NATIONAL EMISSIONS
                  INVENTORY
                 OF SOURCES
U.S. ENVIRONMENTAL PROTECTION AGENCY
    Office of Air and Water Programs
 Office of Air Quality Planning and Standards
Research Triangle Park, North Carolina 27711

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                                           EPA-450/3-74-011
NATIONAL  EMISSIONS INVENTORY


                         OF


       SOURCES  AND  EMISSIONS


                         OF


                     SILVER



                         by

                    GCA Corporation
                 GCA Technology Division
               Bedford, Massachusetts  01730



                  Contract No. 68-02-0601



             EPA Project Officer: David Anderson



                     Prepared for

           ENVIRONMENTAL PROTECTION AGENCY
              Office of Air and Water Programs
          Office of Air Quality Planning and Standards
             Research Triangle Park, N. C.  27711
                       May 1973
                                      O.S. Pnvirohmental Protection Agency
                                      Region 5, Library f-<  • ^ "
                                      77 West Jackson F
                                      Chicago, JL 605;.'-    .   	"iCor

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This report is issued by the Environmental Protection Agency to report technical
data of interest to a limited number of readers. Copies are available free of
charge to Federal employees, current contractors and grantees, and nonprofit
organizations - as supplies permit - from the Air Pollution Technical Information
Center, Environmental Protection Agency, Research Triangle Park, North
Carolina 27711, or from the National Technical Information Service, 5285 Port
Royal Road, Springfield, Virginia  22151.
This report was furnished to the Environmental Protection Agency by GCA Corp-
oration, Bedford, Massachusetts, in fulfillment of Contract No. 68-02-0601.  The
contents of this report are reproduced herein as received from GCA Corporation.
The opinions, findings, and conclusions expressed are those of the author
and not necessarily those of the Environmental Protection Agency. Mention  of
company or product names is not to be considered as an endorsement by the
Environmental Protection Agency.
                    Publication No. EPA-450/3-74-011
                                    11

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                            ACKNOWLEDGEMENT

       The continued cooperation and dedication of Mr. Carl Spangler of
EPA, who served as Program Monitor until his death is deeply appreciated.
       GCA would like to extend thanks to Mr. David Anderson and Mr. James
Southerland of EPA for their cooperation in the preparation of this study.
       In addition, special thanks are also due to Mr. R. Welch and Mr. J.
West, Commodity Specialists, Bureau of Mines, who provided significant
technical inputs to this program.
                                   111

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                           TABLE OF CONTENTS
SECTION                          TITLE                              PAGE
               ABSTRACT                                             vii
  I            INTRODUCTION                                           1

               A.   PURPOSE AND SCOPE                                 1
               TJ.   CONCLUSIONS                                       2

 II            OVERALL U.S. MATERIAL FLOW CHART FOR SILVER            4

               A.   U.S. PRODUCTION AND ORE PROCESSING
                    (45,006,000 ounces)                               4
               B.   IMPORTS AND EXPORTS (Net, 34,671,000 ounces
                    imported)                                         4
               C.   STOCKPILE CHANGES  (NET DECREASE, 101,000
                    ounces)                                           6
               D.   SCRAP RECYCLING (49,318,000 ounces)               6
               E.   PRIMARY SMELTING (81,381,000 ounces)              7
               F.   SECONDARY REFINING (80,043,000 ounces)            7
               G.   CONSUMPTION OF SILVER (129,096,000 ounces)        7

 III           SOURCES AND ESTIMATES OF SILVER-CONTAINING EMISSIONS   9

               A.   DATA PRESENTATION AND ACCURACY                    9
               B.   DEVELOPMENT OF EMISSIONS ESTIMATES - 1970        14
               C.   SUMMARY OF PRINCIPAL EMISSIONS                   24

 IV            REGIONAL DISTRIBUTION OF PRINCIPAL SOURCES AND
               EMISSIONS                                             26

  V            NATURE OF EMISSIONS                                   30

 VI            UPDATING OF EMISSIONS ESTIMATES                       32

               A.   VERIFICATION OF CURRENT ESTIMATES                32
               B.   PERIODIC REVIEW OF ESTIMATES                     32

 VII           REFERENCES                                            34
                                       V

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                      LIST OF TABLES AND FIGURES
TABLE NO.
TITLE
                 SOURCES AND ESTHETES OF SILVER-CONTAINING
                 EMISSIONS

                 PRINCIPAL SOURCES OF SILVER-CONTAINING
                 EMISSIONS - 1970

                 GEOGRAPHICAL DISTRIBUTION OF EMISSION
                 SOURCES AND EMISSIONS

                 PROPERTIES OF METALLIC SILVER
PAGE


 10


 25


 27

 30
FIGURE NO.
                 SILVER MATERIALS FLOW - 1970
                                       VI

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                               ABSTRACT

     A national inventory of the sources and emissions of the element
silver was conducted.  The study included the preparation of an overall
material flow chart depicting the quantities of silver moving from
sources of mining and importation through all processing and reprocess-
ing steps to ultimate use and final disposition.  All major sources of
silver-containing emissions were identified and their silver emissions
into the atmosphere estimated.  A regional breakdown of these sources
and their emissions was also provided.  The physical and chemical nature
of the silver-containing emissions was delineated to the extent that in-
formation was available, and a methodology was recommended for updating
the results of the study every two years.
                                  Vii

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I.   INTRODUCTION

     A.   PURPOSE AND SCOPE

          The Monitoring and Data Analysis Division,  Office  of  Air Quality

Planning and Standards of the U.S. Environmental Protection  Agency  (EPA) has
contracted with GCA Technology Division to conduct a  national inventory  of  the

sources and emissions of the element silver.   The purpose  of the  study was  to

define as accurately as possible, based on existing and  available published
and unpublished information, the levels,  nature and sources  of  silver-contain-
ing emissions for defined geographic regions  throughout  the  United States.

          The scope of this program is outlined below:

               • Develop an overall material flow chart
                 depicting the quantities of silver
                 moving from sources of mining and importa-
                 tion, through all processing and
                 reprocessing steps to ultimate use and
                 final disposition as far as the movements
                 can be traced.

               • Identify all major potential silver-
                 containing emissions emitted to the  atmos-
                 phere from each source.   Emission factors
                 and level, and types of air pollution con-
                 trol will also be provided for each  of
                 these sources to the extent permitted by
                 available information.

               • Define those sources which contribute at
                 least 80% of the total emissions of  silver.

               • Provide a regional breakdown of these major
                 sources and their emissions.

               • Present the nature of the silver-containing
                 emissions for each of these major sources
                 including a delineation of their physical
                 and chemical form and particle size  distri-
                 bution, to the extent that information is
                 available.

               • Provide recommendations as to a methodology
                 for updating the results of this study  every
                 two years.

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     B.   CONCLUSIONS
         1.   Material Flow
             Based on all available  data,  105 x 10   troy  ounces  (29,000
troy ounces  = 1 U.S.  short ton)  of silver  was consumed  in the  U.S.  in
1970.  As shown in Figure 1,  about 25 percent of this was recovered as
old scrap, the remainder being in use or wasted in  various ways.   The
sources of silver included domestic  mining and net  imports, in about 4:3
proportion.   Approximately 160 x 10   ounces underwent primary  or second-
ary refining, of which part was exported and part was recycled as new
scrap.
             The principal users of silver were the following  industries:
                 Photography — 30 percent
                 Contacts and conductors ... 20 percent
                 Sterling and jewelry ...  20 percent
                 Brazing alloys, solders,
                 and electroplating ...  20 percent
                 Other uses ... 10 percent
Certain assumptions made in preparing the above estimates, due to a de-
ficiency of data in certain areas, are explained in detail in Chapter II.
         2.   Principal Emission Sources
             Silver is somewhat unique in that most of the atmospheric
emissions of silver are not associated with  the silver industry  (Chap-
ter  II).  The  principal  sources  (after emission control,  if any) are the
iron and steel industry  (46 percent), cement industry  (25.7 percent),
combustion of  coal and oil  (13.6 percent),  and incineration (5.6 percent)
One  reason for this is  that the  silver  industry is  small in comparison
with the iron  and  steel  and coal industries.  A second reason is  the
value of  silver, which  results  in close attention  to silver processes
in which  aerosols  containing  silver  are generated.
             Within  the  silver  industry,  the most  concentrated  emission
sources  are  primary  and  secondary smelting  and  refining  (1.1  percent).
Although about four  times  as  much silver  is emitted in the wearing of

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electrical contacts, this emission is spread geographically over a
very large number of sources.
         3.  Regional Emissions
             The regions of the U.S. in which most of the estimated
emissions of silver occur are Regions 3*and 5, the east central por-
tion of the U.S.  The region in which the total emission per square
mile is greatest is Region 3, the Pennsylvania-Virginia portion of
the U.S.  As noted above, these estimates result far more from the
geographical distribution and nature of the iron and steel industry
than from the silver industry.
         4.  Nature of Emissions
             The principal emissions of silver are believed to be
elemental silver, with some simple sulphides, oxides, and halides.
This opinion is based on the nature of silver and the characteris-
tics of the high-temperature operations producing the emissions.
             Particles containing silver are probably on the order
of one micron diameter (MMD).   The particles are expected to travel
considerable distances (miles) before being deposited,
         5.  Degree of Control
             The overall level of control of silver emission is es-
timated to have been about 85 percent in 1970.  Large sources under
relatively poor control included open hearth steel production and
municipal incineration.  Large sources under relatively good control
included blast furnace iron production and commercial incineration.
         6.  General Comments
             The silver content of coal, oil, and/or incineration
ash may be sufficient to be of commercial value.  Investigation of
this might result in added interest in controlling these emissions,
and hence, further documentation of this area is recommended.
  See page 26 for a list of regions.

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 II.   OVERALL U.S.  MATERIAL FLOW CHART FOR SILVER
      Figure  1*  presents  a  flow diagram depicting the  total  quantities
 of  silver  products moving  from sources of mining and  importation
 through  the  processing and reprocessing steps  t;o ultimate use  and  fi-
 nal  disposition.   Each of  these sources is discussed  below.
      A.  U.S. PRODUCTION AND ORE PROCESSING (45,Q06,000  ounces)
         Silver is produced mainly  as a co-product  of base  metal ores
 (66  percent  in  1970)  and from silver  ore (32 percent).   '   In  1970,
 the  separate U.S.  sources  were (in  troy ounces;  29,16? fcroy ounces  =
 1 U.S. short ton):
              16,023,000  -  copper ore  processing
              14,258,000  -  silver ore
              11,128,000  -  copper-lead,  lead-zinc, copper-zinc,
                           and  copper-lead-zinc ore  processings
              2,581,000  -  lead ore  processing
                415,000  -  gold ore  processing
                397,000  -  gold-silver ore  processing
                158,000  -  processing  of old mine  tailings;
                           also tungsten and uranium ore  pro-
                           cessings
                 46,000  -  zinc ore  processing
         The Department  of Commerce reports the  1970  mining production
                                (2)
of silver as 47,483,000  ounces.v  '  The  above sum and figures appear
to be more thoroughly documented, however.
     B.  IMPORTS AND EXPORTS  (Net,  34,671,000 ounces  imported)
         In  1970 about 40  percent more  silver wap imported  than  mined
(62,300,000  ounces).   Of this,  about  half was in tfce  form of bullion
or refined silver  (32,600,000  ounces) and half in forms  requiring
                                                             a 3*1
various types and  degrees  of refinement  (29,700,000 ounces).
*
 Data in Figure 1 and in this section are left unrounded for purposes
 of information control.  On average, the typical statistic is accur-
 ate to within 10 percent, in the opinion of the authors.

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Ul

and Processing

Gold Mining
tad Processing

Gold-Silver
Mining & Processing

Copper Mining
Lead Mining
Zinc Mining
and Process ing

Metal Ores

uraniuv & tung-









Treaaury
Release, Net






415


397 ^


•»'
2,581 ^
	 ^— J
11.128


15. ,..




62 300




67,900














45,00















































r*











Prils
ReEln
(63,




	 >-























"1
erles
100)




Se
Re




























8
on
Fin























81
»•



3,0
dir
Ing























,381
224,



43
y
























>2|





























129



























I

09
77



























nd
at
f
f


























67.799
uBtrlal & Pri-
re«9«. Net
Intermediate
Processing
29














23,999
Nev
Scrap































11,437
\ *"
1
1
24.235 +


1
t
31,044 |
1 *"
1,804
'•18i \>
I
i
14,035 T.
1 *
\
6,>42 | _.
1 ^~
I
25.18, ^
1
1
,8, }


1.999


709 | _
4
3.539
I





Sterling




Photographic
Materials
Dental & fedical
Supplies
Mirrors
Brazing Alleys



Contacts and


Bearings


ata jsts

Coinage and
















	 *-


,

	 •*•




	 •*•




















(105,097) 79,778
I ^
i • '" ' ' 	
25,319 rji.t.
Sera











	 i

                             *GCA Estimate
                      Figure I   SILVER 1970 MATERIALS FLCW
                                 (THOUSANDS OF TROY OUNCES; 29,000 TROY  OUNCES « 1 U.S. SHORT  TON)

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         Total silver exported was roughly one-third of that imported
(27,629,000 ounces).  Most of this was refined metal (17,240,000 ounces),
with waste, sweepings, ore and concentrates (10,378,000) comprising the
    .   ,   (1)
remainder.
     C.  STOCKPILE CHANGES (Net Decrease, 101,000 ounces)
         About 50 percent more silver entered the domestic supply from
Federal sources than was mined in 1970 (67,900,000 ounces).  '  This
was chiefly in the form of coinage silver sold by the Treasury,  which
had accumulated in connection with the recent sharp reduction in the
use of silver in coins.  This program of large-scale sale of coinage
silver was completed in late 1970.  Consequently the 1970 stock deple-
tion should be viewed largely as a non-recurring item.   (Note:  The
same reference also gives the 1970 depletion of Treasury stock as
79,000,000 ounces, however without documentation.)
         The U.S. industrial stockpile is estimated to have increased
                             (2)
by 43,800,000 ounces in 1970.^ '  This includes the holdings in U.S.
commodity exchanges, but does not include the silver in private hands
and in banks.   With the cessation of U.S. silver coinage and the
sharp rise of the price of silver, private speculative holdings may
have increased, although data is not available to support this.  We
estimate that in fact the sum of industrial, commodity exchange, and
private holdings increased by the amount 67,799,000 ounces in 1970.
This is approximately the amount of silver released by the Treasury,
which was also an unusual event.  This release of Treasury silver and
the proportionate unusual increase in silver holdings tend to cancel,
leaving the imported, produced, and secondary silver flows about the
same as in other recent years.
     D.  SCRAP RECYCLING (49,318,000 ounces)
         The total new silver entering the economy (mined, imported,
and released from the Treasury) was 175,206,000 ounces.  Of this, part
entered industrial stockpiles and part was exported, leaving 79,778,000
ounces of new silver for ultimate domestic consumption, after scrap
recycling.

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         The amount of new scrap recycled was 23,999,000 ounces.
This is material in relatively pure form requiring a minimum of refine-
ment.  The amount of old scrap recycled was 25,319,000 ounces.      This
includes salvaged products, chemical waste, precipitates, etc., re-
quiring considerable refining.  The total scrap recycled (49,318,000
ounces) combined with the new silver to give a total supply of
224,524,000 ounces.  After exports and stockpile changes, this left
129,096,000 ounces as the domestic supply.  After new scrap, 105,097,000
ounces remained for use in various products.  Old scrap was later re-
covered in the amount of 25,319,000 ounces, leaving 79,778,000 ounces
in the form of new products still in use, discarded products not sal-
vaged, and other wasted silver.
     E.  PRIMARY SMELTING (8.,381,000 ounces/1'
         In addition to the U.S. mining ores and concentrates, U.S.
primary refineries also processed 36,375,000 ounces of silver from im-
ported materials, coinage released by the Treasury (containing 90 per-
cent silver), and recycled materials.  In general, the type of mater-
ial to be refined determines whether it requires primary treatment, or
whether it can be processed more simply by a secondary refinery.
     F.  SECONDARY REFINING (80,043,000 ounces)^'
         In addition to old and new scrap, secondary refineries also
processed various amounts of imported materials and Treasury coinage
silver.  There are many such refineries handling a wide variety of
scrap and  byproducts.  The material may pass through several hands
and stages of refining before attaining a useful form and purity.  The
above figure is therefore an estimate, based on the refineries that
were considered in the references utilized.
     G.  CONSUMPTION OF SILVER  (129,096,000 ounces)
         Purchases of silver were reported as follows:
             38,044,000 - photographic materials
             25,183,000 - contractors and conductors
             24,235,000 - sterling and jewelry

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              14,035,000 -  brazing  alloys and  solders
              11,437,000 -  electroplating
               6,342,000 -  batteries
               1,999,000 -  catalysts
               1,804,000 -  dental and medical  supplies
               1,386,000 -  mirrors
                 709,000 -  government coinage
                 383,000 -  bearings
               3,539.000 -  miscellaneous
   Total     129,096,000   ounces
Whether or not  these reported purchases  include or exclude new scrap
is a matter of  some uncertainty in the silver industry.  The Bureau
of Mines and the Department of Commerce  both publish "industrial
consumption" figures, which however, differ approximately by the
amount of new scrap. (  '  It is probable that the above figures
include new scrap, and  that the remainder, 105,097,000 ounces, was
actually made into products by the above "consuming" markets.  Figure
1 is based on this assumption.  After new scrap, 25,319,000 ounces
was subsequently salvaged as old scrap from expired products as low-
grade wastes, leaving 79,778,000 ounces  for ultimate disposal by buri-
al or incineration.

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III.  SOURCES AND ESTIMATES OF SILVER-CONTAINING EMISSIONS
      A.  DATA PRESENTATION AND ACCURACY
          Table 1 presents a summary of the data from which emissions
were estimated for all major potential sources.  Each of the six col-
umns comprising this table will be discussed below.
          1.  Emission Factors
              Except where indicated, this gives the pounds of total
particulates emitted per ton of production.  Such considerations as:
              . variations in process conditions among
                individual plants comprising a source
                category
              . inaccuracies in existing data
              . a limited quantity of existing data,
may, however, result in an average emission factor  for a source cate-
gory varying by more than an order of magnitude  from the value pre-
sented.  In recognizing the need to  indicate the level of accuracy  of
these emission factors, a reliability code is presented along with
each emission factor value appearing in the table.  This reliability
code system is described below and is based on the  system utilized  in
EPA Document No. AP-42, "Compilation of Air Pollutant Emission Fac-
tors":
              A:  Excellent
                  This value is based on  field measurements
                  of a large number  of sources.
              B:  Above Average
                  This value is based on  a limited  number
                  of field measurements.
              C:  Average
                  This value is based on  limited data and/or
                  published emission factors where  the ac-
                  curacy is not stated.
              D:  Below Average
                  This emission factor is  based  on  engineering
                  estimates made by  knowledgeable personnel.

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                                                          TABLE 1
                                     SOURCES AND ESTIMATES OF SILVER-CONTAINING EMISSIONS
o
Source
Iron and Steel
Sinter Process

Blast Furnace

Open Hearth

Basic Oxygen

Electric Arc

Iron Foundry
Coal
Oil
Gasoline, etc.
[ncineration
Municipal
Commercial
Cement


Uncontrolled
Particulate
Emission
Factor
Ib/ton

20
Sinter
130
Pig Irop
17
Steel
40
Steel
10
Steel
20
NA
HA
NA

NA
--
NA


kg/10\g

10

65

8.5

20

9

10
NA
NA
NA

NA
--
NA


Reliability
1 Code

C

C

C

C

C

C




.


-

Production
Level
(tons/yr)

51,000,000

88,800,000

65,800,000

48,000,000

16,800,000

22,000,000
33,800,000a
287,000°
450,000,000

ioo,oooa
	
7,790,000C


7. Ag in
Emissions

0.01

0.01

0.05

0.004

0.05

0.008
0.0007
0.005
o.oooooib

0.037
	
(0.008-
0.015)
0.01e
Reliability
Code

D

D

C

D

D

D
A
A
B

B

B


Ag Emissions
Before Controls
tons/yr

51

578

280

38

42

18
236
14
4.5

37
220
896d


106oz/yr

1.5

16.8

8.2

1.1

1.2

0.5
6.9
0.41
0.13

1.1
6.5
26. Od


Estimated
Level of
Emission
Control
(%)

90

99

40

99

78

75
82
0
0

37
99
88


Ag Emissions
After Controls
tons/yr

5.1

5.8

168.0

0.38

9.2

4.5
42.5
14.0
4.5

23.0
2.2
107.0


106oz/yr

0.15

0.17

4.90

0.01

0.27

0.13
1.24
0.41
0.13

0.68
0.07
3.1d



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            2-   Level  of Production Activity
                This column depicts the quantity of material produced
  (unless  otherwise stated) annually.  When multiplied by  the emission
  factor,  an estimate  of the  total particulate emissions for that source
  in pounds  per  year is obtained.

                The values in this column are based on the material flow
  calculations presented in Section II.  Consequently, they have the
  same accuracy  as those material flow values which is estimated at
 + 10 percent.
           3-   Percent Metal in Emissions
               The method of analyzing or assaying a dust sample for
 the amount of metal it contains determines to a large extent the re-
 liability of  the data.   For example,  analytical chemistry techniques
 for dust containing  substantial fractions  of metal  can be accurate to
 within a small percentage.   On the  other hand,  optical  spectroscopy
 methods for determining  concentrations  on  the order of  parts  per mil-
 lion can be inaccurate by a  factor of 2.   Because of this variability,
 the reliability codes discussed above for  the emission  factors are
 also utilized  to estimate the  relative  accuracy of  the  percentage
 values  listed  in column 3.
           4-   Level of Emissions Before  Control
               The values  in  this column  are  derived  by  multiplying
 the values  in  columns 1 through 3.  The  result  is converted to tons/
 year  of emissions before  control.
           5.  Estimated Level  of Emission Control
              The overall effectiveness of control  for  a  source cate-
 gory is based on two  factors:

               . the portion of  the processes which are under control
               . the typical degree of control
For example, if 60 percent of vertical roasters have some type of
particulate emission control, and these  include both scrubbers and

                                12

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precipitators such that the apparent weighted average efficiency of
control is 85 percent, the overall control effectiveness is estimated
60 x 85 = 51 percent.
              The accuracy of control efficiency data varies with the
degree of control.  For a wet scrubber operating at 80 percent effi-
ciency; i.e., passing 20 percent material, the actual emission may
safely be assumed to be between 15 and 25 percent because of the rela-
tive ease of making determinations at this level.  Thus the emissions
after control may be assumed to be accurate within + 5/20 or 25 per-
cent.  On the other hand, for a baghouse reported as being 99 percent
efficient, or passing only 1 percent of the material, the actual emis-
sion may vary from 0.5 percent to perhaps 2 percent because it is fre-
quently difficult to make low-level measurements with accuracy.  In
such case, the resulting emission data could be in error by a factor
of 2.
              Unless otherwise specified, it is assumed that the re-
ported overall level of particulate control applies equally to all
silver-containing particles, independent of size, resistance and other
important collection parameters.  This assumption results in a correct
estimate of silver emissions after control when the particulate is
chemically homogeneous; i.e., silver is contained in the same concen-
tration in all particles.  If however, silver is concentrated in cer-
tain particles and in addition the efficiency of the control equip-
ment is not uniform for all particles, then the utilization of an
average control level is less valid for calculating silver emissions
after control.  Data on the preferential control of silver-containing
particles is seldom available, but is included in this report when
possible.
              The accuracy of estimating the level of control for a
specific source category is dependent on the quality of available data.
The investigators feel that, in general, the level of control data
will contribute an accuracy to the resulting emissions estimates with-
in + 25 percent.
                                 13

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            6>  Level of Metal Emissions After Control
                The values in this column are derived by multiplying the
  values in column 4 by the value (100 minus estimated  Level  of Control).
        B.   DEVELOPMENT OF EMISSIONS ESTIMATES -  1970
            Due to the  value of silver,  careful control of  all  processes
  involving silver is standard  practice.  Wasting  of  silver,  including
  airborne  particulate,  is  tolerated only as  an economic  or practical
  necessity.   Consequently,  the  emissions containing  silver,  listed  in
  Table  1,  tend to be smaller in proportion,  as well  as in magnitude,
  than have been identified  for  the  other metals in this review.  The
  largest silver emissions  (iron and  steel processing; coal combustion;
  incineration)  comprising about  85 percent of all silver emission, are
  not a part of  the silver industry, but are  the inadvertent results of
  other practices.  Data pertaining to these  largest emissions are lim-
 ited for two reasons:   The silver industry has not been interested in
  them as economic sources of silver; and silver has thus far  had a low
 priority as an air pollutant.
           1.   Iron and Steel Production
               Very little information has  been found giving  typical
 Ag contents  of the emissions from the common iron and  steel  manufac-
 turing  processes.  Orban,  et al.(4) found  a  "trace"  of Ag20  in the
 emission from a Bessemer  converter,  with an  apparent resolution of  his
 tests of about 0.02 percent.   Hammond,  et  al.(5>  reports 0.05  percent
 Ag in the  particulate  discharge from an open hearth  furnace, based
 on "qualitative"  spectrographic analysis with  an  apparent  test  resolu-
 tion of 0.01  percent.  The  same  authors also give an average of  0.0091
 percent Ag in samples  from  a baghouse serving a gray iron cupola
 furnace, based  on a qualitative  analysis.  No other directly useful
 data was found.

              Additional perspective is gained indirectly,  however,
in other ways.  The average concentration of Ag in the earth is
0.000002 percent;(6) and in coal ash, 0.0007 percent (see below). Ag
                                14

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tends to occur naturally with some other metals, zinc in particular,
and also copper, aluminum, and manganese.  These metals bracket the
melting and vaporizing temperatures of Ag (960 C and 1950 C, respec-
tively, see Section V).  Because they are usually emitted in larger
concentrations, they are more easily measured and more often reported.
Because of their similarity to silver's thermal characteristics, the
ratio  of silver to these metals may tend to be preserved in emissions
from high temperature processes.  In those iron and steel emissions
for which data is available, the ratio of silver to zinc appears to
be of the order of 0.003, and of silver to copper, 0.10.  Data on zinc
and copper emissions from all processes listed in Table 1 are general-
ly available.   '    Using these known emissions and the apparent ratios,
plus the actual silver emission data cited above, estimates of silver
emission were made as given in the table.  They vary from 0.004 to
0.05 percent.
              Table 1 indicates that the iron ore blast furnace gener-
ates one of the largest quantities of silver, equal in magnitude to
one-third of all the silver mined in the U.S. annually.  Because the
blast furnace is well controlled, however, the final silver emission
is not outstanding.  The open hearth furnace, on the other hand, be-
cause of a lower level of particulate control, emits approximately 37
percent of all Ag emissions in the U.S.  This quantity is equivalent
to about 10 percent of the silver mined domestically.
              Iron and steel production as a whole is estimated to
contribute 58 percent of the silver emission.  It is noteworthy that
the silver content of these emissions is estimated to be similar to
those of copper and lead refinery emissions.  The latter are collected
when possible and processed for their valuable metal contents.  A
silver content of 0.01 percent is equivalent to 2.9 ounces/ton, a
marginal concentration in ore form, but perhaps more attractive in
fume form.  Current prices of refined silver are approximately $2.00/
ounce.
                                15

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            2-  Coal and Oil Combustion
                Silver and coal sometimes occur together in nature.  For
  example, in Utah in the 1870's, thin scales of silver were found along
  with small deposits of minable lignite in sandstone.   Evidently almost
  any concentration of Ag in coal could be encountered  depending on the
  size of the coal sample and its source.   Abernathy and Gibson,(9) in
  a survey of trace metals in coal,  cites reports  of maximum silver con-
  tents of 0.0001 to 0.0084 percent  in the ash of  a variety of western
  and West Virginia coals.   The geometric  mean is  about 0.0009 percent.
  •n    (")
  Brown    gives the maximum silver  content of coal ash as  5 to 10 ppm,
  equivalent to 0.0005  to 0.0010 percent silver.   Accordingly,  the av-
  erage of 0.0007 percent is  used in Table 1
                Table 1  estimates  that slightly  less  silver emission is
  developed  from coal combustion than from the open hearth  process.
  Furthermore,  coal  power plants  are controlled  about three times  as well
  as  the  open hearth process  (82 percent(32) versus 40  percent  control).
  Thus, controlled silver emissions  from coal  burning contributes  about
  15 percent of  the  U.S.  silver  emissions.
               The above references  indicate that  the ratio of
 silver to copper in both the earth, and in coal,  is about 0.002;
 and  of silver  to zinc,  about 0.0005.  These ratios may be useful
 in arriving at order of magnitude estimates of the silver content
 of other samples  of coal ash that have been tested for copper or zinc,
 but  not  for  silver.
               Gerstle,  Cuffe,  et  al.(10>11) report the emissions  of
 numerous  other  trace metals  in coal ash,  but  not  silver.   Their data
 give  the  efficiency  of  an electrostatic precipitator on each  of the
metals.   The copper-zinc ratio in the  ash was reduced  by one-half  in
passing through the precipitator.   This suggests  that  silver may also
be differentially controlled by the equipment in  use.  We  have  used
the average 82 percent level of control, however.
              The combustion temperatures of coal are in the vicinity
of 1700 C, approaching  the vaporization temperature of silver.  Thus,
                                 16

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part of the silver in the coal may be vaporized within the firebox.
It is probable that this silver vapor condenses into the ash as the
combustion products cool.  Thus, we have assumed that the ash assay,
as reported above, includes essentially all of the silver emitted by
the process.  The same assumption applies to iron and steel and other
high  temperature process emissions in Table 1.
              Analysis of  the  ash from  fuel oil would be  expected to
be  similar  to that  from  coal,  in  the sense that both are  fossil fuels.
Comparisons  of  typical analyses of each show  similar concentrations
of  copper  and zinc.   Levy,  et  al.(21) report  a concentration  of 0.0018
percent silver  in oil ash  (optical emissions  spectroscopy), moderately
higher than the coal  ash assay.   On  the other hand, Walsh     reports
 a concentration of 0.03  percent silver  in oil ash (spectrographic
analysis).   Trace metal  content of oil  is known to  vary by  factors
                                               (13)
of  25 or more,  depending upon the type  of oil.v    All factors
considered,  an  average of  0.005 percent is used in  Table 1.   Oil
 combustion emissions  are uncontrolled,  resulting in a  level of
 silver emissions from fuel oil combustion (0.41 x 106  ounces)
which is about  one-third the level  emitted from coal  firing.
           3.  Gasoline and Other Light Fuels
               Analyses of premium and low-lead gasolines indicated
 silver concentrations ranging from less than 0.001 to 0.4 ppm with
 apparently reliable data of 0.002 ppm  (neutron activation), 0.02 ppm
 (spark source mass spectroscopy), and 0.05 ppm (spark source mass
 spectroscopy),  being reported.<23>  An average content of 0.01 ppm
 is assumed.  The silver contents of other light  fuels were not
 available, and were assumed to be the  same as for gasoline.  It
 is further assumed that the silver in  these  fuels is entirely emit-
 ted  to the atmosphere.  Including kerosene,  light distillates, and
 jet  fuels with gasoline, 3.4 x 109 barrels or about 450  x 10  tons^
 were burned in 1970.  The resulting emission  estimate of 0.13 x 10
 ounces of silver is  shown in  Table 1.
                                   17

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             4'   Incineration
                 Assays  of samples  of  fly  ash  from  refuge  combugtion  have
   indicated  a  silver  conf-pnt-  of  •>  »-~  n
                      content  of  2  to  9  ounces per  ton  of  ash  (equivalent
   to  0.006 to  0.028 percent As)(14)   A™^                     q«"-vaient
                    percenc AS;-       Another  source reports a content of
   19  ounces  per  ton  (0.059 percent Ag).<15)

                An estimated  average  value of 12 ounces per ton of fly-
   ash, or 0.037 percent Ag, is used in Table 1.   Note that at this rate
   the recovery value of the silver is about 14 times greater than the
  cost of disposal of the ash that was recently  estimated to be $1.50/
            The net emission of 0.68  x 106 ounces is the third highest
  emission in the table.

                Recently,  special purpose  commercial incinerators  have
  been developed  specifically  to  recover the  silver used in photographic
  materials.*     Of  the 38 x  106 ounces of silver  used  annually by  the
  mdustry, it  is  estimated that  14 x  106  ounces  is recycled as preci-
  pxtates  from photographic processing solutions.   Of the  remainder   it
  is estimated that 6.5 x  106  ounces is  processed by the special incin-
 erators, the rest being burned  in municipal incineratprs  or wasted  in
 various other forms.  The special incinerators  are reported to recover
 at least 99  percent of the silver, resulting in a net emission of only
 0.07 x 10  ounces from commercial incinerating  operations.
           5.   Cement
               Assays  of dust from three cement plant  clinker  coolers
 indicated  0.015  percent silver  (spectrographic analysis)  according to
 a  review of EPA  data.<  2>  Assays  of  dust  from thre£  air  separators
 indicated  0.008  percent silver,  also  from  EPA data.   Based  on these
 Percentages (0.008  to 0.015  percent),  the  range  of  silver emissions
 xs 75 to 140 tons/year  after 88  percent control  with  an intermediate
value of 107 tons/year  in this survey.  The resulting emission esti-
mate of 0.32 x 10  ounces is only about 3 percent of  the total U.S.
silver emission.
                                 18

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          6.   Production of Non-Ferrous Metals
              a.   Mining
                  Mining and milling operations are estimated to gen-
erate 200 pounds of emissions per 1,000  tons of production,  for each
of several non-ferrous metals.<17'18) If one assumes that the concen-
tration of silver in the emitted dust is the same as in the ore being
processed, then 200 pounds of silver emissions are generated for each
1,000 tons of silver produced.  In 1970, 45 x 10  ounces of silver
were produced.  Thus the estimated emission of silver from all non-
ferrous mining and milling operations generating silver as a co-product
is 4,500 ounces.  This is after particulate control, which is minimal.
              b.  Primary Smelting
                  In the case of copper smelting, Davis reports 10.1
ounces of silver per ton of  emitted  dust  (0.035 percent Ag), and 10
pounds of emitted dust per  ton of copper produced, after control by
an electrostatic precipitator at about 97 percent efficiency.
This measurement was made  at the stack, where  effluents from various
operations had been combined, notably, roasting, reverberatory  furnace
smelting, and  converting.   This  indicates an effective before-control
generation of  333 pounds of dust per ton  of copper.   In other  plants,
it was reported  that  emission factors of  704 pounds  of dust per ton
of product was generated in smelting before 99 percent control;  1833
pounds per ton of product  in smelting before  99 percent control;  and 3.1
pounds per ton of product  in unspecified  processes  before control.
Using  an average 1,000 pounds per  ton generated, with a copper produc-
 tion of  1,765,000 tons in  1970 and  a control efficiency of 99 percent,
results  in approximately  90,000 ounces  of emission as shown in Table 1.
                   In the  smelting  of other ores,  an estimated 50 per-
 cent of  the  1970 U.S.  silver production was derived through lead,
 zinc,  lead-zinc, and silver ores.(1) The silver content  in these ores
 averages about 8.7  ounces  per ton,  whereas in copper ore  the content
 is only about 0.07  ounces  per ton (1963 data).(19)  The ore is first
                                  19

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concentrated by flotation in which little aerosol is generated.   After-
ward, there is still a much higher proportion of silver along with
these other metals than with copper.   A limited amount of emission data
             (24)
is available.      Sintering and sinter crushing at a lead smelter is
reported to generate 0.3 pounds of dust per ton of product before an
average control of 92 percent.   For a lead blast furnace and a rever-
beratory furnace, emissions are reported to be 20 and 36 pounds  per
ton, respectively, before 95 percent control.  Zinc smelting in gener-
al is reported to emit 7.0 pounds per ton before an average 90 percent
control.
                  In none of these cases is the silver content of the
emitted particulate reported.  Since the data base is insufficient
for a complete computation of silver emission, the following estimates
are made:  particulate emission averages 25 pounds per ton, on a base
of 1,460,000 tons of heavy metal produced in 1970; the average assay
of the particulate is five times greater than for copper due to the
higher proportion of silver present;  and control efficiences average
95 percent.  As a result, 45,000 ounces are estimated to be emitted
after control.
                  Less than 1 percent of the silver produced in the
U.S. in 1970 was produced by the processes of amalgamation and cyani-
dation.  In the former process, after crushing, washing and drying of
the ore, it is mixed with mercury and then heated in a retort furnace.
In the latter process, the crushed ore is leached, after occasional
roasting, and the silver is precipitated from the leachate before en-
tering a reverberatory furnace.  It is estimated that 1 percent of
the silver produced by these two processes escapes as aerosol, or
1,200 ounces.
              c.  Secondary Refining
                  The refining of scrap metals other than  silver  scrap
is believed to be relatively free of silver emissions since most
scrap has a low silver content.  One possible exception is copper
scrap from electrical products, which contains considerable silver in

                                 20

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the form of electrical contacts and conductors.  The 1970 consumption
of silver for contacts and conductors was 25 x 10  ounces; and the con-
sumption of copper by the electrical industry, about 50 percent of the
U.S. copper consumption was 1.0 x 10  tons.  The resulting ratio is
25 ounces of silver per ton of copper.  Emissions of copper from sec-
ondary copper refining after controls have been estimated at 210 tons
per year.      If the consumption ratio applies to these emissions,
then it is estimated that up to 5,250 ounces of silver is emitted
during secondary copper refining.  At 97 percent control efficiency,
this would be 167,000 ounces before control.

                  Emissions from the secondary refining of lead in
                                         (22)
blast furnaces are reported in two cases.      One furnace controlled
by scrubber (estimated efficiency 90 percent) produced 1.14 pounds per
ton of particulate after control, containing approximately 30 ppm of
silver.  The second furnace controlled by cyclone and fabric filter
(estimated efficiency 99 percent) produced 0.17 pounds per ton of par-
ticulate after control containing about 170 ppm of silver.  The com-
puted pre-control emission factors average about 15 pounds per ton,
and the post control assays average 0.01 percent.   Only about 75,000
tons of scrap lead were refined in 1970, resulting in a negligible
0.05 tons of silver generated before control.
                  Other than the commercial incineration of photo-
graphic materials included above, silver scrap is generally refined
by melting followed by electrolytic refining.  A typical reverbera-
tory furnace may emit 30 pounds per ton of metal,  and an electrolytic
cell, 2 pounds per ton,      for a total emission of 32 pounds per ton.
These emissions are controlled at an estimated 98.5 percent.   Since
only 80,043,000 ounces of silver underwent secondary refining in 1970,
the emission is estimated to have been 1,280,000 ounces before control,
and 19,200 ounces after control.
          7.   Intermediate Silver Products
              Practically all of the 129,096,000 ounces of silver con-
sumed by the  various markets first passes through  intermediate hands,

                                 21

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  where it is processed in various  ways/20)   The  metal,  in various  de-
  grees of purity,  may be alloyed;  shaped  into wire,  sheet,  powder,  etc;
  or converted chemically or electrochemically.  Few,  if  any,  of  these  '
  processes emit significant amounts  of  silver,  because relatively few
  firms convert most  of the  silver.   Also,  these processes usually in-
  volve limited amounts of silver and are  closely  supervised.
                In  forming powdered silver, a  jet  of molten metal is
  combined  with a high  velocity air jet.  From 40  to 90 percent of the
  particles  thus formed  are  50 microns or under.   It is unlikely that
  any appreciable number  of particles 5 microns  or smaller are produced
  by this process.  Since  larger particles will be well controlled, it
  is assumed  that the resulting emission of silver is negligible.
               Nearly all silver for photographic consumption is  first
 converted to  silver nitrate by dissolving the metal in hot nitric acid
 in an enclosed vessel.  The fumes  that escape this vigorous reaction
 are scrubbed to control the nitrogen oxides  produced.  The literature
 on this process is preoccupied with  gaseous  control problems rather
 than silver loss.   It is unlikely  that  any appreciable  quantity  of
 silver escapes.   Similarly,  electrochemical  conversion  of  silver into
 silver sulphate may  involve the boiling of hydrogen gas, with possible
 minor  emission of  silver.  Silver  sulphate,  chloride, cyanide, and
 oxides are produced  in relatively  small quantities  compared  to silver
 nitrate.

               Little  aerosol is emitted in shaping  silver.   The various
 steps  may  include weighing  and charging a  crucible  for melting; poring
 and casting  into molds;  rolling, slitting, drawing.  As a percentage
 of all U.S.  emission of  silver, these sources are estimated  to be
 negligible.
          8.   Consumption of Silver
              a.  Electrical Contacts
                  About one-half of the 25,183,000 ounces of silver
used for contacts and conductors,  or  12,000,000 ounces is estimated  to
                                 22

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be used  annually  for  solid  (cast or machined) and composite  (laminar)
contacts.  Although silver  is used because it withstands sparking and
mechanical wear well, it is evident that the contacts do nevertheless
undergo  wear.  It is  assumed that the contacts are designed  to last
the  life of  the rest  of the electrical equipment, which is typically
about 20 years.   That is, it is estimated that 5 percent of  the silver
consumed annually is worn away in the form of aerosol.  This results
in 600,000 ounces of  emission per year.  This is spread over a very
large number of locations,  as most appliances, automobiles,  telephones,
etc. use some  silver  contacts.
               b.  Brazing and Soldering
                  About 14,000,000 ounces of silver are consumed by
brazing.  Although the production of these alloys is relatively non-
emitting and easily controlled, the brazing process emits a consider-
able amount of fume.  An estimated 1 percent of silver in these alloys
is emitted, the rest of the metal remaining at the point of joining.
Most of  the brazing is done in specialized locations (air conditioning
and refrigeration is estimated to consume 20 percent; automotive and
aircraft, 30 percent) which permits these emissions to be better con-
trolled  than others (plumbing and heating, and electrical appliance
brazing  tend to be non-concentrated).   Assuming that emissions from
brazing  and soldering are 50 percent controlled, the net emission es-
timate is 70,000  ounces of silver.
          9.   Other Sources
              GCA estimates that these sources contribute  43,000
ounces of silver emissions, or about one-half percent of the total.
The following minor sources have been considered:
                                               Emission Estimates
              Silver Consumption               	(ounces)
      Conductors,  spray painting                    10,000
      Bearings and lubricants,  loss  of
      flake silver lubricant in use                   2,000
      Mirrors,  spraying of  solutions                 1,500
      Batteries,  sintering,  electrolytic
      processes,  chemical  losses                        900

                                23

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              Silver Consumption
      Electroplating, chemical and liquid
      spills
      Catalysts, preparation,  regenera-
      tion and erosion
      Sterling and jewelry, buffing and
      polishing
      Brazing alloys and solder, production
      Medicine and dentistry,  preparation of
      materials
              Miscellaneous Sources
      Non-metallic mineral operations emit-
      ting dust with trace silver
      Forestry and agricultural burning  of
      unwanted waste containing trace silver
      (Note:  Forest fires not included)
      Cloud seeding
      Wear of coinage
Emission Estimates
	(ounces)	
        250

        250

        200
        150

        100


     20,000

      7,500
     negligible
     negligible
      C.  SUMMARY OF PRINCIPAL EMISSIONS
                                            TOTAL   42,850
          Table 2 summarizes the largest 1970 emissions of silver, as
the estimates were developed in Table 1.  These are grouped into in-
dustrial sources, those directly associated with the silver industry,
and inadvertent sources, those having little to do with the silver in-
dustry.  In the case of silver, the latter category is the larger.
                                 24

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                        TABLE 2




PRINCIPAL SOURCES OF SILVER-CONTAINING EMISSIONS - 1970
Source
Inadvertent Sources
Iron and steel production
Cement production
Coal burning
Municipal incineration
Oil burning
Silver Industry Sources
Electrical contacts
Primary smelting
Percent of U.S. Total
Ounces /year
5,630,000
3,100,000
1,240,000
680,000
410,000
600,00
133,000
Tons /year
193.0
107.0
42.5
23.3
14.0
20.6
4.5
Percent*
46.3
25.7
10.2
5.6
3.4
4.9
1.1
97.2
Percent of Table 1 total, 12,100,000 ounces/year.
                          25

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 IV.   REGIONAL DISTRIBUTION OF PRINCIPAL SOURCES AND EMISSIONS
      For purposes of showing  geographical  distribution,  the  U.S. was
 divided into ten regions  identical  to  the  Regional  Branches  of EPA:
                                     States
                      Connecticut, Maine, Massachusetts,  New  Hampshire
                      Rhode Island,  Vermont
             II       New  Jersey, New York, Puerto Rico,  Virgin Islands
            III       Delaware, Maryland, Pennsylvania, Virginia, West
                      Virginia, District of Cplumbia
             IV       Alabama,  Florida,  Georgia, Kentucky, Mississippi,
                      North Carolina, South Carolina, Tennessee
              V       Illinois, Indiana, Michigan, Minnesota, Ohio,
                      Wisconsin
             VI       Arkansas, Louisiana,  New Mexico, Oklahoma, Texas
            VII       Iowa,  Kansas,  Missouri, Nebraska
          VIII       Colorado, Montana, North Dakota, South  Dakpta,
                      Utah,  Wyoming
             IX       Arizona,  California,  Nevada, Hawaii and the South
                      Pacific
             X       Alaska, Idaho^, Oregon, Washington
Emissions from the principal sources listed in Table 2 are.distributed
among these  ten regions as  shown in Table  3.  Also, the number of plants
producing the  emissions i.s shown in the table when such information is
available.
     The accuracy of  the distributions by region varies^ with the cate-
gory.  The number of  plants per category ranged from one to  several thou-
sand in this study.  When  the number of plants was  less than about 100,
an attempt was made to identify each plant and plant location, and in-
clude it in one of the ten regions.  When production or capacity figures
for these plants were available, total production or capacity for each
region was computed,  and the U.S. emission estimate for that category
was distributed by region accordingly.   When production or capacity
figures were not available, the emission was distributed by  the number
of plants in each region.   If the number of plants was very  small or
                                  26

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                          TABLE 3
GEOGRAPHICAL DISTRIBUTION OF EMISSION SOURCE AND EMISSIONS
Emission Source
Inadvertent Sources
Iron and Steel
Open Hearth
Other
Coal Burning
Municipal Incineration
Oil Burning
Cement Production
Silver Industry Sources
Electrical Contacts
Primary Smelting
Totals
EPA Regions
1

3.7
1
1.4
23
0.3
0.7
3.8
16.6
2.5
18.0
0.6
1
1.2
5.8
0
0
13.0
2

3.7
1
2.0
33
2.4
5.7
5.5
24.2
4.1
29.1
7.7
13
2.6
12.5
0.2
2
28.2
3

65.7
18
6.7
111
9.3
21.8
4.1
17.7
2.1
15.0
16.8
28
2.4
11.5
0.4
4
107.5
4

7.3
2
2.4
39
9.1
21.1
2.7
11.8
1.3
9.6
15.8
27
3.2
15.7
0.2
2
42.0
5

62.3
17
8.8
146
17.6
41.3
5.5
24.0
1.1
7.6
17.9
30
4.4
21.6
0.4
4
118.0
6

7.3
2
1.2
20
0.6
1.4
0.8
3.5
0.5
3.7
15.8
27
2.0
10.0
1.1
11
29.3
7

0
0
0.3
5
1.7
4.1
0.3
1.4
0.1
0.9
11.8
20
1.1
5.5
0.3
3
15.6
8

7.3
2
0.1
2
1.4
3.3
0.1
0.3
0.3
1.8
5.3
9
0.5
2.7
0.7
7
15.7
9

11.0
3
1.7
29
0.3
0.7
0.1
0.5
1.6
11.6
11.2
19
2.3
11.3
1.0
10
29.2
10

0
0
0.4
7
0.1
0.3
0
0
0.4
2.7
4.1
7
0.7
3.2
.0.4
4
6.1
Totals

168
46
25
415
42.5
100
23
100
14
100
107
181
20.6
100
4.5
47
405
Units

(TPY)
(O.H. Plants
(TPY)
(All types
Plants)
(TPY)
(Percent
Coal)
(TPY)
(Percent
Capacity)
(TPY)
(Percent Oil)
(TPY)
(Plants)
(TPY)
(Percent
Population)
(TPY)
(Plants)
(TPY)
	
Reference


25

25

1

26

27

28

29

30,20


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  there was reason  to believe  that certain plants were larger or produced
  more emission, distributions were weighted accordingly.
      On  the other hand, when the estimated number of plants was greater
  than about 100, and the distribution of plants was not known, the re-
  gional breakdown was made on a different basis, such as population,
  geographical area, or shipments reported, as most appropriate for that
  category.  Whether the distribution was by plant size,  number of plants,
  or another statistic, the distribution is believed to be accurate to
 within 10 percent in most cases.
      The emissions distributions in Table 3 are made on  the following
 basis:
      Inadvertent Sources
        Iron and Steel Production:   Proportional to the  percentage of
                                    U.S.  plants in each  region
                     Coal Burning:   Proportional to coal shipments,  by
                                    state of  destination
          Municipal  Incineration:   Proportional to incinerator  capacity,
                                    by  state
                     Oil Burning:   Proportional to percentage of  re-
                                    sidual  oil  burned
                Cement  Production:   Proportional to number  of plants,
                                    by  state
     Silver Industry Sources
             Electrical  Contacts:   Proportional to population; i.e.,
                                    consumption of  equipment containing
                                    contacts
                Primary  Smelting:   Proportional  to number  of smelters
                                   of all types, by state
     The  largest emissions of silver in  1970 are estimated to have been
in Regions 3 and 5 (the east central portion of  the U.S.).  This con-
clusion is strongly influenced by the production of steel by the open
hearth process in these regions, and by  the concentration of silver re-
ported in open hearth fumes.   Since this concentration report was ap-
parently based on a single measurement of questionable reliability, it
is urged that further tests be made of open hearth fumes before these
estimates be widely adopted.

                                  28

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     Region 3 has the smallest geographical area in relation to the
emission of silver in that area (123,000 square miles), or in other
                                                                 -3
words, the greatest emission of silver per square mile (0.88 x 10
tons of silver per square mile-year).  Again, this is largely the re-
sult of the estimates of silver emissions from open hearth steel pro-
duction.
                                  29

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V.  NATURE OF EMISSIONS
    Practically no data describing the particulate containing silver
has been found.  It is, therefore, necessary to estimate the character-
istics of these particles based on the nature of silver and the processes
that generate the emissions.
    Table 4 lists some physical characteristics of silver, the most
important of which may be the boiling point, 2210°C.  Elemental silver,
because of its high boiling point, will not be emitted in significant
quantities as a vapor by processes operating at lower temperatures.
Simple silver salts (halides, sulphides) and oxides are the most proba-
ble forms of silver.

                                TABLE 4
                    PROPERTIES OF METALLIC SILVER*
Melting point:
Boiling point:
Density:
Atomic weight:
Heat of vaporization:
Hardness:
961°C
2210°C
Q
10.5 grams/cm
108 awu
60.7 kg-cal/g-atom
2.8 (standard minerology
scale)
*
Reference 30, Table 3-169. See also Table 3-1.
    Whether these compound forms are produced from elemental silver at
high temperatures, or the reverse, depends on the excess oxygen, sulphur,
chlorine, etc., and also on the presence of cyanide ions.
    Iron and steel producing processes are typically on the order of
1000°C, although in an electric furnace local temperatures must be ex-
tremely high due to the concentrated electric current.  Particulates
from these processes range in size from submicrometer to 5 micrometers.
                                  30

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There is no data to indicate the size of the silver-containing
particles within this range.  After release from a stack, any of
these particles are capable of traveling long distances before
settling to earth.
    Combustion processes (coal, oil, or incineration) tend to be at
lower temperatures.  The particulate produced, however, is somewhat
larger, ranging up to approximately 25 microns.  Although the largest
particles will settle out fairly quickly, smaller particles including
a small fraction of submicroraeter ones will remain airborne for long
periods.
    Since metallic silver is a relatively stable material, there is no
reason to expect significant chemical changes following emission.
Likewise there is no reason to expect unusual physical behavior of par-
ticles containing silver.  Dispersion, agglomeration, and settling may
be presumed to proceed at normal rates for these particles.
    Silver is not widely known as a toxic material.  In nitrate form
it is applied to the eyes of babies, and is used externally in cases of
severe burn.  In the vicinity of non-ferrous smelters where the toxic
effects of zinc and lead are well known, emissions of silver have not
been reported as problematic.  The extent to which silver, as an air
pollutant, might be considered hazardous  has not yet been established.
                                   31

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VI.  UPDATING OF EMISSIONS ESTIMATES
     The following recommendations are made for periodically updating
the estimates made in this study.
     A.  VERIFICATION OF CURRENT ESTIMATES
         1.  Because the estimated high emissions levels from open
hearth steel production significantly influence the conclusions of this
report, improved data for this emissions source should be obtained.
         2.  Within the silver industry, the emission of silver from
non-ferrous smelters and refineries constitutes the most concentrated
source, i.e., significant emissions from a small number of sources.
Therefore, within the industry, these sources offer the most obvious
opportunities for improved emission control.  Compilation of additional
data is recommended to supplement the estimated emissions data from
these sources.
     B.  PERIODIC REVIEW OF ESTIMATES
         1.  The Bureau of Mines' estimates for material flow, industry
practices, and trends provide the best estimates of the size of the
industry.
         2.  EPA activities are currently generating the best emissions
data and should be reviewed using:
             a.  Overall industry studies; e.g., Reference 31;
             b.  The Source Test Program in which specific in-
                 dividual plant emissions are measured.  This
                 information provides emission factors for spe-
                 cific examples of typical industry operations;
                 and also provides some analyses of the partic-
                 ulate, usually including trace metal content
                 and particle size;
             c.  NEDS (National Emissions Data System) is steadily
                 being enlarged and improved.  This system can
                 provide emission factors for specific plants
                 and plant operations,  the  type  of  particulate
                 control equipment in use, and the actual, or
                 estimated, control efficiency.  The system may
                 eventually be expanded to include description
                 of the emissions.
                                  32

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          3.    The silver industry should be consulted for its opinion and
suggestions regarding the most recently published estimates.   This  may be
best accomplished by interviewing the Silver Commodity Specialist,  Division
of Non-ferrous Metals, Bureau of Mines in Washington; or by interviewing
one or more of the principal companies in the industry.
          4.    The literature should be reviewed  using (a) industrial
views as published from time to time in Chemical Engineering,  for example,
and (b) environmental views as summarized in Pollution Abstracts, for example.
          5.    Individual companies or plants may be approached for opinions,
data, or cooperative tests of their own operations.   This is a difficult
approach to the obtaining of fresh information due to the natural reluctance
of the plants to discuss environmental problems.  However, data thus obtained
can have a relatively high degree of reliability.
          6.    State agencies in which specific plants are located may be
able to provide useful information and should be contacted.
                                       33

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 VII.  REFERENCES

 1.  West, J.  M., "Silver",  Minerals Yearbook,  1970,  Bureau of Mines,
     U. S. Dept. of Interior.

 2.  Survey of Current Business,  Bureau of Economic Analysis, U.  S. Dept.
     of Commerce.

 3.  Personal communication regarding the commodity  "Silver", Paul Zinner,
     U. S. Bureau of Mines,  Wash.,  D. C., November,  1972.

 4.  Orban, A. R.,  et. al.,  "Research on Control of Emissions from Bessemer
     Converters" J.A.P.C.A.. 11(3)  103-13, March 1961.

 5.  Hammond,  W. F., et al., "Steel Manufacturing Processes", in  Air Pollu-
     tion Engineering Manual,  999 AP-40, U.S.D.  H. E. W.,  1967.

 6.  Fairbridge, R. W., ed., The  Encyclopedia of Geochemistry and Environ-
     mental Sciences Series, Vol. IVA,  Van Nostrand Reinhold Co., N.Y.,  1972.

 7.  Varga, J.,  et. al., A Systems  Analysis Study of  the  Integrated  Iron and
     Steel Industry, Battelle Memorial Institute, Columbus,  Ohio, Report to
     N.A.P.C.A., U.S. Dept.  of Health,  Education and  Welfare, 15  May  1969.
     (PB 184 577)

 8.  Kearney,  A.T., and Co., Systems Analysis of Emissions and Emissions
     Control in the Iron Foundry  Industry, 3 Volumes, Chicago, 111.,  Report
     to E.P.A.,  Contract No. CPA  22-69-106, February  1971  (PB 198 348).
 9.  Abernathy,  R.F., and Gibson, F.H.,  Rare Elements in  Coal, U. S.  Bureau
     of Mines  circular No.  8163,  1963.
10.  Gerstle,  R.W., et al.,  "Air  Pollution Emissions  from  Coal-Fired  Power
     Plants",  Report No. 2,  J.A.P.C.A..  15(2)59-64, February.
11.  Cuffe, S.T., et. al.,  "Emissions from Coal-Fired Power Plants, A Compre-
     hensive Summary," N.A.P.C.A.,  U.S.  Dept. of H.E.W.,  1967 (PB 174  708).
12.  Walsh, R. T.,  "Gaseous and Liquid Fuels",  in Air Pollution Engineering
     Manual, 999 AP-40, U.S. D. H.E.W.,  1967.
13.  Smith, W. S.,  Atmospheric Emissions from Fuel Oil  Combustion,  999 AP-2,
     U.S. D. H.E.W., 1962.

14.  Anon., "Gold,  Silver Content Seen at $14 per Ton", Solid Wastes  Manage-
     ment, Refuse Removal Journal,  11^:78, May 1968.
15.  Wilson, E.B.,  and Akers,  D.J., "Chemical and Physical Characterization
     of Metropolitan Incinerator  Refuse and Fly Ash", Second Mineral  Waste
     Utilization Symposium,  Chicago, U.S. Bureau of Mines, March  1970.

16.  Ewell, T.W., and Piper, J.,  "Design of New Silver-Recovery  Incinerator",
     A.S.M.E., New York, Incinerator Div., Proc. National  Incinerator Conf.,
     Cincinnati, Ohio, 1970.
17.  Davis, W.E., National Inventory of Sources and  Emissions: Barium, Boron,
     Copper, and Zinc, Section III, Copper,, Report to EPA Office  of Air
     Programs, Contract No.  68-02-0100,  April,  1972.
                                       34

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18.   Ibid.,  Section V,  Zinc,  May 1972.

19.   Butts,  A.,  and Coxe,  C.D.,  Silver:   Economics,  Metallurgy,  and Use,
     Van Nostrand,  1967.

20.   Charles River  Associates,  Inc.,  Economic Analysis of the Silver Industry,
     Report  to the  General Services Admin.,  Contract No.  GS-OO-DS-(P)-85005,
     Sept.  1969.   (PB 191  464)

21.   Levy,  A., et al.,  A Field Investigation of Emissions From Fuel Oil
     Combustion for Space  Heating, report by Battelle Institute, Columbus,
     Ohio,  to American Petroleum Institute,  API Proj. SS-5, 1 Nov. 1971.

22.   EPA Source Test Reports.  From analysis of selected  test reports,
     emission factors and/or  particulate analysis data were obtained to
     supplement the data found in the literature.

23.   Lehmden, D.J., Jungers,  R.H., and Lee,  R.E., The Determination of  Trace
     Elements in Coal,  Fly Ash,  Fuel  Oil, and Gasoline, Part I,  presented
     at the  American Chemical Soc. Mtg., Dallas, Texas, April 1973.

24.   National Emissions Data  System (NEDS) information, based on reports
     made by individual plants.   Only reliability code (1) and (2) data
     is used in the present study.  Information furnished by EPA.

25.   American Iron  and Steel  Institute,  "Iron and Steel Producing and
     Finishing Works of the U.S.", in Directory of I & S  Works of the
     U.S. and Canada, 1970.

26.   Arthur D. Little,  Inc.,  Cambridge,  Mass., Systems Study of Air Pol-
     lution from Municipal Incinerators, 1970.

27.   American Petroleum Institute, "Total Sales of Residual Fuel Oils (Ail
     Uses)  by States, 1934-1969", Petroleum Facts and Figures, 1971.

28.   Pit and Quarry Publications, Inc.,  Chicago, 111., Portland Cement
     Plants, (map), 1969.

29.   Bureau of Census,  U.S. Dept. of  Commerce, Statistical Abstracts of the
     U.S.

30.   Perry's Chemical Engineer Handbook, 4th Edition, McGraw-Hill, New
     York,  1963.

31.   A.G. McKee and Co., San  Francisco,  Calif., Systems Study for Control
     of Emissions,  Primary Non-ferrous Smelting Industry, 1969.

32.   Vandegrift, A.E.,  et  al., Particulate Pollutant System Study, Vol. Ill,
     Handbook of Emission Properties, EPA Contract No. CPA 22-69-104.
                                      35

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                                     TECHNICAL REPORT DATA
                              (Please read Instructions on the reverse before completing)
 * 1 PKPORT NO.

      EPA-45n/3-74-011
               3. RECIPIENT'S ACCESSION-NO.
 p 1. ri TLE AND SUBTITLE

      National  Emissions  Inventory of  Sources and
      Emissions of Silver
               5. REPORT DATE
                  May 1973
               6. PERFORMING ORGANIZATION CODE
   AUTHOR(S)
                                                              8. PERFORMING ORGANIZATION REPORT NO.
     ^FORMING ORGANIZATION NAME AND ADDRESS
      GCA Corporation
      GCA Technology Division
      Bedford,  Massachusetts 01730
               10. PROGRAM ELEMENT NO.
                  2AE132
               11. CONTRACT/GRANT NO.
                                                                 68-02-0601
  12. SPONSORING AGENCY NAME AND ADDRESS
      Environmental  Protection  Agency
      Research Triangle Park, N.  C.  27711
               13. TYPE OF REPORT AND PERIOD COVERED
                 Final
               14. SPONSORING AGENCY CODE
 15. SUPPLEMENTARY NOTES
           A national  inventory of the sources  and emissions  of the element silver
     was  conducted.   All  major sources of silver-containing  emissions were iden-
     tified and their silver emissions into the  atmosphere estimated.  Also,  a
     method for updating  the results of the study every two  years was recommended.
                                 KEY WORDS AND DOCUMENT ANALYSIS
                   DESCRIPTORS
     Silver
     Air Pollution
     Emission
     Inventories
     Sources
                                                b.lDENTIFIERS/OPEN ENDED TERMS  C.  COS AT I Field/Group
             STATEMENT
                                                19. SECURITY CLASS (ThisReport)
                            21. NO. OF PAGES
     Release Unlimited
20. SECURITY CLASS (Thispage)

      Unclassified
                                                                           22. PRICE
EPA Form 2220-1 (9-73)
                                               36

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Region 5, Ln^rv

77 \Vc3tJac1  :
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 inuaU, iL  ^ *j•-'--•- -

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