  and benefits  of  alternative
processes.
  Of the 10 presentations, one was made by a
MERL researcher and 4 were made by MERL
grantees. The meeting was attended by over 110
persons. The papers will be  published in  a
proceedings.

IJC Chlorine Objective Task Force

  The first  Chlorine Objective Task  Force was
formed  in 1975  by the International Joint Com-
mission to address the following issues: (1) the
technical capabilities for monitoring the pro-
posed maximum ambient concentration of total
residual chlorine of 0.002 mg/l in the boundary
waters of the Great Lakes; and (2) to  investigate
methods for achieving the proposed objective. In
1978, a second Chlorine Objective Task Force was
constituted  to assess the economic  and social
implications of achieving the chlorine objective
and to evaluate alternative disinfectants for use in
achieving the objective.  A MERL staff member
actively participated on the second Task Force in
the past year.  A  final report is being drafted and
should be available to the public early next year.

Analysis of Bio-available Phosphorus

  Control technology for limiting phosphorus in-
puts into natural waters is becoming more re-
fined. As these inputs diminish it would appear
important to measure the fraction of  total phos-
phorus that might readily stimulate the growth of
algae.
  Clarkson  College, Potsdam, New York, is ex-
perimenting with a Dual Culture Diffusion Appa-
ratus (DCDA) shown in Figure 15.
.Figure 15. Dual culture diffusion apparatus.
  The sample to be analyzed is placed in one half
of the DCDA. The other half contains a defined
algal culture. The two halves are separated by a
membrane  which allows  only soluble con-
stitutentsto interchange between the two halves.
The measured accumulation of phosphorus in
the algal portion of the apparatus yields an esti-
mate of the  bio-available phosphorus liberated
by the sample under the test conditions. Results
are being correlated to chemical tests for rapid
estimation of phosphorus bio-availability.
  Samples for analysis were obtained from a
field  survey  of four municipal treatment plants
located in the Great Lakes drainage basin.

Oxygen Transfer Standard

  A voluntary Subcommittee formed under the
American  Society of Civil  Engineers' (ASCE)
Technical Council on Codes and Standards  and
partially sponsored by EPA has  been working
since early 1978 to develop a tentative interim
oxygen standard and/or procedural manual. The
effort was initiated with a state-of-the-art work-
shop in April 1978 and will culminate in the spring
of 1980 with the completion of an interim report.
This  report will cover the Subcommittee's  rec-
ommendations on: (a) Modeling and Data Inter-
pretation,  (b) Clean Water and Unsteady State
Tests, (c) Respiring System Field Tests, (d) Alpha,
Beta, and Temperature Corrections, and (e) The
Effect of Geometry and Mixing on Scale-up. If and
when these recommendations are adopted as a
final  consensus oxygen transfer standard,  uni-
form recognized procedures will be available to
enable equitable comparative testing and data
interpretation from one test  site to another.

European Aeration Survey

  An on-site survey of second generation  fine
bubble diffuser  installations in the United King-
dom was conducted during September-Novem-
ber 1979. The survey was carried out for EPA by
the U.S. Association of Metropolitan Sewerage
Agencies (AMSA) in cooperation with the Water
Research Centre of Stevenage, England. The ob-
jectives of this project were to review, evaluate,
and document the operating  and maintenance
experiences of approximately ten treatment
plants  utilizing  fine bubble ceramic dome dif-
fuser systems arrayed in total floor coverage pat-
terns. Emphasis was placed on collecting data
related to headloss buildup and diffuser clogging
rates, associated diffuser cleaning  techniques,
preferred diffuser and blower design configura-
tions, operating power consumption, and proc-
ess performance. These data will be compared to
the minimal information available on similar sys-
                                                                                      35

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terns in the United States and also with coarse
bubble diffuser operational data and costs for
publication in 1980.
Full-Scale Aeration Evaluation

  Three types of fine bubble submerged air aera-
tion  systems will be evaluated  over a 2-year
period in full-scale aeration trains of the Los
Angeles  County Sanitation Districts' (LACSD)
Whittier Narrows Plant. The three systems se-
lected are ceramic dome diffusers, plastic tube
diffusers, and jet aerators. The  selection  was
based on the results of earlier clean water un-
steady state oxygen transfer tests conducted by
LACSD on  various aeration systems including
both fine and coarse bubble devices. The data to
be generated in the second phase field study are
divided into three categories: (a) long-term dif-
fuser headless  and maintenance studies in
mixed liquor, (b) oxygen transfer under respiring
biological environmental conditions, and (c)
process performance as a function of organic
load. System design is underway with startup
scheduled for the spring of 1980.

Deep Shaft Project Underway

  The first municipal Deep Shaft pilot demon-
stration system in the United States started up in
October 1979 at Ithaca, New York. The Deep Shaft
process was originally conceived and developed
in the United  Kingdom  and later refined in  Can-
ada where several systems are now operational.
The unique features of Deep Shaft are the use of
flotation to achieve final clarification and the in-
jection of air  to drive mixed liquor circuitously
through a U-tube to create a vertical activated
sludge reactor. In addition to savings in land and
reactor volume, claimed advantages of the proc-
ess include reduced power consumption, re-
duced excess sludge production, and the crea-
tion of a concentrated waste sludge that does not
require separate thickening priorto handling and
disposal. The Ithaca shaft is 18 in. (0.5 m) in diam-
eter by 435 ft (133 m) deep and has a  design
capacity  of 200,000 gpd (757 m3/day/m2) at  a
nominal detention time of 38 minutes. Operating
and performance data will be collected  over  a
planned 16-month experimental program which
will terminate in Match 1981.

ABF Project Nearing Completion

  A 15-month assessment of Helena, Montana's
existing activated bio-filter (ABF) system will be
completed by the end of February 1980. This proj-
ect represents the first full-scale comprehensive
evaluation of a municipal ABF facility operating
at or near the manufacturer's full recommended
design organic and hydraulic loadings. These de-
sign loadings are 200 Ib BOD5/day/1000 ft3 (3.2 kg/
day/m3) on the first-stage redwood  bio-filter and
45 minutes of nominal detention time in the sec-
ond-stage aeration tank. By removing various
segments of the secondary treatment  facility
from service, an experimental program has been
carried out which examined: (a) both the  bio-
filter and the aeration tank at approximately half
design load - Phase I, (b) the bio-filter at approx-
imately full design load and the aeration tank at
approximately half design load - Phase II, and (c)
both the  bio-filter and the aeration tank at ap-
           TABLE 8. OPERATIONAL & PERFORMANCE SUMMARY OF ABF PROJECTS*
        Parameter
                                                   Phase I
                     Phase II
Phase III
Dates

Duration (weeks)
Flow(mgd)**
Final Eff. BOD5 (mg/l)
Plant BOD5 Removal (%)
Final Eff. SS (mg/l)
Plant SS Removal (%)
Bio-filter Organic Loading
(Ib BODs/day/IOOft3)***
Nominal Aeration Time (min)
12/1/78-
2/22/79
12
3.67
15
91
10
92
91
110
2/23/79-
7/12/79
20
3.75
21
86
24
86
184
104
8/13/79-
9/13/79
6 (partial)
3.48
26
84
27
85
177
56
  * Project summary through September 1979
 **1 mgd = 3785 m3/day
***1 lb/day/1000 ft3 = 0.016 kg/day/m3
 36

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proximately full design load - Phase III. Phases I   screened raw wastewater and extended aeration
and II are over, and as expected, the ABF system   plant effluent used as system feed. Influent flow
performed satisfactorily. Effluent quality for   was alternated on a daily basis between the two
Phase III  is more than meeting a 30/30 BOD5/   first-stage filter trenches to allow for a period of
suspended solids standard after the first 6 weeks,   drying and stabilization of the organic matter
with the critical 1979-80 winter months still to go.   trapped on and in the filter.
                                              Although  substantial nitrification was ob-
T    , .  _      „    */•>   / *  w             served, insufficient overall nutrient removal  oc-
Troph,c System Project Completed             curred t() justjfy uti|ization of the MP, system in a
  An evaluation of the Max Planck Institute (MPI)   tertiary treatment mode. As a secondary treat-
system has been completed at the  Moulton   ment  option receiving raw wastewater feed,
Niguel (California) Water District. The  MPI sys-  Moulton Niguel's system was able to consistently
tern consists first of two filter trenches filled with   meet the Federal 30/30 BOD5/suspended solids
three layers of gravel (15 cm of 5 cm gravel over-  standard with hydraulic loadings of  15,000-
lain by 30 cm of 2 cm gravel overlain by 71/2 cm of   25,000 gpd (57-95 m3/day). Some form of effluent
pea gravel) topped with a 71/2 cm layer of sand in   disinfection would  be required where a bacte-
which the reed Phragmites is planted and actively  riological standard was imposed. Although addi-
growing. Perforated plastic pipe at the bottom of  tional research would be beneficial in the areas of
the filter trenches transport first-stage effluent to   plant harvesting and filtered sludge removal, the
a single  second-stage polishing elimination   MPI system offers the small community a low-
trench filled with gravel and  planted with   energy treatment alternative with minimal me-
bulrushes. Studies were conducted with both   chanical maintenance needs.

RELATED RESEARCH PUBLICATIONS

 1. Barth, E.F., and R.L Bunch. BIODEGRADATION AND TREATABILITY OF POLLUTANTS. Municipal
   Environmental Research Laboratory, Cincinnati, Ohio 45268. EPA-600/9-79-034, October 1979.
 2.  Hais, A.B., and A.D.  Venosa. EPA  OVERVIEW OF MUNICIPAL WASTEWATER DISINFECTION.
   Journal for Water Pollution Control Federation 50 (11): 2470-2476. Also presented at the Water
    Pollution Control Federation Annual Conference, Philadelphia, Pennsylvania, September 2-7,1977.
 3.  Middlebrooks, E.J., C.H. Middlebrooks, B.A. Johnson, J.L.  Wright, J.H. Reynolds, and A.D.
    Venosa. MPN AND MF COLIFORM CONCENTRATIONS IN LAGOON EFFLUENTS. Journal for Water
    Pollution Control Federation 50 (11): 2530-2547.
 4.  Venosa, A. D. WASTEWATER DISINFECTION ALTERNATIVES. Presented at the 42nd Annual Con-
    ference of the Indiana Water  Pollution Control Association,  November 7, 1978, Indianapolis,
    Indiana.
 5.  Venosa, A.D. PROGRESS IN WASTEWATER DISINFECTION. Presented before the Sanitary Engi-
    neering Institute, University of Wisconsin-Extension, Madison, Wisconsin, March 1-2,1979.
 6  Venosa, A.D., E.J. Opatken and  M.C.  Meckes. COMPARISON OF OZONE  CONTACTORS FOR
    MUNICIPAL WASTEWATER EFFLUENT DISINFECTION: PACKED COLUMN VERSUS JET SCRUB-
    BERS. EPA 600/2-79-098. In press.
 7.  Venosa, A.D., ed. PROGRESS IN WASTEWATER DISINFECTION TECHNOLOGY. Proceedings of the
    National Symposium, Cincinnati, Ohio, September 18-20,1978. EPA 600/9-79-018, June 1979.
 8.  Venosa, A.D. WASTEWATER  DISINFECTION: ISSUES AND ANSWERS. Presented  at the New
    England Water Pollution Control Association 50th Anniversary Meeting, June 17-20,1979, Newcas-
    tle, New Hampshire.
 9.  Venosa, A.D. OZONE DISINFECTION: STATE-OF-THE-ART. Presented at the Water Pollution Control
    Federation Pre-Conference Workshop on Wastewater Disinfection, October 7,1979. Proceedings to
    be published.
10. Venosa, A.D., M.C. Meckes, E.J. Opatken, and J.W.  Evans. DISINFECTION OF FILTERED AND
    UNFILTERED SECONDARY EFFLUENT IN TWO OZONE CONTACTOR. Presented at the Water
    Pollution Control  Federation Annual Conference, Houston, Texas,  October 8-11, 1979 and to be
    submitted for publication in the Journal for Water Pollution Control Federation.
11. Reid, G.W. and L Streebin. PERFORMANCE EVALUATION OF EXISTING AERATED LAGOON SYS-
   TEM AT BIXBY, OKLAHOMA. University of Oklahoma, Norman, Oklahoma 73019. EPA-600/2-79-
   014, March 1979.
12.  O'Brien, W.J., and R.E. McKinney. REMOVAL OF LAGOON EFFLUENT SUSPENDED SOLIDS BY A
    SLOW-ROCK FILTER. University of Kansas, Lawrence, Kansas 66045. EPA-600/2-79-011, June 1979.

                                                                                    37

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13. Gurnham, C.F, B.A. Rose, and W.T. Fetherston. PERFORMANCE EVALUATION OF THE EXISTING
   THREE-LAGOON WASTEWATER TREATMENT PLANT AT PAWNEE, ILLINOIS. Gurnham and Asso-
   ciates, Inc., Chicago, Illinois 60606, July 1979.
14. PROCEEDINGS: PERFORMANCE AND UPGRADING OF WASTEWATER STABILIZATION PONDS.
   Edited by E. Joe Middlebrooks and Donna H. Falkenborg, Utah State University, Logan, Utah 84322
   and Ronald F Lewis, U.S. Environmental Protection Agency, Cincinnati, Ohio 45268. EPA-600/9-79-
   011, May 1979.
15. FULL-SCALE DEMONSTRATION OF OPEN TANK OXYGEN ACTIVATED SLUDGE TREATMENT.
   Edited by Stephen R. Pearlman, Metropolitan Denver Sewage Disposal District No. 1, Denver,
   Colorado  80229 and Donald G.  Fullerton, FMC Corporation, Englewood, Colorado 80110.
   EPA-600/2-79-012, May 1979.
16. Nash, N., W.B. Pressman, and RJ. Krasnoff. OXYGEN AERATION AT NEWTOWN CREEK. Environ-
   mental Protection Administration, The City of New York, New York 10007. EPA-600/2-79-013, June
   1979.
17. PROCEEDINGS: WORKSHOP TOWARD AN OXYGEN TRANSFER STANDARD. Edited by William C.
   Boyle, University of Wisconsin, Madison, Wisconsin 53706. EPA-600/9-78-021, April 1979.
18. Drnevich, R.F. BIOLOGICAL-CHEMICAL PROCESS FOR  REMOVING PHOSPHORUS AT
   RENO/SPARK, NEVADA. Union Carbide Corp., Tonawanda, New York 14150. EPA-600/2-79-007,
   February 1979.
19. Johnson, B.A., J.L. Wight, D.S. Bowles, J.H. Reynolds, and E.J. Middlebrooks. WASTE STABILIZA-
   TION  LAGOON MICROORGANISM REMOVAL EFFICIENCY AND EFFLUENT DISINFECTION WITH
   CHLORINE. Utah State University, Logan, Utah 84322. EPA-600/2-79-018, July 1979.
 Physical-Chemical Treatment Section

  During the past two years, the emphasis of the
 Section has been shifted from research on physi-
 cal-chemical treatment processes to investiga-
 tions of toxic or hazardous compounds, organic
 and inorganic, in wastewaters. Thus research re-
 sults will  be presented both on physical-chemical
 studies which were completed  during the year
 and preliminary results just now becoming avail-
 able on toxics research.

 Physical-Chemical Process Research

  A report is available on the operation of a series
 of physical - chemical systems, during the period
 from June 1975 to January 1978, located at Rose-
 mount, Minnesota. During the demonstration
 period, the facility treated an average flow  of
 approximately 0.25 mgd (946 m3/day) by a treat-
 ment system consisting of chemical clarification,
 filtration, carbon adsorption and ammonia re-
 moval by clinoptilolite. Both the activated carbon
 and the ammonia ion-exchange media were re-
 generated on-site.  Performance data are sum-
 marized according to five process flow schemes.
 Cost data developed from this small demonstra-
 tion were used to estimate the cost of operation
 and maintenance of a 10 mgd  (38,000 m3/day)
 facility. The study demonstrated that despite con-
 siderable fluctuations in raw wastewater influent,
 the treatment efficiency did not vary significantly
 in terms of percent removal which during the
 two-year period averaged 93 percent for BOD, 99
 percent for suspended solids and 94 percent for
phosphorus. Formation of sulfide was encoun-
tered when the carbon contactors were operated
in a downflow mode, but the study showed that
this problem could be controlled by addition of
sodium nitrate and by daily backwashing of the
columns. The capital and operating cost of a 10
mgd (38,000 m3/day) facility similar to the dem-
onstration system was estimated to range from
$0.56 to $0.83 per 1000 gal (3.785 m3).
  The study showed that a physical-chemical
system is fully capable of producing consistently
not only a high quality effluent in terms of BOD
and suspended solids but also an effluent low in
both ammonia nitrogen and phosphorus. The
cost of this system compares favorably with the
cost of biological systems producing an effluent
of equal quality.
  In another report, the operation of a 5 mgd
(19,000 m3/day) physical-chemical tertiary plant
at Piscataway, Maryland, is  described. Effluent
from an activated sludge  plant was treated by
lime, precipitation either single- or two-stage -
followed  by  dual media filtration and activated
carbon. Significantly, the single-stage  lime treat-
ment produced results similar to the  two-stage
system but at approximately one-half the dose of
lime. Lime was recovered by calcination in a mul-
tiple-hearth furnace, while the combustion gases
were used for recarbonation.
  The carbon system consisted of three parallel
trains of two columns, each column providing 18
minutes of empty bed contact at a hydraulic load-
ing of 6.5 gpm/sq ft (265 l/min m2). Carbon was
regenerated  in a  multiple hearth furnace. Three
 38

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regenerations of the carbon were accomplished
during the project period. Because of difficulties
in obtaining accurate measurements of carbon,
only estimates of carbon losses incurred during
transfer and regeneration  could  be  obtained,
which were 8-10 percent per regeneration cycle.
  The operation and evaluation of this full-scale
tertiary system - biological treatment followed
by a physical-chemical series of processes -
demonstrated that a very high quality of effluent
is produced which  is suitable for a  variety of
reuse purposes.
  Granular media filtration  is considered  to be
one of the most important tertiary processes for
plants to meet the  requirements of  minimum
monthly average effluent quality of 30 mg/l for
suspended solids and BOD, established by the
Environmental  Protection Agency in  1973. The
filters are  particularly useful for small plants, 5
mgd (19,000 m3/day). A report has been prepared
on a study of the clarification efficiency of eight
full-scale tertiary granular media filters. The re-
sults of this study are described in more  detail
elsewhere in this progress report underthe head-
ing "Tertiary Wastewater Treatment."

Toxics Control

  More recent activities of the Section  have been
concerned with toxics in publicly owned waste-
water treatment plants. Studies initiated during
the past one to one and one-half years are only
now beginning to produce results for the several
objectives of the program. The first objective is
the development of a data base on the occur-
rence and concentration of priority pollutants en-
tering the Nation's wastewater treatment plants.
Three studies were funded for this objective, with
only preliminary data available at this time.
  A second objective in the  research on toxics is
the determination of thetreatability/removability
of priority pollutants (Figure 16). Pure compound
research to  determine treatability  is being con-
ducted on phenomena such as activated carbon
adsorption, biodegradability, volatility  and ozone
oxidation. This research is being supplemented
by pilot-scale studies to determine removability
by treatment systems. Initial  pilot plant studies
will investigate removals  obtained by con-
ventional  activated  sludge  systems.  Mass bal-
ance  calculations, obtained  from analyses of
influent, effluent, sludges and air emissions, will
indicate the predominant  mechanisms of re-
moval; volatility, biodegradation or sorption on
the sludge. It is likely that all these mechanisms
of removal, plus others such as precipitation, hy-
drolysis, etc., will be involved.
  A third major objective is evaluation of  modi-
Figure 16. Modification of chemical extraction
           of priority pollutants.
fications to conventional processes for the en-
hanced removal  of toxics. One  of the more
promising  approaches  is the  addition of
powdered carbon to a biological reactor. The
study will include, besides carbon, other solid
additives such as chars and powdered coal.
  A major benefit that will be derived  from the
above investigations, is the development of ana-
lytical procedures for trace organics and metals
in such "difficult"  media as raw wastewater and
sludges. Without this analytical methodology, re-
search on the priority pollutants would be se-
verely hampered.
  One of the major studies on development of
data bases is a survey of 25 cities for all priority
pollutants in a variety of treatment plants located
throughout the country. This study is being coor-
dinated with and will be complemented by a 40-
city survey  being conducted by  the  Office of
Water and Waste Management  in Washington.
Thus, sampling  a total  of 65 cities located
throughout the country and representing a wide
variety of treatment processes and influent com-
                                                                                        39

-------
 position (industrial/municipal waste mixture) will
 provide an ample data base for the occurrence
 and removal of the priority pollutants in POTW's.
  Some very early results show that some 61
 priority pollutants have been found in waste-
 water influents; comprising 31 base/neutrals, 21
 volatile and 9 phenolic compounds. Removals
 are highly variable, 16 to 99 percent, not unex-
 pected considering the great diversity of chemi-
 cal compounds on the list. Early evidence also
 shows substantial accumulation of compounds
 in the sludges, particularly the substituted ben-

 RELATED RESEARCH PUBLICATIONS
 zenes such  as methyl- ethyl- and chloro-
 benzenes. While the lower molecular weight
 phthalates were removed, probably by biological
 degradation, the higher molecular weight com-
 pounds, such as bis(2-ethylhexyl)  and
 butylbenzylphthalates tended to accumulate in
 the sludge, presumably because of their lesser
 biodegradability and greater sorption on sludge.
  Within the next  year much will be learned
 about the presence and behavior of priority pol-
 lutants in municipal wastewaters as the results of
 these studies unfold.
 1.  Cohen, J.M. PILOT PLANT INVESTIGATIONS ON PHYSICAL-CHEMICAL TREATMENT. Proceedings
    of Second Assises Internationales de /'Environment, Paris, France, December 5-6, 1978.
 2.  Cohen, J.M. OBSERVATIONS ON PHYSICAL-CHEMICAL TREATMENT IN THE USA. Proceedings of
    Second Assises Internationales tie /'Environment, Paris, France, December 5-6, 1978.
 3.  Cohen, J.M. TREATABILITY/REMOVABILITY OF TOXICS FROM WASTEWATERS. Briefing for Dr.
    Stephen Gage, Assistant Administrator for Research and  Development, U.S.E.P.A., Washington,
    D.C., June 1979.
 4.  Westrick, J.J. and M.D. Cummins. COLLECTION OF AUTOMATIC COMPOSITE SAMPLES WITHOUT
    ATMOSPHERIC EXPOSURE. Journal of Water Pollution Control Federation, In Press (1979).
 5.  O'Farrell, T.R and R.A. Menke.  OPERATIONAL RESULTS FOR THE PISCATAWAY MODEL 5 MGD
    AWT PLANT. EPA-600/2-78-172, September 1978.
 6.  Polta, R.C., et al. EVALUATION OF PHYSICAL-CHEMICAL TREATMENT AT ROSEMOUNT. Metro-
    politan Waste Control Commission, St. Paul, Minnesota 55101. EPA-600/2-78-201, December 1978.
 7.  FitzPatrick, J.A. and C.L. Swanson. EVALUATION OF FULL-SCALE TERTIARY WASTEWATER FIL-
    TERS.  Northwestern University, Evanston, Illinois 60201. To be published.
 8.  Fochtman, E.G. and W. Eisenberg. TREATABILITY OF CARCINOGENIC AND OTHER HAZARDOUS
    ORGANIC COMPOUNDS. NT Researh Institute, Chicago, Illinois 60616. EPA-600/2-79-097 (August
    1979).
 9.  Fochtman, E.G., W. Eisenberg, and R.A. Dobbs. OZONE OXIDATION OF CHEMICAL CARCINOGENS
    IN AQUEOUS SOLUTION. Fourth  World Congress on Ozone Technology, Houston, Texas, Novem-
    ber 27-29, 1979.
TECHNOLOGY DEVELOPMENT
SUPPORT BRANCH

  The Technology Development Support Branch
provides  technical and support services to the
Division.  It operates and maintains pilot plants
and provides analytical services to all Division
technology development operations. It is com-
posed of  the Pilot and Field Evaluation Section
and the  Waste Identification and Analysis
Section.

Pilot and  Field Evaluation Section

  The Pilot and Field Evaluation  Section is re-
sponsible for conducting most of the WRD pilot
plant studies. These are conducted with U.S. EPA
personnel at the Test  and Evaluation Facility in
Cincinnati, Ohio and under contract with the Los
Angeles County Sanitation Districts, Los Angeles
County, California. In addition, personnel of this
Section manage the national program in Instru-
mentation and Automation for Wastewater Treat-
ment Systems. Some of the instrumentation and
automation work is conducted at the pilot plant
facilities mentioned above, but most is imple-
mented through contracts and grants.
  During this year construction of the new Cin-
cinnati Test and  Evaluation  Facility was com-
pleted. This facility  provides over 30,000 square
feet of experimental, pilot  plant, laboratory  and
office space. It was designed to serve as a multi-
purpose facility for environmental technology re-
search, and will  be the main site of MERL pilot
plant studies (Figure 17). The MERL projects se-
lected for the Test and Evaluation Facility are:
    1) A determination of the fate of the organic
      substances on  the  priority  pollutant list
      once they gain entrance into the munici-
      pal wastewater collection  system. The
      major objective is to determine the sinks
40

-------
Figure 17. The U.S. Environmental Protection
           Agency Test and Evaluation Facility
           in Cincinnati, Ohio.

      for those substances which are not bio-
      degraded, and the degree of removal of
      priority pollutants which can be expected
      prior to the discharge of wastewater to the
      environment.
    2) An evaluation of the effect of adding sani-
      tary landfill leachate to municipal waste-
      water. The purpose of  this  study is to
      determine if it is feasible to treat leachate
      by putting it into the municipal collection
      system. A primary concern is the potential
      for activated sludge upsets caused by
      leachate.
    3) A comparative evaluation of several types
      of Ozone Contactors. The major purpose
      of this is to develop mass transfer kinetic
      data on various types of ozone sewage
      contactors. These data can then be used
      by engineers and  regulatory officials to
      reach cost effective decisions on the use
      of ozone for disinfection of sewage.
    4) A comparative evaluation of sludge de-
      watering equipment. The purpose  of this
      study  is to develop information on the
      performance of pilot scale  dewatering
      equipment such as vacuum  filters, vari-
      ous types of centrifuges, and various
      types of belt pressure filters in parallel on
      the same types of sludges.
  Provisions have been made in this facility for
cooperative projects with the other Cincinnati
EPA Laboratories, and to allow for  quick re-
sponse to special needs of the regions and oper-
ating programs.  Development  of one  or  more
cooperative  projects  is anticipated  in the next
year.
  Under the contract with the Los Angeles
County Sanitation Districts three projects were
completed in the past year. An evaluation of a
rotary kiln for regeneration of granular activated
carbon was conducted. It was found to achieve
the same results as a multiple hearth furnace at
about the same cost. The rotary kiln has a lower
capital cost but higher operational expense. An
evaluation of dechlorination with sulfur dioxide
indicated that state-of-the-art control  systems
can function adequately to automate the system
provided the chlorine  residual probe is
periodically exposed to some residual chlorine. If
it is not, it loses its sensitivity to a chlorine re-
sidual. Shortly after dechlorination conforms re-
appear in the effluent. It was found that this was
not regrowth but rather an infestation from natu-
rally  occuring coliforms  in the air and soil. The
third study involved test tank evaluation of vari-
ous generic types of aeration equipment. It was
found that 2 types of fine  bubble diffusers had
markedly  superior oxygen transfer capability.
These will be tested in LACSD treatment plants to
determine if clogging occurs and  the  actual
power savings potential.
  The Lebanon Pilot Plant  was closed this year
coincident with the Test  and Evaluation Facility
opening. Prior to the close some short studies on
anaerobic digestion were completed. In one of
these powdered activated carbon was added to
anaerobic digestion systems. Contrary to claims
reported by others it had  no positive effect on
process performance over the detention time
range of 30 days to 5 days. A second study evalu-
ated  the kinetics of volatile acid production in
anaerobic digestion. These data  will allow con-
struction of a new time dependent model of this
process. The model will be used in computer
simulation optimization studies.

Automation and Instrumentation Program

  The basic  purpose of  this program is to de-
velop and demonstrate automation and  instru-
mentation which will improve performance and
economics of wastewater treatment plants. The
foundation of the program  is fostering the use of
reliable cost effective instruments. Because field
surveys have often indicated customer dissatis-
faction with the performance and reliability of
many instruments, an instrument certification
program  has been initiated. One aspect  of this
certification program is development of pro-
tocols for instrument testing  and certification.
These are being developed for various types of
flow measurement devices and selected chemi-
cal analysis instruments under an IAG with the
National Bureau of Standards. The protocols will
address:  evaluation of manufacturers specifica-
tions for adequacy in the application of the instru-
ment to  the  wastewater area, bench test pro-
                                                                                       41

-------
cedures, maintenance procedures, and field
evaluation procedures. The protocol for venturi
type flow measurement devices will  be pub-
lished in the early part of 1980. These protocols
will enable professionals  in this field to make
rational judgements on purchase specifications
and acceptance tests for instrumentation.
  A second objective of this program is to pro-
mote the establishment of a certification center
or laboratory at which instrument testing can be
conducted. The protocols developed under the
NBS program described above would be utilized
by this testing center. Such a center would pre-
clude the need for individual organizations to test
instruments and would thus serve as a center of
information on environmental instrumentation.
Public Technology Incorporated completed a pre-
liminary feasibility study of such a center. They
recommend  that it be set up as a private non-
profit  organization which tests instruments and
makes its results available only to its members.
Instrument manufacturers could have  their  in-
struments tested for a fee but could not be mem-
bers. A "cooperative  agreement" is now being
considered for the next stage which will involve
detailed planning of the organizational structure,
staffing, physical facilities and cost evaluations.
  Another major area of concern is the elucida-
tion, implementation and demonstration of pro-
cess control  strategies. Under a  grant with  the
Metropolitan Waste Control Commission of Min-
neapolis-St.  Paul, automation of  sludge con-
ditioning, vacuum filtration and  incineration is
being  tested. During this year all of the instru-
mentation and computer  programming neces-
sary to control the latter two devices was
completed. In addition a correlation  between
sludge specific resistance and pH, ORP and shear
stress was developed. These.parameters can be
monitored on-line. Thus as sludge characteristics
change, the dose of chemical conditions can be
automatically changed to maintain an acceptable
rate of sludge filtration. During the coming year
the overall automated sludge handling system
will be tested in parallel with a manually operated
system to ascertain cost effectiveness.
  A third major area of effort is in the technology
transfer area. During this year an automation and
instrumentation Design Handbook for Activated
Sludge Treatment Plants was completed. This
document is  intended to serve as a guideline for
design engineers and regulatory officials who
became involved in the design and/or review of
automation and instrumentation of wastewater
treatment systems. It includes a description of
control strategies now being utilized in the field,
and detailed instrumentation diagrams for  im-
 plementing these. The strategies addressed are
 not only those for the activated sludge reactor
 and its sedimentation tank but for all of the liquid
 and sludge handling processes at a conventional
 treatment plant. Also included in this document
 are sections on control theory,  generic types of
 instruments, cost analysis and computer sys-
 tems. The Office of Water Programs has tenta-
 tively approved this document for use in review
 of designs for construction grant funding. During
 the next year a technology transfer seminar
 based on this document will be developed.

 Waste Identification and Analysis Section

 Analytical Support

  Modern computerized equipment is used to
 provide accurate analyses of a wide variety of
 pollutants and to handle the increasingly large
 sample load. Analyses include heavy metals, al-
 gal nutrients, total  and suspended solids and
 gross organics in wastewaters and sludges (Fig-
 ure 18).
Figure  18.  Heavy metals analysis using atomic
           adsorption.

  The several analytical procedures have been
developed  to support the analytical needs of
WRD. The most recent development was the ad-
aptation of  the COD test to an automated, com-
puterized autoanalyzer, which provides a  more
rapid output of COD analyses and quality control
data not  readily available  with manual
procedure.
  The protocol developed for the analysis of
organics in  sludges has been used to analyze a
42

-------
 number of sludges generated by the Physical-
 Chemical Treatment Section. These sludges were
 a result of a treatability/removability study which
 involved eight of the volatile and non-volatile pri-
 ority pollutants.
  The Computer Services and Systems Division,
 in conjunction with contractors, is preparing a
 sample file control system to be added to our
 computerized laboratory system. The sample file
 control will provide us with a more systematized,
 rapid a"nd  efficient way of keeping records of the
 workload and backlog, and  of providing final re-
 ports for the  requestors. The sample file control
 will also provide better quality control through
 the preparation of control charts and  statistical
 data on recoveries,  standard deviation, etc.
 MERL is serving as one of several model systems
 to demonstrate the utility of sample file control
 for the entire Agency.

 Development of Procedures for
 Municipal Sludges

  Several  procedures for the  determination of
 organics in municipal sludges continue to be
 evaluated. A  "unified" procedure involving ex-
 traction and centrifugation  followed by a chro-
 matographic clean-up, and a modified  Bellar
 technique for the volatiles was tested for the anal-
 ysis of PCB's, pesticides and the volatile materials
 in sludges (Figures 19-21).
 Figure 20.  Priority pollutant extract clean-up
            using liquid chromatography.
Figure 19.  Continuous  extraction of organic
           priority pollutants.
Figure 21. Gas chromatograph/mass spectro-
           meter analysis  of  organic priority
           pollutants.
                                                                                       43

-------
  The two alternatives, of base/neutral and acid
extractions or acid/neutral and base extractions
followed by gel permeation and silica gel chro-
matography clean-up procedures have been par-
tially successful with sludges but are unsatisfac-
tory for the analysis of all the priority pollutants,
particularly some of the phenols. Additional
steps such as "base" wash of the acid extract and
steam distillation have been  tried but are still not
satisfactory for all of the phenols.
concentration exceeded 500 g/l. The presence of
this compound in the leachate was confirmed by
the Laboratory  in Region 2 and investigation
showed it to be present in the surface waters in
the surrounding  area.
  Analysis  of the Cincinnati  sample revealed
fewer of the priority pollutants  and in smaller
concentrations.
Landfill Leachate Analyses
  Samples of leachates from a landfill in Cincin-
nati and the LiPari landfill in Glassboro, New
Jersey, were analyzed using modification of the
sludge analysis procedures on behalf of the Solid
and Hazardous Waste Research Division. Results
showed the presence of a number of priority pol-
lutants, particularly various phenols and phthal-
ates. One of the most significant contaminants
found in the  LiPari samples was bis(2-chlo-
roethyl) ether. It is extremely carcinogenic and its
Future Support

  The Finnigan GC/MS System Model 4023 con-
tains the latest Incos data system and will en-
hance our present capabilities considerably. The
new capabilities will allow us to have three sys-
tems operating simultaneously, both analyzing
and/or interpreting the data. This should increase
our capacity to provide the Division and the T&E
Facility with critical organic analytical services
needed for toxic studies.
RELATED RESEARCH PUBLICATIONS

 1. Bishop, C.F METHODS DEVELOPMENT FOR SLUDGE ANALYSIS IN PUBLICLY-OWNED TREAT-
   MENT WORKS. \n: Proceedings of the Effluent Guidelines Division's Seminar "Analytical Methods
   for Priority Pollutants," March 8-9,1979, Norfolk, Virginia.
 2. Caragay, A.B. and RL. Levins. EVALUTION OF PROTOCOLS FOR PESTICIDES AND PCB'S IN RAW
   WASTEWATER. EPA-600/3-79-166, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
   100 pp.
 3. Cummins, M.D., I.J. Kugelman, A.L Petrasek, J.F Roesler and W.W. Schuk. ANNUAL REVIEW OF
   THE LITERATURE FOR INSTRUMENTATION AND AUTOMATION OF WASTEWATER COLLECTION
   AND TREATMENT SYSTEMS. Journal Water Pollution Control Federation, 51(6):1294-1301,1979.
 4. Heidman, J.A.  SEQUENTIAL NITRIFICATION-DENITRIFICATION IN  A PLUG-FLOW ACTIVATED
   SLUDGE SYSTEM. Final Report — Contract No. 68-03-0349. In press.
 5. Kugelman, I.J., M.D. Cummins, W.W. Schuk and J.F Roesler. PROGRESS IN INSTRUMENTATION
   AND AUTOMATION. In: Proceedings of the Sixth U.S.IJapan Conference on Sewage Treatment
   Technology, Cincinnati, Ohio, October 1978. In press.
 6. Manning, A.W. and D. Dobbs. DESIGN HANDBOOK FOR AUTOMATION OF ACTIVATED SLUDGE
   TREATMENT PLANTS. Final Report — Contract No. 68-03-2573. In press.
 7. Pellizzari, E.D. and L Little. COLLECTION AND ANALYSIS OF PURGEABLE ORGANICS EMITTED
   FROM WASTEWATER TREATMENT PLANTS. Final Report — Contract No. 68-03-2681. In press.
 8. Polta, R.C. and D.A. Stulc. AUTOMATIC SLUDGE BLANKET CONTROL IN AN OPERATING GRAVITY
   THICKENER. Interim Report — Grant No. S803602. In press.
 9. Rodriguez, C.F, W.A. McMahon and R.E. Thomas. METHOD DEVELOPMENT FOR DETERMINA-
   TION  OF POLYCHLORINATED HYDROCARBONS IN MUNICIPAL SLUDGE. Interim Report —Con-
   tract No. 68-03-2606. In press.
10. Skrentner, R.G., A.W. Manning and I.J. Kugelman. DESIGN  APPROACH FOR AUTOMATION OF
   ACTIVATED SLUDGE TREATMENT PLANTS. In: Proceedings Instrument Society of America An-
   nual Meeting, October 1979.
11. Warner, J.S., G.A. Jungclaus, RM. Engel, R.M. Riggins and C.C. Chuang. ANALYTICAL PRO-
   CEDURES FOR  DETERMINING ORGANIC PRIORITY POLLUTANTS IN MUNICIPAL SLUDGES. Final
   Report — Contract No. 68-03-2624. In press.
44

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SYSTEMS AND ENGINEERING
EVALUATION BRANCH

  The  Systems  and Engineering  Evaluation
Branch is composed of the Urban Systems Man-
agement Section, the Storm  and Combined
Sewer Section, and the Systems and Economic
Analysis Section. Its programs include the study
of methods for improving the design and opera-
tion of publicly owned treatment works and for
developing approaches to controlling urban wet
weather discharges. The Branch is also respon-
sible for providing design  methods for rural,
institutional and individual home systems for
conducting a program for water conservation
and wastewater reuse.

Municipal Wastewater Reuse and
Water Conservation

  The objectives of the Reuse and Conservation
Program are the: (1) implementation of research
that proves the feasibility of the near term, less
controversial, nonpotable use of wastewater to
extend valuable water supplies by source sub-
stitution, and the longer term, or possible emer-
gency use of wastewater for potable purposes;
and (2) the development of data on the advan-
tages and disadvantages of water conservation
so that individuals and communities can make
informed decisions on implementing programs
for their own specific situations. The Wastewater
Research Division (WRD) is supporting projects
in both of these areas and is  coordinating  its
activities with the EPA Health and Drinking Water
Programs, and with other concerned Federal,
State  and municipal organizations  engaged in
similar research. A cooperative agreement with
the American Water Works Research Foundation
(AWWARF) provides for dissemination  and ex-
change of information among  participating re-
use oriented organizations.
  In order to assess the impact of unplanned
potable reuse  on water  supplies, the Office of
Drinking Water is using the results of a WRD
project whose purpose was to determine the
quantity of wastewater present  in surface water
supplies of U.S. cities of over 25,000 population.
Twenty cities with-a total population  of over
seven million were determined to have surface
supplies containing from 2.3 percent to  16 per-
cent wastewater during average flow conditions
and from 8 percent to 350 percent during low
flow conditions.
  To assist implemention of reuse opportunities
involving the use of reclaimed wastewater for
direct recharge of groundwater reservoirs that
have been depleted by years of over-pumping.
Phase 1 of a project using  injection of treated
wastewater has been completed at Water Factory
21 in Orange County, California, and a new study
involving several methods of recharge has been
undertaken on Long Island, New York at facilities
of the Nassau County Department of Public
Works.  Continuous operation and detailed
monitoring programs at Water Factory 21 have
demonstrated the reliability  of advanced waste-
water treatment to remove trace contaminants.
Data necessary to evaluate the effectiveness of
these treatment technologies  to remove  mate-
rials of public health concern is being collected to
show that reclaimed wastewater is a viable and
safe source of water for groundwater recharge.
  Reuse of wastewater for potable purposes has
received National attention as an alternative in
selected areas for providing an additional source
of water to  meet expanding water demand.
However, many health questions concerning the
safety of these waters for  use in domestic pur-
poses need answers. As a result of Congressional
action, Section 1444(a)(2) of RL. 93-523, the Safe
Drinking Water Act, authorized the establishment
of a program to demonstrate the reuse of waste-
water for drinking purposes. A $7 million project
with the Denver Water Department was initiated
as part of this program and will take advantage of
most recent advances in treatment technology
and includes the most complete health effects
program  ever considered  in relation to reuse.
This phase of the program  is scheduled  to be
completed in 1988. In addition, a $4 million, five
year program has been initiated and will comple-
ment the Denver project by taking advantage of
existing municipal treatment facilities producing
high quality water to provide more near-term in-
formation on the feasibility for potable  reuse of
systems less sophisticated (no reverse osmosis)
than the system  planned for Denver. The pro-
gram will include a thorough evaluation of the
treatment effectiveness and system depen-
dability at several sites having: (1) different geo-
graphical characteristics;  (2) different  climatic
conditions; (3) different institutional constraints;
and, (4)  different treatment processes. Health
effects studies are anticipated and, beca'use of
the shorter time frame for projects  in this pro-
gram compared to the Denver project, they are
expected to provide useful input to the design of
the Denver analytical and health effects program.
  If water conservation is to warrant national em-
phasis as cited in President Carter's water policy
message of June 1978,  measurements, in eco-
nomic terms, are needed on its relative merits.
Results of a  project with the State of California
Department of Water Resources designed  to
                                                                                     45

-------
evaluate the  impacts of water conservation
practices implemented during the 1976 to 1977
drought on wastewater collection and treatment
facilities show no significant adverse effect on
these facilities and indicate expected savings in

RELATED RESEARCH PUBLICATIONS
capital costs at a 30 percent reduction in indoor
water use. Also, data collected on treatment plant
effluent quality indicated the impact of water
conservation on wastewater reclamation was not
significant.
 1.  English, J.N. RECLAMATION AND REUSE OF WASTEWATER AND URBAN RUNOFF Water Con-
    servation and Alternative Water Supplies. Proceedings of Southeast Regional Conference, Novem-
    ber 8-9,1978, pg. 185-207, Georgia Institute of Technology.
 2.  Swayne, M.D., et al. WASTEWATER IN RECEIVING WATERS AT WATER SUPPLY ABSTRACTION
    POINTS. EPA Report 1979.
 3.  Sproul, O.J. CRITICAL REVIEW OF VIRUS  REMOVAL BY COAGULATION PROCESSES AND pH
    MODIFICATIONS. EPA Report 1979.
Urban Systems Management Section

Treatment Plant Operation and Design

  The expansion in program activities during
1979 is evidenced by the change in program title
from Operation and Maintenance (O&M) to Treat-
ment Plant Operation and Design Program. Sig-
nificant progress has been made in improving
POTW performance and reliability, reducing con-
struction and operating costs of municipal collec-
tion and treatment systems, encouraging energy
conservation in plant designs and operation, and
providing data and specific support to the
Agency's  operating programs and enforcement
activities.
  The Treatment Plant Operation and Design Pro-
gram provides improved design information in
the form of specific design  guidelines based on
comprehensive cost, engineering analysis, per-
formance and operational studies of existing
POTW's as well as emerging treatment processes
and techniques. Design manuals and guidance
information are developed and  specific con-
densed guidance and checklists are provided to
improve the state and federal review process
with respect to design, plant start-up, operation,
plant trouble-shooting and evaluation tech-
niques. Specific studies identify and  document
improved  process operation and improved unit
process and system designs incorporating cost
effective, reliable technology.
  The detailed  findings of the National O&M
Cause and Effect Survey have provided the action
impetus for decision  makers who have made
proper plant operation and design their priority
concern. The 31/2 year study that was conducted
nationwide identified and ranked the specific fac-
tors causing poor plant performance and de-
veloped and implemented an approach, called a
Composite Correction Program (CCP), to improve
 plant performance and move it toward
 compliance.
  Because of the success achieved with the CCP
 this approach to improving compliance levels of
 municipal plants is being demonstrated by the
 State of Colorado on a statewide basis. The ob-
 jectives of this areawide application of the CCP in
 the State's enforcement programs are to docu-
 ment the cost effectiveness and management
 feasibility of the CCP approach to improving per-
 formance on a statewide basis, increase levels of
 compliance, evaluate the integration of private
 sector technical expertise and state assistance in
 the  implementation of  a cost effective com-
 pliance/enforcement program, and provide guid-
 ance in the development of a state level com-
 pliance and enforcement strategy incorporating
 the CCP approach.
  Recognizing that proper plant performance is
 the critical element in assuring POTW continuing
 compliance a methodology for conducting com-
 prehensive  plant  performance evaluations  has
 been developed. The protocol responds to the
 expressed requirements of the Office of Enforce-
 ment and Regional Offices in compliance enfor-
 cement activities and will assist the Regional
 Offices and States that may need to prescribe
 interim O&M requirements prior to and during
 major upgrading of existing facilities. The eval-
 uation methodology is applicable to a wide range
 of plant sizes and types of attached growth  and
 suspended growth biological systems. Specific
 detailed  guidance is  given for all phases of the
 plant evaluation from  initial  plant contact
 through presentation of findings and report
 preparation. The  procedural recommendations
 have been  developed and prepared as a user
 oriented analysis protocol and field manual
 which will be used by EPA, State or contract in-
 vestigators who visit plants and submit reports. It
 46

-------
contains instructional descriptions and direc-
tions for use including all necessary graphs, fig-
ures, tables, forms, and checklists required.
  Design of municipal wastewater treatment pro-
cesses has been further emphasized during 1979.
The major focus on design has been the develop-
ment of the Design Information and Guidelines
Series. This Series is a Wastewater Research Divi-
sion effort, in conjunction with other Agency pro-
grams, to provide clear, concise, and up-to-date
guidance for process design. The guidelines are
intended to include the  latest most widely ac-
cepted design practice and the most current re-
search  results from all old programs. The
Treatment Plant Operation and Design Program
has taken the lead role in planning and managing
the guidelines development program and for de-
veloping the format  and  content of each
guideline to be published.

Improving Plant Performance and Design

  During 1979 many research projects have been
initiated that are directly related to process de-
sign. A study of design deficiencies has defined
1,700 instances on which correction modules will
be developed for both new designs and existing
facilities. The impact  of peak flows on process
performance has been recognized and a project
funded  to  determine the importance of peak
flows for process design. The potential for perfor-
mance problems in Rotating Biological  Contactor
(RBC) facilities which reach  their  design flows
has been recognized. This has led to a research
project to study RBC performance and  design.
Performance data and present design criteria at
26 operating RBC plants will be evaluated at de-
sign flow and changes in design procedures rec-
ommended if necessary. The continuing indict-
ment of in-plant sidestream flows  as  major
causes of poor plant performance has led  to a
study of the impact of these flows on mainstream
process performance. This project includes the
characterization of 23 separate sidestreams and
the development of operational procedures and
design guidance to minimize the impact of side-
streams.
  Comprehensive dye tracer studies on eight
common types of secondary clarifiers have re-
vealed the complex  phenomenon controlling
clarifier performance. Although all of the phe-
nomenon have not been quantified, it is obvious
that factors in addition to surface area and weir
length are  important. Internal  physical factors
such as size, shape, inlet  configuration  and
sludge removal mechanism have been found to
impact clarifier performance. However, there are
external factors, such as flow balancing between
parallel units and the duration and frequency of
peak flows, that may have a greater impact than
the internal factors.
  O&M costs represent a major commitment that
municipalities must make in the future if they are
to protect their investment in wastewater treat-
ment facilties. Cost data have been collected in
the past, but it has been too general in nature to
be of any assistance in the management of plant
operations. In cooperation with the Drinking
Water Research Division a study has been funded
to develop a cost analyses system where both
water and wastewater utilities can  track their
O&M costs. This cost analysis system will be a
useful management tool to determine, if possi-
ble, reduction in O&M costs are possible.
  Reliability projects continue to make progress.
A study of the impact of toxic organics on acti-
vated sludge process reliability  is determining
what concentration of toxic organics can be re-
ceived by the process before overall performance
is affected. Data on the reliability of mechanical
components has been  collected and  analysis of
this data  is proceeding. From these  results, re-
liability design guidelines will be  developed
which will incorporate reliability concepts into
the design and operation of municipal facilities.

Improving Plant and Systems Management

  The Wastewater Treatment  Process  Com-
puterized Data Base, containing extensive data
on over 300 facilities, is operational.  Data from
the 1978 Needs Survey is being incorporated so
that  information on national trends in waste-
water treatment technology can be  developed.
Customized reporting and  plotting programs are
being developed by the WRD staff as information
requests on the data base  are received.
  Research in instrumentation and automation
has concentrated on development of  new or ver-
ification of existing control strategies for the acti-
vated sludge process and selected sludge hand-
ling  stabilization techniques. These areas are
most important because of the large expendi-
tures scheduled for these  processes under the
construction grant regulations. Emphasis has
been placed on  demonstration of the control
strategy concept, and deliniation of improve-
ments in process performance and/or process
cost  effectiveness. For  the activated sludge pro-
cess emphasis has been placed on strategies in-
volving dissolved oxygen level control, and
instantaneous food-to-microorganisms ratio
control (F/M). The major recent effort was to pro-
duce a design handbook which could be used to
aid engineers in designing the most cost effective
systems. This  recently published manual dis-
                                                                                      47

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 cusses the various activated sludge modifica-
 tions, aeration methods, equipment and applica-
 tion techniques, compressors and blowers, D.O.
 control  methods,  and presents an economic
 analysis of manual versus automatic D.O. con-
 trol. Under automatic D.O. control power savings
 of over 10 percent were achieved as well as im-
 provements in BOD removals.
  Studies of centralized managment of waste
 treatment plants are investigating potential O&M
 cost reduction  and improved performance
 through  changes in  operational modes, re-
 sources allocation, administrative procedures,
 and institutional structures. Specific functions
 which may be impacted include the following:
 performance monitoring and control, preventive
 and emergency maintenance,  laboratory analy-
 sis, training, personnel administration, account-
 ing, purchasing, billing, spare parts control,
 regulatory reporting and liaison.
  For each function, a variety of centralized ap-
 proaches are possible. Studies are defining these
 alternatives and estimating the relative changes
 in costs and plant performance. Initial emphasis
 has been  placed upon changes in operational
 control, including evaluation of remote telemetry,
 automated monitoring, microprocessors, and
 various circuit rider schemes.

 Small Flows

  Implementation of the Clean  Water Act
 Amendments of  1977  (PL 95-217) has directed
 considerable attention to the continuing efforts
 of the Small flows Research  Program.
  The impact of the 1977 Clean Water Act on
 program  activities  has been: reassessing of re-
 search priorities and objectives to meet the im-
 mediate  needs  of engineers,  planners, and
 regulatory authorities;  providing technical assis-
 tance to a diverse array of people involved with
 small scale technologies for wastewater treat-
 ment and disposal; and instituting a series of
 seven Technology Transfer design seminars
 across the country on rural wastewater treatment
 alternatives.
  The Small Flows Research Program has three
 main objectives. These include: (1) improved,
 cost-effective methods of planning, design, con-
 struction and management for small community
wastewater systems; (2) evaluation of alternative
technologies, with respect to performance, costs,
 applicability and  limitations, and environmental
 impacts; and (3)  development of new concepts
for waste utilization, recycling, treatment and dis-
 posal which are  commensurate with society's
goals in the 21st Century.
  In past  years  the majority of program re-
 sources has been  devoted to the evaluation of
 alternative technology for small communities.
 Ongoing efforts in this area include studies of
 composting toilet and graywater system perfor-
 mance and public health risks through a grant to
 the California Water Resources Control Board. A
 continuing grant to the Oregon Department of
 Environmental  Quality which is providing data
 on a variety of alternative on-site wastewater sys-
 tems has produced several  designs which  are
 performing well in the field and  has  provided
 information on some less successful  alterna-
 tives. A study which documents the costs, perfor-
 mance and success of several alternative black-
 water systems installed in Appalachia six to eight
 years earlier has been completed. Of the seven
 alternatives installed, those systems employing
 conventional toilets and septic tanks followed by
 soil absorption or sand filters were found to have
 performed best, while recycling and incinerating
 toilets were generally unsuccessful due to high
 operation and maintenance requirements which
 often resulted in abandonment by the users.
  Two studies of septic tank pumpings (septage)
 disposal at wastewater treatment plants were
 completed by the University of Lowell. The first
 documented the effects of receiving this waste in
 the plant mainstream on primary clarifiers and
 on biological processes without primary clar-
 ifiers. As  a result, the  recommended septage
 loading for extended aeration plants with suffi-
 cient aeration capacity is as follows:
       % Design
   Wastewater Loading

          25
          50
          75
         100
Recommended Continuous
      (% Volume)
	Septage Load	

         3
         2
         1
         0
  Slug loads are permissable, but at one-half the
rate shown above. The second study showed that
septage could not be vacuum filtered, even with
chemical  conditioning. However, mixtures of 20
percent to 50 percent septage with thickened
waste activated  sludge, preconditioned  with
alum, iron or acid, were amendable to vaccuum
filtration.  The cost of handling septage directly in
the sludge stream of a small wastewater treat-
ment facility appears to be lower than the main-
stream addition. Three other studies have been
completed on septage management by compost-
ing, anaerobic digestion, and a variety of other
systems based on a nationwide survey.
  Other continuing studies include the demon-
stration of improved construction techniques for
soil absorption systems  at the University of
48

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Wisconsin, a study of the cost competitiveness of
innovative household evaporation systems, and
a desktop study of the costs,  performance and
applicability of alternative on-site technologies.
  State-of-the-art reports  on pressure and vac-
uum sewers have been developed, and numer-
ous  demonstration projects  have been  com-
pleted that deal with these technologies. Re-
cently, a project was completed that was de-
signed to collect data on cost, performance,
operation and maintenance requirements, and
type of treatment provided for a number of pres-
sure sewer installations in operation across the
country.  Another  project has been completed
which documents the performance of a small
physical-chemical treatment plant with nitrifica-
tion in packed towers.
  In  response to the needs  of the EPA Con-
struction Grants Program several  studies have
been undertaken to  improve the grants process
as it applies to small communities. A project has
been completed which offers guidance to facility
planners (Step 1)  on how to develop the most
cost-effective wastewater management for small
(<3,500 population) communities. Another con-
tinuing project is developing a manual of on-site
alternative systems for this application. A grant
with Pennsylvania State University is attempting
to quantify the value of water conservation sys-
tems in restoring to proper operation failing soil
absorption systems.  Desktop  analyses indicate
that this approach may be the most cost-effective
retrofitting alternative for many cases.
  The 1977  Clean Water  Act stipulates that a
"management district" or other public body must
guarantee proper operation of individual sys-
tems for them to be grant eligible. In response,
the Small Flows Research  Program has an ongo-
ing research contract which will include detailed
case studies of existing  on-site management
practices and policies at the local and state levels.
An analysis will be made of the appropriateness,
effectiveness, and costs of alternative manage-
ment approaches under different local situations.
Recommendations will be outlined for selection
and implementation of management structures
and techniques.
  For future years,  rt  is anticipated that, while
basic research will  continue  to be supported,
more emphasis will be placed upon providing
improved means of applying low-technology, de-
centralized alternatives which are viable, cost-
effective approaches to ensuring environmen-
tally sound  waste management practices for
rural and suburban communities.
Innovative and Alternative Technology
innovative and alternative (I/A) technology was to
be promulgated by the EPA through the Con-
struction Grants Program. Several positive incen-
tives, including  increased grant assistance, are
provided to municipalities which adopt solutions
to their wastewater and other waste treatment
needs that conserve or recover energy, reclaim or
reuse water,  recycle wastewater constituents,
eliminate surface discharge, or lower total an-
nual costs. The significance of I/A technology is
reflected in the projection that one out of every
four Fiscal Year  1981 grant dollars will  involve
such technology. Program Operations Memoran-
dum (POM) 79-3 established four important pro-
gram support activities within the Agency for I/A
technology, of which one, the Technical Support
Group (TSG), was located in MERL. The functions
of the TSG are primarily to coordinate the  I/A
program as a central point of contact providing
technical assistance to the regional offices and to
ensure that technical information on I/A projects
is properly disseminated nationwide through the
Innovative  and  Alternative  Technology
Clearinghouse.
  Approximately thirty  proposed Innovative or
Alternative Projects with accompanying facility
plans have been reviewed by the TSG with rec-
ommendations  submitted to the Regional Ad-
ministrator through the Municipal Construction
Division Director. The number of projects to  be
reviewed for potential I/A funding have steadily
increased with time, and the TSG is now receiv-
ing two or three applications per week for review.
It is expected that these activities will continue to
increase with  time.
  In addition to formal  application reviews, the
TSG consults with the Regional  I/A Coordinators
and the regional ad hoc review groups  on a
frequent basis  regarding  details of  technical
analyses  on I/A provisions  and eligibility
determinations.
  A draft I/A Technology Manual was prepared
and disseminated earlier in the year, and was
revised based on comments submitted from all
interested sources. A significant resource com-
mitment was required to develop the draft man-
ual. Not only the TSG staff, but other members of
the Urban Systems Management Section, the
Wastewater Research Division, and the R. S. Kerr
Environmental Research Laboratory contributed
significantly to this effort. The manual contains a
users guide, I/A screening methodology, cost and
energy effectiveness criteria and guidance pro-
cedures, as well as 123 two-page fact sheets con-
taining costs, energy, performance, design and
other pertinent data.
  The Clean Water Act of 1977 clearly stated that    The purpose of the Innovative and Alternative
                                                                                      49

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Technology Clearinghouse (IATC) is to insure that   technologies.
technical and other information regarding I/A    An I/A Technology public information brochure
projects is collected and analyzed with  results   was developed and is being published. A Tech-
appropriately disseminated. The I/A project in-   nology Transfer I/A Program was developed, and
formation is  collected from EPA Regional Office   these two-day seminars were provided to each of
submittals of I/A technology and application   ten EPA regions. In addition, ten two-day semi-
clearinghouse records. The data sheets which   nars/workshops were provided for federal  and
are submitted are processed through a com-   state facility plan reviewing officials at ten other
puterized system, and the summary report is dis-   locations around the country. Additional presen-
tributed to the Regional Administrators through   tations have been made for several national and
EPA Headquarters on a quarterly basis. The  Re-   statewide organizations.
gional Offices distribute copies to the appropri-    The future trends of the I/A technology  pro-
ate State agencies and other interest groups.      gram at MERL are to become more active in  pro-
  Data which is collected and summarized in-   moting I/A technology, to monitor and document
eludes project and set-aside fund status on a   the performance of the I/A systems constructed
State and Regional basis, project classification   under the new Construction Grant regulations, to
according to  qualifying criteria, and certain addi-   more actively disseminate I/A technology infor-
tional technical information when appropriate,   mation, and to periodically review and transform
The Clearinghouse Report also contains  project   to design guidelines the more successful tech-
descriptions  and other relevant information  ex-   nologies, starting with improved  sludge hand-
tracted from the Clearinghouse forms describing   ling and energy savings concepts.
pending and  approved innovative and alternative

RELATED RESEARCH PUBLICATIONS

 1.  Segall, B.A.,  C.R. Ott, and W. Moeller. MONITORING SEPTAGE ADDITION TO WASTEWATER
    TREATMENT PLANTS — VOLUME I: ADDITION TO THE LIQUID STREAM. EPA-600/2-79-132, U.S.
    Environmental Protection Agency, Cincinnati, Ohio, 1979.
 2.  Bennett,  E.R. SEWAGE DISPOSAL  BY EVAPORATION-TRANSPIRATION. EPA-600/2-78-163,  U.S.
    Environmental Protection Agency, Cincinnati, Ohio, 1978.
 3.  Condren, A.J. PILOT SCALE  EVALUATIONS OF SEPTAGE TREATMENT  ALTERNATIVES.
    EPA-600/2-78-164, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1978.
 4.  Heidman, J.A. SEQUENTIAL NITRIFICATION — DENITRIFICATION IN A PLUG FLOW ACTIVATED
    SLUDGE  SYSTEM.  EPA-600/2-79-157, U.S.  Environmental Protection Agency,  Cincinnati, Ohio,
    1979.
 5.  Evans, EL. III. SUMMARY OF NATIONAL OPERATIONAL AND MAINTENANCE CAUSE AND EFFECT
    SURVEY.  Technology Transfer Newsletter, U.S. Environmental Protection Agency, Cincinnati,
    Ohio, July 1979.
 6.  Bender, J.H. THE OXIDATION  DITCH PROCESS: SUPERIOR PERFORMANCE AND RELIABILITY AT
    LOW COST. EPA Environmental News Brief, U.S. Environmental Protection Agency, January 1979.
 7.  Gray, A.C., RE. Paul and H.D. Roberts. EVALUATION OF OPERATION AND MAINTENANCE  FAC-
    TORS LIMITING BIOLOGICAL WASTEWATER TREATMENT PLANT PERFORMANCE. EPA-600/2-79-
    078, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
 8.  Hegg, B.A., K.L Rakness and J.R. Schultz.  EVALUATION OF OPERATION AND MAINTENANCE
    FACTORS LIMITING MUNICIPAL WASTEWATER TREATMENT PLANT PERFORMANCE.
    EPA-600/2-79-034, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
 9.  Hegg, B.A., K.L. Rakness and J.R. Schultz. A DEMONSTRATED APPROACH  FOR IMPROVING
    PERFORMANCE AND  RELIABILITY  OF BIOLOGICAL WASTEWATER TREATMENT PLANTS.
    EPA-600/2-79-035, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
10.  Harber, A.F and R.C. Bain. NOVEL METHODS AND MATERIALS OF CONSTRUCTION. EPA-600/2-79-
    079, U.S.  Environmental Protection Agency, Cincinnati, Ohio, 1979.
11.  Ongerth,  J.E. EVALUATION OF FLOW EQUALIZATION IN MUNICIPAL WASTEWATER TREATMENT.
    EPA-600/2-79-096, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
12.  COMPUTER-AIDED SYNTHESIS OF WASTEWATER TREATMENT AND SLUDGE DISPOSAL SYS-
    TEMS. L.A. Rossman, ed. EPA-600/2-79-158, U.S. Environmental Protection Agency, Cincinnati,
    Ohio, 1979.
13.  INNOVATIVE AND ALTERNATIVE TECHNOLOGY ASSESSMENT MANUAL (DRAFT). J.M. Smith, ed.
    EPA-430/9-78-009, MCD 53, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.

50

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 Storm and Combined Sewer Section

   Control and/or treatment of storm sewer dis-
 charges and combined sewer overflows (CSO's)
 are major problems in the field of water quality
 management. Every time it rains, in the majority
 of the oldest and largest cities, tremendous vol-
 umes of mixed pollution laden urban runoff and
 raw sewage (CSO) spill into and contaminate re-
 ceiving waters. Another problem area during wet
 weather exists due to man's land development
 activities which have initiated severe, highly un-
 desirable, and damaging alterations in the natu-
 ral sedimentation cycle, particularly in local
 areas, by drastically accelerating the erosion-
 sedimentation process. Over the past decade
 much research effort has been expended and a
 large amount of information has been generated,
 primarily through the Storm and Combined
 Sewer Section (SCSS).
   Storm and Combined Sewer research and de-
 velopment effort has been directed to abatement
 of pollution loads from CSO. The technology that
 has been developed for CSO control  in many
 cases has almost direct and complete application
 for the  control of urban stormwater from sepa-
 rate storm drainage systems as well as aspects of
 sedimentation control.
   There has been increased realization that,
 along with technology development, there is a
 need  to better define the actual  effects of wet-
 weather discharges on receiving waters. Results
 from  work in this area are currently being evalu-
 ated.  Also, because of the  high  capital cost of
 treatment methods, there is an increased effort
 being undertaken to consider other approaches
 that have much lower capital cost. These include
 management practices such as improved street
 sweeping and flushing of sewers during dry
 weather to reduce the amount of sediment that
 would otherwise be removed by the next storm.

 Treatment and Control

   Due to adverse and intense flow conditions and
 unpredictable shock loading effects, it has been
 difficult to adapt existing treatment methods to
 storm-generated overflows, especially the micro-
 organism-dependent biological processes.  The
 new physical/chemical treatment techniques
 have shown more promise in overcoming these
 adversities. To reduce capital investments, pro-
 jects have been directed towards high-rate opera-
 tions approaching maximum loading boundaries
 by using the swirl,  microstrainer,  high rate filter,
 and dissolved air flotation processes. These pro-
 cesses,  or combinations of these processes, can
•be adjunct to the existing sanitary plant or serve
 as remote satellite facilities at the outfall and
 the SCS Program recommends their acceptance
 in  the  201  and Innovative/Alternative (I/A)
 Programs.
   Major work in this area during 1979 include
 pilot demonstrations of the SALA-Magnetics
 high gradient magnetic separator which were
 conducted on combined sewer overflow and raw
 sewage in the Boston area. These tests built on
 the data from the first phase lab-scale project,
 with special emphasis on specific design and op-
 erational  parameters, long-term durability and
 maintenance problems, and system adaptability
 to  integrated wet and dry weather flow  condi-
 tions. Results showed the effectiveness of mag-
 netic filters for the dual treatment of CSO and raw
 sewage. At 90 gpm/ft2, suspended solid (SS) re-
 movals approach 95 percent. A grant  proposal
 from the Detroit Water and Sewer District for the
 full-scale demonstration of a 1 mgd high gradient
 magnetic  separator is currently being prepared.
 The SCSS is planning to ride piggy-back on the
 project with anticipated funding from the Region
 V108 Program.
  A demonstration project in Boston will evalu-
 ate the swirl, helical bend and Teacup  solids
 concentrators.

 Source  Control and Low Structural Cost
 Approaches

  Nonstructural and low structurally intensive al-
 ternatives, termed best management practices
 (BMPs), offer considerable promise as the first
 line of action to control urban runoff pollution. By
 treating the problem at its source, or through
 appropriate legislation curtailing its opportunity
 to develop, multiple benefits can be  derived.
 These include  lower cost, earlier results, and
 an  improved  and  cleaner neighborhood
 environment.
  The greatest difficulty faced by BMPs is that the
action-impact relationship is almost totally un-
quantified. It is clear that onsite storage, for ex-
ample, can be closely related to reduced down-
stream conduit  requirements but the net  water
quality benefits are far less defined. Similarly,
cleaner streets and neighborhoods and enforced
legislation will eradicate gross pollution sources
butto what limit should they be applied and who
will bear the cost? The final answers of cost effec-
tiveness will not be found  short of trial imple-
mentation. Key  demonstration projects in this
regard are ongoing this year. At Bellevue, Wash-
ington, and Orlando, Florida cost-effectiveness
of various  BMPs will be evaluated. Austin, Texas
has been chosen to demonstrate various types of
porous pavements to evaluate their effectiveness
                                                                                      57

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in the control of both flooding and pollution from
urban stormwater runoff.
  Other significant BMP demonstration projects
have been ongoing throughout the year and have
yielded  important results. A study at San Jose,
California has developed sampling procedures to
test street cleaning equipment performance in
real-world conditions. The street cleaning equip-
ment test showed that different test area condi-
tions affected performance more than dif-
ferences in equipment type.
  In  Rochester, New York, the SCS Program is
providing technical advisors to Region II and to
the Great Lakes Program on a combined sewer
overflow project which will evaluate along with
other minimal  structural improvements an over-
all BMP  program that  includes sewer  mainte-
nance, catchbasin cleaning and street sweeping
practices.
  Another BMP project funded in the San Fran-
cisco area will investgate the treatment of storm-
water runoff in a saltwater marsh.  Evaluation will
include water, sedment and biological conditions
and the  preparation of a manual on best vegeta-
tive control practices.
  An investigation of periodic sewer flushing
during dry weather for first flush relief has
recently been completed  in Boston, Mas-
sachusetts. A set of generalized procedures for
estimating pollutant loadings associated with
dry weather sewage solids deposition in com-
bined sewer systems has been prepared to
provide planners, engineers, and municipal man-
agers with technical information so that they can
make intelligent informed decisions on potential
sewer flushing programs  in combination with
other combined sewer management controls.

Collection System Controls

  Collection system control pertains to manage-
ment alternatives for wastewater interception
and transport.  These include sewer separation;
improved  maintenance  and design  of
catchbasins, sewers, regulators and tide gates;
and remote  flow  monitoring and control.  The
emphasis, with the exception of  sewer  separa-
tion, is on optimum use of existing facilities and
fully automated control. Because added use of
the existing  system is employed, the concepts
generally involve cost-effective, low-structurally
intensive control.
  The Program state-of-the-art and manual of
practice  on infiltration/inflow (I/I) identified a sig-
nificant problem which led to national emphasis
on I/I control and fruitful  countermeasure  re-
search. This year  Program developments have
included detection methodology and instrumen-
tation; improved materials and improved in-
stallation, construction and rehabilitation tech-
niques. Three new user's manuals including a
product and equipment guide are available.
  It is estimated that over 90,000 miles of new
sewage collection pipe, at a cost of approx-
imately $17 billion will be required nationally by
1990. Obviously, even a minor decrease in sewer
construction related costs could result in a sig-
nificant savings in the overall EPA construction
grants  program and other  construction
programs.
  In San Antonio, Texas a project evaluated the
strength increases, corrosion resistance and re-
sulting infiltration prevention from sulfur im-
pregnation of concrete pipe. Since pipe costs are
significant, an increase in strength could lead to a
decrease  in pipe materials and construction
costs. A final report is at press. Additionally, the
benefits of impregnation as related to I/I reduc-
tion will be of major significance to the 201 pro-
grams (in lowering treatment and control costs).
  The recent withdrawal of AM-9 grout by Amer-
ican Cyanamid has left the I/I rehabilitation pro-
gram without a reliable product capable of being
used with available equipment. Accordingly,
there is an urgent need to assess the potential of
products for use as sewer sealants. (Several
products are currently available which  have been
identified as being of possible use.)
  Last year the Office of Water Program Opera-
tions (OWPO) requested assistance from the SCS
Program in identifying substitutes for  AM-9. Ac-
cordingly, the Program entered a project to sat-
isfy this objective. This project will also concen-
trate on field testing potential grouting materials
along with possible equipment redevelopment
work.
  As a result of this project in  conducting the
current grouting assessment, the 3M  Company
has invested $500K on the development of a suit-
able replacement for AM-9 which can  be utilized
in existing equipment. This new material is an
elastomeric  hydrophilic polymer known as
CR250. Preliminary field tests yielded excellent
results.  In-house toxicity tests indicated  that
CR250 is safe and exhibits  no evidence of the
neurotoxic characteristics of AM-9 (acrylamide
grout).
  Two new demonstration projects in coopera-
tion with Regions III and V were started this year
to determine the feasibility of relining deterio-
rated  sewers with the new  Insituform process.
The process involves the use of a flexible polyes-
ter tubing inserted into a damaged sewer via an
existing manhole. After hardening, a  new pipe-
within-a-pipe is formed. The basic advantages
52

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are that it does not require expensive and disrup-
tive excavation and it takes the form of a struc-
turally sound pipe.
  In the City of Hagerstown, Maryland an ORD
funded evaluation will be made on 7,700 feet of
Insituform lining funded by construction grants.
A similar evaluation is being performed in North-
brook, Illinois.
Receiving Water Impacts

  Data on the environmental impacts of urban
runoff are being gathered  as a first step in de-
veloping methodology to quantify pollutant
stress and evaluate the impact in relation to re-
ceiving water standards and desired uses. Ongo-
ing SCS Program projects as well as case studies
of documented receiving water impacts are
being reviewed and characterized in a project
with the University of Florida. The project is ex-
pected to help identify the types  of impacts re-
quiring further verification and the research
needed to quantify receiving water stresses.
  A nationwide survey of dissolved oxygen
meters indicated that large  dissolved oxygen de-
creases in streams following storms over urban
areas are not found in the majority of cases. The
greatest effect is found in streams where the dis-
solved oxygen is  already somewhat depressed
from dry weather discharges. One river showing
a measurable effect  in dissolved oxygen  from
urban  runoff is the Scioto below Columbus,
Ohio. A more detailed dissolved oxygen study of
a stretch of that river will be conducted in 1980.
The study will provide data for verification of
oxygen balance models.
  A sediment transport model has been adapted
to urban runoff  particulates  and  has been
checked approximately with solids data from the
Cuyahoga River. Furtherverification of the model
might be carried out on the Scioto River.

Systems and Economic Analysis Section

  This group carries out a wide variety of mathe-
matical and statistical analyses  in support of
other efforts within MERL.
  Total phosphorus loading from municipal
wastewater treatment plants to the Great Lakes
was estimated together with the cost of alterna-
tive treatment strategies for the International
Joint Commission (IJC). The IJC list of plants
greater than 1.0 mgd numbered 325 plants for all
the Great Lakes and 199 plants for  Lakes Erie and
Ontario. The plant size distribution was fit with a
log-normal  probability density function to esti-
mate the number of plants in any size range be-
low 1.0 mgd. The total number of plants was 974
for all the Great Lakes and 645 for Lakes Erie and
Ontario. Total plant flow was 4258 mgd for all the
great Lakes and 3085 mgd for Lakes  Erie and
Ontario. Treatment alternatives considered were
(1) chemical addition in all plants greater than 1.0
mgd, (2) chemical addition in plants between 0.1
and 1.0 mgd,  (3) doubling the settlers and in-
creasing the chemical dose by 10 percent in all
plants greater than 1.0 mgd, (4) dual media filtra-
tion in plants greater than 1.0 mgd, and (5) PHO-
STRIP process in plants greater than  1.0 mgd.
Assumed  effluent quality was 1.0 mg/l P for
chemical addition, 0.75 mg/l  P for doubling the
settlers, and 0.5  mg/l P for dual media  filtration
following chemical addition. The PHO-STRIP pro-
cess was found to be competitive with chemical
addition in the larger plant sizes when the influ-
ent  phosphorus concentration was relatively
great, but for the 5.8 mg/l P influent phosphorus
assumed for present conditions the cost advan-
tage never exceeded 20  percent. Thus, PHO-
STRIP was not included in any of the treatment
strategies  studied. Chemical addition in plants
greater than 1.0  mgd was found to be the most
cost-effective alternative at a unit cost  of about
$0.90/lb P  removed. Doubling the settlers in
plants greater than 1.0 mgd and  adding chemi-
cals in plants between 0.1 and  1.0 mgd were
about equivalent in cost at about $3.5/lb P re-
moved. The most expensive alternative was  dual
media filtration at about $7.8/lb P removed. Ap-
plying combinations of treatment alternatives to
plants grouped by size was also considered with
a modest increase in cost-effectiveness shown.
  The windrow composting process for waste-
water treatment plant sludge has been simulated
with a time-dependent mathematical model. The
trapezoidal cross-sectional  area was divided into
rectangular and triangular areal increments (Fig-
ure 22) and the model computes the flux of air,
oxygen, water vapor, and  heat into each incre-
ment over each time interval. The pile is assumed
to be aerated  mechanically with the pressure
source at the bottom center of the pile. Although
this mode of aeration is not typical, it appears to
have a number of advantages over conventional
operation and  is  being pilot tested. Water vapor
within the pile is assumed to be saturated at the
local temperature. Water vapor and oxygen are
transported by advection and diffusion and oxy-
gen is used by the microbiological activity.  The
rate of microbiological activity is a function of the
local temperature and the  remaining con-
centration  of biodegradable organic material.
Heat transfer is by conduction and by movement
of water vapor and air. Heat lost from the boundry
with atmospheric air is by convection and by
evaporation of surface moisture. Heat transfer to

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                                                   10   11    12    13    14    15
Figure 22. Discreditization scheme for numerical integration of windrow composting performance.
the soil is by conduction. Airflow streamlines are
established first and used throughout the time-
dependent  integration. A time  increment of 15
minutes has been found to be satisfactory. Run-
ning time on the PDP-11 computer is about one
minute per day of real time. Initial runs show that
the temperature history of the pile approximates
that seen in experimental work with aerated com-
posting windrows.
  A study was undertaken to investigate the im-
plications of designing municipal treatment sys-
tems on  the basis of either cost- or energy-
effectiveness. A computer model called EXEC/OP
was used to select the least-cost and least-energy
designs for a conventional treatment system
from over 20 different unit processes that could
be arranged into almost 14,000  different config-*
urations (Figure 23). The differences in these de-
signs for variations in design flow, effluent
quality, and the price of energy was examined.
  Results showed that the gap between least-
cost and least-energy designs is reduced  as
attached  growth biological processes are sub-
stituted for  activated sludge treatment and ana-
erobic digestion with gas  recovery is employed
in sludge treatment. These changes can result in
significant energy savings at rather modest  in-
creases in cost. However, the imputed energy
cost associated with these changes (i.e., the price
of energy which would make these changes cost-
effective) can be much higher than the actual
market price. For secondary treatment levels, in-
creases in energy prices are much more influen-
tial in making digester gas recovery cost-effective
than in making changes in the most cost-effective
model of biological wastewater treatment. It was
shown how EXEC/OP could be useful in generat-
ing several noninferior system designs that offer
alternative cost-energy combinations.
  A key feature of EPA's national program  for
controlling toxic materials  discharged from
POTW's is the establishment of categorical pre-
treatment standards for industries that utilize
municipal treatment systems. Industrial pretreat-
ment standards can be relaxed to the extent that
reliable pollutant removal is provided by the
POTW. A mathematical decision model for plan-
ning cost-effective integrated industrial-munici-
pal pretreatment programs has been developed.
The model seeks to determine the degree of in-
dustrial pretreatment and  POTW treatment
needed in a sewer district so  that all POTW dis-
charge requirements can be met at minimum
cost. The basic premise which it explores is that
54

-------
PUMPING


PRELIMINARY
TREATMENT
                                 PRIMARY
                              SEDIMENTATION
                                                ACTIVATED SLUDGE
                                              (MECHANICAL AERATION)
   ACTIVATED SLUDGE
   (DIFFUSED AERATION)
                                                 TRICKLING FILTER
                                                ROTATING BIOLOGICAL
                                                    CONTACTOR
                 GRAVITY THICKENING
                       NULL
  FLOTATION THICKENING
         NULL
                 LIME STABILIZATION
                ANAEROBIC DIGESTION
                 AEROBIC DIGESTION
                  HEAT TREATMENT
                       NULL
U
                                                AEROBIC DIGESTION
        NULL
                 GRAVITY THICKENING
                    ELUTRIATION
                       NULL
                                                     NULL
                 VACUUM FILTRATION
                   CENTRIFUGATION
                    DRYING BEDS
                       NULL
      DRYING BEDS
         NULL
                     LANDFILLING
                  LAND SPREADING
                    INCINERATION
 Figure 23.  Multi-option flow diagram for conventional treatment system used in the cost- and
           energy-effectiveness study.
in some situations it may be more economical to
have the POTW assume some of the burden in
treating toxic pollutants rather than relying en-
tirely on industrial  pretreatment. The model is
currently classified as a prototype  because of
several simplifying  assumptions used in its de-
                                                                                     55

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velopment. Work is proceeding on integrating   structure and in assessing its utility as a practical
our growing understanding of the occurrence   tool for effective toxics managment.
and fate of these pollutants into the model's


RELATED RESEARCH PUBLICATIONS

 1. Allen, D.M., TREATMENT OF COMBINED SEWER OVERFLOWS BY HIGH GRADIENT MAGNETIC
   SEPARATION. EPA-600/2-78-209, December 1978.
 2. White, C.A. and A.L Franks. DEMONSTRATION OF EROSION AND SEDIMENT CONTROL TECH-
   NOLOGY- LAKE TAHOE REGION OF CALIFORNIA. EPA-600/2-78-208, December 1978.
 3. Innefeld, H., et al. DUAL PROCESS HIGH-RATE FILTRATION OF RAW SANITARY SEWAGE AND
   COMBINED SEWER OVERFLOWS. EPA-600/2-79-015, March 1979.
 4. Prah, D.H. and PL  Brunner. COMBINED SEWER OVERFLOW TREATMENT BY SCREENING AND
   TERMINAL PONDING. EPA-600/2-79-084, August 1979.
 5. Drehwing, FJ. COMBINED SEWER OVERFLOW ABATEMENT PROGRAM, ROCHESTER, NEW
   YORK: VOLUME II. EPA-600/2-79-031b, July 1979.
 6. Huber, W. and J. Heaney. URBAN RAINFALL - RUNOFF QUALITY DATA BASE: UPDATE WITH
   STATISTICAL ANALYSIS. EPA-600/8-79-004, August 1979.
 7. Characklis, W.G., et al. MAXIMUM UTILIZATION OF WATER RESOURCES IN A PLANNED COM-
   MUNITY- EXECUTIVE SUMMARY. EPA-600/2-79-050a, July 1979.
 8. Characklis, W.G., et al. MAXIMUM UTILIZATION OF WATER RESOURCES IN A PLANNED COM-
   MUNITY-STORMWATER RUNOFF QUALITY: DATA COLLECTION, REDUCTION AND ANALYSIS.
   EPA-600/2-79-050b, July 1979.
 9. Diniz, E.V. and W.H. Espey. MAXIMUM  UTILIZATION OF WATER RESOURCES IN A PLANNED
   COMMUNITY- APPLICATION OF THE STORM WATER MANAGEMENT MODEL: VOLUME I.
   EPA-600/2-79-050C, July 1979.
10. Diniz, E.V. and W. Espey. MAXIMUM UTILIZATION OF WATER RESOURCES IN A PLANNED COM-
   MUNITY - APPLICATION OF THE STORM WATER  MANAGEMENT MODEL: VOLUME II (APPEN-
   DICES). EPA-600/2-79-050d, NTIS only, July 1979.
11. Hammond, B. and J. Bishop Jr. MAXIMUM UTILIZATION OF WATER RESOURCES IN A PLANNED
   COMMUNITY- CHLORINE AND OZONE TOXICITY EVALUATION. EPA-600/2-79-050e, August 1979.
12. Davis, E.M. MAXIMUM UTILIZATION OF WATER  RESOURCES IN A PLANNED COMMUNITY -
   BACTERIAL  CHARACTERISTICS OF STORM WATERS IN DEVELOPING  RURAL
   AREAS.EPA-600/2-79-050f, August 1979.
13. Bergstedt, L.M., et al. LABORATORY EVALUATION OF METHODS TO SEPARATE FINE GRAINED
   SEDIMENT FROM STORMWATER. EPA-600/2-79-076, July 1979.
14. Medina, M. LEVEL  III: RECEIVING WATER QUALITY REMODELING FOR URBAN STORMWATER
   MANAGEMENT. EPA-600/2-79-100, August 1979.
15. Foreman, K.M. FIELD TESTING OF PROTOTYPE  ACOUSTIC EMISSION SEWER FLOWMETER.
   EPA-600/2-79-084, August 1979.
16. Meinholz, T.L, et al. SCREENING/FLOTATION TREATMENT OF COMBINED SEWER OVERFLOWS -
   VOLUME II: FULL SCALE OPERATION, RACINE, WISCONSIN. EPA-600/2-79-106a, August 1979.
17. Meinholz, TL, et al. SCREENING/FLOTATION TREATMENT OF COMBINED SEWER OVERFLOWS -
   VOLUME II: FULL SCALE OPERATION, RACINE, WISCONSIN. EPA-600/2-79-106b, NTIS only, Au-
   gust 1979.
18. Buxton, H. and FT.  Caruccio. EVALUATION OF SELECTIVE EROSION CONTROL TECHNIQUES -
   PIEDMONT REGION OF S.E. UNITED STATES. EPA Report No. Pending.
19. Drehwing, F, et al. DISINFECTION/TREATMENT OF COMBINED SEWER OVERFLOWS, SYRACUSE,
   NEW YORK. EPA-600/2-79-134, August 1979.
20. Pisano, W.C., et al. DRY-WEATHER DEPOSITION AND FLUSHING FOR COMBINED SEWER OVER-
   FLOW POLLUTION CONTROL. EPA-600/2-79-133, August 1979.
21. Pitt, R. DEMONSTRATION OF NONPOINT POLLUTION ABATEMENT THROUGH STREET CLEAN-
   ING PRACTICES. EPA-600/2-79-161, August 1979.
22. Koncza, L, et al. LAWRENCE AVENUE UNDERFLOW SEWER SYSTEM INTERIM REPORT PLAN-
   NING AND CONSTRUCTION. EPA Report No. Pending.
23. Berwick, R. SELECT TOPICS IN STORMWATER MANAGEMENT PLANNING FOR NEW RESIDEN-
   TIAL DEVELOPMENTS.  EPA Report No. Pending.


56

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                    DRINKING WATER RESEARCH DIVISION
  The Drinking Water Research Division (DWRD) of MERL determines the occurrence of contaminants
and conducts research and development to establish the water treatment and control technology, in
accordance with the provisions of the Safe Drinking Water Act of 1974 (Public Law 93-523). The Division
maintains liaison with the Office of Drinking Water in the Office of Water and Waste Management so
that requirements of the Act can be met in a timely fashion.
  The Division Director provides a focal point for the coordination of all water supply activities in ORD,
including Municipal  Environmental Research Laboratory, Cincinnati, Ohio; Health Effects Research
Laboratory, Cincinnati, Ohio; Environmental Monitoring and Support Laboratory, Cincinnati, Ohio; the
Environmental Research Laboratory, Athens, Georgia; and the Environmental Research Laboratory,
Ada, Oklahoma. The Office of Drinking Water provides resources to these groups for technical
assistance to the states, to water utilities, and to the  general  public.
  Major issues that have spotlighted the research effort during the past year include the investigation
of treatment practices to minimize the presence of organics in treated water, the  examination of
treatment technology and associated costs to reduce contaminant levels to those specified in the
National Interim  Primary Drinking Water Regulations (NIPDWR), the use of disinfectants other than
chlorine and the determination of whether harmful by-products are formed, the removal of asbestos
fibers from  drinking water, the removal of Giardia lamblia from public water supplies not  using
filtration, the development of rapid methods for the detection of bacteria, the relationship of turbidity
to disinfection efficiency, the role of viruses in disinfection, and the evaluation of  point-of-use treat-
ment devices.
PHYSICAL AND CHEMICAL CONTAMINANTS
REMOVAL BRANCH

  The objectives of the in-house and extramural
research conducted by the Physical and Chemi-
cal Contaminants Removal Branch are to develop
economic drinking water treatment unit pro-
cesses to allow a water utility of any size to meet
the Drinking Water Regulations,  either  those
presently effective or those contemplated in the
future, and to devise techniques to allow the dis-
tribution of water to the consumer without deteri-
oration in quality. To accomplish this, the Branch
isdivided into five research areas: InorganicCon-
taminants, Particulate Contaminants,  Organic
Contaminants, Economic Analysis, and Distribu-
tion System Quality.

Inorganic Contaminants

  In-house studies and extramural research
grant programs on the removal of trace metals
and other inorganics listed in the National Inte-
rim  Primary Drinking  Water Regulations
(NIPDWR) stressed the development of technol-
ogy to remove the four significant ground water
contaminants that impact small communities: ar-
senic, fluoride, nitrate, and selenium.
  Activated alumina, which has been effectively
used to remove fluoride from water, continued to
be investigated for the removal of selenium and
arsenic. This material was shown to remove se-
lenium IV and VI and arsenic III and Vfrom water
under certain conditions. Studies also showed
that slightly different regeneration processes for
activated alumina may be required for the three
contaminants of fluoride, selenium and arsenic.
Ion exchange treatment was investigated for ar-
senic removal and results showed that strong
base resins were effective for arsenic V, but not
for arsenic III.
  Field  projects  to  complement in-house re-
search continued to investigate the removal of all
the inorganic contaminants listed in the NIPDWR
from ground water by  reverse osmosis; se-
lenium from ground water by activated alumina;
and nitrate from ground water by ion exchange
and reverse osmosis (Figure 24). A new project
was also funded to  study the effectiveness of
conventional package plant systems that have
specific application  for small  communities. A
mobile pilot plant housing activated alumina
treatment, ion  exchange, reverse osmosis, and
electrodialysis was developed by the University
of Houston. This mobile system will be operated
                                          57

-------
in small communities to provide practical infor-
mation for the design and operation of treatment
systems for small water supplies. Economic data
will also be developed in all of the field projects.
  Detailed information on completed jar test and
pilot plant studies for trace metal removal by
conventional  treatment and lime  softening is
being published in a series of articles in the Jour-
nal of the American Water Works Association.
RELATED RESEARCH PUBLICATIONS
                                             Figure 24. Reverse osmosis for the removal of
                                                        inorganics from drinking water.
 1. Sorg, T.J., M. Csanady, and G.S. Logsdon. TREATMENT TECHNOLOGY TO MEET THE INTERIM
   PRIMARY DRINKING WATER REGULATIONS FOR INORGANICS: PART 3 (CADMIUM, LEAD AND
   SILVER). Journal of American Water Works Association, 70(12) :680-691,1978.
 2. Sorg, T.J. TREATMENT TECHNOLOGY TO MEET THE INTERIM PRIMARY DRINKING WATER REG-
   ULATIONS FOR INORGANICS: PART 4 (CHROMIUM AND MERCURY). Journal of American Water
   Works Association, 71(8):454-466,1979.
Particulate Contaminants

  Particulate removal studies continued for two
types of contaminants- asbestos fibers and Giar-
dia cysts. A comprehensive report on water filtra-
tion for asbestos fiber removal was prepared in
order to explain results reported by other inves-
tigators, to provide information for designers of
water filtration plants, and to give guidelines for
the successful operation of filtration plants that
are removing asbestos fibers from drinking
water. This document reviews  the literature of
other investigators (mostly Canadian), summar-
izes filtration studies funded by U.S. EPA at Du-
luth and Seattle, and presents monitoring data
gathered  at water treatment plants in  Phila-
delphia, Chicago, the San Francisco Bay area,
and the Lake Superior North Shore.
  Results of treatment for asbestos removal are
now available for a number of widely separated
geographic locations from coast to coast in the
United States and Canada, for  a wide range of
source waters, from a pristine mountain lake to
turbid rivers and estuarine waters, and for varia-
tions in flow  from 10 gallons per minute  or
smaller to more than 200 million gallons per day
and  several modifications  of  granular media
filtration.
  Data from Seattle and Lake Superior show that
chrysotile and amphibole fiber concentrations in
drinking water can be substantially reduced by
granular media filtration. Reductions of up to
99.99 percent were reported during storm condi-
tions at Duluth, Minnesota. Effective granular
media filtration required very diligent plant oper-
ation with careful control of pH, coagulant doses,
and filtered water turbidity.
  When a granular media filtration plant is prop-
erly operated, turbidity readings can be used as a
guide to fiber  removal efficiency even though
turbidity cannot directly measure asbestos fibers
in the concentrations found at water treatment
plants. Filtered water turbidity should be 0.10
nephelometric turbidity units (ntu) or lower to
maximize fiber removal. Turbidity increases of 0.1
or 0.2 ntu above this value generally were accom-
panied by  large increases in asbestos fiber con-
centrations.  The 1  ntu Maximum Contaminant
Level (MCL) for turbidity is not a satisfactory
quality goal if asbestos removal is needed.
  Some of the results presented suggest that fi-
ber removal  is more easily accomplished when
source waters have turbidities greater than 1 ntu,
which is the raw water turbidity typical of Lake
Superior and Seattle's Tolt Reservoir.
 58

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  Diatomaceous earth filtration was found effec-
tive for asbestos fiber removal in bench-scale and
pilot plant studies. A full scale diatomite filtration
plant has not yet been evaluated forfiber removal
efficiency. Research to date indicates that coating
the diatomaceous earth filter aid with aluminum
hydroxide substantially increases the removal of
both amphibole and chrysotile fibers. Duluth re-
sults indicate that filtered water turbidity should
be 0.10 ntu for most effective fiber removal.
  Research on Giardia cyst removal by water fil-
tration continued in the laboratory, with the use
of G. muris, a mouse parasite, because the
human  parasite, G. lamblia, was not generally
available in the Cincinnati area. G. lamblia and G.
muris are  similar in  size,  and both  are  elec-
tronegative (negative zeta potential), so results
obtained with G. muris should be a good indica-
tor of the behavior of G. lamblia under similar
conditions.
  Diatomaceous earth filtration studies showed
that operating technique is important. Cyst re-
moval with a clean filter operating at 1.0 gallons
per minute per square foot (gpm/sf) ranged from
99.8 to 99.98 percent. At 1.5 gpm/sf removal
ranged  from 99.95 to 99.998 percent. Cyst re-
moval at 1.0 gpm/sf by a  filter that was not uni-
formly precoated dropped to 99.36 percent.
  Granular media filtration tests utilizing dual

RELATED RESEARCH PUBLICATIONS
media (coal and sand) show that for this kind of
filtration proper operating technique is again es-
sential.  Bench scale tests with a 1.5 inch (4 cm)
diameter f ilter indicated that changes that upset
the equilibrium condition in the filter can result in
the release of floe and cysts that had been stored
in the media, or can result in the passage of cysts
through the filter media. Abrupt increases in fil-
tration rate, loss of chemical feed, and turbidity
breakthrough at the end of a run all resulted in
substantial increases in cyst concentration in fil-
tered water. Small increases in turbidity (0.1 or 0.2
ntu) were associated with increases in cyst con-
centration often to one hundredfold.
  When clear waters (1-5  ntu)  are  filtered,
treated water turbidity must be well below the 1
ntu Maximum Contaminant Level for turbidity for
the most effective cyst removal. Cyst  removal
generally exceeded 99.0 percent when effluent
turbidity was in the range of 0.2 - 0.3  ntu.
  Research on G. lamblia cyst removal by water
filtration is under way in a pilot plant study at the
University of Washington.  The  Drinking Water
Research Division is completing construction of a
trailer-mounted 20 gpm package plant for use by
the University of Washington at various locations
in the State of Washington. This work will be
done during the 1980 calendar year.
1.  Logsdon, G.S. WATER  FILTRATION FOR ASBESTOS FIBER REMOVAL. EPA 600/2-79-206, U.S.
   Environmental Protection Agency, Cincinnati, Ohio, December 1979.
2.  Logsdon, G.S. FILTRATION WORKS OUT ASBESTOS FIBERS. FX. Schleppenbach and TM. Zaudtke.
   Water and Sewage Works, 126(10):44-46,1979.
Distribution System and Water Quality

  In-house studies utilizing sections of asbestos
cement (A/C) pipe inserted in circulating systems
with varying water quality conditions in the dif-
ferent systems have shown  that (1) pH 8.2 and
zinc concentrations =ฃ 0.3 mg/l  will protect A/C
pipe from attack regardless of the zinc compound
used to provide the zinc and that even waters
with very low calcium concentrations do not at-
tack the A/C pipe when these conditions exist; (2)
calcium carbonate saturation of the water will
prevent attack on A/C pipe;  (3) sodium silicate
added to the water can provide protection to A/C
pipe; and (4) the same aggressive waters that do
not attack the A/C pipe at pH 8.2 with zinc will
attack A/C pipe when zinc is not present. A grant
with  the city  of  Greenwood, South Carolina
showed that a concentration of  0.3 mg/l zinc
provides much better protection of A/C pipe than
do concentrations of s 0.1 mg/l zinc.
  Energy dispersive X-ray spectral  elemental
analyses using the electron microscope show
that A/C pipe surfaces protected against attack by
coatings, such as iron  or zinc, have  significant
calcium peaks as well as iron and zinc peaks. A/C
pipe surfaces showing attack have none or very
low calcium peaks and  insufficient iron or zinc
peaks to indicate protection. The size  of calcium
peak for the protected pipe depends  on the de-
gree of coating. As the coating thickens the cal-
cium peak size will decrease and a heavy coating
of iron or zinc could very well eliminate the cal-
cium peak for a protected pipe.
  In-house studies on the corrosion of lead pipe
are  continuing by evaluating control techniques
involving pH and alkalinity  adjustments. Litera-
ture references to lead solubility diagrams had
shown that the solubility of lead hydroxide de-
creased with increasing alkalinity and that mini-
mum solubility occurred at pH 8.6. However,
                                                                                       59

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laboratory corrosion rate meaurements using
linear polarization techniques suggested that the
protective coatings became more unstable as the
alkalinity was increased while maintaining  pH
8.5.  Computer generated solubility diagrams
showing the  response of lead solubility to dis-
solved carbonate later showed that increased
carbonate concentration would tend to dissolve
lead hydroxide. Furthermore, these solubility di-
agrams showed that the minimum  solubility of
lead hydroxide would occur at pH 9.5  at an al-
kalinity of about 20 mg/l as calcium carbonate.
Preliminary corrosion rate measurements ap-
peared to  confirm these predictions. Raman
Spectroscopic techniques, which have been
shown to be  capable of analyzing surface films
on lead pipes, will be used to corroborate these
results.
  In a grant with The Metropolitan Water District
of Southern California, the EPA Mobile Water
Quality Monitoring Labortory was used in a
study to evaluate the effects of blending waters of
different quality and to relate their composition
to the corrosive effects of the water on the sys-
tem. The mobile lab proved to be an effective tool
for data collection at thirty Southern California
locations in the Los Angeles area, especially after
automation of the calcium deposition tester and
modifications  to the corrosion test  equipment.
Corrosion rates were correlated with the Lan-
gelier saturation index, the Ryzner index, the cal-
cium concentration and conductivity. The cal-
cium carbonate deposition test (CCDT)  could
readily detect changes in alkalinity or calcium
hardness. The addition of corrosion inhibitors
such as zinc orthophosphate could be detected
by the CCDT.  Although a number of effects of
blending waters of various quality were observed
during this study, none of the effects of blending
imported surface waters with local groundwaters
generated any serious problems in water in the
distribution systems of the area. This work  has
now been completed and a final report has been

RELATED RESEARCH PUBLICATIONS
received for publication.
  The mobile laboratory was moved to the Law-
rence Berkeley Laboratory where it is undergoing
extensive updating and renovation under an in-
teragency agreement with  The Lawrence
Berkeley Laboratory. A new computer and data
acquisition system has been received so that all
data can be handled at the mobile lab rather than
through the outside terminal. After renovation,
the mobile lab will be used in a study on corro-
sion control treatment for the  water supply of
Seattle, Washington.
  Investigations are continuing  at the University
of Florida  to evaluate water quality parameters
for establishing a corrosion index that would be
more useful in predicting  corrosion rates in a
metal pipe. Laboratory corrosion  rate testing is
being done on coupons in forty-eight sample
containers under carefully controlled conditions.
Data obtained for  mild steel showed that corro-
sion rates  in deaerated systems were low com-
pared to those in aerated systems, and that there
may be a relationship of corrosion rate to chlo-
rine residual levels.  Pipe loops studies using
these metals are also in progress.
  A laboratory cortosion study  at John Hopkins
University was completed to isolate the source of
lead and other metals present in the drinking
water in portions of  Carroll County, Maryland.
The  lead in Carroll County's system is being
picked  up from the copper pipe distribution sys-
tems because lead is not detectable in the source
water.  The corrosion studies were conducted
with copper pipe loops constructed with solders
of various compositions to evaluate the effect of
various water quality parameters and flow rates
on corrosion rates. Test data showed highest lead
levels when low pH (5.5), low alkalinity (10 mg/l)
and low hardness  (10 mg/l) simultaneously oc-
curred. The effect of dissolved oxygen on corro-
sion rate was present at low pH  and negligible at
higher pH. Maximum lead levels were achieved
within fifteen minutes.
Buelow, R.W., J.R. Millette, E.F McFarren, and J.M. Symons. THE BEHAVIOR OF ASBESTOS-CEMENT
PIPE UNDER VARIOUS WATER QUALITY CONDITIONS - A PROGRESS REPORT, PART I - EXPERIMEN-
TAL RESULTS, Proceedings of 99th Annual AWWA Conference, San Francisco, California, June 27,
1979 (In Press). Manuscript available.
Organic Contaminants

  The basic objective of our field investigations
efforts is to evaluate and  develop water treat-
ment technology that minimizes the presence of
potentially  harmful organics in drinking water.
The research projects involve organic  sub-
stances associated with the disinfection of drink-
ing water, such  as trihalomethanes and  precur-
sors, and specific organic substances that occur
in  the source waters and are not substantially
removed by commonly used water treatment
methods. The projects also include evaluation of
60

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the costs required for a given technology, when-
ever the scale of the project is large enough.

Surface Water Studies

  Current investigations include studies of ad-
sorbents, alternative disinfectants and modifica-
tion of the points of application of disinfection to
minimize  organic  contamination. Also, onsite
granular activated  carbon reactivation technol-
ogy is under investigation.
  Two extramural research projects on the com-
bination of ozone and granular activated carbon
(GAC) as a means of extending activated carbon
bed life are expected to have the pilot plants in
operation  by December 1979. Shreveport, Loui-
siana will operate a 10 gpm pilot plant and Phila-
delphia, Pennsylvania will operate a 20 gpm pilot
plant.
  In-house studies are continuing on the com-
bination of oxidants with granular activated car-
bon. A pilot scale in-house project is examining
the effects of ozone followed by deep bed filtra-
tion (to maximize biodegradation of trace
organics before  adsorption). A parallel study is
using hydrogen peroxide as the oxidant to see if
the effects are similar to those obtained in earlier
studies with ozone.
  Granular activated carbon (GAC) studies invol-
ving both  full-scale gravity contactors and  pilot
columns are progressing at a site along the lower
Mississippi. Four, six-month phases of full-scale
operation  of gravity GAC beds  using lower Mis-
sissippi river water  have been completed (Figure
25). One bed was operated as a system. Prelimin-
ary results were reported in June 1979 at the
AWWA in  San Francisco, California and at the
Figure 25. Overview of the New Orleans Water
           Treatment Plant.
May 1979 EPA/NATO/CCMS sponsored Adsorp-
tion Techniques Conference held in Reston, Vir-
ginia. Preparation of the final project report has
begun.
  At a site on the Ohio River, a recently instituted
second phase of pilot column investigation using
two types of carbon operated as post filter adsor-
bers along with columns operated as sand re-
placement  systems in parallel with virgin and
once reactivated carbon has been completed.
Construction of the full scale water supply GAC
post filtration pressure contactors is  complete
and one of the four 1 million gallon per day con-
tactors was placed into operation in October. The
remaining two  will  be put into operation at one
month intervals. The on-site fluid bed carbon re-
activation system  is scheduled for shakedown
tests and full operation by December 1979.
  In 1979, full-scale operation of the on-site fluid
bed carbon reactivation systems was begun at
Manchester, New Hampshire. The system is reac-
tivating carbon that has  been used for surface
water treatment.
  Studies evaluating the potential of an electric
furnace for reactivating granular carbon are near-
ing completion  at the Little Falls, New Jersey site.
Thus far, the infrared furnace looks very promis-
ing as an alternative to fossil fuel devices. Also
encouraging are the indications that simple and
inexpensive tests such as iodine  numbers and
apparent densities are reliable monitors of reac-
tivation efficiencies. On a smaller scale, studies
were  initiated to  compare three different type
furnaces for reactivating granular carbon used in
a sand replacement operation mode and a pro-
ject was started to examine the potential for sol-
vent  regeneration by  supercritical carbon
dioxide.
  A lower Ohio River study is using the full-scale
plant as a control and a pilot plant at this location
is being used for comparison of the effects of
chlorine and  chlorine dioxide disinfection both
with and without GAC. Various modes of opera-
tion of the pilot plant have been  evaluated in
short term tests and a mode has been selected for
long-term evaluation. Using pre and post chlo-
rine dioxide disinfection, the performance of vir-
gin activated carbon and subsequent off-site
regenerated carbon will be evaluated (Figure 26).

Ground Water Studies

  Groundwaters, particularly from deep well
sources, have traditionally been considered less
susceptible to organic pollution than surface wa-
ters. Improved  analytical procedures,  however,
combined with more widespread monitoring are
showing an alarming number of groundwaters

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 Figure 26. Carbon contactors at Evansville,
           Indiana.

contaminated with industrial solvents. In almost
all cases, the water was being analyzed for other
constituents (mainly trihalomethanes) when the
solvents were discovered.
  Currently (October 1979) dozens of wells serv-
ing several thousand people have been reported
contaminated in New England, New Jersey, New
York (particularly Long Island), Pennsylvania and
Florida. California, Arizona, Michigan and Vir-
ginia also have reported isolated incidences of
ground water pollution resulting from surface
activities. More cases are expected as monitoring
increases.
  For the past two years the Drinking Water Re-
search Division (MERL-Cincinnati) has conducted
treatment experiments for  removing these sol-
vents from drinking water. Cooperative pilot
scale studies with the U.S. Air Force and a utility
in Connecticut  and one in New  Jersey have
provided  important information on the  useful-
ness of treatment techniques  such as aeration
and adsorption (Figure 27).
  In addition to our in-house activities, an extra-
mural treatment project was started last fiscal
year with a utility on Long Island  and another
indepth project is likely to be funded in New
England at a utility that has no alternate source of
water.
  At the request of Region III, the DWRD partici1
pated in a workshop/seminar in Philadelphia, at
which  the  state-of-the-art for treatment of
organic contaminated groundwaters was the
topic.
  Pilot  plant testing for the removal of organic
contaminants from ground water began this year
at Glen Cove, New York (Long Island), where sev-
eral wells have been closed down; The processes
of adsorption by a synthetic resin (XE-340ฎ) and
Figure 27. Pilot scale aeration and adsorption
           units  to  study groundwater
           decontamination.
aeration are being investigated as techniques for
the  effective removal of primarily  tri-
chloroethylene and tetrachloroethylene. In situ
steam regeneration of the exhausted resin is tak-
ing place and represents the first such applica-
tion for drinking water studies.
  A third extramural research  project on the
combination of ozone and GAG (a 100 gpm pilot
plant) will be in operation by December 1979 in
Miami, Florida. Preliminary data from the Miami
project were reported at the Reston meeting.

General Studies  •

  Research  is continuing to investigate the re-
moval of specific organic compounds using GAC.
Isotherm and kinetic data are also being gener-
ated to be used for evaluation of dynamic adsorp-
tion  models developed  under  projects to be
compiled in 1979.
  Gas chromatographic methods using glass
capillary column technology and both flame io-
nization and  mass spectrometric detection have
advanced to the point that they are being used to
assess qualities of water samples from all stages
of treatment  including granular activated carbon
effectiveness (Figure 28). This technology has
62

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of an intense research effort. Progress has been
made on several fronts. Firstly, a three year study,
originally designed to determine mechanisms of
trihalomethane formation from aquatic humic
material, has been successful in compiling more
information on humic structures and chlorina-
tion byproducts than previously available in the
literature, as well as  in meeting the initial
objectives.
  Secondly, work on development of a routine
method for measurement of organic substituted
halogen  has progressed to the point of accep-
tance of a standardized technique. Organo-
halides are adsorbed onto activated carbon, the
carbon is combusted in a pyrolysis tube under a
continuous gas flow, and the resulting chloride is
determined  by microcoulometric titration. The
method and apparatus have been modified and
simplified for routine laboratory use. The tech-
nique is being used to provide information on the
degree of halogen substitution on  high molecu-
lar weight compounds caused by various disin-
fectants including chlorine,  chlorine dioxide,
chloramines, and ozone. This work is  being car-
ried out on both  laboratory model  mixtures and
various tap waters. In 1979 an expanded program
to investigate the nature of these higher molecu-
lar weight  disinfection  byproducts  will  be
initiated.
 Figure 28. Gas chromatograph/mass spectro-
           meter  instrumentation  for  the
           confirmation of organics present in
           water.

now been applied at a number of full scale plants
to gain qualitative impressions of unit process
performance. A detailed broad spectrum quan-
titative analysis now seems to be a realistic goal.

Disinfection Byproducts

  Organic byproducts of disinfection other than
trihalomethanes have continued to be the subject

RELATED RESEARCH PUBLICATIONS

 1.  Dressman, R.C., B.A. Najar, R. Redzikowski, et al. THE DETERMINATION OF CARBON ADSORBA-
    BLE ORGANIC HALIDES AS CHLORIDE (CAOX AS C1 ) IN WATER BY MINI-COLUMN ADSORPTION,
    PYROLYSIS, AND CHLORIDE-ION MEASUREMENT - AN EVALUATION AND COMPARATIVE
    STUDY. In:  Proceedings of the American Water Works Association Water Quality Technology
    Conference, Philadelphia, Pennsylvania, December 1979 (In Press).
 2.  Dressman, R.C., A.A. Stevens, J. Fair, and B.  Smith. COMPARISON OF METHODS FOR DETER-
    MINATION OF TRIHALOMETHANES IN DRINKING WATER. Journal of the American Water Works
    Association, 71(7):392-396, 1979.
 3.  Symons, J.M. and A.A. Stevens. PHYSICO-CHEMICAL PRETREATMENT FOR REMOVAL OF PRE-
    CURSORS. In: Proceedings of the International Conference on Oxidation Techniques in Drinking
    Water Treatment, September 9-12, 1978, Karlsruhe, FRG,September 1979.
 4.  Stevens, A.A.  FORMATION OF NON-POLAR ORGANOCHLORO COMPOUNDS. In: Proceedings of
    the International Conference on Oxidation Techniques in  Drinking Water Treatment, September
    9-12, 1978, Karlsruhe, FRG, September 1979.
 5.  Stevens, A.A., D.R. Seeger, J. DeMarco, and L Moore. REMOVAL OF HIGHER MOLECULE WEIGHT
    ORGANIC COMPOUNDS BY THE GRANULAR ACTIVATED CARBON ADSORPTION UNIT PROC-
    ESS. In: Proceedings of the Conference on Practical Application of Adsorption Techniques in
    Drinking Water TreatmentNATOICCMS, EPA International Conference, Reston, Virginia, April 30,
    May 1-2, 1979. (In Press) Manuscript Available.
 6.  Murin, C.J. and V.L Snoeyink. COMPETITIVE ADSORPTION OF 2,4-DICHLOROPHENOL and 2,4,6-
    TRICHLOROPHENOL IN  THE NANOMOLAR TO MICROMOLAR CONCENTRATION RANGE.  En-
    vironmental Science and Technology, 13:305, 1979.
 7.  Varma, M.M., M.R. Siddique, K.T Doty and A. Machis. ANALYSIS OF TRIHALOMETHANES IN
    AQUEOUS SOLUTIONS: A COMPARATIVE STUDY. Journal of the American Water Works Associa-
    tion, 1'1(7): 389-392, 1979.
                                       63

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 8. Stevens, A.A. and J.M. Symons. FORMATION AND MEASUREMENT OF TRIHALOMETHANES IN
    DRINKING WATER. In: Proceedings of Seminars on Control of Organic Chemical Contaminants in
    Drinking Water, Cincinnati, Ohio, October 10-11, 1979.(In Press) Manuscript Available.
 9. Miller, G.W., et al. AN ASSESSMENT OF OZONE AND CHLORINE DIOXIDE TECHNOLOGIES FOR
    TREATMENT OF MUNICIPAL WATER SUPPLIES; EXECUTIVE SUMMARY.  EPA-600/8-78-018, U.S.
    Environmental Protection Agency, Cincinnati, Ohio, October 1978.
10. Love, O.T, Jr. and J.M. Symons. BASIS FOR DECISION MAKING - ENGINEERING EVALUATIONS
    OF APPROACHES TO SYNTHETIC ORGANIC CONTROL: PILOT STUDY DESIGN. In: Proceedings of
    Seminars on Control of Organic Chemical Contaminants in Drinking Water, Cincinnati, Ohio,
    October 10-11, 1979 (In Press) Manuscript Available.
11. Symons, J.M. UTILIZATION OF VARIOUS TREATMENT UNIT PROCESSES AND TREATMENT
    MODIFICATION FOR TRIHALOMETHANE CONTROL. In: Proceeding of Seminars on Control of
    Organic Chemical Contaminants in Drinking Water, Cincinnati,  Ohio,  October 10-11, 1979. (In
    Press) Manuscript Available.
12. Love, O.T, Jr. and W.R. Inhoffer. EXPERIENCE WITH INFRARED FURNACE FOR REACTIVATING
    GRANULAR ACTIVATED CARBON (A PROGRESS REPORT). In: Proceedings of Practical Applica-
    tions of Adsorption Techniques in Drinking Water, Reston, Virginia, April 1979, (In Press) Man-
    uscript Available.
13. Symons, J.M., J.K. Carswell, J. DeMarco and O.T. Love, Jr. REMOVAL OF ORGANIC CON-
    TAMINANTS FROM DRINKING WATER  USING TECHNIQUES  OTHER THAN GRANULAR ACTI-
    VATED CARBON ALONE - A PROGRESS REPORT. In: Proceedings of Practical Applications of
    Adsorption Techniques in Drinking  Water, Reston, Virginia, April 1979. (In Press)  Manuscript
    Available.
14. Love, O.T, Jr. EXPERIENCE WITH REACTIVATION OF GRANULAR ACTIVATED CARBON. In: Pro-
    ceedings of the Preconference Seminar "Controlling Organics in  Drinking Water" at the 99th
    Annual American Water Works Association Conference, San Francisco, California, June 1979 (In
    Press).
15. DeMarco, J. and N. Brodtmann, Jr. PREDICTION OF FULL-SCALE PLANT PERFORMANCE FROM
    PILOT COLUMNS. In: Proceedings of Practical Applications of Adsorption Techniques in Drinking
    Water,  Reston, Virginia, April 1979. (In Press) Manuscript Available.
16. Wood,  R and J. DeMarco. TREATMENT OF GROUND WATER WITH ACTIVATED CARBON. In:
    Proceedings of Practical Application of Adsorption Techniques in Drinking Water, Reston, Virginia,
    April 1979 (In Press) Manuscript Available.
17. Brodtmann,  N., W. Koffskey, and J. DeMarco. TECHNIQUES  FOR THE EVALUATION AND
    MONITORING OF GAC PERFORMANCE. In: Proceedings of the Preconference Seminar "Controll-
    ing Organics in Drinking Water" at the 99th Annual American Water Works Association Con-
    ference, San  Francisco, California, June 1979  (In Press).
18. DeMarco, J. and  R Wood. DESIGN DATA FOR ORGANICS REMOVAL BY CARBON BEDS. In:
    Proceedings of National Conference on Environmental Engineering Research Development and
    Design, American Society'of Civil Engineers, 1978, p. 149.
19. Wood, R and J. DeMarco. EFFECTIVENESS OF VARIOUS ADSORBENTS IN REMOVING ORGANIC
    COMPOUNDS FROM WATER- PART I, REMOVING PURGEABLE HALOGENATED ORGANICS AND
    PART II, REMOVING TOTAL ORGANIC CARBON AND TRIHALOMETHANE PRECURSOR SUB-
    STANCES. In: Proceedings of Symposium on Activated Carbon Adsorption of Organics from the
    Aqueous Phase, Ann Arbor Science Publication, Ann Arbor, Michigan (In Press).
20. Brodtmann, N.V., J. DeMarco and D. Greenburg. CRITICAL STUDY OF LARGE-SCALE GRANULAR
    ACTIVATED CARBON FILTER UNITS FOR THE REMOVAL OF ORGANIC SUBSTANCES FROM
    DRINKING WATER. In: Proceedings of Symposium on Activated Carbon Adsorption of Organics
    from the Aqueous Phase, Ann Arbon Science Publication, Ann  Arbor, Michigan. (In Press).
Economic Analysis

  Economic factors are to be considered in the
implementation of the various provisions of the
Safe Drinking Water Act.  One of the major eco-
nomic concerns facing EPA is small systems
compliance. Economies of scale insure that small
utilities have higher unit costs than do larger
utilities. If these small water systems are forced
to invest in additional expensive treatment proc-
esses, the cost burden may be more than many
small communities can afford. Therefore, the
Drinking Water Research Division is devoting a
significant portion of its economic analysis effort
to problems relating to small systems and the
64

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management of technology in small utilities.
  For example, the economic analysis unit has
conducted a field survey of 10 small utilities in
EPA  Regions III, V,  VI, VIM, IX and X. A report
discussing the results of the data collected in
Regions III, V and VI  has been completed. An-
other phase of the small systems study deals
with  the use of package plants as a  means of
providing cost effective treatment for small water
utilities. Package water treatment plants are pre-
fabricated units constructed on site. A study has
been completed and a report published detailing
the results of a study of 36 small utilities utilizing
package plant technology in Kentucky, Ten-
nessee, and West Virginia.
  Another important item in the study of water
utility economics is that of standardized account-
ing systems. A cost analysis system that can be
used by all utilities has been implemented in
Kenton County Water District Number 1, in Ken-
ton County, Kentucky. Included  is a financial
reporting system that will utilize data from the
cost accounting system to generate standardized
fiscal reports. A two  volume report  has been
completed; one volume describes the philoso-
phy and implementation procedures for the sys-
tem and the second volume contains a series of
detailed flowcharts that will allow the system to
be implemented as a water utility  management
tool.
  The Drinking Water  Research Division has re-
cently completed a detailed study of the cost of
water supply unit treatment processes. This four
volume report contains costs for 99 unit proc-
esses. It provides examples of how cost analysis
can be conducted; shows typical flowcharts for
several of the more common  treatment proc-
esses; and contains the listing for computer pro-
grams that allows these cost data to be used in an
efficient manner.
  A study has been initiated to analyze the im-
pacts and trade-offs associated with regional
water supply systems. A computer model is
being developed that allows users to make a real-
istic  assessment of the cost of joining or not
joining a regional water supply system.
  A study has been undertaken to  find an  effi-
cient computer-based system for analyzing re-
search data generated  from  the Division's field
and in-house  studies. When  fully implemented,
the system will be  interactive, allowing the  pro-
ject officers to manage and  analyze their data
efficiently and effectively.
  Several studies have been conducted and pa-
pers and  reports completed  detailing the costs
associated with the treatment of organics in
drinking water. These studies are primarily ori-
ented toward the use of granular activated
carbon. Costs have also been developed for alter-
native disinfection systems  such as ozonation,
chlorination, and chlorine dioxide. A study was
conducted in which a selected sample of utilities
was  studied  in-depth to establish a cost record
over a period of time and to examine the  eco-
nomic impact of Safe Drinking Water Act.
RELATED RESEARCH PUBLICATIONS

 1. Clark, M., R.G. Stevie, and G.D. Trygg. AN ANALYSIS OF MUNICIPAL WATER SUPPLY COSTS.
   Journal of the American Water Works Association, 70(10) :543-547,1978.
 2. Clark, M., J.A. Machisko, and R.G. Stevie. COST OF WATER SUPPLY: SELECTED CASE STUDIES.
   Journal of the Environmental Engineering Division of the American Society of Civil Engineers,
   105(EEI):89-100, 1979.
 3. Clark, R.M., Y.H. Kim, and G. Huband. ENERGY UTILIZATION IN WATER TREATMENT. In: Proceed-
   ings of the Conference on Engineering Conservation and the Design of Water Quality Facilities,
   Kansas City, August 1979. (In Press) Manuscript Available.
 4. Clark, R.M. and P. Dorsey. INFLUENCE OF OPERATING VARIABLES ON THE COST OF TREATMENT
   BY GAC  ADSORPTION. In: Proceedings of Practical Applications of Adsorption  Techniques in
   Drinking Water, Reston, Virginia, May 1979. (In Press) Manuscript Available.
 5. Clark, R.M. LABOR, WAGE RATES, PRODUCTIVITY AND THE COST OF WATER SUPPLY. Journal of
   the American Water Works Association, 71 (7):364-368,1979.
 6. Clark, R.M. and R.G. Stevie.  MEETING THE  DRINKING WATER STANDARDS: THE PRICE OF
   REGULATION IN SAFE DRINKING WATER: CURRENT DIRECTIONS AND FUTURE PROBLEMS. C.S.
   Russell, ed. Resources for the Future, Research Paper 12,1978.
 7. Clark, R.M. SMALL WATER SYSTEMS: THE ROLE OF TECHNOLOGY. Accepted for publication by
   the Journal of the Environmental Engineering Division of American Society of Civil Engineers.
 8. Clark, R.M. THE ROLE OF TECHNOLOGY IN MANAGING SMALL WATER  UTILITIES.  In: Proceed-
   ings of the EPA Conference on Small Water Systems, November 1978.
 9. Clark, R.M. REGIONALIZATION FOR WATER SUPPLY: A CRITICAL EVALUATION. Journal of the
                                                                                    65

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    Water Resources Planning and Managment Division of the American Society of Civil Engineers,
    105(WR2):279-294, 1979.
10.  Gumerman, R.C., R.L Gulp, and R.M. Clark. COST OF GRANULAR ACTIVATED CARBON IN THE
    USA. Proceedings of Practical Applications of Adsorption Techniques in Drinking Water, Reston,
    Virginia, (In Press) and Journal of The American Water Works Association, 71(11):690-696,1979.
11.  Guttman, D.L and R.M.  Clark. COMPUTER COST MODELS FOR PORTABLE WATER TREATMENT
    PLANTS. EPA-600/2-79-181, Municipal Environmental Research Laboratory, U.S. Environmental
    Protection Agency, Cincinnati, Ohio, September 1978.
12.  Gillean, J.I., W.L Britton, Jr., J.H. Brium and R.M. Clark. DEVELOPMENT OF A WATER SUPPLY COST
    ANALYSIS SYSTEM- VOLUMES I AND II. EPA-600/2-8fK)12a and EPA-600/2-80-012b, U.S. Environ-
    mental Protection Agency, Cincinnati, Ohio (In Press).
13.  Gumerman, R.C., R.L. Gulp and S.R Hansen. ESTIMATING WATER TREATMENT COSTS: VOLUME I
    - SUMMARY. EPA-600/2-79-162a, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
14.  Gumerman, R.C., R.L Gulp and S.R Hansen. ESTIMATING WATER TREATMENT COSTS: VOLUME II
    - COST CURVES APPLICABLE TO 1 TO 200 MGD PLANTS. EPA-600/2-79-162b, U.S. Environmental
    Protection Agency, Cincinnati, Ohio, 1979.
15.  Gumerman, R.C., R.L Gulp and S.R Hansen. ESTIMATING WATER TREATMENT COSTS: VOLUME
    III - COST CURVES APPLICABLE TO 2500 GALS PER DAY TO 1 MGD TREATMENT PLANTS.
    EPA-600/2-79-162c, U.S. Environmental Proection Agency, Cincinnati, Ohio, 1979.
16.  Lineck, T.S., R.C. Gumerman and R.L. Gulp. ESTIMATING WATER TREATMENT COSTS: VOLUME IV
    - COMPUTER USERS MANUAL FOR RETRIEVING AND UPDATING  COSTS. EPA-600/2-79-162d.
    U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
17.  Stevie, R.G., R.M. Clark and J.T. Adams. MANAGING SMALL WATER SYSTEMS: A CASE STUDY-
    VOLUME I. EPA-600/2-79-147a, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
18.  Gillean, J.I., K.W. Adams and R.M. Clark. MANAGING SMALL WATER SYSTEMS: A CASE STUDY-
    VOLUME II. EPA-600/2-79-147b, U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979.
19.  Morand, J.M., C.R. Cobb, R.M. Clark and R.G. Stevie. PACKAGE WATER TREATMENT PLANTS: A
    PERFORMANCE EVALUATION  - VOLUME I.  EPA-600/2-80-008a, U.S. Environmental Protection
    Agency, Cincinnati, Ohio (In Press).
20.  Stevie,  R.G. and R.M. Clark. PACKAGE WATER TREATMENT PLANTS: A COST EVALUATION -
    VOLUME II. EPA-600/2-80-008b, U.S. Environmental Protection Agency, Cincinnati, Ohio (In Press).

MICROBIOLOGICAL TREATMENT BRANCH       enteroviruses vary greatly in their  resistance to
  -r.         .  x  x    *   xi. ...   •-•  i   •  .   chlorine; 2) the presence of inorganic ions can
  The research strategy for the Microbiological   have prOnouneed effects on enterovirus inactiva-
TreatmentBranch.sdes.gnednotonlytosupport   tion ^ gnd a,SQ Qn  h  aggregation charac.
the  implementation of the National Interim Pn-   teristjcs of vj       3) wnNeyv9iru9s aggregation
mary Drinking Water Regulations but to begin to   can cause differences  in inactivation rates, ex-
lay  a foundation of knowledge for anticipated   treme protection from disinfectants due to ag-
revised regulations. Microbiological research to   gregation has not been observed; 4) turbidity can
support these program needs include the broad   have  major effectg Qn enterovirus and co^orm
areas of: 1) disinfection m alternative treatments;   disinfection rates, the effects being largely de-
21 water supply distnbut.on quality; and 3) meth-       dent on the t    of turbidjt   *esenat rather
ods development.                             tnan the amount
Disinfection                                   Because of its  increasing importance as  a
                                            cause of waterborne giardiasis research on the
  Final reports on  several  primarily virus-ori-   protozoan etiologic agent, Giardia lamb/ia, and
ented studies included studies on the range of   the effects of water  treatment processes, par-
resistance of enteroviruses to chlorine and stud-   ticularly disinfection, on the cysts of the
ies of the effects of various  kinds of turbidity on   organism, was initiated in 1976. Success in de-
the  resistance of viruses and bacteria to ozone   velopment of a culture method for determination
and chlorine dioxide. A  three year study of the   of Giardia cyst viability has made it possible to
effects of virus aggregation on the disinfection   conductthe disinfection studies on this organism
resistance of enterovirus, and a field study of the   currently in program. In addition to studies of G.
effects of water treatment processes on virus in-   lamblia, the species pathogenic for humans, in-
activation or removal are being completed.       house disinfection  research  on G. muris, a
  Overall, the results of these studies indicate: 1)   related species infectious for mice is being con-

66

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ducted. Reports on several aspects of this re-   widespread impression that the cysts are vir-
search are available and other reports are in   tually impossible to kill by disinfection. Our
press. The proceedings of a Symposium on Wa-   Branch participated in preparing a Report to Con-
terborne Transmission  of Giardiasis, jointly   gress on the current status of information on
sponsored by MERL and HERL also has been   viruses in water. The report, which will serve as a
published and distributed. While we do not have   guide to  Congress and the Agency in determin-
precise information on the chlorine resistance of   ing the future cause of virus research related to
G. lamblia cysts, the  information thus far de-   drinking water, has been published and
veloped indicates that the cysts can be inacti-   distributed.
vated by chlorine. This is contrary to the

RELATED RESEARCH PUBLICATIONS

 1.  Engelbrecht, R.S.,  M.J. Weber, C.A. Schmidt, and B.L Salter. VIRUS SENSITIVITY TO CHLORINE
    DISINFECTION OF WATER SUPPLIES. EPA-600/2-78-123, U.S. Environmental Protection Agency,
    Cincinnati, Ohio, 1978. 52 pp.
 2.  Scarpino, P.V., FA.O. Brigano, S. Cronier, and M.L Zink. EFFECT OF PARTICULATES ON DESTRUC-
    TION OF ENTEROVIRUSES BY CHLORINE DIOXIDE. EPA-600/2-79-054, U.S. Environmental Protec-
    tion Agency, Cincinnati, Ohio, 1979. 68 pp.
 3.  Sproul, O.J., C.E. Buck, M.A. Emerson, D. Boyce, D. Walsh, and D. Houser. EFFECT OF PARTICUL-
    ATES ON OZONE DISINFECTION OF BACTERIA AND VIRUSES IN WATER. EPA-600/2-79-089, U.S.
    Environmental Protection Agency, Cincinnati, Ohio, 1979. 86 pp.
 4.  Brigano, FA.O., RV. Scarpino, S. Cronier, and M.L. Zink. EFFECT OF PARTICULATES ON INACTIVA-
    TION OF  ENTEROVIRUSES  BY  CHLORINE DIOXIDE. In: Progress in Wastewater Disinfection
    Technology. A.D.  Venosa, ed. EPA-600/9-79-018, U.S. Environmental Protection Agency, Cincin-
    nati, Ohio, 1979. pp. 86-94.
 5.  Hoff, J.C. THE RELATIONSHIP OF TURBIDITY TO DISINFECTION OF POTABLE WATER. In: Evalua-
    tion of the Microbiology Standards for Drinking Water, C.H. Hendricks, ed. EPA-520/9-78-OOC, U.S.
    Environmental Protection Agency, Washington, D.C., 1978. pp. 103-117.
 6.  Floyd, R. and D.G. Sharp. INACTIVATION OF  SINGLE POLIOVIRUS  PARTICLES IN  WATER  BY
    HYPOBROMITE ION, MOLECULAR BROMINE, DIBROMAMINE, AND  TRIBROMAMINE. Environ-
    mental Science Technology 12:1031-1035,1978.
 7.  Young, D.C. and D.G. Sharp. PARTIAL REACTIVATION OF CHLORINE-TREATED ECHOVIRUS. Ap-
    plied Environmental Microbiology, 37:766-773,1979.
 8.  Jensen, H. and D.G. Sharp. AGGREGATION OF COXSACKIE B 5 VIRIONS. Abstract Annual Meeting
    of the American Society for Microbiology, Q60:229,1979.
 9.  Young, D.C. and O.G. Sharp. EVIDENCE FOR TWO INFECTIOUS CONFORMATIONAL STATES FOR
    ECHOVIRUS DURING CHLORINE INACTIVATION. Abstract Annual Meeting of the American So-
    ciety for Microbiology, Q(H)7:235,1979.
10.  Reach, C.D., Jr., L  Hemphill, and J.T. O'Connor. VIRUS AND BACTERIAL QUALITY OF MISSOURI
    RIVER WATER. Proceedings 1979 Annual Conference and Exposition, San Francisco, California,
    June 24-29,1979. (In press).
11. Foster, FM., M.A. Emerson, C.E. Buck, D.S. Walsh, and O.J. Sproul. OZONE INACTIVATION OF CELL
   AND FECAL ASSOCIATED VIRUSES AND BACTERIA. Journal of Water Pollution Control Federa-
   tion, 1979.  (In press)
12. Walsh, D.S., C.E. Buck, and O.J. Sproul. OZONE INACTIVATION OF HYDRATED ALUMINUM OXIDE
    FLOC ASSOCIATED VIRUSES AND BACTERIA. Journal of Environmental Engineering, American
   Society of Civil Engineering, 1979. (In press)
13. Sharp, D.G., D. Young, F  Floyd, and J.D. Johnson. EFFECT OF IONIC ENVIRONMENT ON THE
    INACTIVATION OF POLIOVIRUS IN WATER BY CHLORINE. Applied Environmental Microbiology,
   1979. (In press)
14.  Meyer, E.A. DETERMINATION OF GIARDIA CYST VIABILITY. EPA-600/2-79-063, U.S. Environmental
   Protection Agency, Cincinnati, Ohio, 1979. 35 pp.
15.  Bingham, A.K. and E.A. Meyer. GIARDIA EXCYSTATION  CAN BE INDUCED IN VITRO IN ACIDIC
   SOLUTIONS. Nature 277:301-302,1978.
16. Jakubowski, W. and J.C. Hoff. WATERBORNE TRANSMISSION OF GIARDIASIS. EPA-600/9-79-001.
   U.S. Environmental Protection Agency, Cincinnati, Ohio, 1979. 306 pp.


                                                                                  67

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17. Bingham, A.K., E.L Jarroll, Jr., E.A. Meyer, and S. Radulescu. INDUCTION OF GIARDIA EXCYSTA-
   TION AND THE EFFECT OF TEMPERATURE ON CYST VIABILITY AS COMPARED BY EOSIN EXCLU-
   SION AND IN VITRO EXCYSTATION. In:  Waterborne Transmission of Giardiasis. W. Jakubowski
   and J.C. Hoff eds. EPA-600/9-79-001,1979. pp. 217-229.
18. Hoff, J.C. DISINFECTION RESISTANCE OF GIARDIA CYSTS: ORIGIN OF CURRENTCONCEPTS AND
   RESEARCH IN PROGRESS. In: Waterborne Transmission of Giardiasis. W. Jakubowski and J.C.
   Hoff eds. EPA-600/9-79-001,1979. pp. 231-239.
19. Bingham, A.K., E.L Jarroll, Jr., E.A. Meyer, and S. Radulescu. PHYSICAL FACTORS OF EXCYSTA-
   TION IN VITRO, AND EXCYSTATION VS. EOSIN EXCLUSION AS DETERMINANTS OF VIABILITY.
   Exp. Parasitol. 47:284-291,1979.
20. Hoff, J.C., E.W. Rice, and E.E. Geldreich. INACTIVATION OF GIARDIA MURIS CYSTS BY CHLORINE.
   Abstract Annual Meeting of the American Society for Microbiology, Q55:228,1979.
21. Jarroll, E.L, A.K. Bingham, and E.A. Meyer. GIARDIA CYST DESTRUCTION:  EFFECTIVENESS OF
   SIX SMALL QUANTITY WATER DISINFECTION METHODS. American Journal of Tropical Medicine
   and Hygiene (In Press).
22. HUMAN VIRUSES  IN THE AQUATIC ENVIRONMENT: A STATUS REPORT WITH EMPHASIS ON
   THE EPA RESEARCH PROGRAM. (REPORTTO CONGRESS) EPA-579/9-78-006. U.S. Environmental
   Protection Agency, Cincinnati, Ohio, 41 pp. 1978.
Distribution System Studies

  In addition to providing effective treatment,
municipal potable water supplies must be con-
tinually alert for contamination problems in their
distribution systems and the possible occurence
of microbial degradation of water quality and
pipe integrity. The  persistence of organisms in
pipe networks is influenced by a variety of physi-
cal and chemical conditions in the water, the type
and age of pipe, and the availability of suitable
sites for colonization. These sites are often cre-
ated, in part, by corrosion, turbidity or inade-
quate treatment processes, including corrosion
control.
  Problems related to the use of corrosion con-
trol chemicals are currently being evaluated.
Often the effectiveness  of calcium carbonate or
orthophosphate as corrosion inhibitors is im-
peded  by flow characteristics, high pH or high
sulfate concentrations in the water that prevent
the formation of a uniform coating on pipe sur-
faces. Porous or irregular coatings of these so-
called "corrosion inhibitors" can actually entrap
and protect bacteria, promote tuberculation and
finally enhance corrosion rates. Use of the cor-
rect chemical at the correct dosage in any given
water supply, is essential for effective corrosion
control.
  Turbidity in finished water also  contributes to
sediment accumulations and in some cases, pro-
tects the  microbial  population from inactivation
by residual disinfectants. Research programs in-
vestigating the effects of turbidity on bacterial
survival have, in general, indicated that inorganic
particles  such as  clay and flocculating agents
may trap microorganisms, but provide little pro-
tective effect against disinfection. In contrast, cell
debris, sewage solids, or other organic particul-
ates, can provide microorganisms with protec-
tion from disinfection, an attachment site for
population growth  and a deposit of absorbed
nutrients. A striking series of electron micro-
graphs, obtained as part of our in-house effort in
this area, very graphically demonstrates bacterial
survival and protection in particulates. It appears
that microorganisms are predominantly seen at
the surface or near-surface areas, where nu-
trients and oxygen are constantly present.
  Bacterial survival and regrowth in distribution
systems is an extremely complex phenomenon
that is dependent on  many interacting condi-
tions. Most of the above mentioned studies have
been  characterizing bacterial populations that
are existing and multiplying in  finished water
distriBution systems.  How these various bacte-
rial populations affect one another is not yet
clear,  but grouping those identifiable isolates to
genera or species, does provide
useful information about the occurrence of bac-
teria that  may have pathogenic  significance or
that may interfere with coliform persistence or
isolation. One current project is studying patho-
gen survival under varying conditions in an un-
used section of a full scale  distribution system
within a military base.
  The effects of handling and storage on bacte-
rial densities in potable water samples  is being
investigated. Often, problems in shipment or
transport of samples to an examining laboratory
result in  delays exceeding the 30 hour recom-
mended time prior to  analysis. Changes in col-
iform  and standard plate count populations may
occur during this time and would directly impact
on compliance with the Drinking Water Standard.
Additionally, an attempt to  consider all of the
above processes and interactions and how they
 68

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should impact on sampling frequency in com-
pliance with the National Interim Primary Drink-
ing Water Regulations, is continuing.
  In short, microbial quality degradation of
drinking water transmitted  through distribution
systems may be minimized  with an effective dis-
infectant residual. However, this entire effort is
superfluous without a good understanding of
treatment dosages and a conscientious system
maintenance program to present the accumula-
tion of sediment and corrosion products which
provide the nutrient substrate and  protection
necessary for microbial survival.
 RELATED RESEARCH PUBLICATIONS

  1. Ridgway, H. and B.H. Olson. MECHANISMS OF CHLORINE RESISTANCE IN BACTERIAL ISOLATES
    FROM WATER DISTRIBUTION SYSTEMS. Abstracts of the Annual Meeting of the American Society
    for Microbiology, N4,1979.
  2. Reilly, J.K. and J.F Kippin. ENCAPSULATED COLIFORM - CHLORINE RESISTANT. Presented at the
    New England Water Works Association Conference, Lake Placid, September 1978.
  3. Snead, M.C., V.R Olivieri, C.W. Kruse, and K. Kawata. BENEFITS OF MAINTAINING A CHLORINE
    RESIDUAL IN WATER SUPPLY SYSTEMS. EPA-600/2-80-010, U.S.  Environmental Protection
    Agency, Cincinnati, Ohio (In Press).
  4. Allen, M.J., E.E. Geldreich, and R.H. Taylor. THE OCCURRENCE OF MICROORGANISMS IN WATER
    MAIN ENCRUSTATIONS. Presented at 7th Annual AWWA Water Quality Technology Conference,
    Philadelphia, Pennsylvania, December 1979.
Methods Development

  The agar pour plate procedure for enumeration
of the  aerobic heterotrophic bacterial  count of
water (standard plate count) is used to monitor
changes in the bacterial concentration of finished
water throughout a distribution system.
However, the pour plate procedure is limited by
the volume of sample that can be examined thus
creating a need for a procedure that would allow
examination of sample volumes larger than one
milliliter. Medium-standard plate count (M-SPC)
medium  used with  the membrane filter tech-
nique was developed to permit analysis of sam-
ple volumes ranging from decimal dilutions to
more than one liter when necessary or desired.
Though not yet acceptable as a standard method,
the m-SPC procedure generally yields  bacterial
count results equal to or greater than the stand-
ard plate count procedure. A total of 1,970 drink-
ing water samples from 50  different sampling
sites were examined by both the m-SPC and the
standard plate count procedure in order to estab-
lish comparability of the m-SPC medium with the
accepted standard method. Commercial prepa-
ration of the  m-SPC medium is available on spe-
cial request and results in a significant savings in
time and effort over preparing the medium from
individual ingredients. By permitting bacterial
plate count analysis of samples larger than the
one milliliter maximum volume used in the
standard pour plate procedure, the  number of
statistically acceptable sample results should be
increased significantly for most users.
  Development has been completed on a rapid 7-
hour test medium (m-7HrFC) for fecal coliform
bacteria. This membrane filter procedure uses a
lightly buffered lactose and mannitol based me-
dium and  incubation  at 41.5ฐC for detection of
fecal coliform  bacteria in 7-hour to 7.25-hour
m-7HrFC medium can be utilized in an emer-
gency situation to detect gross contamination of
potable water due to events such as line breaks or
cross-connections.
  The 7-hour fecal coliform test can also be used
to monitor bathing beach waters. Results  from
the 7-hour fecal coliform test can be used to
judge the  necessity for opening or closing
bathing  beaches to public use. The procedure
may also be useful for stream survey work.
RELATED RESEARCH PUBLICATIONS

 1. Taylor, R.J. and E.E. Geldreich. A NEW MEMBRANE FILTER PROCEDURE FOR BACTERIAL COUNTS
   IN POTABLE WATER AND SWIMMING POOL SAMPLES. Journal of the American Water Works
   Association, 71(7):402-405,1979.
 2. Reasoner, D.J., J.C. Blannon, and E.E. Geldreich. RAPID SEVEN-HOUR FECAL COLIFORM TEST.
   Applied and Environmental Microbiology, 32(2): 229-236,1979.
 3. Reasoner, D.J. MICROBIOLOGY-DETECTION OF BACTERIAL PATHOGENS AND THEIR OCCUR-
   RENCE. Journal Water Pollution Control Federation, 51(6):1760-1778,1979.
                                                                                    69

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4. Geldreich, E.E. MICROBIOLOGY OF WATER. Journal Water Pollution  Control Federation,
   51(6):1721-1743, 1979.
5. Allen, MJ. MICROBIOLOGY OF GROUNDWATER. Journal Water Pollution Control Federation,
   51(6):1743-1746, 1979.
6. Reasoner, D.J. and E.E. Geldreich. A NEW MEDIUM FOR THE ENUMERATION AND SUBCULTURE
   OF BACTERIA FROM POTABLE WATER. Abstracts Annual Meeting of ASM, N7:180,1979.
7. Allen, M.J. MICROBIOLOGY OF POTABLE WATERS. Journal Water Pollution Control Federation,
   51(6):1747-1751, 1979.
70

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                           INTERNATIONAL ACTIVITIES

  During 1979 the Municipal Environmental Research Laboratory (MERL)-Cincinnati received 59 for-
eign visitors representing national and local governments, industry, academic and other institutions
from 15 countries. The countries represented by these visitors and the number from each during this
period were: Japan, 15; People's Republic of China, 9; Canada, 7; Sweden, 7; England, 4; Poland, 3;
South Africa, 2; Netherlands,  2; Mexico, 2; Germany,  2; Australia, 2; and one each from Italy,
Switzerland, and Pakistan.
  These visitors were interested in all phases of work in MERL. Quite often other laboratories within the
Environmental Research Center were also visited.

Committee on the Challenges to Modern Society (CCMS)

  This NATO-sponsored committee attempts to bring together several countries in various peaceful
endeavors.  The Municipal Environmental Research Laboratory  has been involved in projects on
wastewater treatment and drinking water supply research. Dr. Robert L. Bunch, WRD, is a member of
the Advanced Wastewater Treatment Group and U.S. Representative.
  ORD's active participation in CCMS began in January 1973 and is to continue with yearly workshops
to provide various technical discussions of wastewater technology and serve to acquaint all partici-
pants with the research going on in member countries.
  Two projects were conducted,  one on advanced treatment of wastewater by physical-chemical
processes and one on the use of pure oxygen in activated sludge pilot plant at Wuppertal, Germany.
  The last meeting of the delegates was in London on June 14,1979. The final report on the Advanced
Wastewater Treatment studies done at Coleshill, England, has been completed and published as NATO/
CCMS Report No. 90.
                                                                             APAN 15
                                                                   PEOPLE'S REPUBLIC
                                                                         -OF CHINA 9
               SWEDEN 7
   _      NETHERLANDS 2
ENGLAND  4 ^GERMANY 2
             SWITZERLAND 1|POLAND  3
             ITALY 1 _^^
                          PAKISTAN  1
                                                                   AUSTRALIA
                                 SOUTH AFRICA 2
                                          71

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PUBLIC LAW (PL) 480 Projects

  Under PL 480, the U.S. is financing projects in foreign countries designed to advance scientific and
technical research that is of mutual benefit to both countries. Project Officers from MERL supervise the
following projects:
    TITLE: Water Reclamation and Useful Utilization of Sewage Solid Waste
    LOCATION: University of Karachi, Karachi, Pakistan
    GRANT PERIOD: October 1,1976 to December 21,1980
    PRINCIPAL INVESTIGATOR: Dr. M. Zain-ul-Abedin
    PROJECT OFFICER: Robert L  Bunch, MERL-Cincinnati, WRD, TPDB (Phone: 684-7655).

    TITLE: Investigations of Biodegradability and Toxicity of Organic Compounds
    LOCATION: Institute of Meterology and Water Economy, Warsaw, Poland
    GRANT PERIOD: March 1,1975 to February 28,1978, extended to February 28, 1979
    PRINCIPAL INVESTIGATOR: Dr. Eng. Jan Dojlido
    PROJECT OFFICER: Robert L.  Bunch, MERL-Cincinnati, WRD, TPDB (Phone: 684-7655).

ENGINEERS EXCHANGE PROGRAM

  Two Japanese engineers were sponsored under the auspices of the United States/Japan Environ-
mental Agreement (Sewage Treatment Technology Project) to work at the Municipal Environmental
Research Laboratory in Cincinnati, Ohio.
  Dr. Tadahiro Mori, Japan Sewage Works Agency, Today City will work in the Ultimate Disposal
Section, Wastewater Research Division from September 1,1979 through February 28,1980.
  Mr. Shunsoki, Ministry of Construction Tokyo will work at the Test and Evaluation Facility, Wastewater
Research Division from September 1,1979 through August 31,1980.

FOREIGN TRAVEL AND MEETINGS ATTENDED

Dr. Robert L. Bunch

  Monitored research project PL  480, "Investigations of Biodegradability and  Toxicity of Organic
Compounds," at Warsaw,  Poland  in May 1979. The project is now completed and the final report
published in March 1980.
  In May 1979 presented a paper,  "Pilot Plant Development of Ozone Disinfection," at Marie Curie-
Sklodowska University in Lublin, Poland.
  Participated in the 4th International Liquid Chromatography Symposium in Strasbourg, France, on
October 23-26,1979.
  In October 1979 trips were made  to Karachi and Islamabad, Pakistan, to monitor research project PL
480, "Waste Reclamation and Useful  Utilization of Sewage Solids Waste," at Univesity of Karachi.
Lectures were given on "Wastewater Treatment Processes" at University of Karachi and on "Advances
in Wastewater Treatment"  at Quaid-e-Azam University at Islamabad.

Dr. James A. Ryan

  Visited the University of  Guelph and Canada Centre for Inland Waters to discuss land application of
sludges on October 24-26,1979 in  Burlington and Guelph, Ontario, Canada.

Dolloff F Bishop

  On November 6-8, 1979 in  Toronto, Ontario, Canada attended the 33rd  meeting  of the Science
Advisory Board of the International Joint  Commission (IJC).

Edwin E. Geldreich, Jr.

  Attented a World Health  Organization Conference to develop "WHO Guidelines for Drinking Water
Quality," and served on  a Microbiological Contaminants Subcommittee on December 17-21, 1979 in
Medmenham, England.

John J. Convery

  Attended  and participated  in the International Joint Commission's (IJC) Great  Lakes  Research

72

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 Advisory Board 29th meeting on February 5-7,1979 in Windsor, Ontario, Canada.
   On May 8-10, 1979 attended and participated in the Science Advisory Board meeting in Windsor,
 Ontario, Canada.
   Attended and participated in a meeting of IJC Phosphorus Management Strategies Task Force on
 December 5-7, 1979.

 Richard I. Field

   Participate and present paper entitled "Urban Stormwater Pollution Control in the United States" at
 the Second (1979) Short Course on Urban Water Resources Workshop sponsored by the University of
 Toronto. Also reviewed on-going project at LaSalle Hydraulic Laboratory in Montreal. This trip oc-
 curred on March 12-16,1979 to Montreal and Toronto, Canada.

 Douglas C. Ammon

   Represented Storm & Combined  Sewer Section  at the EPA Storm Water Management Model
 (SWWM) meeting sponsored by the Office of Air, Land and Water and  Canadian  Ministry of the
 Environment on May 23-29,1979 in Montreal, Canada.

 James F Kreissl

   On September 15 thru October 1,1979 in Oslo and Aas, Norway; and Malmo and Stockholm, Sweden
 exchanged information on research activities on alternative systems for small communities and
 individual homes with three European countries most active in this area.

Albert D. Venosa

  Attended the International Joint Commission (IJC) Meeting of Chlorine Objective Task Force on
 March 14-15,1979 and  October 24-25,1979 in Windsor, Ontario, Canada.

Michael Roulier

  On June 3-9,1979 participated as a member of the U.S. Delegation to the NATO/CCMS Pilot Study
Meeting on "Disposal of Hazardous Wastes (Phase 2)." This participation related primarily to landfill
 research activities and required several presentations of papers discussing the current SHWRD/MERL
research activities in this overall area. The meeting was held in Vancouver, British Columbia, Canada.

Richard Carnes

  Participated in a roundtable discussion on incinerator technology for hazardous wastes on Decem-
ber 11-13, 1979 in Ottawa, Canada. This was part of a continuing coordinated  research between the
SWMB, Environmental Canada and the Disposal Branch, SHWRD/MERL.

Dirk Brunner

  From September 17 thru  October 7,1979 traveler visited London, England; Paris, France; and Zell,
Dannenberg, and Berlin, Germany. The purposes for the trip were to participate (by invitation) in an
International Roundtable Discussion on Landfilling of Municipal Waste, specifically baled refuse and
gas production; to attend an Energy and Materials Recovery International  Conference; to observe a
proposed hazardous waste disposal site near Dannenberg; and to observe solid waste management
practices in Berlin where land use is intense.

Norbert Schomaker.

  In  Munich, Germany on September 24 thru October 13,1978 participated as a member of the U.S.
Delegation at the  NATO/CCMS Pilot Study Meeting "Disposal of Hazardous Wastes  (Phase 2)" and
presented a paper which described the USEPA landfill research programs with specific emphasis on
the chemical fixation activities.
  On June 3-9,1979 participated as a member of the U.S. Delegation to the NATO/CCMS Pilot Study
Meeting on "Disposal of Hazardous Wastes (Phase 2)." This participation related primarily to landfill
research activities and required several presentations of papers discussing the current SHWRD/MERL
research activities in this overall area. The meeting was held in Vancouver, British Columbia, Canada.
  Again on October 13-21,1979 traveler attended an experts meeting of the NATO/CCMS Pilot Study on

                                                                                      73

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Hazardous Waste Disposal (Phase 2). A paper was presented describing the U.S. EPA landfill research
programs with specific emphasis on planned revisions to the current program regulations relating to
hazardous waste disposal as it relates to the Resource Conservation Recovery Act. This meeting was
held in Paris, France.

Carlton Wiles

  Represented EPA at Norchem Laboratories in Oslo, Norway in discussions about hazardous waste
encapsulation. Inspected hazardous waste emplacement into salt mines, observed technical opera-
tions, and obtained data on precautions used, waste handling procedures, and waste containerization
methods.

Haynes Goddard

  Attended a meeting of the Organization for Economic Cooperation and Development (OECD) and
met with experts on waste policy research for planning research programs for the next several years in
Paris, France, on October 3-6,1978.
 74

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                                  TECHNICAL REPORT DATA
                           (Please read Instructions on the reverse before completing)
 REPORT NO.
  EPA 600/9-80-014
                                                           3. RECIPIENT'S ACCESSION NO.
 TITLE AND SUBTITLE

  "REPORT OF PROGRESS--MERL 79"
                                    5. REPORT DATE
                                              JUNE 1980
                                    6. PERFORMING ORGANIZATION CODE
 AUTHOR(S)
                                                           8. PERFORMING ORGANIZATION REPOI
i. PERFORMING ORGANIZATION NAME AND ADDRESS
 Office of the Director
 Municipal Environmental Research Laboratory
 USEPA, 26 W. St. Clair Street
 Cincinnati, Ohio       45268
                                     10. PROGRAM ELEMENT NO.

                                         A73D1C
                                     11. CONTRACT/GRANT NO.
                                          N/A
12. SPONSORING AGENCY NAME AND ADDRESS
 Municipal Environmental Research Laboratory  -  Gin,  Ohio
 Office of Research  &  Development
 U.  S.  Environmental Protection Agency
 Cincinnati, Ohio 45268
                                     13. TYPE OF REPORT AND PERIOD COVERED
                                       Progress - 1979	
                                     14. SPONSORING AGENCY CODE

                                          EPA/600/14
15. SUPPLEMENTARY NOTES

 Contact - Diana Irwin
     (513-685-7957)
16. ABSTRACT
      The Municipal  Environmental Research Laboratory is the EPA research
 organization responsible for the development  of technology, systems,  and
 processes to control  or remove environmental  pollutants that trouble  our
 communities and municipalities.  The MERL Report of Progress will  provide
 you with updated  information about the programs of the Laboratory  in  1979.

      The report will  discuss the development  and demonstration of  cost-
 effective pollution control methods in the  areas of municipal wastewater,
 solid and hazardous wastes, public drinking water supplies, and urban
 systems management.
      Although some  of its content is technical, the report is written to be
 informative for the broader audiences in business and industry, education,
 and government, and others who are interested in the environment and  related
 fields.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                              b.IDENTIFIERS/OPEN ENDED TERMS
                                                                         c.  COSATI Field/Group
 Pollution
 Abatement
 Water Reclamation
 Wastes
Water Supply
Sewage Treatment
Water Treatment
Waste Disposal
Solid Waste  Research
Hazardous Waste Research
Drinking Water Research
Wastewater Research
13B
18. DISTRIBUTION STATEMENT

 Release Unlimited,  Upon Request
                        19. SECURITY CLASS (ThisReport)
                          UNCLASSIFIED
                           21. NO. OF PAGES
                                79
                        20. SECURITY CLASS (Thispage)
                          UNCLASSIFIED
                                                   22. PRICE
EPA Form 2220-1 (Rev. 4-77)
                                             75
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