United States Environmental Protection Agency Environmental Sciences Research Laboratory Research Triangle Park NC 27711 Research and Development EPA-600/S3-84-087 Sept. 1984 Project Summary Evaluation of the Pollution Episodic Model Using the RAPS Data William R. Pendergrass and K. Shankar Rao The Pollution Episodic Model (PEM) is an urban-scale model capable of pre- dicting short-term average ground- level concentrations and deposition fluxes of one or two gaseous or particu- late pollutants at multiple receptors. The two pollutants may be nonreac- tive, or chemically coupled through a first-order chemical transformation. Up to 300 isolated point sources and 50 distributed area sources may be con- sidered in the calculations. Concentra- tion and deposition flux estimates are made using the hourly mean me- teorological data. Up to a maximum of 24 hourly scenarios of meteorology may be included in an averaging period. This report describes an evaluation of the PEM that used data from the St. Louis Regional Air Pollution Study (RAPS). This evaluation was designed to test the performance of the model by comparing its concentration esti- mates to the measured air quality data by using appropriate statistical meas- ures. Twenty days, ten summer and ten winter, were selected from the RAPS data base for the PEM evaluation. The model's performance was judged by comparing the calculated 12-h average concentrations with the corresponding observed values for five pollutant species: SO2, fine and course sulfates, and fine and coarse total mass. A first- order chemical transformation of SO2 to fine sulfate was considered in the calculations in addition to the direct emission and dry deposition of all five pollutants. For the twenty PEM evaluation days, PEM predicted average concentrations of SO2, and fine and coarse sulfates to within a factor of two. The model over- predicted the average concentrations of fine and coarse total mass by a factor of three to four over the evaluation period. This was attributed primarily to overestimation of emission rates and incorrect location of area sources, which dominate the fine and coarse total mass emission. Other possible sources of errors in the calculations are listed and discussed. This Project Summary was de- veloped by EPA's Environmental Sci- ences Research Laboratory, Research Triangle Park, NC, to announce key findings of the research project that is fully documented in a separate report of the same title (see Project Report or- dering information at back). Introduction The Pollution Episodic Model (PEM) is an urban-scale model capable of pre- dicting short-term ground-level concen- trations and deposition fluxes of one or two gaseous or particulate reactive pol- lutants in an urban environment with multiple point and area sources. It is in- tended for studies of the atmospheric transport, transformation, and deposi- tion of acidic, toxic, and other pollutants in urban areas to assess the impact of existing or new sources or source mod- ifications on air quality, and for urban planning. The effects of dry deposition, sedimentation, and a first-order chemi- cal transformation are explicitly ac- counted for in PEM. This report describes an evaluation of the PEM that uses the St. Louis Reg- ------- ional Air Pollution Study (RAPS) data. This evaluation was designed to test the model's performance by comparing its concentration estimates to the mea- sured air quality data by using several standard statistical measures of perfor- mance. Twenty days, ten summer and ten winter, were selected from the RAPS data base for the PEM evaluation. The model's performance was judged by comparing the calculated average con- centrations with the corresponding ob- served values for the following five pol- lutant species: SO2, fine sulfate, coarse sulfate, fine total mass, and coarse total mass. In these species, the cut-off size between fine and coarse particle frac- tions was 2.5 |j.m. A first-order chemical transformation of SO2 to fine sulfate was considered in the calculations in addition to the direct emission and dry deposition of all five pollutants. Data Base Twenty days, ten summer and ten winter, were selected from the RAPS data base by the U.S. Environmental Protection Agency (EPA) for the PEM evaluation. Detailed emission inven- tories of the RAPS region and meteorol- ogy and concentration measurements corresponding to these evaluation days were supplied by the EPA from the RAPS data base. Hourly area and point source emis- sion inventories for a typical winter day and a typical summer day for the St. Louis metropolitan area were supplied by the EPA on two magnetic tapes. The emission inventories were supplied on a numerical grid with a fixed origin at XUTM = 710 km and YUTM = 4250 km, which extended to 60 km in both x and y directions. The size of each emission grid cell for area sources was 5x5 km, thus giving 144 emission squares in the grid. Data tapes contained information on SO2, sulfate, total paniculate mass emissions, and the particle size derived from the 1976 RAPS Emission Inven- tory. An average conversion rate of 1.85% of S02 emissions was used to es- timate the sulfate emission rates for both area and point sources from the known information on SO2 emission, provided particulate emissions existed. in the case of point sources with no par- ticulate emissions, but relatively large S02 emissions, the sulfate emissions were calculated on the assumption that in a short period of time, the conversion of SO2 to SO3 occurs and contributes to 2 the total mass in the region of interest. However, in the case of area sources, the SO2 emissions were relatively small (3% of total SO2 emissions); therefore, sulfate emissions could be neglected if there were no associated particulate emissions. The size distributions of sulfate parti- cle emissions from area and point sources were more difficult to estimate. Approximate base size distributions of sulfate for typical winter and summer days were determined. Based on other studies, about 50% of the sulfate was assigned to the size range less than 0.25 |o,m for the summer aerosol, and ap- proximately 25% of the sulfate was as- signed to this size range for winter aerosol. The base size distributions ap- proximated were then used to estimate the sulfate size distributions in the area and point sources by relating the total particulate emissions (with associated size spectrum) from these sources to sulfate emissions. Hourly measurements of wind speeds and directions, and tempera- tures from the 25 station Regional Air Monitoring System (RAMS) network were supplied by the EPA. Input files contained urban mixing heights, wind speeds and directions, atmospheric sta- bility class, and temperatures: the input winds were RAMS network resultant winds. The stability classifications were supplied in the format required by PEM (i.e., stability classes 1-7). Data tapes containing the observed gas concentration values from the RAMS network, corresponding to the twenty evaluation were provided. Sepa- rate files of high-volume and dichoto- mous sampler data were also provided. The data files were scanned for hourly average SO2 concentrations, and 12-h average concentrations of total mass and total sulfur. The observed gaseous total sulfur concentrations were used to approximate SO2 concentrations at the RAMS stations where the latter were not measured. The high-volume and dichotomous sampler data contained total sulfur and total particulate mass concentrations in |j,g/m3. The particu- late data were further divided into fine and coarse categories based on a cut- off size of 2.5 jj,m. The total sulfur mea- surements were multiplied by a factor of three (the ratio of the molecular weight of SO4 to the molecular weight of sulfur) to obtain the equivalent total sulfate concentrations. Concentration measurements were not made at all of the 25 RAMS stations. The observed S02 concentrations are 1- h average values. The total sulfur and total mass concentrations measured by eight out of the ten reporting RAMS sta- tions were 12-h average values; only stations 103 and 105 recorded 6-h aver- ages. To facilitate comparison with the model calculations, the observed con- centrations of SO2, fine and coarse sul- fates, and fine and coarse total mass were converted into 12-h averages. This procedure gave two (12-h average) ob- served concentrations per day for each of the five pollutants. Model Evaluation Results PEM concentration predictions were evaluated against the measured con- centrations for five pollutants: SO2, fine particulate sulfate, coarse particulate sulfate, fine particulate total mass, and coarse particulate total mass. These five quantities were calculated in three model runs that used different sets of input data. It was assumed that SO2 chemically transforms into fine sulfate at a constant rate, and there is no con- tribution to coarse sulfate concentra- tions from this transformation. A chemical transformation rate of SO2 to fine particulate sulfate of 5% per hour was used. This value was held constant throughout the model runs re- gardless of meteorological and other conditions. Deposition (Vd) and gravitational settling (W) velocities were varied de- pending on the pollutant in each model run. For example, Vd was 2.0 cm/s and W was assumed to be zero for SO2. No attempt was made to vary them by the atmospheric stability class or other meteorological conditions. PEM uses a fixed calculation and re- ceptor grid system. A grid system was designed such that PEM receptors either matched or formed a grid around the actual RAMS network stations. For point comparisons with the RAMS net- work stations, the four receptors in the grid squares around the RAMS station were summed and their average was assigned to the RAMS station location. The numbers of point sources in this evaluation were 286 in winter and 275 in summer, thus nearly utilizing the maximum capacity of the model of 300 point sources. For point source calcula- tions in this evaluation, a modification was made to the PEM program such that concentrations were calculated only for the receptors surrounding each RAMS station and not at the rest of the receptors. This required calculation o' ------- only 84 out of a total of 2500 receptors. The model performance was evaluated by using several statistical measures. Two general measures of performance were used here: a) measures of differ- ence, which included bias, variance, gross variability or root mean squared error (RMSE), and average absolute gross error; b) measures of correlation paired in space and time. The ratio of the calculated (P) and ob- served (0) means for SO2, P/O, was 1.24, and the ratio of the corresponding standard deviations was 1.12. However, the correlation coefficient was only 0.23 over the compared range (6.5 - 250 jj,/ m3) of concentrations. This suggests a large degree of randomness in the indi- vidual case-by-case comparisons of SO2 concentrations. The differences D, between observed and calculated SO2 concentrations showed a clear bias for PEM to overpredict observed concen- trations less than 75 |xg/m3 and under- predict observed concentrations greater than about 125 (xg/m3. The bias D over the entire evaluated range of SO2 concentrations was -12.8 |o,g/m3. Thus, PEM was conservative, with a tendency to slightly overpredict the av- erage SO2 concentrations. The average absolute gross error IDI was 48.5 |xg/ m3, which was less than the mean of observed concentrations. Therefore, on the average, PEM predictions are within a factor of two of the observed SO2 con- centrations. For fine sulfate concentrations, P/O was 1.1 and the ratio of the correspond- ing standard deviations was 1.2. The correlation coefficient was 0.41 over the compared range (1 to 30 (xg/m3) of the concentrations. The model tended to overpredict O, < 18 ^g/m3 and under- predict O, > 20 |j,g/m3. The bias D over the entire range of concentrations was -1.0 jxg/m3, (i.e., the model is slightly conservative). The average absolute gross error IDI was 4.8 jxg/m3, which was much less than the mean of ob- served concentrations. Therefore, aver- aged over the entire data base, PEM cal- culations of fine sulfate concentrations were within a factor of two of the cor- responding observed values. Coarse sulfate (particle size ^ 3 ^m) concentrations from the model evalua- tion results for direct emissions of sources only were low (generally less than 3 |j,g/m3). The ratio of the means of calculated and observed values of concentrations, P/O, was 0.52, and the ratio of the corresponding standard de- viations was 0.9. The correlation coeffi- cient was 0.38 over the compared range of concentrations. The model slightly underpredicted the concentrations, with a bias of D = 0.5 n-g/m3 and an average absolute gross error of 0.66 |xg/ m3. The latter was 59% of the mean of observed concentrations. Thus, on av- erage, the calculated coarse sulfate con- centrations were within about a factor of two of the corresponding observed values. The model performed some- what better in winter than in summer. The results clearly showed that PEM overpredicted fine total mass concen- trations. The observed concentrations were less than 80 |xg/m3, but the corres- ponding calculated values ranged up to 300 |xg/m3. The larger calculated con- centrations were generally associated with weak diffusion conditions charac- terized by strong stabilities, low wind speeds, and shallow mixing depths that were typical of several of the winter evaluation days. The ratio of the means, P/O, was 3.1 and the ratio of the corres- ponding standard deviations was 6.0. The model significantly overpredicted the concentration, with a bias of D = -70.8 jjig/m3 and an average absolute gross error of 72.1 |o,g/m3, which was 2.1 times the mean of observed concen- trations. The model overpredicted con- centrations at stations within the city by a factor of three or less, and accurately modeled the two outlying stations. The model evaluation results for coarse total mass (particle size ^ 3 |^m) concentrations were qualitatively simi- lar to those obtained for fine total mass evaluation. Conclusions This report described an evaluation of PEM that used twenty days of data from the St. Louis RAPS. This evaluation was designed to test the model performance by comparing its concentration esti- mates for five pollutants to the mea- sured air quality data by using appro- priate statistical measures of perfor- mance. For the twenty evaluation days, PEM predicted average concentrations of S02 and fine and coarse sulfates to within a factor of two. The model over- predicted the average concentrations of fine and coarse total mass by a factor of three to four over the evaluation period. The significant differences between the calculated and observed total mass concentrations may be attributed to a number of reasons: 1. Hourly point and area source emis- sion inventories were available for only one winter day and one sum- mer day. These inventories were further averaged over two 12-h periods per day for use as input to PEM. Analysis of the emission inven- tories indicated a core of steady emission sources with various other area and point sources coming on or off line throughout the modeling period. Running PEM on an hour-by- hour basis might account for this variability of emissions but the mod- eling costs would be prohibitive. De- spite this variability, both fine and coarse sulfates were predicted to within a factor of two for the total means as well as across the 12-h av- eraging period. However, the vari- ability in emissions appears to be very important for fine and coarse total mass, because these emission rates were significantly larger and dominated by ground-level sources. 2. Point sources dominated the emis- sions of SO2 and fine and coarse sul- fates. Area sources dominated the emissions of fine and coarse total mass, and the sulfate components of fine and coarse total mass emissions from area sources were negligible compared to the nonsulfate compo- nents. The nonsulfate total mass consisted of fugitive dust, highway, residential, commercial, industrial, and other particulate emissions of different sizes that were difficult to estimate accurately. No information is available on the variability of these emissions. Any errors involved m the estimation and location of these sources would significantly affect the calculated concentrations due to the relatively large emissions from area sources. 3. Because of the 12-h averaging for periods 00-12 and 13-24 h, little can be said about the diurnal variation of model performance in this evalua- tion. There were also significant dif- ferences between the first and sec- ond averaging periods in the mean residuals of fine and coarse total mass. This may have been as- sociated with the diurnal variability of area source emissions of these species and with errors in stability classification. The first 12-h averag- ing period was generally charac- terized by stable conditions, with weak diffusion conditions. Hence, the calculated concentrations and re- siduals were larger for this period. ------- 4. Constant deposition and settling ve- locities and transformation rates were used throughout the 12-h av- eraging period. This ignores the de- pendence of these variables on meteorological conditions such as wind, humidity, and thermal stratifi- cation. Also, using one constant set of values for deposition and settling velocities to describe the broad parti- cle size spectrum ^ 3 i^m may not accurately represent the behavior of particles of different sizes. 5. The wind speed and direction input to PEM were the RAMS network re- sultant values These are approxima- tions to real conditions. Errors in wind direction may cause the model to affect particular receptors that may be completely ignored in real- ity. An underestimation of the actual wind speed leads to overprediction of the calculated concentrations. Additional effort should be directed toward an examination of the model's response to emission variability, stabil- ity classification, and area source emis- sions and location. Experience has shown that area sources are the pri- mary determinant in modeling urban ground-level concentrations of nonsul- fate particulate matter. William R. PendergrassandK. ShankarRaoare with Atmospheric Turbulence and Diffusion Division, National Oceanic and Atmospheric Administration, Oak Ridge, JN 37830 Jack H. Shreffler is the EPA Project Officer (see below) The complete report, entitled "Evaluation of the Pollution Episodic Model Using the RAPS Data." (Order No PB 84-232 537; Cost. $10.00, subject to change) will be available only from. National Technical Information Service 5285 Port Royal Road Springfield, VA22161 Telephone. 703-487-4650 The EPA Project Officer can be contacted at. 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