EPA-450/4-87-002
Analysis and Evaluation of Statistical
       Coastal Fumigation Models
                          By

                      S. SethuRaman

          Department of Marine, Earth and Atmospheric Sciences
                 North Carolina State University
                   Raleigh, NC 27695-8208
                     EPA Project Officer
                      Jawad S. Touma
             U.S. ENVIRONMENTAL PROTECTION AGENCY
                   Office of Air and Radiation
              Office Of Air Quality Planning and Standards
                 Research Triangle Park, NC 27711
                   »

                       February 1987

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                                         DISCLAIMER
This report has been reviewed by the Office of Air Quality Planning And Standards, U.S. Environmental
Protection Agency, and approved for publication as received from the contractor. Approval does not signify
that the contents necessarily reflect the views and policies of the Agency, neither does mention of trade
names or commercial products constitute endorsement or recommendation for use.

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                      Table of Contents

LIST OF TABLES 	    V

LIST OF FIGURES 	  vii

LIST OF SYMBOLS 	   xi

SUMMARY 	    1

1.0 INTRODUCTION 	  1-1

2.0 THE THERMAL INTERNAL BOUNDARY LAYER 	  2-1

    2.1 TIBL Dynamics 	  2-1
    2.2 Review of the TIBL Height Prediction
        Equations 	  2-6
    2.3 Impact of TIBL Variation on Coastal
        Dispersion 	*	 2-17

3.0 COASTAL DISPERSION MODELING 	  3-1

    3.1 The Mechanics of Fumigation 	  3-1
    3.2 The Lyons and Cole (1973) Model 	  3-4
    3.3 The CRSTER Shoreline Fumigation
        Model (CSFM)  	  3-8
    3.4 The Misra Shoreline Fumigation
        Model (MSFM)  	 3-14
    3.5 Empirical Modification to MSFM	 3-18
    3.6 Downdraft Modification of the MSFM Model 	 3-22

4.0 BRIEF REVIEW OF COASTAL DISPERSION STUDIES 	  4-1

    4.1 Nanticoke (NEMP) Study -- General Description   4-3
    4.2 Nanticoke Plant Characteristics 	  4-3
    4.3 NEMP Instrument Deployment - Boundary
        Layer Measurements 	  4-4
    4.4 NEMP Instrument Deployment - Plume
        Characteristics and Air Quality Measurements    4-8
    4.5 Data Requirements for  Running the Models 	 4-10

5.0 COASTAL DISPERSION MODEL EVALUATION PROTOCOL 	  5-1

    5.1 Brief Overview of Model Evaluation Techniques   5-1
    5.2 Statistical Evaluation Protocol 	  5-4

6.0 THERMAL INTERNAL BOUNDARY  LAYER EQUATION
    EVALUATION 	  6-1

    6.1 The Brookhaven Coastal Meteorology
        Experiments 	   6-3

                             iii

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    6.2 The Kashimaura Coastal Meteorology
        Experiments 	    6-4
    6.3 The Stable Upwind Overwater Case 	    6-8
    6.4 The Unstable Upwind Overwater Case 	   6-11
    6.5 Evaluation of TIBL Equations 	   6-18
    6.6 Analysis by Wind Category 	   6-22
    6.7 Analysis by Stability Category 	   6-26

7.0 COASTAL DISPERSION MODEL EVALUATION 	    7-1

    7.1 Overall Evaluation 	    7-1
      7.1.1 Results 	    7-1
      7.1.2 Discussion of Results 	    7-9
    7.2 The June 1, 1978 Case	   7-18
    7.3 The June 6, 1978 Case 	   7-31
    7.4 The June 13, 1979 Case 	   7-45
    7.5 The June 14, 1979 Case 	   7-48
    7.6 Sensitivity Analysis 	   7-50

8 . 0 CONCLUSIONS	    8-1

9 . 0 RECOMMENDATIONS 	    9-1

10.0 REFERENCES 	   10-1

11.0 APPENDIX 	   11-1
                              IV

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                       LIST OF TABLES


4.1         Input factors for the CSFM and MSFM base
            models 	  4-13

5.1         Test cases used for model comparison 	  5-11

6.1         Listing of TIBL data bases 	   6-2

6.2         TIBL parameters used for BNL data base ...   6-6

6.3         TIBL parameters used for Kashimaura data
            base 	   6-9

6.4         BNL #13 meteorological data 	  6-10

6.5         BNL #6 meteorological data 	  6-14

6.6         Comparison of h vs h + hQ TIBL values ....  6-16

6.7         Statistical results of non-categorized
            TIBL predictions 	  6-19

6. 8a        Statistical results of wind categorized
            TIBL predictions (Ul) 	  6-24

6.8b        Statistical results of wind categorized
            TIBL predictions (U2) 	  6-25

6.9a        Statistical results of stability
            categorized TIBL predictions (Si)  	  6-28

6.9b        Statistical results of stability
            categorized TIBL predictions (S2)  	  6-30

6.9c        Statistical results of stability
            categorized TIBL predictions (S3)  	  6-31

6. 9d        Statistical results of stability
            categorized TIBL predictions (S4)  	  6-33

7.1         Statistical results of overall model
            performances 	   7-7

7.2         Statistical results of model performances
            for June 1, 1978 	  7-30

7.3         Location of maximum downwind concentration
            for June 6, 1978 	  7-44
                              v

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7.4         Statistical results of model  performances
            for June 6, 1979	  7-46

7.5         Statistical results of model  performances
            for June 13, 1979	  7-49

7.6         Statistical results of model  performances
            for June 14, 1979 	  7-52
                             vx

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                       LIST OF FIGURES
2.la        Category I TIBL case with stable overwater
            stability 	  2-4

2.1b        Category II TIBL case with neutral
            overwater stability 	  2-4

2.2         Historical flowchart of TIBL prediction
            equation development 	  2-8

2.3         Impact of TIBL variation upon location of
            downwind maximum concentration 	 2-19

3.1         Vertical plume geometry of Lyons and Cole
            (1973) model 	  3-6

3.2         Plume geometry of CSFM model 	 3-10

3.3         Flowchart of CSFM model 	 3-15

3.4         Flowchart of MSFM model 	 3-19

4.1         Deployment map of the various measuring
            systems of the NEMP study 	  4-5

4.2         Cross-sectional deployment diagram  of the
            NEMP boundary layer sensing systems 	  4-6

4.3         Cross-sectional deployment diagram  of the
            NEMP air quality measuring systems  	 4-11

5.1         Hypothetical model output graph showing
            deceptively perfect correlation 	  5-5

6.1         Map of Long Island showing flight tracks
            for TIBL experiments 	  6-5

6.2         Map of Kashimaura-Kujukurihama, Japan
            TIBL experiment area 	  6-7

6.3         Graph of observed vs predicted TIBL height
            for BL #13	 6-12

6.4         Sounding for BL #6 	 6-15

6.5         Graph of observed vs predicted TIBL height
            for BL #6 	 6-17

7. la        Scatterplots for the MSFM model 	  7-2

                             vii

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7.1b        Scatterplots for the CSFM model 	   7-3

7.1c        Scatterplots for the empirical model 	   7-4

7.Id        Scatterplots for the downdraft model 	   7-5

7.2         Plume-TIBL relationship for June 1,  1978   7-20

7.3a        Concentration isopleths for June 1,  1978
            (0900-1000 EOT) 	  7-21

7.3b        Concentration isopleths for June 1,  1978
            (1000-1100 EOT) 	  7-22

7.3c        Concentration isopleths for June 1,  1978
            (1130-1200 EOT) 	  7-23

7.3d        Concentration isopleths for June 1,  1978
            (1230-1300 EDT) 	  7-24

7.3e        Concentration isopleths for June 1,  1978
            (1330-1400 EDT) 	  7-25

7.3f        Concentration isopleths for June 1,  1978
            (1430-1500 EDT) 	  7-26

7.3g        Concentration isopleths for June 1,  1978
            (1530-1600 EDT) 	  7-27

7.3h        Concentration isopleths for June 1,  1978
            (1630-1700 EDT) 	  7-28

7.4         Plume-TIBL relationship for June 6,  1978   7-33

7.5a        Concentration isopleths for June 6,  1978
            (0900-1000 EDT) 	  7-35

7.5b        Concentration isopleths for June 6,  1978
            (1000-1100 EDT) 	  7-36

7.5c        Concentration isopleths for June 6,  1978
            (1300-1400 EDT) 	  7-37

7.5d        Concentration isopleths for June 6,  1978
            (1400-1430 EDT) 	  7-38

7.5e        Concentration isopleths for June 6,  1978
            (1500-1530 EDT) 	  7-39

7.5f        Concentration isopleths for June 6,  1978
            (1530-1600 EDT) 	  7-40

                            viii

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7.5g        Concentration isopleths for June 6,  1978
            (1600-1630 EOT)	 7-41

7.5h        Concentration isopleths for June 6,  1978
            (1630-1700 EDT-) 	 7-42

7.6         Graph of model results for 1200 EOT
            June 6, 1978 	 7-43

7.7         Plume-TIBL relationship for June 13,  1979  7-47

7.8         Plume-TIBL relationship for June 14,  1979  7-51

7.9         w*/U sensitivity analysis with normalized
            concentration 	 7-55

7.10        "A" sensitivity analysis with normalized
            concentration 	 7-56

7.11        FQ sensitivity analysis with normalized
            concentration 	 7-58

7.12        Brunt-Vaisalla frequency (N) sensitivity
            analysis with normalized concentration ... 7-60
                             IX

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                       LIST OF SYMBOLS


a   = temperature gradient upwind (K m  )

A   = TIBL factor containing physics needed for TIBL
      parameterization (generally ranges from 2 to 6)

A(t) = fraction of fumigant entrained into TIBL with
       respect to time (MSFM/empirical variation)

C   = concentration (PPB, PPM, p-g m~^)

C   = non-dimensional concentration
                                           f
Cp  = specific heat at constant pressure (0.24 cal g~*K

Cg  = concentration in stable air (PPB, PPM, /*g m~^)

Cu  = frictional coefficient  (dimensionless)

C.  = heat coefficient  (dimensionless)
 o
DL  = length of day

d   = index of agreement value, also stack diameter (m)

E   = heat emission rate

EV  = gas volume emission rate (m^s~*)

F   = entrainment fraction

Fe  = entrainment flux

FQ  = buoyancy parameter (ITKS~^)

f~L  = function used in describing TIBL turbulence

g-^  = function used in describing TIBL turbulence

Hc  = 20% of the solar constant (W m~2)

He  = effective stack height (m)

HQ  = heat flux (W m~2)

HS  = stack height (m)

h   = TIBL interface height (m)
                             XI

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h^  = mean TIBL height (m)

ho  = initial TIBL interface height under neutral or
      unstable overwater conditions

Kx „ = eddy diffusivity

k   = von Karman's constant

N   = Brunt-Vaisalla frequency (s"-*-)

0   = observed value

P   = predicted value
                                  f
p   = a function used in Lyons and Cole model

P!  = stack height atmospheric pressure (mb)

Q   = source strength (g s~*)

Q-  = mass of plume segment in CRSTER Shoreline Fumigation
      Model  (g s"1)

r   = correlation coefficient
 9
r   = coefficient of determination

S   = 30/3z  potential temperature gradient overwater
             (K/lOOm)

SQ = standard deviation of observed values

Sp = standard deviation of predicted values
 2
SQ = variance of observed values

Sp = variance of predicted values

T   = air temperature (K)

TA  = average temperature in TIBL (K)

TL'^L = temperature at 2 m above land surface (K)

TS  = stack gas temperature  (K)

TW,0W = temperature at water surface (K)

T1  = air temperature at stack height (K)
                             xn

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t   = time (s)

ts  = time since sunrise (s)

t   = non-dimensional time

tf  = non-dimensional time at final fumigation point

Um  = mean wind speed in TIBL (m s~*)

Ue  = mean wind speed at stack height in stable air (m s~
 o

U^Q = mean wind speed at 10m (m s"-"-)

u*  = friction velocity (m s"1-)

Vf  = gas exit velocity (m s~^)

V_  = stack gas velocity (m s"1)
 o

w^  = downdraft velocity (m s~^)

we  = entrainment velocity (m s~"*)

w*  = convective velocity scale (m s~l)

(w'0')i = heat flux at TIBL height (W m~2)

(w'fl')0 = heat flux at surface (W m~2)

x,X = downwind distance from shoreline (km)

XB  = downwind distance where fumigation begins (m)
      (Lyons and Cole)

xE'xf = en<^ °^ fumigation downwind (Lyons and Cole, MSFM)

XQ  = location of where pollutants begin entraining into
      the TIBL (MSFM model)

xQ  = location of TIBL perturbation [Lyons et al.  (1983)
      TIBL model]

XQ  = virtual point source location (Lyons and Cole
       model)

X   = non-dimensional distance

Y   = lateral distance (m)

z   = height (m)

                            xiii

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Zs  = stack height (m)

Z'  = Z/h

a   =s constant (Equation 2.13)

Ahg = plume rise (m)

A0  = change in potential temperature overwater from 10 m
      above the water to base of the inversion (K)

A0Q = inversion (K)

 7  = lapse rate OT/8z) overwater (K/lOOm)

 f  = solar insolation factor

 p  = density of air  (1.2 x 10"^ g m~^)

 «r  = lateral dispersion coefficient (generic) (m)

 <* f(x,s) = lateral dispersion coefficient in fumigation
            zone (m)

 ffyf .  .  = same as  a f(x,s) but represents'individual
    1^    dispersion coefficient for the plume segment

 vvh = dispersion coefficient in TIBL (MSFM model)

 
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                      Acknowledgements


     The author would like thank R.  Lee and J.  Dicke of
OAQPS/EPA for the helpful discussions and their support for
this project.
     This report is based on material used to fulfill the
requirements for a Master of Science degree at the North
Carolina State University for Mr. M.J. Stunder.  His
dedication and enthusiasm for this study were a major factor
in its successful completion.  Finally appreciation is
extended to Suzanne Viessman who performed much of the
technical editing and organization of this report.
                             xv

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                         Summary





     Fumigation caused by elevated sources in coastal areas



has  been simulated by  two base  models:   the CRSTER



Shoreline Fumigation Model  (CSFM)  and the Misra Shoreline



Fumigation Model  (MSFM).   These two models,  along with



variations of the MSFM model, are evaluated in this study.



     Plume  dispersion in  the  CSFM model is treated as a



point source  upon  intersecting  the Thermal Internal



Boundary Layer  (TIBL).   Dispersion  coefficents  are



determined using the Pasquil1-Gifford  approach.   In



comparison, the  MSFM model treats the plume as an areal-



type source upon  intersecting  the TIBL  and utilizes  the



convective velocity  type equations  to account  for updrafts



and downdrafts in the convective  boundary layer occurring



under the TIBL.   Both of the base models assume uniform,



instantaneous mixing  downward  of  the  plume upon TIBL



intersection.   Variations  of  the MSFM  model,  however,



assume that the  plume is not uniformly,  instantaneously



mixed downward  and  instead use either weighting factors,



based on laboratory results,  to  displace  the  plume



downwind, or  use probability  estimates  of downdrafts to



influence the maximum concentration location downwind.



     The  statistical evaluation procedures  incorporated in



this study involve  the use of  scatterplots, variances and



total and systematic root-mean-square errors.  In addition,

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an index of agreement value  (d)  is used in  place of the
standard statistical  correlation coefficient (r).
     The two-year,  comprehensive  Nanticoke,  Canada power
plant study is used for evaluation purposes.   The 13 test
cases taken from  this data base met the criteria of daytime
onshore flow and  sufficient  land-water  temperature
difference.
     Initial evaluation indicates that the  MSFM base model
performed better  than the CSFM base model.   This  decision
was based on (among other  factors)  the comparatively high
index of  agreement values  (0.76 vs. 0.46)  for  the MSFM
model.  Reasons  for  the comparatively poor performance of
the CSFM model can be viewed in terms  of  the  Gaussian dif-
fusion formulation (using  the Pasquill-Gifford  stability
classification)  versus the convective  velocity scaling
approach of the MSFM model and of  the point  source versus
areal-type dispersion approach.
     Subsequently,  attention  was  given  to evaluating two
variations of the MSFM  model.   This evaluation  indicates
that the  MSFM/downdraft  model  outperformed  the
MSFM/empirical model, but  did  not outperform  the base MSFM
model.  Reasons for the better performance of  the  base MSFM
model are given  in terms of the near-instantaneous assump-
tion not being critical in highly convective TIBLs.
     Sensitivity    analysis  of   the  various   model   input
parameters   (i.e.,   convective velocity scaling,   buoyancy
                            2

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flux, Brunt-Vaisalla  frequency and TIBL  parameteriza-



tions) revealed  that  TIBL parameterization was the most



sensitive variable.   This supports the contention that



proper TIBL  parameterization is the key to  coastal disper-



sion modeling.



     Evaluation of the TIBL height equations is undertaken



separately.   Six TIBL  models are identified  from the



literature and  compared using two  TIBL   experimental data



bases from Long Island and Japan.   The  statistical evalua-



tion methods  are  the same  as  those used in the dispersion



model evaluation.   The  data  are also classified according



to wind speed  and overwater stability.   The  evaluation



indicates  that  the Weisman  (1976)  formulation,  which



includes heat  flux  and  wind speed  along  with  overwater



lapse rate all  raised  to the  half  power, performed the



best.   Classifications  according to wind  speed  and



stability  also showed  that  the heat flux type of equation



worked reasonably well.

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 1.0 INTRODUCTION
     The diffusion and transport of gaseous pollutants
released into the atmosphere in coastal  areas  have  been  of
great  concern to  those involved  in air  quality impact
analyses.   The growth  of  industrial  facilities  in  coastal
areas  has  created a need  for accurate  point source air
dispersion models that  can handle the unique meteorological
conditions wnere  a land-water  surface discontinuity  plays a
major  role.   One  such phenomenon is the development  of a
convective boundary layer  generally known  as  the Thermal
Internal  Boundary Layer  (TIBL), which  develops over the
land for onshore flows when the  air  temperature over  land
is warmer  than the water surface temperature.  Above the
TIBL the air  mass is generally stable, while below the  TIBL
air is unstable due to convective heating  from below.   A
tall stack situated at the shoreline emits pollutants  into
the stable layer first.  The plume travels  with relatively
little diffusion in this  layer,  but  upon intersecting the
TIBL,  fumigation occurs  leading  to high ground level
concentrations.
     Several  methods  are available to model the prediction
of the ground level concentration in the coastal fumigation
zone (Lyons and Cole,  1973;  Misra,  1980a;  Cole and  Fowler,
1982;  Van  Dop et  al. ,  1979,  etc.).   The purpose  of  this
study  is to  evaluate   several Gaussian  dispersion  models
using the  best available  air quality and  meteorological
                            1-1

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data bases,  to identify the assumptions,  uncertainties and



applicability of these models and to identify  the model



components (e.g.,  TIBL  formulation) that are  most valid.



Finally,  some recommendations are provided regarding the



meteorological  and  stack  parameters  needed   to  utilize



a selected coastal fumigation model.
                            1-2

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 2.0  THE THERMAL INTERNAL BOUNDARY LAYER



     A reasonably thorough treatment of  the  unique atmos-



pneric processes present in  a coastal  area can be included



in a numerical model, but such models are rarely  used  for



operational  or regulatory  purposes  because of their



complexities.   There are several  statistical  models  (Lyons



and Cole, 1973;  Misra, 1980a; Cole and Fowler, 1982)  in  use



which  compute ground-level  concentrations  based on  the



assumptions of a Gaussian distribution or  a mixed layer



hypothesis.   An  important  component of  these coastal



fumigation models is the Thermal Internal Boundary Layer



(commonly called TIBL) that usually originates at the land-



water interface and increases in height downwind.  Interac-



tion between the TIBL and a  plume from an  elevated coastal



source influences the distribution of the ground-level con-



centration and the  location  of  its maximum value.   The



concept  of the TIBL is crucial in understanding shoreline



dispersion processes.  In this  chapter the physics of TIBL



formation, the cnaracteristics of the TIBL prediction equa-



tions and  the general impact of the TIBL  on  coastal  plume



dispersion are presented.



 2.1  TIBL DYNAMICS



     Internal  boundary layers  ("internal"  because  they  are



within the higher  planetary boundary layer)  develop  near a



coastline  because  of the  two basic  physical  differences



between land and water:  roughness and temperature.



                           2-1

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     Roughness  over  the water is generally less than rough-



ness over the land.   Frictional effects on air moving over



a water  surface  are minimal  and mechanical turbulence



produced  by varying wave heights is  generally low.  The



mechanical turbulence produced  by  roughness  elements over



land  may be  quite high.   Thus,  with  onshore flow  a



mechanically-forced  internal boundary  layer  develops from



the change in  shear  stress because of the roughness discon-



tinuity present at  the shoreline.   The roughness internal



boundary layer is generally dominated,  however,  by thermal



effects of the surface discontinuity (Raynor et al., 1979).



Other definitions  of coastal internal  boundary  layers



pertain to discontinuities in  specific humidity and momen-



tum (Gamo et al.,  1982),  however, these internal boundary



layers are also dominated  by thermal affects.



     A convective internal boundary  layer  forms because of



differences between  land  and water temperatures (hence the



name  "Thermal  Internal  Boundary Layer").   The formation of



the TIBL based on flow adjustment theory has been given by



various authors (Herman et al.,  1982;  Lyons, 1975).   An



airmass advected over a cool  lake or  ocean  surface is not



destabilized by convective elements as would be° an overland



airmass.  Instead,  the marine air mass cools from below



via   conduction  from the  water's  surface  and thus becomes



stable.  As the  stable marine   air crosses  the   shoreline



 (i.e., onshore flow) it  must   adjust  itself,  first   in the



                            2-2

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lowest levels,  then in the  higher  levels,  to  the  resulting
discontinuity  in  temperature.   This  adjustment  is
accomplished by the generation of  turbulence  which  acts  as
a transport  mechanism for  surface heat  from the  land
surface.   The  TIBL  interface generally  slopes  upward  from
the coastline until at some point  downwind  (X)  it  assumes
an "equilibrium height" which  is the height  of the inland
mixed  layer.   The adjustment  of the once  stable  onshore
flow is complete  at tnis equilibrium height.   TIBLs  tend  to
grow faster with marginally stable, overwater conditions
than with intensely stable, overwater  conditions  (Lyons  et
al., 1983;  Raynor et al., 1979).  This is because the over-
land thermals have  less resistance to rise  with a weaker
capping  marine stable layer  than with  a stronger  capping
layer.
     The TIBL can be classified by stability into two broad
categories  for descriptive purposes, as  shown in Figure
2.la.  Category I TIBLs are  characterized by overwater
stable lapse rates.  In this case TIBL growth begins at the
shoreline (X=0) and continues until an equilibrium point  is
reached downwind.  Category II TIBLs are  characterized  by
overwater  stabilities that are near-neutral or  unstable.
In this case the TIBL  does  not  begin  at  the  coastline, but
instead grows  out   of  the  marine  neutral layer  with  some
initial height ho,  as  shown in Figure 2.1b.
     Several   definitions   of  the   height  of  the  TIBL
                            2-3

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         •I                .
                                                       JC
                                                       4J
                                                        CO M
                                                        
                                                       M  «0
                                                       H  
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interface  (h)  are  given in the  literature.   Venkatram
(1977)  defines  the  TIBL  interface as being the point where
a temperature profile jump  occurs (i.e.,  a  change in
stability from  neutral to stable).   Anthes  (1978)  in his
numerical sea breeze model defines the TIBL height as being
the first  level greater than  180 meters  above ground at
which the potential temperature gradient  exceeds  1 C km   .
     Lyons (1975)  defined the TIBL  height as  being the
average maximum height  to which turbulent  penetrative con-
vective elements are reaching at  a given place  and time.
Lyons  (1975)  presented turbulence data to  illustrate the
sharp turbulence variation  across  the TIBL interface.   An
analysis of the variation of the standard deviation of ver-
tical velocity  (<*w) with  height  for  several coastal cases
(SethuRaman et  al.,  1982) shows turbulence variations of a
factor of 5 across  the TIBL interface. Other investigators
(Raynor  et al., 1979;  Gamo  et al.,  1983)  have  also found
sharp turbulence changes across the TIBL  interface.
     Gamo et  al. (1982)  have  investigated the  variation in
TIBL height (n) based  on the  two  definitions and have con-
cluded that the interface defined by turbulence  is  higher
than the interface defined by temperature.    A  similar
result was  obtained by Raynor et al.  (1979).  In  this study
the more common turbulence definition of TIBL  height is
adopted.
     It is  important  to note that the TIBL can  develop in
                           2-5

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either sea breeze or gradient type flows.  TIBLs can begin
a few kilometers off snore, in response to  warm water
pockets creating  the  necessary  atmospheric thermal
discontinuity.   Finally, TIBLs  can  also form  during  off-
shore flow if there is a sufficient  land-water temperature
contrast.   In this  case  the  TIBL  develops  over  warmer
water.   The  structure of  the  TIBL  in terms of its height
and the vertical  variation  of wind and temperature  within
it will be governed by the  mesoscale phenomena both upwind
and downwind  of the  coast.
     It has  been shown  in this  section that a  distinct
change  in the   air  mass  can  occur  at the  land-water
interface because of two reasons.   One is the  change in
roughness and another is the change  in surface heating due
to the difference in surface temperature between  land and
water.  During daytime conditions, with warmer  land surface
temperatures, the latter process  usually dominates the air
mass modification.   This modified layer generally grows in
height  downwind of the coastline over land  with onshore
flow and is called the TIBL.  A knowledge of the height of
the TIBL at  various downwind distances will be useful for
developing appropriate diffusion  models  for  elevated
sources.
 2.2 REVIEW OF THE TIBL HEIGHT PREDICTION EQUATIONS
     A   review    of  the   literature    indicates  several
approaches to determining  the  TIBL height.  A  historical
                           2-6

-------
flow chart  of TIBL  equation development is presented in

Figure 2.2.   Early efforts in specifying the TIBL  height

are  given by  Van der  Hoven  (1967)  based on  work done by

Prophet (1961).  The  general  equation is:

                                (\ 0.5
                           X    \                    (2.1)
                          «m*«  )

where:

    h = TIBL height (m)

    X = distance downwind  from the land-water interface (m)

   Um = mean wind speed in TIBL  (m s~^)

   A0 = temperature difference between the top and bottom
        of the overwater inversion layer  (C m"1)

     The relationship was  empirically derived to fit obser-

vational  data and is  not dimensionally homogeneous.   The

importance of the upwind stability, generally characterized

by the A0 term and the parabolic dependence on  downwind

distance were first recognized in this formulation.

     The first of two  recent approaches involves the work

of Raynor et al.  (1975) and Venkatram  (1977).  Raynor et

al. (1975)  derived an equation of the  following form based

on physical and dimensional considerations:

                                      (\0.5
                             X|TT-TW| \
                                |y|I              (2.2)

 where:

    u* = downwind surface  frictional velocity  (m s~^)

    TL = downwind surface  land temperature at a height of
         2 m (K)

                           2-7

-------
                       VAN DER HOVEN (1967)


                        h,8.8 ( —-	)
                             \u A0/
RAYNOR (1975)

 ht!is
     VENKATRAM (1977)
       umL  S(1-2F)
                               I975
                                         PLATE (I97I)
                                          PETERS (I975)

                                          hi     2Hox
                                            pCpu(TL-Tw)
                                     WEISMAN (I976)

                                     h8/2H°x f
                                       \PcpSu /
                                      LYONS (I977)
                                                       [x-x0)r
Figure 2.2:
         Historical flowchart showing development of the
         TIBL prediction equations  (symbols defined in
         text).
                             2-8

-------
    TW = upwind  surface water temperature (K)


    Y  = absolute lapse rate upwind  (K m"1)


    U  = downwind mean wind speed at a height of  10 m


     The equation is  dimensionally homogeneous and  incor-


porates use of the  land-water temperature difference.  The


vertical structure  of TIBL  turbulence  (and therefore the


TIBL height)  has been shown to depend significantly on the


land-water temperature differential  (SethuRaman et al.,


1982).   A drag  coefficient  type parameterization (u*/U),


was  incorporated into Equation 2.2  to account for the


change in surface roughness.


     Equation 2.2  does not directly take into account the


surface  heat  flux  over land,  which is important  in the


convective growth  of the  TIBL.   Another problem is with


singularity as Y approaches  0  in  the near-isothermal over-


water condition.


     The TIBL has  been treated  analytically by several


authors as a  horizontally inhomogeneous mixed layer in a


steady-state  condition (Venkatram, 1977;   Gamo et al.,


1983).   By considering the TIBL  as  being two-dimensional,


the  mixed layer energy equation can be written following


Venkatram's (1977) notation as:
                hum ^m = 
-------
(w'0')0 j_ = heat flux  at  the surface and at the TIBL
            height,  respectively

     Venkatram (1977)  assumed that vertical motion is small

compared to entrainment velocity.  A simplified entrainment

hypothesis was used  which assumed that the temperature jump

at the  inversion,  A0Q,  is proportional to the TIBL depth

and the temperature  gradient above the TIBL, such that:

                      A(90 = FR7 h                     (2.4)

where  FR  is an  entrainment  fraction  and  A0  is  the

temperature jump across  the TIBL.   The  ratio  of  heat flux

at the TIBL interface  to  that at the surface has been shown

to equal  a constant  (c)  (Betts, 1973),  where c is also

equal to F(1-2F)~ .   Surface heat flux (w'0')Q is given by

C0U*(0^-0m)  where C^  is  the heat coefficient.  This yields

a relation for the heat flux at the TIBL top as:

                                  ^-               (2-5)
where Cu is the frictional  coefficient.  Substituting Equa-

tion 2.5 into Equation 2.4  yields:
                  hdh = _C,fiu_Sm(l.1^1pLat            (2.6)
                              y  (1-2F)

Integrating Equation  2.6,  substituting  Umdt  = dX  and

assuming  Cs = u*/Um   and   0m = 0W, one  obtains the  TIBL

equation of Venkatram (1977):


                        /          \°'5
               h =   u* I 2X | TL-TW | \
                     Um I SU-2F)  I                 (2.7)


where S = the potential temperature gradient over water.

                           2-10

-------
     Equation  2.7 assumes that  the TIBL is  dominated by



buoyancy.   In  addition, Equation 2.7 assumes that  the  layer



is well-mixed  and therefore produces uniform  vertical



potential  temperature profiles and velocity  gradients.  The



well-mixed assumption  may  not hold true  under  all



conditions, as  shown by  SethuRaman (1982).   For strongly



stable, upwind conditions with a surface-based inversion, a



low-level  supergeostrophic jet is usually  found  over the



ocean.  This layer retains its characteristics for appreci-



able downwind  distances in the TIBL.  Supergeostrophic wind



velocities are observed  over land in the coastal  region in



spite of convective conditions.   Equations  2.2  and 2.3,



derived analytically, are  essentially similar except for



the entrainment variable F  (~0.2)  which  increases the



estimates  of h by a factor of about two.



     Peters (1975) developed a  scheme  of determining TIBL



height with the assumption that  the  upward turbulent



transport  of energy in the boundary layer causes a tempera-



ture gradient  which  corresponds  to a constant,  near-ground



vertical heat  flux.  The average overland TIBL temperature



may be written as:




                 TA - 0.5(TW + ah + TL)              (2.8)



where:



    TA = average temperature of the TIBL layer and



    a  = temperature gradient upwind (K  m~^)



     Peters   (1975)   defines   (Tw  +  ah)  as  being



                          2-11

-------
representative of  the  temperature profile  over both  land


and water.   Equation  2.8  therefore  relates  the TIBL layer


temperature obtained over  a given width of land.  An energy


balance performed  on the area under h yields the following:



HQX = pcpU10[0.5(Tw +  ah + TL) - 0.5(2TW + ah)]  h     (2.9)



where:

                                         o
    HQ = surface heat  flux over land (W m~z)


    CD = specific  heat at  constant pressure
     e   (0.24 cal g^lT1) and


    P  = density of air  (1.2 X 103 g m~3)


The first term in  Equation 2.9 is the average overland TIBL


temperature as given  in  Equation 2.8 and  the  second  term


represents the average overwater temperature.


     Solving for h, Peters (1975) obtained:
                          2 HQX	               (2.10)
                         />cpU  (TL-TW)



The  linear  nature   of   Equation  2.10   implies   that


Peters'  (1975)   scheme  should  predict a  fast  growing


TIBL.   In addition,  this  model cannot  be  used for large


downwind distances because  of  the  linear  growth predicted


by the model.  Observations indicate a parabolic growth.


     Plate (1971),  using earlier work by Ball (1960),


derived an equation for  the height of  the  free convective


boundary layer  capped by a stable  layer.  He assumed that


the heat flux at  the  top of the  convective boundary layer


                           2-12

-------
is equal to the surface heat flux,  so that:
                     (w'Oi = (w'0')0               (2.11)

     If a constant surface  heat  flux  and  sharp temperature

discontinuity at the  TIBL interface are assumed,  then using

the  geometry   of  the  assumed  thermal   structure    (see

Plate, 1971) total heat input can be written as:

               h dT + (TL  + Sh - T) dh =  2HQ        (2.12)
                 dt                  dt   pcp
               f
where T is the temperature at height h. Assuming  that the

temperature  change  and  TIBL thickness  are proportional,

                        _ dh - dT                     (2.13)
                         dt   dt

and
                     «h = T - TL                    (2.14)

where « is an arbitrary constant approximately equal  to  S.

By combining  Equations 2.12,  2.13  and  2.14 and solving

algebraically for n,  Plate (1971) obtained the following:

                       Sh2 = 4H0t_                    (2.15)

                              PCP
which yields,
                    h  = /	4H0X_ \                 (2.16)
                           pcp SU
In Equation 2.16 t  was  replaced by X/U, where U was  taken

to be representative of  the mean TIBL wind.   Weisman (1976)

suggested using an equation similar to Equation 2.16  as  an

extension to  Peters'  (1975)  Equation  2.10, but with  a

parabolic  variation of   TIBL height.   It is  not clear how

Weisman  (1976) derived   his equation, which appears as:

                            2-13

-------
                                     0.5
                   h  = /   2H0X_  \                 (2.17)
                               SU
Alternatively, Gamo  et al .  (1983)  have derived Equation

2.17 from a mixed  layer  theory basis.   Gamo et  al.  (1983)

assumed that the TIBL is heated uniformly and that the heat

flux decreases linearly with height such that:

                 U 30(X)   =  -1  3H(X,Z)             (2.18)
                   3X        pep 3z

Ignoring tne temporal variation of 9 and horizontal  varia-

tion of  heat  flux,  Gamo et al.  (1983)  integrated Equation

2.18  with the  boundary conditions   H = hQ  at z = 0  and

H = 0 at z = h and obtained:

                               H0OO                  (2.19)
                             _     __
                    ax       pcp Uh(X)

The change  in temperature  with respect  to change in TIBL

height may be defined as :

                        aj =  S                     (2.20)
Combining  Equations   2.19  and  2.20,  Gamo et al.  (1983)

obtained:

                     a_h(X) =  _ H (X)                (2.21)
                     BX       pcp SUh(X)

Integration of Equation 2.20 yields:

                      e  = 9Q + S(h - h0)             (2.22)

Integration of Equation 2.21 yields:
I  H(
J xo
                 -  (2   HQ(X)dX + h)-   +  h0     (2.23)
                            2-14

-------
Here the subscript "o" refers to  the  initial  value at the

shoreline    (X =  XQ) .   At the  shoreline (hQ = 0, X = 0),

Equation  2.23 becomes:


                          r x
        h = (PC..SU)"0-5  (2   H0(X)dX +  ti^)0'5         (2.24)
               F           Jo

and Equation 2.22  can be  conveniently rewritten as:

                        0 = S h                       (2.25)

Assuming that  the surface heat  flux does  not change with

respect to inland  distance then  Equation  2.25 becomes:

                                 \  0.5
                          2J0X	  ]
                         P cp  SU    I                   (2.26)

Equation 2.26 is  in reality the Weisman  (1976) formulation

(Equation 2.17).   Gamo  et al.  (1982, 1983) give a more

detailed explanation  of  the above  condensed derivation.

     There are two practical  problems  in using the Weisman

(1976) approach.   To begin, the determination of heat flux

is  difficult in  most  meteorological applications.

Secondly,  the   singularity  question may arise  as S

approaches 0 in the near-neutral  case.  In addition, for

operational use Weisman  (1976) selected 100 cal m~2 to fit

the measured TIBL data to the predictive equation, yet it

is commonly  known  that  heat  flux  varies with time of day,

latitude and cloud cover.

     Lyons et al.   (1983) have  modified  Equation  2.17  to

account for the time  dependence  of heat flux by introducing


                           2-15

-------
various parameters such as a  solar insolation factor  and

elapsed  time since  sunrise.   Tne use  of  this heat  flux

parameterization closely follows the heat flux scheme  used

in a numerical sea breeze model by Anthes (1978).

     The modified   Equation  2.17  given  by  Lyons et al.

(1983) is:

  h  =  hn  + /_2^_Hf,_sin_(7rte./DT )  \     (x-x_)R    (2.27)
         \j    •   i   w ~   _• M i.  Q -... j_j -'"" I         \j


where:

  f = solar insolation factor which was chosen arbitrarily
      as:

      0.1 for very low insolation

      0.3 for low insolation

      0.6 for moderate insolation and

      1.0 for strong insolation

   HC = 20% of the solar constant

   tg = time since sunrise

   DL = length of day

   R  = a variable exponent

   hQ = initial depth of TIBL at downwind distance xo —
        allows for changes in TIBL shape

   h  = depth of TIBL at downwind distance x

Once again  Equation  2.27 has a  singularity problem with S

approaching 0.

     Additional problems arise  from questions of determin-

ing  
-------
for four TIBL cases.  This value may be highly dependent.

It appears  from different analytical  and  dimensional

approaches  (Plate,  1971; Venkatram, 1977; Raynor et al.,

1979)  that R is equal to 0.5.

     Finally,  it  is  important to  note  that some  coastal

dispersion  modelers  (Van Dop et  al., 1979; Misra  and

Onlock,  1982)  prefer to simplify  the TIBL  equations such

that:

                       h = A[X]°-5                 (2.28)

 where:

     A = a factor containing different physical parameters
         necessary for TIBL determination.

In this  section,  all the TIBL  equations except  that of

Peters (Equation  2.10)  can  be written in the form of Equa-

tion 2.28.   The quantity A, constant for given surface  and

meteorological  conditions, will  vary  between different

formulations,  however.  In a later section these TIBL for-

mulations will be examined  against two different data sets

to determine the  best TIBL equation  for use in diffusion

modeIs.

 2.3  IMPACT OP TIBL VARIATION ON COASTAL DISPERSION

     The specific mechanisms involved in  coastal dispersion

will  be presented  in Section 3.2.   In this  section,

however, the physical processes  involving  interaction

between  the TIBL  and an elevated  plume at  the coastline

will be discussed.


                           2-17

-------
     Two important physical processes concerning dispersion

in coastal regions are fumigation and trapping.   Plumes

emitted into the  stable marine air at the shoreline (X  =  0)

normally  move inland with  onshore  flow  and  at some point

intersect the deepening  TIBL.   Intense downward mixing  at

the point of TIBL impaction  can cause  high ground-level

concentration.  Plumes have  been  observed  to  travel 20-to-

30 km downwind before fumigating  (Portelli, 1982).

     Trapping  conditions occur  when stacks  are  located

within the TIBL at some  inland distance  such that plumes

are  emitted into the  convectively mixed  TIBL  and are

effectively capped by the  TIBL interface.  If a plume  is

sufficiently buoyant and a stack is located close to the

TIBL interface the plume  may actually penetrate into the

stable marine air and then fumigate back into  the TIBL  at a

point of intersection  further  downwind.   The  importance  of

TIBL variation on fumigation is illustrated by a practical

example  shown in Figure  2.3.  Various  parameters used  in

Figure 2.3 are:

     Hc =  160 m  (stack height)
      9

    Ahs =  90 m (plume rise)
     Um =  5 m s'1
                  ,0.5
  hx(X)  =  5.61  (X)u-3   typical maximum (A)  factor  (Misra
                        and Onlock, 1982)
  h2(X)  =  2.71  (X)0-5   typical minimum (A)  factor  (Misra
                        and Onlock, 1982)

The  TIBL  heights h^(X) and h2(X) were calculated  using a


                           2-18

-------
                                                  6*0     O
                                                  3 C    -P
                                                  E «0 -O
                                                  -H     CO)
                                                  x ^  -i
                                                            0)
                                                  0)
                                                   C-H  Q)
                                                            0)
                                                            J-l
                                                      0)
E  o:
3 03
                                                   3
                                                   C
                                                   O CQ
                                                  •O H  O  «0
                                                     E* -P
                                                  «W        (1)
                                                   O O  >H  W
                                                     4*  OJ-H
                                                   C    M-l  H
                                                   O M  0)
                                                  -H tt)  J-l  fl)
                                                  •P«w     E
                                                   (0 <1>  013
                                                   O M O. rH
                                                   o        a
                                                  ^ -^«o
                                                     x  c  o
                                                   c —  i V4
                                                  4J— -rH
                                                   (8 X  Q) JS
                                                        O   •  -P
                                                         a>  >ijc
                                                  j   .  (Xi-t  C7»
                                                  03  C  W  0)  -H
                                                  M  O    0)
                                                  EH -H  M -H  £
                                                     4J    *J
                                                  «w  flj   ~ O  .*
                                                   O  MN  
-------
simplified  TIBL equation  (Equation  2.28).   Minimum  and
maximum (A)  factors  were obtained from observations.
     For the case of h-jjx), the TIBL grows sharply from the
coast, reaching a height of 250 m just after 2 km downwind.
Fumigation  of  plume PI  begins  at  this  point.    For
simplicity,  it is  assumed  that plume Pi is mixed instan-
taneously into the TIBL.   The  fumigation  zone  is depicted
as about 2 km long.
     For  the  h2(X)  case, the  TIBL is  seen to grow  less
sharply than for the h-^(X) case.  The TIBL  height  at  2 km
is about  120  m,  which is  considerably below the effective
stack height of  250 m.  In this  case  plume  P2  impacts  the
shallow TIBL around 9 km downwind.   Fumigation  of plume P2
begins at this point.
     The difference  between h-^(2  km) and h2<2 km)  is about
130 m.   This  simple example  illustrates that even  a rela-
tively  small  difference  in  predicting TIBL height at a
given downwind  distance  may  cause  serious  problems in
predicting the location of the  ground-level  fumigation  and
hence  the  location of  the maximum ground-level
concentration.  Every coastal dispersion model  must there-
fore have  a reliable  TIBL   variation   module  in order to
predict the ground-level fumigant concentration.
                           2-20

-------
 3.0  COASTAL DISPERSION MODELING



     This  chapter briefly presents  the mechanics of fumiga-



tion both  inland and  at the coast and presents a review of



the various  shoreline dispersion models and modifications




to each model.



 3.1  THE  MECHANICS OF FUMIGATION



     The phenomenon of fumigation  has  been observed for



several centuries.   One of the earliest uses of the word



"fumigation" was in the book by John Evelyn  (1661) entitled



"Fumifugium: or the Inconvenience of the Aer and Smoake of



London  Dissipated, Together With some Remidies" (as cited



by Dooley,  1976).



     In the early  twentieth century numerous  cases  of



fumigation were  reported  in  Anaconda,  Montana and San



Francisco,  California, among other places (Dooley,  1976).



The first  real  study of fumigation occurred in the late



1930's  at  Trail,  British Columbia and is  reported  by



Hewson and Gill (1944).



     Basically, fumigation is a transitional process which



involves  a plume  in  a stable  layer impinging upon  an



unstable  turbulent lower layer.   The  impingement may be



because of temporal  or spatial  turbulent layer growth.



Bierly  and   Hewson  (1962)    defined   three   different



types of fumigation:



        Type I:  Nocturnal inversion breakup
                           3-1

-------
        Type  II:  Flow of air over an artificial heat
                 source

       Type III:  Continuous, occurring over natural heat
                 sources such as shorelines

     Type I  fumigation  generally  occurs around mid-morning

as the overnight inversion  lifts to plume height  level.

Three  factors  influence the  growth of  this mixed layer

(Lindsey and  Ramsdell, 1983):

         1. Surface heating

         2. Increased surface level winds

         3. Increased upper boundary layer winds

Increased surface  heating  warms  the near  surface  air

resulting in an upward transfer of sensible heat.  This

causes the  near surface  air  to  become unstable  and

turbulence is  no longer suppressed by  buoyancy  forces.

Increasing surface winds caused by the transfer of momentum

between recoupling levels aids in continually increasing

the turbulence, which allows for increased mixed layer

height.  Shear induced  turbulence (aiding in mixed layer

growth)  is possible if higher  level winds increase under

stable conditions.

     A typical  Type  I fumigation  case generally results in

fumigation for  1 or 2 hours.  Plumes initially emitted into

the stable nocturnal  inversion exhibit a fanning type dis-

persion pattern.  During  early  morning the  nocturnal

inversion layer gradually  lifts until mid-morning,  when it

reaches the base of the plume.  Fumigation results when the

                            3-2

-------
plume becomes entrained  into the growing  well-mixed  layer.

Assuming  that complete fumigation  results  in  uniform

vertical  dispersion between the plume  top  and  the ground,

the ground-level  concentrations under Type I conditions may

be  obtained  by  using  the  Gaussian  fumigation  equation

(Turner,  1970):
   C = _ Q _ exp[(-y2/2

where 
-------
originated from other areas  (Munn,  1959).   This process is
made possible by the  so called "heat island effect"  of a
city.
     The concern here is with Type  III  fumigation, which
occurs  during onshore  flow and generally during daylight
hours.   Plumes emitted  into the stable  marine air even-
tually impinge upon  the  growing TIBL and fumigate downward,
as briefly outlined  in Chapter 2.   Fumigation zones may
range in size from  a  hundred  meters to  several kilometers
long and from  tens of meters  to  a  few  kilometers  wide
(Dooley, 1976).
     The following  sections  briefly describe different
coastal fumigation models that have appeared in the litera-
ture with discussion of  their similarities and differences.
Modifications to take into account non-instantaneous mixing
conditions when the  plume impacts the TIBL (the real world
situation), will also be suggested.
 3.2  THE LYONS AND  COLE (1973) MODEL
     Before dispersion models were developed, early coastal
dispersion studies (Hewson et al.,  1963)  concentrated on
photographing smoke  released near shorelines.  Later Lyons
and  Cole (1973), in a study of a large, four stack fossil
fuel plant on the western shore of Lake Michigan, presented
a modification of Turner's fumigation scheme (presented in
the  previous section)  for shoreline   locations.  The Lyons
and Cole (1973)  model divides  the downwind dispersion area
                            3-4

-------
into three zones :

         Zone I:  Undisturbed dispersion  zone   (X-^)

         Zone II:   Plume fumigation  zone        (X2)

         Zone III:   Plume trapping zone         (X-j)

A diagram depicting the vertical  plume geometry appears in

Figure 3.1.   The assumptions  of the  model are:

          (1) "Steady-state"  concentration

          (2)  Flat terrain

          (3)  No initial plume dilution

          (4)  For a given plume, wind direction and speed
               are constant in space.  Therefore the effect
               of shear cannot be incorporated.

     In Zone I, where  C is  a function  of X,Y,Z:He, the

elevated plume is emitted into a homogeneous stable layer

and  therefore  remains  unmodified  in shape.   The basic

Gaussian fumigation  formulation  (Equation  3.1) for finding

elevated concentrations in this zone may be written as:
C(XfY,Z:H)  =
              2Uir
-------
NOIJ.VH1N30NOO   HfWlXVh
    c en
   •H c  •
—    •* 4J


O\ _Q D -H
i—I -H    I)
—  >-4 T3 .C
    O C
 0>  CO (0 .*
^H  0>    O
 O T3 Cn (0
U    C -P
    CO -H w
T3  C C
 C  O C OJ
 (0 -H -H >
    o^ Cn-r^
 (Q  (U 0) -P
 C  M J2 U
 O       0)
 >t4J (U 4-1
^3  C *C ^i
    0) -P 0)
 (1)  M
•C  d) O (U
-P M-l 4-1 J^
   M-l    [ i
4-1 -H (-1
 O 'O <1J 03
      U-l -iH
 >i O 0)
ti ij I. ^<
4->
OJ >•
E OJ X
O '-M
Q) Oj
C" !-< C
      (D
d)  n   •
E   -me
•3  CNX O
                                                   r-l    4J CT>
                                                   (C    X -H
                                                   O   •   e -P o
                                                           0)
                                                   0)
                                                   )-i
                                                   D
     3A08V 1H9I3H '2
        3-6

-------
TIBL.   Figure  3.1  depicts  this  zone  as falling  between

points XB  (beginning of fumigation) and XE  (for end of

fumigation).   The beginning  of fumigation occurs at the

point h  =  He  - 2 . 15 
-------
     In the third zone the plume is assumed to be trapped
with a variable  TIBL lid height  as  an upward boundary.
Concentrations  once  again  are assumed to be uniform in the
vertical  below  the TIBL.   The choice of dispersion coeffi-
cients in  this region must be  done  with care, since the
initial  standard dispersion coefficients are not  valid
within the TIBL.    Therefore, to determine  dispersion
characteristics  in Zone  III  one  must  choose a  virtual
                                   f
source at  some point x^, which lies  between XB and XE in
Zone II.   The  plume trapping formula of Turner  (1970),
along with a virtual point source  method to determine the
new dispersion  coefficient, is  used in  this  zone.
     In the mid-70's  the Lyons and Cole (1973) model  was
modified  to a regional type model  for urban, coastal use.
The new  model  was called GLUMP (Great Lakes  University
Mesoscale  Project).  The  model  incorporated Equation 2.19
for the TIBL parameterization and  included multiple verti-
cal atmospheric layers with independent parameters.
 3.3  THE CRSTKR  SHORELINE FUMIGATION MODEL  (CSFM)
     The CRSTER  Shoreline Fumigation  Model (CSFM) is an
interactive version of EPA's  Single-Source CRSTER model
which  has  been modified  to handle shoreline  dispersion
conditions.   The model  can handle  stacks located  both
inside and outside the TIBL.   The model consists of four
main  modules:  two  plume rise   modules,  a diffusion module
and a fumigation  module.  Concentration calculations can be
                           3-8

-------
made at 180  receptors arranged in 5 rings  (at a time) of 36



receptors for  each ring.



     The fumigation module incorporates the Lyons and Cole



(1973)  scheme  described in  the previous section with



several modifications.  The model  assumes that a pollutant



parcel  entering the TIBL  from  the stable  layer  is



completely mixed in the TIBL  and that this mixing takes



place instantaneously.  However,  unlike the Lyons and Cole



(1973) model,  which treats dispersion in the fumigation



zone as   
-------
     LATERAL VIEW
     SEGMENT
                               THE VIRTUAL
                               POINT SOURCE
                               CONCEPT APPLIED
                               TO SEGMENT q.
                                              1 TRAVEL
                                             _ PATHS
                     H, +2.15 «t
      WATER
              1	3	3
       DOWNWIND DISTANCE (km)
Figure 3.2:
Plume geometry of the CSFM model showing
individual entraining plume  segments (q^/
q2 refer to  segments  1 and 2,  respectively)
                              3-10

-------
the point  of TIBL  plume intersection.  A  virtual point

source is introduced at the TIBL impaction point which  has

a a  equal  to yf . -U h(X)
                             J  1]
The coefficient  
-------
proportion  of the  normally distributed plume that  has
entered  the TIBL at  some distance x.  In  this case,  p is
defined by:
                      P = h - Hc                     (3.9)
                          
-------
trapping occurs, since the plume  is  not buoyant enough to



penetrate the TIBL  interface.   Penetration  occurs if the



resulting rise is greater than  the TIBL height (i.e., the



plume  punctures the  TIBL).   In  this case the height of



penetration is determined and a  two staged  plume rise model



by Holzworth (1978)  is utilized.



     The Holzworth (1978) scheme  generates 25  m  interval



layers up to  500 m  in addition  to a  layer at stack height



and a layer at TIBL  height.   Temperature and wind speed are



estimated  for each layer and a  height (Zn)  is  assigned



where n  represents  the  level number.   A buoyancy flux (F)



is computed at  Zs (stack  height)  until  a negative flux is



found.   The initial  buoyancy  (Fj,  m s   ) is  empirically



determined by (Holzworth,  1978):



                    F± =  (37 X  10~6)  E              (3.11)



where E (cal s~M  is  the heat  emission rate and is given



by:



                E    =   83.45  EVP1(TS-  T^T,,'1        (3.12)







and where:



    EV = gas volume  emission  rate  (m^s~^)



    P! = atmospheric pressure at stack height  (mb)



    Ts = effluent  temperature at top of  stack  (K)



    TI = air temperature at stack  height (K)



Plume  rise  and subsequent   fluxes  at  higher   levels  are



calculated  by  formulas  also  given  by Holzworth (1978).



                           3-13

-------
After  these calculations, receptor concentrations are

determined as previously described.

     A flowchart summarizing  the most important aspects  of

the model appears in Figure 3.3.  The model reverts  to the

standard CRSTER output if the  input  data indicates  that the

conditions are not appropriate  for  a TIBL to  form  (e.g.,

insufficient land-water temperature  difference).

 3.4  THE MISRA SHORELINE FUMIGATION MODEL (MSFM)

     Misra  (1980a) presented  a  model for coastal point

source application based on the equation of conservation  of

mass.  The assumptions made by Misra (1980a) include:

     (1) Constant wind speed with height and independent  of
         shoreline distance

     (2) Perpendicular wind direction to the shoreline

     (3) Instantaneous homogeneous mixing of the plume
         upon TIBL impaction

     (4) Concentration distribution  is Gaussian

     (5) Plume is emitted into the stable marine air

     (6) Dispersion coefficients are a function of  w*

Two key differences between  the Misra (1980a)  and  the CSFM

models are:

     (1)  The plume fumigates  everywhere at the
          interface between the stable air and  the
          TIBL.  Thus the three-zoned approach  is
          changed to a stable  zone and a fumigating
          zone.'

     (2)  After TIBL impaction, the  plume is assumed to
          be dispersed based on the  parameters  of the
          mixed layer (such as convective velocity
          scaling) and not on the derived stability
          ffyf of each plume segment  as in CSFM.

                            3-14

-------
           CSFM MODEL FLOWCHART
                 Inout  MET
                   and
                  Source
                 Conditions
Figure 3.3:   Flowchart of  the CSFM model.

                     3-15

-------
The model assumes  that the movement  of pollutants into the

TIBL are caused by two mechanisms:

     (1)  Entrainment of the plume downwind by the
          growing  TIBL and

     (2)  Processes which affect plume dispersion in
          stable air

The  dominating   mechanism  is assumed to  be  plume

entrainment.   Plume dispersion in the TIBL is assumed to be

described as:
   f-

        Fe(X,Y) =  Cs(X,Y,h) ( Us dh +_KZS dCs )       (3.13)
                                dX   Cs  dZ

where  Fe is  the  entrainment flux  through  the  TIBL

interface,  C0(X,Y,h) is  the concentration distribution
             •5

along  the TIBL interface,  Us is  the wind  speed in  the

stable  layer at height h and KZS  is  the diffusion coeffi-

cient in the stable layer   defined  by  KZS = 1/2  d/dtf^g),

where 
-------
TIBL.
     Misra  (1980a)  uses  similarity theory  in order  to
obtain diffusion parameters  both above and in  the TIBL.  He
assumes  that the parameters in the stable layer are only
affected by the turbulence created by the plume itself and
not  by  atmospherically  induced turbulence.   (This is a
reasonable assumption since  turbulence  levels  are  low in
the stable layer.)   This  means that v ys  and  4.5/N         (3.14)
 _.   _ a  / T?  / TT \ -L / J J_ ^ / J
  V^ ~"  "3    O  S

where a^,  a2  and 33  are  experimental constants and where:
N = Brunt-Vaisalla  frequency  (s"1)   [(g/6  )d0/dz)]°'5
FQ = plume buoyancy  (m4s~3)
Us = mean  wind speed in  the stable  layer (m s~^)
t = travel time (s), defined  as (x/Us) with x the downwind
    distance
The value  4.5/N represents a  time  limit  and for a  stable
atmosphere is assumed to correspond to the time after which
the plume  levels off (Misra,  1980a).
     Characterization of  
-------
The variable w* is a function  of buoyancy,  heat flux and
TIBL height.  The Misra (1980a)  model makes  the assumption
that w* is  independent  of  downwind  distance.  Following
Lamb (1978), a  ^ can be written as:

 »yh(X) = 0.333 hUm/w*

This type of dispersion  coefficient parameterization has
also been recently used in the Maryland Power  Plant  Siting
Program  (PPSP) model  by Weil and Brower (1984)  with good
success.
     Misra (1980b)  showed  that the predicted  and observed
ground-level  concentrations  agreed if  w*/Um> 0.07.
However, detailed validation of  the MSFM model  was not un-
dertaken at that time.  A flowchart of the  basic components
of  the MSFM model  appears  in Figure 3.4.   Output for the
MSFM type models consists  of concentration  values in  a
simple XY type  format along with the meteorological data.
 3.5  EMPIRICAL MODIFICATION TO MSFM
     The  approaches of Lyons  and Cole (1973) and Misra
(1980a)  assume that the  plume is instantaneously mixed
downward after impacting the TIBL,  however,  variability  in
the TIBL (or mixed layer)  height may require a longer time
for total plume fumigation.

                           3-18

-------
                            MSFM MODEL  FLOWCHART
                                          /Plum must\
                                           be emitted }
                                           into stable /
                                          ^marine city
                              Determine
                               Plume
                               Rise
                              (Briggs)
Figure 3.4:
Flowchart of  the MSFM model.   (Note  that the  plume
must  be emitted initially into stable  marine  air.)
                                  3-19

-------
     Water tank laboratory experiments involving  entrain-



ment of a  tracer  into a convectively mixed boundary layer



were recently performed by Deardorff and Willis (1982).



The mixed  layer was assumed to undulate between heights h-^



and hj because of the  presence of  convective  eddies.   The



change in the height (h2 - h-^) was  observed to be  30%.  For



modeling purposes,  the mixed  layer  was assumed to  be repre-



sented by a mean value.



     The  location XQ  is where pollutants begin to entrain



into the TIBL.  Diffusional  travel  time  can  be related to



downwind  distance  X  so that X  -  XQ = UHI^ ~ to^>  Using



nondimensional     distance   parameters   (w*/hUm)    the



dimensionless downwind distance was  written as:



                   X*  =  (X - X0) w*/hUm             (3.18)



Additionally, dimensionless time  was written as:



                        t* =  tw*/h                   (3.19)



and dimensionless concentration as:



                       C* = CUmh2/Q                 (3.20)



Two  categories of  entrainment  (slow  and   fast)  were



examined  to show the  variability  of ground-level



concentrations.



     An adjustment factor based on the laboratory results



is given  by Deardorff  and  Willis (1982).  The factor takes



into account the influence of a  variable TIBL  height and



non-instantaneous  vertical mixing.   It is assumed that the



plume has  small vertical dispersion before hitting the TIBL



                           3-20

-------
interface.   A fraction of  the  potential  fumigant  [A(t)]  is

entrained over a time t with 0 < A < 1 .   Therefore,  the  mass

of pollutant per unit length  which is intercepted per  time

dt is:
                        Q 3A  dt                    (3.21)
                          at

In nondimensional notation,  if the vertical "element"

containing  A(t) were  to  be mixed  upon TIBL  entry,  the

concentration distribution may be written as:

         dC*(0,0,t*)  =  OA/3t) [\X2lP (  */h)]~l        (3.22)
Deardorff and Willis  (1982)  integrated  Equation 3.22 and

obtained an equation which  represents the summation of the

various  elements   that  had  started  fumigating  at some

arbitrary time t ' :


 C(0,0,t*)  = vT2TT| (3A/3t')[ 1

where t" = (t*-t')/4.

According  to Deardorff  and Willis  (1982) this means that

only  16% of the well-mixed  value  from  any particular

entrained  parcel  of  fumigant  is  supposed  to appear  at

ground-level  one  time constant  (t") later,  while  84%  of

its  well-mixed value  appears three  time  units after the

                           3-21

-------
entrainment and 100%  after 4 time units.



     The empirical  adjustment  of  Deardorff and Willis



(1982) that accounts for the delay in touchdown  at ground-



level of the pollutants entrained into  the  TIBL has  been



incorporated into the MSFM base model via Equation 3.13.



     Another approach to account for the non-instantaneous



nature of the fumigation process is  based  on a statistical



model  suggested by  Misra  (1982) for  convective boundary



layers.  This approach  is discussed in the next section.



 3.6  DOWNDRAFT MODIFICATION OF THE MSFM MODEL



     The Convective  Boundary Layer (CBL) which occurs under



the TIBL interface contains  both updrafts (thermals) and



downdrafts.   Based  on an  analysis of the Minnesota data,



Caughey (1982) has shown that  the downdraft  regions  in the



CBL were more  spread out and  lasted longer  than updrafts.



Probability density  analysis  of vertical  velocity  in the



CBL (Lamb, 1982) indicates  that the area under the density



profile is larger for the negative  half than for the posi-



tive  half, meaning  that downdrafts occupy  more than half



the horizontal reference  plane  through the  CBL.  The



analysis showed that updrafts  covered 40% of the area while



downdrafts covered  60% of the area.  Mass continuity,



however, dictates that  the  updrafts have higher  velocities



than the downdrafts.  Lamb  (1982) shows that more energy  is



contained in updrafts  due to  surface layer shear.  He also



shows  that  turbulence  within   the    central  core  of   a



                           3-22

-------
downdraft will  be low due  to  subsidence.



     Misra (1982) proposed a  revision to the Gaussian type



approach based  on the prevalence of these downdrafts in the



CBL.   The Misra  (1982)  downdraft model assumes that the



pollutant particles are non-buoyant and that a large number



of downdrafts pass over a  stack during a given time period.



To  apply this approach  to  MSFM,  it is  assumed that  no



downdrafts occur  in  the stable air  prior to TIBL penetra-



tion  by the plume and that the  processes related  to



downdrafts  are responsible  for vertical dispersion within



the TIBL.  Thus,  even though entrainment at the  top of the



TIBL will be dominated by  the characteristics of the inter-



facial  layer (Wyngaard,  1984),  it  is  plausible that the



entrained material will be carried  to ground-level  by the



downdraft.



     Misra (1982) assumes  that the vertical velocity of the



downdrafts follow a function  described as:



                     v7d =  a fx(z)                    (3.28)



and






fx(z) = -(Z/h)°-333(l - 1.1 Z/h)   0. 025 
-------
the upper 1/3 of the boundary layer.  Another  function g(z)

which  is  an  integral   form that  defines  the  downdraft

velocity at plume-TIBL intersection can be defined as:


             fl               fO.675
g(0.025) = h   (dZ'/0.225)  +  h   (dZ ')/(Z°•333(1 - 1.1 Z'))
            J 0.675           J 0.025

         = 3.34h                                     (3.32)


where Z' = Z/h.

It is assumed  that  the  elemental  area  source as described

in Misra  and  Onlock (1982) has  a height  equal to the TIBL

height at that  location.   Since  the  material  can mix into

the  TIBL from  this location only when  it is caught in

downdrafts, the effects  of updrafts are  ignored.   It is

also  assumed that  a downdraft  has  a  sufficient lifetime

such that materials  emitted  into it  remain  inside until

they touchdown at the ground-level.

     Substituting the approximate values of  f^(z),   
-------
parameterizations  of  Lamb  (1979) presented earlier.



      The downdraft  model was evaluated by Misra  (1982)



using  Lamb's (1978)   numerical data input.  The  model was



not evaluated using real air quality data.
                           3-25

-------
 4.0  BRIEF REVIEW OF COASTAL DISPERSION STUDIES



     In this chapter coastal dispersion studies are briefly



reviewed.   In addition,  the experimental  setup of  the



Nanticoke study  is  presented.  This study will be used for



coastal dispersion  model evaluation  in  Chapter 7.   This



chapter  is concluded  with a description  of model  data



requirements.



     The characterization of  dispersion  in coastal  areas



has been investigated during several field experiments.  In



the  early  1960's  substantial work  was  done by  Prophet



(1961)  to  characterize aerosol  dispersion  in coastal



regions.  Later studies such  as  the  one by Munn and



Richards (1967)  began focusing on  regulatory aspects  of



coastal dispersion.   The dramatic increase in space flight



operations  during the mid-to-late 1960's  created the  need



for  several studies of toxic contaminant dispersion  in



coastal launch areas such as  Vandenburg  Air Force  Base,



California  and Cape Canaveral, Florida (Record, 1970).



     In the 1970's  considerable attention was devoted to



identification of coastal dispersion regimes and develop-



ment of coastal  dispersion models in  the Great Lakes  area.



Lyons  et  al.  (1974)  and Lyons  (1977),  for  example,



presented  data  taken from power plants along the we'stern



shore of Lake  Michigan  and used  this  data for development



of  a  regional  coastal  dispersion   model.  Rizzo  (1975)



conducted  extensive   acoustic  sounder   studies  on  the




                           4-1

-------
shoreline of Lake Michigan during this  time period and used



the data  develop a regional, coastal  mixing depth climatol-



ogy data  base.



     A comprehensive  study  of coastal meteorological



processes was  undertaken  by Brookhaven National Laboratory



(BNL) during the mid-to-late 1970's  (Raynor  et al.f 1975,



Raynor et  al.,  1983).   Some  of the  results of the  BNL



studies  along  with a similar Japanese effort in the mid-



1970's appear in Chapter 6.



     The  SEADEX  (Shoreline  Environment Atmospheric Disper-



sion Experiment)  field program was sponsored by  NRC to



obtain data for the evaluation  of dispersion models.   The



field  study was conducted  in  the  vicinity  of Kewaunee,



Wisconsin during the period May  28  -  June 8, 1982.   Ten



tests were run using SF6 tracer gas  and oil fog.  Real-time



concentration  distributions aloft  were determined  by a



Cessna 337 aircraft  equipped with an alpha airborne lidar



instrument. Acoustic  sounder units, minisonde units and a



ship provided  meteorological data.   Preliminary results



(Johnson  et al.,  1983)   of  the June  8, 1982  case indicated



a three  dimensional, helical  lake  breeze  circulation



pattern,  however the  data is  not  available for  public



distribution at  this time.



     The  next   section  presents  the  methodology  of  the



Nanticoke study  which will be used for  model  validation.
                           4-2

-------
 4.1   NANTICOKE  STUDY — GENERAL DESCRIPTION

     The Ontario Ministry of  Environment  (OME )  in

conjunction  with the Canadian Atmospheric  Environment

Service (AES)  and the Ontario Hydro Power Company conducted

a comprehensive study of the  Nanticoke Generating  Station

(NGS)  plume  during the summer of 1978  and 1979.  NGS is

located on the north shore of Lake Erie across from Erie,

Pennsylvania.

     The basic  coastal  dispersion  objectives of  the

Nanticoke Environmental Management Program (NEMP) were:

       (1)  To  obtain detailed meteorological  measurements
           of  the vertical structure of onshore flows

       (2)  To  characterize the dispersion of  S02 under
           fumigation conditions by developing  a realistic
           shoreline dispersion model

The first field phase (NEMP I) occurred from  May 29 to June

16, 1978. The  second field phase (NEMP  II)  occurred from

May 28 to June 14, 1979.

 4.2  NANTICOKE PLANT CHARACTERISTICS

     Operated by the  Ontario  Hydro Company,  the NGS con-

sists of two stacks,  each of which is 198 m  high.   Each

stack has four flues with a  load capacity of  500 mw each.

Flue diameter is 5.49 m.   Total plant  load  capacity is

4000 mw  with  approximately  156,000 tons of  SO2 per year

emitted  under present conditions.  Plume  rise  has been

observed to average around 400 m  from stack base  (Ontario

Ministry of Environment, 1979).
                           4-3

-------
     The fly  ash  emission rate was 150 - 220 kg h   during

the   study   period.   The   plant   has    99%   efficient

precipitators.

 4.3  NEMP INSTRUMENT DEPLOYMENT - BOUNDARY  LAYER
      MEASUREMENTS

     Boundary  layer  measurements  were  taken  using  a

combination  of minisonde units  (MS),  acoustic  sounders

(AS), surface flux units (SF) and tethersonde units (TS).

Figure  4.1 shows the position of these  various fixed

systems.  Symbols A and B  represent the  minisonde  unit

positions.  The numbers following A and B  refer to downwind

distance (km) from NGS,  while numbers with other  symbols

are for unit  identification purposes.  Measuring systems TS

2, AS  2  and  SF were co-located for comparison purposes.

Figure 4.2 gives  a more  detailed  cross-sectional type  view

of the TIBL instrument deployment.

     The tethersonde units provided wind,  humidity and tem-

perature  information up to  600  m and were  particularly

useful  in the  first several kilometers inland  from the

coast.  Both continuous and vertical profiling modes  were

employed.  The  2  kg instrumental package  consisted  of  a

pair  of  rod  thermistors for temperature  measurements,  a

premium  hygristor  for  relative humidity  measurements,  a

Feuss  barometer  and  miniature  blade/cup  anemometers  for

wind  measurements.  Accuracies   of  the   wind speed  were

±0.1 m s~^.   Wind direction accuracy was ±3°.  The  package


                           4-4

-------
                                                            a,
                                                             0)
                                                            s:
                                                             to
                                                             Ul
                                                             >i
                                                             (0

                                                             O^

                                                            •H
                                                             M
                                                             D
                                                             U)
                                                             m
                                                              rH

                                                             0)  V
                                                            s: -P
                                                            -P  n
                                                                o
                                                            M-l fri
                                                             O

                                                            -P  O
                                                             C  )-i
                                                             (U M-l
                                                             e —
                                                             >i
                                                             o  >i
                                                            r* T3
                                                             a  D
                                                             
                                                            Q  CO
                                                            0)
                                                            J-i
                                                            D
4-5

-------
                                                      (0
                                                     'D
                                                      c
                                                      a
                                                      o
                                                     XI'
                                                      0)
                                                     .c
                                                     -p
                                                      O CD
                                                        cr>
H   -

   r-l
   •H
   cu
                                                     -P
                                                      C
                                                      OJ
                                                      E
                                                      ae
                                                      0)  O
                                                     •C  M
                                                      (C
                                                      c
                                                      o
    CO

    OJ
4J ^j
O  U]
(U  >i
CO  U]
 I
co  VH
co  i
H  (0
O ^H
                                                     (N
                                                       •
                                                     •«•

                                                      0)

                                                      a

                                                     •H
4-6

-------
was sent aloft using a large balloon.   A  tethersonde  unit



located at TS 1 determined the onshore flow prior to over-



land modification,  while  TS 2  was  located  at some distance



inland  to  allow for measurements of a shallow TIBL.   The



acoustic sounding units located at AS 1, AS 2 and  AS 3  were



also able to determine the  structure of the TIBL.



     The MS systems were  mobile, therefore allowing great



flexibility in deployment and potential  in terms of  com-



plementing the AS systems.   Sites A5, A12 and  A15  were



chosen as  the main  launch  locations,  since the prevailing



wind direction was  from the southwest.   Sites  BIO,  B14 and



B20 were used as alternate launch locations when the  wind



direction was south-southeast.  The  system consisted of  an



instrument  package containing a  temperature sensor and a



transmitter attached to  a free floating balloon.   Wind



speed and  direction were  obtained by a double theodolite



tracking system.   Launches began  at  0800 hours  and  con-



tinued to the end of the  study period.



     The SF unit was located inland to determine the fluxes



of momentum, sensible and  latent  heat  and correlate  these



fluxes to TIBL evolution.   Sensible  heat flux was obtained



by  using  platinum resistance elements which  gave  the



necessary gradient data.   Net radiation  was measured  by



solarimeters.   A three component  sonic anemometer/thermo-



meter  was  used to  obtain  measurements  necessary  for the



eddy   correlation   technique.   A  laser  scintillometer,



                           4-7

-------
which estimates surface  heat flux from path-averaged

measurements  of the scintillations of monochromatic laser

light, was also located at the site.

     Wind measurements were  taken at  an  85  m tower  located

10 km inland  and also at the stack height.   In addition,

some of the mobile air quality units contained wind  measur-

ing equipment.

 4.4  NEMP INSTRUMENT DEPLOYMENT  — PLOME CHARACTERISTICS
      AND AIR  QUALITY MEASUREMENTS

     The ground-based  air  quality measuring component con-

sisted  of eight measuring  systems including both  mobile,

in-situ and fixed monitors.   A mobile lidar  unit was used

to obtain plume height, bearing and dispersion characteris-

tics  (2

concentrations.  The COSPEC  unit utilizes the UV absorption

of zenith sky  radiation which  determines the burden of SC>2

over the unit.   The  voltage output  of  the unit  is

proportional   to  the    integral  of   the  path  of  gas

concentration.   This   value   is  usually  expressed   as


                            4-8

-------
concentration times path length or ppm-m.   Plume traverses
were generally averaged  over one-half hour periods and then
projected  onto an axis normal to  the plume.   One COSPEC
unit was always assigned to  the area  within 7 km  of  the
plant.  Two  other  roving  units were assigned to strategi-
cally important area.   Over 700 COSPEC measurements were
made during the study.
     The two roving COSPEC  units also  had SIGN-X  S02
monitors which obtained  ground-level concentrations.   In
addition, a helicopter with a SIGN-X instrument was used to
obtain vertical profiles of pollutant concentration and to
direct ground units to the  plume area.  The helicopter runs
included five traverses  of  five different elevation heights
repeated three times.   A twin engine Piper  Navajo was also
used for S02 and 03 airborne mapping.
     Sixteen Ontario Hydro Power Company Phillips S02 type
monitors (Figure 4.1,  open circles and squares) reported
one hour averaged concentrations.  The monitors consisted
of two portable glass fiber boxes which can be placed on
the ground.   The  measuring principle involved continuous
colorimetric titration with bromine.
     Mobile chemistry units (Figure 4.1, symbols M  1  and
M 2) which  contained  gas analysis systems were deployed for
plume  chemistry measurements.  Unit M 1  (mobile air lab)
contained  analyzers   for  S02,  NOX,  H2S,  CO,  03,  HC,
methane, sulphates,  nitrates, metal particles and  oxides
                           4-9

-------
(Portelli,  1982).   Flow was sampled  at 5 m above  ground.
Unit M 2  (mobile chemical lab) contained  an SC>2 and 03 TECO
type monitor.   The labs operated in  an in-situ mode upon
arriving at  the  monitoring  site.   Figure 4.3  shows the
typical cross-sectional  deployment  of the plume measuring
equipment.  The use of these various  instrument systems has
allowed detailed  analysis of  the  plume behavior  (Hoff et
al.f 1982).
 4.5  DATA REQUIREMENTS FOR RUNNING THE MODELS
     The coastal  dispersion  models  described in Chapter 3
allow the  user to  compute concentration values on an hourly
basis  or  in  some cases  (as  with CSFM)  on a monthly or
yearly  (climatological) basis.   The coastal dispersion
model  input  requirements  can be broken  into two  broad
areas: site  specific and  meteorological.  Site specific
variables  include  stack height and location, exit velocity,
stack gas  temperature, stack  diameter, emissions rate and
effective  stack height (based on site specific parameters).
Meteorological  input  variables  include wind speed, surface
heat  flux (for TIBL  and w* calculations),  TIBL  height
(including the  A factor) and the Brunt-Vaisalla frequency
(N) which  is used to characterize  the stable  air  mass.
CSFM incorporates the Lyons and Cole model.   Hence it was
decided that  the  best results can be obtained by comparing
CSFM  and MSFM, which  make  different assumptions  and use
different  methods   in   modeling  fumigation.  The   input
                           4-10

-------
                                        HELICOPTER
Figure 4.3:  Cross-sectional  deployment view of the NEMP air
             quality measuring  systems (from Portelli, 1982)
                             4-11

-------
necessary for each model  is  listed in Table 4.1.
     The CSFM output consists of concentration values along
a "ring"  (similar  to  the regular  CRSTER model)  at some
distance X from the source.  The model can also be used for
emissions from islands, offshore  sources or under offshore
wind  flow,  although in  this study the model has not been
evaluated under those conditions.  Output for the MSFM type
models  consists  of concentration  values in a simple X Y
type grid along with the  meteorological  input data.
                           4-12

-------
                       TABLE 4.1
                 INPUT FOR BASE MODELS
Input
Factors
                      CSFM
                        MSFM
Site Specific

Stack height

Stack location
Gas exit
velocity

Stack gas
temperature

Stack diameter

Emissions rate

Effective stack
height
                       X

                       X
               (can handle inland
                stacks; needs
                angle of shore)

                       X
                       X


                       X

                       X

                       X
                from Briggs, 1975
                   (only for
                    shoreline
                    releases)
                      uses F,
                         X
                 from Briggs, 1975
Meteorological
Information
U
u
speed

direction
Heat flux (HQ)
      X

      X

      X




Weisman (1976)
N

w*/U
                                  (not required but
                                   useful to
                                   determine w*
                                   if not given)

                                   h = AxO-5
                                   [if measured or
                                   Weisman (1976)]

                                          X

                                          X
                          4-13

-------
 5.0  COASTAL DISPERSION MODEL EVALUATION PROTOCOL

     Much attention has been given to the technical  aspects

of air pollution models.  The ultimate concern,  however,  is

in how well a model simulates  actual measured data.   In

this  section a brief overview of model  evaluation  efforts

is presented, followed by  the  evaluation  protocol and a

summary  of the criteria and  test days  chosen for model

evaluation.
                       f

 5.1  A BRIEF OVERVIEW OF MODEL EVALUATION TECHNIQUES

     The increase  in  air pollution regulations  during the

past decade has stimulated regulatory agencies and industry

to develop statistical  methods for model evaluation.   The

meaning  of the word  "evaluation"  itself has undergone

extensive changes  in  definition.   For the purposes  of this

study, "evaluation" will be defined  to be  the  process  of

examining  and appraising  model performance by  using  field

data to establish  the accuracy of a model or  technique.

This is similar to the definition of  Fox (1981).

     The need  for performance measures in  air  pollution

model  evaluation  has been discussed by  Johnson  (1972).

Brier (1975)  first suggested the following general steps  in

model evaluation:

   (1)  Complete sensitivity analysis of the model

   (2)  Calculation of mean square errors of the residuals
        (P -  0)

   (3)  Completion of a regression analysis of predicted
        and observed concentration

                           5-1

-------
   (4)   Examination of  the  frequency distribution of
        predicted and observed  concentrations

   (5)   Examination of  the  overall model bias

     In 1978, EPA published the Guideline on Air  Quality

Models.  The guidelines gave  the following broad procedures

for model evaluation and comparison:

   (1)   Compare predicted P vs. observed 0 concentration
        values

   (2)   Determine the cause of  discrepancies

   (3)   Correct and improve data bases as needed

   (4)   Change the model if required to reflect better
        mathematical representation of physical reality

   (5)   Document procedures

      A dispersion model performance  workshop  in 1980

brought together the American Meteorological Society and

EPA  to discuss  evaluative procedures  for air  quality

models.  Fox  (1981) summarized recommendations made at the

workshop.  The  participants  agreed on four key areas that

would limit air quality model calculations:

   (1)   Quality of meteorological data

   (2)   Quality of comparative  ambient air quality
        measurements

   (3)   Emissions data  quality

   (4)   Algorithmic capability  to reproduce natural events

Fox  (1981)  suggested, with  the above limiting factors in

mind, that:

   (1)   Plume data be grouped into observed and predicted
        concentration field values, paired for a particular
        location in space at  a  particular time

                            5-2

-------
   (2)   Plume data be developed into a peak concentration
        data set with various degrees of time and space
        pairing

   (3)   Cumulative frequency distributions of unpaired (in
        time) observed and predicted concentration
        values be developed

The specific performance measures  outlined by Fox (1981)

included both residual  (difference)  analysis,  which allows

a quantitative  estimate of (¥ - C)) and  correlation, which

allows a quantitative measure of agreement between 0 and P.

The residual analysis methods from Fox (1981) include:

   (I)   Mean Bias Error   (MBE)
                           i  n
                   MBE = N"1 £ (Pi-Oi)                (5.1)
                            i=l
        or Mean Absolute Error  (MAE)

                   MAE = N-1 £ | P{ - Of |               (5.2)
                            i=l
   (2)   Variance of the difference
                   o         i £            •>
                  Si = (N-l)-1^ (Pi-0-j-MBE)2         (5.3)
                              i=l
   (3)   Gross error of the difference
        Mean Square Error  (MSB)

                   MSB = N"1 £ (P.--O.J )2               (5.4)
                            i=l
        or Root Mean Square Error  (RMSE)

                  RMSE = [N"1 £ (Pi -Of )2]0-5          (5.5)
The correlation analysis methods of Fox (1981)  include:

   (1) time correlation   (r At)

   (2) space correlation   rs = f [Co(x,t) ;Cp(X,t) ]

   (3) time and space combined (r)

The recommended correlation equation is:
                            5-3

-------
         r  =     (CQ-C0)(Cp-CD)	                  (5.6)
           VIS (C0-C0)22(Cp-Cp)2]
Fox (1981)  also notes that future research is required to
establish the  statistical tests  needed for different  air
quality models.
 5.2  STATISTICAL EVALUATION PROTOCOL
     Willmott  (1982a) proposed several  modifications to the
Fox (1981)  recommendations.  In particular, Willmott (1982)
argues  strongly against using the Pearson moment correla-
tion coefficient (r)  with the  Fisher statistic  confidence
interval or its  companion, the coefficient of  determination
(r2),  as  an "ultimate" means of predicted  vs.  observed
value association.   The statistics  r  and r2 do  describe
proportional changes  (either increasing or decreasing) with
regard  to  the means of the  two quantities  in question.
However, distinctions between the  type  or magnitudes of
variables  are not indicated by the value of r.  Willmott
(1981) for instance presented a simple  hypothetical example
of an evaluation of  model A and  model  B.  The hypothetical
plot  of model A and model B output (shown in  Figure 5.1)
indicated  that the curves for  models A and B both fell
equidistant (one on the positive Y and one on the negative
Y  axis) from  the observed  curve.   This means that a
perfect correlation  (r  =  1.0) exists between the two
models.  In this  case the  r = 1.0  value does  not account
for  differences  in  proportionality or  additive constant
                           5-4

-------
     12.00
      8.00
      4.00
      0.00
     -4.00
     -8.00
                    Three Hypothetical Climatic Time Series
                                                           Model B
                                                       i •  Observed

000   0.80   1.60   2.40   3.20    4.00    4.80    5.60
                           Time
                                                           Model A
                                                          6.40   7.20
Figure  5.1:
      Hypothetical  model output showing  deceptive  perfect
      correlation.   Great differences  in magnitude exist,
      however, that the correlation coefficient  cannot
      resolve  (from Willmott,  1982a).
                                 5-5

-------
differences between the two models (Willmott,  1981).


     Willmott and Wicks (1980) presented rainfall data that


showed  statistically significant r and r^  values to be


unrelated to the 0 - P differences.  They have shown that


small differences  between 0 and P could occur with low or


negative values  of r.  Other studies (Willmott,  1982b) also

                                     •p
indicate as to how the use of r and r"6  can be  misleading.


Venkatram and Vet  (1981)  have  indicated that  the


correlation analysis is  of  little value if  the  observed


variance  is close to the  expected variance  between model


predictions and  measurements.


     In addition, Willmott  (1982)  is generally  critical of


the MBE (Equation  5.1)  and  S^ (Equation  5.3).  MBE repre-


sents the  mean  of  the difference between "o and  P~ which


really does not indicate  as much as a  comparative  analysis


of "0  and  P"  alone.   The parameter  S^ is  shown to  be

                                _   «—  O
approximately equal to  MSE - (P - 0)f which  adds little


additional information.   Both parameters also describe the


frequency distribution of  the difference  and do not


identify the sources  of error wnen compared to  the perfect


prediction line.


     Willmott  (1981,  1982)  suggests using  the  index of


agreement  (d)  and the Root Mean Square Error (RMSE) to


circumvent  the   problems   associated   with    correlation


coefficients  MBE  and  S^   type  parameters.   The  index of


agreement can be interpreted  as a measure of how error free


                            5-6

-------
a model  predicts a variable.   Thus the index (d) determines
the extent  to  which magnitudes and signs of  the observed
values about 0>   are related to the  predicted deviations
about 0.  It is assumed that 0 and  O are error free.   The
maximum possible  difference between the predicted and
observed values may be described by:
                  |P± - (J|  +  |0± - 0|                 (5.7)
Squaring this maximum  possible difference and  summing  over
all observations one  obtains a  potential   error  (PE)
variance   (Willmott,  1981)  and therefore the condition
0 < (RMSE)2 < N"1 (PE)2 is satisfied.   The statistical,
descriptive  relative error measure  which indicates  the
degree  to  which  predicted  values  approach  the observed
values can  then be written as:

                   d » l-N(RMSE)2                    (5.8)
                          (PE)2
and expanded to,
           n         n
    d =  l-Z^Pi-C^)2/ £ (|P£|  +  |0.{| )2     0 
-------
interpreted exclusively, since d  becomes  unstable  when  the


denominator is small.  Difference measures provide  the most


rigorous  and useful information regarding  overall model


performance (Willmott, 1981).  However, models contain both


systematic and unsystematic  errors.  The  d  index should


therefore  be used  in-con junction with  the difference


measures such as the mean square error and its  components


the systematic MSB (MSES)  and the unsystematic MSB (MSEU).


Systematic errors  result from causes which  persist or  are


consistent.   Unsystematic  errors consist of a number of


small effects such as the  imprecision  of  a  constant.  Some


of these  effects are positive  and some are negative in


terms of affecting the final  output value.


     The best model,  therefore, has a systematic  difference


of zero, since it should  explain most of  the systematic


variation in 0, while the  unsystematic  difference should


approach the MSB.   The value of  MSB should  be minimized so


that  the  model is predicting at peak accuracy.   A larger


value of MSEU when compared  to MSES may  indicate  that  the


model is' as good as possible under present  conditions.   In


terms of statistical  notation, the  systematic mean square


error  is  the  error caused by  model  additive  or pro-


portional problems and can be expressed as:


                   MSES = N~XZ(P - 0±)2             (5.10)

      A
where P = a + bO^.


The unsystematic mean square  error is expressed by:


                            5-8

-------
                            ,  n
                   MSEU = N^E (P± - P.:)2           (5.11)
                             i=l


The total MSB can therefore be written as:


                     MSB = MSES + MSEU               (5.12)


The values of RMSE  (square roots of  the MSB)  are  generally


computed to make  the  numbers  easier  to use  for qualitative


.or quantitative comparisons.   The total RMSE may be written


as:
                 RMSE = N/RMSES2 +  RMSEU2            (5.13)


The use of the RMSE is advantageous because it is a conser-


vative measure of accuracy.  The analysis  of  RMSE  also  has

                                        2
an advantage over an analysis of r  or  r*  since  errors in  r


may be hidden by  high values  of  observed  and predicted


variances or appear  significant  due  to  low magnitudes of


observed and predicted variances (Willmott, 1981).


     Finally, in addition  to  RMSES, RMSEU and  d,  Willmott


(1982) suggests that summary measures  such as "6,  P~,  S2  and

  o
Si,  along  with  simple  linear regression,  should  be


reported since they are easily understood.


     In this study, while following the general  philosophi-


cal recommendations of Fox (1981) in terms of using several


statistical measures,  the more precise  approach  of Willmott


(1982a) is   adopted.   Therefore the parameters and  proce-


dures used for model evaluation are:


   (1) Scatterplots of P vs 0 concentration values


   (2) Univariate summary measures


                            5-9

-------
          a.  P

          b.  0

          c.  S2

          d.  S|

          e.  P = a + bO^  (least  square regression to obtain
                          a  and  b)

   (3) Specific difference measures

          a.  RMSE, RMSES,  RMSEU

          b.  Index of agreement  (d)

Statistics based on traditional highest and second highest

concentration values and  on frequency distribution are not

chosen in this  study,  since the data represents more of a

case description of coastal  fumigation  as opposed  to the

more  typical monthly or annual  climatological  receptor

analysis.

     The 13 test periods  listed in Table 5.1 were selected

because  they have  met the established criteria (Cole and

Lyons, 1972;  Lyons, 1975)  for  onshore  coastal  fumigation

occurrences.   The criteria are:

   (1) Onshore flow outside  ±10  degrees  relative to the
       angle of the shoreline (e.g.,  the angle of the
       shoreline with respect to North at  NGS is 80
       degrees; therefore, the allowable windflow angles
       for fumigation to  occur are 90 degrees to 250
      ° degrees)

   (2) Hours of occurrence from 7  AM  to  7  PM  (daytime)

   (3) Hourly wind speed  greater than 2  m  s~^

   (4) Land-water temperature difference greater than
       0.5 C
                           5-10

-------
TABLE 5.1

TEST
1.
2.
3.
4.
5.
6.
7.
8.
9.
10.
11.
12.
13.
LIST OF TESTS

June
June
June
June
June
June
June
June
June
June
June
June
June
USED FOR MODEL
DATE
1, 1978
1, 1978
1, 1978
1, 1978
1, 1978
6, 1978
6, 1978
6, 1978
6, 1978
6, 1978
13, 1979
14, 1979
14, 1979
COMPARISON
TIME (EOT)
1100
1200
1300
1400
1500
1200
1400
1500
1600
1700
1700
1400
1600
   5-11

-------
     It is also  important  to  note that  the tests  only



occurred under  stable marine air conditions.  No cases were



observed  with  neutral  or  unstable  marine  air



characteristics.   Four models  (CSFM,  MSFM,  Deardorff



Modification and  Downdraft  modification) were evaluated



based on the NEMP I and II  experimental  days listed  in



Table 5.1.



     The summary measures  combined  with the  specific



measures should provide a good indication of the ability of



a model to predict concentrations under coastal fumigation



situations.  Now that a protocol for statistical comparison



of different models  is established,  it is proposed to first



compare  the various TIBL  formulations given in Chapter 2



and determine the  best.  This formulation  will be  incor-



porated  in   the  two   dispersion   models  selected  for



comparison and  then  evaluated using  the Nanticoke data set.
                           5-12

-------
 6.0  THERMAL  INTERNAL BOUNDARY LAYER EQUATION EVALUATION
     Importance of  the air  mass modification and  the
development  of the TIBL at the coastline  were  addressed in
earlier chapters.   Effect of  variation of the TIBL height
on the fumigation  process and the  location of  maximum con-
centration  were discussed  in Chapter  2.   A reasonably
accurate  depiction of the TIBL is necessary to simulate
coastal fumigation processes.   In this section an evalua-
tion of the  various TIBL formulations against  comprehensive
field  data  is made to statistically determine  the best
avai1able mode1.
     Seven TIBL  data bases and reports have been identified
from the  literature and  other  sources and  are  shown in
Table  6.1.   The most complete  data bases  in  terms of
overland,  overwater and aircraft measurements  are the east-
ern Long Island and Kashimaura,  Japan studies.  These two
data bases  were  used  to  evaluate the various  TIBL
formulations.   NEMP  studies were not used for  TIBL evalua-
tion purposes  because they did not have as complete a set
of overwater observations  as  the Brookhaven and Kashimaura
studies.
     First presented  are  two  typical  days (one with stable
overwater conditions and one with  unstable overwater
conditions) to  demonstrate  some  of  the  variations in the
values  obtained  from   TIBL  prediction  equations under
different meteorological  situations.   The two data bases
                           6-1

-------
                         TABLE 6.1
                      TIBL DATA BASES
DATA BASE
SOURCE
Brookhaven (BNL)
Kashimaura (Japan)
NanticoJce (Canada)
Wisconsin/Lake Michigan

Avon Lake/East Lake,
Cleveland

Maine

Tampa Bay
Raynor et al. (1979)
and unpublished data

Gamo (1981); Gamo et
al. (1982)

Lui (1977); Portelli
(1982); Kerman et
al. (1982)

Lyons (1977)

Unpublished data


Fritts efal. (1980)

Unpublished data
                            6-2

-------
are then combined  to  describe  the  TIBL  prediction  equation
variation in terms of an overall  comparison.   This section
is concluded with  a categorization of the TIBL cases by
stability and wind.   Six TIBL formulas  have been evaluated
(Equations 2.1,  2.2,  2.7, 2.10, 2.16 and 2.17).
     Twenty-nine hours  (cases) of TIBL measurements span-
ning twenty-four days were  examined.  Each hour  of data is
considered a case.   The  experiments were conducted during
the period from March  to  November.   Generally, each  case
contained between  four and twelve  TIBL measurements
downwind.  Observed TIBL heights were determined  every  2 km
downwind  for  the Kashimaura data base and every 1 km
downwind for the  BNL data base.   The total number of
observed TIBL heights for the twenty-nine cases is  203.
 6.1  THE BROOKHAVEN  COASTAL METEOROLOGY EXPERIMENTS
     The Atmospheric Sciences Division  of the  Brookhaven
National Laboratory investigated  development  and  charac-
teristics of the TIBL over Long Island,  New York  during the
mid-and-late 1970's as  part  of  their  coastal meteorology
program.  Terrain  of  the study area  varies from  sandy  near
the coast to shrub and tree covered further inland.
     Measurements of turbulence  and temperature were made
from aircraft and  tower-mounted  instruments.  These data
were  plotted as  a  vertical  cross-section by  combining
various  heights  along the  flight track.  Observations of
land  and  ocean surface  temperatures   were  made   with an
                           6-3

-------
infra-red sensor from the aircraft.  Flight  tracks  across
Long Island are  shown in Figure 6.1.  For this study  tracks
3 and 4 were chosen since they provided the greatest over-
land distance for TIBL  growth  and were  not influenced  by
inland bodies of water.  Wind profiles were determined from
pilot balloon soundings.
     Methods for determining various parameters used  in the
TIBL  equations are  given  in Table  6.2.,.  Wind  speeds
observed  near BNL  were used for  overland values.   A
complete  description of the experimental program is given
by Raynor et al. (1979).
 6.2  THE KASHIMAURA COASTAL METEOROLOGY EXPERIMENTS
     The Japanese National Research Institute for Pollution
and Resources  conducted a  TIBL  investigation  in the
Kashimaura-Kujukurihama region  of Japan during the  1970's.
The study will be referred to as Kashimaura for simplicity.
The region is located  100 km  east  of  Tokyo  and is  sandy
with some shrubs and farmland.  Figure 6.2 shows the  trian-
gular configuration  of the coast.   Occasionally, the
Kashimaura sea breeze  joined  the  Kujukurihama sea breeze.
These cases were not considered in  the  analysis.   Aircraft
measurements of  turbulence and temperature  were made  from
heights  of 50 m to 2000 m.   Pilot balloon soundings were
taken inland and at various  points  along the  coast.   Tower
measurements  of  wind   and  temperature  were also made at
several  coastal and inland sites.  Land and  ocean surface
                           6-4

-------
                                                       m  j
                                                       M  OQ
                                                       EH  M
                                                           EH
                                                        tH
                                                        O  W
                                                        CO  4J
                                                       X
                                                        O  C
                                                        (C  -H
                                                           0)
                                                       4->  CQ
                                                       .C  D
                                                        D^
                                                       •H  Q)
                                                       •->  lH
                                                       MH  0)
                                                        C T
                                                       -H
                                                        3 ^a
                                                        O
                                                       £ m
                                                        CO
                                                           CO
                                                       T3 .*
                                                        C O
                                                        (0 (C
                                                       r-t >-J
                                                        CO EH
                                                        c -P
                                                        O C
                                                        i-3 0)
                                                        a a D
                                                        (0 X -P
                                                        S 0)  to
                                                        a
                                                        CTI
                                                       •H
6-5

-------
                    TABLE 6.2
   TIBL  PARAMETERS USED FOR THE BNL DATA BASE
Parameter        Method
      z          10 meter winds from tower near BNL,
     '           Uz from wind profiles

                 Overwater temperature profiles

  u*             Logarithmic profile relation with
                 an average ZQ of 0.3 m

  T^             Infra-red sensor from aircraft

  TW             Infra-red sensor from aircraft

  7,5            Overwater temperature profiles

  F              0.2 (Venkatram, 1977)

  HQ             Surface similarity relationship
                 H0 = pCpU*kz(d0/dz), where k is
                 von Karman's constant (0.4) and z
                 is the height over which temperature
                 measurements were taken
                       6-6

-------
Figure 6.2:  Map of Kashimaura-Kujukurihama,  Japan experimental
             TIBL areas.
                             6-7

-------
temperatures  (IR)   were  taken  at 1 km intervals.   Flight
tracks were made across the  entire region.   Solar  insola-
tion data was  available from  the Choshi Observatory  located
at the apex  of the triangle.  Methods for determining  the
various  TIBL  parameters for this data base are listed in
Table  6.3.  A complete description  of  the experimental
methods is given  by Gamo et al. (1982).
 6.3  THE STABLE  UPWIND OVERWATER CASE
     Stable conditions over water upwind of the coastline
are generally  observed during the  spring  and early  summer
seasons and lead to an ideal fumigation condition downwind
of the coastline.  Hence this was  selected  as one   of  the
two examples for comparison of TIBL height values obtained
using various  formulations.
     Upwind stable  conditions over water  off Long  Island
are very common, particularly in the  spring and  summer
seasons.   The case presented  is Brookhaven experiment
BL #13,  which was  conducted  on June 16,  1979  from  1330 to
1500 EST.  A listing of the meteorological data pertaining
to the experiment  appears  in Table  6.4.   A surface-based
inversion was present  over the  water up  to a level  of
150 m.  The water temperature was 14 K cooler than the land
temperature.  The presence of this strong temperature dif-
ferential between the  land and the water caused the  TIBL to
be shallow (less  than  340 m high), since the warming of the
marine air was gradual.  TIBL observations continued out to
                           6-8

-------
                    TABLE 6.3


TIBL PARAMETERS USED FOR THE KASHIMAURA DATA BASE


Parameter     Method
  U-^Q z       10 meter winds from towers, Uz from
     '         pilot balloon wind profiles

  A0          Overwater aircraft traverses

  u*          ~
-------
              TABLE 6.4






     BL #13  METEOROLOGICAL DATA






  Parameter                   Value



     U                       4.5 m s"1



    40                       3.0 K



     u*                      0.5 m s"1



     TL                      303 K



     Tw                      288.5 K



     H0                      162 W m~2



   dT/dz                     0.015 K m""1



Wind direction               150°
                 6-10

-------
12   km   downwind,  where   an   equilibrium   height  was



approximately  reached.



     The predicted TIBL values for downwind distances up to



12 km are given in Figure 6.3,  which shows  that for this



case Equation 2.2 (Raynor et al.,  1975)  predicts  the TIBL



height the best.  Equation 2.1  (Van der  Hoven,  1967) also



predicts  the  temporal pattern of the  TIBL height fairly



well, but tends to systematically underpredict  the height.



This may be because  of the lack of TIBL forcing terms such



as TL or TW in the equation.   Equation  2.10  (Peters,  1975)



underpredicts the TIBL height for all  downwind distances.



This may  be attributed  to  the  land-water temperature



difference appearing in the denominator.



     Equation  2.7  (Venkatram,  1977)  overpredicts  the TIBL



throughout.   Much of  this overprediction (as compared  to



the  Raynor  et al.  1975 formulation  and  observations)



appears to have been created by a difference factor of 1.83



between the term [2/(1-2F)]°-5,  where F  =  0.2  (Venkatram,



1977)   and the terms  in  the Raynor et  al.  (1975)



formulation.   Equation 2.17  (Weisman, 1976)  underpredicts



the TIBL for this case.



 6.4  THE UNSTABLE OPWIND OVERWATER CASE



     As was discussed in a previous section,  one of  the



controlling parameters  for TIBL  growth  is the upwind ther-



mal  stability  over water.  An upwind,  thermally  unstable



case is selected for evaluation in this  section in contrast



                          6-11

-------
    800
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 468
Downwind Distance (km)
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                                            12
         A

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            -•a Raynor (R)
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Figure  6.3:   Observed  vs predicted TIBL heights for BL  #13
                             6-12

-------
to the stable case  in  the  previous  section because of the
existence  of an  initial,  shallow  mixed  layer over  the
ocean, capped by an  elevated thermal inversion.
      The upwind unstable case is most common in winter and
early  spring.  The  case  selected  for  unstable condition
analysis  was Brookhaven experiment BL #6, which occurred on
March  18,  1975,  1130  to  1330 EST.   A  listing  of  the
meteorological data  pertaining to the experiment appears in
Table 6.5.   The  sounding shown in Figure 6.4 indicates that
a shallow,  superadiabatic layer existed over the ocean near
the surface, capped by a stable layer.   The TIBL equations
are therefore modified by adding  a  constant  hQ to  the
original  equation.  For example, Equation 2.2 now becomes:
              h  = h0 +  (u*/U)(x|TL-Tw|/y )°'5         (6.1)
This modification is made because the equations assume that
offshore  conditions are  stable.   The  hQ  in this case was
determined to be  150 m based on  the overwater temperature
profile.   Table 6.6 gives an interesting comparison of the
predicted values of  the TIBL with and without hQ.  The TIBL
prediction equations without  hQ greatly underpredict  the
TIBL.
     The TIBL grew very rapidly  for  this case  after 2 km
because of the development  of  intense  overland convection.
Figure 6.5 shows  the TIBL height with  downwind distance X.
Weisman's  (1976)   formulation  with  the  hQ  modification
predicts    the   best   along   with   Venkatram's  (1977)
                           6-13

-------
              TABLE 6.5
     BNL #6  METEOROLOGICAL DATA
  Parameter

     U

     A 6

     u*
     T,
      W

     Ho

   dT/dz
       .-1
  Value

 4.5 m £

 5.0 K

 0.5 m s'

 290 K

 281.3 K

 276 W m~2

-0.0131 K m
          -1
Wind direction
150 m: hQ is
the initial
TIBL height due
to unstable or
near-neutral
overwater
conditions

150°
                 6-14

-------
HOOr
                                         — Oceon
                                         - BNL
                           Temperature (*C)
          Figure 6.4:   Sounding for BL  #6,
                          6-15

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Figure  6.5:   Observed vs predicted TIBL heights for BL  #6,
                             6-17

-------
formulation.   It is possible that Venkatram's  (1977)  for-
mulation predicts  better  values than in the previous case
because of  the relatively  uniform winds  in  the  lowest
levels.   The  average  h difference  between the Weisman
(1976)  formulation  and the  Venkatram (1977) formulation
was about  10  m, which is within observational error.
     Two typical cases of differing upwind stability have
indicated mixed results  in  terms of  the predictive
capabilities of  the various  TIBL equations.   This would
suggest that  some caution  be exercised when applying  even
the determined,  best predictive  equation.  Statistical
evaluation of these equations using  the two data  bases
should allow for a better evaluation of the effectiveness
of the  various TIBL equations.
 6.5  EVALUATION  OF TIBL EQUATIONS
     A statistical analysis  of the predicted and observed
TIBL values  was  first undertaken to determine the  best
overall predictive equation.   The data was not categorized
according to wind  speed, stability and so forth at this
point.   The  summary  measures, regression coefficients and
difference measures appear in Table 6.7.  An analysis of
'O vs. "P values indicates that  the Plate (1971),  Venkatram
(1977)  and Raynor et al. (1975) formulations all on average
overpredicted the  TIBL height.   Equation 2.7 (Venkatram,
1977)  has  the most  deviation  from the  observed value.
The greatest   scatter (based  on the  comparison  of Sp) is
                          6-18

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exhibited by the Plate  (1971)  equation.   All equations,
however,  show a rather  large scatter.
     The linear regression coefficients present a rather
confused picture of  small  "a" values, yet small "b" values.
It is very difficult to draw conclusions from examining the
coefficients alone.   The correlation coefficients have been
included for completeness,  although  they either show mini-
mal  significance  or  are  not  significant  at the  95%
confidence level.  The difference measures indicate  that
the Weisman  (1976) and  Plate (1971)  equations are perform-
ing the best.  The equations are  ranked from best predictor
to worst predictor as follows:
         (1)  Weisman (1976)
         (2)  Plate  (1971)
         (3)  Van der Hoven  (1967)
         (4)  Peters (1975)
         (5)  Raynor et al.  (1975)
         (6)  Venkatram (1977)
The decision to  rank the  Weisman (1976)  equation first is
based on the index of agreement value of 0.68, which is the
highest value of any model.  This means, for example, that
68% of the  potential for  error is explained  by the model.
Secondly,  even though both  the Weisman  (1976)  and
Van der Hoven  (1967) equations have  identical RMSEs,  the
real  differences  between  the two approaches  lie in  the
systematic  and unsystematic errors.  The systematic errors
                           6-20

-------
of the Weisman  (1976) model, for example, are much lower
than the systematic errors of the  Van der Hoven  (1967)
model.
     An examination of  the regression  coefficients also
shows  that  the  Weisman  (1976)  and  Plate (1971)  models
outperform  all  the other models.   The summary  measures
indicate  that  the  Weisman  (1976)  and Plate (1971)  models
underpredict  or overpredict,  respectively, with regard to
0^ vs F.  The other  three rankings are based on a combined
analysis of the difference  measures, summary measures and
regression coefficients.
     The  Peters  (1975) model  (ranked  fourth overall) makes
the physically  unrealistic assumption that the TIBL is
linear, with no  entrainment at the TIBL interface.  Peters
(1975), of  course,  also cautions  that his equation  should
not be used  for  long downwind distances.   This is because
of the linear rapid growth  of the  predicted TIBL height.
The Raynor  et al.  (1975) formulation  cannot handle the
neutral  case  and the results were  affected by those par-
ticular  observations close to neutral conditions.   The
VenKatram (1977)  model, which contains state-of-the-art
analytical reasoning, surprisingly finishes  last in overall
rank.  There may be several  reasons contributing  to the
poor performance of the  model.  First,  the model  is to be
used  under  steady-state  conditions, meaning  that it can
only be applied  when the atmosphere  is  in   an "equilibrium
                          6-21

-------
state,"  which  lasts  for a  few hours during  daytime
conditions.    Unfortunately,  the coastal  meteorological
processes do not always  satisfy steady-state  conditions.
The amount of heat flux could be cut back by clouds for a
time in mid-day, thus  causing  sudden  temporary collapse of
the TIBL.   Secondly,  the  inversion  (i.e., TIBL  interface)
heat flux controlling  the  TIBL  height is assumed to be a
fixed part of the surface heat flux.  This  assumption may
be restrictive  as the  strength of  the TIBL  interface
decreases  with  decreasing thermal  stratification  of the
marine  air.   This  is  similar to  the  argument  of
Zilitinkevich (1975).  Also, the use  of  a fixed entrainment
factor (FR) may  limit the applicability  of the equation to
varying entrainment rates  along the TIBL interface.
 6.6  ANALYSIS BY WIND CATEGORY
     The TIBL data base contained different  meteorological
conditions in terms of water temperature, thermal stability
over  water and wind  speed.    It  will  be of  interest to
determine if some of the  models  do better  under certain
meteorological conditions.  The data  base was divided into
smaller  segments depending  on wind speed and  thermal
stability and tne statistical analysis was carried out.  In
this section classification by wind  speed is made.   In the
next  section data  are classified  according to thermal
stability.  Classification by wind speed allows linking the
TIBL  models  somewhat   to the  different mesoscale  (i.e.,
                           6-22

-------
higher winds  under sea  breeze conditions)  and synoptic



scale conditions (i.e.,  gradient winds  due  to  the location



of high pressure systems) in the study area.   Category  Ul



contained 101  cases and included wind speeds of  4.0 m s"1



or less.   Category  U2  contained 102 cases and included wind



speeds greater than  4.0  m  s~ .  Lower  wind speeds will



generally  lead to near-free  convection  conditions  and



higher TIBL heights  as shown  by  Raynor  et  al.  (1979).



Table 6.8 a-b  shows the various  evaluative  statistics for



the Ul and U2  categories.



     It appears that the  formulation of Weisman (1976) per-



forms the best under low  wind conditions, based on analysis



of d and  RMSEs.  The rankings are:



         (1)  Weisman  (1976)



         (2)  Van der  Hoven  (1967)



         (3)  Plate (1971)



         (4)  Peters (1975)



         (5)  Raynor et al.  (1975)



         (6)  Venkatram  (1977)



It is also  interesting to see that  the top three rankings



for the Ul case are relatively consistent  with  the  general



analysis given in Section  6.5.   In this  category the



Venkatram (1977) model does  very poorly,  finishing last  in



rank.



     The  inherent  difficulty with  most of these models  is



that  the  effects  of  advection  are  represented  by  one



                           6-23

-------








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horizontal wind velocity  which is assumed constant  with
height.  Even the Venkatram (1977) model,  which requires a
mean mixed layer wind,  does not take  into account marine
stable air wind velocities.   Thus,  wind  shear effects are
not accounted for in any of the models.   Readings et al.
(1973) have  shown, however,  how wind  shear at the  CBL -
stable air interface is important in  entraining sensible
heat and momentum.
     Table 6.8 b displays  the  evaluative statistics for the
higher wind category, U2.   The results are markedly similar
to  the Ul  results.   Under  higher  wind conditions the
Weisman  (1976)   formulation   once   again  performs  well.
The rankings  are:
         (1)  Weisman (1976)
         (2)  Plate  (1971)
         (3)  Van der Hoven (1967)
         (4)  Peters  (1975)
         (5)  Raynor  et  al.  (1975)
         (6)  Venkatram  (1977)
The Van der Hoven (1967)  formulation is  shown to under-
predict the TIBL height.  The Venkatram (1977) formulation
is consistently last in rank for both categories.
 6.7  ANALYSIS BY STABILITY .CATEGORY
     The combined data  base was divided into four stability
categories labelled  Si, S2, S3 and S4.  The partitioning of
the  data is in  accordance with  the  recommendation   of
                           6-26

-------
Fox (1981)  regarding data interpretation using small  net-
work comparison by meteorological categories.  The division
of each stability category  is  as follows:
         SI:  dT/dz<-0.012  K m"1           (fairly unstable)
         S2:  -0.012 -cdT/dz<-0.005 K m'1      (near neutral)
         S3:  -0.005 •< dT/dz < 0.005 K m"1        (isothermal)
         S4:  dT/dz<0.005                         (stable)
The dT/dz values  refer  to  the lapse  rates over the water,
therefore the TIBLs are classified by overwater  boundary
layer characteristics.
     It is important to note that category Si contained
only nine observations.   Conclusions based on this category
should  be  used with some  caution because of this  small
number of observations.  Category  S3  was observed only in
the BNL data base.  Table 6.9 a - d  gives the statistical
measures  used to  evaluate the equations under  all  four
stability classifications.
     The statistics for the Si case appear in Table 6.9 a.
The ranks for the various TIBL models  are:
         (1)  Weisman (1976)
         (1)  Venkatram  (1977)
         (3)  Plate (1971)
         (4)  Peters (1975)
         (5)  Raynor et  al.  (1975)
         (6)  Van der Hoven  (1967)
      It would appear  from the evaluative statistics that
                           6-27

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both the  Weisman (1976)  and Venkatram (1977)  formulation



best predict TIBL height under unstable marine  conditions.



This may be because  of the inclusion of an hQ term to each



equation,  which would account for the  initial  TIBL height




caused  by offshore convective  conditions.  It is hard to



draw inferences,  however,  on such a limited  Si  category




data base.



     The statistics  for  the S2 category (near neutral case)



appear in Table 6.9  b.   The rank for the models  are:



         (1)  Peters  (1975)



         (2)  Weisman (1976)



         (3)  Raynor  et al.  (1975)



         (4)  Venkatram  (1977)



         (5)  Van  der Hoven  (1967)



         (6)  Plate (1971)



It is not surprising to  see the Peters  (1975)  equation



performing well for  this category  since the  equation does



not contain any  direct stability type terms  and instead



relies on TL-TW and  heat  flux terms,   which would not be



affected by temperature  gradient singularity.   It  is inter-



esting  to note that most of the equations tend to over-



predict the TIBL height  on average.  This  cannot  be



directly  accounted for,  except to say that perhaps dif-



ficulties in determining hQ may have aided  in the  process.



     The  evaluation  statistics   for  the    S3  category



(isothermal)   appear in Table  6.9 c.   The  ranks of  the



                           6-29

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 models are:



         (1)  Van der Hoven  (1967)



         (2)  Weisman (1976)



         (3)  Peters (1975)



         (4)  Plate (1971)



         (5)  Venkatram (1977)



         (6)  Raynor et al. (1975)



The Van der Hoven (1967)  formulation has  one  of  the  highest



RMSE values,  which implies that most of the  error involved



in the equation is systematic and can be attributed to  the



coefficient  in Equation  2.1.  The Raynor  et  al.  (1975)



equation, which ranks last in this  category, appears to do



so because of the lapse rate term and singularity problems



as discussed before.



     Finally,  the more typical overwater stable category



(S4) results indicate that the Weisman  (1.976) equation per-



forms the best.  The ranks of  the models  are:



         (1)  Weisman (1976)



         (2)  Van der Hoven (1967)



         (3)  Peters (1975)



         (4)  Raynor et al. (1975)



         (5)  Plate (1971)



         (6)  Venkatram (1977)



and the  statistical  results appear  in  Table  6.9 d.   It is



apparent   that   the   Van der Hoven  (1967)   formulation



contains  a large  systematic   error, even  for  the   stable



                           6-32

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-------
overwater case.   The closeness of the  3rd,  4th and 5th
ranks makes  interpretation difficult.   It is clear,
however,  that the  Venkatram (1977)  formula performs poorly
under the prevalent  conditions of  a stable overwater
boundary  layer.
     Based on these  three  different types of  analyses,
using the two available  data bases,  it  appears  that
Weisman's (1976)  formulation predicts the TIBL heights
best.   Weisman's equation was used  in  the TIBL modules for
the various   fumigation models that are  compared  statisti-
cally in  the  next chapter.
                          6-34

-------
 7.0  COASTAL DISPERSION MODEL EVALUATION



     In this section  results of both  the overall model



evaluation  (all  data)  and  specific cases  (daily data)  are



presented.   In  addition, attempts are made to gain insight



into the reasons for  better  model performance for certain



meteorological  conditions.  The  CSFM, MSFM and  two varia-



tions  of MSFM  (empirical  and downdraft) models  are



examined.



 7.1  OVERALL EVALUATION



   7.1.1 RESULTS



     Scatterplots  (Figures 7.1 a-d)  of  the predicted  vs.



observed values  of each model  were generated since  they



represent an initial  means  of  readily  displaying  the



various relationships between 0 and P values.  The various



general error  patterns of the models  are apparent with



respect to  the  a  = 0  (intercept), b = 1 (slope)  prediction



line.  The  MSFM model  appears to have  the least  scatter



about  the  perfect prediction line  although all models



exhibit considerable  scatter, especially in predicting



large  concentration  values.  Three of the models tend to



show an underprediction of concentration values while  the



MSFM model  gives slight overprediction  of concentration



values.  These  scatterplots provide  a qualitative  initial



means of determining under and overprediction, but they say



nothing about   the quantitative  magnitude of error  or  the



accuracy.



                           7-1

-------
        600
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Figure  7.la:
Observed  vs  predicted concentration values  for
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                              7-2

-------
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Figure  7.1b:
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the CSFM  model.
                              7-3

-------
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Figure  7.1c:
Observed  vs predicted concentration values  for
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                              7-4

-------
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Figure 7.Id:
Observed vs  predicted concentration values for

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                             7-5

-------
     A listing  of  the various summary measures,  regression
coefficients and difference measures that  give a better
understanding  about  the degree of error appear  in Table
7.1.  The U vs F  summary measures indicate  that on the
average  the  CSFM, MSFM/empirical modification  and
MSFM/downdraft modification underpredict  concentration
values while MSFM slightly overpredicts.   The  MSFM model
exhibited the  smallest average error  of 26,  while  the
empirical modification had the largest average  error of
-117.  A comparison of  SQ  and Sp with regard to how close
the two  standard  deviations approach each other gives a
relative  indication of how well  a model performs.  Thus,
from Table 7.1  it  appears that the  MSFM model  is best able
to describe the observed variability.  The MSFM/empirical
modification  deviation  difference is over 100 (large
compared  to the other three models), which  suggests that
this modification is not able to completely describe some
of the larger concentrations and variability.
     The  two measures which are  not univariate summary or
difference statistics  are the regression  coefficients.
They have been  included for completeness, since they are
used to  compute  the more representative  measures such as
RMSEs.   Willmott  (1984) mentions two problems in  the
interpretation  of  a and b.   The  first problem is  that the
two coefficients are not independent of one another and the
second, related problem,  involves   correlation  analysis
                           7-6

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between the  coefficients and  other summary  variables.
Ideally,  however,  an outcome  of a = 0.0 and  b  = 1.0 is
desired.   This condition  is most  closely met by  the MSFM
model.  It is difficult  to interpret the other model coef-
ficient values  since some of  the "a" values  are rather
large, yet  the "b" values are extremely small  (see for
example the  MSFM/empirical modification,  Table 7.1).
     The difference measures such as RMSE generally agree
with the univariate summary measurements  with regard to the
capabilities of  the various models to predict concentration
values.   Table 7.1 indicates  that the MSFM model has the
least overall RMSE.   The  MSFM model also fits the  criteria
of the systematic error being comparatively small  (although
not  "close"  to zero)  and  of the  unsystematic  error
approaching  the  overall RMSE.
     The difference measures of  the CSFM model  show the
RMSES  to  be comparatively similar to  the downdraft model,
but still comparatively higher  than the MSFM model.   The
MSFM/empirical modification has a  small  difference between
overall RMSE and RMSES,  which implies that this modifica-
tion might contain numerous systematic errors.   Table 7.1
also  indicates that the  MSFM/downdraft  modification
performs  better in terms  of  both overall RMSE and RMSE,.
                                                        o
values than  the  MSFM/empirical modification.
     The relatively   comprehensive difference  measure of a
coastal dispersion  model's ability to predict the  downwind
                           7-8

-------
concentration,  the  index  of agreement  (d), suggests



(following Willmott,  1982)  the percentage of the potential



for error in predicting concentrations  that has  been



explained by the model.   Thus for  the MSFM model, 76% of



the potential for error  has  been explained by  the model.



The d  values for the other models are  in the middle-to-



upper 40th percentile range,  which is considerably less



than the MSFM model.



   7.1.2  DISCUSSION OF RESULTS



     The above  results  suggest that the  appropriate rank-



ings of the models  in terms of performance should be:



          (1)  MSFM



          (2)  MSFM/downdraft modification



          (3)  CSFM



          (4)  MSFM/empirical modification



The high d value clearly stands out as the most  striking



difference measure in supporting the  relative  accuracy of



the MSFM model.   The high d value implies  that there is low



error in the MSFM model  results when compared to the other



models.  Most of this error in MSFM is comparatively unsys-



tematic  and would therefore  be harder to correct than a



systematic error.



     The two variations  of  the MSFM model  (empirical and



downdraft modifications)  in  fact show higher degrees of



systematic error, which would suggest that these variations



do little to  enhance the  concentration  predictability of



                           7-9

-------
MSFM.  The univariate summary measures also imply that MSFM
is the most accurate model, especially given the ability  of
So to emulate Sp.
     The MSFM/downdraft model  ranks second  in terms  of
potential accuracy  for  several reasons.  The d value  of the
MSFM/downdraf t model, when  compared to the two remaining
models (MSFM/empirical  modification and  CSFM),  is higher.
Secondly,  even though the  systematic  error of both the
downdraft and CSFM  models is equal, the unsystematic  errors
do indicate a big discrepancy,  with  the  downdraft model
having the better RMSE value.  Thirdly,  comparative  values
of the slope of the predicted  vs observed  best fit line
alone suggest that  the  MSFM/downdraft model outperforms the
remaining two models.   Lastly,  the summary univariate
statistics, although not showing a closeness in the average
sense of <0 and P~ for the downdraft model  compared to the
CSFM model,  certainly show  the better  ability of the
downdraft model to  reproduce  the scatter  as evidenced  by
the SQ and Sp values.
     The CSFM model, while ranking a close third behind the
MSFM/downdraft  model,  outperforms  the  empirical
modification, particularly in the  areas  of univariate sum-
mary measures and RMSEs.   In terms of univariate  summary
measures, the  CSFM model clearly  shows  a  closer agreement
when    comparing  U   and  f   than   the   MSFM/empirical
modification.  The  CSFM model also shows a somewhat  closer
                           7-10

-------
agreement between  SQ  and S_ values  than  the MSFM/empirical
modification.   A RMSE comparison between the  two models
illustrates  the quantitative problems associated with the
empirical modification.  The  RMSES  nearly approaches the
overall  RMSE,  indicating  the possibility of  systematic
errors in the empirical  modification, particularly given
the wide difference in the univariate summary measures of (D
and P~ and also  SQ  and S_.  For these reasons, the empirical
modification  is ranked fourth.
     It is important  not to base  the argument for the best
performing model just on the  quantitative description of
model  results.  Significant physical differences exist
between  the  two base models  (i.e.,  CSFM and MSFM)  and
between MSFM  and its variations (empirical  modification and
downdraft  modification).  These physical differences can
only be adequately presented  in the  qualitative,  descrip-
tive  sense by looking  at  the common physical parameters
(such as treatment of dispersion coefficients)  that are
used by these models.
     Physical  differences  between  the base models of CSFM
and MSFM are  found in the treatment  of the  dispersion coef-
ficients (a  and 
-------
base models and the MSFM  variations stem from  the use of
uniform,  instantaneous vs  non-uniform,  non-instantaneous
mixing assumptions.
     The problem of the change in dispersion  coefficients
across  the TIBL interface  was  addressed as early as the
original  Lyons and Cole  (1973)  model.  The split sigma
concept used in CSFM relies on the basic premise that the
horizontal dispersion in  the  stable zone can  be charac-
terized by a dispersion  coefficient ffys> which  is deter-
mined by the standard Pasquill-Gifford  (PG)  curve.  The PG
coefficients were constructed  from data taken  over flat
terrain and refer  to  ground-level, neutrally buoyant tracer
sources,  not elevated sources.   The  averaging  time to
determine  the coefficients was  three minutes and the
concentration measurements were made out to only  about 800
meters from the ground-level release.
     Pasquill and  Smith (1983) caution against the applica-
tion  of the PG coefficients  without regard to terrain or
circumstances.   Use of  the PG  type coefficients  has  been
shown  in summary form to be unrepresentative of  diffusion
in coastal areas (see,  for example, MacRae  et al., 1983).
In addition, an application of the  EPA  RAM model, modified
by using the Lyons and Cole (1973) approach for a power
plant in Wisconsin (Ellis  et al., 1979), indicated that the
PG coefficients were  not helpful  in predicting ground-level
concentrations  under fumigation  conditions.  In  addition,
                           7-12

-------
use of Turner's  stability criteria by CRSTER has  been shown
to be  biased toward neutral  stability  by  Weil  and Jepson
(1977) and Weil  (1979).
     The MSFM  approach, on  the other  hand, allows  for
direct calculation of a   based on  the  influence of self-
induced  plume  turbulence created by plume  momentum and
buoyancy.  This  means that, following Briggs (1975), o- s is
proportional to plume  rise  only,  since  ambient  turbulence
in the stable air is negligible.   This  is  physically more
realistic  than the method  for determining  o-    by CSFM,
which  relies on the empirical PG  curves  that are  not
expected to be valid for the above conditions.
     If the plume remains in the stable layer a long time
then low frequency eddies  could cause  significant meander.
Observations indicate 
-------
effective stack height) to the dispersion coefficient



This factor (He/8)  is  based on empirical arguments given in



Chapter 3.0 by Turner  (1970),  who assumed  that the  plume



spreads outward at 15  degrees and that »yfi is independent



of source height.



     The more  realistic and  useful "state of  the art"



method of determining  horizontal diffusion  in the unstable



convective TIBL has been outlined by Lamb (1978) and Willis



and Deardorff  (1978).   The dispersion  coefficient  is both



physically obtained from the w*  parameter, which represents



the convective velocity scale in the  TIBL  and by assuming



that a  ~ x.   The assumption  that 0  ~ X  has  shown  to be



valid by Maul et al. (1980).  Venkatram and Vet (1981) sug-



gest  that the enhanced  plume  spreading in the convective



boundary layer is caused  by a conversion of downdraft ver-



tical  kinetic energy into horizontal kinetic energy upon



the air hitting the ground.   Venkatram (1977) has  shown,



however,  that heat flux decreases with downwind distance;



thus w* is basically  invariant.  This  assumption  may need



further field testing.



     Both base models  assume instantaneous, uniform verti-



cal mixing of fumigant within the TIBL  (i.e., 
-------
Thus the  amount of  plume interception by the TIBL is a
maximum,  since the plume is entrained into the TIBL fairly
soon  after  being  emitted  into the  stable marine air.
However,  if the TIBL is not as steep,  the plume  entrains
through a greater TIBL surface area  and thus can become
non-uniform and not  mix down  instantaneously.  In addition,
the fumigant may not become instantaneously entrained over
a large downwind distance  and  could  wind up "smeared out"
over a large downwind distance.
     The  MSFM/empirical modification assumes that  at the
initial plume-TIBL intersection  (point where the lower part
the plume  first intersects  the TIBL interface), the rate of
interception is small and similar to the final plume-TIBL
interception rate.   The rates of mixing between initial and
final plume-TIBL intersections  are  dependent on water tank
empirical  values for  fast  and slow entrainment.
     The  plume is expected to exhibit higher ground-level
concentrations closer to the  stack  under fast entrainment
conditions.  Under slower entrainment conditions the plume
concentration will be more  spread-out since the fumigant is
entraining over a broad TIBL interface.   Under increasing
thermal stratification the plume will exhibit less growth
and thus  have faster entrainment in the marine air, yield-
ing higher concentrations (Kerman,  1982).  Increasing TIBL
stratification,  however,   aids  in  decreasing  TIBL growth
and  therefore  decreasing  entrainment.  One  can see  how
                           7-15

-------
difficult it is to determine  qualitatively whether fast or
slow entrainment  is occurring  and then apply  the
appropriate non-dimensional t  to represent  fumigant dis-
persion  in the convective TIBL.   Kerman  (1983), in fact,
states that the normalized entrainment rates for  the NEMP
experiments ranged from 0.055  to 0.21.  The rates were
consistently larger  than those  obtained by  Deardorff  and
Willis (1982)  in their water tank experiments.
     Deardorff  and  Willis  (1982)  also make  the assumption
that  entrainment is constant  throughout the convective
boundary layer.   This assumption may not  qualitatively hold
all the time,  however, since in a TIBL the  entrainment rate
could vary as a function of TIBL interface  structure.
     In the  case analysis sections  to  follow it has also
been noticed that the point of  maximum  concentration  for
the  MSFM/empirical modification  has been pushed downwind
considerably farther than either  observed  values  or  the
other model's output values.   This observation is consis-
tent  with the  faster  observed entrainment  argument of
Kerman  (1983) above.  The reason given  by Deardorff and
Willis (1983) for the displacement  of the  fumigation zone
downwind is the representation of the  initial laboratory
plume as being compact  at the point  of  TIBL interception,
such  that  
-------
     The NEMP  plume on the average had a ratio of  
-------
quantitative and qualitative arguments.
 7.2  THE JUNE 1, 1978 CASE
     The mesoscale meteorology associated  with the NEMP-I
group  of  experiments has  been  described  by Kerman et  al.
(1982), Hoff et al.  (1982) and Misra and Onlock (1982).   In
summary, June 1, 1978 was characterized by  high pressure
over the  NEMP area  which  produced  light northerly  winds
during the very early morning  hours,  shifting to southwest
winds by 0900 EOT.
     The 0800  EOT plume lidar  profile taken at the  stack
indicated the plume bearing to be 165 degrees, or offshore.
Lidar  measurements taken  at  1030 EDT  indicated a  plume
bearing of 12'degrees, or onshore.  This was also confirmed
by  10  meter tower  winds which  shifted to a southwesterly
direction  (onshore) around  0900  EDT.   The land-water
temperature  difference  at this  time  was  3  degrees
(increasing to 10 degrees by day's end), which aided in  the
development of the TIBL.
     Data presented by Kerman  et  al.  (1982)  indicated that
the  TIBL  reached a  maximum between  1000  and 1100 EDT  and
then gradually decayed during the afternoon period.  Kerman
et al.  (1982) suggests that early morning light winds  along
with rapid surface heating  aided in  the development of  a
deep initial TIBL.  He also attributes the sharp increases
in  wind  speed  aloft   to  the  suppression  of  the  TIBL
during the day.  One  interesting  note  from the  boundary
                           7-18

-------
layer study  is the observation of a shallow inversion layer
at the shoreline  through  1200 EOT  replaced by the creation
of a shallow superadiabatic  layer  by  1300  EDT.  This could
be attributed to  the  presence of warmer water close to the
shore  creating  a shallow superadiabatic layer.   It is
believed that its depth (hQ)  was not significant enough, as
compared  to the hQ  observed by  Gamo  et al.  (1982)  and
SethuRaman  et al.  (1984),  to  influence  the ground-level
concentration.
     Plume measurements described by Hoff et  al.  (1982)
indicate that no fumigation  occurred  until the time period
1000 to 1100 EDT.  This is confirmed  by lidar measurements
which  showed the effective plume height to be 410 m at a
distance of  2.65  km  while MS based TIBL heights  at that
point  were  200  m.   Assuming  no further  spread  in the Z
direction, the plume  would be expected  to impact the TIBL
around 6.5 km downwind.
     Lidar measurements taken  later  in  the day (e.g.,  the
1445  EDT  lidar profile)  indicated  the  effective plume
height to be 380 m at a distance of 1.24 km from the stack.
Now, however, the TIBL has decreased to a height of 325 m
at 7.1 km downwind  thus allowing  the fumigation  zone to
move  inland and increase in  size (Kerman et al., 1982).
Plots  of  effective  stack height  related to TIBL height
appear  in Figure 7.2.  Isopleths of  observed ground-level
concentrations  appear  in  Figure 7.3 (a-h), adopted  from
                          7-19

-------
  6001
  500-
 400-
  300-
.§200-
      WATER
8       12       16
   DISTANCE (km)
                                                     20      24
  Figure  7.2:   Plume-TIBL  relationship  for June 1,  1978.
                            7-20

-------
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-------
Hoff et al.  (1982).  Stack emissions for the day were  about
6000 g s~* of S02 and the plant  was  generating  an  average
of one-third  its  capacity (1300 MW) .
     The MSFM/downdraft model  is  shown  (based  on the
summary statistics  of Table 7.2) to best  predict the
downwind concentrations.   Even  though  the index of
agreement value of the MSFM/downdraf t  model is relatively
close to that of  the MSFM model and the slopes  appear  to be
closely related,  it  is believed the  other measures  such as
0 vs P (MSFM  overpredicts on average by almost  100 ppb) and
RMSE  suggest the superiority of  the downdraft model  under
these conditions.
     One should  note that the overprediction  of the con-
centration values by the MSFM model during the afternoon
period may be because  of the  instantaneous  mixing  assump-
tion not being valid when  the TIBL is suppressed by higher
wind  speeds  aloft and  when the plume is  becoming more
spread-out in the X and  Y directions (see,  for  example, the
isopleths of  Figure 7.3  e and f).
     In addition,  under  higher  wind speeds  (and lower TIBL
heights)  the  downdraft velocities  will  increase since the
downdraft velocity (wd)  is proportionally related to f^Z),
which  is a  function  of (Z/h).   This implies  that more
fumigant will be brought down to  the  ground by downdrafts;
however,  this is   mitigated by the  fact that less fumigant
is available  at  any time  because of the  shallow nature of
                           7-29

-------
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-------
the TIBL.
     Finally, the  ground-level  concentration isopleths
(Figure 7.3 a-h)  also  indicate  that  the  plume  veered  with
the wind.   This  can be observed by eye and more closely
observed by mentally placing a  line  from the power plant
(NGS)  through the pronounced kinks in the coastline side  of
the concentration  isopleths and finally to the maximum
concentration point (i.e., mentally duplicate the plume
centerline).  The fumigation zone  rotated 50 degrees during
the day.  Lyons (1977)  suggests  two reasons for the veering
of plumes  in coastal  environments.  The first reason  is
that  as the plume  experiences vertical  mixing due  to
convection,  the  vertical  wind  shear enhances spreading  in
the Y  direction.   Secondly, flow meander caused by low
frequency  eddies may cause  variations  in  plume spread
downwind.
     Both base models  totally  ignore  the effect of wind
shear.   This means that  spatial determinations  of model
accuracy are limited  to downwind location  (in  terms  of
distance)  of the  maximum concentration as opposed  to
downwind location of the maximum in terms of  both  distance
and direction from  the stack.   Better future parameteriza-
tions of the wind sheer should  aid in characterizing the
veering of  coastal plumes.
 7.3  THE JUNE 6, 1978 CASE
     The mesoscale meteorology  associated with the June  6,
                           7-31

-------
1978 case is similar to the June  1,  1978 case.   The high
pressure system which was over the NEMP area earlier  in the
week had  by June 6th moved  eastward,  providing  a general
southwesterly gradient flow over the NEMP area  during the
morning  hours.   Winds  aloft at  850  mb were  west-
southwesterly at 10  m s  .
     The TIBL  was  observed to grow during the morning
hours,  collapse during the  early afternoon and  then grow
again later in the  day.   Collapsing of the  TIBL  has been
attributed (Kerman et al.,  1982) to  the  turning of the
boundary layer winds from the  southwest during the morning
hours  to  the south  by noon,  thus  contributing to an
increase in stability of the marine air  during  this time
period.   Heat flux data  (Kerman et al,  1982) indicated a
drop in the amount of heat flux around noon, with a short
rise after 1300 EDT.  Kerman et al. (1982) suggest that the
strong heat flux persisted  (although decreased) throughout
the afternoon and contributed to TIBL regrowth.
     Plume fumigation was observed as early as  1000 EDT
although the first model runs were made  based on 1200 EDT
data due to a lack  of some meteorological  input parameters.
The advent of boundary  layer  collapse  is  evident  both from
Figure  7.4 and  from an  examination of  plume  rise data.
Lidar data indicated a  negative plume  rise  around 1230 EDT
and a  suppressed  and comparatively  small  plume rise  by
1400  EDT.  This is a  result  of  the  increased  thermal
                           7-32

-------
  60Oi
  500-
  400
  300-
.§200-
(9
UJ
  100-
                                 1600 EOT
                                            I5OOEDT
         __ TIBL INTERFACES


         	PLUME PATH
                I20O
       PLUME
       RISE
       Ah,
                                                  1700 EOT
      WATER
                                6
     12        16
DISTANCE (km)
24
   Figure  7.4:   Plume-TIBL  relationship for  June  6, 1978,
                                7-33

-------
stratification mentioned earlier.
     Figure 7.5  a-h (Hoff  et al., 1982) show the  observed
concentration  isopleths for  June 6,  1978.  Figures 7.5 b
and c show observed concentrations  for the  pre-TIBL col-
lapse and TIBL collapse time periods, respectively.  Model-
ing results  during the pre-collapse period  indicated that
the MSFM model  was able to  predict concentrations quite
well (see Figure 7.6 for the  1200 EDT model predictions)^.
The CSFM model  totally overpredicts the  concentration
values,  particularly immediately  after 1400 EDT.  It is
difficult to  attribute  the  overprediction in the  immediate
post-TIBL collapse  period  to any one factor.  In  addition,
the CSFM model  predicted a   (estimated to be 285 m) cannot
adequately represent the true a  of about 800 m.
     Fumigation  became very intense  (Figure 7.5  g - h ),
with ground-level concentrations  recorded  as  high  as
782 ppb  after  TIBL regrowth.   The MSFM model,  while not
able to match the exact intensity of the  fumigation event,
was able to  reproduce both  the propagation  of  the
fumigation zone  closer  to the  stack and the relative in-
crease in ground-level  concentration.   The CSFM model was
once again unable to handle  the increase  in  concentration
and the  change in concentration location toward the stack.
This is illustrated in Table 7.3, which summarizes the peak
ground-level  concentration locations for June 6th.
     A  complete  summary  of the  overall  statistics  for
                           7-34

-------
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                   TABLE 7.3
  QUANTITATIVE MEASURES OF COASTAL DISPERSION
               MODEL PERFORMANCE
LOCATION OF MAXIMUM CONCENTRATION DOWNWIND (km)
TIME (EOT)
1200
1400
1500
1600
1700
MSFM
25
28
11
9
13
CSFM
8
6
7
8
12
EMPIRICAL
MODIF.
30
30
20
15
25
DOWNDRAFT
MODIF.
30
30
30
30
29
OBSERVED
17
16
7
9
10
                      7-44

-------
June 6th  appears in Table  7.4.   From the table  one can
readily  see  that the  MSFM model  outperforms the  other
models  in several key areas.   The  index of agreement value
alone is almost  two  times  the  values for the other models,
indicating that  the  MSFM model explains 80% of the error.
Secondly,  the total  RMSE is lower than the other models
total RMSE.   Finally, the  P  and 0 values are very close
together.   Qualitatively, it  would appear that the  MSFM
model is  more suited  to  the  "steady-state"  (in terms of
non-rotating  fumigation zone)  case  than the MSFM/downdraft
mode1.
 7.4  THE JUNE 13, 1979 CASE (NEMP-II)
     June 13, 1979  was characterized  by  a general west-
southwesterly flow.   There were a  few cloudy periods which
inhibited the growth of the TIBL.  Fumigation began rela-
tively  late  in  the  day (after  1500  EDT)  because  of the
variable  nature of  the TIBL.   The plume was found to be
patchy  and spread-out over  the length  of  a traverse taken
at 17.8  km downwind.   Unfortunately, the NEMP-II study did
not have  the spatial  resolution  of  the NEMP-I study, so
detailed surface  concentration isopleths  cannot  be
presented.   It  was  observed, however, that the plume was
nonrotating and  not greatly influenced by wind  shear.
     Figure 7.7  shows the plume  rise  related  to the  TIBL
for 1700 EDT  (judged to be the  most complete meteorological
hour).     All   four    models   show  substantially   less
                           7-45

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 6001
500H
                 TIBL INTERFACES
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     WATER
     12       16
DISTANCE (km)
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Figure  7.7:  Plume-TIBL  relationships for  June 13,  1979,
                             7-47

-------
concentration values than  that observed under the NEMP-I
study.  The  lesser  concentration  values  may be attributed
to meteorological differences, but may also be attributed
to a considerable reduction  in  plant load during NEMP-II.
     Table 7.5 indicates that the MSFM model  is  best able
to  represent the  dispersion of the plume under  these
conditions, although it  is  not as able  to reproduce  the
good  results of NEMP-I.   It is very curious to note that
all four models have a  high systematic error,  which means
that  some  variable within each model  is  causing an error.
Sensitivity analysis (Section 7.6)  may allow some  insight
into  the  important input variables.   From  Table  7.5 it is
also observed that the P~ values fall  generally a factor of
two below  the 0^ values.  This  is  particularly true of  the
MSFM/empirical modification  case, where it is believed that
the very slow entrainment  process, with a comparatively
shallow TIBL, diffuses the plume appreciably, thus creating
small ground-level concentrations.
 7.5  THE JUNE 14, 1979  CASE
     June  14,  1979  was   characterized   by   a   south-
southeasterly wind  early  in the  day.   Later,  the winds
shifted from south to southwest, which caused the plume to
veer during the afternoon similar to the June 1, 1978 case.
The hours  of  1400 .EDT and 1600  EDT were chosen since those
hours provided the most  comprehensive  set of meteorological
and plume measurements.
                            7-48

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     Figure 7.8  shows  the  plume rise related to the  TIBL
for this  case.   The  point of plume-TIBL interception  is
around 4 km.  The point of highest ground-level  concentra-
tion cannot be determined because of  the spatial  limita-
tions placed on NEMP-II,  however, it  is  known that the
fumigation zone extended at least 4 km  based on  SIGN-X and
helicopter data.
     Table  7.6 indicates  that  both  the  CSFM  and
MSFM/downdraft models  perform the best based on index  of
agreement and RMSE values.  The  table shows  that the  CSFM
model on  average underpredicts and the  MSFM model over-
predicts the concentration values.   It  is  seen  again  that
most of the  error associated with the models is  systematic
and therefore can only truly be described  by a  more  com-
prehensive analysis  than given  here.
     The MSFM model is unable to adequately reproduce the
concentrations of this day.  It appears  (from model  output)
that the model senses  the  plume at  4 km and then  brings the
plume down much too  fast.
 7.6  SENSITIVITY ANALYSIS
     The sensitivity analysis  of  the base  models (MSFM and
CSFM) examines the impact of the model input data on the
calculated concentrations.  The sensitivity analysis  will
allow identification of the most critical model  variables.
An evaluation of these critical model variables will aid  in
the  collection  of  data  (i.e.,  what  type  of   data are
                           7-50

-------
   6001
    500-
   1400 EOT
   1600 EOT
       WATER
 12     16
DISTANCE (km)
                                                  20     24
Figure  7.8:   Plume-TIBL relationships  for June  14,  1979,
                             7-51

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needed for predicting concentrations),  quality  assurance

procedures and model  applicability  in the future.

     The  sensitivity analysis  consisted of variations in

the magnitude of each input variable.   June  1,  1978 (1300

EOT) was chosen as  an arbitrary  model hour.  The variables

considered for sensitivity  analysis were:

          (1)  w*/U:  ratio of convective  velocity to mean
                   wind speed   (allows  for some repre-
                   sentation of turbulence)
                r
          (2)  A: as  in h  = A X0-5   (TIBL  height sensitivity)

          (3)  FQ:  Buoyancy flux,  (allows  for some
                 representation of  plume rise)

          (4)  N: Brunt-Vaisalla frequency (allows for
                plume characterization in stable air)

The sensitivity parameters  to be studied for the CSFM model

were chosen on the basis of what is unique to this version

of CRSTER.  Previous  sensitivity studies such as Freas and

Lee (1977) have shown CRSTER to be  more  sensitive to source

parameters than to meteorological parameters.  Thus, only

the A factor in the TIBL formulation has  been chosen  for

CSFM  sensitivity analysis since  this  is  really the only

non-CRSTER input  variable.

     The parameter  w*/u  has been used as a scaling variable

by several authors  (see,  for example, Deardorff and Willis,

1978).  An increase in  the value  implies  increased heat

flux  (i.e.,  solar radiation)  which also implies increased

plume  instability.   This means  that higher values of w*/u

create  more   of  a crosswind  dispersion, thus  moving the

                           7-53

-------
maximum concentration spot closer  to the stack and reducing
ground-level  concentrations.  In the  MSFM model w*/U  is
used in  the  calculation of the  TIBL  crosswind dispersion
coefficient (ffy^)•
     The sensitivity  analysis  of w*/U on  normalized
concentration, C/Q, appears in  Figure 7.9.  It appears from
Figure  7.9 that the physical reasoning of the previous
paragraph holds  true.   The smallest w*/U  factor  (.1)  cor-
responds to both the highest concentration value (C/Q)  and
the farthest downwind peak.  This means  that the  plume  is
not  as  dispersed  (resulting  in higher ground-level
concentrations)  and is advected comparatively  farther
downwind.   Consequently, higher values of w*/U indicated
lower concentrations.  A gradual shift  in the maximum con-
centration location toward the  stack is also seen  from
Figure 7.9.  This agrees with the physical reasoning  of
Lamb  (1979)  with regard  to «r h parameterized by w*/U.
However, use of w*/U  as a dispersion type  parameter
requires good heat flux data input as suggested by Weil and
Brower (1984).
     The factor  A takes  into account all  of  the physics
necessary for computation of the TIBL height.  Thus  the
factor A directly represents the  affect of the TIBL height
variations  on concentration.  Figure  7.10 indicates  the
MSFM  model  sensitivity  to varying  TIBL heights.  Higher
values of A mean  that the TIBL is  steep and  therefore high
                           7-54

-------
          o.isr
           o.io
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          0.05
          0.00
                            10      IS      20
                          Downwind Distance (km)
                                   25
30
                  •—•••••• w*/U= .14
                  A—^ w*/U= .22
                             .30
                                    x
                              w*/U *  .18
                              w*/U>  .26
                              w*/U =  .10
Figure  7.9:
w*/U sensitivity analysis with normalized
concentration.  Lower  w*/U values  yield higher
concentrations.
                              7-55

-------
        O.I5r
        0.10-
      O
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        0.00
                         10      15      20
                        Downwind Distance (km)
                   -• A = 6
                   - • A = 3
	X.  A=4
---^  A= 5
Figure 7.10:  "A"  sensitivity analysis with normalized
              concentration.  Higher  A values mean a steeper
              TIBL,  thus higher and closer to shoreline
              concentration maximums.
                            7-56

-------
concentrations of pollutant should result close to  the
source and in a short fumigation zone.   This is shown in
Figure  7.10 by the  curve going up sharply to C/Q  =  0.14.
Lesser values of A are shown to push both the magnitude of
the maximum concentration  downward and the location  further
downwind.  Very shallow TIBLs  (A =  2)  are shown by Figure
7.10 to cause peak concentrations at or beyond 30 km.   This
is particularly important  in strong,  thermally stratified
onshore  flow where  the TIBL is suppressed and the  plume
will travel far downwind.   This analysis  supports the con-
tention  in Chapter  2  that TIBL height  determination is
critical in coastal dispersion modeling.
     The  use of  FQ  (plume buoyancy)  allows  one  to
implicitly draw conclusions  about the behavior of the  plume
in  the  stable air since FQ is used  in the calculation
of  
-------
  0.15
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                   Downwind  Distance (km)
                                            25
30
          	o  Average Fo    •	•  Fo = -25%

          	A  Fo = -50%    •	*  Fo = +25%

          	x  Fo = +50%
Figure  7.11:
            FQ sensitivity  analysis with normalized

            concentration.   Decreasing  FQ increases

            concentration.
                      7-58

-------
written as:
                  N = [(g/0)(d0/dZ)]°-5              (7.1)
     The average  Brunt-Vaisalla  frequency for the  NEMP-I
and  II  experiments was  determined  to  be 0.0195  s~*  by
Kerman et al.  (1982).  The maximum N  value was 0.0445 s"1.
Figure  7.12  illustrates the  effect of varying  N  on  the
normalized  concentration.
     The higher N values  (i.e., N = 0.0445 and N = 0.0293)
result  in  higher concentrations of  fumigant close to the
source.   The reason for the higher concentration values may
stem from plume suppression because of increased marine air
stability.   This  means the plume has  even less of a chance
to disperse  in  the stable  air and thus becomes more con-
centrated upon TIBL  impaction.   Decreasing  the  value of N
aids  in the  increased  (albeit  small) dispersion  of  the
plume in the  stable air, thus  aiding  in reducing  the
ground-level concentrations after plume impaction.
     It  is  important  to note  that in the sensitivity
analysis for  N,  the TIBL  height is kept constant.   In
reality, however, changing the  Brunt-Vaisalla frequency
will alter  the stability  of  the marine stable air and thus
suppress  or increase the TIBL  height  and  affect
concentrations.   The sensitivity  analysis indicates that
the A variable  used in  the TIBL calculation is the most
sensitive  variable based  on the magnitude  of the  change
in  concentration and  the  spatial   displacement  of  the
                          7-59

-------
         0.25
         0.20 -
         0.15 -
       O
       •^
       O
                    5      10
                         Downwind

                o	o N= .0195
                A	A N= .0244
                       N« .0097
                   15      20     25

                   Distance (km)

                     x	x  N = .0445
                     a	a  N= .0293
                     •	«  N= .0146
30
Figure 7.12:
Brunt-Vaisalla (N)  sensitivity  analysis with
normalized  concentration.  High N  values imply
more stable air above TIBL.
                             7-60

-------
 8.0  CONCLUSIONS

     In this study two coastal  dispersion  base models  (CSFM

and MSFM)  and two variations  of MSFM  (empirical and

downdraft)  have been evaluated.  The study was conducted

using a comprehensive coastal dispersion data  base.  An

independent evaluation was  also undertaken to determine the

best  TIBL  predictive  equation.   The conclusions  of this

study are listed  below.
   (1)  The most significant factor  affecting  plume
        dispersion in coastal areas  is  the  shape of the
        TIBL.   A steep TIBL produces high concentrations
        close  to the stack,   while a shallower TIBL
        results in more diffusion farther away from the
        stack  and consequently lesser ground-level
        concentrations.

   (2)  Several TIBL prediction models  have been identified
        and evaluated with two independent  data bases.
        From this evaluation it is concluded that the best
        predictive TIBL equation is  the Weisman (1976)
        formulation.  Strong consideration  should be
        given  to the use of  an initial  TIBL height term
        when using the Weisman (1976) equation with
        unstable or neutral  marine air.

   (3)  Based  on the analysis of dispersion data from the
        comprehensive NEMP studies it is concluded that the
        MSFM model of Misra  (1980) is the better model for
        predicting ground-level concentrations from stack
        releases at the shoreline.

   (4)  The standard Pasquill-Gifford curves,  even with
        Turner's correction  factor,  do  not  seem appropriate
        to use in coastal areas.  Convective velocity
        scaling appears to be a better  method  for
        characterizing dispersion in the TIBL.  Weil and
        Brower (1984) also arrived at the same conclusion
        in their study of dispersion coefficients.
                            8-1

-------
     The standard air quality models do not  include some of
the necessary modules  (i.e.,  TIBL,  fumigation) required to
handle  the  complexity  of  dispersion in coastal  areas.
These models  should therefore be modified before being used
to simulate  shoreline meteorological conditions such as
fumigation or trapping.  Modifications to the models should
be undertaken to incorporate  a trapped plume algorithm as
in the CSFM model.  Caution should also be used in applying
the MSFM model to inland coastal releases.
     The  effects  of wind  shear  on plume  dispersion
particularly  near the TIBL interface need to be determined.
The literature survey undertaken for this study  indicates
that  no statistical model  takes  into account shear.  The
affect of rotating winds  with  time  because  of  sea
breeze/mesoscale influences  has  also not  been simulated by
the models.
     The plume data presented  by  Hoff et  al.  (1982)  and
used  in the  study along with  the physically  known non-
steady state  condition of the fumigation zone  and  varia-
tions in TIBL height suggests the  need for  a strong mobile
monitoring component in any coastal dispersion study.  Many
times during  the Nanticoke  study mobile monitors were able
to track the plume and record high concentrations, while
nearby fixed  monitors indicated low concentrations.
     Finally, it is  suggested that  a comprehensive  study
such  as  the  one  recommended  by the  Brookhaven  coastal
                            8-2

-------
workshop (SethuRaman, 1983) be undertaken to corroborate



the  results  of this  study.   The coastal dispersion



models  should  be  re-run  on the  new  data  and  cross-



comparisons  should be made between the two studies.
                           8-3

-------
 9.0 RECOMMENDATIONS


     The present  study  using  the Nanticoke  data  set

suggests Misra's model as the best for estimating downwind

concentrations of material released from  a tall stack at

the  coastline.   Following are the parameters that need to

be determined in order to  use Misra's model:


Stack Parameters
••— • •  —..i      	                               r

  Plume buoyancy -  FQ  (m^s~^)

  Source strength - Q  (g s )

  Stack height - HS (m)
     •

Overwater Parameters

  Brunt-Vaisalla frequency - N

     The Brunt-Vaisalla  frequency  is  given  by:

N = [(g/0)d0/dz]l'  , where 6 is the mean potential tempera-

ture (K) in the surface-based  inversion  layer  and d0/dz is

the mean temperature profile.

       The mean temperature profile  over water should be

measured offshore ideally, but coastal  measurements  will

be  acceptable  if  the temperature difference represents

unmodified  air and the measurements are made  close  to the

water.
                           9-1

-------
Overland  Parameters



  Surface heat flux - HQ (W m~2)



     The  value of  downwind surface heat flux over land is



required to estimate the  TIBL height and  convective



velocity  scale used in diffusion parameterization.   This



value is difficult to obtain.   Eddy correlation  using



direct measurements  of fluctuations of temperature  and



vertical velocity is probably the best  method,  but



would require research-grade instrumentation.   In  the



absence  of such  measurements, indirect methods  using



temperature  gradients (Stunder and Sethu Raman,  1985)  or



approximations  based on  solar radiation (Lyons  et al.,



1983) can be employed,  but  the errors involved  in such



usage should be kept in mind  while applying the  results.



     The  temperature gradient method  involves using values



of mean temperatures measured at two  different  levels from



a tower  or  vertical soundings and  an estimation of eddy



diffusivity  for heat KR, so that:



                  HQ  =  PCpKH  dfl/dz



where p is  air  density and  CD  is the specific heat  at



constant  pressure.   One approximation for K^ is to assume



it to be equal  to  the eddy diffusivity for  momentum,  KM,



which is equal to u*kz for neutral conditions  in the



surface  layer.  Here u*  is  the friction velocity, k is



von  Karman's constant  and   z   is  the  height  above  the



surface.   The  friction velocity can  be obtained  from mean



                          9-2

-------
wind profiles in the atmospheric surface layer.

     The method based on solar radiation is of the form:
              H0  =  pcp,AHcsin( * ts/DL)

where  ^  is  the solar insolation  factor,  HC is 20%  of  the

solar  constant, t  is the  time  since  sunrise and  DT   is
                  O                                   J-l

the length of day.


Other parameters of interest are:


  Mean wind speed at stack height in the stable layer - Us

  (m s"1)


  Mean wind speed in the TIBL - Um (m s"1)
  This can be obtained from tower measurements over land,
  provided the tower is about 100 m high.


  Convective velocity scale - w*  (m s  )
  This is given by the equation:
               w* = (gH0h/pcpTA)
                                1/3
  where g is the acceleration due to gravity,  h is the TIBL
  height and the other terms are as defined.
  Average temperature in the TIBL - TA (C)
  This can be obtained from tower measurements or vertical
  soundings.
Mean  values of  the  constants  a^,  &2 and  a3  maY  be

obtained  by  experimentally  determining  values  of   FQ,

us' azs an<^ ''ys an<^ then solving  Equation 3.14:


                          t2/3               t < 4.5/N
         =  a2                               t > 4.5/N

     ys  -  a3 
-------
where terms are as defined on page  3-17.
Based on Nanticoke data, values of a-^ and a.-$ were observed
to be  0.4  and 0.67,  respectively (Misra, 1980a).  With t
equal to 4.5/N  and a^ equal  to 0.4  (Misra, 1980a), through
substitution a2 may be determined  from Equation 3.14 as:

                  a2  =   1.1(F0/USN2)1/3

Coefficient c, used in  the equation  for plume rise (refer
to the  Evaluation  Function routine in the MSFM program) ,
may  be  obtained  by   experimentally   determining  values
of Ahs,  FQ,  U_   and   x  and then  solving  the  equation:

               Ahs =  c(F0/Us)1/3(x/Us)2/3

where  Ahs  is  plume rise, FQ is plume buoyancy,  Us is the
mean wind  speed  at  stack  height in the  stable layer and x
is the downwind distance  (Misra and Onlock,  1982).  Values
of this coefficient were observed  to  be  1.3  (1978 Nanticoke
data)  and  0.9 (1979   Nanticoke  data).  Misra and Onlock
(1982)  note that these values are  quite lower  than the
recommended value of  1.6  (Briggs,  1975).   The discrepancy
is  considered a  result of  the higher  value  (~0.8)  of
entrainment constant obtained for  the Nanticoke plume.
                            9-4

-------
 10.0  REFERENCES
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	, and W. Lyons, 1972: The impact of the Great Lakes on
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Deardorff, J.W. 1972: Numerical investigations of neutral
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                            10-1

-------
	 and G.E. Willis, 1983: Response to ground-level
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	 and G.E. Willis, 1982: Ground-level concentration
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	 and G.E. Willis, 1975: A parameterization of
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Dooley, J.C., 1976: Fumigation from power plants in the
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Ellis, H.P., P. Lui, C. Bittle, R. Delarid, W. Lyons and
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Gamo, M.S., 1981: A study on the structure of the free
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     Pollution and Resources  (Japan) #19, 89 pp
                            10-2

-------
	, S. Yamamoto, O. Yokoyama and H. Yashikado, 1983:
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	,  1982: Airborne measurements of the free convective
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Hewson, E.W., G.L. Gill and G.J. Walke, 1963: Smoke
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     , 1944: Meteorological investigations in the
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Hoff, R.M., N.A. Trivett, M.M. Millan, P. Fellin,
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     Nanticoke shoreline diffusion experiment,
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     Atmos. Environ, 16, 439-454

	 and F.A. Froude, 1979: Lidar observations of plume
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Holzworth, 1978: Estimated effective chimney heights
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Johnson, W., 1972: Validation of air quality simulation
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Kerman, B.R., 1983: Response to ground-level concentrations
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     Atmos. Environ, 17, 1030-1032

       1982: A similarity model of shoreline fumigation.
     Atmos. Environ., 16, 467-477
                            10-3

-------
	, R.E. Mickle, R.V. Portelli and N.B. Trivett, 1982:
     The Nanticoke shoreline diffusion experiment/ June
     1978-11 Internal Boundary Layer Structure.
     Atmos. Environ., 16, 423-437

Lamb, R.K., 1982: Diffusion in the CBL.  In; Atmospheric
     Turbulence and Air Pollution Modeling by F. Nieuwstadt
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	, 1978: A numerical simulation of dispersion from an
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     Atmos. Environ., 12, 1297-1304

Lenschow, D.H, 1970: Airplane measurements of planetary
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     874-889

	 and P.L. Stevens, 1980: The role of thermals in the
     convective boundary layer.  Bound. Layer Meteor., 19,
     509-532

Lindsey, C. and J. Ramsdell, 1983: Fumigation potential at
     inland and coastal power plant sites.  NUREG/CR-3352
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Lui, 1977: A literature review of boundary layer models.
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     Environmental Protection Agency

	, 1975: Turbulent Diffusion and Pollutant Transport
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     and Environmental Impact Analysis, American
     Meteorological Society, Boston, MA 136-208

	, C.S. Keen and J.A. Schuh, 1983: Modeling mesoscale
     diffusion and transport processes for releases within
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     Nuclear Regulatory Commission.  NUREG/CR - 3542

     ^  K. Dooley, L. Keen, J. Schuh and K. Rizzo, 1974:
     Detailed field measurements and numerical models of
     SO2 from power plants in the Lake Michigan shoreline
     environment.  APAL, U. of Wisconsin-Milwaukee,  218 pp

     _, and H.S. Cole, 1973: Fumigation and plume trapping
     on the shores of Lake Michigan during stable onshore
     flow.  J. Appl. Meteor., 12, 494-510
                            10-4

-------
MacRae, B.L.,  R.J. Kaleel and D.L. Shearer, 1983:
     Dispersion coefficients for coastal regions.  United
     States Nuclear Regulatory Commission, NUREG/CR 3149,
     45 pp

Maul, P.R., F.R. Barber and A. Martin, 1980: Some
     observations of the meso-scale transport of sulphur
     compounds in rural east midlands.  Atmos.  Environ.,
     14, 339-354

Misra, P.K., 1982: Dispersion of non-buoyant particles
     inside a convective boundary layer.  Atmos. Environ.,
     16, 239-243

	, 1980a:  Dispersion from tall stacks into a shoreline
     environment.  Atmos. Environ., 14, 396-400

	, 1980b:  Verification of a shoreline dispersion model
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     501-507

	 and R. Onlock, 1982: Modeling continuous fumigation
     of the Nanticoke generating station plume.
     Atmos. Environ., 16, 479-489

	 and P. McMillian, 1980: On the dispersion parameters
     of plumes from tall stacks in a shoreline environment.
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Moore, G.E., T.E. Stoeckenius and D.A. Stewart, 1982: A
     survey of statistical measures of model performance
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     EPA-450/4-83-001

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     Nanticoke area.  ARB-TDA Report Number 61-80  August,
     314 pp

Pasquill, F. and F.B. Smith, 1983: Atmospheric Diffusion,
     Third Edition.  Ellis Howard Limited, England  437 pp

Peters, L.K.,  1975: On the criteria for the occurrence of
     fumigation inland from a large lake.  Atmos. Environ.,
     9, 809-816

                            10-5

-------
Plate, E.J.,  1971: Aerodynamic characteristics of
     atmospheric boundary layers.  United States Atomic
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     Formation and characteristics of coastal internal
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	, P. Michael, R.M. Brown and S. SethuRaman, 1975:
     Studies of atmospheric diffusion from a nearshore
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     Analysis of lower atmospheric data for diffusion
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	, 1982b: Proceedings of the Workshop on Coastal
     Atmospheric Transport Processes.  Brookhaven National
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                            10-6

-------
Turner, D.B.,  1970: Workbook of Atmospheric Dispersion
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                            10-7

-------
Willmott, C.f 1984: On the evaluation of model
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                            10-8

-------
 11.0  APPENDIX

     Listed below is the computer code for running the
Misra Shoreline Fumigation Model on the UNIVAC computer
system.
                                       r********************
C MISRA SHORELINE FUMIGATION MODEL WITH THE TWO VARIATIONS:
C      1. DOWNDRAFT
C      2. EMPIRICAL (DEARDORFF)
C MODIFIED FOR EPA/SRAB IN FINAL FORM - FEBRUARY, 1987
C
C THE PROGRAM CONSISTS OF FOUR PARTS:
C
C
C
C
C
C
1. MAIN PROGRAM
2. SUBROUTINE CALPK
3. FUNCTION EVAL (USED BY CALPK)
4. SUBROUTINE SIMP (USED BY CALPK FOR SIMPSON'S RULE
   CALCULATION)
Q********************* MAIN PROGRAM ***********************
C  THE FOLLOWING CODE IS THE MAIN PROGRAM WHICH BASICALLY
C  ALLOWS FOR INPUT OF THE DATA FILES (BOTH INTERACTIVE AND
C  FROM INPUT FILES) AND OUTPUT OF THE CONCENTRATION DATA.
C  NOTE:  THE DATA INPUT FILES SHOULD BE INPUT USING
C  @ STATEMENTS.  ALSO, REMEMBER THAT ONE INPUT DATA FILE
C  IS USED FOR MET INFO, WHILE THE OTHER INPUT DATA FILE IS
C  USED FOR RECEPTOR ORIENTATION.  CHANGE DATA FILE INPUT
C  CAREFULLY 	 WATCH THE FORMAT/NAMELIST COMMANDS.

C
C  DEFINE VARIABLES:
C
C   A     =  TIBL A factor, given by:
C            ((2*HO)/(RHO*CSUBP*DTHDZ*U))**0.5
C     RHO    =  atmospheric density
C     CSUBP  =  specific heat at constant pressure
C   B     =  w*/U
C   BPARM =  plume buoyancy — Fo in Misra (1980) (m4s-3)
C   CA    =  coefficient "c" in the equation:
C            DELTAh = c (Fo/U)**l/3(X/U)**2/3
C            (see Misra and Onlock, 1932).
C     DELTAh  =  plume rise
C   DTHDZ =  potential temperature gradient overwater  (S)
C   Fo    =  plume buoyancy
C   HO       heat flux
C   HSTK  =  stack height
C   N     =  Brunt-Vaisalla frequency
C   NR    =  number of receptors

                            11-1

-------
C   Q     =  source strength
C   T     =  ambient temperature over land
C   UM    =  mean wind speed in the TIBL
C   US    =  wind speed at stack height in the stable  layer
C   X     =  downwind distance

      DIMENSION COMENT(20,6),
      TITLE(20)/XPP(200),CANS(200),YPP(200)
      COMMON/ONE/ XP,YP,A,B,UM,US,H,HSTK,CN,BPARM,CA
C     SET UP NAMELIST SPECIAL FORTRAN INPUT COMMAND
      NAMELIST /METIN/ A,B,UM,US,BPARM,Q,T,DTHDZ,NR,HSTK
      DATA BLKSS /'   '/
      DATA JA /'YES'/
      WRITE (6,100)
100   FORMAT ( '1 MISRA SHORELINE  DISPERSION MODEL USING',
     #' SIGMA Z GROWTH METHOD...'//' ORIGINALLY MODIFIED',
     #' BY MARK STUNDER - NORTH CAROLINA STATE UNIVERSITY',
     #' FOR SRAB — 10/84'//)
C
C   DETERMINE WHAT VERSION OF THE  MODEL WILL BE USED
C
      WRITE (6,90)
90    FORMAT('1 WHICH VERSION OF THE MODEL WOULD YOU',
     #'LIKE ?')
      WRITE (6,91)
91    FORMAT (' ENTER: 1=BASE 2=DEARDORFF 3=DOWNDRAFT  ')
      READ (5,92) 1C
92    FORMAT(II)
      WRITE(6,110)
110   FORMAT (' ENTER DESCRIPTIVE  TITLE USING UP TO 80',
     #'CHARACTERS')
      READ (5,120) (TITLE(I),1=1,20)
120   FORMAT (20A4)
121   CONTINUE
      WRITE(6,130)
130   FORMAT (' ENTER UP TO 20 COMMENTS.  END COMMENTS',
     #'WITH A BLANK LINE. ')
      1=0
135   1=1+1
      READ(5,140)(COMENT(J,I),J=1,20)
140   FORMAT(20A4)
      IF  (COMENT(1,I) .NE. BLKSS  .AND. I  .LT. 20) GOTO 135
      NC=I-1
145   CONTINUE
      WRITE(6,150)
150   FORMAT(//' ENTER METEOROLOGY AND SOURCE VARIABLES:  ')
      WRITE (6,160)
160   FORMAT (' EXAMPLE:  '/'&METIN A=5.69,B=0.99,CA=1.0',
     #'UM=7.0,US=7.5,BPARM=614.,Q=5340.,T=300. ',
     #'DTHDZ=-1.31,NR=28,HSTK=198.  ')
                            11-2

-------
C     READ IN NAMELIST (METIN) DATA
      WRITE(6,165)
165   FORMAT(' NOTE:  YOU CAN USE @ADD FILE.ELEMENT HERE  ')
      READ(5,METIN)
C   INPUT SPECIAL METEOROLOGICAL VARIABLES
      WRITE (6,236)
236   FORMAT('1 WHAT IS YOUR VALUE OF N ?  ')
      READ (5,237)CNNN
237   FORMAT(IX,F6.4)
      CN=CNNN
      WRITE(6,240) CN
240   FORMAT(/' THE S TO THE 1/2 PARAMETER IS:  '  ,F6.4)
C     CALCULATE DTHETA DZ FROM N VALUE
      DTHDZ=(CN*CN*T)/9.8
C
C      INPUT HEAT FLUX
C
161   WRITE (6,158)
158   FORMAT ('1 WHAT IS THE OVERLAND HO IN W/M2  ?  ')
      READ (5,159) HO
159   FORMAT (F4.0)
C
C     DETERMINE A
      A=((2.*HO)/(1004.*1.275*DTHDZ*UM))**0.5
C
169     DO 170 J=1,NC
171   FORMAT(IX,20A4)
170   WRITE(6,171)(COMENT(II,J),11=1,20)
      WRITE(6,175)
175   FORMAT(//)
C
      WRITE(6,180) A
180   FORMAT(/' THE TIBL A FACTOR IS:',F7.2)
C
      WRITE(6,190) B
190   FORMAT*/' B=W*/UM =',F4.2)
C
      WRITE (6,195) UM
195   FORMAT (/' THE MEAN WIND SPEED IN THE TIBL  IS:',F5.1)
C
      WRITE (6,197) US
197   FORMAT (/' THE WIND SPEED AT STACK HEIGHT IS:',F5.1)
C
      WRITE(6,200)  BPARM
200   FORMAT(/' THE BUOYANCY PARAMETER IS:',F5.0)
C
      WRITE(6,210) Q
210   FORMAT(/' THE EMISSION RATE IS:',F6.0)
C
      WRITE(6,211) HSTK
211   FORMAT(/' THE STACK HEIGHT IS:',F6.0)

                            11-3

-------
      WRITE(6,220) T
220   FORMAT(/' THE AMBIENT TEMPERATURE OVER LAND IS',
     #' lX,F5.1fIX, 'DEC. K')
C
      WRITE(6,230) DTHDZ
230   FORMAT(/' THE OVERWATER LAPSE RATE IS: ' ,F5.3)
C
      WRITE (6,231) HO
231   FORMAT('1 THE HEAT FLUX IS', IX,F4.0,IX,'W/M2  ')
C
C     READ IN RECEPTOR LOCATIONS  (USER INPUTTED)
244   WRITE(6,250)
250   FORMAT(IX,' ENTER RECEPTOR LOCATIONS  IN X AND  Y',
     # ' COORDINATES ')
C
      WRITE(6,260)NR
260   FORMAT( '1 YOU MUST INPUT',IX,12,IX, 'RECEPTOR PAIRS')
      WRITE (6,265) NR
265   FORMAT (IX,'INPUT 999 AFTER',IX,12,IX, 'PAIRS,  BUT',
     # ' MAYNOT BE NES')
      WRITE(6,270)
270   FORMATdOX,' X LOCATION', 1 OX,' Y LOCATION')
      DO 280 1=1,NR
      READ(5,281) XPP(I),YPP(I)
281   FORMAT(2X,F6.0,15X,F6.0)
      F=BPARM
       IF (XPP(I) .EQ. 999  .OR. YPP(I) .EQ.  999) GOTO  330
       XP=XPP(I)
       YP=YPP(I)
C
C                 CALL TO CALPK SUBROUTINE
C   ** BRINGS BACK THE CONCENTRATION VALUES  FOR  PRINTING  **
C
      CALL CALPK(ANS,IFLAG,ERROR,IC)
       CANS(I)=ANS
C      THIS CONVERTS ANSWER TO PPB
      CANS(I)=CANS(I)*Q/(2.6049*1.E-06)
280   CONTINUE
C        PRINT OUT CONCENTRATION VALUES
330   WRITE(6,300)
300   FORMAT('1 RECEPTOR LOCATIONS AND CONCENTRATIONS  IN',
     #' PPB  ')
      WRITE(6,310)
310   FORMAT(// 2X,' X LOCATION',10X, ' Y LOCATION',10X',
     # ' CONCENTRATION')
      DO 315 1=1,NR
       WRITE(6,320) XPP(I),YPP(I),CANS(I)
320    FORMAT(2X,F6.0,15X,F6.0,16X,F8.3)
315        CONTINUE
C      280 CONTINUE
                            11-4

-------
      WRITE(6,350)
350   FORMAT(' DO YOU WANT ANOTHER HOUR?')
      READ (5,360) IRESP
360   FORMAT (A4)
      IF (IRESP  .NE. JA)GOTO 335
      WRITE (6,370)
370   FORMAT(' WILL THE STACK PARAMETERS BE DIFFERENT?')
      READ (5,360) JSTK
      JSREAD=0
      IF (JSTK .EQ. JA) JSREAD=1
       GOTO 121
335   WRITE (6,340)
340   FORMAT (' END OF MODEL RUN')
      STOP
C   DEBUG UNIT(6),INIT,SUBCHK,SUBTRACE
      END
                            11-5

-------
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
C     SUBROUTINE CALPK
C
C     DEFINE VARIABLES:
C
C     A    = A IN H=AX**0.5   (TIBL height "A" factor)
C     ACC  = Desired accuracy of answer
C     BL   = Boundary layer height
C     EVAL = Name of function whose integral is desired
C     H    = Plume height
C     PI     Constant 3.1415927
C     UM   = Mean wind speed in the TIBL
C     US   = Wind speed at stack height in the stable layer
C     XP   = Distance from source along wind
C     YP   = Distance from source cross wind
C
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
SUBROUTINE CALPK(ANS,IFLAG,ERROR,IC)
      EXTERNAL EVAL
      COMMON/ONE/XP,YP,A,B,UM,US,H,CN,BPARM,CA,HSTK
      REAL LB
C   THIS LITTLE SECTION INSURES AGAINST ERRORS WITH SMALL
C   NUMBERS
      ACC=10.0E-6
      PI=3.1415927
      IF(XP.GT.0.001)GOTO 1000
      AREA=0.0
      ERROR=0.0
      ANS=0.0
      IFLAG=0.0
      GOTO 100
1000  LB=10.00
      ANS1=0.0
C    NEED TO DETERMINE TRAVEL TIME IN STABLE AIR
C    THIS IS FROM MISRA (1980a) (4.5/N)*US
      XP1=(4.50/CN)*US
C
C    GET TIBL HEIGHT
C
      BL=A*SQRT(XP)
      IF(XP.GE.XP1)GOTO 12
      CALL SIMP(EVAL,LB,XP ,ACC,ANS,ERROR,AREA,IFLAG,IC)
C   USE CALL TO SIMP IN VARIOUS WAYS DEPENDING ON WHERE
C   PLUME HITS TIBL DOWNWIND
      GOTO 10
12     CALL SIMP(EVAL,LB,XPl,ACCfANS,ERROR,AREA,IFLAG,1C)
      CALL SIMP(EVAL,XP1,XP,ACC,ANSI,ERROR,AREA,IFLAG,1C)
10    ANS=ANS+ANS1
100   RETURN
C      DEBUG UNIT  (6),SUBCHK,INIT,SUBTRACE
      END

                            11-6

-------
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
C     EVALUATION FUNCTION
C     DEFINE VARIABLE:
C     BL  = AX*SQRT(X)
C     CYS = Constant for SIGMA YS (a3 in Misra 1980a)
C     CZS = Constant for SIGMA ZS (al or a2 in Misra 1980a)
C     D     Time = X/US
C     EVALl, C - Name of function whose integral is desired
C     HSTK = stack height
C     VARZS  = VARZ*VARZ
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
C
      FUNCTION EVAL(X,IC)
      COMMON/ONE/XP,YP,A,B,UM,US,H,HSTK,CN,BPARM,CA
      REAL MF(2)
      IFLG=0
      ICFLG=1
C   MAKE THINGS SIMPLER BY CALLING LARGE QUANTITIES A
C   SIMPLE VARIABLE
      F=BPARM
      FU=F/US
      FN=4.50/CN
      IF(X.LE.0.001)GOTO 10
      D=X/US
      CZS=0.40
      CYS=0.67
   -   CH=CA*(FU**(l./3.))
      VARYS=CYS*(D**(2./3.))*(FU**(l./3.))
C   THIS IS THE DISPERSION COEFFICIENT SIGMA Y IN STABLE
C   AIR PER LAMB 1978,1979,1982
      BL=A*SQRT(X)
      BL1=A*SQRT(XP)
C     CLIMIT=3. *BL1/B
C     IF((XP-X).LT.CLIMIT)ICFLG=2
C     ICFLG=1
C
C   FIRST PIECE OF MISRA'S GAUSSIAN DISTRIBUTION FUNCTION
C   EQUATION
C
      MF(!)=!./(2.*3.14159*BL1*UM)
C     MF(2)=1.78/(6.28138*B*UM)
C     SIGMA Z IN STABLE AIR PER LAMB 1979
      VARZ=1.1*(FU/(CN*CN))**(!./3.}
      VAR=B*(XP-X)/3.0
C   IF((XP-X).GT.BL1/B)
C   VAR=(B*(BLl**(l./3.))*((XPX)**(2./3.)))/3.
      IF(D.GT.FN)GOTO 200
C   *D(TIME) LESS THAN AND EQUAL TO LIMITED*
C   CALCULATE PLUME RISE
      H=(CH*(D**(2./3.)))+HSTK
      VARZ=CZS*(D**(2./3.))*(FU**(1./3.))

                            11-7

-------
C   DERIV=
C         ((UM**(2./.3.))/(CZS*(X**(2./3.))))
C        *{(132./X)-A/(6*SQRT(X)))
C   CALCULATE THE VALUE OF THE DERIVATIVE.  WHEN LOOKING AT
C   THIS PART, HAVE MISRA (1980) HANDY
      DERIV =(-l./6.)*(A*UM)/(CZS*(F**(l./3.)))
     #*(X**(-7./6.)) +
     #(HSTK * UM)/(CZS*(F**(l./3.)))*(2./3.)*(X**(-5./3.))
C
C   BRANCHING — DEPENDS ON VALUE OF 1C  (WHAT VERSION
C   OF THE MODEL YOU WANT).
C       1 = BASE  2 = DEARDORFF  3 = DOWNDRAFT
C       THIS BRANCHES TO VERSION 2 - DEARDORFF
C
       IF (1C .EQ. 1 .OR. 1C .EQ. 3)GOTO 950
       TDP=B*(XP/BL1-X/BL)/4.
        IF (TOP .EQ. 0)GOTO 10
        IF (TOP .GE. DGOTO 950
         DERIV=DERIV*(3.-2.*TDP)*TDP*TDP
950     VARZS=VARZ*VARZ
        GO TO 300
C
C     *D(TIME) GREATER THAN LIMITED*
C
200   VARZS=VARZ*VARZ
      DERIV=A/(2.*SQRT(X)*VARZ)
        IF(IC .EQ. 1 .OR. 1C .EQ. 3)GOTO 300
C       FURTHER BRANCHING FOR DEARDORFF
        TDP=B*(XP/BLl-X/BL)/4.
         IF(TDP .EQ. 0)GOTO 10
         IF(TDP .GE. DGOTO 300
         DERIV=DERIV*(3.-2.*TDP)*TDP*TDP
300   SIGS=(VARYS*VARYS+VAR*VAR)
      BLDIFS=(BL-H)*(BL-H)
C
C   TIBL DECISION: DID PLUME HIT TIBL ??
C   NOW WE NEED TO CALCULATE CONCENTRATION
C   THE ALOG IS A FANCY WAY OF TAKING AN EXPONENTIAL IN  THE
C   ORIGINAL FORTRAN CODE.  WE HAVE NOT TAMPERED WITH  IT.
C
      Cl=-.5*(BLDIFS/VARZS+YP*YP/SIGS)
      C=ALOG(DERIV)+Cl-(ALOG(SIGS))/2.0
      IF(ABS(C).GT.70.0)GOTO 10
C   TAKE EXP OF WHOLE EXPRESSION .... BEST  TO  HAVE MISRA
C   1980 HANDY HERE
       EVALL=EXP(C)
C        THIS BRANCHES TO VERSION  3 - DOWNDRAFT
C
       IF(IC .EQ. 1 .OR. 1C .EQ. 2)GOTO  666
                            11-8

-------
C   NOTE:  G{Z) = 0.623*L, WHERE L=A*X**l./2.
C   (TIBL HT. IS L)
C   THIS WAS OBTAINED BY SOLVING THE INTEGRAL USING CRC
C   HANDBOOK
C
        GZ=1.78*A*(X**l./2.)
        GZTEM=(((GZ*0.225*UM)/(XP-X))-.l)**2.
C       DETERMINE SIGMA W
C       B = WSTAR/UM
C       SIGMAW = .37*WSTAR
C
        WSTAR = B*UM
        SIGMAW=.37*WSTAR
C
        GZTEM=(GZTEM/(SIGMAW**2.))*{-.5)
        TEM = EXP(GZTEM)
        XTEM=((A*UM*(X**l./2.))/(.284*SIGMAW*(XP-X)))*0.225
       EVALL=EVALL*TEM*XTEM
C
c     ****** END OF DOWNDRAFT ROUTINE ******
C
C       CFACT=0.
C     IF(ICFLG.NE.2)GOTO 666
C     ARG=-((((1.632*BL1)/((XP-X)*B))-0.198)**2)
C     CFACT=(l./((XP-X)))*EXP(ARG)
C     IF(ABS(ARG).GT.70)CFACT=0.
666   CONTINUE
C       RENAME A PIECE OF THE MISRA GAUSSIAN EQN TO XF
      XF=MF(1)
C     IF(ICFLG.NE.1)XF=MF{2)
C     MUTIPLY THE PIECE BY THE REST OF THE GAUSSIAN EQN
      EVAL=EVALL*XF
C     IF(ICFLG.NE.1)EVAL=EVALL*CFACT*XF
8889  FORMAT(1X,I2,3(2X,E16.5))
8888  FORMAT(1X,I2,7(2X,E12.4))
      GOTO 20
10    EVAL=0
20    CONTINUE
C      DEBUG UNIT(6),SUBCHK,INIT,SUBTRACE
      END
                            11-9

-------
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
C     SUBROUTINE SIMPSON
C   SIMP IS AN ADAPTIVE, ITERATIVE CODE BASED ON SIMPSON'S
C   RULE.  IT IS DESIGNED TO EVALUATE THE DEFINITE INTEGRAL
C   OF A CONTINUOUS FUNCTION WITH FINITE LIMITS OF
C   INTEGRATION
C
C   DEFINE VARIABLE:
C     A,B   = Lower and upper limits of integration
C     ACC   = Desired accuracy of ans.
C     ANS   = Approximate value of the integral of F(X)
C             from A to B
C     AREA  = Approximate value of the integral of
C             ABS (F(X)) from A to B
C     ERROR = Estimated error of ans.
C     F     = Name of function whose integral is desired
C     IFLAG =  1 for normal return
C              2 If it is necessary to go to 30 levels or
C                use length.
C                Error may be unreliable in this case.
C              3 If more than 2000 function evaluations
C                then complete the computations and error
C                is usually unreliable.
C
ccccccccccccccccccccccccccccccccccccccccccccccccccccccccccc
C
      SUBROUTINE SIMP(EVAL,A,B,ACC,ANS,ERROR,AREA,IFLAG,1C)
      DIMENSION FV(5),LORR(30),FIT(30),F2T(30),F3T(30),
     #DAT(30),ARESTT(30),ESTT(30),EPST(30),PSUM(30)
C     SET U TO APPROXIMATELY THE UNIT ROUND-OFF
      U=9.0E-7
C
C     INITIALIZE
C
      FOURU=4.0*U
      IFLAG=1
      EPS=ACC
      ERROR=0.0
      LVL=1
      LORR(LVL)=1
      PSUM(LVL)=0.0
      ALPHA=A
      DA=B-A
      AREA=0.0
      AREST=0.0
      FV(1)=EVAL(ALPHA,1C)
      FV(3)=EVAL(ALPHA+0.5*DA,1C)
      FV(5)=EVAL(ALPHA+DA,1C)
      KOUNT=3
      WT=DA/6.0
      EST=WT*(FV(1)+4.0*FV(3)+FV(5))

                            11-10

-------
1     DX=0.5*DA
      FV(2)=EVAL(ALPHA+0.5 *DX,1C)
      FV(4)=EVAL(ALPHA+1.5 *DX,1C)
      KOUNT=KOUNT+2
      WT=DX/6.0
      ESTL=WT*(FV(1)+4.0*FV(2)+FV(3))
      ESTR=WT*(FV(3)+4.0*FV(4)+FV(5))
      SUM=ESTL+ESTR
      ARESTL=WT*(ABS(FV(1))+ABS(4.0*FV(2))+ABS(FV(3)))
      ARESTR=WT*(ABS(FV(3))+ABS(4.0*FV(4))+ABS(FV(5)))
      AREA=AREA+((ARESTL+ARESTR)-AREST)
      DIFF=EST-SUM
C
C     IF ERROR IS ACCEPTABLE GO TO 2.  IF INTERVAL  IS TOO
C     SMALL OR TOO MANY LEVELS OR TOO MANY FUNCTION
C     EVALUATIONS, SET A FLAG AND GO TO  2 ANYWAY.
C
      IF(ABS(DIFF).LE.EPS*ABS(AREA))GOTO  2
      IF(ABS(DX).LE.FOURU* ABS(ALPHA) )GOTO 5
      IF(LVL.GE.30)GOTO 5
      IF(KOUNT.GE.2000)GOTO 6
C
C     HERE TO RAISE LEVEL, STORE INFORMATION TO PROCESS
C     RIGHT HALF INTERVAL LATER.  INITIALIZE FOR  'BASIC
C     STEP' SO AS TO TREAT LEFT HALF INTERVAL.
C
      LVL=LVL+1
      LORR(LVL)=0
      FIT(LVL)=FV(3)
      F2T(LVL)=FV(4)
      F3T(LVL)=FV(5)
      DA=DX
      DAT(LVL)=DX
      AREST=ARESTL
      ARESTT(LVL)=ARESTR
      EST=ESTL
      ESTT(LVL)=ESTR
      EPS=EPS/1.4
      EPST(LVL)=EPS
      FV(5)=FV(3)
      FV(3)=FV(2)
      GOTO 1
C
C     ACCEPT APPROXIMATE INTEGRAL SUM.   IF IT WAS ON A LEFT
C     INTERVAL GO TO 'MOVE RIGHT'. IF A RIGHT INTERVAL
C     .ADD RESULTS TO FINISH AT THIS LEVEL.  ARRAY
C     LORR(AMNEMONIC FOR LEFT OR RIGHT)  TELLS WHETHER LEFT
C     OR RIGHT INTERVAL AT EACH LEVEL.
2     ERROR=ERROR+DIFF/15.0
3     IF(LORR(LVL).EQ. 0)GOTO 4
      SUM=PSUM(LVL)+SUM

                           11-11

-------
      LVL=LVL-1
      IF(LVL.GT.1)GOTO 3
      ANS=SUM
      RETURN
C
C     'MOVE RIGHT'.  RESTORE SAVED  INFORMATION  TO PROCESS
C     RIGHT HALF INTERVAL.
C
4     PSUM(LVL)=SUM
      LORR(LVL)=1
      ALPHA=ALPHA+DA
      DA=DAT(LVL)
      FV(1)=FIT(LVL)
      FV(3)=F2T(LVL)
      FV(5)=F3T(LVL)
      AREST=ARESTT(LVL)
      EST=ESTT(LVL)
      EPS=EPST(LVL)
      GOTO 1
C
C     ACCEPT 'POOR' VALUE.  SET APPROPRIATE  FLAGS.
C
5     IFLAG=2
      GOTO 2
6     IFLAG=3
      GOTO 2
C      DEBUG UNIT (6),SUBCHK,INIT,SUBTRACE
      END
                            11-12

-------
                                    TECHNICAL REPORT DATA
                            (Please read Instructions on the reverse before completing)
1. REPORT NO.
 EPA 450/4-87-002
                              2.
                                                            3. RECIPIENT'S ACCESSION NO.
4. TITLE AND SUBTITLE
 Analysis and  Evaluation
 Fumigation Models
of Statistical  Coastal
                                                            5. REPORT DATE

                                                              February  1 Qfi7
                                  6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)

 S.  SethuRaman
                                                            8. PERFORMING ORGANIZATION REPORT NO
                                                             10. PROGRAM ELEMENT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
 Department of  Marine, Earth and  Atmospheric Sciences
 North Carolina State University
 Raleigh, NC  27695-8208
                                   11. CONTRACT/GRANT NO.
12. SPONSORING AGENCY NAME AND ADDRESS
 Monitoring and  Data Analysis Division
 Office of Air Quality Planning and  Standards
 U. S. Environmental Protection Agency
 Research Triangle Park, NC  27711
                                                             13. TYPE OF REPORT AND PERIOD COVERED
                                  14. SPONSORING AGENCY CODE
                                    EPA 200/04
15. SUPPLEMENTARY NOTES
 Project Officer:   Jawad S. Touma
16. ABSTRACT

 This report summarizes the result  of a study to evaluate two coastal  dispersion models
 using a comprehensive coastal dispersion data base.   A sensitivity analysis of the
 various model  input parameters  indicates that the  height of the Thermal 'Internal
 Boundary Layer (TIBL) is the most  sensitive variable.   Six equations  to  describe the
 TIBL height are  identified from the scientific literature and compared  using two
 experimental data  bases.  The report concludes that  the Misra Shoreline  Fumigation
 Model using the  Weisman equation to characterize the TIBL is the best coastal fumiga-
 tion model.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                     b.IDENTIFIERS/OPEN ENDED TERMS
                                                                          e.  COSATI Field/Group
 Air Pollution
 Coastal Fumigation  Models
 Lake Shore Fumigation
 Meteorology
18. DISTRIBUTION STATEMENT
 Unlimited
                                               19. SECURITY CLASS (ThisReport)
                                                Unclassified
                                                21. NO. OF PAGES
                                                    214
                                               20. SECURITY CLASS /This page I
                                                Unclassified
                                                                          22. PRICE
EPA Form 2220-1 (Rev. 4-77)   PREVIOUS EDITION is OBSOLETE

-------
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       Include ZIP code.

  13.  TYPE Of REPORT AND PERIOD COVERED
       Indicate interim final, etc., and if applicable, dates covered.

  14.  SPONSORING AGENCY CODE
       Insert appropriate code.

  15.  SUPPLEMENTARY NOTES
       Enter information not included elsewhere but useful, such as: Prepared in cooperation with, Translation of, Presented'at conference of,
       To be published in, Supersedes, Supplements, etc.

  16.  ABSTRACT
       Include a brief (200 words or less) factual summary of the most significant information contained in the report. If the report Contains a
       significant bibliography or literature survey, mention it here.

  17.  KEY WORDS AND DOCUMENT ANALYSIS
       (a) DESCRIPTORS - Select from the Thesaurus of Engineering and Scientific Terms the proper authorized terms that identify the major
       concept of the research and are sufficiently specific and precise to be used as index entries for cataloging.

       (b) IDENTIFIERS AND OPEN-ENDED TERMS - Use identifiers for project names, code names, equipment designators, etc. Use open-
       ended terms written in descriptor form for those subjects for which no descriptor exists.

       (c) COSATI FIELD GROUP - Field and group assignments are to be taken from the  1965 COSATI Subject Category List. Since the ma-
       jority of documents are rmiltidisciplinary in nature, the  Primary Field/Group assignment(s) will be specific discipline, area of human
       endeavor, or type of physical object. The application(s) will be cross-referenced with secondary Field/Group assignments that will follow
       the primary posting(s).

  18.  DISTRIBUTION STATEMENT
       Denote releasability  to the public or limitation for reasons other than security for example "Release Unlimited."  Cite any availability to
       the public, with address and price.

  19.8.20. SECURITY CLASSIFICATION
       DO NOT submit classified reports to the National Technical Information service.

  21.  NUMBER OF PAGES
       Insert the total number of pages, including this one and unnumbered pages, but exclude distribution list, if any.

  22.  PRICE
       Insert the price set by the National Technical Information Service or the Government Printing Office, if known.
EPA Form 2220-1 (R*v. 4-77) (R«».r»«)

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