United States Environmental Protection Agency Environmental Sciences Research Laboratory Research Triangle Park NC 27711 Research and Development EPA-600/S3-84-079 Aug. 1984 Project Summary An Evaluation of Alternative Gaussian Plume Dispersion Modeling Techniques in Estimating Short-Term Sulfur Dioxide Concentrations Thomas E. Pierce A routinely applied atmospheric dispersion model was modified to evaluate alternative modeling tech- niques that allow for more detailed source data, onsite meteorological data, and several dispersion methodol- ogies. These techniques were evaluated using hourly measured SO2 concentra- tions at fixed receptors around coal- fired power plants near Paradise, Kentucky, during 1976, and near Johnsonville, Tennessee, during 1977. A significant finding of the evaluation was that the more sophisticated models did not appreciably outperform the routinely applied models. The models using airport meteorological data performed as well as the models using onsite wind data. With the Pasquill- Gifford and Briggs dispersion schemes, small differences in model performance were observed. More substantial differ- ences occurred with models using onsite turbulence measurements. The model using Pasquill's recommenda- tions tended to overpredict peak concentrations. The models based on Draxler's and Cramer's approaches using onsite turbulence yielded mixed results, perhaps in part because the lateral standard deviation of wind direction available was the 1 -h average of 5-min values (rather than a 1 -h value), thus eliminating the longer period fluctuations that are important in estimating 1-h concentrations in addition to the shorter period fluctuations. Additional research is recommended to improve the application of onsite turbulence measurements and to provide more accurate estimates of plume trajector- ies for input to atmospheric dispersion models. This Project Summary was developed by EPA 's Environmental Sciences Re- search Laboratory, Research Triangle Park, NC. to announce key findings of the research project that is fully docu- mented in a separate report of the same title (see Project Report ordering in- formation at back). Introduction The EPA routinely uses Gaussian plume models to make decisions having important environmental and economic impacts on air quality. Despite the economic and environmental importance placed on air quality modeling, the predic- tions from dispersion models are often no better than within a factor of two of the observations. Recognizing the limitations of these models, the EPA and the Ameri- can Meteorological Society (AMS) have initiated steps to improve current modeling practices. The general consensus is that more validations of air quality simulation models are needed to improve existing models and to guide the development of future models. ------- In the current study, a Gaussian plume dispersion model incorporating alterna- tive techniques was evaluated using a comprehensive data base developed for two Tennessee Valley Authority coal- fired power plants: Johnsonville and Paradise. Alternative modeling tech- niques were included in a routinely applied Gaussian dispersion model, in- cluding different approaches for emis- sions, meteorology, and dispersion. The benchmark model from which the alternatives were developed was the MPTER algorithm. Multiple Point Gaussian Dispersion Algorithm with Optional Terrain Adjustment, an air quality simulation model that is used by EPA in regulatory applications. The MPTER was especially suited for this study because actual coordinates for each monitoring site could be specified, along with the physical separation between stacks. Furthermore, the author's in-depth experience with MPTER allowed for careful and expedient inclusion of the alternative models. Modeling Alternatives Used In modeling for regulatory applications, the design capacity or the maximum operating capacity of resulting SO2 emissions and source parameters are often required as model inputs. The daily and seasonal operating rates vary significantly at most coal-fired power plants. Furthermore, maximum surface concentrations at a power plant can occu r under less than full-load conditions. Thus, for the Johnsonville and Paradise locations, hourly S02 emissions, stack gas temperatures, and gas exit velocities were computed for comparison to full- load conditions. The meteorological data required for EPA regulatory applications are often selected from the National Weather Service (NWS) stations that are most representative of the site being modeled. In this study, the airport data from Nashville, Tennessee (BNA) were used as model inputs for the Paradise and Johnsonville sites. Evansville, Indiana (EW) surface data were also included for comparison at the Paradise site. Because the use of onsite meteorological data is preferred, the hourly average 110-m onsite wind data were used at both power plants. An accurate estimate of dispersion is critical in air quality analysis. In this regard, much effort was made in developing the alternative models in this study. The MPTER uses Pasquill-Gifford (PG) dispersion coefficients. As one alternative, Pasquill's approach for estimating buoyancy-induced dispersion (BID) was evaluated. Briggs' rural disper- sion coefficients combined with Pas- quill's1, Draxler's2, and Cramer's3 that use onsite turbulence measurements were evaluated for the Johnsonville site. A matrix of model alternatives was developed for use in Paradise in 1976 and for use in Johnsonville in 1977. These matrices are shown in Tables 1 and 2 respectively. In the development of the alternative models, an effort was made to keep each change in a technique inde- pendent of the other techniques. Accomplishments Short-term S02 concentrations were evaluated at Paradise with seven model- ing alternatives and at Johnsonville with eleven modeling alternatives. The accomplishments of this study included the following: 1) The development of two years of data (one year for Paradise and one year for Johnsonville) consisting of hourly S02 emission rates and stack characteristics, hourly S02 concen- trations monitored at ten to twelve receptor sites, hourly average onsite meteorological parameters, and hourly NWS meteorological data collected at BNA, and EW; 2) The incorporation of alternative modeling techniques into the EPA Gaussian plume dispersion model, MPTER, including modifications of MPTER to allow for the input of onsite meteorological data, the development of an algorithm for calculating dispersion using Briggs' rural interpolation formulae, and adaptations of onsite turbulence schemes using methods described by Pasquill, Draxler, and Cramer; 3) The implementation of these models using the available data on EPA's UNIVAC computer; and 'Pasquill, F. 1976. Atmospheric Dispersion Parame- ters in Gaussian Plume Modeling Part II Possible Requirements for Change in Turner Workbook Values. EPA-600/4-76-030b. Environmental Pro- tection Agency Research Triangle Park, North Caro- lina. 53 p. 2Draxler, R. 1976. "Determination of Atmospheric Diffusion Parameters."Atmos. Environ. 10: 99-105. 3Cramer, H. E. 1976 "Improved Techniques for Mod- eling the Dispersion of Tall Stack Plumes." In: Pro- ceedings of the Seventh International Technical Meeting on Air Pollution Modeling and Its Applica- tion. N. 51, NATO/CCMS Airlie House, Virginia, pp. 731-780. 4) The analysis of the model's results and observed S02 concentrations using relatively straightforward sta- tistical comparisons. Results Paradise At the Paradise plant, greater differ- ences in predicted SO2 concentrations resulted from using various emissions data than from using alternative disper- sion schemes and meteorological data. Furthermore, the "conservative"full-load emissions models compared more favor- ably to peak observed concentrations than the "more realistic" models using hourly emissions data, which underpre- dicted peak concentrations by about a factor of two. This unexpected result was attributed to inaccuracies associated with estimating stability, mixing heights, wind vectors, and/or S02 emission rates. Another unexpected feature of the Paradise analysis was that the models incorporating onsite wind data did not show significant improvements over the models using airport meteorological data. Although the concentrations from the two modeling alternatives differed hour to hour, the overall results, especially for the peak concentrations, were similar. Although emissions input and meteorological data have been recognized as having important effects in dispersion modeling, dispersion schemes are usually discussed as a primary basis for model differences. The concentra- tions predicted with the three dispersion schemes at Paradise, however, resulted in average differences of less than 10 percent. Buoyancy-induced dispersion did seem to increase concentrations with the models using the Briggs and PG dispersion coefficients, although the Briggs coefficients potentially can yield lower concentrations for downwind distances up to two kilometers. Furthermore, measurements taken from receptors closer to the source than those located at Paradise should be examined for comparison with the Briggs and PG curves. Johnsonville With the 11 Johnsonville alternative models, the principal emphasis was on the prediction of peak concentrations, especially the concentrations related to the National Ambient Air Quality Stand- ards for SO2. Some additional analyses were used to diagnostically evaluate the models. The significant differences between the emissions data alternatives that were ------- Table 1. Modeling Alternative Matrix Used for Paradise Model Number Technique Emissions input Full-load conditions Hourly averages Meteorology input BNA airport data EVV airport data Onsite wind data Dispersion scheme PG PC with BID Briggs formulae with BID Table 2. Mode/ing Alternative Matrix for Johnsonville Model Number Technique 2 3 10 11 Emissions input Full-load conditions Daily averages Hourly averages Meteorology input BNA airport data BNA, exclude calms Onsite wind data Dispersion scheme PG PG with BID Briggs with BID Pasquill's 1976 scheme Draxler's scheme Cramer's scheme XXXXXXXX X X X X X X noted in the Paradise analysis were not evident in the Johnsonville analysis. In fact, the models using full-load emissions data compared similarly to the models using hourly and daily emission data for the peak concentrations. The differences between the models using daily and hourly emissions data seemed insignifi- cant; in retrospect, it probably would have been more cost effective to use the daily emission rates rather than the hourly emission rates. The similar performance noted for the models using full-load, daily, and hourly emission rates may have been due to the increased plume rise associated with full-load stack parameters, which would cause a reduc- tion in maximum surface concentrations. It appeared that the procedure to elim- inate calm winds had little effect on peak concentrations. At other power plant sites where the receptors are located closer to the source and where A- and B- stability has a greater effect on peak concentrations, the elimination of calm winds might be an important consideration. As with Paradise, little additional bene- fit was gained by using onsite wind data in preference to airport data. This is probably because the airport site, BNA, and the Johnsonville site are similar in topography. In the diagnostic evaluation, the model using onsite wind data did show better performance over the airport model, resulting in higher correlations and mean fractional errors closer to zero. The differences between the models using different dispersion schemes were again small in contrast to the differences noted with the emission and meteorolog- ical alternatives. In predicting the peak concentrations, the three basic disper- sion models (PG, PG with buoyancy- induced dispersion, and Briggs) performed about equally. The models using on-site turbulence data, however, did not perform as well as expected. The Pasquill scheme overpredicted most peak concentrations. The modeling alternatives using the Cramer and Draxler dispersion schemes gave results that were comparable to the models using the PG curves but differed substantially, on occasion, from the observations. Because the Cramer and Draxler models limited dispersion during nighttime hours, further work is needed to develop a scheme to practically estimate dispersion using routine meteorological measurements during all meteorological regimes.' In this study, the PG model appeared to perform as well as the other dispersion schemes. Conclusions and Recommendations In studies of this kind, the results often suggest a need for improving modeling techniques and for obtaining more so- phisticated input data. This study did not deviate from this tradition. The alterna- tive modeling approaches used with the Johnsonville and Paradise plants yielded results that were within an order of magnitude of the peak SO2 concentra- tions. Yet, further improvements are possible with more accurate source term data, more site-specific meteorological data, and more refined dispersion schemes. The major differences in model per- formance resulted from differences in emission rates and to a lesser extent from the use of different meteorological data. The use of alternative dispersion schemes was not as significant. However, efforts to improve the measure- ments of the standard deviations of horizontal and vertical wind direction (as well as other turbulence parameters) could provide a more reliable means for estimating dispersion. The task of model evaluation in this study was especially onerous, because slight differences in predicted plume trajectories overwhelmed the statistical comparison used to examine the alternative modeling approaches. This further substantiates the observation that the Gaussian plume dispersion model is especially sensitive to the input of wind direction. Model evaluations could perhaps be simplified by following the advice of Calder and Johnson, i.e., that each model component be separately evaluated. Otherwise, it is difficult to compare the strengths and weaknesses ------- of different modeling techniques. The difficulty in performing model evaluation is further compounded by lack of field data. The availability of field data from studies such as Cinder Cone Butte, Idaho, and Kincaid, Illinois, will hopefully make the tasks of model evaluation and model improvement less formidable. The EPA author Thomas £. Pierce was on assignment to the Environmental Sciences Research Laboratory, Research Triangle Park, NC 27711 from NOAA, U. S. Department of Commerce {presently with NUS Corporation, Gaithersburg, MD). D. Bruce Turner is the EPA Project Officer (see beiow). The complete report, entitled "An Evaluation of Alternative Gaussian Plume Dispersion Modeling Techniques in Estimating Short-Term Sulfur Dioxide Concentrations," (Order No. PB 84 -223 62 7; Cost: $16.00, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield. VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Environmental Sciences Research Laboratory U.S. Environmental Protection Agency Research Triangle Park, NC 27711 US GOVERNMENT PRINTING OFFICE, 1984—759-015/7775 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati OH 45268 Official Business Penalty for Private Use $300 T i' T t- I -, X A n Y ' ' i n 'I S T N i f i t I ------- |