United States          Office of Water          EPA~440/'5-80-074
                 Environmental Protection     Regulations and Standards    October 1980
                 Agency             Criteria and Standards Division
                                 Washington DC 20480
&EPA         Ambient
                 Water  Quality
                 Criteria  for
                 Thallium





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      AMBIENT WATER QUALITY CRITERIA FOR

                 THALLIUM
                 Prepared By
    U.S. ENVIRONMENTAL PROTECTION AGENCY

  Office of Water Regulations and Standards
       Criteria and Standards Division
              Washington, D.C.'

    Office of Research and Development
Environmental Criteria and Assessment Office
              Cincinnati, Ohio

        Carcinogen Assessment Group
             Washington, D.C.

    Environmental Research Laboratories
             Corvalis, Oregon
             Duluth, Minnesota
           Gulf Breeze, Florida
        Narragansett, Rhode Island

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                              DISCLAIMER
     This  report  has  been reviewed by the  Environmental  Criteria and
Assessment Office, U.S.  Environmental  Protection  Agency,  and approved
for publication.   Mention of trade names or commercial products does not
constitute endorsement or recommendation for use.
                          AVAILABILITY  NOTICE
      This  document  is available  to  the public through  the National
Technical Information Service, (NTIS), Springfield, Virginia  22161.
                                    11

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                               FOREWORD

    Section 304  (a)(l)  of the Clean Water Act  of 1977 (P.L. 95-217),
requires the Administrator  of the Environmental  Protection  Agency to
publish  criteria for water  quality accurately reflecting  the  latest
scientific knowledge on the  kind  and extent of all identifiable effects
on  health  and  welfare which may  be  expected from  the presence of
pollutants in  any body of water, including^ground water.  Proposed water
quality criteria  for the  65  toxic  pollutants  listed under section 307
(a)(l) of  the  Clean Water  Act  were developed  and  a notice  of  their
availability was published for public comment on March 15, 1979 (44 FR
15926), July 25,  1979 (44  FR 43660), and October 1, 1979 (44 FR 56628).
This document  is a revision  of  those  proposed criteria  based  upon a
consideration  of  comments received from other  Federal  Agencies,  State
agencies,  special  interest  groups,  and  individual  scientists.    The
criteria contained in this document replace any previously published EPA
criteria for  the  65 pollutants.   This  criterion  document is  also
published in satisifaction of paragraph 11 of the Settlement Agreement
""n  Natural  Resources  Defense Counci 1. et.  al..  ys. Train,  8 ERC 2120
(D.D.C. 1976), modified, 12 ERC 1833 (D.D.C.  1979).

    The term "water  quality criteria"  is used  in  two  sections  of the
Clean Water Act, section 304  (a)(l)  and section 303 (c)(2).  The term has
a different program  impact  in each  section.   In section 304, the term
represents a non-regulatory,  scientific   assessment of  ecological  ef-
fects. The criteria  presented in  this  publication are such scientific
assessments.   Such  water quality  criteria  associated with  specific
stream uses when  adopted as  State water quality  standards under section
303 become  enforceable maximum  acceptable  levels  of  a  pollutant in
ambient waters.  The water quality criteria adopted in the State water
quality standards could have the same numerical limits as the criteria
developed under section  304.  However, in many situations States may want
to adjust water quality criteria  developed under section 304 to reflect
local   environmental  conditions  and  human exposure  patterns  before
incorporation   into  water  quality  standards.    It  is not until  their
adoption as part  of the  State water quality standards that the criteria
become regulatory.

    Guidelines to  assist  the  States  in   the modification  of criteria
presented  in  this  document,  in  the  development  of  water  quality
standards,  and  in  other water-related programs  of this Agency, are being
developed by EPA.
                                    STEVEN SCHATZOW
                                    Deputy Assistant Administrator
                                    Office of Water Regulations and Standards
                                  111

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                                   ACKNOWLEDGEMENTS
 Aquatic  Life  Toxicity

    William  A.  Brungs,  ERL-Narragansett
    U.S.  Environmental  Protection Agency
David J. Hansen, ERL-Gulf Breeze
U.S. Environmental Protection Agency
 Mammalian  Toxicology  and  Human  Health  Effects

    Paul  B. Hammond  (author)
    University  of  Cincinnati                  *

    Christopher DeRosa (doc. mgr.)  ECAO-Cin
    U.S.  Environmental  Protection Agency

    Jerry F.  Stara (doc. mgr.),  ECAO-Cin
    U.S.  Environmental  Protection Agency

    Thomas  Clarkson
    University  of  Rochester

    Karl  L. Gabriel
    Medical College  of Pennsylvania
   John W. All is, HERL
   U.S. Environmental Protection Agency

   J.B. Lai
   National  Institute of Occupational
     Safety  and Health

   Gordon Newell
   National  Academy of Sciences
Rolf Hartung
University of Michigan

John Carroll
U.S. Environmental Protection Agency

S.M. Charbonneau
Health and Welfare, Canada

Patrick Durkin
Syracuse Research Corporation

David H. Groth
National Institute of Occupational
  Safety and Health

Terri Laird, ECAO-Cin
U.S. Environmental Protection Agency

Steven B. Lutkenhoff, ECAO-Cin
U.S. Environmental Protection Agency
William W. Sutton, EMSL-Las Vegas
U.S. Environmental Protection Agency
Technical Support Services Staff:  D.J. Reisman, M.A. Garlough, B.L. Zwayer,
P.A. Daunt, K.S. Edwards, T.A. Scandura, A.T. Pressley, C.A. Cooper,
M.M. Denessen.

Clerical Staff:  C.A. Haynes, S.J. Faehr, L.A. Wade, D. Jones, B.J. Bordicks,
B.J. Quesnell ,  T.  Highland,  R.  Rubinstein.
                                        IV

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                       TABLE  OF  CONTENTS

                                                            Page

Criteria Summary

Introduction                                                A-l

Aquatic Life Toxicology                                     B-l
  Introduction                    *                         B-l
  Effects                                                   B-l
    Acute Toxicity                                          B-l
    Chronic Toxicity                                        B-2
    Plant Effects                                           B-2
    Residues                                                B-3
    Miscellaneous                                           B-3
    Summary                                                 B-3
  Criteria                                                  B-4
  References                                                B-ll
Mammalian Toxicology and Human Health Effects               C-l
  Exposure                                                  C-l
    Ingestion from Water                                    C-l
    Ingestion from Food                                     C-3
    Inhalation                                              C-5
    Dermal                                                  C-6
    Exposure to Thallium from Food, Water, and Air as a
      Basis for Estimating Daily Absorption                 C-6
  Pharmacokinetics                                          C-7
    Absorption                                              C-8
    Distribution                                            C-9
    Excretion                                               C-ll
    Total Daily Excretion of Thallium as a Basis for
      Estimating Daily Absorption                           C-18
    Body Burden of Thallium as a Basis for Estimating
      Daily Absorption                                      C-22
  Effects                                                   C-23
    Acute, Subacute and Chronic Toxicity                    C-23
    Synergism and/or Antagonism                             C-32
    Teratogenicity                                          C-33
    Mutagenicity                                            C-34
    Carcinogenicity                                         C-34
  Criterion Formulation                                     C-35
    Existing Guidelines and Standards                       C-35
    Current Levels of Exposure                              C-35
    Special Groups at Risk                                  C-37
    Basis and Derivation of Criterion                       C-38
  References                                                C-42

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                              CRITERIA DOCUMENT



                                   THALLIUM



CRITERIA



                                 Aouatlc  Life



    The available data for thallium indicate that acute and chronic toxicity



to  freshwater  aauatic life occur  at  concentrations as low  as  1,400 and 40



ug/1,  respectively,  and  would occur  at  lower  concentrations  among species



that are more  sensitive  than  those tested.  Toxicity to one species of fish



occurs at concentrations  as low  as  20  yg/1  after 2,600 hours of exposure.



    The  available  data for thallium  indicate  that acute  toxicity to salt-



water  aauatic  life  occurs  at  concentrations  as low as  2,130  ug/1  and would



occur  at lower  concentrations  among  species  that  are more  sensitive than



those  tested.   No  data  are  available  concerning  the  chronic  toxicity  of



thallium to sensitive saltwater  aquatic  life.







                                 Human Health



    For the protection of human health from the toxic properties of thallium



ingested through water and contaminated  aauatic organisms, the ambient water



criterion is determined to be  13  yg/1.



    For the protection of human health from the toxic properties of thallium



ingested through  contaminated aauatic  organisms alone,  the  ambient  water



criterion is determined to be  48  yg/1.

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                                 INTRODUCTION

    Thallium  is an element having  the  chemical  symbol  Tl  and is a soft, mal-
 leable,  heavy metal  with  a  silver-white luster (Lee, 1971).  Industrial uses
 of  thallium  include  the manufacture of alloys,  electronic  devices,  and spe-
 cial  glass.   Many thallium-containing catalysts have been  patented  for in-
 dustrial  organic  reactions  (Zitko,  1975).*  Production  and use  of  thallium
 and  its compounds approximated  680 kg  in  1976 (U.S. Dept.  Interior,  1977;
 Zitko,  1975).
    Thallium  has  an  atomic  weight of  204.37,  a melting  point  of 303.5°C,  a
 boiling  point of  1,457 ^ 10°C,  and  a specific  gravity  of  11.85   at 20°C
 (Weast,  1975).  Thallium exists  in either tne  monovalent (thallous)  or tri-
 valent  (thailie)  form,  the  former  being  the  more  common  and   stable  and
 therefore  forming more  numerous  and  stable  salts  (Hampel,  1968).   Thai lie
 salts  are  readily reduced by  common  reducing  agents  to the  thallous  salts
 (Standen, 1967).
    Thallium  is  chemically reactive with air  and  moisture, oxidizing slowly
 in air  at 20°C and more rapidly  as the temperature  increases,  with  the pre-
 sence  of moisture enhancing this  reaction  (Standen,  1967).  Thallous oxide,
 formed  by  oxidizing  the  metal  at low  temperature,   is  easily  oxidized  to
 thallic  oxide  or  reduced to thallium.   Thallous oxide is a very hygroscopic
 compound and has a vapor pressure  of 1 mm Hg at 580°C  (Lee, 1971).  Thallous
 hydroxide is  formed  when thallium contacts water  containing oxygen  (Hampel,
 1968).   While  thallium itself is  relatively  insoluble  in  water (Windholz,
 1976),  thallium compounds  exhibit  a wide range  of  soluoilities,  as  shown in
Table 1.
                                    7C-I"

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                                    TABLE 1

                 Water  Solubilities  of some Thallium Compounds3
Compound
Thallium sulfide
Thallium bromide
Thallium chromate
Thallium chloride
Thallium sulfate
Thallium carbonate
Thallium bromide
Thallium hydroxide13

Thai lium fluoride
Molecular Formula
T12S
TIBr
Tl£Cr04
T1C1
T12S04
T12C03
TIBr
T10H

TIP
Solubility
(mg/1)
220
240
300
2,100
27,000
42,000
160,000
259,000
520,000
780,000
Temperature
(°C)
20
0
60
0
0
15
20
0
40
15
aSource:  Standen, 1967
bWeast, 1975
                                     A-2

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                                  REFERENCES

Hampel, C.A.  (ed.)   1968.   The Encyclopedia of Chemical  Elements.   Reinhold
Publishers, New York.

Lee,  A.G.   1971.    The  Chemistry  of  Thallium.    Elsevier  Publishing  Co.,
Amsterdam.                               *

Standen,  A.  (ed.)    1967.   Kirk-Othmer  Encyclopedia of  Chemical  Technology.
Interscience Publishers, New York.

U.S.  Department of  the Interior.   1977.   Commodity  data summaries.   Bur.
Mines.

Weast, R.C.  (ed.)   1975.   Handbook  of Chemistry and Physics.   56th  ed.   CRC
Press, Cleveland, Ohio.

Windholz,  M.  (ed.)   1976.   The Merck  Index.   9th  ed.   Merck and Co.,  Inc.,
Rahway, New Jersey.

Zitko, V.   1975.  Toxicity  and pollution potential of thallium.  Sci. Total
Environ.   4:  185.
                                     A-3

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Aquatic Life Toxicology*
                                  INTRODUCTION
     The  data  base for the effects  of  thallium on freshwater organisms does
not  permit  any determination  of  the effects  of water  quality  on toxicity.
There  are sufficient data to  indicate  that  thallium is chronically toxic to
fish  and  invertebrate species  at concentrations as  low as approximately 20
ug/1.  Algae  are  also sensitive  with effects  occurring at concentrations as
low as 100 ug/1-
     There  are a  variety of  results  for  thallium  and  saltwater organisms
from tests conducted using  static test  procedures.  No adverse acute effects
were  observed  at  concentrations  lower than  2,130  ug/1.   An embryo-larval
test  with the  sheepshead  minnow resulted  in  adverse  effects  at concentra-
tions  as  low  as  8,400 ug/1,  a  concentration  about  one-half  of  the 96-hour
LCgQ for  that  species.
                                    EFFECTS
Acute Toxicity
     Daphnia magna 48-hour 50  percent  effect  concentrations  were 2,180 and
910 ug/1  (Table 1).   The  fathead minnow was  of similar  sensitivity  with  a
96-hour  LC50   of  1,800 ug/1  (Table  1).   Two  96-hour  LC50  values for the
bluegill  were  132,000  and 121,000 ug/1  which results indicate that this spe-
cies is rather  insensitive to thallium.
     The  saltwater  shrimp species,  Mysidopsis  bahia, was more sensitive than
the tested  fish species  with  an  LC5Q  value of  2,130 ug/1  (Table  1).  The
*The reader  is referred  to  the Guidelines  for Deriving Water  Quality Cri-
teria for the Protection of Aquatic Life and  Its Uses  in  order to better un-
derstand the  following  discussion  and recommendation.  The  following tables
contain the  appropriate  data  that  were found  in  the literature, and  at the
bottom of each  table  are calculations for deriving  various  measures of tox-
icity as described in the Guidelines.
                                      B-l

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 sheepshead  minnow  (U.S. EPA, 1978)  and  the  tidewater silverside (Dawson, et
 al.  1977)  are  similarly  sensitive with  LC5Q values  of 20,900  and 24,000
 ug/1, respectively  (Table  I).
 Chronic Toxicity
     A  life cycle  test with  Daphnia magna  (Kimball,  Manuscript)  has  been
 conducted and  the  chronic value  was 130 ug/1  (Table 2).  The  acute-chronic
 ratio for this species  is  7.0.           *
     An embryo-larval test has  been conducted (U.S. EPA, 1978) with the fat-
 head minnow and  adverse effects were observed  at  the lowest tested thallium
 concentration of 40 ug/1  (Table  2).  Kimball  (Manuscript)  also conducted an
 embryo-larval test  with the  same species and  observed  adverse effects at 81
 ug/1 but  not at 40 ug/1  (Table 2).  When  the chronic value for this  species
 (57  wg/1)   is divided   into  the 96-hour LC5Q,  an  acute-chronic ratio of 32
 results.
     The only chronic  test with  a  saltwater  species  has been conducted with
 the  sheepshead  minnow   (U.S.   EPA, 1978).   No  adverse effects  during  an
 embryo-larval test  were observed  at 4,300  ug/1 (Table 2).  At 8,400 ug/1 ad-
 verse effects  were detected.   The acute-chronic   ratio  for  the  sheepshead
minnow is 3.5.
     Species mean acute and chronic values are summarized in Table 3.
 Plant Effects
     There was a 40 percent  inhibition  of  oxygen  evolution  by the freshwater
alga, Chlamydomonas reinhardi,  exposed  to  a concentration  of 40,800  ug/1
 (Table 4).   The 96-hour  EC,-,,  values for  chlorophyll £  inhibition  and  cell
number of the  alga, Selenastrum  caporicornutum,  was 110 and 100  ug/1,  re-
spectively (U.S. EPA,  1978).
                                      B-2

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     There  was a  50 percent  inhibition  of photosynthesis  by  two saltwater
algal species  at thallium concentrations of 4,080 and 51,200 ug/1  (Table 4).
Residues
     Muscle  tissue of  Atlantic  salmon (Zitko, et  al.  1975) bioconcentrated
thallium  to a concentration  130  times that  in  the  water (Table  5).   The
bluegill  (whole body)  bioconcentrated  thallium 34  times and the tissue half-
life was  greater than 4 days  (U.S. EPA, 1978).
     Zitko  and Carson  (1975) observed bioconcentration factors  of 18 and 12
for the soft shell  clam and blue mussel, respectively  (Table  5).   These re-
sults indicate that saltwater clams and mussels do not bioconcentrate thal-
lium as much as freshwater fishes.
Miscellaneous
     Zitko, et al.  (1975) exposed  Atlantic  salmon  for as long as 2,600 hours
and observed  40 and 70  percent  mortality at  approximately 20  and  45 wg/l»
respectively (Table  6).   No effects were observed  for  other species at con-
centrations close to those affecting the salmon.
     Early development of sea  urchin eggs was inhibited at concentrations of
thallium between 41,000 and 204,000 wg/1 (Table 6).
Summary
     Daphnia magna  and  the  fathead minnow were of  similar acute sensitivity
to  thallium  with  LC^Q  values in  the  range  of concentrations  from  910  to
2,180 yg/1.   The  bluegill  LCgg values  were  about  two orders  of magnitude
higher.    The chronic values for  Daphnia  magna and  the fathead minnow  were
also similar,  130  and  57 ug/1,  respectively.  There were  50  percent reduc-
tions in chlorophyll a_ and  cell  numbers  of  an alga  at  concentrations of 110
and 100 ug/l»  respectively.  The highest bioconcentration  factor  for fishes
                                     B-3

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was' 130 for  muscle  tissue of  Atlantic salmon.  This  species  apparently is
rather  sensitive  to  thallium  with partial  mortality after about 100 days ex-
posure  to concentratons as  low  as 20 wg/1.
     The  sheepshead  minnow and  tidewater  silverside were of  similar sensi-
tivity  to thallium with  96-hour LCgQ values of  20,900 and  24,000 wg/1, re-
spectively.   The  mysid   shrimp  was  more  sensitive  with an  lC,-n  value  of
2,130 wg/1.   Chronic effects  on the sheepshead  minnow were observed at 8,400
wg/1.   There  was  a  50 percent  inhibition of photosynthesis  in  a saltwater
algal species at  4,080 ug/1.  Two bivalve  species were exposed for 40 and 88
days and the bioconcentration factors were less than 20.
                                   CRITERIA
     The  available data  for  thallium indicate  that acute and  chronic  tox-
icity to freshwater aquatic life occur  at  concentrations as  low as 1,400 and
40 wg/1, respectively, and  would occur  at  lower concentrations among species
that are more sensitive than  those  tested.  Toxicity to  one  species of  fish
occurs at concentrations as low  as 20 wg/1  after 2,600 hours of exposure.
     The available data  for thallium indicate  that acute toxicity  to salt-
water aquatic  life occurs  at concentrations  as low as  2,130  wg/1  and would
occur at  lower concentrations   among species  that  are more sensitive  than
those tested.   No  data   are  available   concerning  the  chronic toxicity  of
thallium to sensitive saltwater  aquatic  life.
                                     B-4

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                                                            Table  1.  Acute  values  for thai HIM
to
 I
Species Mean
LC50/EC50 Acute Value
Species Method* (ua/D (W9/D
FRESHWATER SPECIES
Cladoceran, S, U 2,180
Daphnia magna
Cladoceran, S, H 910 1,400
Daphnia roagna
Fathead minnow, FT, M 1,800 1,800
Plmephales promelas
Blueglll, S, U 132,000
Lepofflls macrochlrus
Bluegill, S, U 121,000 126,000
Lepomis macroch i rus
SALTWATER SPECIES
Mysid shriRf>, S, U 2,130 2,130
Hysldopsls bah la
Sheepshead minnow, S, U 20,900 20,900
Cyprtnodon variegatus
Tidewater silverside, S, U 24,000 24,000
Henidia beryl Una

Reference
U.S. EPA, 1978
Klnball, Manuscript
Mwball, Manuscript
Oawson, et at. 1977
U.S. EPA, 1978
*
U.S. EPA, 1978
U.S. EPA, 1978
Dawson, et al. 1977
                                * S = static, FT = flow-through, U = unmeasured, M  = measured


                                  No Final Acute Values are  calculable  since  the mini gun data  base  requirements are not  met.

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                                                           Table 2.  Chronic values for thallium
                                  Species
                                  Cladoceran,
                                  Daphnla magna

                                  Fathead minnow,
                                  Plmephales promelas

                                  Fathead minnow,
                                  Plmephales promelas
                                        LlMltS
                             Method*    (U9/I)
                     Species Mean
                     Chronic Value
                        (ug/l)
                                   FRESHWATER SPECIES

                              LC       100-181          130
                              E-L         <40
                              E-L       40-81            57
      Reference
                                      Kimbal I, Manuscript
                                      U.S. EPA, 1978
                                      KimbalI, Manuscript
CO
 I
Sheepshead minnow,
Cyprlnodon varlegatus
      SALTWATER SPECIES

E-L       4,300-        6,000
          8,400
      U.S. EPA, 1978
                                  * E-L = embryo-larva I, LC = life cycle or partial life cycle
                                                                    Acute-Chronic Ratios
                                                 Species
                                                 Cladoceran,
                                                 Daphnia magna

                                                 Fathead minnow,
                                                 Plmephales promelas
                                       ChronIc
                                        Value
                                        (U9/I)
                                          130
                                           57
                                                 Sheepshead minnow,       6,000
                                                 Cyprlnodon varlegatus
                     Acute
                     Value
                     (ug/l)

                       910
                     1,800


                    20,900
Ratio

  7.0


 32


  3.5

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                                               Table 3.  Species Mean acute and chronic  values  for  thai HIM
 I
-J
Nunber
3
2
1
3
2
1
Species
Blueglll,
Lepomls macrochlrus
Fathead minnow,
Plmephales prontelas
Cladoceran,
Daphnla magna
Tidewater sllverslde,
Menldia beryl Una
Sheepshead minnow,
Cyprlnodon varlegatus
Mysid shrimp,
Mysldopsls bah la

Species Mean Species Mean
Acute Value* Chronic Value
(ug/l) (ug/l)
FRESHWATER SPECIES
126,000
1,800 57
1,400 130
SALTWATER SPECIES
24,000
20,900 6,000
2,130
Acute-Chronic
Ratio"
32
7.0
3.5
                                 * Rank from high concentration to  low concentration  by  species mean  acute value.


                                 **See the Guidelines for derivation of this  ratio.

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                                                          Table 4.  Plant values for thai HUM
Species
Alga,
Ch 1 amydomonas relnhardl
Alga,
Selenastrum capr 1 cornutum
Alga,
Selenastrum capr 1 cornutum
Effect
FRESHWATER SPECIES
40? Inhibition of
oxygen evo 1 ut Ion
96-hr EC50 for
ch 1 orophy 1 1 a
Inhibition
96-hr EC50 for
eel 1 number
Result
(ug/l)
40,800
110
too
Reference
Overnel 1,
U.S. EPA,
U.S. EPA,
1975a
1978
1978
CO
 I
oo
Alga,
Dunallella tertollecta
 SALTWATER SPECIES


50J inhibition of    4,080      Overnel I,  1975b

photosynthesis                                 „
                                    Alga,                          50* inhibition of   51,200      OvernelI, 1975b
                                    Phaeodactylum trIcornutum      photosynthesis

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Table 5.  Residues for thallium
CD
1
VD
Species
Atlantic salmon
( juvenl le),
Sal mo salar
Bluegill,
Lepomis macrochirus
Soft shel 1 clam,
Mya arenaria
Blue mussel,
Myt i 1 us edu 1 i s
B locon cent rat Ion
T 1 ssue Factor
FRESHWATER
muscle tissue
whole body
SALTWATER
edible portion
edible portion
SPECIES
130
34
SPECIES
18
12
Duration
(days)
12.5
28
88
40
Reference
Zitko, et al.
U.S. EPA, 1978
Z 1 tko i Carson
Zltko & Carson

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                              Table 6.  Otter data for thai HIM
 I
H
O
Cladoceran,
Daphnla sp.

Rainbow trout,
Salmo galrdneri

Atlantic salmon
(juveni le),
Sal mo salar

Atlantic salmon
(juvenile),
Salmo salar

Fathead minnow,
Pltnephales promelas

Frog (embryo),
(unidentified)
                                                            Duration          Effect

                                                                     FRESHWATER SPECIES

                                                              3 days     Initial effects


                                                              3 days     Initial effects


                                                          2,600 hrs      LC40
                                                          2,600 hrs
LC70
                                                              7 days     LC50
                                                             56 days     Mortality
                                                               Result
                                                               (U9/I)
                      2,000-
                      4,000

                     10,000-
                     15,000

                         20
       Reference



       Nehrlng, 1962


       Nehrlng, 1962


       Zltko, et al. 1975
45     Zltko, et al. 1975
                        800     U.S. EPA, t978
                        409     0111 ing & Healey,
                                1926
Sea urchin,
Paracentrotus  llvldus
                                                                      SALTWATER SPECIES

                                                                         Cessation of early
                                                                         development of
                                                                         ferti I ized eggs:

                                                                           4 eel I stage

                                                                           8-16 eel I stage

                                                                           Blastula
                                                              204,000

                                                               82,000

                                                               41,000
                                Lai Her, 1968

-------
                                  REFERENCES

Dawson,  C.W.,  et al.  1977.   The  acute toxicity of  47  industrial chemicals
to fresh and saltwater fishes.  Jour. Hazard. Mater.  1: 303.

Dilling, W.J.  and C.W. Healey.   1926.   Influence  of lead  and  the metallic
                                           *
ions of  copper,  zinc,  thorium, beryllium and  thallium  on  the germination of
frogs' spawn and on the growth of tadpoles.  Ann. Appl. Biol. 13:  177.

Kimball, G.   The effects of  lesser known metals and one  organic to fathead
minnows  (Pimephales promelas) and Daphnia magna.  Manuscript.

Lallier, R.   1968.  Investigation  of the  toxicity of thallium  ions  in the
eggs  of the  sea  urchin,  Paracentrotus  lividus.   C.R.  Acad.   Sci.  Paris
267: 962.

Nehring, D.  1962.   Experiments on  the  toxicological  effect of thallium ions
on fish and fish-food organisms.  Zeitz. Fisch.  11: 557.

Overnell, J.  1975a.   Effect  of some heavy  metal ions on photosynthesis in a
freshwater alga.  Pest. Biochem. Physiol.  5: 19.

Overnell, J.   1975b.   The effect  of heavy meals on  photosynthesis and loss
of cell potassium in two  species of marine  algae,  Dunaliella tertiolecta and
Phaedoctylum tricornutum.   Mar. Biol.  29: 99.
                                     B-ll

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U.S.  EPA.   1978.   In-depth  studies on  health  and environmental  impacts of
selected water  pollutants.   U.S.  Environ. Prot. Agency,  Contract  No. 68-01-
4646.

Zitko,  V.  and  W.V.  Carson.   1975.  Accumulation  of  thallium in  clams and
mussels.  Bull. Environ. Contam. Toxicol.  14: 530.
                                          •&
Zitko,  V.,  et al.  1975.   Thallium:  Occurrence in the  environment and tox-
icity to fish.  Bull. Environ. Contam. Toxicol.  13: 23.
                                     B-12

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Mammalian Toxicology and Human Health Effects
                             EXPOSURE
Ingestion from Water
     The major problem in assessing the  amount of  thallium  ingested
from water is the inadequate sensitivity of analytical methods for
thallium.  An almost equally serious problem  is the limited amount
of information available utilizing even the  inadequate methodolo-
gies currently available.  As a matter of  fact,  essentially all the
information available is to be found in two reports.  The  first of
these  is a U.S.  EPA study  which was conducted in cooperation with
the National Heart  and Lung  Institute and the National Center for
Health Statistics.   Its  main purpose was to  delineate the occur-
rence  of  inorganics in  household  tap water  and  relationships to
cardiovascular mortality  rates  (Greathouse,   1978).    The second
study was not concerned  with  average or usual exposures.   Rather,
it was concerned  with worse situations,  namely the concentration of
thallium in the  run-off  from  slag  heaps and holding ponds associ-
ated with ore processing and mining operations  (U.S. EPA,  1977).
     In the first study  grab  samples of tap water were taken from
3,834  homes.   The study began  in  July  1974  and  was  completed in
December 1975.  Multi-elemental analyses were conducted using pro-
ton-induced x-ray emission (PIXE).  The procedure and its charac-
teristics of precision and sensitivity are described in a  separate
report (U.S.  EPA, 1978a).  The  limit of  detectability as applied to
water was 0.3 ppb.  Samples of tap water were collected from 3,834
households which  were randomly selected  from 35 geographic  areas by
                               C-l

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the  Bureau  of Census  to  provide  a "representative" sample of  the
U.S. population.   Thallium  was  detectable in only 0.68 percent of
the  samples.  The  average thallium concentration, when detectable,
was 0.89 ppb. Assuming a water consumption of 2 1/d  for the average
adult, over  99 percent  of adults would consume  <1  ug Tl per day.
     So far  as worse  situations are  concerned, the so-called Cal-
span Report  (U.S. EPA, 1978a) reviews in great detail  the basis  for
concluding that the leaching of  thallium  from ore  processing opera-
tions  is  the major source  of  elevated thallium  concentrations in
water.   Thallium  is  a  trace metal  associated  with copper,  gold,
zinc and cadmium.  Thus, wherever  these metals  have been mined  and
processed, an enrichment of  the environment  with  thallium was also
suspected to occur.   This led  to analyses of  run-offs from mining
and smelting operations involving these other metals.  The sensiti-
vity of the  analytical methodology for thallium was not as good as
for  the tap  water  studies  referred to earlier.  The overall limit
of sensitivity was reported to  be 10  ppb,  but values as low  as 3  ppb
are  reported.  It  is  not clear  how this apparent  shift in sensiti-
vity occurred.  Mines and processing  operations from Washington  and
California to New  Jersey and Pennsylvania were  studied.  The high-
est  concentrations reported  were 30  ppb in  slag  run-off near Kel-
logg, Idaho and  21  ppb in the Colorado River just below  the Big Wil-
liams  River  which  drains  the  Planet Mine,  an operation  in which
copper is extracted from iron ore.  It is not at all  clear as to  how
much of the Colorado River thallium came  from that particular mine,
since this was a generally ore-rich area.   The only  other source of
information  as  to  discharges   from  Canadian  ore  operations  into
                               C-2

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streams  is  a  study by Zitko, et  al.  (1975)  in which he  indicates
concentrations of  0.7-88 ppb.
Ingestion from Food
     Data concerning  the  intake of thallium from food are  sparse.
So  far  as thallium in man's  usual diet  is  concerned,  only  three
studies  are available.   They provide only a limited  indication  as
                                    »
to  what  might  constitute  the total contribution  of  food to  daily
intake under  normal  circumstances.  Vegetables (lettuce, red cab-
bage, green cabbage,  leek,  and endive)  averaged 68.2  ppb  dry weight
(Geilmann, et  al.  1960).   Assuming 85 percent water  content, this
would amount to 10  ppb, wet weight.  From the same  study,  bread con-
tained 0.75 ppb, dry weight.  The  only data  concerning thallium  in
meat report  that  the concentration  in rib  eye beef and  veal  is
<0.5 ppm (Mitteldorf and Landon,  1952).  Due  to  the  poor analyti-
cal sensitivity, this study is  not very helpful.  It  seems  unlike-
ly, however,  that  meats contribute as much thallium to the  total
diet as vegetables.  This  is based on  two  considerations:  1)  vege-
tarians excrete  in their urine  four times as much thallium  as non-
vegetarians (Weinig and  Zink, 1967);  and 2)  the  concentration  of
thallium in human skeletal muscle is  only  approximately  1 ppb  (Wei-
nig and  Zink,  1967).   This raises the  interesting  question as  to
why vegetables should contain so much more  thallium  than meat.   It
is possible that this is related to the relatively high concentra-
tion of thallium in fertilizer.  Geilmann, et  al. (1960) found 37-
230 ug Tl/kg in 4 samples of potash fertilizers containing 35  to  43
percent potassium.   Since   these  studies  were  conducted  on a very
limited number of vegetables  and fertilizer  samples  in Germany,  it
                               C-3

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is difficult to estimate just how  representative  these data  are  of

the situation  in  the  U.S.   In any event, if one accepts that most

dietary thallium  is to be found  in  vegetables and that 10  ppb  is  the

average fresh  weight  concentration,  an estimate can be made as  to

the contribution  of  food  to total intake of thallium in man.  The

average adult consumption of vegetables in the  U.S.  is estimated  at
                                  *
0.38  kg/d  (Toscano,  1975), and  the  total food consumption  is 1.6

kg/d  (U.S. Dep. of Agric.,  1968).   Assuming  the cited concentration

figures are correct  and  they  apply to the average diet of vegeta-

bles, the daily intake of  thallium from  vegetables would be  (0.38)

X (10 jug) or 3.8  jag.  As will be shown  in the  section on Criterion

Formulation, this is probably  a high  estimate.   In all probability,

the data  cited as to  concentrations  of  thallium in a few selected

vegetables are really not  representative of what  is normally eaten

in the category of vegetables.  Based on the solubility character-

istics of thallium,  it  is  also  possible that a good deal of thal-

lium  is leached out during  food preparation.

     A bioconcentration factor (BCF)  relates  the concentration of a

chemical  in aquatic  animals to  the  concentration in the water  in

which they live.  An appropriate BCF  can be  used with data concern-

ing food intake to calculate the amount  of thallium which might  be

ingested from  the consumption of fish and shellfish.  Residue data

for a variety  of inorganic compounds  indicate that bioconcentration

factors for the edible portion of most aquatic  animals is similar,

except that for  some compounds bivalve  molluscs  (clams, oysters,

scallops,  and  mussels) should be  considered  a  separate group.    An

analysis  (U.S. EPA,  1980)  of  data from  a  food survey  was used  to
                               C-4

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estimate  that  the per capita consumption of  freshwater  and  estua-
rine  fish and shellfish  is 6.5  g/day  (Stephan, 1980).   The  per
capita consumption of bivalve molluscs is 0.8 g/day and that of all
other freshwater  and estuarine  fish  and  shellfish  is  5.7 g/day.
     Zitko,  et al.  (1975)  reported  a BCP of 130  for thallium  in
muscle of atlantic salmon, whereas  Zitko  and Carson  (1975)  found
BCP values  of  18  and 12 for the edible portions of the  soft shell
clam and  blue  mussel, respectively.   If  130  and  the geometric mean
of 18 and 12 are used with the consumption  data,  the weighted aver-
age bioconcentration factor for thallium and  the edible  portion  of
all  freshwater   and  estuarine  aquatic  organisms   consumed  by
Americans is calculated to be 116.
Inhalation
     The  concentration  of thallium  in  ambient urban air from six
major U.S.  cities was reported in  a U.S.  EPA study  conducted  by
Battelle  Columbus Laboratories (U.S. EPA, 1971).   The  concentra-
tions of  thallium were  given as weighted  averages  from data  from
all cities:  low, ^_.02; high, 0.1 and typical, <^0.04.
     The  concentration of  thallium  in fly  ash has been  estimated,
however,  and on this basis the ground level concentration of thal-
lium near a coal-fired plant might be 700 ug/m  (Carson  and  Smith,
1977).   This can  hardly be used as a  basis for judging usual expo-
sure for  the general population,  but it  does suggest a worse  case
situation.  Assuming inhalation of 20 m /d  and 35 percent retention
of the thallium-bearing aerosol,  700  ng  Tl/m  would  result  in the
daily absorption of 4.9 ug Tl.  The air level  in Chadron, Nebraska
is stated to be .04-.48 ng  Tl/m .  This may be  the more  typical level
                               C-5

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of exposure  (Carson and Smith, 1977).  Assuming  20 m /d  inhalation
and 35 percent retention, 0.48 ng/m  = 3.4  ng Tl/d from  air.
     Inhalation  of  thallium in cigarette  smoke  may,  on the  other
hand, be a very significant source.   The  urinary  excretion of  thal-
lium  in  smokers  is  about  twice  that in  non-smokers  (Weinig  and
Zink, 1967)  and  the  concentration in cigar  stubs  was  shown  to  be
57-170 ng/g  (Geilmann, et al. 1960f, about  20 times the  concentra-
tion estimated for the diet.
Dermal
     The dermal  absorption of thallium  presumably would normally
occur as  a  result of  bathing and  from  contact with  thallium  in
clothing.  It is virtually  impossible to estimate  the contribution
of these potential sources to total  intake.   Suffice it to say that
the concentration  of thallium in  tap water is  less  than  in  body
tissues (<0.3 tig/1 vs.—" 1 ug/kg in tissues).   From this it  would
seem that the net flux of thallium as a result of bathing would,  if
anything, be outward rather than inward.   As to  thallium in cloth-
ing, there does not appear  to be any information.

Exposure to  Thallium  from Food,  Water and  Air as  a  Basis  for Es-
timating Daily Absorption
     In summary,  this  section  on  various sources of exposure  pro-
vides only a very  broad  perspective as  to  the  relative contribu-
tions of known environmental media to which  the general  population
is exposed.   The  most reliable data, fortuitously,  concern  thal-
lium in drinking  water.   It is possible  to state  with  reasonable
assurance that >99 percent of Americans probably absorb 
-------
3.8 ug/day (see Ingestion from Foods)  and  air  is  probably an insig-
nificant source, being probably no more  than 3.4  ng/day  (see Inhal-
a tion).  If foods other than vegetables are assumed  to  have a con-
centration of 1 jug/kg, then their contribution at approximate con-
sumption levels of 1.2 kg  (total daily consumption of 1.6 kg minus
daily vegetable consumption of  0.38  kg) would be 1.2 ug/day, i.e.
(1.2 kg/day x 1 jug Tl/kg  in  non-vegetable food).  Thus, the total
daily input based on data reviewed above is "Cl ug  (water) + 3.8 ug
(vegetables) +  .0034  ug  (air)  + 1.2 jug (non-vegetable  food) 
-------
which  man  is exposed via  water,  attention will be drawn wherever
possible to the distinction between the  pharmacokinetics of massive
doses  and the pharmacokinetics of small doses.   Unfortunately, such
distinctions can be drawn  only from consideration of animal data.
Absorption
     The only study of gastrointestinal absorption  in man was con-
ducted  in  a middle-aged woman with  terminal osteogenic carcinoma
(Barclay, et al. 1953).  Following oral administration of a single
                204
tracer  dose  of     Tl,  only approximately  0.5  percent  of  the dose
was  excreted in the  feces during the  succeeding  72 hours, while
urinary excretion  rose dramatically.   This suggests that no bolus
   204
of    Tl passed unabsorbed.  Complete  absorption of tracer doses of
204
   Tl  administered orally  in rats  is suggested  by the data of Lie,
et al.  (1960).   They  found approximately the  same fraction of a
                       204
single  tracer dose of    Tl in various organs  at  1,  2 and 7 days
regardless of whether  the  dose was given  orally or by any one of
four parenteral routes.   There  is  no information available concern-
ing  the deposition and clearance of inhaled  thallium aerosols.  As
with almost all metallic salts, the pattern of  deposition of thal-
lium aerosols would  depend upon  particle  size (aerodynamic);  and
the rate of clearance  would depend upon  the solubility of the salt.
From the report of the Task Group on Lung Dynamics  it would be pre-
dicted, however, that all  salts  of thallium  (oxide, hydroxide and
halide  excepted)  would  be cleared rapidly  (days) and  that none
would be cleared slowly  (years) (ICRP, 1966).
     The skin as a route  of absorption  has  not  received much atten-
tion, as is  the  case with most metallic salts.   At one time thallium
                               C-8

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was  applied  to  the skin as an  ointment  containing 3 to 8 percent

thallous acetate.   Numerous cases  of systemic poisoning have been

documented  to  result  from this practice (Munch, 1934).  This does

not mean that skin is a significant portal  of  entry under usual ex-

posure  conditions  however.   The net movement of  thallium through

the  skin is  dependent  on the  concentration gradient, and the con-
                                    *•
centration  of  thallium  to which  the skin  is normally exposed  is

miniscule in comparison  to the concentration  under which signifi-

cant absorption has been demonstrated.

     As a summary  statement  it may be said with reasonable confi-

dence that thallium is completely  absorbed  from all  the usual por-

tals of entry, with the possible exception  of the  skin.

Distribution

     Thallium is widely distributed in the  body.   It is distributed

preferentially to the intracellular space.   Based on  tracer studies

in rats, the apparent volume  of distribution has been calculated  to

be 20 I/kg (Rauws, 1974).  This indicates a high degree of concen-

tration in one or more parts  of the body.   To  some  extent at least,

this preferential  intracellular distribution  is analogous and re-

lated to mechanisms  which favor the  intracellular localization  of

potassium.   Active  transport of  thallium into erythrocytes,  medi-

ated by (Na-K)ATPase,  has been demonstrated by a number of investi-

gators  (Gehring and Hammond,  1964;  Cavieres and Ellroy, 1974).   In

spite of  the considerable  avidity of erythrocytes  for thallium,

Rauws (1974) estimated that,  in rats at  least,  under steady state

conditions 61  percent  was distributed to  the blood cells as com-

pared  to  39 percent  in  the  plasma.   Gibson  and  Becker  (1970)
                               C-9

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similarly reported a cell-plasma ratio of 1.5-2 in rats.  The very


minor degree of preferential  thallium  distribution to blood cells


is probably due to the very high concentration of potassium  in  the


blood, which competes with thallium for active transport.  Factors


other  than  active transport  into  cells must  be  operative  in  the


localization of thallium in various organs and  systems, since there
                                    &
does exist some organ-specific concentration.   Thus,  in both  condi-


tions of normal thallium exposure  and fatal exposure  in man, there


is a tendency for  thallium to  concentrate  in the kidneys,  colon  and


hair (Weinig and Zink, 1967; Cavanagh, et al.  1974).  In  other  re-


spects the distribution of thallium is not  remarkable.


     Thallium distributes rather freely from the maternal circula-


tion to  the  fetus.   The  fetal-maternal ratios of tracer doses of

O C\ A
   Tl in rats  and mice  are  reported to be,  respectively, 0.84  and


0.46 under  steady  state conditions (Gibson, et  al.  1967).  These


observations were made  on gestation days  18  and 19  for  mice  and


rats respectively.   It was also found  that thallium administered on


days 1 and 7 postnatally was distributed in a manner quite similar


to  that  for adult  animals.    In  a later publication,  Gibson  and


Becker (1970)  reported  that simultaneous  thallium ratios in whole


fetuses and  in maternal rat  blood plasma  were approximately 0.07


over a wide range of  thallium infusion rates  (0.2-6.4 mg/min/kg),


indicating that dosage does not seem to alter  the kinetics of dis-


tribution from mother to  fetus.  The  fetal-maternal  ratio in this


instance is not contradictory  to the authors' earlier observation,


cited above, that fetal-maternal ratios in  rats  and  mice are 0.84


and  0.46,  respectively,  since  steady state  conditions  did   not
                               C-10

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prevail in the latter study.  Low dietary potassium did not signif-



icantly alter  fetal-maternal distribution  of  thallium.



     So far as distribution of  thallium  to the  human  fetus is  con-



cerned, there  is essentially no  quantitative  data.  One  report in-



dicates that no thallium was found  in  the  5-month  fetus  of a woman



who died of thallium poisoning.   Thallium was  demonstrated in vari-

                                  **

ous tissues of the mother  (Neal, et al.  1935).  Absence  of detect-



able thallium in this fetus does not rule out  its  presence, even at



abnormally high concentrations since the spectrographic method  used



probably was neither  very  sensitive nor very  precise.   It  is  only



possible to surmise  that fetal concentrations were lower  than ma-



ternal concentrations.   Richeson (1958)  cites one report  in which



thallium was found in the  tissues of a baby whose  mother had taken



1.2 g thallium at term.  The infant died five days  after birth.



Excretion



     There have  been numerous  reports of the  characteristics  of


                                                          204
thallium excretion in animals using both tracer doses  of    Tl and



rather large  (up  to 10 mg/kg)  carrier  doses.   By contrast, there



are only  two  studies reported  of  thallium excretion  in man  from



which may be derived any useful  kinetic constants.  Worse,  each of



these two  studies  involved only a  single subject.   This  serious



limitation must  be  remembered  in  judging the  reliability of  the



safety assessment which ultimately must be made in  this  document.



     The  first  study  traced  the  fate of  an orally-administered


               204
tracer dose of    Tl  given to a middle-age woman with  osteogenic



carcinoma metastatic  to the lungs  (Barclay,  et al.   1953).   The



dose  of  thallium  given  was  0.5  mci,  containing  2.3  mg total
                               Oil

-------
 thallium.   In  addition,  single  oral doses  of  45  mg non-radioactive
 thallium  sulfate  (presumably »  8.7 mg Tl)  were  also given  every  3
 days  until  225 mg had been administered.  Excretion of  radioacti-
 vity  in the urine and feces was determined for  the succeeding  5.5
 days.   It  is  evident  that fecal excretion was  inconsequential as
 compared  to urinary  excretion (Figure 1).   Based on these  data,  a
                                    &  -. 1
 first  order rate  constant of 0.032 day"  was estimated  for excre-
 tion.  The  t^  for  rate of  excretion of  the dose  would  therefore be
 21.7 days.  Based  on a rate  constant  of  0.032 day   , the amount of
 thallium  remaining in the  body  at  the time of death  (24  days after
                   204
 administration  of     Tl)  would  have been 46.3 percent of the dose
 from:

 where:
     A a  percent dose in body at 24  d
     AQ » 100 percent
     k »  0.032
     t •  24 d
     The  amount actually recovered in the body at the time of death
was stated  to be 45  percent.  It is not clear how this  figure  was
                                                 204
obtained.    The  cumulative  urinary excretion of    Tl,  illustrated
 in Figure 1 has a  hyperbolic form  during the first 48 hours, con-
sistent with a first  order  rate  process.  Subsequently, the  cumula-
 tive urinary excretion is  linear with time.   This is  inconsistent
with animal studies and with the only other human  study  discussed.
In these  studies a first order  rate process  prevails,  even  months
following dosing.    The  supplementary  doses  of  thallium  sulfate
                              C-12

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           •S r
              6  (2
                    2«
                                                     120   UZ
                                 MOUJIS
                             FIGURE 1

                      204
     The excretion of    Tl by a human after oral administration of
500 JJG of activity plus  five  45 mg  doses  of thallous sulfate oral-
                   7D4
ly.  The  level of    Tl  in  the  blood at 2, 4,  8,  24,  and 48 hour
intervals after administration  of  the radioactive  isotope is also
included.
Source:  Barclay, et al.  1953
                               C-13

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                                       204
given subsequent to  the single dose of    Tl would  not  likely  have



altered the form of the excretion curve.  These  supplementary doses



no  doubt  increased  total  thallium excretion,   but  this would  not



affect the rate of    Tl excretion since  dilution of the   Tl  pool



with  "cold"  thallium  would precisely  cancel   any  enhancement  of


204
   Tl excretion resulting from  the increased  total thallium concen-

                                    *?•

tration presented  to the kidney.



     The  only  other paper  which  sheds  light   on  the kinetics  of



thallium excretion in man was a  report of a single  case of poison-



ing  (Innis  and Moses,  1978).   Approximately four  weeks following



the  time  of  intoxication a series of  urine  analyses for thallium



were  performed.    These  data   are  presented   in  graphic   form



(Figure 2).  The estimated t,   for urinary excretion  was  30  days



(k = .023 day"1).



     The discrepancy in rate of  urinary  loss of  the body burden  in



the  two above-described  cases  (k = .032 vs. k  = .023)  is not  re-



markable.   The rate  constant  calculated  for the  first  subject was



based on  excretion data which behaved in  a kinetically anomalous



fashion.  On the other  hand,  the rate constant calculated for  the



second subject may have been influenced by  the fact that she was



experiencing clinical manifestations of  thallium  poisoning.  It  is



known from  experimental  studies  in  rats  that  the  rate  of  body



clearance of thallium is considerably slower following a toxic  dose



than following  a tracer dose.  Thus, Gehring  and Hammond (1967) re-



ported a rate constant  for  total  thallium excretion  of 0.0353 day



in rats  receiving a single iv injection of 10 mg Tl/kg  as compared



to a rate  constant of 0.0790 day   in rats receiving a  tracer  dose
                               C-14

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     3.0
     2.0
T1, mg/1
urine
     1.0
     0.5
     0.2
                                       \
                                             X

                     30
60
days
90
                               FIGURE 2

   The Excretion of Thallium in the Urine of  a  Patient, Beginning
       Approximately Four Weeks after  Thallium Intoxication.

                   Source:   Innis and Moses,  1978
                                 C-15

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 «0.1 mg Tl/kg).  These constants were for animals on low dietary
 potassium.  When dietary potassium was  high, tracer doses were more
 rapidly excreted (k = 0.146 day" ).   In summary,  for people not ex-
 periencing overt signs of thallium poisoning,  it  seems that the ap-
 propriate  rate  constant lies between  0.032 and  0.023  day~ .   The
 slower rate constant (0.023)  will be  assumed in the criteria formu-
 lation for purposes of calculating the accumulation of thallium  in
man, since this represents the more conservative approach.
     It should be noted  that excretion of thallium in animals dif-
 fers from excretion in man in two respects.  The rate of excretion
 is much more rapid in animals.   For example, in Gehring and Hammond
 (1967) the  rate constant  for  total  excretion in  rats on  a  high
 potassium diet  was  0.146 day~ .  Lie,  et  al.  (1960)  calculated a
 rate constant of 0.210 day    for  rats receiving single tracer doses
 and Rauws (1974) calculated a rate constant of 0.173 day"  in rats
 receiving single doses  of  10 mg/kg.    The  average  rate  from these
 three studies was 0.18 day" .  Another  major difference between man
 and animals  is  the  relative  contribution of  fecal  and  urinary ex-
cretion.    Whereas the  gastrointestinal  tract seems to  be a very
minor excretory  pathway in  man,  the  rate  of fecal excretion   is
about 3 to 4  times the rate of urinary excretion in  the rat  (Gehring
and Hammond, 1967; Lie, et al. 1960).  In the rabbit the contribu-
 tion of the  two  routes of excretion is about equal (Truhaut, 1952).
     The  rate of urinary  excretion under steady state conditions of
 intake should reflect accurately the  rate of total  thallium absorp-
 tion.   This  proves  to be an extremely  important consideration  in
light of  the fact that reliable estimates of intake based on known
                              C-16

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concentrations  in  food,  air and water are virtually  non-existent.
The  only  published estimate of  total dietary  intake  is 
-------
 increase  thallium  excretion and perhaps dietary intake  (Table  1).
 In the second study  (Goenechea  and Sellier, 1967) no such distinc-
 tion is made, and  the average urinary concentration of  thallium is
 somewhat lower though similar (Table 2).  From the data  in the last
 three  papers it seems  safe  to assume  that  the  concentration  of
 thallium in urine seldom exceeds 1.5  ug/1.   The discrepancy between
 the data in the last two studies, ©.81 vs.  0.23 jug/1, cannot  be  ex-
 plained.  Even if one assumes that the higher  of the two  figures is
 correct and that average daily urinary excretion  is  1.5  Jug/1, aver-
 age daily  thallium excretion in  the urine would be 1.2 ug (0.81
 ug/1 x 1.5 1).
Total Daily  Excretion  of Thallium as a  Basis for Estimating Daily
Absorption
     It  is  useful  to  estimate  total daily excretion  of thallium
 since this can reasonably be assumed  to be  the same as  total daily
 absorption,  at least under  steady state conditions.   To the daily
excretion via the  urine  must be added the following miscellaneous
 routes:
     1)   gastrointestinal excretion  (including cell exfoliation)
     2)   hair
     3)   exfoliating epithelium of  the skin
     4)   sweat
     The  contribution  of gastrointestinal excretion  is probably
very minor in man,  at  least based on the  data of  Barclay,  et  al.
 (1953).  From Figure 1,  it  can  be estimated that cumulative fecal
excretion was 0.5 percent of the dose of    Tl at 72 hours, whereas
cumulative urinary  excretion at  the  same time was approximately 11
percent of the dose.  On  this basis, one  might  add  to the average
                               C-18

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                            TABLE 1

  Thallium Concentration in the Morning Urine of Vegetarians,
           Smokers and Non-smokers with Normal Diets*
Subject
Vegetarian
"
n
Smoker
n
n
Non-smoker
n
it

*Source: We
a
Sex Years of a
D Age Urine sp.g.
F
M
M
M
M
M
M
F
F

inig
C i — ,
40
43
12
28
25
24
26
60
48

and Zink,
.
1.024
1.034
1.032
1.019
1.023
1.018
1.008
1.025
1.030
overall
1967

Ave . Tl , ug/1
Tl, ng/g for group
1.34
1.69
0.92
1.42
0.40
0.69
0.13
0.39
0.53
average



1.28


0.82


0.34

0.81


calculated from the authors' data in the table
                             C-19

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                        TABLE 2


Naturally-Occurring Thallium Concentration in the Urine
  and Feces of Humans Under Physiological Conditions*
Case
1
2
3
4
5
6
7
8
9
10
Urine,
jug/kg
0.1"
0.4
0.1
0.2
0.1
0.1
0.3
1.0
0.2
a
a
Feces,
ug/kg
0.6
3.0
b
b
b
b
0.1
b
b
a
0.1
average0 0.23
   *Source:  Goenechea and Sellier, 1967

   abelow detectable limit, which is 0.02


    not determined

   ^
    assumes urine samples below detectable limit
    = 0.02 jag/kg
                        C-20

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urinary  excretion  an additional increment of  1.2  x 0.5/11 = 0.06

ug/d.


     So  far as excretion via hair  is concerned,  it was reported by


Barclay, et al.  (1953)  that at autopsy  7  percent  of the original

        204
dose of    Tl was localized in scalp hair.  During  this same period


55 percent of  the  original dose had been  lost by  other excretory

                         O f\ A
routes.  Minor  loss of  ^U*T1  via  fiair  was  also reported  in rats

                                                            O f\ A
(Lie, et al.  1960).   Seven days following a pulse dose of    Tl,


approximately 75 percent of the radioactivity  had  been excreted in


the urine and feces.  Only 1.56 percent  of the residual amount was


localized  in  hair.   Assuming  that total excretion  via  hair  = 2X


scalp hair excretion,  14 percent could  conceivably  have  been re-


moved  from  the  body in  this  manner.  An  additional increment of


1.26 >ug x 14/55 or 0.32 ug results.


     Exfoliation of skin and sweat probably do not contribute sig-


nificantly to total thallium excretion,  at least probably not more


so than the gastrointestinal tract which has a larger surface area


than the skin,  a very rapid turnover  rate of  epithelium, and a high


rate of  secretory activity.   It would  seem conservative to assign


the skin an excretory role similar to the role of  the gastrointes-


tinal tract.   In summary,  total excretion of  thallium  per day in


adults not exposed  to  unusual sources  of  thallium is  probably as


follows:
                              C-21

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                  Excretory route             ug Tl/d
                  urine                        1.20
                  feces                        0.06
                  hair                         0.32
                  skin and sweat               0.06
                                   Total       1.64
Body Burden of Thallium as a Basis for Estimating Daily Absorption
     There is an alternate basis for  estimating daily absorption of
thallium.  It  begins with certain assumptions.   First,  it is as-
sumed that the excretory process is essentially first-order, where-
in the rate of excretion  is proportional to the amount in  the body
at that  time.   Second,  it assumes that input  is fairly constant  -
essentially zero order.   For  the  steady  state condition,  the fol-
lowing relationship exists:
     A   -tS.
      B   k where:
     A_  = amount in the body

     A,  = amount absorbed per day
     k = elimination constant (day~  )
The amount of  thallium  in the  body (AB)  of persons not unduly ex-
posed has been estimated  to  be  100 ug per  75  kg  (Weinig and Zink,
1967).    Using  the elimination constant of  Innis and Moses  (1978),
k =  0.023,  the daily  absorption  of  thallium to  attain a steady
state body burden of 100  ug would  be:
     100 ug = ~  or x =  2.3 wg.
That is approximately  1.4X  the value obtained using the estimated
sum of excretion by all pathways, and approximately 0.4 times  the
                               C-22

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intake value derived  from estimates of  input  from  food, water, and



air.  Since the estimated body burden is based on data from only two



cadavers,  the small difference in estimated daily absorption is not



surprising.  Order-of-magnitude agreements using two different ap-



proaches  to the  problem  of intake  are about  all  one  can  expect



given the  small amount of hard data available.



                             EFFECTS



Acute, Subacute,  and  Chronic Toxicity



     The vast majority of  the  cases  of adult human poisoning have



been  acute, usually  involving single  doses,  taken  by  reason of



homicidal  or  suicidal intent.   Acute  poisoning  in  children has



resulted from  ingestion of  thallium-containing  rat  and ant  bait or



from thallium's therapeutic use as a depilatory agent.  It  is pos-



sible to estimate at least roughly the  minimum lethal dose.   As for



the minimally toxic dose, the former practice of using thallium as



a depilatory agent makes it possible to make  an estimate, at  least



for children.



     Cavanagh,  et al. (1974)  investigated a  homicidal  attempt on



three men,  two of whom died after being given 930 mg  thallous ace-



tate (721 mg Tl).  The third man survived a dose of  310 mg  (240 mg



Tl).  In another  series of  seven  cases of suicidal attempts, four



survived  the  consumption  of one  tube  of Zelio Paste  (263  mg Tl)



with signs  of  poisoning,  two  survived  after eating  two  tubes of



Zelio Paste  (526  mg  Tl),  and  one died  after  eating five tubes of



Zelio Paste (Grunfeld and Hinostroza,  1964).   Assuming  an  average



weight of  70  kg,  the average toxic, non-fatal  dose for  adults is



about 4-8  mg/kg and   the minimal  fatal dose  is probably somewhat
                               C-23

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less than 10 mg/kg.  The minimal acute  lethal  dose  is quite similar
for a variety of animal species and the range  from  the highest non-
lethal  dose  to  the  lowest   lethal   dose  also  is quite  narrow
(Table 3) (Downs, et al. 1960).
     Based  on  the limited data  available,  children seem to be no
more sensitive  to the  acute  toxic or   lethal  effects  of thallium
                                   <3*
than adults.  In  a series of 8,006 children estimated to have been
given single oral doses of  3.1-7.8 mg  Tl per  kilogram body weight
of thallous acetate as a depilatory,  447 (6  percent) became  ill and
eight (0.1 percent) died (Munch, 1934).  Given the  imprecise nature
of reports  as to  incidence of  toxic effects,  it  is of course quite
possible that substantially more than  6  percent of the children in
this series experienced  signs  or symptoms of  poisoning.  It is not
even known  how  consistently the therapeutic objective of alopecia
was attained in this series of  cases.
     Acute  thallium  poisoning  is a disease entity which has been
widely described.  The initial signs and symptoms involve primarily
the gastrointestinal tract and  peripheral nervous system.  Alopecia
does not  generally occur until  several weeks following intoxica-
tion.  Indeed,  in fatal cases  death  may supervene  before alopecia
occurs.   The detailed description of three cases  of acute poisoning
by Cavanagh, et al.  (1974)  is  rather  typical  of what  has been de-
scribed by many other  investigators (see, for example, Paulson, et
al. 1972; Papp, et al.  1969).   Initially, the subject experiences
gastrointestinal  pains,  diarrhea,  and  vomiting.   This is followed
by paresthesia of the upper and lower  limbs, dizziness, and facial
weakness.   These  signs  first appear   in 2-5  days.    A frequent
                              C-24

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                                                TABLE 3


                                 Acute  Toxicity of Thallium Compounds*
n

KJ
cn
Thallous Acetate
Route

iv
ip


po



Species

rabbit
rabbit
guinea pig
rat
rabbit
guinea pig
rat
dog
1

7
9
25
41
4
4
37
3
Sex

F
F
M,F
F
F
M
F
M,F
lethal range**
mg Tl/kg
12-20
8-13
4-7
13-20
12-19
8-12
18-29
10-20
*

3
3
3
41
3
10
42
3
Thallic Oxide
Sex

F
M
F
F
M *
M,F
F
M
lethal range**
mg Tl/kg
24-39
30-60
10-30
62-92
10-30
3-5
9-20
20-30
      *Source:  Downs,  et  al.  1960


      **lethal  range  =  highest  non-lethal dose - lowest dose showing any lethality during 14-day
      period.

-------
complaint  is  pain  and  tenderness of the lower limbs, particularly
of the  knees.   Dysphagia and dyspnea  also  are commonly reported.
Sensory  impairment  occurs  frequently.   The cranial nerves as well
as the spinal nerves are affected.   The central nervous system also
is affected to varying degrees.  Attention span is reduced; somno-
lence and  delerium or coma  may  occur.  Various  abnormalities of
                                    &P
cardiac  function  have been  reported,  including  sinus tachycardia
and flattening or inversion of the  T-wave.  These and other cardiac
effects have been variously  attributed  to vagus involvement and to
myocardial damage.   The  electroencephalogram  is frequently abnormal
(Cavanagh, et al.   1974).  These effects and others occur in vari-
ous combinations.   Chamberlain, et  al.  (1958)  summarized the inci-
dence  of  effects  in  their  series   of  14  cases  in  children
(Figure 3), as did  Grunfeld and  Hinostroza  (1964) in  a series of
adult cases (Figure 4).
     Although  acute poisoning is  a somewhat  protracted disease,
with effects lingering  for  several months,  the prognosis for full
recovery in adults seems to be good.  Such does not appear to be the
case in children.   In a  follow-up  study of 72 cases, Reed, et al.
(1963)  found  that  26  of 48 had neurologic abnormalities when they
were followed up for an average of  4 years.  The neurologic abnor-
malities  found  at  follow-up  usually   represented persistence  of
signs found during the initial stages of the  disease  (Table 4).  It
should  be  noted  that mental  abnormalities  and muscle weakness or
paralysis  actually increased  in  incidence  during  the  follow-up
period.
                               C-26

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                        Number of children
                                   5
                    H
                                               10
           (Alopecia)
             At aid a
           Weakness
         Somnolence
            Trim or
           Irritability
           Headache
             Coma
         Hyperreftet
         Convulsion!
         Paresthesios
             P to sis
       Resp. Paralysis
       Polh. ReHexes
           Paralysis
                            23%
50%
75%
                            FIGURE  3
Incidence  of Gastrointestinal  (Top)  and Neurologic Signs
        and Symptoms of ThaliotOKicosis  in Children
              Source;  Chamberlain et al.,  1958
                               C-27

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          Svmoton
                            tuicir of cam
                       FIGURE 4



Signs and Symptoms in Seven Cases of  Thallotoxicosis



       Source:   Grunfeld and Hinostroza,  1964
                         C-28

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                             TABLE 4

   Percent of  26 Patients with Abnormalities at Follow-up Stage
        (Southern Texas Thallotoxicosis  Study, 1954-1959)*
Symptoms
ataxia
tremor
abnormal reflexes
convulsions
abnormal vision
mental abnormalities
abnormal movements
muscle weakness
or paralysis
Acute Stage
of Illness, %
81
57
62
27
15
15
15
4
Follow-up
Stage, %
23
19
38
15
4
58
8
15
*Source:  Reed et al.,  1963
                            C-29

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     It is not surprising that acute thallium poisoning should  lead
to irreversible damage, or at least to only  slowly-reversible  dam-
age to the central and peripheral nervous system.  Degeneration of
peripheral nerve fibers and chromatolysis of  motor  nerve cells  were
frequently reported  in man  (Munch, et al. 1933; Gettler and Weiss,
1943), and in animals  (Zook and Gilmore, 1967; Zook, et al. 1968).
                                     ^
     So far  as  subacute  and chronic thallium poisoning in man are
concerned, there are very  few  reports of any kind and those which
are available  provide  little information as to  duration of expo-
sure, level of exposure as  reflected  in thallium concentrations, or
doses  in  either the external environment or in  the affected  sub-
jects.  In one  brief report concerning 13 men exposed 3-4 months,
the signs and  symptoms were pains in the legs, weariness, loss of
hair,  disturbance  of sensation, psychic  trouble,  albuminuria and
nephritis (Meyer, 1928).  Generally speaking, these findings corre-
spond to the  usual  description  of  acute poisoning.  The author  also
reports that lymphocytosis was a  constant  finding.   Gettler and
Weiss  (1943)  reported  that in  two cases of  chronic poisoning the
only symptoms observed were pain in the  legs, mild symptoms resem-
bling  those  of  encephalitis, alopecia, and  oliguria.   The sugges-
tion  that  renal damage  is  a feature of chronic  poisoning is not
surprising.   In  the  description of  acute cases of poisoning,   fre-
quent  reference is made to manifestations of  renal damage  (Fischl,
1966).  Postmortem  evidence of  renal  damage,  at least  in acute  poi-
soning, also has been reported  (Gettler and Weiss,  1943*).  Finally,
there also is one report of a case of  chronic  intoxication  in a man
                               C-30

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exposed  24  years.   The main effects  were  loss  of hair, ascending
polyneuritis and disturbances of speech and vision (Egen, 1955).
     Rats fed  thallous  acetate  in  their diet for 105 days experi-
enced no  reduction  in weight gains at  concentrations of  5  and 15
ppm.  Doses  of 30  ppm for 105  days  proved fatal to approximately
half of the  animals.   The only toxic effect noted  at 15 ppm was loss
of hair  (Downs, et al. 1960).  It was first noted at  two weeks.  It
must be recognized,  however,  that there  has been  very little effort
to  search  for  more  subtle effects  at exposure  levels  below those
causing  alopecia.  A  study of  the  toxic effects of chronic admin-
istration  of  thallium  in  animals  (>90  days)  was reported  by
Tikhonova  (1967).   In  this  instance,  thallium  administration in
rabbits  resulted in  paralysis  and  pathological  changes  in   the
liver, kidneys and stomach mucosa.
     It seems from the limited  number of reports  that regardless of
whether  thallium intake occurs  in one dose or over several months,
the effects  are  qualitatively  very similar, if  not identical.   It
is not possible to state with any degree of certainty which of  the
many effects reported is the  one to which man is  most  sensitive.  It
would seem that in cases of acute poisoning in man alopecia is  the
most consistent  effect  among those surviving more than two weeks.
In  the series  of children studied  by Chamberlain, et  al.  (1958),
this was clearly the  case.  In the series of adult cases  reviewed by
Grunfeld and Hinostroza (1964),  (see  Figure 4), nausea and vomiting
occurred  in  one  case  where alopecia  did  not  occur.   That subject
survived only  5  days  after ingesting thallium.   Among  documented
cases of chronic poisoning no specification as to the frequency of
                               C-31

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various signs and symptoms has been recorded.   In summary,  the most
consistently reported effect  is alopecia.  Unfortunately,  consist-
ency cannot be equated a priori with sensitivity.
Synergism and/or Antagonism
     Potassium has long been  known  to exhibit  significant  interac-
tions with thallium,  both in the pharmacokinetic  sense  and  in toxic
interactions.   Lund  (1956) first  demonstrated that potassium  in-
creases the renal clearance of thallium.  Mullins and Moore (1960)
demonstrated  that  the influx  and  efflux patterns  of  thallium  in
frog muscle were quite similar to  the  fluxes of potassium.  Gehring
and Hammond (1967)  extended these  earlier observations  to show that
potassium markedly enhanced the rate of  thallium excretion in both
rats and  dogs.   The excretion  occurred for the most  part in  the
urine.   Salivary secretion of potassium, when  stimulated  with  de-
oxycorticosterone,  was accompanied by a corresponding increase  in
thallium  excretion.   Potassium also  increased somewhat  the acute
LDj.. of  thallium,  suggesting that  mobilization  from the  receptor
sites is  responsible for the  toxic effects.
     As a result of these  studies  in animals,  the use of potassium
was  instituted  in  the  management  of thallotoxicosis in  man.    Re-
sults have  been  somewhat equivocal.  The  use  of potassium in  the
management of thallotoxicosis does  result  in  some increase in  the
urinary excretion of thallium, but this  mobilization is accompanied
by a temporary accentuation of the  neurological  signs and  symptoms
(Innis and Moses, 1978; Papp, et al. 1969).
     Several other  interactions have been reported, but  their sig-
nificance  is  difficult  to  evaluate.    Levkovitch  (1938)  reported
                               C-32

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that  ambient  temperature  had an  effect on  thallium  toxicity  in
sheep and rabbits, and that confinement and  dietary  restriction en-
hanced  toxicity.   Levander and Argrett  (1969) observed that  thal-
lium  reduced  the exhalation of  volatile selenium metabolites,  an
action  shared  with  mercury and arsenic.  Unlike arsenic, however,
neither  thallium  nor  mercury  increased biliary excretion concomi-
tantly.
Teratogenicity
     There are two  reports  in  the  literature which  suggest a  tera-
togenic effect of thallium.  The first was a study of the effect  on
chick embryos  (Karnofsky,  et  al.  1950} in which T12SO. (0.4  - 0.7
mg/egg)  was  administered during  incubation.   The  primary  defect
produced was achondroplasia.  Thallium also  produced early embryon-
ic death and reduced embryonic size.   Thus,  the study did not ful-
fill  the  usual criteria for teratogenesis wherein  the effect must
be evident at doses not otherwise  grossly toxic.
     Only one study of  thallium  teratogenesis  in mammalian species
has been  reported.   Gibson and Becker  (1970)  studied  the terato-
genic effects of  thallium  in rats  under  conditions  of both low and
normal dietary potassium.  Thallium administered intraperitoneally
to  the  mothers early  (d.  8,9,10)  at  2.5 mg/kg/dose,  or  late (d.
12,13,14) at 2.5 and 10 mg/kg,  resulted in reduced fetal weight and
in  increased  incidence  of  teratologic effects (hydronephrosis and
missing or non-ossification of vertebrae).   It  was observed that  at
both dosage levels  thallium caused maternal  toxicity as manifested
by diarrhea,  lethargy,  irritability,  poor hair  luster and body hair
loss.    One  interesting aspect of  this  study was  in regard  to the
                               C-33

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effects  of  dietary  potassium deficiency.   A  low-potassium diet
increased the  toxicity  of  thallium to the dams  and  was  of  itself
teratogenic, but  it  did not  potentiate  the  teratogenic  effect of
thallium.  Given  the  types  of malformation reported, the evidence
of maternal  toxicity and  the reduced fetal weights,  it is quite
likely  that  these effects  were due  to  delayed  fetal maturation
(see, for example, Kimmel and Wilson,  1973).  In  both studies thal-
lium was administered by a parenteral route and  in both cases gen-
eral fetotoxic  effects  were  apparent.   Thus,  it is  impossible to
distinguish teratogenicity from a more geasral toxic effect.
Mutagenicity
     No pertinent information could be found in  the  available lit-
erature concerning the mutagenicity of thallium.
Carcinogenicity
     There are  no  available published reports  on the carcinogeni-
city of  thallium;  however,  there  are  two carcinogenicity studies
on-going at the time of this  document's preparation.   Carcinogeni-
city/mutagenicity/teratogenicity  evaluations  of  thallium sulfate
are  being  conducted  by  Litton  Bionetics  under   EPA  contract;
Sprague-Dawley rats are being fed  thallium sulfate  in  the diet at
three dose levels.  The National Institute for Occupational Safety
and Health (NIOSH)  in  Cincinnati, Ohio  is  investigating the carcin-
ogenicity of thallic oxide by inhalation  in rodents.
     Without any  implications as to  non-carcinogenicity  it  is of
interest to note that thallium has mild anti-carcinogenic effects,
along with other metals of Group Ilia  (Adamson, et al.   1975).
                              C-34

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                      CRITERION FORMULATION
Existing Guidelines and Standards
     There is a threshold limit value (TLV) of 0.1 mg/m  for thal-
lium in workplace air (ACGIH, 1971).  This value is based on anal-
ogy to other  highly  toxic  metals.   This standard has been adopted
by the Occupational Safety  and Health Administration  (OSHA), and is
the same as that for East Germany and* West Germany (Winell, 1975).
The U.S.S.R. standard is 0.01 mg/m  .  No criteria have been devel-
oped for thallium in irrigation water, drinking water, fresh water
or other media.
Current Levels of Exposure
     It is extremely difficult  to  specify current levels of expo-
sure  for  either man or  animals because  of  the scarcity  of  good
data.   This is  due  to  the  fact  that analytical methods which have
been applied  to  the  problem have generally  not been sufficiently
sensitive for determination of  thallium in major media (air, food,
water) or in normal man.  This  is not to say that adequate methods
do not exist.   For  example,  the  mass spectroscopic-isotope dilution
procedure used by Weinig and  Zink  (1967)  could detect thallium in
urine  in  the  range  of  .01-0.1  ng/g.  There  probably has not been
sufficient motivation to develop alternate  sensitive methodology to
define human exposure adequately in the normal range.
     Certain approximations as  to usual human  exposure are possi-
ble.   Thus, based  on one extensive study  it  seems  that tap water
seldom exceeds 0.3 ug Tl/1  (Greathouse, 1978).   Assuming that the
average adult consumes  2 liters  of water per day,  total  input would
be somewhat less than 1 ug/d.
                               C-35

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     Even  in  the  worst conditions of water pollution, the concen-
tration  of thallium  probably  seldom exceeds  30 jug/1  (U.S. EPA,
1977).   These conditions  occur  in  the  immediate  vicinity of ore
processing  operations and  possibly  in  streams  draining ore-rich
soils,  e.g.  the  Colorado  River  as it  courses  through western
Arizona.
     Limited  data on  thallium  in vegetables  suggest  that,  as  a
class of food, these  may  have considerably  higher concentrations of
thallium, perhaps 10 jug/kg wet weight, than other classes of  foods
(Geilmann,  et  al.  1960).  Bread and muscle,  for example, contain
1 jag/kg or less.   This may explain the observation  that vegetarians
excrete considerably more thallium in the  urine  than  non-vegetari-
ans.   Assuming that  total food  consumption is  1.6  kg/d,  (DSDA,
1968), that 0.38 kg is in the form of vegetables, and that the re-
mainder  has a concentration of only  1 ug/kg, total daily  thallium
intake would be (0.38)  (10)  + (1.2) (1) = 5  jug.  This estimate  prob-
ably  is  on the high  side since  prepared  vegetables  would  likely
have less thallium than  raw vegetables due to leaching of  thallium
into water during cooking.
     So  far  as ambient  air  as a source is  concerned,  the  single
largest anthropogenic source of  thallium is considered to be  stack
emissions from coal-fired plants.  It has  been estimated  that flue
gas would contain about  0.7 mg/m , with a  likely ground level con-
centration  of  0.7 ug/m  .   Given that a large  factor of dilution
would result by dispersion  from  the  base of  a stack,  it seems un-
likely  that the  contribution  of coal  combustion to  thallium in
ambient  air would be significant.   The  highest measurement  of
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thallium  reported  in ambient  air indicated  a  range of  0.04-0.48
ng/m   (Carson and Smith, 1977).
     Inhalation  of  thallium in cigarette  smoke may, on  the  other
hand, be a very significant source.   The urinary excretion of  thal-
lium  in smokers  is  about  twice  that  in  non-smokers (Weinig  and
Zink,  1967)  and  the  concentration in cigar  stubs  was shown  to  be
57-170  ng/g  (Geilmann, et  al.  1960),*about  20 times  the concentra-
tion estimated for the diet.
     Total intake in the general  non-smoking  adult population cal-
culated on the basis  of exposure data thus  would consist of no more
than 1.0  ug/d  from  water and  no  more  than 5 ug/d from food,  even
assuming that virtually all  ingested thallium is absorbed.
     The total daily assimilation of thallium by adults in the gen-
eral population has also been arrived at by consideration  of excre-
tion data  and  estimated body  burden.   The estimated daily intake
arrived at by consideration of food  and  water  exposure and by  these
other two methods is as follows:

              Basis               Estimated Daily Adult Intake
   Food, air and water exposure             <  6
   Excretion data                          1.64 ug/d
   Body burden data                        2.30 ug/d

Special Groups at Risk
     From the  standpoint  of age,  there  is  no basis for  believing
that children  are  more susceptible  to  thallium intoxication  than
adults.  Children,  however,  experience  neurological  sequelae, while
adults do not.   There  is no  reason  for  suspecting  that  the  fetus  is
unusually sensitive.   Essentially  nothing  is  known regarding sex
                              C-37

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differences  in  susceptibility.   One  study  in rats indicated  that
females  are  more  resistant to  sub-chronic  toxicity  than males.
From the standpoint of exposure hazard,  it  would seem  that smokers
may have twice as great a level of thallium intake as  non-smokers.
This suggestion is based solely on data concerning  urinary  thallium
excretion in six people and on very limited information concerning
thallium in  cigars.   Obviously,  people  occupationally exposed  to
thallium may constitute a  special risk category.   This matter has
received little attention because the  total annual industrial  pro-
duction of  about 0.5  tons of thallium is so small.   In  the U.S., the
main source of poisoning, thallium-containing rodenticides and in-
secticides, has been terminated.  The manufacture and  distribution
of these products is no longer permitted.
Basis and Derivation of Criteria
     The proposed criterion  for  thallium in water is  derived  from
1) estimated least toxic level on chronic intake in man, 2) intro-
duction  of  a margin  of safety,  and  3)  relative  contribution  of
water and other media to total daily intake in the general popula-
tion.
     In estimating the  least  toxic  level of intake,  the effect  to
which man  is most  sensitive is probably  alopecia.   Loss  of scalp
hair in man and of body  fur  in animals seems to occur at  somewhat
lower levels  of  intake than any other known effects. This is not  so
clearly the case in  adults  as  in  children and animals.  There is,
however, no  great difference  between the  acute  or  chronic   dose
causing  alopecia  and the  dose causing  neurologic effects.   The
least daily amount of thallium which, when  taken for a lifetime,  will
cause alopecia  can  only be estimated  on  the  basis of sub-chronic

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animal exposure data combined with some kinetic considerations.   In

the Downs,  et  al.  (I960) study alopecia  occurred  in 2 weeks as  a

result of the administration of thallium at 12 ppm  in the  diet.   At

this dose level, either  effects  occurred  within two weeks or they

did not occur  with  continued intake.   This is consistent with  the

rapid turnover of thallium  in  rats and the consequently rapid  at-

tainment of a  steady  state  level of thallium in the body.  Within

two weeks,  a  steady  state  is virtually  achieved  since  14 days

represents more  than  three  half-lives for thallium  clearance from

the body.  Rats at the next lowest dose (5  ppm  thallous  acetate or 4

ppm thallium)  fed  for 105 days  showed  no alopecia or other toxic

effects.  Therefore, the  highest  no observable adverse  effect level

(NOAEL) would be 4 ppm (4 jug/g) of  thallium.

     In the  following calculation the  average  weight of rats, 0.075

kg,  is  derived  from  inspection  of Figure  1 (male  rats)  in  the

author's report;  the average daily  food intake is  assumed to be 10

g at that weight.   Therefore,  the "safe"  ADI for  rats can be cal-

culated as:

          (4.0 ug/g) (10 g)  =  40 jug/0.075  kg  = 533  jug/kg.

     Conversion  to  an  acceptable daily intake (ADI) for man would

be as follows:

     ADI , 533 ug/kg x 70 kg = 37>1 yg
                   1,000

where:

     70 kg = average weight  of man

      1,000  =safety factor as  recommended  by  NAS (1977) for com-
     pounds  where there are:   "No  long term or acute human data.
     Scanty  results on experimental animals.  No indication of
     carcinogenicity."
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For  the  purpose of establishing  a water quality criterion,  human
exposure  to  thallium  is  considered  to  be based on ingestion  of
2 liters  of  water  and 6.5  g of  fish/day.   The  bioaccumulation
factor for thallium has been established  to be  119.
     The criterion  (C)  is derived  from  this data  as follows:
          (C  x  2 liters) -t- (C x 119 x 0.0065)  = 37.3 jug.
Solving  for  C  gives:  C  =  13.4  jag/liter.  Thus,  the  recommended
water quality  criterion for thallium is  13.4  ug/liter.  The  cri-
terion can alternatively be expressed, if exposure is assumed to be
only from ingestion of contaminated fish and shellfish,  as 48 jug/1.
     It  is interesting to note the similarity  between  the  minimal
body burden  causing alopecia  in  rats (on chronic  administration)
and  the  single dose causing  alopecia,  with moderate incidence  of
other effects,  in children.  For the  rat:
     1.6 mg/kg/d = 8.88 mg Tl/kg
     0.18 day"
For  children,  the  average acute  dose associated with  alopecia  is
3.1  to 7.8 mg/kg (Munch, 1934).
     So  far  as  a safe  level of thallium  in drinking water  is  con-
cerned,  there does  not seem to be any reasonable possibility  that
even the most  thallium-polluted  waters  would  have  a toxic  effect.
In the worst case  identified  by  Zitko,  et al.   (1975),  the  concen-
tration  of thallium was 88  ug/1.   Assuming that  this were  a  human
water supply,  the  daily  input at  2 liters per  day would  be  only
176 jug Tl, 4.74 times the ADI calculated for  man  in the document
and well within the 1,000-fold safety factor.
     The great  difference  between estimated minimally  toxic  expo-
sures  and  current  total  exposure  in  the  general  population  is
                               C-40

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reassuring.  One  cannot  be  totally sanguine, however, since  there

is a paucity of chronic data, including information on mutagenici-

ty,  teratogenicity  and carcinogenic!ty.   For that reason  it  seems

prudent to keep levels of exposure at or  below their present  lev-

els.  From the  data available,  it would seem that  few  if  any public

water supplies  would ever contain more than 4 pg/1.  Thus,  the cri-

terion  of  13  pg/1  is  approximately  threefold  greater  than  the

likely maximum in public water supplies.

     In summary form, the dose and exposure  parameters for man are

estimated to be:



     minimally lethal single dose       4-10 ing/'kg

     recommended criterion              13  pg/1 water

     ADI for 70 kg/man                  37.3

     probable limit for ^> 99 percent    ,     ,.
     of U.S. tap waters                 L P9/L

     probable current level of daily-
     adult thallium consumption  from    <^~L  pg/d
     drinking water
                              C - 41

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                            REFERENCES







Adamson, R.H., et al.  1975.   Studies  on  the  anti-tumor activity of



gallium nitrate (NSC-15200)  and other  Group Ilia metal salts.  Can-



cer Chemo. Rep.  59: 599.







American Conference  of  Governmental*Industrial Hygienists.  1971.



Documentation of threshold limit values for  substances in workroom



air.  3rd ed.







Barclay, R.K.,  et  al.  1953.   Distribution and excretion of radio-



active thallium in the  chick embryo, rat  and  man.  Jour. Pharmacol.



Exp. Ther.  107: 178.







Carson, B.L. and I.C. Smith.   1977.  Thallium.  An appraisal of en-



vironmental exposure.   Tech.  Rep.  No. 5,  Contract  No.   N01-ES-2-



2090.  Natl. Inst. Environ.  Health Sci.







Cavanagh, J.B., et al.   1974.   The  effects of thallium salts with



particular  reference  to the  nervous  system changes.   Jour.  Med.



43: 293.







Cavieres, J.D.  and J.C. Ellroy.   1974.    Thallium  and  the sodium



pump in human red cells  Jour. Physiol.  243: 243.







Chamberlain, P.H., et  al.   1958.  Thallium poisoning.  Pediatrics.



p. 1170.
                               C-42

-------
Downs, W.L., et al.  1960.  Acute and subacute  toxicity  studies  of



thallium compounds.  Am. Jour.  Ind. Hyg. Assoc. Jour.  21:  399.







Egen,  B.    1955.    Gewerbliche  thalliumvergiftung.    Zentralblatt



Arbeitsmed. Arbeitsschutz.  5:  141.







Fischl, J.  1966.  Aminoaciduria in thallium  poisoning.  Am. Jour.



Med. Sci.  251: 40.







Gehring, P.J.  and  P.B.  Hammond.   1964.   The  uptake of thallium  by



rabbit erythrocytes.  Jour. Pharmacol. Exp. Ther.  145:  215.







Gehring, P.J.  and  P.B.  Hammond.  1967.   The  interrelationship be-



tween  thallium and potassium  in animals.    Jour.  Pharmacol. Exp.



Ther.  155: 187.







Geilmann, W. ,  et  al.   1960.   Thallium ein regelmassig vorhandenes



spurenelement  im tierschen und pflanzlichen organismus.   Biochem.



Zeit.  333: 62.







Gettler, A.O.  and C.A. Weiss.   1943.   Thallium  poisoning.  III.



Clinical toxicology of  thallium.  Am. Jour. Clin. Pathol.   13: 422.







Gibson, J.E.  and  B.A.  Becker.   1970.   Placental transfer,  embryo



toxicity  and   teratogenicity  of  thallium  sulfate  in normal  and



potassium-deficient rats.  Toxicol. Appl. Pharmacol.   16: 120.
                               C-43

-------
Gibson, J.E., et al. 1967.   Placental transport and distribution of
thallium-204  sulfate  in newborn  rats and  mice.   Toxicol.  Appl.
Pharmacol.  10: 408 (Abst.)

Goenechea, S.  and K.  Sellier.  1967.   Uber die naturlichen thal-
liumgehalt des menschlichen korpers.  Deutsche  Zeit.  Gericht. Med.
60: 135.

Greathouse, D.G.  1978.  Personal communication.

Grunfeld, 0. and Y. Hinostroza.  1964.  Thallium poisoning.  Arch.
Int. Med.  114: 132.

Hamilton, E.I. and M.J. Minski.  1972/1973.   Abundance  of  the chem-
ical elements  in  man's diet and possible  relations  with environ-
mental factors.  Sci.  Total Environ.  1: 375.

Innis, R. and H. Moses.  1978.  Thallium poisoning.  Johns Hopkins
Med. Jour.  142: 27.

International  Cancer   Research Program.    1966.   Deposition  and
retention models  for  internal dosimetry of  the human respiratory
tract.  Health Phys.  12: 173.

Karnofsky, D.A., et al. 1950.   Production of achondroplasia in the
chick embryo with thallium.  Proc.  Soc. Exp. Biol. Med.  73: 255.
                               C-44

-------
Kinunel, C.A. and J.G. Wilson.  1973.  Skeletal deviations  in  rats:
malformations or variations?  Teratology.  8: 309.

Kubasik, N.P. and M.T. Volosin.  1973.  A simplified determination
of urinary cadmium, lead and thallium, with  use of  carbon  rod  atom-
ization and atomic absorption spectrometry.  Clin. Chem.   19:  954.

Levander, O.A. and L.C.  Argrett.   1969.   Effects of arsenic,  mer-
cury,  thallium and  lead  on selenium metabolism in rats.   Toxicol.
Appl. Pharmacol.   14: 308.

Levkovitch, L.I.   1938.   The influence  of  external  temperature,
diet and emotion on the  pharmacological action of  thallium.   Bull.
Biol. Med. Exp. USSR. Chem. Abst.   34: 24618 (1940).

Lie, R. , et al.   1960.   The distribution and excretion  of  thallium-
204  in  the rat,  with  suggested  MFC's and  a  bio-assay procedure.
Health. Phys.   2: 334.

Lund,  A.   1956.   Distribution  of  thallium in  organisms and  its
elimination.  Acta Pharmacol. Toxicol.  12: 251.

Meyer, S.   1928.  Changes in the  blood  as  reflecting industrial
damage.  Jour. Ind. Hyg.   10: 29.
                               C-45

-------
Mitteldorf, A.J. and D.O.. Landon.  1952.  Spectrocheinical determi-


nation  of  the mineral-element  content  of  beef.     Anal.  Chem.

24: 469.




Mullins, L.J. and R.D.  Moore.  1960.   The  movement of  thallium  ions

in muscle.  Jour. Gen. Physiol.  43:  759.
                                   &>



Munch, J.C.   1934.   Human thallotoxicosis.   Jour. Am. Med. Assoc.


102: 1929.




Munch, J.C.,  et al.  1933.   The 1932 thallotoxicosis outbreak  in


California.  Jour. Am. Med. Assoc.  100:  1315.




National  Academy  of Science.   1977.    Drinking Water and Health.

Washington, D.C.




Neal, J.B., et  al.   1935.   An unusual occurrence of  thallium  poi-

soning.  N.Y. Med. Jour.  35: 657.




Papp, J.P., et  al.  1969.   Potassium chloride treatment  in thallo-


toxicosis.  Ann. Intern. Med.  71: 119.




Paulson,  G. ,  et al.   1972.   Thallium  intoxication  treated  with


dithizone and hemodialysis.  Arch. Intern. Med.   129:  100.
                               C-46

-------
Rauws, A.G.  1974.  Thallium pharmacokinetics and  its modification



by  Prussian   Blue.     Naunyn   Schmiedeberg's   Arch.  Pharmacol.



284: 295.







Reed, D., et al.  1963.   Thallotoxicosis.   Acute manifestations  and



sequelae.  Jour. Am. Med. Assoc.  183: 516.








Richeson, E.M.  1958.   Industrial thallium intoxication.   Ind. Med.



Surg.  2: 607.








Stephan, C.E.   1980.  Memorandum  to J. Stara.  U.S. EPA.  July  3.







Tikhonova, T.S.   1967.   Toxicity of thallium and  its compounds  in



workers.   Nov. Dannye  Toksikol.  Redk. Metal.  Ikh Soedin.   Ghent.



Abst.  71: 53248J, 1969.








Toscano, V.A.  1975.   In;  Nutrients  in  Processed Foods.  Publishing



Sciences Group, Inc.,  Acton, Massachusetts.  pp.  111-123.








Truhaut,  R.    1952.   Les effets  biologiques du  thallium.   Ph.D.



Thesis.  Faculty of Sciences.  University  of Paris.








U.S. Department of Agriculture.   1968.  Food consumption  of house-



holds  in  the United States,   spring, 1965.   U.S.  Gov.  Printing



Off., Washington, D.C.
                               C-47

-------
U.S. EPA.  1971.  Identification and estimation of ions, molecules

and  compounds  in particulate matter  collected from  ambient air.

Contract CPA-70-159, Air Programs by Battelle Columbus Lab.


U.S. EPA.  1977.  Heavy metal pollution  from  spillage  at ore smelt-

ers  and mills.  EPA-600/2-77-171.  Washington, D.C.
                                   ti»

U.S. EPA.   1978a.   The multielemental  analysis of drinking water

using  proton-induced  x-ray  emission  (PIXE).    EPA-600/1-78-058.
Washington, D.C.


U.S. EPA.  1978b.   In-depth studies on health and environmental  im-

pacts  of  selected  water  pollutants.    Contract   No.  68-01-4646.

Washington, D.C.


U.S. EPA.   1980.   Seafood  consumption data  analysis.   Stanford

Research Institute  International.  Menlo  Park,  California.   Final

Report, Task 11.  Contract No. 68-01-3887.


Weinig, E. and  P.  Zink.   1967.   Uber  die quantitative massenspek-

trometrische bestimmung des  normalen thallium-gehalts im menschli-

chen organismus.  Arch. f. Toxikol.   22: 255.


Williams,  N.  and  A.L.  Riegert.   1971.   Epidemic  alopecia areata.

An outbreak in an industrial setting.   Jour.  Occup. Med.  13: 535.
                               C-48

-------
Winell, M.   1975.   An international comparison  of hygienic stan-



dards for chemicals  in the  work, environment.   Ambio.  4: 34.







Zitko,  V.  and  W.V.  Carson.   1975.   Accumulation  of  thallium  in



clams and mussel.  Bull.  Environ.  Contam.  Toxicol.  14: 530.







Zitko,  V., et  al.   1975.   Thallium:" occurrence in the environment



and toxicity to  fish.   Bull.  Environ. Contam. Toxicol.  13: 23.








Zook, B.C.  and C.E.  Gilmore.   1967.  Thallium poisoning in dogs.



Jour. Am. Vet. Med.  Assoc.   151:  206.







Zook, B.C.,  et al.  1968.   Thallium poisoning  in  cats.   Jour.  Am.



Vet. Med. Assoc.  153:  285.
                                         • U. S. GOVERNMENT PRINTING OFFICE : ! 9BO 72C-016/4396
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