United States
Environmental Protection
Agency
Office of Air Quality
Planning and Standards
Research Triangle Park NC 2771 1
EPA-450/4-80-007^3
April 1980
    X
Air
Engineering Reference
Manual for Coding  NEDS
and EIS/P&R Forms
Volume III: Compendia
of Processes

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                                EPA-450/4-80-007
 Engineering Reference Manual for
Coding  NEDS and EIS/P&R Forms

 Volume III: Compendia of Processes
                National Air Data Branch
            Monitoring and Data Analysis Division
          U.S. ENVIRONMENTAL PROTECTION AGENCY
             Office of Air, Noise, and Radiation
           Office of Air Quality Planning and Standards
          Research Triangle Park, North Carolina 27711

                   April 1980

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This report is issued by the Environmental Protection Agency to report technical data of
interest to a limited number of readers.  Copies are available - in limited quantities - from
the Library Services Office (MD-35),  U.S. Environmental Protection Agency, Research
Triangle Park, North Carolina 27711;  or, for a fee, from the National Technical Infor-
mation Service, 5285 Port Royal Road, Springfield, Virginia 22161.
                        Publication No.  EPA-450/4-80-007
                                        11

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    ENGINEERING REFERENCE  MANUAL  FOR

     CODING NEDS AND EIS/P&R  FORMS
     Volume III:   Compendia  of Processes
          National  Air Data Branch
    Monitoring and  Data Analysis  Division
    U.S. ENVIRONMENTAL PROTECTION AGENCY
    Office of Air, Noise, and Radiation
Office of Air Quality Planning and Standards
Research Triangle Park, North Carolina  27711

                 April 1980

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                                CONTENTS
7.      METALLURGICAL INDUSTRY                                         ,
        7.6     PRIMARY LEAD SMELTING	      ;•?"
        7.7     PRIMARY ZINC SMELTING	      '•l'\
        7.8     SECONDARY ALUMINUM OPERATIONS  .  .  ... .  •  •      '•«-'
        7.9     SECONDARY COPPER SMELTING AND ALLOYING  .  .  .      7.9-1
        7.10    GRAY IRON FOUNDRIES	     '•'""{
        7.11    SECONDARY LEAD SMELTING	     '•  ''
        7.13    STEEL FOUNDRIES  	     /'IJ"'
8.      MINERAL PRODUCTS INDUSTRY                                     .  .
        8.1     ASPHALTIC CONCRETE PLANTS  	      °-'~
        8.3     BRICK MANUFACTURING  	      °-;f
        8.6     PORTLAND CEMENT  MANUFACTURING  	      8.6-1
        8.9     COAL CLEANING	      B:;rJ
        8.15    LIME MANUFACTURING	;  •  ••  •  •     J-Jj"'
        8.19    SAND AND GRAVEL  QUARRYING  AND  PROCESSING   .  .     8.19-1
        8.20    STONE QUARRYING  AND  PROCESSING	     b./JU-i
10      WOOD  PRODUCTS  INDUSTRY                                      ,  7 ,
         10.1.2 SULFATE (KRAFT)  WOOD PULPING  	    In  Ml

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                    7.6  PRIMARY LEAD SMELTING




                   1-4
PROCESS DESCRIPTION



     Much of the lead produced in the United States is used in



lead batteri^o and in gasoline additives.  Vvith stricter restric-



tions on lead emissions, however, its use in lead additives is



declining.  Primary lead smelting is the process of separating



lead metal from ores, the most common of which is the sulfide



galena  (PbS).  Lead ores are commonly found with zinc ores,



together with smaller amounts of other metals such as iron,



copper, gold, silver, arsenic, and antimony.  Except for Missouri



deposits, which contain 75 percent PbS,  lead content of most ores



averages 3 to 8 percent.  Figure 7.6-1 is a flow diagram of the



smelting process.



     Most lead smelters are located near the mines, from which



ore or  ore concentrates are transported  by truck or rail.  More



than 80 percent of the  lead produced in  the United States  is from



the rich Missouri deposits, which do not require beneficiation



before  smelting.  Other ores must be concentrated.  This is



accomplished at the mines by first crushing and pulverizing the



ores and then utilizing a beneficiation  step  such  as flotation,



magnetic separation,  or a similar physical operation.   Flotation



involves slurrying with chemicals that float  lead-bearing  mate-



rials  and allow waste to sink.   The  floating  froth is skimmed and


                               7.6-1

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                     RAW MATERIAL
                      TRANSFER^   J
RECYCLE
OUST S
, SINTER
A T r^
f PART (^-_f
^V
3-OymMZ
RAH MATERIAL
PILES
0
VART T> TPART./T H?sofl PLANT *
" N 043 (95) S0?
>' "' , 	 1 CONTROL


3-03-010-04 3-03-010-14 BAGHOUSE 017 (99) CONTROL
ORE CRUSHING MIXING ESP 01° (991' 	 i 1
\PART- 5 ' PART/- , REC
J ^ S^
?
i
CONTROL BAGHOUSE 017 (99) ^pAR1 "

^XS. SO-, . i 3-03-OiQ- 1^

( ) sas!.f C 3 " s«
                              3-03-010-05
                            MATERIALS HANDLING
III POUTO5 Kl SCC IMIT
                                                 Figure  7.6-1.  Primary  Lead Smelting

                                                                    7.6-2

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dried to about 60 percent moisture, at which point it contains 45
to 60 percent lead and 10 to 30 percent sulfur and often enough
zinc to make its recovery economical.
     The three major steps at a lead smelter are sintering,
reduction, and refining.  The purposes of sintering are to con-
vert metal sulfides to oxides by driving off sulfur, to drive off
part of the volatile impurity metals such as arsenic and anti-
mony, and to produce a material physically strong enough to be
treated in the blast furnace.  The blast furnace reduces lead
oxide to molten lead; refining removes impurities trapped in the
lead during reduction.
     Charges of raw materials to the blast furnace include ore
concentrates, coke, and fluxing agents such as limestone, silica
sand, and iron ore.  Proportioned amounts of concentrates, coke
breeze  (fines), and fluxing agents are first ground in a hammer
mill, mixed, and then rolled into pellets, which are fed to a
sinter machine.  Sintering is performed on a moving conveyor of
perforated metal plates.  Two types of machine are used, downdraft
and updraft.  In the former, a layer of pellets about 5 in. deep
is spread on the moving belt, and the top is ignited by an oil or
gas burner.  Air is drawn down through the bed and the burning
zone deepens as the bed travels on the conveyor.  In an updraft
machine, a 1-in. layer of pellets is spread and ignited and
another 10- to 14-in. layer is added to it.  Air is forced up
through the bed, and the burning zone rises.  Coke and sulfur
provide the necessary heat, and no extra fuel is needed.  The
sulfur content of the discharged sinter is about 1 to 2 percent.
                              7.6-3

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     Essentially all updraft sinter machines have two separate
exhaust collection systems, one at the feed (ignition)  end and
one at the discharge (tail) end.  This separation enables collec-
tion of a high-SO_, low-volume gas flow at the feed end and a
low-SO , high-volume gas flow at the discharge end, where oxida-
tion has generally ceased.  The concentrated S02 flow is usually
used for sulfuric acid manufacture.
     The sintered cake falls into a breaker  (crusher), which is
followed by an additional  crusher and a screen.  Oversize mate-
rial from screening is conveyed to blast furnace charge bins,
whereas undersize, unsuitable for charging, is crushed and  cooled
and returned to the sinter feed bins.  Sinter, coke, and  addi-
tional  fluxing agents are  charged into the  top of  a  blast furnace,
a  water-cooled column about 5 ft wide, 12  to  20  ft long,  and  16
to 24  ft high.  Dust from  particulate collection systems  may  be
added.  Air is blown into  the bottom  of  the furnace, oxidizing
the coke to carbon monoxide.  As  the  charge moves  downward
through the furnace, contact with coke and carbon  monoxide
reduces the lead  oxide  in the  sinter  to  molten lead.  A slag  of
zinc,  iron, and  calcium silicates,  which also contains copper,
 some lead,  and other metals, floats on  the molten lead.   Slag and
 lead are either tapped (withdrawn)  separately or the molten
material from the furnace is first discharged into an adjacent
 box-shaped settler,  from which the slag overflows into a slag
 granulator.   Zinc is often recovered from the slag in a  slag-
 fuming furnace.
                               7.6-4

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     The first step in refining the molten lead,  called bullion,
is dressing.   The molten metal is agitated in a cast-iron kettle;
sodium carbonate, ammonium sulfate, and sulfur are often added.
The metal is cooled to about 700°F, and copper and other impur-
ities that are not soluble in the lead at that temperature rise
to the surface and are skimmed off.  The dross is processed in a
reverberatory furnace to recover any lead or copper.
     The drossed bullion still contains impurities; these are
removed by several refining steps, not all of which may be
carried out at a lead smelter.  About 1 to 2 percent of the
bullion is composed of zinc, arsenic, antimony, tin, gold, and
silver.
     The next step in refining is  softening, which  is  carried  out
in a kettle or reverberatory furnace.  Arsenic, antimony, and  tin
 (which  harden lead) are  removed  as an oxide  scum  by agitation  and
air blowing.  Caustic soda  and sodium nitrate  are added  in kettle
softening.  In the third step, enough  zinc  is  added to the
bullion in a kettle to  float up  the gold  in a  crust, which  is
 skimmed off.  More zinc  is  added,  and  a  second crust containing
 silver  is also skimmed  off.   Some copper  and other metals also
 accumulate  in the  crusts.   The zinc remaining  in  the molten  lead
 is now  recovered,  usually by  vacuum distillation.  Because  it has
 a lower boiling  point than  lead, it can be withdrawn in a vacuum
 and condensed.   The  dezinced  lead may be treated with  caustic
 soda before being cast into pigs  (about 100 Ib)  or ingots (about
 2000 Ib).
                               7.6-5

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EMISSIONS1'5'6



     Particulate and SO2 are the major pollutants from lead



smelters.  The S02 is emitted mainly from the sintering operation



and a relatively small amount comes from the blast furnace.



Emission sources are identified in Figure 7.6-1.  Emission factors,



listed on the process flow diagram, are given in AP-42.   Average



emission rates for other sources were obtained from other docu-



ments and are mentioned in the following source descriptions:



     Raw material handling operations cause fugitive particulate



emissions.  Emissions from unloading of limestone, silica, lead



ore concentrate, and iron ore range from 0.03 to 0.4 Ib/ton of



material, whereas those from coke unloading amount to about 0.4



Ib/ton of coke.   Emissions from loading these materials onto



piles, from vehicular traffic, loading out, and wind erosion are



estimated to be 0.3 Ib/ton of material.  Emissions from handling/



conveying and transfer of these materials are as follows:  lime-



stone, 0.2 Ib/ton; silica, 0.3 Ib/ton; ore concentrate, 1.64 to



5.0 Ib/ton; iron ore, 2.0 Ib/ton; and coke, 0.13 to 3.4 Ib/ton.



     Raw material crushing/pulverizing and mixing operations are



also sources of fugitive emissions, which are controlled at  some



plants.  Similarly, emissions from discharge of sinter onto  the



breaker are also fugitive unless confined and vented.  Reference



6 estimates particulate emissions of  0.55 to 2.45 Ib/ton of



sinter from sinter machine discharge  and sinter crushing and



screening.  Emissions from subsequent sinter transfer operations



are estimated to be 0.25 to 0.75 Ib/ton of sinter.   Sinter  that
                               7.6-6

-------
is not suitable for charging to the blast furnace is returned to



sinter feed bins; emissions from sinter return handling are



estimated to be 4.5 to 13.5 Ib/ton of sinter.



     The sintering operation results in emissions of particulates



and sulfur dioxide.  The exhaust from a single-stream sintering



machine, whether upflow or downflow, contains about 2 percent



sulfur dioxide and has an emission factor of 423 Ib/ton of con-



centrated ore.  The single-stream sintering emission factor for



particulates is 164 Ib/ton of concentrated ore.  In a dual-stream



sintering machine, the strong stream (feed end) contains about 4



to 7 percent SO  and the weak stream (discharge end), approxi-



mately 0.5 percent SO .  Particulate emissions from leakage



around the sinter machine range from 0.25 to 1.1 Ib/ton of



sinter.




     The blast furnace is another major source of particulate and



SO  emissions.  Fugitive particulate emissions from charging and



tapping of the blast furnace are 0.08 to 0.23 Ib/ton of lead



product.   Particulate emissions from the pouring of lead into



the dross kettle are about 0.93 Ib/ton of lead product, and those



from slag pouring and cooling are 0.47 Ib/ton of lead.



     Slag fuming furnaces are usually hooded to capture partic-



ulate emissions.  They range from 2.3 to 6.9 Ib/ton of lead



produced.   Emissions from the dressing kettle amount to 0.24 to



0.72 Ib/ton of lead product and are often vented to the blast



furnace control system.
                              7.6-7

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     Emissions from the dross reverberatory furnace are vented



through a control device.   Fugitive particulate emissions due to



leakage around the furnace range from 1.5 to 4.5 Ib/ton of lead




produced.



     The softening kettle is generally hooded and vented.  Par-



ticulate emissions from the gold and silver recovery kettles and



additional refining are fugitive.  Reference 6 reports emissions




of 0.9 to 2.7 Ib/ton of lead product from a building that houses



lead refining operations.  No data are available on emissions



from individual operations.  Particulate emissions from  lead



casting  are reported to be 0.43 to 1.30 Ib/ton of lead produced.






CONTROL  PRACTICES3'5'6



     Raw material handling operations are usually uncontrolled,




although some plants use water  sprays to reduce emissions.



     High-SO  concentration  streams  from dual-stream  sinter




machines are usually cleaned of particulate by  a baghouse or



electrostatic precipitator  (ESP)  and conducted  to  a single-stage



sulfuric acid plant.   Low-concentration  streams are usually



combined with the  off-gas  from  the blast furnace,  cleaned of



particulate by  a baghouse  or ESP, and discharged to the atmos-



phere  without SO  control.   Emissions from single-stream sinter



machines are usually cleaned of particulate as described above,




but SO  is not  controlled.



      Emissions  from sinter handling operations are usually not



 controlled.  Sometimes they are vented  through the sinter machine




 control system or through a separate baghouse.




                              7.6-8

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      The blast furnace is vented through a baghouse or ESP.   Some

 plants vent emissions from charging and tapping through the

 furnace control system.   Others either do not control them,  or

 they vent them through a separate baghouse.

      Exhaust gases from reverberatory furnaces and dressing

 kettles are often combined with those from the blast furnace and

 vented through a baghouse.   Emissions from other refining  oper-

 ations including vacuum dezincing are generally not controlled.

 Some plants vent lead casting  emissions through a baghouse.
 CODING NEDS  FORMS7"9


      The  emissions  sources  and  the pollutants
 Source

 Raw material unloading

 Raw material piles

 Raw material transfer

 Materials handling

 Ore crushing

 Mixing

 Sintering, single stream

 Sintering, feed end

 Sintering, discharge end
     SCC

 3-03-010-11

 3-03-010-12


 3-03-010-13

 3-03-010-05

 3-03-010-04

 3-03-010-14

 3-03-010-01

 3-03-010-06

 3-03-010-07
they emit are:

      Pollutant(s)
Sinter discharge, crushing,   3-03-010-15
 screening

Sinter transfer

Sinter return handling

Blast furnace, off-gas

Blast furnace, charging
3-03-010-16

3-03-010-17

3-03-010-02

3-03-010-18

7.6-9
      Particulates

      Particulates

      Particulates

      Particulates

      Particulates

      Particulates

      Particulates,  SO?

      Particulates,  SO?

      Particulates,  SO_

      Particulates



      Particulates

      Particulates

      Particulates,  SO

      Particulates

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Source
Blast furnace, tapping

Lead pouring

Slag pouring

Slag fuming furnace

(In-process fuel-coal)

Dressing

Dross reverberatory furnace   3-03-010-03
    SCC

3-03-010-19

3-03-010-20

3-03-010-21

3-03-070-08

(3-90-002-99)

(3-03-010-09)
Pollutant(s)

Particulates

Particulates

Particulates

Particulates,
combustion products


Particulates

Particulates,
combustion products
 (In-process fuel)
  Distillate oil
  Natural gas

 Softening

 Lead  refining

 Lead  casting
(3-90-005-99)
(3-90-006-99)

 3-03-010-24

 3-03-010-22

 3-03-010-23
 Particulates

 Particulates
      Standard NEDS  forms for each of  the sources,  Figures 7.6-2

 through 7.6-24,  show entries for the  SCC's and other codes.

 Entries in the data fields give information common to lead smelt-

 ing plants.  Information pertinent to coding the source is

 entered on the margins of the forms and above or below applicable

 data fields.  Entries for control equipment codes, other optional

 codes, emission factors, and required comments minimize the need

 to refer to the code lists.

      Typical data values for operating parameters, control equip-

 ment efficiencies, and other source information are  shown on the

 form  (or in the text) only  to  aid  in rapid, approximate  checks of

 data  submitted by  the plant in a permit  application  or  similar


                               7.6-10

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 report.  Data entered in EIS/P&R and NEDS must be actual values
 specific to and reported by the plant, rather than typical values
 Contact the plant to validate or correct questionable data and to
 obtain unreported information.  See Part 1 of this manual for
 general coding instructions.
      For fugitive particulate emission sources, where there is no
 control device or where liquid sprays are used, enter zeros in
 the stack heighL and diameter fields, 77 in the temperature
 field, and zeros in the common stack field.  Where liquid sprays
 are used,  enter 061 or 062  as a control equipment code.   In the
 comments field on Card 6 identify other equipment used to reduce
 emissions.
      Figures  7.6-2  through  7.6-4  show standard NEDS  forms for raw
 material unloading,  stockpiling,  and transfer operations.   The
 emission source  labeled  "raw material piles"  includes loading
 onto  piles, wind  effects while the materials  are  stored,  and
 retrieval activities.  Raw  material  transfer  operations not
 included under unloading, storage piles,  crushing and pulver-
 izing,  and mixing are  grouped  under  the emissions source  labeled
 "raw material transfer."
     Emissions data on these sources  are  scarce.   When a plant
 furnishes emissions data for these sources, code  the  values
 given.  Where detailed emissions data for each of  the raw mate-
 rials are available, code a form for each and identify the
material in the comments field.  Enter "Emission Estimates Given
by Plant" in the comments field on Card 7.  Where emission rates

                               7.6-11

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for individual operations are unavailable,  code these sources on
one form under Materials Handling,  as shown in Figure 7.6-5.
This source covers all the operations associated with raw mate-
rial handling, including the mixing operation but excluding
crushing/pulverizing operations.
     Emissions from crushing/pulverizing are usually not con-
trolled.  Code these operations on one form as shown in Figure
7.6-6.  Figure 7.6-7 shows a standard NEDS form for the mixing
operation.
     Combustion gases from the sinter machine are captured by one
or two exhaust systems.  Where there are two systems, code a form
for each.  When dual-stream capture systems are used, the feed-
end exhaust gases are first vented to particulate controls and
then to a sulfuric acid plant for S02 control.  Since the gases
are vented to a sulfuric acid plant, the associated emissions will
be accounted  for on the NEDS forms for the acid plant.  Therefore,
on the  feed-end NEDS  form, enter zeros for emission estimates and
allowable emissions,  and fives  for the estimation method.  The
five denotes  a special  emission factor,  in this case, emissions
are vented to another plant.  Leave  the  stack  data  fields  blank.
Code the  sulfuric acid  plant as described  in  the  compendium  on
sulfuric  acid manufacturing.  Three  standard  NEDS  forms for  a
sinter  machine are  shown  in  Figures  7.6-8,  9,  and  10.   When
coding  a  form, enter  the  appropriate SCC in  the SCC field.
      Some plants  vent emissions from sinter  machine discharge,
crushing,  and screening through a  baghouse.   Unless confined,
these  emissions  are fugitive.   Emissions from sinter transfer
                               7.6-12

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 operations are usually not controlled.  Figures 7.6-11 and


 7.6-12 show standard NEDS forms for these two sources.  Sinter


 that is unsuitable for changing is returned to the raw material


 mixing operation.   Sinter return operations could cause signif-


 icant fugitive particulate emissions.   Figure 7.6-13 shows a


 standard NEDS form for sinter return handling.


      Exhaust gases from the blast furnace are vented through a


 particulate control device,  but usually not through an SO
                                                          &

 control system.  Figure 7.6-14 shows a standard NEDS form for the


 blast furnace.   The sintering discharge end,  the blast furnace,


 the  slag fuming  furnace,  and the dressing kettles are usually


 vented to a common control system.   Where this  is so,  the sources


 must be assigned consecutive point  ID  numbers and Columns 56


 through 59  of Card 2  filled  with the lowest and  highest point ID


 numbers for the  four  sources.


      Some plants vent  emissions  from blast  furnace  charging  and


 tapping through  a  baghouse.   At  other  plants, these  emissions are


 not  controlled.  Figures  7.6-15  and  7.6-16 show  standard  NEDS


 forms  for these  two sources.


     Emissions that occur when molten  lead is poured from the


 kettle  into the  dross kettle  are sometimes partially controlled


 by venting them  through a baghouse.  Similarly, some plants


 control emissions from slag pouring.  Figures 7.6-17 and 7.6-18


 show standard NEDS forms for these two sources.


     Emissions from the slag fuming furnace are usually vented


through a baghouse  often through the blast furnace control


system, as are emissions from the dressing kettle and the dross


                              7.6-13

-------
reverberatory furnace.   Standard NEDS forms for these three



sources are shown in Figures 7.6-19 through 7.6-21.



     A standard NEDS form for softening is shown in Figure 7.6-



22.  Desilverizing, degolding, and additional lead refining



treatment operations are grouped here under "lead refining."



Figure 7.6-23 shows a standard NEDS form for lead refining.  In



coding these operations, identify the operations grouped in the



comments field on Cards 6 and 7.  Where one of these operations



is controlled, code that operation separately and identify the



operation in the comments field.  Enter the emission data furnished




by the plant.



     Some plants vent emissions from the lead casting building



through a baghouse.  Figure 7.6-23 shows a standard NEDS form for




lead casting.




CODING EIS/P&L FORMS



     The EEC's for  use  in EIS/P&R  forms are:



          Source                        BEC



Raw material  unloading                  700



Raw material  piles                      700



Raw material  transfer                   700



Materials handling                     700



Ore crushing                            650




Mixing                                  804



Sintering  (all)                         226



Sinter  discharge,  crushing,  screening  660



Sinter  transfer                         700



Sinter  return handling                  700




                               7.6-14

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     Source




Blast furnace (all)



Lead pouring



Slag pouring



Slag fuming furnace



Drossing



Dross reverberatory furnace



Lead refining



Lead casting
BEG



No code*



No code*



No code*



No code*



No code*



9f 9



No code*



No code*
*As of September 1978.
                             7.6-15

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       Figure 7.6-2.  Standard NEDS form for primary lead  smelting -  raw material unloading.
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-------
      Figure 7.6-3.  Standard NEDS form for lead smelting - raw material piles.
I
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Pljni 10
Si t. County -»OCR N...,,l.,.
1 23451 7 1 9 10 11 12 13
- -o
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3332
O "? Boiler Owiqn c "
5 S Capacity Primary S<£
^ £ 106 BTU/hf Pan £
16 7 16 19 2C ? '2 2 '4 2S 26 2
1 1 1 1 1 Toi 1 1 lolol
°i ANNUAL THHUPUT NO
o* °>E
^ 3 Dec- Mar. June Scot- S
> tc feb May Au>| Nov
o|
;l Pan.cuaie
16 £7 18 9 20 2 22 2 24 25 6 2?
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i 3 5
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16 17 18 19 20 2 22 23 21 25 26 27
RAW MATERIAL __ 3 0 1 0.1 .0 H __
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Point 3 5
ID ^ I 1 II III IV C
U 15 16 17 IS 19 20 21 22 23 2» 25 26 I

NATIONAL EMISSIONS DATA SYSTEM (NEDS)
ENVIRONMENTAL PROTECTION AGENCY
OFFICE OF AIR PROGRAMS
Establishment Name and Address
'8|29|30|3l|32l33l34|35|36l37|3S|39|<0|4l|l2|43|44|4S|46|47|4S|49|SO|51|52|53|S4|55
OHOINATES STACK DATA
Vertical , f »™ H"9hl
km Heigh 111) Oum III Templ"FI Flo.. R.ile [l|J/min> III no stack ll
28 21 10 31 3? 33 34 35 36 37 38 39 40 4 42 43 44 45 46 4 4) 19 50|S1 52 53 54 5'
CONTROL > EQUIPMENT ^ >
I~ I. I.j |0 EST1
Pum.ry §8 Prim,-, |° P,,m.,., 5 i! Pnr-a- , |S
SOT *- NO, £ HC y, CO $ Pa'i
28 29 30 31 3: 33 34 35 36 3; 38 39 40 7 12 43 44 45 4S 4 4H 1} 50 SI 52 53 54 55
olololoiolololololololololololololololololololoiol 1 1
,'aT*Ujc EMISSION ESTIMATES nons.yeatl
| ? Paniculate SO, NO, HC
2: 2' i: 31 :2 33 4 :5 36 ! 3! 39 40 41 42 4: 11 15 46 : 15 41 50 5! 52 S3 54 55
M 1 II 1 1 1 1 1 II 1 II 1 |ol 1 1 it 1 lol II I
ALLOWABLE EMISSIONS llonsiyearl -""scHT
a
O? NO, HC CO £ Voai
28 25 30 31 3' 33 4 )5 31 3! 3! :9 4 41 42 4 41 45 4S 17 K 11 50 5 52 53 54 5
0 0 0 _,_ 0 	
An™* SCC UNIT - TONS OF RAW MATERIAL
uel Process Hou'l. =r - 3 "• ^ Fui;l
UI..HVIM.- Vj.imurr Oesn" ^^H *" := »' •< Con'ent
.-. 	 P.>" R.I- u U lt>>:' =Tu '"-
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DMMENTS
23 21 30 31 K 33 34 35 36 3: 38 39 10 41 12 13 4; J5 :» 1 :i ;9 50 51 52 V3_ 51 _

POINT SOURCE FORM APPROVED
Input Fotm OMH NO IMH009S
Name of Perion
4
Contact • Pe-sonal C
56 57 5! 59 60J.I 62 S3 64 65 S6 67 68 69 70 71 72 73 7
P«;"" ^-0000 IF NO COMMON STACK
"TaTk0^ xxxx POINT ID'S IF COMM0'
56|5)|5al59 (0|6l|62|63|64|65|6S|67|68|S9|70|7l|7r|73|
MATED CONTROL EFFICIENCY (M
SOi NO, HC CO
56 5! 58 59 50 61 62 63 64 55 55 67 68 69 70 71 2 73
.0. 0 _£ ^jO
ESTIMATION
METHOD
5 C? O u O *• Space
; CO S ° ° I u H.j,
56 5~ Tj 1? 6C 61 62 63 64 5 66 67163 69 70 71 72 73
0 00000 _, 0
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UPDATE a.
56 jY S8J59 6CJ61 62(63 6-U5J66 s7J68 69 70 71 72 73
Comments tsi C
5 56 57 53 59 iO j K S3 64 S5 66 67 51 S9 70 71 72 73
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_ _ -. — -

-------
   Figure 7.6-4.  Standard NEDS form for primary lead smelting  -  raw  material  transfer.
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NATIONAL EMISSIONS DATA SYSTEM (NEDS) 'OINT s
ENVIRONMENTAL PROTECTION AGENCY "*""
OFFICE OF AIR PROGRAMS Nameol Person
Completing Form
Establishment Name and Address
22

23

if
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22

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Capacity
106 8TU/hr
6 19

Dec-
Feb
8 19

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21

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May
20

21

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0
23

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25

26

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24

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June
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28

29

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32

33

34

35

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33
34
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36

37

38

39

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37

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40

41

42

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44

45

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1 . I rv | . 1
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24

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8 19

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61 62


63

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65

66

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70

71

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75

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•^ XXXX POINT ID'S IF COMMON STACK
60

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62

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-------
Figure  7.6-5.     Standard  NEDS  form  for  primary   lead  smelting   -  materials   handling.
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                                                         NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                           ENVIRONMENTAL PROTECTION AGENCY
                                                                OFFICE OF AIR PROGRAMS
                                                                                                             POINT JURCE
                                                                                                              Input cotm
                                                Name o( Perton
                                                Completmg Fo"n
                                                                             FORM APPROVED
                                                                             OMB NO 158 R009S
                                                                             Dai.	
                         f X

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      MATERIALS HANDLING
                                20 21
                              u 20 21
                            3l3l3l2|o
                                                                       t Name and Add-cji
                                    11 21 21 25 28 11 .'8 21 30 ]l 32 33 34 35 3S 3? 3J 39 1 43 »\>i >t » >i 49
                              oiler Dmqn
                              Cdcaott
                              10^ BTU'hr
                             S 19 2C 21 22 2) 24 ?i
                                          UTM COOHDINAfES
                                        2t 25 2S 27
                                                28 29 10 31 32
                                                                    38 39
                                                                        STACK DATA
                                                                                            50 51 52 53 M
                                                                                4) 45 46 41 4) 49
                                    r'vme tieiqht
                                   1 "ryci"i
                                   50| 51 52 S3 54
                                                              CONTROL   EQUIPMENT
                             > ANNUAL THHUPUT
                             Dec Mo-  Jur^ Seoi
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                                                                                                                    a H (4 85 « 47 U
                                                                                                                                              75 76 l][lt
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                                                                                                         co^oni^-  xxxx poINT ID,S IF COMMON STACK ;
                                                                                                    ESTIMATED CONTROL EFFICIENCY (M
                                                                                                  53 5«I55
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                                                                                                              59 SO 61
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                                                      3I 3: '-3 14 35 5} !
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                                                   ALLOV\AoLb E
                              19 20 21 22 23 24
                              19 20
                                        24 25
                                            26 21 28 29 30|!1
                                                        32 33 34 15 >.S 31 U
                                                                      39 40 41 42 43 44 45
                                                An,,UJ,SCC UNIT - TONS  LEAD  PRODUCED
                                              Fuel  Pfxr,.^        Mou'1,
                                               Sol.,10 INC.-
                                                                                                  53 54 55 % 57
                                                                                                        56 5!
                                                                                                              59 60 61 62 63
                                                                                                             COMPLIANCE
                                                                                                               STATUS
                                                                                                               UPDATE
                                                                                                            58 59
                                                                                                                62 61
                                                                    ESTIMATION
                                                                     METHOD
                                                                                                                              (7 63 69  70
                                                                                                                          0   0000
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                                                                      CONTROL REGULATIONS

                                                                   Rc^ I      R«>i 2  I  Reg 3
                                                                                                                          65 66 67 6i
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                                                          33 34 35 ii :  i
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                                            25 27 23 21 30 31 32 33 34 35 ;s
                                                                      !9 40 41 42 43 4
                                                                                            50 51 52 S3 54 5: 5c 5! 5j 59 SO 61 62 6! 6:

-------
Figure 7.6-6.  Standard NEDS form for primary lead smelting - ore crushing.
PljMI 10
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NATIONAL EMISSIONS DATA SYSTEM (NEDS) -
ENVIRONMENTAL PROTECTION AGENCY
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En b .sumfi Name jnd Add c«
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-------
            Figure  7.6-7.   Standard NEDS form for primary lead smelting -  mixing,
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GLOSSARY


Beneficiation - The processing of ores for smelting by flotation
     or magnetic separation to remove waste rock.

Bullion - A semirefined alloy containing sufficient precious
     metal to make recovery profitable.

Dross - An oxide-sulfide scum of impurities on molten lead.

Dressing - The process of forming and removing dross.

Gangue - A waste rock or slag material remaining after most of
     the metal values have been removed.

Matte - A floating layer, mostly of copper and iron sulfide.

Reverberatory furnace - A furnace in which a flame reflects
      (reverberates) from the furnace roof onto the charge.

Sintering - A process that agglomerates  fine ore particles into
     large pieces and removes most of the sulfur.

Slag - Waste material from blast and reverberatory furnaces,
     mostly silicates.

Smelting - A reduction of the lead oxide in the  ore  to produce
     elemental  lead.

Softening - A refining step usually performed  after  dressing  to
     remove antimony, arsenic,  and tin  (which  cause  lead to
     harden) .

Speiss  - A mixture of arsenides and antimonides  produced as  a
      floating waste  layer during  smelting.
                             7.6-38

-------
                   REFERENCES  FOR SECTION 7.6
 1.   Background information for New Source  Performance  Standards:
     Primary Copper,  Zinc,  and Lead Smelters.   Volume 1:   Pro-
     posed Standards.   EPA-450/2-74-002a.   U.S.  Environmental
     Protection Agency.    October 1974.   pp.  3.170-3.200,  5.28-
     5.40.

 2.   Kirk-Othmer Encyclopedia of Chemical Technology.  Vol.  12,
     2nd ed.   John Wiley &  Sons, New York.   1967.   pp.  208-238.

 3.   Control of Sulfur Oxide Emission in Copper, Lead,  and Zinc
     Smelting.  Information Circular 8527.   U.S. Bureau of Mines.
     Washington, D.C.   1971.

 4.   Thomas,  R., ed.   Operating Handbook of Mineral Processing.
     McGraw-Hill, Inc.,  New York.  1977.  pp.  299-303.

 5.   Complication of  Air Pollution Emission Factors.   2nd ed.
     Publication AP-42,  U.S. Environmental  Protection Agency.
     February 1976.   pp. 8.6-1, 8.6-4, C16.

 6.   Technical Guidance for Control of Industrial Process Fugi-
     tive Particulate Emissions.  EPA-450/3-77-010.  U.S.  Envir-
     onmental Protection Agency.  March 1977.

 7.   Aeros Manual Series, Volume II:  Aeros User's Manual.  EPA-
     450/2-76-029 (OAQPSNo. 1.2-039).  U.S.  Environmental
     Protection Agency.   December 1976.

 8.   Aeros Manual Series, Volumn V:  Aeros  Manual of Codes.   EPA-
     450/2-76-005 (OAQPS No. 1.2-042).  U.S.  Environmental Pro-
     tection Agency.   April 1976.

 9.   Standard Industrial Classification Manual.   Office of Man-
     agement and Budget.  Available from Superintendent of
     Documents, Washington, D.C.

10.   Loquercio, P.,  and W.J. Stanley.  Air  Pollution Manual of
     Coding.   U.S. Department of Health, Education, and Welfare.
     Public Health Service Publication No.  1956.  1968.
                             7.6-39

-------
                    7.7  PRIMARY ZINC SMELTING






PROCESS DESCRIPTION1"3



     The largest use of zinc is as an anticorrosion agent in the




form of zinc coatings for the protection of steel and iron.  It




is also used as an anode in batteries and fuel cells, in many




types of castings, in brass products, as rolled zinc in the




construction industry, and as zinc oxide in paints.




     Primary zinc smelting is the process by which zinc retal is




recovered from its ores.  The primary ore is sphalerite or ~inc




sulfide, which is commonly found with lead minerals and usually




contains some iron, cadmium, and other metals.




     Zinc ore must be concentrated, before smelting.  This con-




centration, called beneficiation, is usually carried out at the




mine and is not discussed here.  The zinc ore, in the form of a




relatively dry and fine concentrate, is transported to the




smelters by rail, barge, or truck.  The concentrate is usually



unloaded and stored in a covered building or silos at the plant




to protect it from moisture and from losses due to wind.  When




needed it is removed from storage by clamshell.  The steps of




zinc smelting are shown in Figure 7.7-1.




     Several types of roasters are used to remove lead and




sulfur from the zinc concentrate.  This is followed by either
                               7.7-1

-------
                                                                                  Figure  7.7-1.    Primary  zinc  smelting.
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-------
acid leaching  (electrolytic recovery) or thermal reduction



 (pyrometallurgical production).



     Multiple hearth roasters  are used ahead of fluid-bed



roasters to remove lead from the ore concentrate.  In the past,



these roasters were commonly used for desulfurization; and this



application may still be found in a few plants.  During desul-



furization, a large amount of  air is introduced into the multiple



hearth, and large amounts of S02 are emitted.  In current practice,



the multiple hearth is most often used for deleading.  The ore



concentrate enters the top center of the roaster where it is



heated to 1750° or 1800°F in a low oxygen atmosphere.  As the



material moves in a zigzag path to the bottom of the roaster,



between 90 and 95 percent of the lead sulfide  (PbS) is sublimed



and carried in the exhaust gases as particulate, with minimal



amounts of SO- emissions from oxidation.  The deleaded material



may require crushing and screening to break up lumps prior to



entering the fluid-bed roaster.




     The fluid-bed roaster is used to remove sulfur.  The feed is



either ore concentrate or deleaded ore concentrate from the



multiple hearth roaster.   Concentrate is suspended and oxidized



in a stream of upflowing air;  part of the calcine is withdrawn



from the floating bed in the bottom of the roaster.  The re-



mainder is carried with the gas stream to air pollution control



equipment where it is recovered and returned to the process.



     The flash roaster is also used to remove sulfur from ore



concentrate.   The material is  fed to the bottom,  where drying






                              7.7-3  '

-------
      place.   It is conducted to the top and then falls down



through an ascending stream of hot air that oxidizes the con-



centrate converting zinc sulfide to zinc oxide and releasing



sulfur in the exhaust gases.  Both the fluid bed and the flash



roaster are self-sustaining and need no extra fuel once ignited.



The product of both roasters is referred to as calcine.



     Electrolytic recovery is the most common method of obtaining



the zinc metal from the calcine.  The roasted ore is leached in



sulfuric acid to form a zinc sulfate solution.  Electrolysis



takes place after the iron, cadmium, and other impurities are



precipitated out.  The zinc sheets  (cathodes) that are formed



during electrolysis are stripped and melted in a reverberatory or



electric furnace.  Alloying agents are added to the matte zinc,



and it is alloyed in pot furnaces and cast into slabs or plates.



     Pyrometallurgical recovery is the other method for extract-



ing the zinc.  Before thermal reduction takes place, sintering  is



done to agglomerate the small calcine particles into a feed of



the desired physical properties.  A mixture of calcine, coke, and



sometimes sand is ignited  on a  strand  (travelling metal con-



veyor) ; sand  is  added to provide  strength  to the sinter that will



be used in an electrothermal furnace.  Air is pulled down through



the bed of material, which burns  from top  to bottom as  it moves



along  the strand.   In the  breaking  and  cooling phase,  sinter



falls  onto a  slab,  where it is  crushed  by  hammers,  and  usually  is




formed into briquettes.
                               7.7-4

-------
     Two types of thermal reduction furnaces  are  used to produce




high-purity zinc from zinc oxide;  they are the vertical retort



and the electrothermal furnace.   The vertical retort furnace is



an upright rectangle measuring about 1 ft wide by 7 ft long and



35 ft tall.2  Sinter  (which usually has been formed into bri-



quettes) and coke are intermittently fed into the top of the



furnace.  The charge is heated to 2400°F by firing natural gas in



chambers that surround the furnace.  Zinc oxide is reduced to



zinc metal as the charge settles in the furnace;  an upflow of gas



carries zinc vapor to a condenser, which condenses the vapor to



molten  zinc.  The noncondensable gases are discharged  to the



atmosphere through a particulate control device.   Residue  is



withdrawn from the bottom of the furnace for  further treatment.




The molten zinc  is cast into slabs or plates.



     The electrothermal furnace is similar to the vertical  re-




tort,  except  that heat is provided by current flowing  between



electrodes placed at  the top and bottom of the furnace,  rather



than by natural  gas.  Hard sinter, with silica sand  added,  must



be used in it.   Zinc  vapor is swept out and  condensed  as in the




vertical retort,  followed by casting.



     Various  kinds  of heat exchangers  are  used in  the  smelter  to



cool exhaust  gases  and to preheat  combustion air for the roasters



     Particulate from collection  devices  on  roaster off-gas is



sent to calcine storage;  at other  smelters it is combined with




 the  calcine on the  sinter  strand.
                               7.7-5

-------
EMISSIONS1"3'5'6

     Emissions from zinc smelters include particulates and

sulfur dioxide.   Emission sources are identified in Figure 7.7-1.

For some of the sources, AP-42  provides emission factors, which

are listed on the process flow diagram.   For other sources of

emissions, average emission rates obtained from other documents

are mentioned in the following source descriptions.

     Raw material unloading creates fugitive particulate emis-

sions of 0.03 to 0.4 Ib/ton of zinc ore concentrate, 0.03 to 0.4

Ib/ton of sand, and 0.4 Ib/ton of coke unloaded.

     Because the ore concentrate is often stored in silos or

buildings to protect it from weather, emissions are usually

minimal from this source.  Minor fugitive emissions occur from

the open storage of sand, coke, coal, and sometimes partial

concentrate storage.  Handling of the raw materials, including

concentrate, sand, coke, and coal, does create  fugitive particu-

late emissions.  When uncontrolled, these emissions are 2.1 to

5.5 Ib/ton of material  handled.

     The exhaust gas from the multiple hearth roaster contains
                                                           3
particulates, and may contain small amounts of  SO2-  AP-42

provides emissions factors for the multiple hearth furnace when

it is used for  desulfurization.  Almost all multiple hearths  are

now used  for deleading  under  different operating  conditions,  and

the emission  factors in AP-42 do not  apply  in this circumstance.
                               7.7-6

-------
     Crushing and screening of the deleaded material generate


particulate emissions.


     Off-gas from flash and fluid-bed roasters contains 50 to 85

                                  2
percent of the feed as particulate  and 5.5 to 12 percent sulfur


dioxide by volume.   Most of the particulate is, however, re-


covered from the gas stream in cyclones and directly recycled to


the process.  The cyclones are part of the process equipment.


Remaining particulate is captured in downstream control equipment


and is partially recycled to the process.  The cleaned gas,


containing SO_, is sent to a sulfuric acid plant for sulfur


recovery.


     Electrolytic processing generates minor amounts of fugitive


particulate emissions including release of acid mists.  The zinc


melting and alloying processes that follow electrolysis also


generate particulate emissions.


     The sintering process has several sources of emissions.


Some fugitive emissions are liberated from the feed end of the


sinter machine during the transfer of material onto the conveyor


strand.  Exhaust from the sinter machine includes small amounts


of SO  from combustion of sulfur in the calcine.  The sulfur


content is usually 2 to 3 percent sulfur.  Particulates carried


in the stream are usually recycled.  One of the largest sources


of particulates at a smelter is the sinter breaking and cooling


section, where sinter leaving the machine is crushed.   Uncon-


trolled emissions from sinter breaking are 0.55 to 2.45 Ib/ton of


sinter.



                              7.7-7

-------
     Reduction furnaces,  both vertical retort and electrothermal,



produce a significant amount of particulate emissions.   They also



produce carbon monoxide,  which is usually returned to the furnace



as fuel and is not released to the atmosphere.



     Casting of the molten zinc both from electrolytic recovery



and pyrometallurgical processes emits 2.52 pounds of fugitive



particulate per ton of zinc produced.






CONTROL PRACTICES '   '



     Emissions from raw material unloading and handling and



transfer are generally not controlled; however, water sprays or



enclosures can be used to reduce fugitive emissions.



     The exhaust gases from the multiple hearth are vented to



particulate control devices, usually to an electrostatic pre-



cipitator  (ESP).  The particulates from the crushing and screening




operation are controlled by passage through a cyclone or bag-




house.



     Off-gas from flash and fluid-bed roasters is exhausted



through particulate and SO2 controls.  The SO2 is removed at



sulfuric acid plants; however, the gas entering a sulfuric acid



plant must be essentially free of particulates to avoid damage to



catalysts and to prevent impurities  in the acid.  Particulate is



therefore removed at the smelter by  a combination of cyclones and



wet ESP's.  Overall efficiencies of  greater  than  99 percent  can



be attained.   The preconditioned gas stream then enters the



sulfuric acid plant, where wet scrubbing  towers and drying towers



clean the  incoming gas of all remaining particulates  and water



                               7.7-8

-------
vapor.   The scrubbing liquid is sulfuric acid.   Single-contact




plants, which are the most common,  have S02 removal efficiencies




of 95 to 98 percent.



     Electrolytic recovery results in a relatively minor release



of acid mist in the cell room from oxygen and hydrogen liberation



at the anode and cathode.  These emissions are not controlled



with air pollution devices, but the cell room is usually venti-



lated to minimize corrosion of equipment.  Various electrolyte




covers and additives are used to reduce misting.



     Particulate emissions from zinc melting and alloying are




controlled with baghouses or scrubbers.



     Emissions from the charging of the sinter strand are not




controlled.



     Exhaust gases from the sinter machine contain particulates



and small amounts of S02.  '   Particulate is removed by baghouses



or ESP's, with efficiencies of 98 percent and 90 to 96 percent,



respectively.  The SO,, is not controlled, but the hot gases are



often vented to the same stack as the gases from the sulfuric




acid plant to add buoyancy.



     Particulates from the sinter breaking and cooling operation



are controlled at all smelters with baghouses with an efficiency




of 99 percent.



     Gases from vertical retort and electrothermal furnaces



contain metallic vapor and carbon monoxide.  The gases pass



through the zinc condenser and then through a venturi scrubber,



which removes entrained  particulates, and the carbon monoxide gas
                              7.7-9

-------
 is used as part of the fuel for heating the retorts.  Blue pow-



 der, a mixture of metallic zinc and zinc oxide, is recovered from



 the scrubbing system and is recycled  or sold as a byproduct.



     Emissions from casting of the molten metal are usually not


 controlled.





 CODING NEDS FORMS8"11



     The emission sources associated with primary zinc smelting
are:



Source



Raw material unloading



Raw material handling and

  transfer



Multiple hearth roaster



Crushing/screening



Fluid-bed roaster



Flash roaster



Electrolytic processing



Zinc melting



Alloying



Sintering
SCC



3-03-030-12





3-03-030-09



3-03-030-02



3-03-030-14



3-03-030-08



3-03-030-07



3-03-030-06



3-03-030-15



3-03-030-16



3-03-030-03
Sinter breaking and cooling   3-03-030-10
Reduction furnace



Zinc casting
3-03-030-05



3-03-030-11
Pollutant(s)



Particulate





Particulate



Particulate



Particulate



Particulate, SO,
               A


Particulate, SO,
               ^


Particulate



Particulate



Particulate



Particulate, SO,
               ^


Particulate



Particulate, CO



Particulate
     Standard NEDS forms,  Figures 7.7-2 through 7.7-13, show



entries for the SCC's and other codes.   Entries in the data field



give information common to primary zinc smelting.  Information





                             7.7-10

-------
pertinent to coding the source is entered on the margins of the



forms and above or below applicable data fields.  Entries for



control equipment codes, other optional codes, emission factors,



and required comments minimize the need to refer to the code



lists.  Typical data values for operating parameters, control



equipment efficiencies, and other source information are shown on



the form (or in the text)  only to aid in rapid, approximate



checks of data submitted by the plant in a permit application or



similar report.  Data entered in EIS/P&R and NEDS must be actual



values specific to, and reported by, the plant rather than typical



values.  Contact the plant to validate or correct questionable



data and to obtain unreported information.  See Part 1 of this



manual for general coding instructions.



     Emissions from unloading the ore concentrate, sand, and coke



are not controlled, and an emission factor has not been developed.



Figure 7.7-2 illustrates the standard NEDS form for this source.



     The emission source labeled "raw material handling and



transfer" includes all pollutants from the handling of ore, sand,



coke, and coal prior to the sintering operation or the electro-



lytic processing.  An emission factor for this source has not yet



been developed.  When a plant furnishes emissions data, code the



value given and enter "Emission estimate given by plant" in the



comments field on Card 7.   When there is no control device (as is



most common) or when water sprays are used to reduce emissions,



enter zeros in the stack height and diameter fields, 77 in the



temperature field, and zeros in the common stack field.  Enter






                             7.7-11

-------
appropriate height in the plume height field.  When water sprays



are used, enter 061 or 062 as a control equipment code.  Identify



other emission reduction practices, such as use of enclosures, in



the comments field on Card 6.  Figure 7.7-3 illustrates the




standard NEDS form for this source.



     When a multiple hearth roaster is used for deleading, it is



coded as shown in Figure 7.7-4.  There is another SCC number that



refers to multiple hearth roasters as a desulfurization method;



however, this is no longer widely practiced, and the emissions



factors associated with it do not apply to deleading.



     The standard NEDS form for crushing/screening is shown in




Figure 7.7-5.



     When a cyclone on a flash or fluid-bed roaster returns its



catch directly to the roaster, it is considered process equipment




and not a control device.  The ESP's are the most common control



devices used at zinc smelters.  Figure 7.7-6 illustrates the



standard NEDS form for flash and fluid-bed roasters.



     Since the gases from the  sinter machine are often vented  to



a sulfuric acid plant, the associated emissions are accounted  for



on the NEDS  forms for the acid plant.  On  the  NEDS  form  for the



zinc smelter, enter zeros for  emission estimates and allowable



emissions and fives for the estimation method.  The  five denotes



a special emission factor; in  this case, that  the emissions are



vented to another process.   Code zeros in  the  stack  data  field.



Code the sulfuric acid plant as described  in the compendium on




sulfuric acid manufacturing.






                              7.7-12

-------
     Emissions from electrolytic processing and casting are not




usually controlled.  Figures 7.7-7 and 7.7-13 show the appro-




priate NEDS forms for these sources.




     Figure 7.7-8 shows entries on the standard NEDS form for




zinc melting.  The in-process fuel may be either oil or natural




gas.  In newer plants that use electric furnaces, no in-process




fuel is needed.




     Figure 7.7-9 is a standard NEDS form for alloying.




     Sinter machine exhaust gases are commonly vented through the




same stack (after control) as the roasting emissions  (after




control in the sulfuric acid plant).  In this case enter the




appropriate point ID's in the points with common stack field, and




enter identical values for stack height and diameter for each




source on the two NEDS forms.  Figures 7.7-10 and 7.7-11 show the




standard NEDS forms for sintering and sinter breaking and cool-




ing.




     Vertical retorts and electrothermal reduction furnaces have




the same emission factors and the same SCC, 3-03-030-05.  Note




that only the vertical retort uses in-process fuel (natural gas),




SCC 3-90-006-05.    Enter a comment telling which type of fuel is




being reported.  The standard NEDS form for the reduction furnace




(vertical retort or electrothermal furnace) is shown in Figure



7.7-12.




     Most smelters have more than one roaster, sinter strand, and




reduction furnace.  Some have three types of roasters.   Code




each unit separately to ensure that all emissions are recorded.






                             7.7-13

-------
CODING EIS/P&R FORMS12



     The EEC's of the equipment in a zinc smelter are:




     Source                                  EEC



Raw material unloading                       700



Raw material handling and transfer           700



Multiple hearth roaster                      287



Crushing/screening                           650



Fluid-bed roaster                            287



Flash roaster                                287



Electrolytic processing                      No code*




Zinc melting                                 978



Alloying                                     No code*




Sintering                                    979



Sinter  breaking and  cooling                  664



Reduction  furnace                            977



 Zinc casting                                 No code*






 *As of  October 1978.
                               7.7-14

-------
         Figure  7.7-2.   Standard NEDS  form  for  primary zinc  smelting  - raw  material unloading.
 I
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                                                    NATIONAL EMISSIONS DATA SYSTEM (NEUS)
                                                      ENVIRONMENT Al PROTECTION AGEMCY
                                                         OFFICE OF AIR PROGRAMS
                                         POINT SOURCE

                                          Input form
FORM APf'HOV E.O
OMfa NO 158 R009b

Date	
                                                                                        ,TRT
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                                                                     IP! i i 1 il.J
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                            i^i-riilitiillfit:
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-------
    Figure  7.7-3.   Standard NEDS  form  for  primary zinc smelting - raw material handling and transfer
                                                                        POINT SOURCE
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NATIONAL EMISSIONS DATA SYSTEM (NEOS)
ENVIRONMENTAL PROTECTION AGENCY
OFFICE OF AIR PROGRAMS
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-------
             Figure  7.7-4.   Standard NEDS  form  for  primary zinc  smelting  - multiple hearth  roaster.
SI4IC.
1 2

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                                                       NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                         ENVIRONMENTAL PROTECTION AGENCY
                                                             Off ICE OF AIR PROGRAMS
                                                                                        POINT SOURCE
                                                                                         Input Form
                                  I
                                                                                  Njm* ol Pe,ion
                                                                                  Complfling Fcwm_
FORM APPROVED
cue NO
Oil*.
                                                                                                                   Conuct  Prr
  ^iLiMZ™^^^^
  LiJ^LLi_j_l_L.i_L_Lj_L_L.J_L LjJJ.i  ij_ J_iJ_L±JJLU.lJJTj^{j7LlT_L^
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       o t'  I Bo,I,, rif- ar.   t-'10    f;   •      f-^'         ?_|.          |^         1^, ;   rSTIMATtO CONTROL 6FFPCI«N':v l\l  J
                                                                                               rSTIMATtO CONTROL 6FFPCI«N':v l\l
                                                                                         nf'    OP,
                                                                                                   ^0,   NO.    MC    CO
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                                                                          EMISSION £Sf'VA7ES (ion* vaad

                       j >0i   k
-------
                    Figure  7.7-5.     Standard  NEDS  form   for  primary  zinc  smelting  -  crushing/screening.
                   Slat
                   TT;
                        3  4  5 6
71 9
      10 II  12 IJ
 I
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                                         Point
                                         11^
                                         llllb
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                                                16 II
                                                16 17
                           CRUSHING/SCREENING

                                                        20 21
                                                    I 19 20 21
                                                    ITTJ
                  NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                    ENVIRONMENTAL PROTECTION AGENCY
                         OFFICE OF AIR PROGRAMS

                         EitabMthment Name and Addieit
                                                                                                                                             POINT SOURCE
                                                                                                                                               Inpul Fotm
                                                                                                       Nam* of Person
                                                                                                       Complftmg Form.
                                                                                                                                      FORM APPROVED
                                                                                                                                      QMS NO IMB0095
                                                                                                                                      Dai.	
                                                            22l?3l24|2>l26l27l28|23|30|3l|32|33|34|3S|36|37|3i » 40 S 46 47T48 49 50 S[ S2 53 S4 SS 56 £ SI  » 60 61_
                                                            22 23
                                                     106 BTU/nr
                                                        20 21
  UTM Cl
Horttontat
  km	
                                                                           OINATES
                                                                            Vertical
                                                                         2! 29 »  31 32
                                                    33 34 3S 3(
                                                            37 38  19 40 41 12 43
                             STACK DATA

                             Temp(°FI  Flow Rate (It3/m
                                                              23 24
                                                      ANNUAL THRUPUT
                        20 21
                                                                       27 21
                                                                     OTO 0 0
                                                                           Pntnary
                                                                            SO?
                                                                           29 30 31
                                                                      NORMAL
                                                                     OPERATING
           29 30
                                                        CONTROL   EQUIPMENT
                                                                ft
                                                                "o
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    Kk ft
                                           41 4S 46 47 41 49 S0| 51 52 S3 54
                                                                                         NO,
                                                                                        3b id 3)
                                                                     Pi.mar,   03
                                                                3      HC    Jj
                                                                                               38 39 40
                                                                                                     41 42 43
                                                  Primary
                                                    CO
                                                                                                                          lo
                                                                                                                                                        Contact • Pertonal
                                                                                                                  62m 6t Us 66 67 6169 70 71 72|73
,0000  If NO COMMON  STACK
 XXXX  POINT ID'S  IF COMMON STACK
                                                                          6116? 63|64 6S 66|67 68 63 70 71 7: 73 74|75 76 77
                                                           ESTIMATED CONTROL EFFICIENCY IXI

                                                          Part    SO?     NO*    HC     CO
                                                                                                                                      Si 57 51
                                                                                                                                            59 (0 (I
                                                                                                                                                   6? 63 «4
                                                                                                                                                         6S 66 67
               31 32 33 X 35 16 37
                                                                         EMISSION ESTIMATES Uoni/year)
                                                                                                     SO2             NO,
                              38 39 40 11 I2l<3 44
                                                46 17 U 4? SO SI
                                                             52 S3 S4 SS S6 S7  SI
                                                       Particulm
                                                    8 U 20 21 22121124
                                                                            ALLOWABLE EMISSIONS llor«/v*arl
                                                                        SO;             NO,
                                                           21 22 23
                                                                     26 27 2112) 30  31
                                                 32  33 34)3sl3t 17 31
                                                                                                 31 10 41  I? UlM IS
                                                                     26 27 21 29 » 31 32
                                                                                    33 34 3S 36 31 31 39
                                    1
                                    m
        SCC  UNIT - TONS PROCESSED   _
 Fuel PioctSt*         Houdy         ?r t   5 - «
 Soi-a Wane      lVa«imum O»>v"     "-^1   "•  |
Opetannq Baie        ** -•-             •      - -
                                                                                                                «,  «! U n SO SI S2
                                                                                               ^COMPLIANCE
                                                                                               « SCHEDULE
                                                                            S9 60 61 62 63 64 6V
                                                                          COMPLIANCE
                                                                             STATUS
                                                                             UPDATE
                                                                                                                                                                61 69 70 71 72 73 74 75| 76 7)
                                                                                           ESTIMATION
                                                                                             METHOD
                                                                                             67 8!  17  48 49 SO
                                                                                                                           Si S2  S3 S4 SS Si S7
                                                                                                                                               60 11
                                                                                                                                      8
                                                                                                                                      1  1
                                                                           29 30 31 32 33
                                                                                             37|3Bh9l40|ilh2|»|»|lS|4«|4l|)8|49|solSl|s;|S3|S4|irfT6 5' 58 S9 60 61 62 63 64 6S 66 67_ it 69 70 71^ 11 73 74  75 76

-------

-------
        Figure   7.7-7.     Standard NEDS  form  for  primary   zinc  smelting  -  electrolytic  processing,
            1 2
 I
NJ
O
               3 4|S
                                14 IS IS II
 PoilM
 ID


ffl
                                    U II
                                    tt
                                    ie|i;
                        ELECTROLYTIC
                         PROCESSING
                                           >M
                                           20 21
                                     NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                       ENVIRONMENTAL PROTECTION AGENCY
                                            OFFICE OF AIR PROGRAMS


                                            EiMblnhinm Njrnr and Artd,en
                                                                                                                      POINT SOURCE
                                                                                                                                             FORM APPROVED
                                                                                                                                             OMB NO 158 R009S
                                               5: 3
                                                     U1M COORDINATES
                                                                31 32

STACK DATA

 Tsmp!nFI  F!
                                                                                            , nitf (M/minf |M
                                                                        CONTROL   EO'J'P''

                                                                                                           Pi,I  I  SOj I  NO,    HC  | CO
          It 19 29 21 22 2! 24
                                ALLOWABLE EWISS'ONC li-m/ytir)


                            S02           "O,
                          5 21 ?S 29 30 31
                                                   sec
                                              .'1 27 23
                         UNITAnn JONS  PROCESSED
                           Furl Piyceis
                            Solid W«|*
                           Op*,fti,'in Rale
                                     ££
                                     > I
                                     itTi;
                                              21 22 23
                                     3? 33 35 Ji jfcjl ;S
                                                  :9!4D 
-------
     Figure  7.7.8.    Standard NEDS  form  for  primary  zinc  smelting  -  zinc melting  in-process  fuel
 i
NJ
I—1
                             Numtef
NATIONAL EMISSIONS DATA SYSTEM (NEDS)
  ENVIRONMENTAL PROTECTION AGENCY
     OFFICE OF AIR PROGRAMS
                                                                                                        POINT SOURCE
                                                                                                         Input Fofm
FORM APPROVED
OMB NO 1&6-R009S
                                                                                                   Name of Ptrton
                                                                                                   Compltting Form
                                   Hl;7|ll|19|2
                                  nimii
                                                                        it Name and Addiesi
                       u.  cr cr>
                                      TTIIE"
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-------
                Figure  7.7-9.    Standard  NEDS  form  for  primary  zinc  smelting  -  alloying.
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                            ot at
                          +  i i
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NATIONAL EMISSIONS DATA SYSTEM (NEDS)
  ENVIRONMENTAL PROTECTION AGENCY
      Of F1CE OF AIR PROGRAMS


      Establishment Name and Address
                                                                                                                     POINT SOURCE
                                                                                                                      Input Form
                                                                                                                Name of Person
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                                                                                                                 FORM APPROVED
                                                                                                                 O*»8 NO 158R009S
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-------
Figure  7.7-10.   Standard NEDS  form  for  primary  zinc smelting  - sintering.
                                NATIONAL EMISSIONS DATA SYSTEM (NEDS)

                                 ENVIRONMENTAL. PROTECTION ACtNCY

                                    OFFICE OF AIR PROGRAMS
                                                                    P'JIMT SOURCE
FOPM APPROVED
OMB NO i$8ncx>95
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         il;!?iMLSSi:STrilTITi t?l"!jj-'I1"i"1 -H:I:] ^ rfifetei^

-------
                    Figure 7.7-11.  Standard NEDS form for primary zinc smelting -

                                    sinter breaking and cooling.
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NATIONAL EMISSIONS DATA SYSTEM (NEDS) POINT
ENVIRONMENTAL PROTECTION AGENCY '"'""
OFFICE OF AIR PROGRAMS NameoiPe.son
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Establ shment Name and Address
221

23

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SOURCE FORM APPROVED
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Contact • Personal
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79 SO



-------
          Figure  7.7-12.    Standard NEDS  form  for  primary zinc  smelting -
         reduction  furnace  (vertical retort  and electrothermal  furnaces).
                                           NATIONAL EMISSIONS DATA SYSTEM (NEDS) .
                                             ENVIRONMENT! PROTECTION AGENCY
                                                OFFICE OF AIR PROGRAMS
POINT SOURCE
                 FOPM APPROVED
                 OMB NO 158 R0095
                                                                                     0000 IF NO COMMON STACK       c
                                                                                     XXXX POINT ID'S IF COMMON STACK
                                         PROCESSED; FORFD
                                                                                S '.« (C <•• ,: fi «: Si 6(. 57 65 09 70 71 'J ,'J )» 75 76 77
       REDUCTION FUPJiACE
INPROCESS FUEL (RETORT ONLY),

-------
Fxgure 7.7-13. Standard NEDS  form  for  primary zinc  smelting -  zinc casting.
1
to
State.
1

j

Counlv
3

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6

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POINTS
Input
Name of Person
Completing Form
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S03
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-------
GLOSSARY

Calcine - The predominantly zinc oxide product of a roaster.

Retort -  A furnace used to reduce zinc oxide to zinc metal.

Sinter -  An agglomerated product produced by heating the material
          to the point of fusion.

Strand -  A travelling metal grate or conveyor belt.
                              7.7-27

-------
                  REFERENCES FOR SECTION 7.7


1.  Background information for New Source Performance Standards:
    Primary Copper, Zinc, and Lead Smelters.  Volume 1:  Pro-
    posed Standards.  EPA-450/2-74-002a, October 1974.  pp.
    3.125-3.169, 5.18-5.27.

2.  Kirk-Othmer Encyclopedia of Chemical Technology, Volume 22.
    2nd ed.  John Wiley & Sons, New York, 1970.  pp. 563-589.

3.  Compilation of Air Pollution Emission Factors.  2nd edition.
    U.S. Environmental Protection Agency.  AP-42, February 1976.
    p. 7.7-1.

4.  Control of Sulfur Oxide Emissions in Copper, Lead, and Zinc
    Smelting.  U.S. Bureau of Mines, Washington, B.C.  Informa-
    tion Circular  8527, 1971.

5.  Development Document for Interim Final  Effluent Limitations
    Guidelines and Proposed New Source  Performance Standards for
    the Zinc Segment of the Nonferrous  Metals Manufacturing
    Point  Source Category.  EPA-440/1-75/032, February 1975.

6  Technical Guidance for Control of Industrial Process Fugi-
    tive Particulate Emissions.  EPA-450/3-77-010, March 1977.
    pp. 2-150-163.

7.  Cotterill,  C.H. and  J.M. Cigan, ed.  Extractive Metallurgy
    of  Lead  and  Zinc:  AIME world symposium on  mining and metal-
    lurgy  of  lead  and  zinc.  Volume II.  New York.   The Metal-
    lurgical  Society of  AIME,  1970.   1090 pp.

8  Aeros  Manual Series  Volume II:  Aeros User's Manual.  EPA-
    450/2-76-029 (OAQPS  No.  1.2-039), December  1976.

 9.  Aeros  Manual Series  Volume V:   Aeros Manual of  Codes.   EPA-
    45/2-76-005 (OAQPS No.  1.2-042),  April  1976.

10  Standard Industrial  Classification  Manual,  1972 Edition.
    Prepared by Office of Management  and Budget.   Available from
    Superintendent of  Documents,  Washington, B.C.
                               7.7-28

-------
11.   Loquercio,  P.,  and W.J. Stanley.   Air Pollution Manual of
     Coding.   U.S.  Department of Health, Education, and Welfare.
     Public Health Service Publication No. 1956.  1968.

12.   Vatavuk,  W.M.   National Emission Data System  (NEDS) Control
     Device Workbook.   U.S. Environmental Protection Agency,
     APTD-1570,  July 1973.
                               7.7-29

-------
                7.8  SECONDARY ALUMINUM OPERATIONS





 PROCESS DESCRIPTION1"4




      In secondary  aluminum operations,  aluminum scrap is melted



 and mixed with other metals to produce lightweight alloys for



 industrial castings.  Copper,  magnesium,  and  silicon are the most



 common alloying constituents.




      The raw materials  for secondary  aluminum plants come from



 three main sources:




      1.    Aluminum pigs.   These may be  primary metal or  may  be



 secondary aluminum produced by a  large  secondary  smelter to  meet



 standard alloy specifications.




      2.    Foundry  returns.   These include rejected castings  and



 mold  components  such  as gates,  risers,  runners, and sprues.



      3.    Miscellaneous scrap.  This  category  includes aluminum



 borings  and  turnings; other items contaminated  with oil,  grease,



 paint, rubber, and plastics; and aluminum mixed with metals  such



 as  iron, magnesium, zinc,  and  brass.




      Figure  7.8-1  is  a process  flow diagram of  secondary  aluminum



 operations.  The raw materials  are sometimes pretreated  to prepare



 them  for smelting, the process  of melting and removing impurities



 such  as oxides.  Used castings  and other foundry returns may need



 to be crushed or screened to bring about the mechanical or



magnetic removal of iron,  and the mechanical separation of dirt






                              7.8-1

-------
                       9
  RAW
MATERIAL
STORAGE
1

SECONDARY
CONTROL
DEVICE
t
1

PRIMARY
CONTROL
DEVICE
FABRIC FILTER 016
ESP 01°
AFTERBURNER 021
WATER SPRAY 003
i PART^U.^)





B

3-04-001-01
SWEATING FURNACE
3-90-OOX-99


O *-°
^-r 6_w
t 0 PW
CONTROL
^ PAR"
CRUSH IN
SCREENI
L
mjRAL
FABRIC
rO
G/
NG
GAS
FILTER 018

3-04-001-08
CRUSHING/SCREENING


CONTROL
DEVICE
AFTERBURNER 021
|i HC O
ROTARY
DRYER
.^

t FABRIC FILTER 016 /~\
! ESP 010 Vj

SECONDARY 1
CONTROL }
1 	 	 1 StlUNUAKT l-ABKlb riLiuiv uiv
f AFTERBURNER 021 CONTROL ESP °>°
1 HIGH FNFBC-v "FT nni BE^ICE






3-04-001-09
BURNING/DRYING
PRIMARY SCKUBBEk t
Cr0J!™L FABRIC FILTER 017
_KYiCE J i PRIORY " HIGH ENERGY WET 001 _
4 * O CONTROL SCRUBBER /^~N fj
| MMRUSTION /T\ DEVICE _ HET CYCLOfK 009 \J ^S
, PROOUOS ^ i  CHLORINATION 4 .-, ^, ,OT /-^
1 PART @ S^™ ? '«T © FLUORIOATION >«T Q 	 l^O

FURNACE INUOI
j 	 -1 L. 	 	 	 ' CAST!
^W1 5 I SSaATORY ^L*^
.a^oox^ tSSSSSSlS
IN-PROCESS I-UEL ' '
4-OIL
6-NATURAL GAS
|
CONTROL FABRIC FILTER 016 i rerun-
DEVICE WET SCRUBBER 002 Llbtnu.
' 1 	 r' Q EMISSION FACTOR*
t PART <^> EMISSION FACTOR HOT DEVELOPED
•* 	 ' — \-/ FOR THIS PROCESS
009 (66.0) DENOTES CONTROL EQUIP.
l ' f.ODE WITH EST. EFF. SHOWN
3^04-001-07 1 IN ( }
HOT r DROSS V DENOTES FUGIT,VE
PROCESSIRG > EMISSIONS
Q DENOTES A STACK
* IN POUNDS PER SCC UH1T
IN-PROCESS FUEL
4-OIL
6-NATURAL GAS
                                         Figure 7.8-1
Secendary Aluminum Operations


   7.8-2

-------
 and  loose  aluminum oxide.  Borings and  turnings  are  burned  and




 dried  in direct-fired rotary kilns to remove cutting oils,



 grease, and moisture.




     Another form of pretreatment is sweating, which is  used  to



 recover aluminum from scrap having a high  iron content.   Open-



 flame  reverberatory furnaces with sloping  hearths are generally



 used,  although grate-type  furnaces also may be used.  The alu-



 minum  scrap is charged into the furnace where the aluminum  melts



 and  is collected while the higher melting  iron,  brass, and  other



 materials  remain.  Aluminum recovered by this process is  referred



 to as  sweated pig.




     Smelting of pretreated and raw aluminum scrap is done  in



 either crucible or reverberatory furnaces.  The  crucible  or pot-



 type furnace is used for melting small quantities of aluminum (up



 to 1000 pounds) and is usually charged  (loaded)  by hand with  pigs



 and  foundry returns.  The reverberatory furnace, with mechanical



 charging,  is used for medium and large capacity  batches.  Both



 gas- and oil-fired units are used.




     After a batch is completely melted, alloying ingredients are



 added to adjust the composition of the product.  The melt is  then



 treated to remove trapped gases and metals, such as magnesium.



This treatment is referred to here as fluxing, with chlorine gas



or other materials used as fluxing agents.  This process  is



carried out either in the smelting furnace, in a separate well in



the furnace,  or in a different unit.   Often the fluxing process



is referred to as degassing or demagging,  depending upon its
                              7.8-3

-------
purpose:  degassing reduces dissolved gases; demagging reduces
the magnesium content of the melt.  These operations can overlap;
chlorine, for instance, can function as a fluxing agent to demag
and also to degas molten aluminum, depending on the state of
chlorine and the amount added.
     Chlorine and fluoride fluxing are accomplished by introducing
chlorine or fluoride through  the molten metal to float the mag-
nesium  to the surface where it is removed with the dross.  The
melt can also be degassed by  bubbling chlorine through the
molten  metal bath.
     Degassing  can  be  accomplished by other methods,  such as
bubbling dry nitrogen  through the melt;  by  mechanical vibration;
or by  application  of a vacuum.
     After  these operations  the  metal  is poured  either  into  ingot
molds  for  shipping or  into preheated crucibles  for product manufac-
 turing and  shipping.
      The dross from the smelting furnace contains enough aluminum
 metal to justify its recovery.  The two methods for recovering
 the metal are wet or dry milling (mechanical);  or hot dross
 processing (pyrometallurgical).   In wet milling, the cooled dross
 is ground,  screened, and magnetically separated.  In dry milling
 the cooled dross is separated by air classification  after grind-
 ing and screening.  In hot dross processing, materials that
 solubilize impurities  are added  to  the molten dross.  The insoluble
 aluminum metal is  tapped off the bottom  and returned to the
 smelting furnace.
                                7.8-4

-------
     A typical plant will have four or five furnaces and produce



100,000 to 1,000,000 pounds of aluminum per day.  Stack heights



for a typical secondary aluminum smelting operation range from 15



to 75 feet, with an average of 40 feet.





EMISSIONS1"6



     Emissions from secondary aluminum operations include fine



particulate matter, some hydrocarbons, and gaseous chlorine or



fluoride.  Emission sources are identified in Figure 7.8-1.



For some of the sources AP-42  provides emission factors, which



are listed on the process flow diagram.  For other sources of



emissions, average emission rates obtained from other documents



are mentioned in the following source descriptions.



     The storage and handling of the scrap raw materials release



insignificant amounts of particulates.



     Pretreatment causes various amounts of emissions.  Crushing



and screening can generate either minor or significant quantities


                                                             4 5
of particulates, depending largely on the grade of the scrap. '



     The burning/drying process is a major source of emissions.



Very little excess air is used, in order to minimize oxidation of



the aluminum.  A dense black smoke of partially burned oils, fine



aluminum, and aluminum oxide particulates is formed.  Other



contaminants, such as chlorides, fluorides, and SO,,, might also



be present.



     The sweating furnace is a major contributor of particulates



because of the contaminated scrap it processes.  Small amounts of



magnesium in the scrap can release large quantities of fumes.




                              7.8-5

-------
Although the majority are captured, some particulates become
fugitive during charging and residue removal; Reference 6 reports
a fugitive emissions rate of 0.72 Ib/ton of metal processed.  The
sweating furnace can also be a source of hydrocarbon emissions
when the scrap is contaminated with oil, grease, or tar.
     Most of the emissions from a secondary aluminum plant are
generated by the smelting process.  These emissions are particu-
lates and some combustion products from the fuel.  Hydrocarbons
are sometimes released from dirty scrap, although most of the
hydrocarbons escape during sweating.
     When chlorine is used for fluxing  it is added so rapidly
that large quantities of aluminum chloride and magnesium chloride
particulates are emitted.  Particulate  emissions during chlorina-
tion are 1000 pounds per ton of chlorine used, or 14.5 pounds per
ton of  product.1  The emissions also  include excess  chlorine and
some hydrogen chloride  (HC1).  At melt  temperatures  the aluminum
chloride is  a vapor; it  cools  in  the  atmosphere  to form fumes
 (submicron particulates), which absorb  moisture  from the  air and
form hydrogen chloride.  These emissions are toxic,  corrosive,
and  irritating.  Data on emissions  from fluoride fluxing  are not
available.
     When  smelting  and  fluxing are performed sequentially in  the
 smelting  furnace,  all  emissions  are vented to  one control system.
At some plants,  the smelting and  fluxing are performed in two
 separate  wells  in  the  furnace; or smelting is  done in the furnace
 followed by fluxing in a separate unit.  In these cases,  the
                               7.8-6

-------
 emissions from smelting and from fluxing are collected and con-
 trolled separately.
      Wet milling emits minor fugitive particulates in the course
 of feeding the cooled dross into a ball mill.  Dry milling may
 emit some fugitive particulates during the handling of the cooled
 dross and during grinding and screening.  Uncontrolled fugitive
 emissions from hot dross handling and processing are estimated at
 0.22 Ib/ton of metal processed.
      Other sources of emissions from secondary aluminum pro-
 cessing include raw material storage and handling,  and pouring of
 the molten aluminum.   Emission  rates for these sources are
 considered to  be minor and  values have not been reported.6

 CONTROL PRACTICES1"7
      Where crushing  and screening cause significant emissions,
 they  are usually  controlled by  fabric  filters.
      The combustible  portions of  the emissions  from the  burning/
 drying  process  are controlled by  afterburners  that  convert hydro-
 carbons  and the carbonaceous matter  into  carbon  dioxide  and
 water.   Afterburners  do not, however,  reduce  the metallic  parti-
 culates  entrained in  the exhaust.
     Emissions released during  the charging of the  sweating
 furnace  are usually vented  through the main furnace control
 system.  Hydrocarbons from  the melting of the aluminum scrap in
 the sweating furnace may be controlled by an afterburner.
Particulates are controlled by passage through a fabric filter,
                              7.8-7

-------
after the exhaust has been cooled by a water spray.  An electro-



static precipitator may also be used to control particulates.



     The smelting furnace, like the sweating furnace, is equipped



with a combination of controls:  an afterburner plus a fabric



filter or electrostatic precipitator.  The afterburner reduces



particulates, which tend to blind the fabric filter.  When hydro-



carbons are emitted they are also reduced by the afterburner.



Instead of an afterburner, a high-efficiency wet scrubber may be



used with or without a secondary control.



     When smelting and fluxing are carried out sequentially in



the furnace, emissions are usually vented to one control system.



Since emissions from fluxing contain corrosive gases, the control



system must include a device to remove the gases, as when fluxing




is done separately.



     A combination of controls is used when the fluxing operation




is separate from the smelting.  Gaseous pollutants, such as



chlorine and HC1, and most of the particulates are removed by



high-efficiency wet scrubbers that use a caustic solution.



Scrubbing is followed by heating and passage through fabric



filters to remove the remaining particulates.  Coated baghouses



that are efficient in removing both the acidic gases and particu-



lates appear to be gaining popularity.   The coating, which



neutralizes acidic gases, must be replaced periodically.  A wet



cyclone is sometimes used for this application, followed by a



fabric filter or electrostatic precipitator.  The precipitator,



however, encounters operational and maintenance problems from



corrosion by the acidic gases.




                              7.8-8

-------
     Data are not available on control devices used to control



emissions from degassing by nitrogen, application of a vacuum, or



mechanical vibration.  Degassing with chlorine or fluoride  is a



part of the fluxing operation.




     The small amounts of emissions from handling of the dross



during wet and dry milling are not usually controlled.  The



grinding/screening equipment used in dry milling is entirely




enclosed, and air for classification is recycled to prevent par-



ticulate emissions.  Fumes and particulates from hot dross proc-



essing are sometimes controlled by hooding and venting through a



fabric filter or scrubber.




     Emissions from the pouring operations are minor and are not



controlled.






CODING NEDS FORMS7"10




     The major sources of emissions from a secondary aluminum



plant are:
                              7.8-9

-------
Source

Crushing/screening

Burning/drying


  In-process fuel

Sweating furnace


  In-process fuel

Smelting furnace
  crucible
  reverberatory


  In-process fuel

Fluxing, chlorination
  fluoridation
SCC

3-04-001-08

3-04-001-09


3-90-OOX-99

3-04-001-01


3-90-OOX-99
3-04-001-02
3-04-001-03
3-90-OOX-99

3-04-001-04
3-04-001-05
                                             Pollutant(s)

                                             Particulates

                                             Particulates,
                                              hydrocarbons
                                             Particulates,
                                              hydrocarbons
                                             Particulates,
                                              hydrocarbons,
                                              combustion prod-
                                              ucts
                                             Particulates
Degassing

Hot dross processing
                    Particulates

                    Particulates
                         3-04-001-06

                         3-04-001-07

     The units for the SCC's are expressed in tons of metal pro-

duced.

     Figures 7.8-2 through 7.8-8 illustrate the standard NEDS

forms for these sources.  Entries in the data fields give infor-

mation common to secondary aluminum plants.  Information per-

tinent to coding the source is entered on the margins of the

forms and above or below applicable data fields.  Entries for

control equipment codes, other optional codes, emission factors,

and required comments minimize the need to refer to the code

lists.   Typical data values for operating parameters, control

equipment efficiencies, and other source information are shown on

the form  (or in the text) only to aid in rapid, approximate

checks of data submitted by the plant in a permit application or

                              7.8-10

-------
similar report.  Data entered in EIS/P&R and NEDS must be actual



values specific to and reported by the plant, rather than typical



values.  Contact the plant to validate or correct questionable



data and to obtain unreported information.  See Part 1 of this



manual for general coding instructions.



     Standard NEDS forms for crushing/screening and burning/dry-



ing are shown in Figures 7.8-2 and 7.8-3.  The codes for controls



generally used are entered to minimize the need to refer to



coding manuals; however, the coder must verify the controls that




are actually used.



     Figure 7.8-4 is a standard NEDS form for the sweating fur-



nace.  A combination of controls is used to reduce emissions.



The afterburner reduces hydrocarbons, and the fabric filter and



ESP reduce particulates.  Enter the code for afterburner under



primary control for hydrocarbons, where used; enter the code for



fabric filter or ESP under control for particulates, where used.



     Figure 7.8-5 is a standard NEDS form for the smelting



operation.  The two SCC codes possible are for the crucible or



reverberatory furnace.  The standard NEDS form for fluxing is



shown in figure 7.8-6.  There are two codes possible, depending



on whether chlorination or fluoridation is practiced.  At some



plants the smelting and fluxing are combined (carried out sequen-



tially in the furnace) and the exhaust is vented to a common



stack.  When this is the case, code two NEDS forms, one for



smelting and one for fluxing, using the same data for stack



height and diameter.  In most cases the emissions from both



operations are vented to the same control equipment; however, it



                              7.8-11

-------
is possible to have different control equipment and one common

stack.  The coder must determine the actual situation.

     Degassing is coded separately when it is accomplished by use

of nitrogen gas, by applying a vacuum, or by mechanical vibra-

tion.  Enter a comment stating which method is used.  Degassing

by use of chlorine or fluoride is considered part of fluxing.

Figure 7.8-7 illustrates a standards NEDS form for degassing.

     A standard NEDS form for hot dross processing is given in

Figure 7.8-8.  When emissions from this source are controlled, a

fabric filter or wet scrubber is used.


CODING EIS/P&R FORMS

      The Basic  Equipment Codes  (EEC's) for  each of  the emission

sources are  as  follows:

Source                        BEC

Crushing/screening           654,  575

Burning/drying                231

Sweating  furnace             942

Smelting  furnace              940,  941

Fluxing (chlorination and
   fluoridation)                982

 Degassing                     NO code*

 Hot dross processing          No code*
   As of September 1978.
                              7.8-12

-------
                   Figure  7.8-2.    Standard  NEDS  form  for  secondary  aluminum  -  crushing/screening.
00
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                 State!  Cot.ntv
                                   Point
                                   10
                      CRUSHING/SCREENING
                                             Boiler Design
                                              Capacity
                                             I0« BTU/nr
NATIONAL EMISSIONS DATA SYSTEM (NEDS)
  ENVIRONMENTAL PROTECTION AGENCY
      OFFICE OF AIR PROGRAMS


      Establishment Name and Address
                                                                                                                        POINT SOURCE
                                                                                                                          Input Form
                                                                                                                   Name of Person
                                                                                                                   Completing Fo»m_
                                                                                                   FORM APPROVE!*
                                                                                                   OMB NO 158-ROJ95
                                                                                                   Dai.	
                                                                        Height (HI
                                                                                     Temp (°FI
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                     Primary
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                                                                                                                             .2|U|MliS «|67
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                                                                                                              ESTIMATED CONTROL EFFICIENCY (M
                                                                                         EMISSION ESTIMATES I
                                                                 ALLOWABLE EMISSIONS Itons/vearl
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                                                                          COMPLIANCE
                                                                            STATUS
                                                                            UPDATE
                                                                                                                         (01(1
                                                                                                                                     ESTIMATION
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                                                                CONTROL REGULATIONS
                                                                                                                                      67163
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                                                          !t 11 !i 23 JO 31 3',
                                                                         34 3S 36 3i 38 39 (0 il
                                                                                                                                    61 67 63 63 70 71 72 73 7< 75 76 77

-------
           Figure  7.8-3.   Standard NEDS  form for  secondary  aluminum -  burning/drying.
00
 I
                                                          NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                           ENVIRONMENTAL PROTECTION AGENCY
                                                               OFFICE OF AIR PROGRAMS
POINT SOURCE

 Input Form
FORM APPROVED
OMB NO 1S8-R009S

D.I.,
                                                                                                         0000 IF HO COmON STACK
                                                                                                         UXX raiHT ID'S IF COMOH STACK
                                                   A*™. SCC WIT - TOUS PROOUCJ3
                                                  fut\. Pioc*«,      Houfl*      *r ;.
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                   IN-PROCESS FUEL
                                                   4-RESIOUAL OIL, 6-NATURAL GAS

-------
               "igure  7.8-4.     Standard   NEDS   form  for   secondary  aluminum   -  sweating   furnace.
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                                         Plant ID
                                         Number
                                        lOlll  12 13
                                                          °S
                                                     Zone  > 1! 20 11 22 23 24
                      ALLOWABLE EMISSIONS lloni/yearl
                 SOj             NO,
                                                        19 20'
                                                                       25 21121 29 30 31
                                                                                    32 33 34 35 36 37 38
                                                                                                    39)40 tl 42  43 44 45
                                                                       SCC/UN4T -  TONS METAL  PRODUCED^
                                                                         Fl Prcess                       •
                                                                                                                   46 47 41 49 50 51 52
                                                                                                                5COMPLIANCE
                                                                                                                M SCHEDULE
                                                                                                                                                59 60 61 62 63 64 65
                                                    COMPLIANCE
                                                      STATUS
                                                      UPDATE
                                                                                                                                              HlSJ
                                                                                                                                                       62163
Hi ?0|?l'7? 73T74 7S|76l
                                                                                                                                                                    61 69 70 7l|72 73 74J7S 76 77
                                                                                                       ESTIMATION
                                                                                                         METHOD
                                                                                                                                                                  67 6S 69 70
                                                                                                                                                                                 74 75 78 77
                                                                                                          CONTROL REGULATIONS

                                                                                                       Heq i      Reg 2    R«« 3
                                                                                                                                                           64 65 86 67lU
                                                                                                                                                                               73|74 75 76 77
                                                                                                                                    79|SO
                 Fuel Procesi
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                Operaii
                                                                       26 27 28 21 30
                                                                                       Maximum Design
                                                                                          Rut
                                                                                      33 34 3S 36 3; 38  39 J.O 41 42
                                                                                                             43 44 4i
                                                                                                                   Mwi Content
                                                                                                                   J6 :,' il 49 50
                                                                                                                                                 Comments
                                                                                                                              SI S2|S3|S4|5S|56Ts7r5« Sslsohl  'o 64 6S|66|67 Sl|69|70
                                                                                                                                                                           !
                                                                                                                       73 74 75 76 77,
                                                                                 -4-RESIDUAL  OIL, 6-NATURAL GAS
                                                                                  3ll32l33|34l35|36|37|38h9|40hl|Kh3|«|i5|
-------
                         Figure  7.8-5.   Standard NEDS  forms for  secondary aluminum -  smelting furnace.
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                                                               NATIONAL EMISSIONS DATA SYSTEM (NEOS)
                                                                 ENVIRONMENTAL PROTECTION AGENCY
                                                                     OFFICE OF AIR PROGRAMS
                                                                                                                 POINT SOURCE
                                                        FOPM APPROVED
                                                        OMB NO 158 nOO?5

                                                        Oitf	
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-------
                      Figure  7.8-6.    Standard  NEDS  form  for   secondary  aluminum  -  fluxing,
                                                                    NATIONAL EMISSIONS DATA SYSTEM (NEDS]
                                                                      ENVIRONMENTAL PROTECTION AGENCY
                                                                          OFFICE OF AIR PROGRAMS
                                                                    POINT SOURCE
                                                                      Input Form
FORM APPROVED
OMB NO. 158-HOO9S
Date
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                                             22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 3t 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60 61
                                                                          62S3H65«£6«6970n7273
                                                                                                                                0000 IF NO COMMON STACK
                                                                                                                                XXXX POINT ID'S IF COMMON STACK
                                                                                                                             60 61 62 63 64 55 66 67 SI 63 70 71 72 73 74 75 76 77
                                                                                           44 45 46 47 48 49 50 51 52 53 54
                                                                                                                ESTIMATED CONTROL EFFICIENCY (%)

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                                  EMISSION ESTIMATES (lom/yearl
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-------
                      Figure  7.8-7.    Standard  NEDS  form for  secondary  aluminum  -  degassing.
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NATIONAL EMISSIONS DATA SYSTEM (NEDS)
  ENVIRONMENTAL PROTECTION AGENCY
      OFFICE OF AIR PROGRAMS
                                                                                                                       POINT SOURCE
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-------
        Figure 7.8-8.  Standard NEDS form for secondary aluminum - hot dross processing.
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-------
GLOSSARY
Degassing - A process used to reduce or eliminate dissolved or
trapped gases.

Demagging - A process used to reduce the magnesium content of the
alloy.

Dross - The scum that forms on the surface of molten metals
largely because of oxidation, but sometimes because of the rising
of impurities to the surface.

Fluxing - Adding substances that absorb impurities or prevent the
formation of oxides in molten metal baths.

Pigs - Crude metal casted into blocks for storage, transporta-
tion, or remelting.

Smelting - Any metallurgical operation in which metal is separ-
ated by fusion from those impurities with which it may be chem-
ically combined or physically mixed.
                             7.8-20

-------
                  REFERENCES FOR SECTION 7.8


1   Compilation of Air Pollutant Emission Factors.  2nd edition.
    U.sT Environmental Protection Agency, AP-42, February 1976.

2.  Air Pollution Engineering Manual.  2nd edition.  U.S. En-
    vironmental Protection Agency.  AP-41, May  1973.

3   Midwest Research Institute.  Particulate Pollutant System
    Study, Volume III:  Handbook of Emission Properties.  EPA-
    22-69-104, May 1971.

4   PEDCo Environmental, Inc.  Environmental Assessment of  the
    Domestic Secondary Aluminum Industry.   (Working Paper)   EPA
    Contract No.  68-03-2477, July  1978.

5   Technical Guidance for Control of  Industrial  Process Fugi-
    tive Particulate Emissions.  EPA-450/3-77-010, March 1977.

6.  Billings, C.D.  (ed.).  Fabric  Filter Manual.   Chapter  IX.
    The Mcllvaine Company, Northbrook,  Illinois,  July  1978.

7.  Vatavuk, W.M.  National  Emission Data System  (NEDS)  Control
    Device Workbook.  U.S. Environmental Protection Agency,
    Publication No. APTD-1570, July  1973.

 8.  Aeros Manual  Series Volume  II:   Aeros User's  Manual.   EPA-
    450/2-76-029  (OAQPS No.  1.2-039),  December 1976.

 9.  Aeros Manual  Series Volume V:   Aeros Manual of Codes.   EPA-
     45/2-76-005  (OAQPS  No.  1.2-042),  April 1976.

10.  Standard Industrial Classification Manual.  1972  edition.
     Prepared by  Office  of  Management and Budget.   Available from
     Superintendent  of Documents,  Washington,  D.C.

11.   Loquercio,  P.,  and W.J.  Stanley.   Air Pollution Manual of
     Coding.   U.S. Department of  Health, Education, and Welfare.
     Public  Health Service  Publication No. 1956.  1968.
                             7.8-21

-------
       7.9  SECONDARY COPPER SMELTING AND ALLOYING

PROCESS DESCRIPTION
     In the secondary copper industry, copper is  recovered  from
scrap metal, which includes both copper and copper alloys.   The
processes used are determined by the type and quality of the feed
material.  Low-grade copper scrap,  which contains less than 30-
percent recoverable metal, is usually utilized in secondary smel-
ting, whereas clean, selected scrap including brass and bronze
may be melted (without smelting) to produce alloys.  Generally,
a secondary copper facility processes the less metal-rich feed
and produces a more refined product.  Alloy processors perform
fewer refining operations.

Secondary Copper Smelting
     Processes involved in copper recovery may be classified as
pretreatment, smelting, and refining.  Figure 7.9.1 presents a flow-
sheet depicting the major processes typically employed in a
secondary copper smelter, producing refined copper from low-grade
scrap.
     Copper-bearing scrap, for industry purposes, has been classi-
fied as either new or old.  New scrap is that produced in fabri-
cating finished products; for example, turnings,  borings, and
other waste from machining copper,  brass, and bronze.  Old scrap
consists mainly of obsolete, wornout, or salvaged articles such
as wire, plumbing fixtures, parts from electrical machinery,
automobiles, and domestic applicances.  Other materials with
copper values include slags, drosses, foundry ashes, and sweepings
from smelters and copper processing industries.  A detailed classi-
fication of copper-bearing scrap materials has been published
by the National Association of Secondary Materials Industries.
                             7.9-1

-------
LOW«RADE _
     SCRAP
IO
ro
1
?

t
SCRAP DR
3-04-O02-I
SCRAP DR>
3-04-O02
SCRAP OR
FUGITIVE EM
3-90-OOX
INPROCESS
0
BAGHOUSE 017 (991
VENTURI SCRUBBER 053 (651 * BA
CYCLONES 009 165) )

SCRAP FLU>< _
FUEL 	 *•
07 n j4\. 3-04-002-WW
ER PAHT<27^> CUPOLA
31 XS. 340-OOX-99
YER PART
-------
Specifications for the various classes have also been defined.
Copper wire and tubing constitute almost half of the scrap used
in the industry.

Scrap Metal Pretreatment
     Feed scrap may contain a great deal of nonmetallic material
including oil, grease, paint, insulation, rubber, and even
chemical? such as antifreeze.  The scrap is segregated for further
treatment by a variety of processes adapted to the considerable
number of input materials.  Generally, it is sorted according to
its copper content and cleanliness; clean scrap may be manually
sorted for charging directly to a melting and alloying furnace.
It is not unusual for this segregation to be performed prior to
shipment to the smelter, but a complete facility provides for
this operation.
     In general, pretreatment processes may be classified as
mechanical, pyrometallurgical (involving heat), or hydrometallur-
gical (involving water).  Their purpose is to concentrate the
valuable metals prior to smelting, refining, and alloying.
Mechanical methods are as follows:
     1.  Hand  sorting - Individuals sort the scrap as it  is
         unloaded before being routed to storage.
     2.  Stripping - Any process involving the mechanical
         removal of insulation from copper cable.
     3«  Shredding - Insulated wire is  reduced 1n size in a
         hammermi11, and conveyed pneumatically to a cyclone
         where the metal and  insulation are gravity-separated.
     4.  Magnets - Magnetic pulleys convey brass and bronze
         scrap and trap loose iron particles.
     5.  Briquetting - A powerful hydraulic press is used to
         reduce bulky scrap to small bales (briquettes).
Pyrometallurgical methods are as follows:
                             7.9-3

-------
     1.   Sweating -  The  separation  of  low-melting point
         metals,  such  as  lead,  solder, and  babbitt metal
         from the desired materials by heating.
     2.   Burning  - The removal  by  incineration of insula-
         tion from wire  scrap which, for some reason,
         cannot be mechanically separated.
     3.   Drying - A  process  employing  a  rotary kiln  to
         vaporize excess  cutting fluids  from machine
         shop chips  or borings.
     Hydrometallurgical  methods include  gravity  separation  by
flotation, leaching  with ammonium  carbonate or sulfuric  acid,
and recovery of copper from  the leachate by chemical processing.

Smelting
     Pretreated scrap containing between 10- and 30-percent copper
is normally smelted  in a cupola furnace  (Figure  7.9-2).   A cupola
furnace is essentially a vertical,  refractory-lined  cylinder open
at the top and equipped  with airports  at the bottom. Air is
supplied by a forced-draft blower.   Alternate charges of scrap,
coke, and limestone  are  placed  on  top  of a  burning  bed  of coke;
the metal melts and  is drawn off through a  tap-hole  and  spout
at the bottom of  the furnace.   Oxides  of copper  and  heavy metals
are chemically reduced.   Various impurities, such as iron, combine
to form a slag, which collects  on  top  of the molten  metal and  can
be drawn off separately.  A typical cupola  furnace  has  a capacity
of about 55  to 65 metric tons  per day,  producing so-called
"black" copper of about 70- to  80-percent purity.  The  impurities
may be sulfides of copper and  iron, as well as  other metals and
their oxides: tin, zinc, lead,  and others.
     In the  typical  system of  Figure  7.9-1, further smelting  and
refining are accomplished using a  reverberatory "holding" furnace,
a converter, and a reverberatory or rotary refining furnace.
These operations are  similar to those used in primary copper
smelting  (q.v.).   The contents of  reverberatory furnaces are  furnaces
                             7.9-4

-------
SPARK
ARRESTER
                      TAPPING SPOU)
                    BOTTOM PLATE
                  S1ND BOTTOM
     Figure 7.9-2  A Cupola  Furnace
                   7.9-5

-------
by radiation heat from burner flames, refractory walls and roofs.
The function of the holding furnace is to retain the melt until
a sufficient batch is accumulated as a charge to the converter
and to allow for tapping the slag.  (An electric-arc furnace can
also be used for this purpose.)
     The converter consists of a cylindrical steel shell which
can be rotated about its longtudinal axis.  An opening in one
side admits the molten charge and vents gases.  Air is blown
through the melt by means of a horizontal row of pipes, with
openings (called "tuyeres") which are below the liquid metal
when the furnace is rotated.  A silica flux is added to remove
iron from the metal, while zinc and any sulfur are converted to
their respective oxides by the air which  is blown in.
     The product from the converter is "blister" copper, usually
90- to 99-percent pure.  This material may  be poured and cast,
or  it may be transferred in the molten state  to another furnace
for a final pyrometallurgical process  known as  "fire refining."
     Feed containing low-copper values can  also be smelted  in
electric crucible furnaces, using oxygen  in place of air for
oxidation.

 Refining
      Blister copper  is,typically,  further purified by  fire
 refining,  to about  the  level  of  99.9-percent  purity.   Electroly-
 tic refining may be  done as  an  additional step  to produce elec-
 trolytic  copper.  These processes are essentially the  same  in
 secondary  smelting  as  in primary smelting of copper.
      Fire-refining  furnaces are,  typically, reverberatory fur-
 naces,  often  of a rotary type.   Capacities usually range from
 about 100  to   35C  metric  tons.   In the  furnace,  air is blown
 through the molten metal  to oxidize impurities  which, as oxides,
                              7.9-6

-------
are removed in the slag which is skimmed or poured off.   Copper
oxide, formed to the extent of less than 1  percent of copper, is
reduced by "poling" (submerging wooden poles in the molten metal)
or by supplying a reducing atmosphere of gas (by fuel-rich combus-
tion).  The usual sequence of events in fire refining is (1)
charging; (2) melting; (3) skimming; (4) blowing; (5) adding
fluxes; (6) reducing; (7) reskimming; and (8) pouring.
     Electrolytic refining separates impurities from the copper
by electrolysis in a solution bath containing copper sulfate  and
sulfuric acid.  Metallic impurities form a sludge ("slime") which
is removed and may be treated for recovery of precious metals.

Melting and Alloying
     To produce bronze or brass rather than copper, an alloying
operation is required.  Where high-grade scrap is used, smelting
may be unnecessary.  Figure 7.9-3 presents a flow diagram for a
typical operation of this kind.
      In the case illustrated, scrap as received is manually and
mechanically sorted to segregate pure copper, especially copper
wire, from copper alloys.  Insulated wire is fed to a wire-burner,
an incinerator in which combustible insulation is removed.  Brass
and bronze scrap is sweated to remove low-melting metals such as
solder, lead, and babbitt metal.  The cleaned copper and alloys
are then melted  in an alloying furnace.  Zinc and other metals
may be added to  bring the resulting mixture  to the desired final
composition.  Fluxes are  added  to  the mixture  to remove  impuri-
ties  and to  protect the melt  against oxidation.  Air or  oxygen may
be blown through the melt to  adjust  the  composition  by oxidizing
excess  zinc.  With  zinc-rich  feed,  the  zinc  oxide  particulate
loading  in  the exhaust  is often  recovered  in a process baghouse.
                              7.9-7

-------
              LEGEND


      EMISSION FACTOR"
O      EMISSION FACTOR NOT DEVELOPED
      FOR THIS PROCESS

 009 (66.0) DENOTES CONTROL EQUIP. CODE
 4            WITH EST EFF. SHOWN IN ( I

X    DENOTES FUGITIVE EMISSIONS

f^\    DENOTES A STACK
                                                                                           BAGHOUSE 016 (991
                                                                                           VENTURI SCRUBBER 053 165)
IO
CD
                        * IN POUNDS PER SCC UNIT
    HIGH GRADE SCRAP -

                  SCRAP METAL
                 PRETREATMENT
                                                                                                           LEAD, SOLDER.
                                                                                                           BABBITT METAL
                                                                  FUEL
                                                                   AIR
                                                BRASS
                                                AND
                                                BRONZE
                                                SCRAP
                                                                                   3-04-O02-09               ..
                                                                               SWEATING FURNACE  PART  O»
                                                                                   3-04402-33
                                                                          SWEATING-FUGITIVE EMISSIONS   PART
                                                                                    3-90-OOX-99
                                                                                 INPROCESS FUEL
                                                         COPPER SCRAP
                                                                 FUEL-
                                      3-04-002-30
                                     SCRAP METAL
                                    PRETREATMENT
                                                                                           AFTERBURNER 021 (90)
                                                                                           SCRUBBER 003
ww
14
15
35
19
37
20
21
23
24
38
MELTING AND ALLOYING FURNACES
REVEHBERATORY-COPPER CHARGE
REVERBERATORY-BRASS/BRONZE CHARGE
REVERBERATORY-FUGITIVE EMISSIONS
CRUCIBLE/POT-BRASS/BRONZE CHARGE
CRUCIBLE/POT-FUGITIVE EMISSIONS
ELECTRIC ARC -COPPER CHARGE
ELECTRIC ARC-BRASS/BRONZE CHARGE
ELECTRIC INDUCTION-COPPER CHARGE
ELECTRIC INDUCTION-BRASS/BRONZE CHARGE
ELECTRIC INDUCTION-FUGITIVE EMISSIONS
PARTICULATE
EMISSIONS FACTOR
5.10
36.00
6.27
21.00
0.49
5.00
11 00
7.00
20.00
0.14
                                                                                            FUEL-
                                                                                            FLUX-
                                                      UNDESIRED SCRAP
                                                                  3-04-002418
                                                                WIRE BURNER   PART
                                                                  3-04-002-32
                                                                WIRE BURNER
                                                              FUGITIVE EMISSIONS   PART<137^
                                                                  3-90-OOX-99
                                                                INPROCESS FUEL
      3-04-002-WW
MELTING AND ALLOYING
       FURNACE
       3-90-OOX-99
    INPROCESSFUEL
                                                                                                                                                                         3 04«>2 39               /\
                                                                                                                                                                    CASTING OPEKATIONS   PART  £015
                                                                                                                                                  SLAG TO DUMP
                                                                   Figure 7 9-3.  High Grade Brass and Bronze Alloying
                                                                                          79-8

-------
     Brass and bronze shapes for working, such as slabs and
billets, are usually produced in large reverberatory furnaces,
of the type also used for secondary smelting and copper recovery.
In smaller operations and to make commercial castings, the metals
are melted in crucible furnaces, pot furnaces, or electric fur-
naces, both arc and induction types.

Casting
     The final step is always casting of the metal into desired
form.  Blister copper is sometimes poured into water for quenching
to produce copper shot, but is usually either transferred in the
molten state to a refining furnace or cast into ingots.  Fire-
refined copper is cast into wirebar, anodes, and cathodes as
well as ingots.
     Brass and bronze are more often cast into special shapes.
The mold, made of cast iron or similar material, is dusted with
charcoal before filling, to facilitate removal of the solid
casting.  After the mold is filled, exposed metal surfaces are
sometimes dusted with charcoal, to reduce skin oxidation due to
oxygen from the air.

Furnace Types
     Furnaces of many types are used in secondary copper operations
and in brass and bronze melting and alloying.  In recovery of copper
from scrap having relatively low copper content, the charge is
commonly treated in a blast furnace or cupola, where heavy-metal
oxides and sulfides are reduced.   Reverberatory furnaces are used
as holding furnaces for the cupola melt,  and sometimes in fire
refining.   Converters are used to oxidize sulfides, zinc, and base
metals by blowing air through the melt.   These and various other
types of furnaces,  frequently encountered in the secondary copper,
brass, and bronze industries,  are described  in the following para-
graphs.
                             7.9-9

-------
Blast Furnace or Cupola
     Although these names are sometimes used interchangeably,
the cupola is generally considered to be a smaller variety of
blast furnace.  The principles of operation are essentially the
same, but the larger furnaces are more common in primary smelting,
where metal is recovered by reducing oxide or sulfide ores. The
cupolas, commonly used in the secondary copper industry, recover
metal from skimmings, slags, and scrap metal in a reducing atmos-
phere provided by the combustion of coke.
     Blast furnaces and cupolas consist essentially of vertical,
refractory-lined cylindrical shells  (also known as "shafts," from
which these furnaces are sometimes called "shaft furnaces") open
at the  top and equipped with air  blowers at the bottom.  The scrap
is intermingled or  layered with coke  and limestone and heated by
combustion.   Molten metal and slag may be tapped separately from
the base of  the furnace, but more commonly  both are  continuously
tapped  into  a "holding"  furnace where they  are  separated.  This  is
usually a stationary  reverberatory  furnace.

Reverberatory Furnaces
     A  reverberatory  furnace operates by  radiating heat  from its
burner  flame, roof, and walls onto  the material being  heated.
Combustion of fuel  occurs directly  above  the molten  bath;  transfer
of heat is accomplished  almost  entirely by  radiation.
      Reverberatory furnaces  are  available  in many  types  and
designs.  Their use will depend  on  specific job requirements,
 such as the  nature and quantity  of  the charge  to  be  handled.
The largest  such  units are  open-hearth furnaces,  which range  in
                           7.9-10

-------
capacity from about 40 to about 500 metric tons.   In the
secondary copper, bronze, and brass industry, such units are often
used as holding furnaces to accumulate and separate the molten
metal ("black" copper)  and slag tapped from the cupola furnace.
They may also be used in fire refining.
     Large open-hearth furnaces are built with heat regenerators,
consisting of brick checkerwork, which absorb heat from the
effluent gases and transfer it to incoming air.  The fuel is oil
or gas.  The charge is introduced through refractory-lined doors
in the front wall; molten metal and slag arc removed through tap-
holes in the rear.
     For melting and holding smaller amounts of copper, brass,
and bronze, cylindrical reverberatory furnaces are common.  (See
Figure 7.9-4.) These are fired.through tangential nozzles and charged
through end doors on top openings.  They usually utilize rotary
tilting mechanisms to facilitate pouring of the molten contents.

Rotary Furnaces

     A more elaborate type of reverberatory furnace, commonly
called a "rotary" furnace, not only tilts for charging and pouring,
but also rotates during the melting period to improve heat
transfer.  (Figure 7.9-5.) Two types are common.  One is charged
through the furnace, opposite the burner.  The other has a side
charge door at the center through which charging, skimming, and
pouring operations are conducted.

Converters
     A converter is basically a cylindrical reverberatory furnace,
mounted to tilt about its longitudinal axis and modified to permit
blowing air through the melt.  Illustrations of the copper conver-
ter and copper converter operation are shown in Figures  7.9-6 and 7.9-7
respectively.  A side charge door  is used for  charging,  skimming,
and pouring.  Air  is supplied through  a  header along the back of
the cylinder  (opposite  the charge  door)  from which a horizontal
row of tuyere pipes extend into  the interior of the vessel.
                              7,9-11

-------
Figure  7.9-4.   Gas-Fired  Cyclindrical  Reverberatory  Furnace
                          7.9-12

-------
Figure 7.9-5.  Rotary-Tilting-Type Reverberatory Furnace
       Venting to Canopy Hood and Stack Vent
                        7.9-13

-------
                            OFF-GAS
TUYERE
 PIPES
                                                            SILICEOUS
                                                             FLUX
                          PNEUMATIC
                          PUNCHERS
                    Figure  7.9-6.  Copper Converter
                                 7.9-14

-------
Exhaust Hood
   CHARGING
                         BLOWING
                                              SKINNING
      Figure 7-9-7  Copper Converter Operation
                       7.9-15

-------
Crucible Furnaces
     Crucible furnaces are indirect-fired furnaces having capaci-
ties of about 10 to 1,000 kilograms.  They are used to melt metals
having melting points not above 1,400°C (2,500'F).  The covers
of the crucible furnaces are constructed of materials similar to
the inner shell lining and have a small hole over the crucible
for charging metal and exhausting the products of combustion.  The
crucible rests on a pedestal in  the center of the furnace and is
commonly constructed  of a refractory material such as a clay-graphite
mixture or  silicon carbide.
      Crucible  furnaces  are  classified  as  tilting, pit,  or stationary
 furnaces.   All  types  are  provided with one  or more  gas  or oil
 burners  mounted near  the  bottom of  the unit.  Flames  are directed
 tangentially around  the inside of the  furnace.   The crucible is
 heated both by radiation  and by contact with  the hot gases.

 Pot Furnaces
      Pot furnaces are indirect-fired furnaces used to melt metals
 having melting points not above 800°C  (1,400°F).  These furnaces
 may be cylindrical or rectangular and  consist of an outer shell
 lined with  refractory material, a combustion chamber,  and a pot.
 The pots are made of pressed  steel, cast steel, or cast iron with
 flanged tops.  The flange  rests on the furnace wall, holds  the
 pot  above  the  furnace  floor,  and seals the contents  of the  pot
 from the  products of combustion of the fuel  used.   The shape of
  the  pot depends upon the operation to be conducted.

  Electric Furnaces
       Most pyrometallurgical operations can be  conducted with the
  use of electricity  rather than fuel for heating.  Major advan-
  tages of the electric furnace over fuel-fired furnaces are furnace
                               7.9-16

-------
atmosphere control and high-temperature operation.  Temperatures
as high as 6,000°F are possible for special processes.
     Resistance furnaces are used mainly for ferroalloys.  The
other three types of electric furnaces are described in following
paragraphs.

Direct-Arc Furnaces
     In the direct-arc furnaces, many and varied arrangements are
used to heat the metal charge, but radiation between arc and the
metal batr, is the principal method.  Here, the heat is generated
by radiation from the arc as well as from the resistance heat
effect with the bath, as shown in Figure 7.9-8.   Graphite and carbon
electrodes are usually used and are spaced just below the surface
of the slag cover.  The current passes from one electrode through
the slag, the metal charge, the slag, and back to the other elec-
trode.  In some arrangements, the current is carried from the
metal charge to the earth.   The slag serves a protective function
by shielding the metal charge from vaporized carbon and the
extremely high temperatures at the arc.

Indirect-Arc Furnaces
     In the indirect-arc furnaces, the metal charge is placed
below the electrodes, and the arc is formed between the electrodes
and above the charge (Figure 7.9*8).   Indirect-arc furnaces  are  used.
mainly in the steel industry.  One of the common smaller furnaces
is the indirect-arc rocking furnace, in which an automatic
rocking action of the furnace is employed to ensure a homogeneous
melt.  This is done by mounting the refractory-lined steel shell
on cog bearings so that the furnace may be rocked through a 200°
range.  Radiated heat from the indirect arc  and conduction from
the preheated refractory lining initially melt small scrap,
forming a pool of molten metal  at the bottom of the furnace.  Then


                             7.,9-17

-------
                          ELECTRODES
         DIRECT
                                       INDIRECT
Figure 7.9-8.   Principles  of Operation of  Direct-Arc and
                 Indirect Arc Furnaces
                           7.9-18

-------
the rocking action is initiated,  and the molten metal  washes
against the refractory, picking up additional  heat, which is  trans-
ferred by convection and radiation to the larger pieces of metal.
During the heat, the rocking action is advanced gradually to
avoid a sudden tumbling of cold metal, which could fracture the
graphite electrodes.

Induction Furnace
     The induction furnace consists of a crucible within a water-
cooled copper coil  (Figure 7.9-9).  An alternating  current in the  coil
around the crucible  induces eddy  currents in the metal charge and
thus develops heat within the mass  of the charge.   Heating is
rapid  and  uniform and  temperature can be accurately controlled.
High-frequency  induction  furnaces are well  adapted  to  copper-rich
alloys (bronzes), but  low-frequency induction  furnaces are more
 suitable for zinc-rich alloys  (brass).

 EMISSIONS
      The principal  air contaminants emitted in secondary copper
 smelting and recovery are various forms of  particulate matter.
 These include organics from the pretreatment and metal oxides from
 the pyrometal.urgical  processes.  Some gases,  including  hydrogen
 chloride and sulfur dioxide,  may be released by burning of insula-
 tion.  Carbon monoxide is emitted in the operation of cupola fur-
 naces.
 Scrap Metal Pretreatment
      Copper reclamation from insulated wire is commonly accomplished
 in  single-chamber incinerators such as tepee burners, which may be
 portable to cover piled scrap.  A great variety of materials com-
 poses the  combustible  insulation: rubber,  paper, cotton, silk,
 plastics,  paint  and  varnish, and others.   During combustion, in the
                               7.9-19

-------
Figure 7.9-9.   Low-Frequency Induction Furnace With Fixed Hood
                    7.9-20

-------
absence of control equipment, black smoke is not uncommon, accom-
panied by disagreeable odors, inorganic materials, and oxygenated
hydrocarbons.  If the insulation contains polyvinyl chloride,
hydrogen chloride is emitted.  Sulfur dioxide is one product of
the burning of rubber insulation and of some synthetic rubbers.
In published results of one test,   particulates recovered from
wire-burning in a single-chamber incinerator amounted to 178 kilo-
grams per metric ton (356 pounds per ton) of combustibles.  The
combustibles constituted 35 percent of the charge.
     Scrap driers consisting of rotary kilns are often used to
burn off oil and volatiles from turnings, borings, and other waste
from machining.  This process can cause discharge of dense smoke
accompanied by volatile hydrocarbons and oxygenated materials.
     Mechanical pretreatment, such as stripping, shearing, crushing,
shredding, and briquetting, is likely to be a source of fugitive
dust in copper recovery operations, both for secondary smelters
and for alloying operations.  Such emissions have not been quanti-
tatively evaluated.

Cupola Furnaces
     Air contaminants emitted from cupola furnaces are (1) gases,
(2) dust and fumes, and (3) smoke and oil vapor.  Typically, the
gases may contain 10 percent or more of carbon monoxide.  Dust in
the discharge gases arises from dirt in the feed material  and from
fines in the coke and limestone charge.  Smoke and oil  vapor arise
primarily from, the partial combustion and distillation of oil
from greasy scrap charged to the furnace.

Reverberatory Furnaces
     Reverberatory furnaces are used both for holding the  melt
from the cupola furnace preparatory to loading the converter
with molten copper, and for melting and alloying in the production
of brass or bronze.
                             7.9-21

-------
     Air contaminants from reverberatory furnaces  include  gases,
smoke, fumes, and dusts.   The particulate matter varies  according
to the fuel, alloy composition,  melting temperature,  type  of  fur-
nace, and various operating procedures.   In  addition  to  fly ash,  carbon,
and mechanically produced dust,  the emissions  generally  contain
fumes resulting from condensation and oxidation of the more vola-
tile elements, including zinc and lead.

Converter Emissions
     Emissions of air contaminants from converter  operations  occur
predominantly during the air-blowing process,  in which zinc and
sulfur are oxidized.  In secondary smelting, sulfur is usually
a  rather minor constituent of the melt, in contrast to the major
fraction encountered in primary smelting of sulfide ores.   Fuel
use  in this operation is also relatively minor,  as the oxidation
of zinc, iron, and sulfur provides most of the necessary heat;
fuel-associated contaminants are therefore minimal.  However, if
the  material charged to the converter is not in  the molten state,
fuel combustion is required in order to melt it  and typical  fuel-
combustion contaminants (i.e., sulfur dioxide, nitrogen oxides,
carbon monoxide, fly ash) are emitted during melting.
     During charging and pouring, significant fugitive emissions
are  likely to occur.  These emissions have not been quantitatively
evaluated.

Emissions in Fire-Refining
      Fire-refining generates relatively little sulfur dioxide or
metallic oxide particulates, since the blister copper charged is
at least 90-percent  pure.  Poling, however, often produces black
soot, which  may be of concern.
                             7.9-22

-------
CONTROL EQUIPMENT
     Due to the wide variety of participates emitted,  many
different control strategies are used.
     Wire burning generates large amounts of particulate matter
in the form of unburned combustibles.   These emissions are most
effectively controlled by a direct flame afterburner.   If the
afterburner combustion temperature is  maintained at a  minimum of
1,000°C (1,800°F)5 an efficiency of 90 percent can be  expected.
If the insulation contains polyvinyl chlori  ie, hydrogen chloride
gas will be a contaminant.  An afterburner will not control this
contaminant, but it can be reduced by a water scrubber.
     Particulate emissions associated with the drying  process
are controlled by a variety of control  devices.  Drying tempera-
tures of 70° to 150°C (150° to 300°F)  are low enough to allow a
baghouse to operate without preceding of inert gases.  Baghouse
efficiencies of 99 percent and above can be anticipated.  Other
means of control used include cyclones (60-  to 75-percent
efficiencies) and wet (venturi) scrubbers with efficiencies of
approximately 65 percent.
     Emissions associated with the charging of scrap to melting
furnaces can be reduced by turning off the burners during charging.
The technique has several effects.  It reduces the volume of
escaping air which can entrain contaminants.  If the furnace
operates in conjunction with a baghouse, the operation of the
baghouse blower with the burner off actually produces  a negative
pressure in the furnace, further reducing emissions.  The escaping
fumes from charging and pouring are commonly captured  by being
drawn upward through ducts to the same control equipment which
services the furnace exhaust gases.
     There are many possible systems for the control of the metal
oxide fumes escaping from the furnace during melting.   Baghouses,

                              7.9-23

-------
electrostatic precipitators, and wet scrubbers are most common.
Due to the small size of the metal oxide particles to be captured
(0.3 to 0.5 microns), the baghouse is the most effective device,
reaching efficiencies well in excess of 99 percent.
     The temperature of the exit gas from the melting furnace is
approximately 1,200°C, which would destroy a baghouse.  Several
practices are used to cool the gases to temperatures the baghouse
can handle (below 260°C).  Figure 7, 9-10 shows a two-stage cooling
system consisting of water-jacketed coolers followed by radiant
cooling which reduces the baghouse outlet temperature to 180°C
(350°F).
      Although electrostatic precipitators are  reputed to be
extremely effective  for  collecting particles  in the  size range
exhibited by these metal  oxides,  experience has shown that collec-
tion  efficiency for  lead and  zinc oxides  is low,  perhaps due  to
unusual  resistivity  in  these  systems.   Electrostatic precipitators
have  been  little used  in control  of  furnace emissions,  as their
optimum  application  appears  to  be for  larger  gas  flow rates.
      Wet scrubber installations  must be restricted to applications
where the  particle  size range is above 1  micron and even then
 collection  efficiencies are only in  the 50-  to 65-percent  range.
                               7.9-24

-------
CODING NEDS FORMS

     The emissions sources  in a secondary  copper smelter  and  in
brass or bronze alloying are:

     Source

Scrap Dryer

Wire Burning (Incinerator)

Sweating Furnace

Blast Furnace/Cupola
  Charge w/Scrap Copper
  Charge w/Wire
  Charge w/Copper Brass

Reverberatory Furnace
  Charae w/Cooper
  Charge w/Brass/Bronze

Rotary Furnace

Crucible/Pot Furnace

Electric Arc Furnace
  Charge w/Copper
  Charge w/Brass/Bronze

Electric Induction Furnace
  Charge w/Copper
  Charge w/Brass/Bronze

Fugitive Emissions
  Scrap Pretreatment
  Scrap Dryer
  Wire  Incinerator
  Sweating  Furnace
  Cupola Furnace
  Reverberatory Furnace
  Rotary Furnace
  Crucible  Furnace
  Electric  Induction Furnace
  Casting  Operations
     SCC

3-04-002-07

3-04-002-08

3-04-002-09
3-04-002-10
3-04-002-11
3-04-002-12
3-04-002-14
3-04-002-15

3-04-002-17

3-04-002-19
3-04-002-20
3-04-002-21
3-04-002-23
3-04-002-24
3-04-
3-04-
3-04-
3-04-
3-04-
3-04-
3-04-
3-04-
3-04-
3-04-
002-30
002-31
002-32
002-33
002-34
002-35
002-36
002-37
002-38
002-39
                       Pollutants

             Particulates,  S09, NO, HC, CO
                             £    A

             Particulates,  S09, NO. HC, CO
                             L.    X

             Particulates,  S02, NOX, HC, CO
             Particulates,  S02
             Particulates,  S02,
                   NO
                   NO
                     x'
          HC,
          HC,
             Parti culates,  S02,
             Particulates,  S02,
Particulates
Particulates,
Particulates,
Particulates,
Particulates,
Particulates,
Particulates,
Particulates,
Particulates,
Particulates
S09,
so;,
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so;,
so?,
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                                      V
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                             L-     X


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             Particulates,  SOp,  NO*   HC,  CO
                             Li     A

             Particulates,  SOp,  NO.  HC,  CO
                             C.     A

             Particulates,  S09,  NOV,  HC,  CO
                             £     X


             Particulates,  S09,  NO ,  HC,  CO
             Particulates,  S02,  NO*,  HC,  CO
                   NO ,  HC,  CO
                   NO*  HC,  CO
HC, CO
HC, CO
HC, CO
HC, CO
HC, CO
HC, CO
HC, CO
HC, CO
                                  7.9-25

-------
CODING EIS/P&R FORMS
     The EEC's for use in EIS/P&R forms are shown herein:
                   Source^                    BEC
     Blast furnace                           H2
     Crucible furnace                        102
     Cupola furnace                          112
     Electric induction furnace              132
     Reverberatory  furnace                   162
     Rotary furnace                          172
     Electric arc furnace                    122
     Scrap dryer                             192
     Wire burner
                                   7.9-26

-------
                                                                Exhaust Manifold 177°C;350°F)
                                                                                                      Exnzust Sta
                                                                                                  5'jctiori Fan
Figure  7.9-10.   Systems  Cooling  Exhaust Gas  Prior to Baghouse Entry

-------
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ptant ID NATIONAL EMISSIONS
<;i»!* County AQCR Number CNV/i RftNMFlMTAl PF
1 l 3 4 5 6 7 t 9 10 11 12 13 OFFICE OF AIP
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ff ALLOWABLE EMISSIONS Itoni/yearl
re "5|
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" 42~ IT 44" 45 46 47 46 45 50 5 5? 53 54 55 56 57 58 59 60 61 62 63 64 65 66 67 61 69 70 71 72 J
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NATIONAL EMISSIONS DATA SYSTEM (NEDS)
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-------
GLOSSARY

Alloy - Any substance having metallic properties and consisting
     of two or more elements; with few exceptions the components
     are usually metallic elements.

Anode - The positive terminal of an electrolytic cell; cast in
     copper for use in electroplating or for electrolysis.

Arc Furnace - A furnace used to heat materials by the discharge
     of electricity from electrodes.

Black Copper - The more or less impure metallic copper (70- to
     99-percent copper) produced in blast furnaces.

Blister Copper - Impure copper (98.5 to 99.5 percent) product
     of converters, having a blistered appearance.

Crucible - A refractory vessel or pot used in a furnace for
     melting or calcining.

Cupola - A vertical cylindrical furnace for foundry use; the
     metal, coke, and flux are put into the top of the furnace
     onto a bed of coke through which air is blown.

Dross - An impurity, usually an oxide, formed on the surface of
     a molten metal.

Flotation - A process used to separate particulate solids by
     causing one group of particles to float; utilizes differences
     in surface chemical properties of the particles, some of
     which are entirely wetted by water while others are not.

Flux - A substance used to promote the fusing of minerals or
     metals, and certain chemical reactions.

Hydrometallurgical - Treatment of ore to recover pure metal by
     wet processes.

Indirect-fired furnace - A fuel-fired furnace in which melt is
     contained in a heated vessel and is not contacted by the
     flame.

Induction Furnace - An electric furnace in which heat is produced
     in a metal charge by electromagnetic induction.

Ingot - A solid metal casting suitable for remelting or working.
                             7.9-40

-------
 Leachate - The material  removed from a mixture by leaching.

 Leaching - Dissolving soluble minerals out of an  ore by use  of
      percolating solutions such as  acids.

 Poling - Insertion of wood poles into a molten metal  bath,
      producing a reducing atmosphere by destructive
      distillation.

 Pyrolysis - The breaking  apart of complex  molecules  into  simpler
      units by the use of  heat, as in the pyrolysis of heavy  oil
      to make gasoline.

 Pyrometallurgical  -  Treatment of ore to recover pure  metal by
      high-temperature processes.

 Refining - Any process used  to improve  the  purity of  a  metal to
      meet product specifications.

 Reverberatory Furnace - A furnace in  which  the  charge  is  heated
      by direct contact with  flame and  by radiation from furnace
      walls.

 Rotary  Furnace -  A cylindrical  furnace  which can be rotated about
      its  (horizontal) cylindrical axis.

 Shaft Furnace  - A vertical,  refractory-lined cylinder in which a
      fixed  bed  (or descending  column) of solids is maintained
      and  through which an ascending stream of hot gas is forced.

 Shot  -  Product made by pouring metal  in finely divided  streams;
      particles solidifying during descent and are cooled in a
      tank of water.

 Slag  - A  nonmetallic product resulting from the interaction of
      flux and  impurities   in the smelting and refining of metals.

 Smelting - The heating of ore or scrap metal mixtures accompanied
      by a chemical change resulting  in the  formation  of liquid
     metal matte.

Tuyeres - An opening in the shell and refractory lining of a
      furnace through which air is forced into the  melt.

Wirebar - Cast copper ingots  used for the manufacture of wire.
                             7.9-41

-------
REFERENCES

Air Pollution Aspects of Brass and Bronze Smelting  and Refining
Industry.  Brass and Bronze Ingot Institute and National  Air
Pollution Control Administration.  PB 190295.   November 1969.

Air Pollution Engineering Manual, Second Edition.   EPA Publication
No. AP-40.  May 1973.

Development Document for Proposed Effluent Limitations Guidelines
and New Source Performance Standards for the Secondary Copper Sub-
category of the Copper Segment of the Nonferrous Metals Manufacturing
Point Source Category.   U.S. Environmental Protection Agency, Office
of Water and Hazardous Materials, Effluent Guidelines Division,
Washington, D.C. November 1974.

Lauber,  D.W. Conley, and D. Barshield, Air Pollution Control  of
Aluminum and Copper  Recycling Processes.   Pollution Engineering.
p. 23-26.  December  1973.

Multimedia Environmental Assessment  of the Secondary Nonferrous,
Metal  Industry,  Volume  II.   Industry Profile.   Final Draft.  Radian
Corporation, Austin, Texas.   Prepared for  the  U.S. Environmental
Protection Agency,  Industrial and  Environmental Research Laboratory,
Cincinnati,  Ohio under  Contract  No.  68-02-1319.  June  21,  1976.

Parti oil ate  Pollutant System Study,  Volume III:  Handbook  of
Emission Properties. Midwest Research  Institute,  Kansas City,
Missouri   Prepared for the U.S.  Environmental  Protection  Agency,
Air  Pollution  Control Office, Durham, North Carolina  under Contract
No.  CPA 22-69-104.   May 1,  1971.
                               7.9-42

-------
                 7.10  GRAY IRON FOUNDRIES





PROCESS DESCRIPTION



     Foundries produce castings for automotive parts,  light




and heavy machinery, pipe, and a wide range of miscellaneous



products.  The process involves melting scrap metal and/or




pig iron (crude iron in the form of blocks weighing about



100 pounds) and pouring the molten metal into prepared



molds.  The two major categories are "gray iron" foundries



and "steel" foundries.  Both gray iron and steel consist



mostly of elemental iron, but the carbon contents differ.




Gray iron contains  2 to 4 percent carbon, and steel contains



1 percent or less.  Gray  iron contains various amounts of




other elements, generally less than 1 percent.  Steel may



also contain alloying elements.  The term "cast iron" is



sometimes used in referring to both "gray iron" and "steel"



castings.  Such terms as  "malleable," "white," and "nodular"



iron are used to describe gray iron castings with specific




properties.



     Figure 7.10-1  illustrates the process flow in a typical



gray iron  foundry.  More  than  80 percent of  the U.S. instal-




lations  use a cupola  furnace to melt the raw materials.



Cupola capacities  range  from 1 to  50 tons of melted metal
                               7.10-1

-------
                                                                                             Figure   7.10-1.     Gray   iron   foundry.
                                                                           9
                                                                                       WET CAP 003(53)
                                                                                       VENTURI SCRUBBER   051(99)
                                                                                      MED.  ENERGY SCRUBBER  002(91)
                                                                                      HI  TEMP  FABRIC FILTER  016(99)
                                                                                      MEO EfFlC. ESP  Oil (93)

                                                                                    AFTERBURNER  021(94)
                                                                                                                            HI EFFIC. GRAVITY COLL 004(75)
                                                                                                                            HED.  EFFIC. CfUWm COLL OOS(50)_
                                                                                                                            HI EFFIC. CENT  COLL  007  (95)
                                                                                                                            LO TEMP. FABRIC FILTER 018(99)
                                                                              PART.JLJ
                                                                              co   (Tit;
                                 PART.O
                                            INPROCESS
                                              FUEL-
                                              COKE
                            COKE
                                              PART. O      ^_.

                                       FROM  CHARGING AND TAPPING
         SCMT NETAL
o
N3
       PART  0        •+-

FROM CHARGING AND TAPPING
                                              PART. O       <-

                                       FROM CHARGING AND TAPPING
                                               	jt      ' *—>
                                                    FROM CHARGING  AND TAPPING
                                                                                                                                                     MED. ENERGY WET SCRUBBER 002
                                                                                                                                                     LO. TEMP.  FABRIC FILTER 018
                                                                                                                                                                                                                                   9 P/WT.0

                                                                                                                                                                                                                                       KC 0 FROM SURFACE
                                                                                                                                                                                                                                                COATING
                                                                                                                  POURING LADLE
                                                                                                                                               POURING
FABRIC  FILTER 017 (95)
ESP 011(95)
VENTURI SCRUBBER
 Or>«99>
                                                                                    FABRIC FILTER  017'95)
                                                                                    ESP 011(95)
                                                                                    VENTURI SCRUBBER
                                                                                    053(99)
                                                                                                                                                                                                      3-90-004- 99 RESD  OIL
                                                                                                                                                                                                      3-90-005-99 DIST. OIL
                                                                                                                                                                                                      3-90-006-99 NAT. GAS
                                                                                                                                                                                                      INPROCESS FUEL
                                                                                                                                                                                   CYCLONE 005
                                                                                                                                                                                   FABRIC FILTER 018
                                                                            ! PART. (2)
                                                                             3-90-004- "RESD. OIL
                                                                             3-90-005- 99DIST. OIL
                                                                             3-90-005- 99RAT. GAS
                                                                                IOCESS FUEL
                                3-90-Qi
                                INPROC
                                                                                                                                                                     SANO GRINOING/HANDLINS
                                                                                                                                                                     IN  MOLD AND CORE MAKING
                                                                                                                             LEGEND

                                                                                                                             Q EMISSION  FACTOR*

0                                                                                                                                 EMISSION  FACTOR NOT DEVELOPED
                                                                                                                                 FOR THIS  PROCESS

                                                                                                                             009 (66.0) DENOTES CONTROL tOUIP.
                                                                                                                             .           CODE  WITH EST. EFF.  SHOWN
                                                                                                                             f          IN (  )
                                                                                                                                                                                                                 O
DENOTES FUGITIVE
EMISSIONS

DENOTES A STACK
                                                                                                                                                                             IN POUNDS PER SCC UNIT
                                                                      3-04-003-02

                                                                     REVERBERATORY
                                                                     3-90-004-99 RESD.  OIL
                                                                     3-90-005-99 DIST.  OIL
                                                                     3-90-006-99 NAT  6AS^
                                                                     INPROCESS  FUEL

-------
per hour;  over 60 percent operate in the range of 3 to 11
tons per hour.3  The other types of furnaces used in on*;
iron foundries are electric arc, electric induct.! on, ,».;d
reverberatory.
     Raw materials are placed in the cupola through a door
in the top of the furnace.  This process is called charging.
The raw materials consist of iron scrap, pig iron, fluxes,
and coke.  Fluxes are limestone or similar minerals, which
absorb impurities after the charge has melted.  Coke is
essentially pure carbon in lump form.  The burning of the
coke provides the heat to melt  the raw materials.  As the
charge melts, it descends to the bottom of the furnace where
the molten metal product  is drained out periodically.  Fresh
raw materials are added to keep the furnace  full.   Operation
of the cupola furnace is  a continuous process.
     The charge  for  electric arc,  electric  induction, and
reverberatory furnaces consists mainly  of  iron scrap, pig
iron, and limestone.  The reverberatory  furnace  is heated  by
firing gas or oil.   These furnaces are  operated  on a batch
basis.
      The molten  metal is  drained from the  furnace at a
temperature  of about 2900°F  into a ladle.   The ladle is used
to pour  the  molten  metal  into  prepared  molds,  which confine
 the iron in  the  form desired until it solidifies.  In pro-
                               7.10-3

-------
duction of high-strength ("ductile iron")  castings,  mag-
nesium is added to the molten iron;  the process is called
inoculation.  After solidification the castings are shaken
out of the molds or the molds are broken away from the
castings.  When they have cooled enough to permit handling,
the castings are cleaned by shot blasting and surface defects
are removed by grinding; these processes are generally
contained in an enclosure.
     Castings intended for certain uses may be annealed
 (heat treated) for several hours at temperatures of 1000 to
1600°F.  Heat treating furnaces, fired by gas or oil, are
referred to by many different names, including "annealing,"
 "hardening,"  "car-bottom," and  "traveling hearth" furnaces.
Castings that have been annealed are often referred to  as
malleable iron castings.  Finishing operations such as
 additional  shot blasting and grinding,  sand blasting, and
 surface  coating may follow the  heat treatment.   These are
 separate operations shown as one  box  in flow diagram  for
 simplicity.
      Production of molds  and cores  is  an integral part  of
 the foundry operation.  A mold  is made of sand mixed  with
 water and  binders such as clay, pitch or resins.  A core is
 a separable part  of  the mold used to  form a cavity in the
 casting.  Cores are  also  made of sand and binders.   After


                                7.10-4

-------
the cores are formed in the desired shape,  they are cured



either in a baking oven (core oven)  at 300-500°F or at room



temperature.  Curing evaporates moisture and hardens the



sand mixture.  Core ovens are fired with gas or oil.




EMISSION?1"7



     Operation of a gray iron foundry generates particulate




and gaseous pollutants.  Emission sources are identified in



Figure 7.10-1.  For some of the sources AP-42 provides



emission factors, which are listed on the process flow



diagram.  For other sources, average emission rates obtained




from other documents are mentioned in the following source




descriptions.



     Fugitive particulate emissions occur from unloading,




storage, and transfer of raw materials, such as sand, flux



materials, and scrap metal.



     The cupola is the largest source of emissions in a gray



iron foundry.  Cupola emissions include particulate matter



such as coke particles, ash, metallic fumes, smoke, and oil



vapor.  Although fugitive particulate emissions are gener-



ated from charging and tapping of the cupola, these emis-



sions are minor compared with those from the furnace.



Gaseous emissions from a cupola include carbon monoxide from




incomplete coke combustion, nitrogen oxides, and small




amounts of sulfur dioxide and fluoride compounds.  Uncon-
                               7.10-5

-------
trolled emissions of nitrogen oxides from cupolas have been
                                            4
reported to be 0.1 Ib/ton of metal produced.

     Particulate and gaseous emissions from electric induc-

tion and reverberatory furnaces are very low compared to

those from cupolas.  Emissions data for the electric arc

furnace in a gray iron foundry are not available, but the

particulate emission factor for an electric arc furnace in

a steel foundry is 13 pounds per ton of steel produced.

     Particulates are emitted in the pouring operation.  Two

studies indicate that these emissions range from 0.6 to 4.1

Ib/ton of metal produced.6'   Particulate emissions from

inoculation are reported to be 3.3 Ib/ton of metal produced.

     Shakeout of castings, an enclosed mechanical operation,

also generates particulate emissions which are reported to
                                       7
be about 12.8 Ib/ton of metal produced.

     Particulates are also emitted from cleaning and  finish-

ing of castings.
     Combustion of  fuel  in annealing generates combustion

products, which include  particulate and gaseous  pollutants.

Quantities depend on the type of  fuel, the combustion  effi-

ciency, and the temperature of the annealing furnace.

     Mold and core  making  processes generate primarily

particulates, which result from sand  screening,  sand  pre-

paration, mixing  of core sand  and binder,  mold making,  and
                               7.10-6

-------
core making.   One source reports that fugitive emissions


from core sand and binder mixing are 8.2 Ib/ton of metal


produced.   Quantitative data for emissions from all other


sources are not reported.  Core ovens, which are usually


fired with gas or oil,  emit mainly combustion products and


hydrocarbons from the binder.


CONTROL PRACTICES2'8'9


     Points of storage  and transfer of raw materials are


rarely controlled except with simple enclosures to protect


the materials from weathering.


     Various devices are used to control particulate emis-


sions from the cupola furnace.  Venturi scrubbers can be 99


percent effective in particulate removal and also can remove

                                    2
small amounts of gaseous pollutants.   Fabric filters can be


99.5 percent effective  in controlling particulate emissions

                                                   2
from a cupola but do not remove gaseous pollutants.   After-


burners, fired with gas or oil, are usually installed to


reduce carbon monoxide  emissions.


     At older installations with reverberatory furnaces,


particulate emissions are exhausted directly to the atmo-


sphere through a stack.  At newer installations, parti-


culates are controlled  with electrostatic precipitators,


baghouses, or venturi scrubbers.  Emissions from the induc-


tion furnaces are usually not controlled.  Emissions from
                              7.10-7

-------
        the charging and tapping of  these  furnaces  are  not  con-




        trolled.



             Either a hood or an enclosed  exhaust system (referred




        to as direct evacuation system)  is used to  capture  emissions



        from the electric arc furnace,  which are then vented to  a



        baghouse, venturi scrubber,  or  electrostatic precipitator.



        Where a hood is used, it also captures emissions from the




        charging and tapping operations.



             In older gray iron foundries, emissions from pouring



        operations generally are not controlled.  In some of the



        newer facilities, a hood is  installed over the  pouring area



        to capture the emissions, which are then vented to a fabric



        filter.  Emissions from the  inoculation operation are vented




        to a wet scrubber or a fabric filter.



             Particulate emissions from shakeout operations are con-



        trolled by hooding the area  and venting it to a wet scrubber



        or low-temperature fabric filter.   Particulates from grinding



4  "      and other cleaning operations are controlled by a dry



        mechanical collector, medium-energy wet scrubber, or bag-



        house.  Finishing operations such as grinding are provided



        with local exhaust hoods connected to high-efficiency



        centrifugal collectors or fabric  filters.  Efficiencies of




        these control  systems are not reported  in  the literature.



        Almost all heat  treating furnaces are vented directly to  the




        atmosphere.
                                       7.10-8

-------
     Dry cyclones and fabric filters are used to control

emissions from mold making and core making.  Most core ovens

are vented directly to the atmosphere through a stack.  A

few foundries are equipped with afterburners to control

hydrocarbon emissions.

CODING NEDS FORMS5'10" 2

     The major emission sources in a cray  iron foundry are:
     Source

Cupola
(In-process fuel)

Reverberatory
  furnace
(In-process fuel)

Electric induction
  furnace

Electric arc
  furnace

Pouring/casting

Casting shakeout

Grinding/cleaning

Annealing
 (In-process fuel)

Finishing

Sand handling
  in mold and core
  making

Core ovens
 (In-process fuel)
    SCC

 3-04-003-01
(3-90-008-99)

 3-04-003-02

(3-90-OOX-99')

 3-04-003-03


 3-04-003-04


 3-04-003-20

 3-04-003-31

 3-04-003-40

 3-04-003-05
(3-90-OOX-99 )

 3-04-003-60

 3-04-003-50
 3-04-003-51
(3-90-OOX-99)
     Pollutants

Particulates, CO, NO


Particulates, CO, NO



Particulates


Particulates, NO
                x

Particulates

Particulates

Particulates

Products of
 combustion



Particulates
HC, products of
 combustion
x
 The  codes  for  X  in  the  SCC's  for  in-process  fuel  are:   4  for

 residual oil;  5  for distillate  oil;  6  for  natural gas.


                                7.10-9

-------
     Standard NEDS forms for each of the sources,  Figures



7.10-2 through 7.10-12,  show entries for the SCC's and other




codes.  Entries in the data fields give information common



to gray iron foundries.   Information pertinent to coding the




source is entered on the margins of the forms and above or



below applicable data fields.  Entries for control equipment




codes, other optional codes, emission factors, and required




comments minimize the need to refer to the code lists.



Typical data values for operating parameters, control



equipment efficiencies, and other source information are




shown on the  form  (or in the text)  only to  serve  as quick,




approximate  checks of data  submitted by the  plant in a



permit application or similar report.   Data  entered in




EIS/P&R  and  NEDS  must be actual  values  specific  to and



reported by  the plant,  rather than  typical  values.  Contact



the plant  to validate or correct questionable data and  to



obtain unreported information.   See Part  1  of this manual




 for general  coding instructions.



      Select  the  appropriate SIC code,  3321  or 3322,  using



 the Standard Industrial Classification Manual (Ref.  12).



      The cupola is the largest  source of emissions in a gray




 iron foundry.  Emissions from the cupola are normally vented




 through a stack,  and the stack data should be entered.



 Figure 7.10-2 illustrates the standard NEDS  form  for this




 source.  If  the  foundry uses an electric induction or a
                                7.10-10

-------
reverberatory furnace,  code this source as shown in Figure




7.10-3.  Where there is no hood over the induction furnace,




code the height of the building vent(s) in the plume height




field.  Code zeros in the stack height and diameter fields,




77 in the temperature field, and zeros in the common stack




field.  Frter "No Hood, Bldg. Vent" in the comments field on




card 6.  Figure 7.10-4 shows the standard NEDS form for the




electric arc furnace.  Note that each of the furnaces has




its own IPP code.




     Other sources of emissions are inoculation, pouring,




shakeout, and cleaning operations.   Code these operations as




shown in Figures 7.10-5 through 7.10-8.  Where emissions




from inoculation and pouring operations are not captured




with a hood, code the height of the building vent(s) in the




plume height field.  Code zeros in the stack height and




diameter fields, 77 in the temperature field, and zeros in




the common stack field.  Enter "No Hood, Bldg. Vent" in the




comments field on card 6.  Where the castings are cleaned by



more than one operation, identify the operation(s) being




coded in the comments field on card 6.  For example, a




foundry may clean the castings by shot blasting and grind-




ing, and each operation may have its own control device.  In




this case, fill out two NEDS forms each with SCC 3-04-003-40.




On one form enter "Shot Blasting" in the comments field, and




on the other, "grinding."  Where the castings are annealed,







                                7.10-11

-------
code this operation separately using SCC 3-04-003-05,  as



shown in Figure 7.10-9.   Figure 7.10-10 shows standard NEDS




form for finishing operations.  In coding the finishirg



operations, follow the example given for cleaning operations.



     Emissions from sand handling operations associated with




raold and core making are very often vented into a common



particulate control device.   In this case, fill out only one



NEDS form  as  shown in Figure  7.10-11.   Enter  "Mold and  Core



Making"  in the comments  field on  card  6.  Where these operations




 are controlled by several  control systems, code each  group




 of operations that vent  to a  common control  system as an



 emission point with SCC  3-04-003-50.   Identify the group  of



 sources controlled by the system in the comments  field on



 card 7.  For example,  where a foundry has separate control




 systems for core making and mold making, fill out two NEDS



 forms, each with  SCC 3-04-003-50.  On one form enter "Mold



 Making" in the comments field, and on  the other, enter "Core



 Making."  Where  cores are cured  in an  oven, code the core




 oven  as  shown in Figure 7.10-12.
                                 7.10-12

-------
CODING EIS/P&R FORMS13



     The EEC's for use in EIS/P&R forms are:
          Source



          Cupola



          Reverberatory furnace



          Electric induction furnace




          Inoculation




          Pouring/casting



          Casting shakeout



          Grinding/cleaning




          Annealing



          F inishing



          Sand handling




          Core ovens
EEC




914




918




916




No code*




124




No code*




No code*




223




220 to 223




260




264
  This is status as of December 1977.
                                7.10-13

-------
CONTROL DEVICE
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-------
                            Figure 7.10-3.   Standard NEDS form for  gray iron  foundry  -  reverberatory


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                                                          NATIONAL EMISSIONS DATA SYSTEM (ME OS)
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-------
                      Figure 7.10-4.   Standard NEDS  form for gray iron foundry - electric arc furnace.
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CONTROL
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-------
         Figure 7.10-6.   Standard NEDS  form for gray iron  foundry - pouring/casting.
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-------
                    Figure  7.10-7.    Standard  NEDS  form  for gray  iron  foundry  -  casting  shakeout.
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-------
                              Figure  7.10-9.   Standard NEDS form  for gray  iron  foundry  - annealing.
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-------
            Figure 7.10-10.   Standard  NEDS  form for  gray iron  foundry  - finishing.
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                                        1    i -   !    I   • • I   >!•••.
                                          ' " I        !  •    ':   I "
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                                                                                  /•EXAMPLE COMMENT
                                                                                   L|AT$iT
                                             .
                                       i"j:tJ n u:t]! r   n.iiiUTmi
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-------
               Figure  7.10-11.   Standard  NEDS  form  for gray  iron foundry  -  sand  handling.
o
 I
                             p.,-1 ID
                             \, •' *
                           NATIONAL FMISVONS DATA SYSTCV i«,'FO$t
                                  r.irNrMi PROTECTION AGENCY
                                OFFICE OF MR OROGPAVS
                                                                                                        PO-'.TSO'.nCE


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                                                                     -  I -..-r -r I =-„,,, ..:•_, ["-•'  .-•' )  | C'~~"/]UU POINT I.D.'S IF COMMON STACK [j; j.,|
                                                                       ^I:3feEILI^EI^4l]
                                                                     I  i  I '  i  ! j  I i
               DEVICE
          LP  TEW. r*B»IC
           FILTER
                      COOE  I EFHC., '
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                                                                                                             rrol lio

                        UNIT TONS SAND HANDLED^

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                                                                                                    .EXAMPLE COMMENT
                                    !  M  i i FT ! i  i~"i
                                      ~~^"~



-------
                             Figure  7.10-12.   Standard NEDS form for gray iron foundry - core ovens,
o
                                                           NATIONAL EMISSIHMS DATA SYSTEM I'.'EOS)
                                                             ENV!Ror:-v.r:;i AI pRcmrTio"; ARfr.'CY
                                                                 OFFICE or AIR PROGHAVS
                               r.,   ;-.,fj,'£                        ,, ., ._..., .,,...,,<,,,                           :     0, „  ri..r.,.      j;
                                IHi: :^nci;I :^[^R7T^™in~!^ini;I^ ^^jM^fT^r^RiFTjiT^
                               jj:ziirnm
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                                                                                   ^0,     I     'JC
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                                              I I  ! I

                      CORE OVENS

                   INPROCESS FUEL
                                               ,SCC tiklS- TONS METAL PRODUCED tflfc FUEl£"OIL-1000 GALLONS: N.G.-MILLION CUBIC FEET'
                                                                       i  i
                                                                    * — ' '  ''
i i.iii.i   1 i .1   I   I   t"'    "T~I  i ~~'<  TM  T I    ! I'l T '[ f-j ;  t-»-r  fij-T-t—M~'^'^T~r'
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                                                                      dLkbhth
                                                 4-RESIDUAL OIL; 5-DISTILLATE OIL; 6-NATURAL GAS



                                                           lil'TT^i^ ;;|:-|;3 :c 
-------
GLOSSARY14

Casting - A metal object produced by pouring molten metal
     into a mold and allowing it to solidify.

Core - A separable portion of the mold that creates a
     cavity in the casting.

Ductile iron - Gray iron containing magnesium, which gives
     high strength and resistance to wear.   Used in machine
     parts.

Flux - Any of several minerals used to absorb impurities
     from molten metal.

Foundry - An operation where molten metal is poured into
     prepared molds to make various shapes.

Gray iron - A mixture of iron and carbon, with carbon
     content generally between 2 and 4 percent.  Often
     called "cast iron."

Ladle - A container for transporting and pouring molten
     metal.

Malleable iron - Gray iron that has been heat treated to
     make the casting readily machinable and corrosion
     resistant.

Mold - A form or matrix for containing a liquid until it
     solidifies in the shape of the mold.

Pig iron - A special type of gray iron casting in the shape
     of a rectangular block weighing about 100 pounds.

Steel - A mixture of iron and carbon, with the carbon content
     generally less than 1 percent.
                              7.10-25

-------
               REFERENCES FOR SECTION 7.10

1.   Background Information for Establishment of National
    Standards of Performance for New Sources (Draft).
    Prepared by PEDCo Environmental, Inc., and Environ-
    mental Engineering, Inc., for the U.S. EPA, under
    Contract No. CPA 70-142.  March 1971.

2.   Report on Systems Analysis of Emissions and Emissions
    Control in the Iron Foundry Industry in the U.S.A.
    Prepared by A.T. Kearney & Co., Inc. for U.S. Environ-
    mental Protection Agency.  Publication No. PB 198348.
    February 1971.

3.   Exhaust Gases from Combustion and Industrial Processes.
    Prepared by Engineering Science, Inc., for the U.S.
    EPA, Washington, D.C.  Publication No. PB-204-861.
    October 1971.

4.   Control Techniques for Nitrogen Oxides from Stationary
    Sources.  Prepared by U.S. Department of Health,
    Education, and Welfare, Environmental Health Services.
    Washington, D.C.  NAPCA Publication No. AP-67.  March
    1970.  p. 7-35.

5.   Compilation of Air Pollutant Emission Factors.  U.S.
    Environmental Protection Agency, Research Triangle
    Park, North Carolina.  Publication No. AP-42.  February
    1976.

6.   A Study of Fugitive Emissions from Metallurgical
    Processes.  Prepared by Midwest Research Institute,
    Kansas City, Missouri for Environmental Protection
    Agency, Research Triangle Park, North Carolina under
    Contract No. 68-02-2120.  Report No. 5.  November 1975.
    p. 29.

7.   A Study of Fugitive Emissions from Metallurgical
    Processes.  Prepared by Midwest Research Institute,
    Kansas City, Missouri for Environmental Protection
    Agency, Research Triangle Park, North Carolina under
    Contract No. 68-02-2120.  Report No. 11.  May 1976.
    p. 19.
                             7.10-26

-------
10.
 8   Particulate Pollutant System Study, Vol.  III.  Handbook
    of Emission Properties.  U.S. Environmental Protection
    Agency, Research Triangle Park, North Carolina.
    APTD-0745.  May 1971.

 9.  Air  Pollution Engineering Manual,  Second  Edition.
    Danielson, J.A.  (ed.).   U.S. Environmental Protection
    Agency, Research Triangle Park, North Carolina.   Pub-
    lication No. AP-40.  May 1973.

    Areos  Manual Series  Volume  V:  Aeros Manual of Codes.
    U.S. Environmental Protection Agency, Research Triangle
    Park,  North Carolina.   Publication No.  EPA-450/2-76-005
     (OAQPS No. 1.2-042).  April 1976.

    Aeros  Manual Series  Volume  II:  Aeros User's  Manual.
    U.S. Environmental Protection Agency, Research Triangle
    Park,  North Carolina.   Publication No.  EPA-450/2-76-029
     (OAQPS No. 1.2-039).  December  1976.

    Standard  Industrial  Classification Manual,  1972  Edition.
    Prepared  by Office of Management  and Budget.  Available
     from Superintendent  of  Documents,  Washington, D.C.

    Loquercio, P.  and W.J.  Stanley.   Air Pollution Manual
    of Coding.  U.S. Department of  Health,  Education and
    Welfare.   Public Health Service Publication No.  1756.
     1968.

14.  McGannon,  H.E.  (ed.).   The  Making, Shaping and  Treating
    of Stee_l,  9th  edition.   United  States  Steel Corporation,
     Pittsburgh, Pennsylvania.   1971.
11.
12.
13.
                           7.10-27
                           7.10-27

-------
                  7.11 SECONDARY LEAD SMELTING

PROCESS DESCRIPTION ~7
     Secondary lead operations reclaim lead from items such as
used storage batteries, pipe, type metal, machining and casting
scrap, and oxides, slags, and drosses from copper and lead
refining.  These materials, plus coke and limestone, are delivered
to the plant by rail or truck, where they are unloaded and stored
in piles until ne&ded.
     The three types of furnaces used in secondary lead produc-
tion are:  blast, reverberatory, and pot furnaces.  Pot furnaces
are generally used for refining and  alloying  the lead produced in
the other two furnaces.  Lead oxide  production by the Barton
process  is widely practiced  at  secondary lead plants.  Figure
7.11-1 diagrams these operations.
      The lead is  reclaimed by either sweating or  smelting.  In
 sweating, only  lead  and  other lower  melting metals  are  selectively
melted,  and  the higher melting  metals that remain  are removed
 periodically.   In smelting,  the furnace charge  (batch)  is com-
 pletely melted  and the melt  treated  to remove impurities  such as
 oxides.
      Some of the  scrap material must be pretreated by breaking
 or crushing before it is charged to  the furnace.   Batteries are
 broken with a saw or guillotine to separate  the lead from the
                              7.11-1

-------
                                                                                      9
                                                                                   SO,CONTR01
                                                                                      DEVICEl
                                       VENTURI SCRUBBER
                                       053 (99)
                                                                                  PARTICIPATE
                                                                                    CD°EVICE
                                       SETTLING CHAMBER  006
                                       BAGHOUSE oie  (>95)
          -PART0       ,;PART0
     RAW  MATERIAL     RAW MATERIAL
      UNLOADING         STORAGE
LEGEND:

Q> EMISSION FACTOR3
O    EMISSION FACTOR NOT DEVELOPED
    FOR THIS PROCESS
009 (66.0) DENOTES CONTROL EQUIP.
i           CODE WITH EST. EFF.  SHOWN
*           IN ( )
\         DENOTES FUGITIVE
                                                                                                                                                                 BAGHOUSE
                                                                                                                                                                 017 (99)
                                                                                                   PART0
                                                                                                                                                                   HOOD
                                                                                                                                                          LJU
                                                                                                                                                      3-04-OQ4-09
                                                                                                                                                        CASTING
                                                                                                                  LEAD
                                                                                                                  INGOTS
                                                                                                                 ' OR
                                                                                                                  CASTINGS
           DENOTES A STACK
 3-04-004-05
  SWEATING

 3-90-OOX-99
 5 -  DIST OIL
 6 -  NAT GAS	

IN-PROCESS  FUEL
           3-04-004-Q2
          REVERBERATORY
             FURNACE
              3-04-004-04
TO POT   ROTARY REVERBERATORY
FURNACE         FURNACE
OR TO        3-90-OOX-99
BARTON       5  -  DIST  OIL
PROCESS      6  -  NAT GAS
           IN-PROCESS  FUEL
COMBUSTION!
PRODUCTS 01
                                                                3-04-Q04-01
                                                                POT FURNACE
     3-04-OQ4-OX
     6 - DIST OIL
     7 - NAT GAS
     POT FURNACE
       HEATER
 *  IN  POUNDS  PER SCC UNIT
                                                               Figure  7.11-1.
                         Secondary  lead  smelting.

                         7.11-2

-------
nonmetallic portions of the battery.   Jaw crushers reduce large
pieces of scrap to smaller sizes suitable for further processing.
     The blast furnace (cupola)  is used to produce hard lead by
smelting lead oxides, such as the slags and drosses from rever-
beratory and pot furnaces.  Wastes from the smelting are recycled
through the blast furnace, together with the pretreated raw
materials.  Typical charge ratios are 4.5 percent rerun slag, 4.5
percent scrap iron, 3 percent limestone, 5.5 percent coke, and
82.5 percent drosses, oxides, and reverberatory slags.   By blow-
ing air for combustion through  the bottom, the charge is heated
to a temperature of  1200°  to 1350°F.  The coke reduces the lead
oxides  to  lead metal, which is  tapped almost continuously.  The
iron and  limestone  form  a slag  that  keeps the molten  lead from
oxidizing.  Slag  is  tapped intermittently, and about  5 percent is
returned  to the furnace.   The hard  lead product contains  5  to 12
percent antimony  and 0.5 to 1.0 percent other metals  (e.g.,
 arsenic,  tin,  copper,  and nickel).
      The  reverberatory furnace  is generally  used  for producing
 semisoft  lead by  sweating or smelting.   When used for sweating,
 only lead scrap  and drosses are charged and  the  furnace  temper-
 ature is  lower,  about 700°F.   In smelting,  the furnace tempera-
 ture is about 2300°F.   An oil or gas flame supplies the heat for
 melting,  and scrap is added at a rate sufficient to keep a small
 pile of solid material on top of the molten bath.  The reverbera-
 tory furnace may be either stationary or rotating; the former is
-more common.   Molten lead containing 0.3 to 0.4 percent antimony
                              7.11-3

-------
and 0.05 percent copper is tapped continuously.    It may be cast



into molds for later processing, or conveyed directly to the pot



furnace for refining.  In sweating, the unmelted charge is re-



moved periodically and charged to the blast furnace.  In smelting,



the slag is tapped intermittently and charged into the blast



furnace.



     Pot furnaces are used after the initial smelting or sweating



to produce soft, highly refined lead.  A smelter often has



several pot furnaces, which are indirectly fired to 1400°F by



heaters using oil or natural gas.  The charge materials are the



molten metal or ingots from the blast and reverberatory furnaces



and dressing agents that combine with impurities to form a



floating layer.  Various agents such as sulfur,  aluminum, sodium



nitrate, and sawdust are used.  Other metals are added to produce



alloys of a desired composition.  Lead having a purity greater



than 99.9 percent can be produced in pot furnaces.   Drosses are



recycled to the blast furnace.  The molten lead is cast into



ingots for shipment.



     A portion  (about 10 percent) of the lead from the blast and



reverberatory furnaces is converted to lead oxide instead of



being refined in a pot furnace.  The lead oxide, which is used in




storage batteries, is manufactured by the Barton process.



Molten lead at a temperature of 800°F is agitated with paddles,



and air is blown through it.  The formed lead oxide  (which con-



tains about 20 percent metallic lead) is captured from the



airstream by baghouses.








                             7.11-4

-------
EMISSIONS

     The emissions from secondary lead smelters are particulates,


sulfur oxides, carbon monoxide,  and hydrocarbons.   Emission


sources are identified in Figure 7.11-1.  For some of the sources,


AP-422 provides emission factors, which are listed on the process


flow diagram.  For other sources of emissions, average emission


rates obtained from other documents are mentioned in the follow-


ing source descriptions.


     The unloading and storage of scrap materials release negli-


gible emissions, because most of the material is in large pieces.


The unloading of coke and limestone releases fugitive particulate


emissions of 0.4 Ib/ton unloaded and 0.03 to 0.4 Ib/ton unloaded,

             O
respectively.   Total emissions from raw material unloading are


small.


     Breaking and crushing lead to minor amounts of particulate


emissions.


     Particulates and sulfur oxides, along with other combustion


products, are emitted during sweating.


     Particulate emissions from blast furnaces consist of par-


ticles  of lead oxide, coke, and other charge materials.  As much


as 7 percent of the charge may become entrained.   Gaseous emis-


sions are sulfur oxides, from the combustion of sulfur in the


charge,  and carbon monoxide and hydrocarbons,  from the combustion


of coke.


     Most of the particulate emissions  from reverberatory fur-


naces are lead oxides.  Sulfur oxides arise from  the  combustion




                            7.11-5

-------
of sulfur impurities in the charge,  and carbon monoxide and other



combustion products are emitted.   Particulates from pot furnaces



consist mostly of metallic fumes  and oxides.   Small amounts of



combustion products are emitted from the pot furnace heater.



     Particulates are emitted during casting of the molten lead.



During lead oxide manufacturing (the Barton process), oxide



particulates may escape from the baghouse.




                 1-9
CONTROL PRACTICES



     Because the emissions from raw material unloading, storage,



and breaking and crushing are minor, these operations are usually



not controlled.



     Particulate emissions from the sweating operation are  con-



trolled by baghouses, wet scrubbers, or both.  Sometimes a  wet



scrubber  is used to reduce sulfur oxide emissions.



     The  blast  furnace  is often controlled by  several devices



that are  used  in series.  An afterburner  burns the  carbon mon-



oxide  and hydrocarbons,  a settling  chamber and baghouse remove



particulates,  and  a wet scrubber  (usually a venturi type)  removes



sulfur dioxide. The  afterburner  is  needed to  prevent  the  carbon



monoxide and  hydrocarbons  from igniting  in the baghouse.   Some



smelters have only the afterburner  and baghouse.   An ESP  is



occasionally  used  after the  baghouse to remove more particulates.



      The particulate emissions from reverberatory furnaces



 (stationary or rotary)  are controlled with baghouses,  wet scrub-



 bers,  or both.  A wet scrubber is sometimes  used to control


                        9
 sulfur oxide emissions.



                             7.11-6

-------
     Particulate emissions from pot furnaces are captured by

hoods over the pots or kettles, and are vented to baghouses.  The

captured particulates are recycled to the blast furnace.   Combus-

tion products from the pot furnace heater do not come into con-

tact with the molten metal.  They are usually not vented through

a control device.  Particulates emitted during casting are

captured by hoods and vented to a baghouse.

     During lead oxide manufacturing, the baghouse that collects

particulates is considered part of the process, rather than

control, equipment.  Efficiencies of greater than 98 percent have

been reported for similar baghouses used on blast and reverbera-

              1
tory furnaces.


CODING NEDS FORMS10"1

     The emission sources associated with secondary lead smelters
are:

  Source

  Sweating
     In-process  fuel

  Blast/cupola  furnace


  Reverberatory furnace
     In-process  fuel

  Rotary  reverb,  furnace
     In-process  fuel

  Pot furnace

  Pot-furnace heater

  Barton  process

  Casting
    SCC

3-04-004-05
3-90-OOX-99

3-04-004-03
3-04-004-02
3-90-OOX-99

3-04-004-04
3-90-OOX-99

3-04-004-01

3-04-004-Ox

3-04-004-08

3-04-004-09


 7.11-7
     Pollutant(s)

Particulates S02,
 combustion products

Particulates, SO2,
 CO, HC

Particulates, SO2, CO,
 combustion products

Particulates, SO2, CO,
 combustion products

Particulates

Combustion products

Particulates

Particulates

-------
     Standard NEDS forms for each of the sources,  Figures  7.11-2




through 7.11-9, show entries for the SCO's and other codes.



Entries in the data fields give information common to secondary



lead smelters.  Information pertinent to coding the source is



entered on the margins of the forms and above or below applicable



data fields.  Entries for control equipment codes, other optional



codes, emission factors, and required comments minimize the need



to refer to the code lists.  Typical data values for operating



parameters, control equipment efficiencies, and other source in-



formation are shown on the form (or in the text)  only to aid in



quick, approximate checks of data submitted by the plant in a



permit application or similar report.  Data entered in EIS/P&R



and NEDS must be actual values specific to and reported by the



plant, rather than typical values.  Contact the plant to validate



or correct questionable data and to obtain unreported informa-



tion.  See Part 1 of this manual for general coding instructions.



     Figure 7.11-2 is a standard NEDS form for sweating.  When



wet scrubbers are used to control particulates, the control code



is 002.  A venturi scrubber is occasionally used to control sul-



fur oxides; in this case the control code is 053.   The coder must



determine what pollutant is being controlled when wet scrubbers



are used.



     Figure 7.11-3 is a standard NEDS form for the blast/cupola



furnace.  The several control devices used in series on blast



furnace exhaust must be coded according to the pollutant that



they control  (see Control Practices).  When a settling chamber






                             7.11-8

-------
and a baghouse control participates,  code the settling chamber as
the primary particulate control device and the baghouse as the
secondary control device.  The venturi scrubber can be a particu-
late control device as well as an S02 control device.  At a par-
ticular plant, the coder must determine what devices are used for
which pollutants and enter the equipment codes that are appro-
priate .
     Baghouses are the primary particulate control device for
emissions from the reverberatory furnace, the rotary reverbera-
tory furnace, and the pot furnace.  When a settling chamber
precedes the baghouse, code the settling chamber as the primary
control device and the baghouse as the secondary control device.
Figures 7.11-4, 7.11-5,  and 7.11-6 are standard NEDS forms for
these three furnaces.
     Combustion products from pot  furnace heaters are usually
vented to a stack with no controls; often, the emissions from the
furnace and heater are vented through a  common stack.  When  a
control device  is used,  enter the  appropriate code.  A standard
NEDS form  is  shown in Figure 7.11-7.
     The baghouse on  the airstream from  the  lead oxide manu-
facturing  is  process  equipment,  not  a control device.  Figure
7.11-8 is  a standard NEDS form  for this  source.
     The standard NEDS form  for casting  is given in Figure 7.11-9.
     The units  for the SCC's,  in all  cases except  lead oxide
manufacturing,  are expressed  in tons  of  metal  charged;  lead  oxide
manufacturing is  expressed in  tons of metal  processed.

                             7.11-9

-------
CODING EIS/P&R FORMS



     The EEC's of the equipment in a secondary lead smelter are:




     Equipment                          EEC



     Blast/cupola furnace               967



     Reverberatory furnace              969



     Rotary reverb, furnace             969



     Pot furnace                        970



     Pot-furnace heater                 283



     Barton process                     292



     Casting                          No code*
   As  of  October 1978.
                             7.11-10

-------
Figure 7.11-2.   Standard NEDS  form for  secondary  lead smelting  -  sweating
                                                                   POINT SOURCE
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GLOSSARY

Alloy - A mixture of metals, or nonmetals with metals, that has
     metallic properties.

Dross - Floating waste materials containing copper sulfide,
     antimony, and other unwanted materials from a pot furnace.
     Dross is usually recycled to the blast furnace.

Hard lead - Lead containing 0.5 to 12 percent antimony.

Semisoft lead - Lead containing 0.3 to 0.4 percent antimony.

Slag - Floating waste material composed of calcium and iron
     compounds.

Soft lead - Very pure lead, containing less than 0.1 percent
     antimony, copper, and  other metals.

Type metal - A series of alloys containing 54  to 95 percent lead,
     2 to 28 percent antimony, and 2  to  20 percent  tin, which  is
     used to make printing  type.

Barton process - A  process  to  manufacture  lead oxide  by inducing
     a draft  of  air over agitated molten lead.
                             7.11-19

-------
                  REFERENCES FOR SECTION 7.11


1.  Danielson, J.A.  Air Pollution Engineering Manual.   2nd
    edition.  Environmental Protection Agency.  AP-40,  May 1963.
    pp. 299-304.

2.  Compilation of Air Pollutant Emission Factors.  2nd edition.
    Environmental Protection Agency.  AP-42, February 1976.  pp.
    8.6-1, 8.6-4, C16.

3.  Background Information for Proposed New Source Performance
    Standards:  Secondary Lead Smelters and Refineries.  Volume
    1.  Environmental Protection 'Agency.  APTD 1352a, June 1973.
    pp. 37-43.

4.  Spity, A.W.  Control of Emissions from Secondary Metals
    Recovery and Asphalt Paving Plants.  A.W. Spity and Assoc.
    Presented at the  68th Annual Meeting of the Air Pollution
    Control Association, Boston, June 15 to 20, 1975.  pp. 4-5.

5.  The Economics of  Clean Air.  Annual Report of the Admini-
    strator of  the Environmental Protection Agency to the
    Congress of the United States.  February  1972.  pp. 4-141,
    4-143.

6  Zada, F.K., T. Briggs,  and T.W. Devitt.   Technical Guide  for
    Review  and  Evaluation of Compliance Schedules for Air  Pollu-
    tion  Sources.  EPA-340/l-73-001-a,  July  1973.  pp. 3-135  to
    3-138.

7.  PEDCo Environmental, Inc.  A Method for Characterization  and
    Quantification of Fugitive Lead Emissions from Secondary
    Lead  Smelters, Ferroalloy Plants,  and Gray Iron Foundries.
    EPA Contract No.  68-02-2515, Task  7,  January  1978.

 8  Technical Guidance  for  Control of  Industrial  Process  Fugi-
    tive  Particulate  Emissions.   EPA-450/3-77-010, March  1977.

 9  Radian  Corporation.  Pollution Control  and Heat  Recovery  in
    Non-Ferrous Smelters  (Draft).   EPA Contract No.  68-02-1319,
    Task  40/41.  February  28,  1977.

10.  Aeros Manual Series Volume  II:  Aeros User's Manual.   EPA-
     450/2-76-029 (OAQPS No.  1.2-039),  December 1976.


                            7.11-20

-------
11.   Aeros Manual Series Volume V:   Aeros Manual of Codes.   EPA-
     450/2-76-005 (OAQPS No.  1.2-042),  April 1976.

12.   Standard Industrial Classification Manual.   1972 edition.
     Office of Management and Budget.   Available from Superin-
     tendent of Documents,  Washington,  B.C.

13.   Loquercio. P.,  and W.J.  Stanley.   Air  Pollution Manual of
     Coding.  U.S. Department of Health, Education, and Welfare.
     Public Health Service Publication No.  1956.  1968.
                             7.11-21

-------
                    7.13  STEEL FOUNDRIES


                   1-4
PROCESS DESCRIPTION


     Foundries produce castings for automotive parts, light


and heavy machinery, pipe, and a wide range of miscellaneous



products.  The process involves melting scrap metal and


pouring the molten metal into prepared molds.  The two major


categories are "gray-iron" foundries and "steel" foundries.


Both gray iron and steel consist mostly of elemental iron,


but the carbon contents differ.  Gray iron contains 2 to 4


percent carbon, and steel contains 1 percent or less.  Steel



may also contain alloying metals.


     Figure 7.13-1 illustrates the process flow in a typical


steel foundry.  The raw materials are placed in the furnace



through a side door or through the top.  This process is


called charging.  The raw materials consist of steel scrap,


pig iron, and fluxes.  Pig iron is gray iron in blocks


weighing about 100 pounds each.  Fluxes are limestone,


fluorspar, and similar minerals, which absorb impurities


after the charge has melted.  Three types of furnaces are


used for melting:  the electric arc furnace, the electric


induction furnace, and the open hearth furnace.  All three


types operate on a batch  basis, each batch being called a
                              7.13-1

-------
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"heat."  The open hearth furnace is heated by firing gas or



oil.   In the open hearth furnace oxygen is sometimes blown



directly onto the molten metal to accelerate '.he melting




process, a procedure called oxygen lancing.



     When the temperature of the charge reaches about 3000°F




the molten metal is drained from the furnace into a ladle.



The ladle is used to pour the molten steel into prepared




molds, which confine the steel in the form desired until it



solidifies.  After solidification the castings are shaken




out of the molds or the molds are broken from the castings.



When they have cooled enough to permit handling, the castings



are cleaned by shot blasting and surface defects are removed




by grinding; these processes are generally contained in an




enclosure.



     Castings intended for certain uses may be heat treated



(annealed) for several hours at temperatures ranging from



1000  to 1600°F.  Heat treating furnaces, fired by either gas



or oil, are referred to by many different names, including



"annealing," "hardening," "car-bottom," and "traveling



hearth" furnaces.  Finishing operations such as additional



shot-blasting and grinding, sand blasting, and surface



coating may follow the heat treatment.  These are separate



operations shown as one block in the process flow diagram




4.or simplicity.
                               7.13-3

-------
     Production of molds and cores is an integral part of


the steel foundry operation.  A mold is made of sand mixed


with water and binders such as clay, pitch,  or resins.  A


core, also made of sand and binders, is a separable part of


the mold used to form a cavity in the casting.  After the


core is formed in the desired shape, it is cured either in a


baking oven (called "core oven")  at 300 to 500°F or at room


temperature.  Curing evaporates moisture and hardens the


sand mixture.   Core ovens are heated by direct firing with


gas or oil.


     Large steel foundries operate 24 hours a day and 7 days


a week, while smaller ones operate 8 hours a day.  Typical


stack heights of the furnaces range from 55 to 85 feet.


Capacities of foundries range from 5 to 240 tons of metal


produced per day.

         1 ? S-Q
EMISSIONS ''


     Operation of a steel foundry generates both particulate


and gaseous pollutants.  Emission sources are identified in


Figure 7.13-1.  For some of the sources AP-42 provides


emission factors which are listed on the process flow


diagram.  For other sources of emissions, average emission


rates obtained from other documents are mentioned in the


following source descriptions.


     Fugitive dust emissions occur in unloading, storage,
                               7.13-4

-------
and transfer of raw materials such as sand, flux materials,




and scrap metal.




     The melting furnace is the largest source of emissions,




which are both particulate and gaseous.  The particulates




include oxide fumes, graphite, and metal; the gases include




hydrocarbons from oily scrap and fuel, carbon monoxide,




sulfur oxides, and oxides of nitrogen.




     Charging and tapping of the furnace generate fugitive




particulate emissions.




     The pouring operation generates particulate emissions.




Two studies indicate that these emissions range from 0.6 to




4.1 Ib/ton of metal produced. '




     Shakeout of castings generates particulate emissions,




as do the various cleaning and finishing operations.  Par-




ticulate emissions from the shakeout operation are reported




to be 12.8 Ib/ton of metal produced.   Combustion of fuel in




heat treating generates combustion products, which include




particulate and gaseous pollutants.  Quantities depend on




the fuel, the temperature, and the combustion efficiency of




the heat treating furnace.




     Mold and core making generate particulates in sand




screening, sand preparation, mixing of sand and binder, mold




making, and core making.  One source reports that fugitive




omissions from sand and binder mixing are 8.2 Ib/ton of
                               7.13-5

-------
metal produced.   Quantitative data for emissions from all

other sources are not reported.  Core oven emissions include

combustion products of the fuel (usually gas or No. 2 oil)

used to fire the ovens and some hydrocarbons from the

binder.

CONTROL PRACTICES1"3'7'8

     Points of storage and transfer of raw materials are

rarely controlled except with simple enclosures to protect

the material from weathering.

     Various devices are used to control particulate emis-

sions from furnace operations.  Table 7.13-1 lists the types

of control devices and their efficiencies.

    Table 7.13-1.  EQUIPMENT USED TO CONTROL PARTICULATE

              EMISSIONS FROM MELTING FURNACES
   Type
of furnace
Electric arc
Open hearth
Open hearth,
 oxygen lanced
Electric induction
 Control
equipment
   ESP
Fabric filter
Venturi scrubber

   ESP
Fabric filter
Venturi scrubber

   ESP
Fabric filter
Venturi scrubber

   None
   Control
efficiency, %
  92 to 98
  98 to 99
     99

  95 to 98.5
    99.9
      99

  95 to 98
    99
    99
     Either a hood or an enclosed exhaust system  (referred
                                7.13-6

-------
to as direct evacuation system)  is used to capture emissions




from the electric arc furnace,  which are then vented to a




particulate control device.   Where a hood is used, it also




captures emissions from the charging and tapping operations.




Combustion (flue) gases from the open hearth furnace are




vented to a device for the control of pa -ticulate emissions.




Emissions from charging and tapping of open hearth furnaces




are not controlled.



     Emissions from pouring operations usually are not




captured, although in some newer facilities a hood is




installed over the pouring area and is vented to a control




device.  Emissions from shakeout operations are usually




controlled by hooding the area and venting the emissions to




a scrubber or baghouse.  Particulates from cleaning opera-




tions are controlled by venting the exhaust hoods to a dry




mechanical collector, fabric filter, or medium-energy wet




scrubber.  Finishing operations such as grinding are nor-




mally provided with an exhaust hood connected to a high-




efficiency centrifugal collector or a fabric filter.  Almost




all heat treating ovens are vented directly to the atmosphere.




     Emissions from mold making and core making operations




are controlled with dry cyclones and fabric filters.  Most




core ovens are vented directly to the atmosphere through a




stack.  A few foundries are equipped with afterburners to




control hydrocarbon emissions from the core ovens.









                               7.13-7

-------
CODING NEDS FORMS10 12

     The major emission sources  in  a  steel  foundry  are:
     Source

Electric arc furnace

Open hearth furnace
(in-process fuel)

Open hearth furnace,
 with oxygen lance
(in-process fuel)

Electric induction
 furnace

Pouring/casting

Casting shakeout

Clean ing

Heat-treat furnace
(in-process fuel)

Finishing
      SCC

 3-04-007-01

 3-04-007-02
(3-90-OOX-99)

 3-04-007-03

(3-90-OOX-99)

 3-04-007-05


 3-04-007-08

 3-04-007-09

 3-04-007-11

 3-04-007-04
(3-90-OOX-99)

 3-04-007-15
Pollutants

Particulates, i;o

Particulates, NO
x
Sand grinding/handling   3-04-007-06
 in mold and core making
Core ovens
(in-process fuel)
 3-04-007-07
(3-90-OOX-99)
Particulates, l."0



Particulates


Particulates

Particulates

Particulates

Products of
combust ion



Particulates
HC, Products of
combustion
The codes for X in the SCC's for in-process fuel are:  4 for

residual oil; 5 for distillate oil; 6 for natural gas.

     Standard NEDS forms for each of the sources, Figures

7.13-2 through 7.13-11,  show entries for the SCC's and other

codes.  Entries in the data fields give information common

to steel foundries.  Information pertinent to coding the

source is entered on the margins of the forms and above or
                                7.13-!

-------
below applicable data fields.   Entries for control equipment
codes, other optional codes, emission factors, and required
comments minimize the need to refer to the code lists.
Typical data values for operating parameters, control
equipment efficiencies, and other source information are
shown on t*o form  (or in the text) only tc serve as quick,
approximate checks of data  submitted by the plant in a
permit application or similar report.  Data entered in EIS/
P&R  and NEDS must be actual values specific to and reported
by the plant,  rather than typical values.  Contact the plant
to validate or correct questionable  data  and  to obtain
unreported  information.   See Part  1  of this manual for
general coding instructions.
      The  major sources of emission  from  steel foundries  are
the  melting furnaces (Figures  7.13-2 through 7.13-4).  An
electric  induction furnace  usually is not controlled  because
 emissions are very low.   Where there is  no hood over  the
 induction furnace, code  the height of the building vent(s)
 in the plume height field.   Code zeros in the stack height
 and diameter fields, 77  in the temperature field, and zeros
 in the common stack field.   Enter "No Hood, Bldg. Vent"  in
 the comments  field on card 6.   Note that each furnace has
 its own IPP code.
      Other sources of emissions are pouring,  shakeout,  and
                                7.13-9

-------
cleaning operations.   Code these operations as shown in



Figures 7.13-5 through 7.13-7.   Where emissions from pouring



operations are not captured with a hood, code the height of



the building vent(s)  in the plume height field.  Code zeros



in the stack height and diameter fields, 77 in the tempera-



ture field, and zeros in the common stack field.  Enter "No




Hood, Bldg. Vent" in the comments field on card 6.  Where



the castings are cleaned by more than one operation, identify



the operation(s) being coded in the comments field on card



6.  For example, a foundry may clean the castings by shot



blasting and grinding, and each operation may have its own



control device.  In this case, fill out two NEDS  forms, each



with SCC 3-04-007-11.  On one form enter "Shot Blasting" in




the comments field, and on the other, enter "Grinding".



Where the  castings are heat treated, code this operation



separately using SCC  3-04-007-04, as shown in Figure 7.13-8.



Figure  7.13-9  shows a standard NEDS  form for  finishing



operations.  In coding the finishing operations,  follow the




example given  for cleaning operations.



     Emissions from sand  grinding/handling operations



associated with mold  and  core making are very often  vented



through a  common  control  system.   In this  case,  fill out



only one  NEDS  form as shown  in  Figure  7.13-10.   Enter  "Mold




and Core  Making"  in  the  comments field on  Card 6.  Where
                               7.13-10

-------
 these operations are controlled by  several control systems,




 code each group of operations that  vent to a common control




 system as an emission point with SCC  3-04-007-06.  Identify




 the group of sources controlled by  the system  in the com-




 ments field on Card 7.  For example,  where a foundry has




 separate control systems  for core making and mold making,




 fill out --wo NEDS forms,  each with  SCC 3-04-OC7-06.  On one




 form enter "Mold Making"  in the comments field, and on the




 other, enter "Core Making."  Where  cores are cured in an




 oven, code the core oven  as shown in  Figure 7  13-11.




 CODING EIS/P&R FORMS13




     The EEC's for use  in the EIS/P&R forms are:




            Source                              EEC




     Electric arc furnace                   923 to 925




     Open hearth furnace                     ')21




     Open hearth with oxygen lancing          )22




     Electric induction furnace               326 to 928




     Pouring/casting                          124




     Casting shakeout                        "to code*




     Cleaning                                ^o code*




     Heat treating                           220 to 223




     Finishing                               113




     Sand grinding/handling                  260




     Core ovens                              264







* Status  as  of  December  1977.






                              7.13-11

-------
                            Figure  7.13-2.   Standard  NEDS form for  steel  foundry  -  electric arc  furnace.
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                                                             ENVIRONMENTAL PROTECTION AGENCY

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FURKACE
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          Figure 7.13-4.    Standard  NEDS  form  for  steel foundry -  electric  induction furnace.
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                       Figure  7.13-5.   Standard NEDS  form  for  steel  foundry  - pouring/casting.
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                                                        NATIONAL EMISSIONS DATA SYSTEM (NEDS)
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-------
        14
GLOSSARY

Casting - A metal object produced by pouring molten metal
     into a mold and allowing it to solidify.

Core - A separable portion of the mold that creates a cavity
     in the casting.

Flux - Any of several minerals used to absorb the impurities
     from molten metal.

Foundry - An operation where molten metal is poured into
     prepared molds to make various shapes.

Gray iron - A mixture of iron and carbon, with carbon con-
     tent generally between 2 and 4 percent.  Often called
     "cast iron."

Ladle - A container for transporting and pouring molten
     metal.

Mold - A form or matrix for containing a liquid until it
     solidifies in the shape of the mold.

Pig iron - A special type of gray iron casting in the shape
     of a rectangular block weighing about 100 pounds.

Steel - A mixture of iron and carbon, with carbon content
     generally less than 1 percent.
                               7.13-22

-------
               REFERENCES FOR SECTION 7.13
1.   Danielson,  J.A.  (ed.).   Air Pollution Engineering
    Manual, Second Edition.  Environmental Protection
    Agency- Research Triangle Park, Nort 4 Carolina.
    AP-40.  May 1973.

2.   Report on Systems Analysis of Emissions and Emissions
    Control in the Iron Foundry Industry in the U.S.A.
    Prepared by A.T. Kearney and Company, Inc., for Environ-
    mental Protection Agency.  PB 198 348.  1971.

3.   Compilation of Air Pollution Emission Factors, second
    edition with Supplements 1-7.  U.S. Environmental
    Protection Agency, Research Triangle Park, North
    Carolina.  AP-42.   February 1976 through April 1977.

4.   Exhaust Gases from Combustion and Industrial Processes.
    Prepared by Engineering Science, Inc.,  Washington,
    D.C. for Environmental Protection Agency.   PB-204-861.
    October 1971.

5.   A Study of Fugitive Emissions from Metallurgical Pro-
    cesses.  Prepared by Midwest Research Institute, Kansas
    City, Missouri for Environmental Protection Agency,
    Research Triangle Park, North Carolina under Contract
    No. 68-02-2120.   November 1975.  Report No. 5.

6.   A Study of Fugitive Emissions from Metallurgical Pro-
    cesses.  Prepared by Midwest Research Institute, Kansas
    City, Missouri for Environmental Protection Agency,
    Research Triangle Park, North Carolina under Contract
    No. 68-02-2120.   May 1976.  Report No. 11.

7.   Background Information for Establishment of National
    Standards of Performance for New Sources  (Draft).
    Prepared by PEDCo Environmental, Inc., and Environ-
    mental Engineering, Inc. for Environmental Protection
    Agency, Durham, North Carolina under Contract No. CPA
    70-142, Task 2.  March 1971.
                              7.13-23

-------
 8.   Particulate  Pollutant  Systems  Study,  Vol.  III.   Hand-
     book of  Emission Properties.   Environmental  Protection
     Agency,  Research Triangle  Park,  N.C.   APTD-0745.   May
     1971.

 9.   Background Information for Standards  of Performance:
     Electric Arc Furnaces  in the  Steel  Industry.   U.S.  EPA
     Office of Air and Waste Management.   Office  of Air
     Quality Planning and Standards.   Research Triangle
     Park,  North Carolina 27711.   EPA-450/2-74-017a.   1974.

10.   Aeros Manual Series Volume V:   Aeros  Manual  of Codes.
     U.S. Environmental Protection Agency, Research Triangle
     Park,  North Carolina.   Publication  No. EPA-450/2-76-005
     (OAQPS No. 1.2-042).  April 1976.

11.   Aeros Manual Series Volume II:  Aeros User's Manual.
     U.S. Environmental Protection Agency, Research Triangle
     Park, North Carolina.   Publication  No. EPA-450/2-76-029
     (OAQPS No. 1.2-039).  December 1976.

12.   Standard Industrial Classification  Manual, 1972 Edition,
     Prepared by Office of Management and Budget.  Available
     from Superintendent of Documents, Washington, D.C.

13.   Loquercio, P. and W.J. Stanley.  Air Pollution Manual
     of Coding.  U.S. Department of Health, Education and
     Welfare.  Public Health Service Publication No. 1956.
     1968.

14.   McGannon, H.E.  (ed.).  The Making,  Shaping,  and Treating
     of Steel, 9th edition.  United States Steel Corpora-
     tion, Pittsburgh, Pennsylvania.  1971.
                                7.13-24

-------
                8.1  ASPHALTIC CONCRETE PLANTS



                   123
PROCESS DESCRIPTION ' '


     Asphaltic concrete is a paving material produced by


mixing coarse and fine aggregates with hot asphalt.   The


aggregate materials consist mainly of crushed stone and


gravel, sand, and some waste materials, such as slag from


steel mills and crushed glass.  These materials are propor-


tioned to produce a specific paving mix of uniform composi-


tion.  After mixing, the hot paving material is loaded into


trucks and transported to the paving site.


     Plants that produce hot-mix asphaltic concrete operate


either by batch production or continuous-mix production.


These operations are identical up to the point of final


mixing.  Batch plants currently account for over 90 percent


of the production capacity in the United States.  Figure


8.1-1 depicts a typical batch plant and Figure 8.1-2, a


continuous-mix plant.  Asphalt plants may be stationary or


portable; portable plants can be readily dismantled and


transported on trailers from one job site to another.  These


portable plants account for 20 percent of the production.
                                .1-1

-------
                                                     Figure  8.1-1.   Batch hot-mix  asphaltic  concrete  plant.
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-------
                                                   Figure 8.1-2.    Continuous  hot-mix  asphaltic  concrete  plant.
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     Different applications for asphaltic concrete require



different aggregate size distributions.   The aggregate



usually comprises 94 to 95 percent by weight of the total



asphalt and aggregate mix.  The raw aggregates are crushed



and screened at the quarries, then brought to the plant site



and stored in open piles or occasionally in silos.



     In both batch and continuous-mix operations, the coarse



and fine aggregates are hauled separately from the storage



piles and placed in hoppers of the cold-feed unit.  The



materials are then discharged onto a conveyor belt and fed



into a rotary dryer fired directly with gas or oil.  The hot



aggregates from the dryer drop into a bucket elevator and



are transferred to a set of vibrating screens that separate



the aggregate into as many as four size classifications.



Screening is required for production of specified concrete



mixtures of different-sized aggregates.   The sized materials



are then stored in hot bins, so called because they store



the aggregates that have been heated by drying.  To this



point, the operations of batch and continuous-mix plants are



the same; the differences occur in subsequent process steps.



     In a batch plant, the classified aggregate  is stored by




size range in four  large  hot bins.  The operator  opens




individual bins and allows the classified aggregates  to drop
                               8.1-4

-------
into a weighing hopper until the desired weight of a spec-
ified size mixture is obtained.   The sized aggregates are
then dropped into a mixer and mixed dry for a short period.
Hot asphalt is pumped from heated storace tanks, weighed,
and then injected into the mixer.  Total mixing time in-
cluding dry mixing is 25 to 60 seconds.  The hot, mixed
batch is then dropped into a truck and hauled to the job
site.
     In a continuous-mix plant, the classified hot aggregate
drops into a set of small hot bins, which are smaller than
those at a batch plant because less storage capacity is
needed.  From the hot bins, the aggregate is continuously
metered through a set of feeder conveyors and a bucket
elevator into the mixer.  Asphalt  is also continuously
metered into the  inlet end  of the  mixer, where  retention  is
controlled by an  adjustable dam.   The  mix flows out  of  the
mixer into a hopper,  from which  the trucks  are  loaded.
      Production capacities  of both batch and continuous-mix
asphalt plants range  from  50  to  1000 TPH, with  an  average of
about 160  TPH.  Total  exhaust  requirements  for  the rotary
dryer and  the  other dust sources (hot  elevators,  hot screens,
hot bins,  and  mixer)  vary according to the  size of plant.
For a 150-TPH  plant,  either batch or  continuous-mix, a
                               8.1-5

-------
typical air flow requirement is 22,000 SCFM,  of which about


3,000 SCFM is required for the other sources.


     Figure 8.1-3 shows the relationship of total exhaust


gas flow rate from the dryer and the other sources to the


asphaltic concrete production rate.  This graph, based on


data from numerous source tests, may be used to check data


submitted by the plant.



EMISSIONS

     Operation of an asphalt plant generates both particu-


late and gaseous pollutants.   Emission  sources  are identi-


fied in Figures  8.1-1  and  8.1-2.   Since emissions from the


final  mixing operation are negligible,  there is little


difference  in  the emissions from a batch mix and a con-


tinuous-mix plant.  Much more significant  are  the differ-


ences  in  emissions  at  individual plants;  these differences


depend on  such factors as particle size distribution of  the


 aggregate,  dryer gas  velocity, and control equipment.


      Fugitive emissions of particulate occur from unloading,


 storage,  and handling of aggregates.  The following  empiri-


 cal expression is given in AP-42 for estimating emissions

                              2
 from aggregate storage piles:



                0.33
               /PE ,2
               (TOO}
                               8.1-6

-------
00


M

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                         50,000
                         40,000 -
                         30,000 -
                     1
                     x
20,000 -
                          10,000-
                                            100            200       '     300.           400


                                                    ASPHALTIC CONCRETE PRODUCTS, TONS/HR
                         Figure 8.1-3.  Total exhaust rate for asphaltic concrete pla.

-------
where:  E = Emission rate, Ib/ton placed in storage

       PE = Thornthwaite1s precipitation-evaporation index


The source activities that contribute to the fugitive emis-

sions and their approximate percentages are as follows:


                                  Approximate percentage
     Source activity                of total emissions

     Loading onto piles                     12

     Vehicular traffic around               40
       storage piles

     Wind erosion                           33

     Loadout from piles                     15

                          Total              100

     Although no quantitative data  are  available on  fugitive

 emissions  attributable to loading of  cold  storage  bins,

 these  emissions  are considered  to be  negligible.   Usually,

 other  fugitive  emission  sources - the elevators, hot screens,

 hot bins,  and mixer -  are well-enclosed and vented by in-

 duced draft through a  common header.   They are  commonly

 vented with the dryer  exhaust into  a  single collector and

 fan system, as  shown in  Figures 8.1-1 and 8.1-2.

      The rotary dryer is the largest source of  particulate

 emissions.   The quantities of particulate and the particle-

 size distributions vary widely from plant to plant.  Dryer
                               8.1-8

-------
design and operation, particle size distribution of feed



materials, and the specific grade of asphaltic concrete



product exert a marked effect on the quantity of emissions.



     Gaseous emissions occur mainly from the combustion of



fuel for the dryer.  Since asphalt is a heavy distillate



from refinery operations, emissions of hydrocarbon vapors



from heated asphalt and from mixing operations are very



small.  ^ ference 6 reports polynuclear hydrocarbon emission




rates of  I.0 x 10   Ib/ton of product without control and



0.8 x 10~6 Ib/ton of product after a wet scrubber control




system on the mixing operation.




CONTROL PRACTICES  '  '



     All plants use a primary dust collection system, such



as a large-diameter cyclone or settling chamber, to control



emissions from the dryer and return the fines to the product




flow.  Since emissions after this primary control device are



still considerable,  secondary and even tertiary pollutant



control devices are  commonly used.  The applicable control



equipment  includes mechanical collectors  (e.g., multiclones),



wet scrubbers, and fabric filters; attempts  to  apply elec-



trostatic precipitators  to dryer exhausts have  met with



little success.   The  exhaust from the other  sources  (i.e.,



elevators, hot screens,  hot bins, mixer)  is  often combined



with  the  exhaust  from the dryer  to control the  particulates




in both with  the  single  collector system.  A scrubber  in the
                               8.1-9

-------
control system provides some reduction of hydrocarbon emis-

sions from the mixer.

     Many plants use a device called a "wet fan" after the

prinuiry device.  A wet fan is a type of scrubber, such as a

Type R Rotoclone, which wets the exhaust gases and then

separates the particulate matter by centrifugal force.

     Hydrocarbon vapors from heated asphalt storage tanks

can be adequately controlled by condensing the vapors with

air-cooled vent pipes.   Hydrocarbon emissions from truck-

loading of asphaltic concrete can be controlled by combus-

tion by venting them into the dryer.  More development work

is required on methods of introducing the hydrocarbons into

the dryer.

CODING NEDS FORMS

     The emissions sources in an asphalt concrete plant are:
  Source

  Rotary dryer
  (in-process fuel)
    SCC
   Pollutants
 3-05-002-01    Particulate/ SO-,
(3-90-OOX-99)   NO  , HC, CO
  Hot elevators, screens,  3-05-002-02
  bins, and mixer
  Storage piles

  Cold aggregate
  handling

  Asphalt heater
 3-05-002-03

 3-05-002-04


 3-05-002-OX
Particulate, HC


Particulate

Particulate
Particulate, SO ,
NO ,  HC, CO
    Includes emissions from loading onto piles, vehicular
    traffic around piles, wind erosion, and load out from
    piles.
                              8.1-10

-------
Standard NEDS forms for each of the sources, Figures 8.1-4



through 8.1-9, show entries for the SCC's and other codes.



Entries in the data fields give information common to



asphalt plants.  Information pertinent to coding the source



is entered on the margins of the forms and above or below



applicable data fields.  Entries for control equipment



codes, oliier optional codes, emission factors, and required




comments minimize the need to refer to the code lists.



Typical data values for operating parameters, control equip-



ment efficiencies, and other source information are shown on



the form (or in the text) only to serve as quick, approxi-



mate checks of data submitted by the plant in a permit



application or similar report.  Data entered in EIS/P&R and



NEDS must be actual values specific to and reported by the



plant, rather than typical values.  Contact the plant to



validate or correct questionable data and to obtain unre-



ported information.  See Part 1 of this manual for general



coding instructions.



     The asphaltic concrete plant mainly emits particulates,



and the dryer is the largest emission source.  The hot



elevators,  hot screens, hot bins, and mixer as a group are



treated as a single source because their emissions are



relatively low and their exhausts are usually vented into a



common header; the group is called "other sources," desig-
                              8.1-11

-------
nated by the SCC 305-002-02.   Figures 8.1-4 and 8.1-5 illus-



trate the standard NEDS forms for the two sources,  dryer and



other.  When the two sources are vented through a common



stack, their point ID numbers must be sequential and these



ID's must be entered in the "points with common stack" field




of both forms.



     For asphalt plants that combine the exhausts from the



dryer and the "other sources" to control emissions with a



single control system, it is acceptable to combine the two



sources as a single emission point, coded on one NEDS form.



The point would be defined by the three SCC's, 3-05-002-01,



3-90-OOX-99, and 3-05-002-02.  The standard NEDS form,



Figure 8.1-6, illustrates this alternative coding.



      Required comments about an asphalt plant include



whether it is batch or continuous, stationary or portable.



Name  the specific  control device when  device code  001 is



entered in a control equipment field.  Where particulates



are  controlled  by  primary,  secondary,  and  tertiary devices,



enter codes for the secondary and  tertiary control equipment



in the code fields of  the form; enter  the  name  and device



code of  the primary  (precleaner) control equipment as com-



ments.  Where  a wet fan  is  used  as  a control device,  enter




code number  001 in the applicable  field  and enter  the re-




ported efficiency.
                               8.1-12

-------
     The plant should report information about the aggregate

stockpiles,  aggregate handling, and asphalt heater.   These

sources are to be coded.   Figures 8.1-7, 8.1-8, and 8.1-9

illustrate the standard NEDS forms for these operations.

The units for the SCC's are tons of asphaltic concrete

produced.


CODING EIS/P&R FORMS

     The EEC's for use in EIS/P&R forms are shown below:

     Source                        BEG

     Rotary dryer                  450

     Hot elevators, screens,       700
     bins, and mixers

     Storage piles               (No code)

     Cold aggregate handling       700

     Asphalt heater                283


GLOSSARY OF TERMS


Aggregate - The  solid mineral  load-bearing constituents  of
     asphalt paving materials, such as  sand and  fragments of
     stone and gravel.

Asphalt - A black material  having  some  of  the  properties of
     cemont, but capable of softening when heated and of
     hardening again when cooled.  Asphalt is  derived from
     the refining of crude  petroleum.   The final asphaltic
     concrete product  is often referred to as  'asphalt.'
                               8.1-13

-------
ROTA
PROC


TYPE OF CONTROL
UNCONTROLLED
PRECLEANER8
HIGH-EFFICIENCY CYCLONE
SPRAY TO'./ERb h
MULTIPLE CENTRIFUGAL SCRUBBER0
BAFFLE SPRAY TOWER0
ORIFICE-TYPE SCRUBBER0
BAGHOUSE
CONTROL
EQUIP.
CODE
000
009
007
001
001
001
001
017
PARTICULATE
EMISSIONS
LB/TON
35.0
11.7
1.3
0.3
0.2
0.2
0.03
0.08
  THE CODE 009 IS FOR LOW EFFICIENCY

h CENTRIFUGAL COLLECTOR.

  IDENTIFY THE SPECIFIC COLLECTOR

  DEVICE IN COMMENTS.
C


(D


CD
i

I-1
 I
                                                                             g.
                                                                             0>
                                                                             n
                                                                             QJ
                                                                             a
                                                                             en
                                                                             W
                                                                             n

                                                                             o
                                                                             o

                                                                             o
                                                                             n
                                                                             ro
                                                                             rt
                                                                             n>
                                                                              8
                                                                              rt
                                                                              &>
                                                                              h
                                                                              H


                                                                              (D

-------
                     ST-T'8
             TYPE OF CONTROL
      UNCONTROLLED
      PRECLEANER*
      HIGH-EFFICIENCY  CYCLONE
      SPRAY IOWERb                 b
      MULTIPLE CENTRIFUGAL  SCRUBBER
      BAFFLE SPRAY  TOWER&
o     ORIFICE-TYPE  SCRUBBER0
3:     3AGHOUSE
                                      CONTROL  'PARTICULATE
                                      EQUIP.   '  EMISSIONS
                                       CODE
                                        000
                                        009
                                        007
                                        001
                                        001
                                        001
                                        001
                                        017
                                                 LB/TON
«  a  THE  CODE  009  IS FOR LOW EFFICIENCY
i  h  CENTRIFUGAL COLLECTOR.
o    IDENTIFY  THE  SPECIFIC COLLECTOR
K    DEVICE  IN COMMENTS.

                     r~;H
                                    -,..., ,4.£U2U  H
                                      o,M m I  (i! '
                                         -o —<_—*	

-
























!T


























is s| ?li OWN H- d 00 • I-1 I en rt fa H O cn O H 3 H) O H 0> en 13 tr rt H- O O O 3 O H fD rt 0) O rt cr 05 H cn O o 0) cn


-------
                       91-1*8
O  -o 50
-<  30 O
2E  O —I
53  o j>
"  m 23
   l/l -C
TYPE OF CONTROL .
UNCONTROLLED
PRECLEANER*
HIGH-EFFICIENCY CYCLONE
SPRAY TOWERb h
MULTIPLE CNETRIFUGAL SCRUBBER
BAFFLE SPRAY TOWERb
ORIFICE-TYPE SCRUBBER6
BAGHOUSE
CONTROL
EQUIP.
CODE
000
009
007
001
001
001
001
017
PARTICULATE
EMISSIONS
LC/TUN
45.0
15.0
1.7
0.4
0.3
0.3
0.04
0.1
t/1
DRYER
S FUEL
THE CODE 009  IS  FOR LOW EFFICIENCY
CENTRIFUGAL COLLECTOR.
IDENTIFY THE  SPECIFIC COLLECTOR
DEVICE IN COMMENTS.
                                                                                r-i
                                                                                O
                                                                                rt

                                                                                s-
                                                                               ><

                                                                                DJ
                                                                                H
                                                                               ^
                                                                                (D
                                                                                H

                                                                                0)
                                                                                3
                                                                                O
                                                                                rt

                                                                                (D
                                                                                H

                                                                                (0
                                                                                O
                                                                                £
                                                                                H
                                                                                O
                                                                                fl>
                                                                                cn
                                                                                     C
                                                                                     i-i
                                                                                     (D

                                                                                     oo
-6
Standard NEDS
                                                                           O
                                                                           H
                                                                           3

                                                                           l-ri
                                                                            0)
                                                                            cn
                                                                           'd
                                                                            tf
                                                                            cu
                                                                            H1
                                                                            rt
                                                                            H-
                                                                            n

                                                                            o
                                                                            o
                                                                            3
                                                                            o
                                                                            n
                                                                            CD
                                                                            rt
                                                                            (D

-------
                    Figure  8.1-7.    Standard  NEDS  form for  asphaltic  concrete  -  storage piles.
00


M
i
Suit
1 ?

Counlv
3

(

S

b

AOCH
)

8

9

PUm 10
ID

11


11 13

C
Illh
1
                                                     NATIONAL EMISSIONS DAT A SYSTEM (NtDSt

                                                      ENVIRONMENTAL PROTLCIU1N ACbNCY


                                                          QFMCE OF AIR PROGRAMS
                                                                            f ur-W AH^HG« ED


                                                                            Of.*b NO 1I>8 H0095
                             LLaiaiili
             j_LLn_LLUa]
                        LU-N : HOI
                                                                                                            ... I!     IILN
                                                                                       KT:7n7ni[io]bi1b?|s3TiiMti|c!|t[r^iT;ir^"^;it7ira|;;l)tl5|Ea
                                                                                       :ti±ii±j±±tl±j±i±ti±LjTiz
                                                                jR'l^-.R^i;l="-]^

                                                                    oioMo1oroTo!Ql'6|ol !'1
                        STORAGE

                         PILES
3lQ|5
.    J_


Q .0 ZJO"
                                                     UNIT - TONS PRODUCE
                                                                                                       0101010
                                                                                                       COM ROL HtGLH AT l
                                                               iiL-itnsni
                                                                                                   jfi
              ._




                  1
                                                    ±
                                                         T
.-.fl.
                                                                          rraTT.;
                                                                          -t-Kb-
bl|uUj|
-------
            Figure 8.1-8.    Standard  NEDS  form  for asphaltic  concrete  - cold aggregate handling.
00
•
t-1
I
I-1
00
                                                     NATIONAL EMISSIONS DATA SYbl EM (NEDSI
                                                       ENVIRONMENTAL PROTECTION AGENCY
                                                          OFFICE OF AIH PROGRAMS
                                                 PO:NT sou
                                                  input F-oi
FGHM API-HOVEL)

OMB NO Iba HJ09b

Daw	__
                                  '-

                                                              j»T17r4:iT• 1

i
Si
4-
driy
_1_L_LL1J
'.1 '-
~i"F


T 'iJ


',)•

y.
•T5T


S.'
V

b! ATI1S
UPDATE
\ , ..fj r/i , li .
r.Td^Ri"pnr
1
St
f"

i
F.i
.«

i
Hill

1
Tu
! ,,2

a
ti

M
.«
W




fi(

1
'•:
ftli

c
i
t)
t1
»

3N
ts
Ti
f-rt

K
6"

t>'J
F.'J

JL
Br
;o


/o

HE
2
71
?
P
?t

-
c
/?
-?

.A
(3


73

no
Iri,


n

NS
3


»

T"
4|L
_j
71
76


;;

_1
c

c
73


7S Sit
6
6
6
fa
cd
J'» 80
P 7
P 7
P 7
P 7

-------
                  Figure  8.1-9.    Standard  NEDS  form for  asphaltic concrete - asphalt heater.
CO

M
I
M
VD
                                                    NATIONAL FMISSIONS t)A]A SYSTEM (NEDS)
                                                      FNVIRONWNT/U PROTECTION Af.U'CV
                                                         OFFICF OF AIR PROGRAMS
                                                                                           POINT SOURCE
                                                                FORM APPROVED
                                                                OMB NO 158 ROOTS
                                      •
                                      6lo to | (HOjolQ[pToto.!QiOjo 1 o]o

                 ASPHALT HEATER
                            r_
                              ciffiffi
                                    ire
                             : s
                                          " SCC UNIT-MILLION "CUBIC FEET FOR NG;  1000 GALLONS FOR OIL
                                                                     ' • -- I

           f±i±

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1

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f
v





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61





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6
6
r,
6
E
NG -6; RESII). OH -7; DIST. OIL -E
                                                                             LIE

-------
                REFERENCES FOR SECTION 8.1
1.   Particulate Pollutant System Study,  Volume III -
    Handbook of Emission Properties.   Midwest Research
    Institute.   Prepared for the U.S.  Environmental Protec-
    tion Agency under Contract No.  CPA 22-69-104.   May
    1971.  p. 339-359.

2.   Compilation of Air Pollutant Emission Factors.  U.S.
    EPA.  Research Triangle Park, North Carolina.   Publica-
    tion No. AP-42.  February 1976.  Section 8.1.

3.   Process Flow Sheets and Air Pollution Controls.
    American Conference of Governmental and Industrial
    Hygienists.  1961.

4.   Asphaltic Concrete Plants Atmospheric Emissions Study.
    Valentine,  Fisher, and Tomlinson,  Consulting Engineers,
    Seattle, Washington.  Prepared for U.S. Environmental
    Protection Agency, Research Triangle Park, N.C., under
    Contract Number 68-02-0076.  November 1971.

5.   Danielson,  J.A. and R.S. Brown.  Hot-Mix Asphalt
    Paving Batch Plants.  In:  Air Pollution Engineering
    Manual, Danielson, J.A.  (ed.).  Environmental Protec-
    tion Agency, Research Triangle Park, N.C.  Publication
    No. AP-40.   May 1973.

6.   Von Lehmden, D.J., R.P. Hangebranck, and J.E. Meeker.
    Polynuclear Hydrocarbon Emissions from selected Indus-
    trial Processes.  Journal of Air Pollution Control
    Association.   15, No. 7:66-68.

7.   Asphalt Concrete Plants.  In:  Background Information
    for Proposed New Source Performance Standards.  En-
    vironmental Protection Agency, Research Triangle Park,
    N.C.  Publication No. 1352 A,  B, and C.  Volumes I and
    II, June 1973.  Vol. III.  February 1974.
                              8.1-20

-------
                    8.3  BRICK MANUFACTURING




                   1-4
PROCESS DESCRIPTION



     Brick manufacturing includes the production of heavy clay



products 'hricks, clay pipe, pottery) and some types of refrac-



tories.  The raw materials, which are mined in open pits or



underground, consist of clay, feldspar, and sand.  Clays are



basically hydrates of alumino-silicates with impurities of feld-



spar, quartz, and other minerals.  Various salts and minerals are



added to the raw materials, such as borax, soda ash, cryolite,



alumina, chromite, and magnesite.  Figure 8.3-1 is a process flow



diagram of brick manufacturing.



     The manufacture of clay products involves the grinding,



screening, and blending of the raw materials.  The ware is then



formed and fired  (maintained at a high temperature) to bring



about the drying and bonding of the materials.  Firing is fol-



lowed by the final cutting or shaping of the ware.  Although



there are many variations depending on the product being made,



these steps are common to all brick manufacturing.  In this



discussion the word "brick" refers to all products of this manu-



facturing, although many different wares are produced.



     When it is mined, the raw material is crushed to remove



stones, ground, and then screened.  During these operations the



separation and recycling of the minerals allow them to be sorted



                              8.3-1

-------
                                                                    Figure  8.3-1.    Brick  manufacturing  plant.
                                                                                                                                                     FABRIC  FILTER 017
                                                                                                                                                     ESP          Oil
                                                                                                                                                     WET SCRUBBER  002 (80-95)
         GRAVITY COLLECTOR    006 (<80
         CENTRIFUGAL COLLECTOR 009 (<80)
         WET SCRUBBER         002  80-95
         FABRIC FILTER        Oil (80-95)
                                                                                                                                                                         PART<2}
CO
 I
S3
                                                                               GRAVITY COLLECTOR      006 (<80
                                                                               CENTRIFUGAL  COLLECTOR  009 (<80)
                                                                               WET SCRUBBER          002 (80-95
                                                                               FABRIC FILTER         Oil (80-95
                                                                                                                          CYCLONE  008
                                                                                                                     MULTICYCLONE  007
J-P5-003-03
RAW MATERIAL
   STORAGE
                                                                                                                (<80)
                                                                                                                <80)
                                                                                                                80-95)
                                                                                                                (80-95)
                                                                                              GRAVITY COLLECTOR     006
                                                                                              CENTRIFUGAL COLLECTOR 009
                                                                                              WET SCRUBBER         002
                                                                                              FABRIC FILTER        Oil
                                                                                COMBUSTION PRODUCTS\

PART
SOX
CO
HC
"°v
TUNNEL KILN
GAS
0.04
Keg.
0.04
0.02
0.15
OIL
0.6
4. OS
Neg.
0.1
1.1
COAL
l.OA
7.2S
1.9
0.6
0.9
PER ODIC KILN
GAS
0.11
Neg.
0.11
0.04
0.42
OIL
0.9
5.95
Neg.
0.1
1.7
COAL
1.6A
12. OS
3.2
0.9
1.4
                                                                                                                                                                                       -SHIPPING
              LEGEND:

              Q EMISSION FACTOR*
              /-\ EMISSION FACTOR NOT DEVELOPED
                  FOR THIS PROCESS
               009 (66.0) DENOTES CONTROL EQUIP.
                  1     ' CODE WITH  EST. EFF. SHOWN
               o
                  IN (  )
                  DENOTES FUGITIVE
                  EMISSIONS
                  DENOTES A STACK
                                                                                 3-05-003-01
                                                                                  DRYING-RAW
                                                                                   MATERIAL
11 TUNNEL KILNS - GAS-FIRED
12 TUNNEL KILNS - OIL-FIBED
13 TUNNEL KILNS - COAL-FIRED
14 PERIODIC KILNS - GAS-FIRED
15 PERIODIC KILNS - OIL-FIRED
16 PERIODIC KILNS - COAL-FIRED

       3-9Q-QOX-99
     IN-PROCESS FUEL

 2 - BITUMINOUS COAL
 4 - RESIDUAL  OIL
 5 - DISTILLATE OIL
 6 - NATURAL GAS
               • IN POUNDS PER SCC UNIT

-------
into the desired particle sizes and composition.  The material



may then undergo calcining, a heat treatment used to drive off



volatile components; or it may be dried to reduce the moisture



content prior to mixing and blending.  The material is then



shipped by rail or truck to the brick manufacturing plant if this



is at another location.  Most clay mining and raw material pre-



paration are located in rural areas.  Brick manufacturing may be




located in metropolitan areas.



     At the plant the various types of clay are combined to



produce a uniform raw material and to allow control of color and



batch composition.  During the mixing operation, bonding agents



such as alkali silicates or organic binders may be added.



     The mixed clay is then molded or formed by one of three



processes:  stiff-mud, soft-mud, or dry-press.  In the stiff-mud



process, clay is mixed with water in a pug mill, which is a



mixing chamber containing two or more revolving blades.  When the



moisture content reaches 12 to 15 percent, the clay is just wet



enough to be plastic.  The clay is forced out through a die in a



screw or auger machine onto a cutting table, where it is cut by



wires to desired lengths.  Most brick and all structural tile are



formed by the stiff-mud process.



     In the soft-mud process, used when the clay is wet and in



making firebrick, water is added to the clay to reach 20 to 30



percent moisture; the mixture is formed in molds that are coated



with a thin layer of sand or water to prevent sticking.
                             8.3-3

-------
     In the dry-press method, clay is formed in steel molds under
500 to 1500 psi pressure.  The water content is 4 to 7 percent,
which makes the clay nonplastic.  High-pressure forming first
requires de-airing, which can be accomplished in one of four
ways:  control of the rate of application of pressure; applica-
tion of a vacuum; double pressing; or use of a gas.  De-airing is
performed as part of the molding operation.
     The wet clay forms are then placed in dryer kilns at 100°F
to 400°F for 24 to 48 hours.  Heat is usually supplied by exhaust
gases from the firing kilns.  Stiff-mud and soft-mud forms must
be dried before firing; the dry-press forms may be dried, de-
pending on the final product and the moisture content of the
forms.
     Firing  (also called burning) is the most crucial step in
brickmaking.  The clay forms are maintained at temperatures up to
2400°F for 40 to 150 hours in tunnel or periodic kilns that are
fueled with gas, oil, or coal.
     In tunnel kilns the bricks are loaded onto cars, which
travel down the kiln corridor at a rate of one 6-foot car per
hour through various temperature zones.  Drying occurs in the
first section at 100° to 400°F, followed by firing at 1400° to
2400°F, and, finally, cooling for 48 to 72 hours.  Because drying
takes place  in the tunnel kiln, no separate dryers are required
where kilns  are used.  In periodic kilns the dried forms are
placed in  furnaces having fireholes into which the fuel  is fired.
The  hot gases from the combustion circulating around the bricks
provide a  uniform  temperature distribution.
                             8.3-4

-------
     Several changes occur during the firing of the ware.  Any



free water not previously removed during drying is evaporated.



Stable mineral forms are developed through the liberation of



chemically combined water (water of hydration), followed by



calcination of carbonates and oxidation of ferrous materials.



Combustible matter is removed and some of the impurities undergo



decomposition.  Vitrification, a partial fusion of the silica,



alumina, and some impurities, produces a molten glassy material



that upon cooling permanently bonds the solid particles into a



tough hard product.  Flashing (color development) is also ac-




complished in the kiln.



     The output of tunnel kilns is from 100 to 250 tons per day,



with an air flow of 15,000 to 37,000 acfm.  The temperature of




the flue gases ranges from 300° to 550°F.



     After firing, the cooled product may be  subject to a final



cutting or shaping depending on its final use.  The product is




then ready for shipping.






EMISSIONS1"5



     The main air pollution problem associated with the brick



industry is the release of particulates, which range in  size  from



submicron particles to visible pieces of material.  Emission



sources are identified in Figure 8.3-1.  For  some of the sources,



AP-42  provides emission factors, which are listed on  the process




flow diagram.
                             8.3-5

-------
     During raw material storage and handling,  particulate emis-



sions arise from unloading,  wind, and retrieval activities.



Crushing and grinding the clay in preparation for forming the



ware also generate particulate emissions.  The  quantity of par-




ticulate emissions from calcining and drying of raw materials



depends upon the materials charged, dryer types, and final mois-



ture content.



     Particulates are emitted during the mixing and blending



operation until the material is sufficiently wet.  No emissions



occur during forming and molding of the wet material.



     The exhaust gas from the kiln contains particulates and



small amounts of SO , NO , HC, and CO.  Pollutants other than
                   X    X


particulates are a result of impurities in the  ware.  The pres-



ence of fluorite and fluoapetite components, for example, leads



to fluoride emissions; sulfur oxides are released at high tem-



peratures from iron pyrites or other sulfur-containing materials.



     The final cutting or shaping may cause minor amounts of



fugitive particulate emissions.





CONTROL PRACTICES1"3



     Emissions from raw material storage are not controlled.



Particulates emitted during crushing/grinding and screening are




controlled by gravity or centrifugal collectors, wet scrubbers,



or fabric filters.  The same devices can be used to control



particulates from raw material drying and calcining.  Emissions



from blending and mixing are not usually controlled, although
                             8.3-6

-------
good plant design and proper hooding are necessary to keep fugi-

tive emissions to a minimum.  When controls are used on these

sources they are the same types used on the crushing/grinding,

screening, drying, and calcining of raw materials.

     Particulates emitted during the drying and firing of the

product are controlled by fabric filters or electrostatic pre-

cipitators.  Wet scrubbers may also be usod for controlling

particulates, gaseous fluorides, and some S02 emissions.  Any of

these devices may be preceded by a settling chamber or a cyclone

or multicyclone.

     Emissions from final cutting or shaping are not controlled.


CODING NEDS FORMS5"

     The emission sources in a brick manufacturing plant are:

     Source                       SCC         Pollutant(s)

     Storage, raw material     3-05-003-03    Particulates

     Crushing/grinding         3-05-003-02    Particulates

     Screening                 3-05-003-08    Particulates

     Calcining                 3-05-003-07    Particulates

     Drying, raw material      3-05-003-01    Particulates

     Blending and mixing       3-05-003-09    Particulates

     Firing  (kiln)             3-05-003-OX    Particulates,
                                               SO. NO  , HC,
                                               COK    X

     In-process fuel           3-90-OOX-99

     Standard NEDS forms for each of the sources, Figures 8.3-2

through 8.3-8, show entries for the SCC's and other codes.

Entries in the data fields give information common to brickmaking

                              8.3-7

-------
operations.  Information pertinent to coding the source is



entered on the margins of the forms and above or below applicable



data fields.  Entries for control equipment codes, other optional



codes, emission factors, and required comments minimize the need



to refer to the code lists.  Typical data values for operating



parameters, control equipment efficiencies, and other source



information are shown on the form (or in the text) only to aid in



rapid, approximate checks of data submitted by the plant in a



permit application or similar report.  Data entered in EIS/P&R



and NEDS must be actual values specific to and reported by the



plant, rather than typical values.  Contact the plant to validate



or correct questionable data and to obtain unreported informa-



tion.  See Part 1 of this manual for general coding instructions.



     The emission source labeled "raw material storage" includes



loading onto piles, wind effects while the material is stored,



and retrieval activities.



     Crushing/grinding and screening are often vented to the same



control device, in which case identical values for stack height



and diameter are coded on the NEDS form for each operation;



consecutive point ID'S are entered under points with a common



stack  (Card 2, columns 56-59).  Figures 8.3-3 and 8.3-4 show



entries for these operations.  When crushing/grinding and screen-



ing are hooded, code the stack data; otherwise, enter a zero in



the stack height and diameter fields, 77 in the temperature



field, and appropriate plume height.
                              8.3-8

-------
     Raw material drying and calcining are not practiced at all



plants.  Figures 8.3-5 and 8.3-6 show the appropriate NEDS



forms.



     Emissions from mixing and blending are usually not controlled,



A standard NEDS form for this operation is shown in Figure 8.3-7.



     Since drying is accomplished with combustion gases from the



kiln, no separate SCC is assigned to the drying operation.



Exhaust gases from firing  (and drying) are often vented through a



control device before discharge to the atmosphere.  Where scrub-



bers are used, they may be used primarily to control gaseous



fluoride emissions.  Code the scrubber as a primary particulate



control device, however, unless it is preceded by another par-



ticulate control device, in which case code the scrubber as a



secondary device.  Figure 8.3-8 shows a standard NEDS form for



firing.






CODING EIS/P&R FORMS6



     The Basic Equipment Codes (EEC's) for use in EIS/P&R forms



are:



Source                          EEC



Raw material storage            712



Crushing/grinding             650, 653



Screening                     575, 579



Calciner                        231



Blending and mixing             485



Firing (kiln)                   231
                             8.3-9

-------
Figure 8.3-2.  Standard NEDS form for brick manufacturing - storage, raw material.
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-------
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Figure 8.3-5.   Standard NEDS  form for brick manufacturing - calcining.

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00
XX
C
64
0
X
3NTROL EFFICIEN
NO, HC
S9|60|61|62 63 64
J
59
n
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5
U
Ytir
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f
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61
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63
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nt>
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7?|73|
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lolo o o ^n
CONTROL REGULA
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1
71

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72 73
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74 75

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71

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ll U
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c
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71 75^ K
r
|
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p

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cd
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-------
Figure 8.3-6.  Standard NEDS form for brick manufacturing - drying (raw material).
oo
u>
I
State,
1

2

County
3

4

5

6

AOCR
7

1

9


Plant IO
Number
10


11


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12



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•


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31
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r


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rx
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106 BTU/h
II

11

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Dec-
41
11
70

71

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May
20
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a
1
II
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19
20
II
11
0




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S





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23
24
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71

u
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71

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sec
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71
n




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n




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T




sec
71



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V

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Sept-
Nov
24_

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74
0




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1





24



75



76
rM
ont
26
77
CO
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27

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1
—
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29
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V
ill
30
1A1
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kn
»
NATIONAL EMISSIONS DATA SYSTEM (NEDS)
ENVIRONMENTAL PROTECTION AGENCY
OFFICE OF AIR PROGRAMS
Ellablithment Nome and Addict!
_3l|32i33|34|35|36l37|34|39|40|4ll42|43|44|4S|46|47[4«|49
rES
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ING
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o
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76





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33





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(1




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f
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41
II
50
.

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111

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lo
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Si
so
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0
ION ESTIMATES Itont
NO,



1||
0
nl
69
70
71
RM APPROVED
KB NO. 168-80095
t»

72
73
1
74
300 IF NO COMMON STACK
KXX POINT ID'S IF COMMON
il
64
EFFICIEN
HC
67

CO
TT

63

77

JCE
5
E
Osv
62 111


64
0
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a.
u
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65
6i
67
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65


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66

t
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fifi

67
a.
61

61

69

(9

70

70

JTIMATION
METHOD
ffd 0 0

-------
Figure 8.3-7.   Standard NEDS form for brick manufacturing - blending and mixing.
00
OJ
1
M
Ui
SI
1

"•»
2

County
3

4

5

(

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IT

i

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10



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14

12

11

C
14

)
11


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Point
10


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-

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-

ty
IS

17

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k O
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16

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16

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16





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-

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—

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11

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}]
70

71

SIC
11
3
13
2
20
5
21
U
NATIONAL EMISSIONS DATA SYSTEM (NEDS) POINTS
ENVIRONMENTAL PROTECTION AGENCY ""*"
OFFICE OF AIR PROGRAMS "'™ °' Per'°"
Completing Form
Establishment Name and Addiesi
22

23

a. £
* 8
. £
22

Boiler Design
Capacity
IO6 BTU/hr
u1

13

XAt
D«-
fto
11

13

20

21

»JNUA
Mar-
Hit
20

21

22

23

24

25

26

21

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Hori/onlal
24

25

Pr miry
Pl.t
23

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June
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22

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24

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Sepi-
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24

Particu ate
11

1
11
3




i
18



13

20

n
13
0




20
5




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19



20



21

22

23

sec
III
21
0




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U




23
3




sec
III
21



22



23



24

25

26

27

28

23

30

31

32

OROINATES
Vt'liu
21

•o «
C J
5 *
»
26

21

NO
OPE
5
i
25|27

21

MM
^A^
Jt
n
21

29

30

31

Pr mary
so? _,
29
U
30
0
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ING
5
23

30

31
U
32

33

34

35

36

Height  6O
ti
a
u
0
39
0
40
0
41

42

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Puma
HC
41
0
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U
43

44

45

46

47

41

49

50

51

52

53

54

A
fclume Height
Flow Rale It^/min [lino slack It
44

45

46

47

41

49

50 51

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43
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Fu., ,.^?.?C W
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25





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21





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33

34

35

36

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33

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41

42

41

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n
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47
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41
0
49
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a
50
0
51
U
ION ESTIMATES (com
NO,
45

ns/year
MC
33

IT - TONS RAW
MOuny
Maximum Design
Rate
33





34





35





36





3;





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41

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53

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56

57

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59

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with
common
stack
U

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+
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57

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/ye«r)
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46

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43

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106 BTU/ICC
46





47





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50





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52
D
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53

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54

55

56

57

IANCE
3ULE
Mo
56

57

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o
4

60

61

OURCE FC
Form O*
Ol
HM APPROVED
«BNO. 1S8-F(0095

Contact • Personal
62

63

64

65

66

67

61

69

70

1

72

73

I
74


75

76

77

0000 IF NO COMMON STACK
-/XXXX POINT ID'S IF COMMON STACK
60

61

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NO,
59

60

61
U
a.

U

64

EFFICIEN
HC
62

63

64
U
65

66

67

CY(%)
CO
65

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53

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S
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Year
51

59

60

61

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rATir
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60

61

62

63

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Day
62

63

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<
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64

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p
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67
n
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60





61





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n

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71





72

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7?





73
L£
r< -5 -; -i.-rl

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R«tj3
73
_
74

75

76

c
ll ' •
< rr
T TK


77


73





74





75





76





77





COMMENTS
11



27



21



25



30



31



32



33



34


35



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37



36



39



40



41



42



43



44



45



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47



48



49



50



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52



53



54



55



56



57



51



SS



60



61



62



63


64



65


66



67



68


69



70



71



72



73



74


75



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71

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78





c
c
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<
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4
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*

73
p
p
p
p
p

79
r
P
P
rt
K
6
6
6
6
S
of
r
7
7

-------
Figure 8.3-8.   Standard NEDS form for brick manufacturing - curing and firing (kiln).

State,
1

7

County
3

4

5

(

00
w
^ 09 TUNNEL KILN,
11 TUNNEL KILN,
12 TUNNEL KILN,
13 PERIODIC KIU
14 PERIODIC KIU
15 PERIODIC KIU
IN-
2 - COAL
4 - RESI
5 - DIST
f> - NAT11
m
AOCH
7

1

9


Plant IO
Number
10


11


Po
.10
u
CAS FIRED
OIL FIRED
COAL FIREI
1, GAS FIRB
^, OIL FIRt
1, COAL Fit
:URING (KII
PROCESS FUI
DUAL OIL
ILLATE OIL
(AT. flAS
12




.D
.D
IEI
JO
:L
Po
U

13





)


ml
IS


"o
1

"o
m
"o
'o
m
I

16


T)

TJ
5
•c
0
•o
5
*
o
11

n

Ut


m


t


I


NATIONAL EMISSIONS DATA SYSTEM (NEDS)
ENVIRONMENTAL PROTECTION AGENCY
OFFICE OF AIR PROGRAMS
2j|?il«lKl>cljjhilj*linhllljl33l34l3Sl36l37lul39l40l4l|42|43|44|45|4.|47|4!|4S|»

4 *
Boiler Detign
Capacnv r
%
D



18

M
ۥ

19

19

Nl
W

20

20

JAL
ir-

S
21
5fi
21

THF
June

cc
HI
22 2
5
22 !

H<
U
>nr
DOS
nmary
(UPU
Se

1

3 24

T
PI-

n
25

fMC
onlal
OOR
> o
Ilo
N(
OPE

0
n

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i
SO;
Solid
•»ien»
7 71

Dir
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17
11
D2
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en
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ES
cal
31
OR
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W 11
r
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ALLOV1
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71

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11

32
33
34
f.
t 1
36
D,
CONTR(
Primary
NO,
35 36 37
:E TABLE 8.
Particulate
3
Jl
JL
31
1
3s
/ABLE EMISSIONS (to
NO,
;; 33 34 : 5 36 3) 31
in
32
UN
F,R
17

m
M
33
^E
ro
n

r -
ixir
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L 1
11
M

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nun
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p
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It
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Is
39
IT
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40
40"
ACK DA'
emo I°FI
41 42 43
JIPMENT
Primary
HC
41 2 43
50;
7T
it/year)
RO
[ 11
11
39
DU
i
r
-o
14
"40
CEI
LM
J4l|
Ab
-G
42
HC
42
D
i
'.
o
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F
AS
"4?
»
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f
44

46
lo
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EMISS
43J44
~43
1
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F

[44]
5
44
:D
[Rl
47

te ll|3/rTlin)
Pnma
CO
47J4I
ry
"49





Plume Height
1 no stack ft
lo
ju
51
ON ESTIMATES lioni
NO,
D
45
:
:
45
;D

46
HI
in
k


CO
[4j«|49]
«'«
[iTI
15
IT

uel
Tl
^L
-0
4?

len
F
IL

[50]
[50
[R
F

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1
:D
[RI
"sT




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Pan
year)
52JS3

1
:D
IF

(/i
a
1
13-
"sT

[si]
nr
SCHE
Year
[S4
-
16
54

1
M
-C
55

POINT S
Input
Name of Person
Completing Form
|56|57|St|S9|60|61
Wl
comr
tta
5«|5T
h
non
rk
«IATEDC(
SO;
[ssj
TT]
3ULE
Mo
S6|57
n
M
OA
sT

IT]
F
L
SI

V)

_^
X
Til
3NTROL
NO,

S
u
Yew
SO
[R
FI!
IT

C
JU
?EI
59



TATU
POAT
Mo
on-
m\
5
60

m«
Tii
IF

OURCE FORM AFWOVED
Forn, O*"8 N0' 'S»-R009S


00
XX.
[fi

uu
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c
I
p
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on
f
31!
65
acl
MO

-------
GLOSSARY


Burning - See Firing.

Calcining - The heat treatment to which raw refractory materials
are subjected preparatory to further proc :ssing or use, for the
purpose oi eliminating volatile chemically combined constituents
and producing volume changes.

Curing - See Firing.

Firing - The controlled heat treatment of ceramic ware in a kiln
or furnace during the process of manufacture to develop the
desired properties.

Flashing - Firing a kiln under reducing conditions to obtain
certain desired colors on clayware.

Plasticity - The property of a material that permits it to be
deformed under stress without rupturing and to retain the shape
produced after the stress is removed.

Refractories - Materials used to withstand the thermal, chemical,
and physical effects in furnaces.  Refractory materials include
firebrick, silica brick, magnesite brick, and chromite brick.

Vitrification - The progressive partial fusion of a clay as a
result of a firing process.  As vitrification proceeds, the pro-
portion of glassy bond increases and the apparent porosity of the
fired product becomes increasingly lower.
                              8.3-17

-------
              REFERENCES FOR SECTION 8.3


Particulate Pollutant System Study.   Vol.  Ill - Handbook of
Emission Properties.  EPA-22-69-104, May 1971.

Compilation of Air Pollution Emission Factors.  2nd edition,
Environmental Protection Agency, Publication AP-42.  February
1976.

Shreve, N.R.  Chemical Process Industries.  2nd edition.
McGraw-Hill Book Co, New York,  1956.

industrial Process Profiles for Environmental Use, Chapter
19:  The Clay Industry.  EPA-600/2-77-023s, February 1977.

Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA-
450/2-76-005  (OAQPS No. 1.2-042), April 1976.

Loquercio, P. and W. J. Stanley.  Air Pollution Manual of
Coding.  U.S. Department of Health, Education  and  Welfare,
Public  Health Service  Publication No. 1956.   1968.

Aeros Manual Series Volume  II:  Aeros User's  Manual.  EPA-
450/2-76-029  (OAQPS No.  1.2-039), December  1976.

Vatavuk, W.M.   National Emission Data System (NEDS)  Control
Device  Workbook.  U.S. Environmental  Protection Agency,
Publication No. APTD-1570,  July 1973.

Standard  Industrial Classification  Manual.   1972  edition.
Prepared  by Office  of  Management and Budget.   Available from
 Superintendent  of Documents,  Washington,  D.C.
                         8.3-18

-------
             8.6  PORTLAND CEMENT MANUFACTURING




                   1-4
PROCESS DESCRIPTION


     The major use of Portland cement IF in making concrete,



which is a mixture of cement, aggregates consisting of sand



and gravel or crushed rock, and water.  The product is used



in construction of highways, dams, buildings, and other



structures.  Cement is produced by heating to the point of



fusion a finely ground combination of limestone, cement



rock, marl or oyster shells, and shale, clay, sand, or iron



ore.  The fused product, called cement clinker, is ground to



a fine powder and shipped  in bags or by bulk carrier.



     Raw materials are received by truck, barge, or rail and



unloaded by a clamshell or discharged into a receiving pit



or hopper.  Many  cement plants are located near stone quar-



ries, which supply crushed stone of  specified  size.  Quarry-



ing  operations  are described elsewhere.  Other  plants use



primary and secondary crushers and screens to produce stone



of  specified  size.   The stone usually  is unloaded  directly



into a crusher  hopper, crushed and screened, and  then trans-



ferred to  raw material piles or  feed silos.  The  other  raw



materials  may be  conveyed to open piles or directly  to  feed



silos.  These materials may or may not  be  crushed.
                             8.6-1

-------
     Raw materials from the silos are proportioned and fed




to a grinding mill.  Depending on the type of grinding, the




cement production process is called dry or wet.  In the dry



process, the raw materials may be dried separately before



grinding, but more commonly, grinding and drying are done



simultaneously.  Some plants grind the raw materials sepa-



rately and then blend them in specified proportion.  Exhaust



from the rotary kiln that follows this step supplies hot



gases for drying.  Figure 8.6-1 is a flow diagram of a



typical dry process plant.



     In the wet process, the slurry leaving the grinding



mill is 30 to 40 percent water; 70 to 90 percent of the



solids are smaller than 200 mesh.  The raw materials may be




proportioned and blended before grinding or the slurries may



be blended after grinding.  The blend may be vacuum-filtered



to about 20 percent water.  Except for the difference  in



grinding, the dry  and wet processes are  identical.  Figure



8.6-2 is a flow diagram of  a typical wet process plant.



     The dry or wet mix is  fed into the  raised end of  a



gently  sloping rotary kiln, the  far end  of which  is fired



with oil, gas, or  coal.  As the  feed travels slowly down the



kiln, which may be as much  as  350  feet long, it is exposed



to  increasingly higher  temperatures  from the hot  gases



traveling up the  kiln.  The feed  is dried, calcined,  and




                             8.6-2

-------
                                                      V  WWT Q
                   1 PART O          » PART. Q
                                                      RAH MATERIAL TRANSFER
                                                       .PART
C3
 i
00
                             LEGEND
                             O EMISSION FACTOR3
                                 ©EMISSION F«CTOR NOT  DEVELOPED
                                 FOR THIS PROCESS
                             009 (66 0! DENOTES CON'RCL EOUIP
                             l          CODE WITH ESI  EFF  SHOWN
                             *          IN ( )
                             \         DENOTES FUGITIVE
                              I         EMISSIONS
                             O       DENOTES A STACK
                                                                                                                                                                                                            ESP 010 (96)
                                                                                                                                                                                                            BAGHOUSE 016(99 8)
                               IN POUNDS PER SCC UNI
                                                                          CEMENT LOADOU
                                                                              Figure  8.6-1.    Dry  process  Portland  cenont  plant.

-------
t PWT.O
UK *TE«IAL
TO 8E CRUSHCO rua. Q , PWT. Q . PA«T. ©
LPRIWHT
cntSHCi
3-05-007-C*
p«N*i ausmm
O
n
^
VIUATIK . SECOP11W __— .
• xaa •• CRUSHER 1 '
3-05-007-11 1 VOWKT-1C 1
SCTSEKW I SECamART cMlilRt 1
9

t SECOHOABY I ' - T^-. ''AC.X)"
•PMT.O PAP.T O / FI.ESTOWSTE 	 8AGHOUSE 016 (99 8 _ _
\ . / OH PROCESS -,---ir,.r c,.« m B»U«USE 018 (99 8! •_, ,„„
DENOTES FUGITIVE FKESJO PA«lt>, SSSl M, SEPARATE «_^

Q OFNOTFI A STACK * fwi Q 	 [' 	 | 	 | \\ Cll*Kt T«A«SF « | 	 1
1 IN POUNDS PER SCC UNIT CMirr SILOS *'" \A S = 5
LOAOIK ^l^^i^^ | | \$\ o d u
JTJr 	 — 7 1 V\/\X \V "OT*" 1 1 	 " - -'
'"*>'° F[«AL PWOOCT CsSfBT KIL|. CL1™
CEMEHT LOADOUT "~' " ' '~J^ ^^^^

CLINKEB GRIKDING -^— _- . Ji-
f
-I
FINES TO
PROCESS
PART 0
R COOLER
't
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                        Figure  8.6-2.   Wet  process Portland cement plant.

-------
eventually partly fused at a temperature of about 2900°F.


Residence time in the kiln is 1 to 4 hours.


     The clinker is discharged from the kiln into a clinker


cooler and is cooled by a stream of air.  At least part of


the clinker-heated air is used as combustion air for the


kiln.  The cooled clinker is transferred to storage piles or


silos.


     Clinker is withdrawn from storage, mixed with about 5


percent gypsum (which regulates the setting time of the


cement), then ground and mixed in a grinding mill.  Milled


cement is classified by a cyclone separator, and the over-


size material is returned to the mill.  Proper sized cement,


about 90 to 100 percent smaller than 325 mesh, is conveyed


to storage silos.  From there the product cement is bagged


or shipped in bulk by truck, rail, or barge.


EMISSIONS4"6


     Particulate is the major pollutant from cement plants.


Emission sources are identified in Figures 8.6-1 and 8.6-2.

                              4
For some of the sources, AP-42  provides emission factors,


which are listed on the process flow diagram.  For other


sources of emissions, average emission rates obtained from


other documents are mentioned in the following source


descriptions.
                            8.6-5

-------
     Particulate emissions occur from raw material unload-



ing, storage piles,  crushing, screening, and conveying and



transfer operations.  Unless confined, all of these are



fugitive emission sources.  Emissions from raw material



unloading range from 0.03 to 0.4 Ib/ton; from storage, 3.0



to 5.0 Ib/ton; from primary crushing, about 0.5 Ib/ton; from



secondary crushing and screening, about 1.5 Ib/ton; and from



conveying and transfer operations, 0.2 to 0.4 Ib/ton.



     In the wet process, no emissions occur from raw mate-



rial grinding and subsequent transfer into the kiln.  In



the dry process, emissions occur from grinding and from




feeding the kiln.



     The kiln and the cooler are the major sources of



particulate emissions.  Burning of fuel in the kiln also



emits combustion products.



     Particulate emissions from discharge of clinker onto



piles, wind effects, and retrieval activities range from  5.0



to 10.0 Ib/ton.   Clinker grinding, transferring the cement



into silos, and subsequent bulk loadout or packaging all



generate particulates.



CONTROL PRACTICES



     Options for reducing or controlling emissions from




unloading include the use of water sprays and enclosures,



with or without venting to a baghouse.  The raw materials
                             8.0-6

-------
are stored in stockpiles or in silos.   Although emissions



from conveying are minimal, conveyors are sometimes par-



tially covered to reduce the emissions.  Emissions caused by



transfer of materials from one conveyor belt to another are



sometimes controlled by venting the transfer point to a



baghouse.  Telescoping chutes, adjustable stacking con-



veyors, and stone ladders are the options available for



reducing emissions from discharging onto t1 e stockpiles.



All of these reduce the free-fall distance and, hence, the



fugitive emissions.  Water spraying of the material before



discharge onto the pile reduces the emission potential.



Stone  is commonly unloaded  (dumped) directly into a crusher




hopper.



     Primary and secondary crushers and  screens are often



located below grade; this  reduces the  potential for fugitive



emissions.  Suppression of dusts by water sprays at the feed



points of both primary and secondary crushing  and screening



operations  is common.  Some plants vent  the discharge




points to a baghouse.



     Raw materials  are usually retrieved from  stockpiles



with a clamshell,  front-end loader, or bulldozer  and  fed  to



a  belt system, which transfers them to the  feed silos.



Emissions  from retrieval  and  subsequent  transfer  to the belt




system usually are not controlled.
                             8.6-7

-------
     In the dry process,  emissions from the grinding circuit



are usually vented to a baghouse.   Cyclones are an integral



part of the grinding circuit.   In the wet process, the



grinding circuit generates no emissions.



     The rotary kiln is equipped with a cyclone followed by



an electrostatic precipitator (ESP) or baghouse to control



particulate emissions.  A large part of the sulfur oxides



(SO-) from burning of fuel is retained in the cement clinker



by the lime.  In addition, about 50 percent of the S02 that



enters the baghouse is removed by reaction with the cement



dust cake on the bags.  Oxides of nitrogen are not con-



trolled.  The cooler usually is equipped with a cyclone



followed by a baghouse or electrostatic precipitator.



     Emissions from discharge of clinkers onto a storage



pile or into a storage pit are sometimes reduced by use of



telescoping chutes, which reduce the free-fall distance.  At



least one plant discharges the clinker into an enclosed



structure vented to a baghouse.  Some plants use open-ended



structures with sidewalls for storage of clinker; usually,



however, these partial enclosures are not sufficiently



confining to prevent fugitive emissions from windage and



loading onto the pile.  A clamshell or front-end  loader



retrieves the clinkers from the pile, or an elevator lifts



the  clinker from the pit, and transfers it onto a belt
                             8.6-8

-------
system,  which conveys the clinkers to the storage or feed



silos for the grinder.  Emissions from clinker retrieval and



subsequent transfer to the belt system usually are not



controlled.  Some plants vent the silo loading points to a




baghouse.



     Emissions from clinker grinding are usually controlled




by a baghouse.  Conveying and transfer of the cement is



accomplished by belt or pneumatic conveyoi and is usually



well confined and controlled both for prevention of product



loss and for particulate control.  Air from the the pneu-



matic transport system is typically exhausted to fabric




filters.



     Cement storage silo vents  (for the discharge of dis-



placement  air as cement is fed  to the silos) are either



uncontrolled, covered by fabric "socks," or exhausted to




fabric  filters, which are part  of the pneumatic conveying



systems.   The trend is toward exhausting to fabric filters.



     Cement loading for bulk truck, rail, and ship/barge



transport  is  typically by gravity feed systems, which are



partially  enclosed  (in truck and rail loading) or unconfined



 (in  ship/barge  loading).  Some  plants exhaust the cement



dust, which  is  emitted with displaced air during  loading  and



packaging, to fabric  filters,-  others use  no controls.   Load-



 ing  or  packaging  aspiration  systems, which  consist  of  a
                             8.6-9

-------
filling spout with an outer concentric  aspiration  duct
vented to a fabric filter, are being  used  increasingly.
CODING NEDS FORMS
                 7-9
     The emission sources associated  with  cement  production
are :
     Source
Raw material unloading
Raw material p^'les
Primary crushing
Secondary crushing
Screening
Raw material transfer
Raw material grinding
Kilns

(Inprocess  fuel)
   Residual  oil
   Distillate oil
   Natural  gas
   Coal
Clinker  cooler
    SCC
 3-05-OOX-07
 3-05-OOX-08
 3-05-OOX-09
 3-05-OOX-10
 3-05-OOX-ll
 3-05-OOX-12
 3-05-006-13
 3-05-OOX-06


(3-90-004-02)
(3-90-005-02)
(3-90-006-02)
(3-90-002-01)
 3-05-OOX-1A
    Pollutants
   Particulates
   Particulates
   Particulates
   Particulates
   Part iculates
   Particulates
   Particulates
   Part iculates,
combustion products
   Particulates
                             8.6-10

-------
     Source                  SCC             Pollutants



Clinker piles            3-05-OOX-15         Particulates



Clinker transfer         3-05-OOX-16         Particulates



Clinker grinding         3-05-OOX-17         Particulates



Cement silos             3-05-OOX-18         Particulates




Cement loadout      -     3-05-OOX-19         Particulates




     The codes for X in the SCC's are:  6 for the dry




process and 7 for the wet process.



     Standard NEDS forms for each of the sources, Figures



8.6-3 through 8.6-16,  show entries for the SCC's and other




codes.  Entries in the data fields give information common



to cement plants.  Information pertinent to coding the



source is entered on the margins of the forms and above or



below applicable data fields.  Entries for control equipment



codes, other optional codes, emission factors, and required



comments minimize the need to refer to the code lists.



Typical data values for operating parameters, control equip-



ment efficiencies, and other source information are shown on



the form (or in the text) only to aid in rapid, approximate



checks of data submitted by the plant in a permit applica-



tion or similar report.  Data entered in EIS/P&R and NEDS



must be actual values specific to and reported by the




plant, rather than typical values.  Contact the plant to




validate or correct questionable data and to obtain unre-




                           8.6-11

-------
ported information.   See Part 1 of this manual for general



coding instructions.



     The emission source labeled "raw material piles"



includes loading onto piles, wind effects while the materi-



als are stored, and retrieval activities.  Raw material



transfer operations that are not included under unloading,



storage piles, primary and secondary crushing, and screening



are grouped under the emission source labeled "raw material



transfer."  Figures 8.6-3 through 8.6-8 illustrate the



standard NEDS forms for these six sources.  Emission factors



for these sources have not yet been developed.  When a plant



furnishes emissions data for these sources, code the values



given.  Enter "Emission Estimates Given by Plant" in the



comments field on Card 7.  Where there is no control device



or where water sprays are used, enter zeros in the stack



height and diameter fields,  77 in the temperature field,  and



zeros in the common stack field.  Enter appropriate height



in the plume height field.   Where water  sprays are used,



enter 061 or 062 as a control equipment code.  In the  com-



ments field on Card 6 identify other  equipment used  to



reduce emissions.   For  example,  enter "stone  ladders"  where



these are used for  transfer onto storage  piles.



      Figure  8.6-9  shows  the standard  NEDS form for  the



grinding mill in a  dry  process  plant.   Rotary kilns and
                            8.6-12

-------
clinker coolers are the major sources of particulate emis-



sions in both dry and wet processes.  Coal is the fuel used



most commonly for firing the kilns.  Figures 8.6-10 and



8.6-11 show standard NEDS forms for these two sources.



     The emission source labeled "clinker piles" includes



discharge (loading) onto piles, wind effects while the



clinkers are stored, and retrieval activities.  The source



labeled "clinker transfer" includes the operations involved



in transferring the retrieved clinkers to the silos.  Figures



8.6-12 and 8.6-13 show standard NEDS forms for these two



sources.



     Figures 8.6-14 through -16 show standard NEDS forms for




clinker grinding, cement silos, and cement loadout opera-



tions.
                            8.6-13

-------
CODING EIS/P&R FORMS10




     The EEC's for use in EIS/P&R forms are:
               Source



     Raw material unloading



     Raw material piles



     Primary crushing



     Secondary crushing



     Screening



     Raw material transfer



     Raw material grinding



     Kiln



     Clinker cooler



     Clinker piles



     Clinker transfer



     Clinker grinding



     Cement silos



     Cement loadout




  As of April 1978.
  BEG




  700



  700



  650



  650



575, 577



  700



653, 654



  230



no code*



  700



  700




653, 654



no code*



  700
                           8.6-14

-------
              Figure  8.6-3.  Standard NEDS form for Portland Cement Manufacturing -  raw material  unloading.
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-------
             Figure 8.6-4.  Standard NEDS  form for Portland Cement  Manufacturing - raw material piles.
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-------
                  Figure  8.6-5.   Standard NEDS form  for Portland Cement  Manufacturing - primary crushing.
CO

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                        n[n
 NATIONAL EMISSIONS DATA SYSTEM (NEOS)
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                   Figure 8.6-15.    Standard NEDS form for Portland  Cement Manufacturing -  cement silos.
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-------
GLOSSARY

Barrel - One barrel of cement weights 376 Ib; there are 5.32
     barrels per ton of cement.

Clamshell - A crane with a bucket having two hinged jaws.

Clinker - The fused product of the kiln, cement chunks.

Stacking cr" veyor - A belt conveyor that discharges at the
     storage pile.  Use of conveyors that rise and fall with
     the storage pile reduces the distance that the material
     must drop.

Stone ladder - A fixed column containing a series of steps
     that allow the falling material to cascade in short
     drops.  As the storage pile increases, the material
     discharges through ports in the sides of the column and
     emissions are reduced.

Telescoping chute - A column that can be raised or lowered
     to maintain a constant distance between the coal being
     discharged and the top of the storage pile.
                            8.6-29

-------
                REFERENCES FOR SECTION 8.6
1.  Kreichelt, T.E., D.A. Kemnitz,  and S.T.  Cuffe.  Atmos-
    pheric Emissions from the  Manufacture of Portland
    Cement.  U.S. Dept. of Health,  Education, and Welfare,
    Cincinnati, Ohio.  PHS Publication No. 999-AP-17.
    1967.

2.  Process Flow Diagrams and  Air  Pollution Emission
    Estimates.  Cincinnati,  American Conference of Govern-
    mental Industrial Hygienists.   Committee on Air Pollu-
    tion.  1973.  pp. 52-54.

3.  Considine, D.M.   (ed).   Chemical and Process Technology
    Encyclopedia.  New York, McGraw-Hill Book Co.  1974.
    pp. 237-240.

4.  Complication of Air Pollution  Emission Factors.  2nd
    edition, 3rd Printing.   Environmental Protection
    Agency, Research Triangle  Park, N.C.  Publication AP-
    42.  February 1976.  pp. 8.6-1 8.6-4, C16.


5-  Inspection Manual  for the Enforcement of New Source
    Performance Standards:  Portland  Cement Plants.
    Environmental Protection Agency,  Research Triangle
    Park, North Carolina. EPA 340/1-75-001. January ly75
6.  Technical Guidance  for  Control of Industrial Process
    Fugitive Particulate  Emissions.  Environmental Protec-
    tion Agency,  Research Triangle Park, North Carolina.
    EPA-450/3-77-010.   March 1977.

7.  Aeros Manual  Series Volume II:  Aeros User's Manual.
    U.S. Environmental  Protection Agency, Research Triangle
    Park, North Carolina.  Publication No. EPA-450/2-76-029
     (OAQPS  No. 1.2-039).  December 1976.
                           8.6-30

-------
 8.   Aeros Manual Series Volume V:   Aeros Manual of Codes,
     U.S.  Environmental Protection Agency, Research Triangle
     Park, North Carolina.   Publication No.  EPA-450/2-76-005
     (OAQPS No.  1.2-042).  April 1976.

 9.   Standard Industrial Classification Manual, 1972 Editxon,
     Prepared by Office of  Management and Budget.  Available
     from Superintendent of Documents,  Washington, D.C.

10.   Loquercio,  P.  and W.J. Stanley.  Air ?ollution Manual
     of Coding.   U.S.  Department of Health,  Education, and
     Welfare.  Public  Health Service Publication No. 1956.
     1968.
                           8.6-31

-------
                     8.9  COAL CLEANING

PROCESS DESCRIPTION
     Coal IF Cleaned to remove impurities s ch as dirt,
clay, rock, shale, iron, wood, and some sulfur.  These
.mpurities are present in coal in its natural state or are
added accidentally when the coal is mined.  Their removal
increases the heating value of the coal and reduces emissions
of sulfur oxides when the coal is burned.
     Coal cleaning plants are usually  located at the mine.
Their  capacities  range  up to  2000 tons per hour, with  an
average  of  about  500 tons per hour.  There are  three basic
types  of coal preparation plants:   (1) complete preparation
plants,  which clean  both coarse  and  fine  coal;  (2)  partial
preparation plants,  which clean  only coarse  coal;  and  (3)
coal crushing plants,  which crush the  coal  to specified
 sizes.  The complete preparation plant is discussed here,
 since its  operations include those of  the other two types.
      Figure 8.9-1 shows a typical coal cleaning plant.  Coal
 is usually carried by belt conveyors to the crusher where  it
 is prepared for the cleaning plant or for shipment.  The
 crusher is designed to discharge the  slate and rock to a
                               .9-1

-------
                                                                                                         WET CLEANING
                                                                                                           PROCESS



o




CHKMON TnOM THERMAL DRYERC

TYPE OF
; DRYER

FLUID BED
FLASH
MULTILOUVERED
V
EMISSIONS
LB/TON

CONTROL .,,.,
DEVICE °01

	 «
20 |
16 ^_
' 3 ;

-*-



CYCLONE

1-FLU ID!ZED BED
2-FLASH
3-MULTI LOWERED
4-ROTARY
5-CASCADE
6-CONTINUOUS
   CARRIER
7-SCREEN
PART.
           LEGEND.

           Q EMISSION FACTOR'

              0EB!5S!ON FKTOR NOT DEVELOPED
              FOR THIS PROCESS
           009 (66.0) DENOTES CONTROL EOUIP
           .          CODE WITH EST. EFF  SHOWN
           O
                     IN  (  )

                     DENOTES FUGITIVE
                     EMISSIONS

                     DENOTES • STACK
             IN POUNDS PER SCC UNIT
                                                                                     Figure  8.9-1.    Coal  cleaning  plant.
                                                                                                          8.9-2

-------
refuse pile.  A bar screen following the crusher separates
the oversize fraction and returns it to the crusher.  The
crushed coal is conveyed to storage silos.  Coal to be
cleaned is conveyed to vibrating screens, which separate the
coal into several size fractions.  The large and small sizes
of screened coal are moved by conveyors to separate cleaning
circuits.
     Impurities are separated by wet and dry processes.  In
the United  States, approximately 93 percent of the  coal
produced is cleaned by the wet process, in which water or a
mixture of  water and hematite is the medium and separation
is effected by gravity, centrifugal force, air, or  a pulsa-
tion column.  In the dry process, air  is the medium and
separation  is done on  "air tables."  In both processes
separation  is based on differences  in  specific gravities of
the various materials.
     Wet separation is followed  by  recovery of the  medium
 (hematite)  and by mechanical dewatering  of the coal, after
which  the  smaller coal particles are sometimes dried ther-
mally,  depending  on product  specifications.   The  dried coal
 is  usually mixed  with  a  larger  coal fraction,  and the
mixture is conveyed  to storage  piles or silos or  is loaded
 directly into railroad cars,  trucks, or barges.
      The fluidized-bed dryer (sometimes called "fluid-bed")
 is commonly used for drying the fine coal.   In this device
                              8.9-3

-------
the coal is suspended in a fluid state above a perforated

plate on a rising column of hot combustion gases.  The

entrained coal is separated from the hot gases by cyclones.

Other types of dryers used for coal drying are flash, multi-

louver, rotary, cascade, continuous carrier, and screen

dryers.  The three most common are the fluidized bed, flash,


and multilouver.



EMISSIONS3'4

     Although combustion products are emitted from the


dryer, coal particulate is the major pollutant in coal

cleaning operations.  Emission sources are identified in
                                             4
Figure 8.9-1.  For some of the sources, AP-42  provides


emission factors, which are listed on the process flow

diagram.  For other  sources,  average emission rates  obtained

from other documents are mentioned in the following  source


descriptions.

     Most coal  cleaning plants are located near  the  mouth of

the coal mines.   Coal is conveyed  from the mine  to the

cleaning plant  by semi-covered belt  conveyors or by  elevator,


Emissions  from conveying  are  minimal.  When  coal is  dis-

charged  (transferred) onto a  storage pile or into a  breaker


or crusher hopper,  fugitive emissions occur because  these


 transfer operations usually are  not enclosed and vented.

 Where coal is received in barges or rail cars,  emissions
                              8.9-4

-------
occur during unloading.  Fugitive emissions that occur in



raw coal storage and retrieval, crushing, screening, and


transfer activities are in inverse proportion to the surface



moisture of the coal.  Emissions from storage are caused



primarily by wind.


     The separation and mechanical dewateri^g operations of



wet cleaning plants do not emit air pollutants.  Substantial



amounts of coal particles are entrained in gases leaving the



thermal dryer.  Combustion of fuel  (usually coal) for the


dryer generates sulfur dioxide, nitrogen oxides, carbon



monoxide, and hydrocarbons.


     In dry process plants, dust particles are emitted in



the air table exhaust.  An air table designed to handle 70



tons of coal per  hour may emit up to 50 pounds per  hour of



particulates.


     Fugitive particulates are also emitted  from storage and



loading of cleaned coal.  Since a wet process plant produces


coal with a  relatively high surface moisture content, emis-


sions are lower than those from a dry process plant.



                  3 4
CONTROL PRACTICES '


     Emissions  from  unloading,  storage,  and  transfer  of  raw


coal are  usually  not controlled.  Most  plants,  however,  use



 stone  ladders,  telescoping chutes,  or  adjustable stacking



 conveyors for loading  onto the storage  piles.   All of these
                              8.9-5

-------
reduce the free fall distance and, hence, the fugitive emis-
sions.  Control options for transfer operations include
spraying the material before the transfer or the use of an
enclosure or hood vented to a particulate control device.
Increasing use of water within coal mines to implement new
health and safety regulations produces coal with relatively
higher surface moisture content and thus reduces fugitive
emissions.
     Emissions attributed to crushing do not occur from the
crushing operation, but from the  feed and discharge points,
which are transfer  sources.  Sometimes the crusher is
housed in a building but not vented.  In these cases the
degree to which emissions are reduced by baffle effects and
internal  settling  is not known; it  is possible that all of
the dust  generated  in  crushing  is eventually emitted to the
atmosphere.
      Although emissions from conveying are minimal, con-
veyors  from the crushers to  the screens  are  usually partially
covered  to  protect the coal  from  wind.   The  screens are
usually  equipped with  water  sprays  to wash some  of the fines
 from  the larger  coal and to  reduce  the  emission  potential.
 Use of sprays at this point also  reduces emissions from
 subsequent transfer and conveying operations,  which are not
 controlled.
                             8.9-6

-------
     Where a fluidized-bed dryer is used, a cyclone is an



integral part of the system.  Particulate emissions from the



dryer are controlled also by several types of scrubbers,



most commonly a venturi scrubber.  Particulate removal



efficiencies for venturi scrubbers are reported to be 99




percent.



     Cyclones also are an integral part of the air table in



a dry process plant.  Particulate emissions are typically



controlled also by fabric filters, which are reported to



reduce emissions to less than 0.01 grain per dry standard




cubic foot.



     Emissions from the discharge of cleaned coal onto



storage piles, and from storage, retrieving of coal, and



loading for shipment are usually not controlled.  In the



transfer of raw coal, however, stone ladders or telescoping



chutes are sometimes used to reduce emissions.






CODING NEDS FORMS



     The emission sources in a coal cleaning plant are:



Source                   SCC                 Pollutants



Unloading            3-05-010-08         Particulates



Raw coal storage     3-05-010-09         Particulates



Crushing             3-05-010-10         Particulates




Coal transfer        3-05-010-11         Particulates



Screening            3-05-010-12         Particulates



Air tables          3-05-010-13         Particulates





                             8.9-7

-------
Source

Thermal dryer

  Fluidized bed


  Flash


  Multilouvered


  Rotary


  Cascade
    SCC



3-05-010-01


3-05-010-02


3-05-010-03


3-05-010-04


3-05-010-05
  Continuous carrier 3-05-010-06


  Screen             3-05-010-07
 (Inprocess fuel
 for all dryers)
  Coal

  Residual oil

Cleaned coal
 storage
(3-90-002-99)

(3-90-004-99)
                                             Pollutants
                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion

                                        Particulates,  products
                                         of combustion
                    Particulates

                    Particulates
                     3-05-010-14

Loading              3-05-010-15

     Standard NEDS forms for each of the sources, Figures

8.9-2 through 8.9-10, show entries for the SCC's and other

codes.  Entries in the data fields give information common

to coal cleaning plants.  Information pertinent to coding

the source is entered on the margins of the forms and above

or below applicable data fields.  Entries for control

equipment codes, other optional codes, emission factors, and
                             8.9-8

-------
required comments minimize the need to refer to the code
lists.   Typical data values for operating parameters,
control equipment efficiencies, and other source information
are shown on the form  (or in the text) only to serve as
quick,  approximate checks of data submitted by the plant in
a permit application or similar report.  Da :a entered in
EIA/P&R and NEDS must be acutal values specific to and
reported by the plant, rather than typical values.  Contact
the plant to validate or correct questionable data and to
obtain unreported information.  See Part 1 of this manual
for general coding  instructions.
     The emission source labeled "storage"  includes  loading
on to piles, wind effects while the coal is  stored,  and
retrieval activities.  Transfer operations  that  are  not
included under unloading,  storage, crushing,  screening,  and
loading are  grouped under  the emission source labeled  "coal
transfer".
     Emissions from coal  unloading,  raw coal storage,
crushing,  coal transfer,  and screening are usually not
 controlled.   Figures 8.9-2 through 8.9-6 illustrate the
 standard NEDS forms for these five sources.  Emission
 factors for these sources have not yet been developed.  When
 a plant furnishes emissions data for these sources, code the
 values given.  Enter "Emission Estimates Given by Plant" in
 the comments  field on card 7.  Where there is no control
                             8.9-9

-------
device or where water sprays are used, enter zeros in the



stack height and diameter fields, 77 in the temperature



field, and zeros in the common stack field.  Enter appropriate



height in the plume height field.  Where water sprays are



used, enter 061 or 062 as control equipment code.  Identify



other equipment used to reduce emissions in the comments



field on card 6.  For example, enter "stone ladders" where



these are used for transfer onto storage piles.



     Thermal dryers are major sources of particulate emis-



sions in the wet process, and air tables in the dry process.



Figures 8.9-7 and 8.9-8 illustrate standard NEDS forms for



these sources.  Note that a fluidized-bed dryer includes



primary cyclones as part of the equipment.  Coal is the most



common fuel used for drying; oil is used rarely.



     Emissions from the handling of cleaned coal are minimal



in the wet process because of relatively high  surface



moisture content.  Figures 8.9-9 and  8.9-10 illustrate the



standard NEDS forms for cleaned coal  storage and loading,



respectively.  The emission source labeled  "cleaned coal



storage"  includes loading on to piles, wind effects, and




retrieval  activities.
                             8.9-10

-------
CODING EIS/P&R FORMS


     The BEC's for use in EIS/P&R forms are:



Source                                  Ul£



Unloading                               70°


Raw coal storage                        no code*



Crushing                                rD°



Transfer                                70°


Screening                               575,577



Air tables                              582



Thermal dryer



  Fluidizcd bed                         464



  Flash                                 464



  Multilouvered                         464



  Rotary                                452



  Cascade                               464



  Continuous  carrier                    464


                                        Af.A
  Screen                                ^D4


Cleaned coal  storage                    no code*



Loading                                 70°



 * As  of .3 -nuary  1978.
                             8.9-11

-------
                 Figure  8.9-2.    Standard NEDS  form  for  coal cleaning  -  unloading.
oo
          ! ,J
            Sffi
                                NAlliAAl I MISSIONS OAF A SYSHM IKE OS)
                                 [NU'.O ."INTAt PHimCT(0*i
                                    Of MCE IH AIR PROGRAMS
                                                                                                                FORM AfPRGVf D
                                                                                                                O»8 NO IbSRIX
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-------
                Figure 8.9-3.   Standard  NEDS  form  for coal cleaning  -  raw coal  storage.
CD
                                                        NAIIDNAl l MISSIONS OA1 A SYSUMlrUDS)

                                                              uMSNIAL PHOTfCMON AGtNCY

                                                             UiHCE (H AIR PROGRAMS
                                                                                FOHM APPfiO^ f ':

                                                                                OM6 NO IW RQO1S
                  1-ANTHRACITE

                  2-BITlimNOUS
11
                                             -JT:! I ;  i ' l-'^^-r-I-l  [•''.'!-•!>-\>^\*].T:.pT:!Tj."t.ni''
                                              mM±^
                    RAW COAL STORAGE : i :3|o]_5


                                 'r-i-l •-
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                                                 SCt UNIT - TONS COAL SHIPPED 4
              -i-1
             -1-4-!

                                                                 4	f
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                                                                                           /EXAMPLE COMMENT
                                                                  -
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±
4f
ft
i .'.
                                                                                                   :r

-------
                   Figure  8.9-4.    Standard NEDS  form  for  coal  cleaning  -  crushing.
00

vo
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                      Bfi
NA1IUNAI EMISSIONS DATA SVSTEM (NEDS)
 ENVinOiMMlNTAL PROTECTION AGENCY
     OFFICE OF AIR PROGRAMS
                   1-ANTHRACITE
                   2-BITUMINOUS
                                                                                                   0000 IF NO COMMON STACK
                                                                                                   XXXX POINT I.D.'S IF COMMON STACK
                          CRUSHING
                                           TJT
                                                  SCC,UNIT - TOHS COAL SHIPPED
                                                    >••
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-------
              Figure 8.9-5.   Standard NEDS  form for col cleaning  -  coal transfer.
oo
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                                                  NATIONAL I MISSIONS DATA SYSftH (NCOS)
                                                             PROTECTION AGINCY
                                                      Of MCE Or AIR PROGRAMS
                                                                                        0000 IF NO COMMON STACK
                                                                                        XXXX POINT I.D.'S IF COMMON STACK
i4Uun:;^M.J44-Ti^^

                                            so'UNIT -"TONS COAL SHIPPD,
                       TRANSFER  MSMSOiro

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-------
                Figure 8.9-6.   Standard NEDS  form  for coal  cleaning  - screening.
00
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                                                     MA1IUMAL EMISSIONS DAT A StSU* Wf OS)
                                                      ENVIRONMENTAL PROTECTION ACINCY
                                                         OFFICE OF AIR PROGRAMS
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                                                                                                 POINT I.D.'S IF COMMON STACKljl
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                                              SCC UNIT - TONS COAL SHIPPED,

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                                                iI-6'8
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FLUID BED
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"UlTI-
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CONTINUOUS
CARPIEP
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-------
                  Figure 8.9-8.    Standard NEDS  form  for  coal  cleaning  -  air  tables
CO


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                                                      NATIONAL EMISQIQSS DATA SYSTEM (MOS)
                                                        ENVIRON.V.FNTAL PROTECTION AGENCY
                                                           OFFICE OF AIR PROGRA.VS
                               POrV -.-Prc^ ED
                               '.>•<> NO 1 SB P',035
                           -UL
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                                                                                                  XXXX POINT I.O.'S IF COMMON STACK
               1 - ANTHRACITE
               2 - BITUMINOUS
                           !  i ;  j  ,-    -    ..   !   .-    -      i    J-.-j^j-  .,,'_>     ' i i  "' ' X   AAAA rUlH I l.U.i It l,UTr*jn 3 I m.h |< ;  ,^
                                                          o7o^ioTip{To^               1  * ! ioiTioi   io;

                                             _       _       __
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                    AIR TABLES
:.y:.. ..;. _:., L -_. ,•._.: T:_: :,_;'.. 4.
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-------
CO
         Ficiure 8.9-3.    Standard -.IEDS  form for  coal  cleaning  - cleaned  coal  storage.






                             if
                     MftllDNAl I MISSIONS OATASYSTlMINf OS)

                      CNvmUhiMlNIAl PROTf CTION AGENCY

                          OFFICt Of AIR PROGRAMS
   KJIWT ioum:c

    IIHM.I Fo«m
FORM APPWOVt o

OMNO IMH009S

                             efflff
                   l-ANTHRACITE-

                   2-BITUMINOUS
                                                                     S1.V> K UAL-
                                 'i-^'-U '••••"•• "•
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                  CLEANED COAL STORAGE
3J01
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                                         ±1±
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                                                  J	[_J	l__L -J	1 —L--L ' i "*-*	>—-—

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                                                                                                             IMS!
                                                                                                              COMHOL
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-------
                  Figure 8.9-10.   Standard  NEDS form for coal  cleaning  -  loading.
00
 I

NJ

O
                                                     NATIONAL EMISSIONS DATA SYSTEM (NCOS)


                                                       ENVIRONMENTAL PROTE CriON ACENCY

                                                          OFFICE OF AIR PROGRAMS
                                               SCC,UNIT - TONS COAL SHIPPED
                         LOAD1K6 .. II

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-------
GLOSSARY

Air table - A device that uses a pulsating air column to
     separate coal from reject material.

Cleaning circuit - The equipment that separates impurities
     from coal.

Coal cleaning - All operations involved in removing impuri-
     ties from coal.

Dry coal cleaning - Use of air to separate impurities from
     coal.

Grizzly - A device used to remove large fragments of rock
     and other materials from coal.  This is a form of a
     scalping screen, except, that it consists of a series
     of heavy steel bars spaced parallel to each other.

Hematite - A mineral Fe203 constituting an important iron
     ore and occuring in crystals or in a red earthy form.
     Hematite is mixed with water to produce mixtures having
     different specific gravities for use in a wet washing
     plant.

Scalping screen - Used to remove large rock, slate, timbers,
     etc. , from coal; the scalper consists of heavy wire
     screen with large openings that permit the coal pieces
     to drop to another series of screens for segregation.

Stacking conveyor - A belt conveyor that discharges at the
     storage pile.  Use of conveyors that use and fall with
     the storage pile reduces the distance that the coal
     must drop.

Stone  ladder - A fixed, rectangular column with a series of
     steps inside that allow the falling material to cascade
     in short drops.  As the storage pile increases, the
     coal discharges through ports in the sides of the
     column and emissions are reduced.

Telescoping chute - A column that can be raised or lowered
     to maintain a  constant distance between  the coal  being
     discharged and the top of  the storage pile.

Wet coal  cleaning - Use of  liquids of varying specific
     densities to separate  impurities from coal.
                              8.9-21

-------
                REFERENCES FOR SECTION 8.9
1.   Keystone Coal Industry Manual.  New York.  McGraw -
    Hill, Inc. 1975.

2.   Coal Preparation.   Leonard, J.W.,  and D.R. Mitchell.
    (ed.).   New York.   The American Institute of Mining,
    Metallurgical, and Petroleum Engineers, Inc.  1968.

3.   Background Information for Standards of Performance:
    Coal Preparation Plants.  Vol. 1:   Proposed Standards.
    Environmental Protection Agency,  Research Triangle
    Park, North Carolina.   Research Triangle Park, EPA
    450/2-74-0219.  October 1974.

4.   Compilation of Air Pollutant Emission Factors, Second
    Edition.  Environmental Protection Agency, Research
    Triangle Park, North Carolina.  AP-42.  February 1976.

5.   Aeros Manual Series Volume II:  Aeros User's Manual.
    U.S. Environmental Protection Agency, Research Triangle
    Park, North Carolina.   Publication No. EPA-450/2-76-029
    (OAQPS No. 1.2-039).  December 1976.

6.   Aeros Manual Series Volume V:  Aeros Manual of Codes.
    U.S. Environmental Protection Agency, Research Triangle
    Park, North Carolina.   Publication No. EPA-450/2-76-005
    9OAQPS No. 1.2-042).  April 1976.

7.   Standard Industrial Classification Manual, 1972 Edition.
    Prepared by Office of Management and Budget.  Available
    from Superintendent of Documents,  Washington, D.C.

8.   Loquercio, P. and W.J. Stanley.  Air Pollution Manual
    of Coding.  U.S. Department of Health, Education and
    Welfare.  Public Health Service Publication No. 1956.
    1968.
                            8.9-22

-------
                    8.15  LIME MANUFACTURING





PROCESS DESCRIPTION1"4



     The manufacture of lime involves the calcining of limestone



(CaCO-. or CaCO 'MgCO_) to release carbon die 
-------
              UGEHD:

              £} OHSSIOH FACTOR*

                  eEMISSIOII FACTOR HOT DEVaOPED
                  FOR THIS PROCES.

              009 (66.0) DENOTES COKTROl EQUIP.
             I          CODE WITH EST. EFF. SHOWN
             f          IM)
              \         DENOTES FUGITIVE
               /         EMISSIONS
              o
DENOTES A STACK
PHOOBCT TWWSFER
(WO CONVEYING
COimOL FWRIC
DEVICE
f PART0
FILTER 018 (99)
              * IK  POUNDS PER SCC UNIT
    3-05-016-07
    RAW MATERIAL
    TRANSFER AND
     CONVEYING
                                            PART0
                                                                      3-05-016-03
                                                                      CALCINING-
                                                                      VERTICAL KILN
  RAH
MATERIAL.
                                                  3-05-016-02
                                                   SECONDARY
                                                   CRUSHING/
                                                   SCREENING
                                                                                                                                                                                             9
                                                                      MET SCRUBBER 001  (95-99)
                                                                      FABRIC FILTER 017  (99)
                                                                      ESP           010  (95)
                                                                                              GRAVITY  COLLECTOR    000 (<80)
                                                                                              CENTRIFUGAL COLLECTOR 009 (<80)
                                                                                                                                                                FABRIC FILTER
                                                                                                                                                                    018 (99)
                                                                                                                                                                                jPAJtrQ    4 PARj Q
FABRIC FILTER
     018 (99)
                                                                                                                            CaO
                                                                                           'PART
                                                     3-90-OOX-99
                                                   IN-PROCESS FUEL
                                                    4-OIL
                                                    6-NATURAL GAS
                                                                                                      VERTICAL
                                                                                                      ROTARY

                                                 3-05-016-10
                                                RAW MATERIAL
                                                STORAGE PILES
                                                                                                                                                                                                          . QUICKL
                                                                                   FABRIC FILTER  017  (99)
                                                                                   CYCLONE        008  (90-95)
                                                                                   WET SCRUBBER   002  (80-95)
                                                                               CALCININ6-
                                                                               ROTARY KILN

                                                                               3-90-OOX-99
                                                                              IN-PROCESS FUEL
                                                                              2-COAl
                                                                              4-01L
                                                                              6-NATURAL GAS
                                                                                                                                                                                         3-05-016-14
                                                                                                                                                                                           PACKING/
                                                                                                                                                                                           SHIPPING
                                                                                                                                                                                                   FABRIC
                                                                                                                                                                                                   FILTER 018 (99
                                                                                                                                                                                                           DOLOm
                                                                                                                                                                                                           PRESSU
                                                                                                                                                                                                           HYDRAT
                                                                                                                                                                                                           LIME
                                                                                                                                                                               9         9
                                                                                                                                      FABRIC
                                                                                                                      9
                                                                                                       HIGH  CALCIUM QUICKLIME
                                                                                                       MO DOLOWTIC QUICKLIME
                                                                             Figure  8.15-1.  Lime  Manufacture
                                                                                                       SPRAYS
                                                                                                WET SCRUBBERS
                                                                                                                                                                           FABRIC
                                                                                                                                                                           FILTER  018 (99)
                                                                                                                                                                                   HIGH C
                                                                                                                                                                                   AND 00
                                                                                                                                                                                   HYDRAT

-------
secondary crushers and screens reduce the stone to the desired




feed size for the calcining kilns.



     In the United States, limestone is calcined in either verti-



cal or rotary kilns.  The limestone feed size for most vertical



kilns is 6 to 8 inches; consequently, only primary crushing is



required.  However, some vertical kilns need a smaller feed size



of 3 to 5 inches.  Material for these kilns must undergo second-



ary crushing   Rotary kilns, which are the most prevalent kilns



in use, also need the smaller feed size.



     Vertical kilns, which are fueled by oil or natural gas, have



four distinct zones from top to bottom:  stone storage zone,



preheating zone, calcining zone, and cooling and discharge zone.



The flow of stone in the kiln is countercurrent to the flow of



cooling air and combustion gases.  The stone is charged at the



top and preheated by the hot exhaust gases from the calcining




zone.  Air blown into the bottom of the kiln cools the lime



before it is discharged.  This air is heated sufficiently by the



time it reaches the calcining zone to be used as secondary com-



bustion air.  The lime is discharged to cars on tracks or to



conveyor belts, and either prepared for shipping or further



processed by hydration.



     The rotary kiln, which is supported by rollers, is a long



inclined horizontal steel cylinder lined with refractory brick.



Most rotary kilns rotate at a speed of about 1 rpm.  The lime-



stone flows countercurrent to the heat, the pebble-size limestone



entering at one end and the hot gases entering at the other.








                               8.15-3

-------
Rotary kilns have three distinct zones:  the feed and drying
zone, the central or preheating zone, and the calcining zone.
Rotary kilns are fueled with coal, oil, or natural gas.  Product
coolers are commonly used after the kiln to recover heat from the
calcined lime.
     In both vertical and rotary kilns, the temperature in the
feed end is kept below 1000°F, and the temperatures in the pre-
heating and calcining zones are between 2000° and 2400°F; higher
temperatures are found in shorter kilns.  At these temperatures,
limestone dissociates to quicklime and carbon dioxide.
                         CaC03 + CaO + C02
     Most of the calcined lime or quicklime is screened, milled,
and transferred pneumatically or by conveyor to storage silos,
where it is kept until it is shipped.  Fines from calcination can
be briquetted, fed to a hydrator, or pulverized, as the market
demands.
     About 10 percent of all the lime produced is converted  to
hydrated  (slaked) lime.
                         CaO + H20 + Ca(OH)2
In the  hydration process, water is added to crushed or ground
quicklime in  a mixing chamber  (hydrator).  The slaked  lime is
dried by the  heat of the hydration reaction, and is conveyed to
an air  separator in preparation for  final  shipment.  Dolomitic
pressure-hydrated lime has  an  additional milling step  prior  to
shipment.  Atmospheric hydrators  are operated continuously;
pressure  hydrators  are operated  in a batch mode.

                               8.15-4

-------
     For shipping, the quicklime and hydrated lime products are



packaged in bags and handled in bulk by truck, rail, ship, or



barge.



     Lime manufacturing plants have capacities between 50 and 650



tons per day.  Plants usually operate 24 hours per day for 6 or 7



days a week.  Stack heights for lime plants range from 250 to 400



feet.






EMISSIONS1""3'5



     Particulate is the major pollutant from lime plants, espe-



cially from the calcining kiln.  Emission sources are identified



in Figure 8.15-1.  For some of the sources, AP-42  provides emis-



sion factors, which are listed on the process flow diagram.  For



other sources, average emission rates obtained from other docu-



ments are mentioned in the discussion that follows.



     Particulate emissions arise during raw material unloading,



open storage piles, crushing, screening, and conveying and



transfer operations.  All of these operations, unless confined,



are fugitive emission sources.  Emissions from raw material un-



loading range from 0.03 to 0.4 Ib/ton; from raw material storage



piles, 3.0 to 5.0 Ib/ton (includes loading onto pile, vehicular



traffic, loading out, and wind erosion); from primary crushing,



about 0.5 Ib/ton; from secondary crushing and screening, about



1.5 Ib/ton; from raw material conveying and transfer operations,



0.8 Ib/ton; and from packaging and shipping of quicklime and hy-



drated lime products by truck, rail, ship, or barge, 0.25 lb/




ton.




                              8.15-5

-------
     The major source of particulate emissions in lime manu-




facture is the calcining kiln.  Emissions vary with kiln type and



composition of limestone burned.  Rotary kilns emit considerably



more particulates than do vertical kilns because the charge



material is smaller, the rate of fuel consumption is higher, and



air velocity through the kiln chamber is greater.  The in-process



fuel also emits sulfur oxides and small amounts of nitrogen



oxides and carbon monoxide.



     Product coolers following the rotary kiln are emission



sources only when some of their exhaust gases are not recycled



through the kiln as combustion air.  Current practice is against



the venting of product cooler exhaust, however, because recycling



makes better use of the fuel.  Cyclones, baghouses, and wet



scrubbers have been used to control particulates from coolers.



Emissions from milling and screening the calcined material are




minor because the operations  are enclosed.



     Few particulates are emitted during hydration, because water



sprays or wet scrubbers are usually installed to prevent the  loss



of  product  in the exhaust gases.  Emissions  from pressure hy-



drators may be greater than from the more  common atmospheric



type; control is more difficult in pressure  hydrators because the



exhaust gases are released  intermittently  over  short  time  inter-



vals.   Particulate  emissions  from  pressure hydrators  after  wet



 scrubbers  are about 2  Ib/ton  of hydrate  produced.    Emissions



 froir  atmospheric  hydrators  after wet  scrubbers  are about  0.1




 Ib/ton  of  hydrate produced.






                               8.15-6

-------
     Minor amounts of particulates are emitted from the air



separator following the hydrator and the milling operation fol-



lowing the pressure hydrator because the processes are enclosed.



Some particulates are entrained in the lime silo ventilation.



Additional particulate emissions are generated during the packing



and shipping operations, and product transfer and conveying.






CONTROL PRACTICES



     Emissions from unloading are generally not controlled.



Building enclosures may be used to reduce emissions.  Liquid



sprays are also sometimes used to suppress emissions during un-



loading.  Occasionally, the unloading area is vented to a bag-




house.



     The limestone is nearly always stored in stockpiles, a



source of fugitive particulate emissions, but in some cases it



may be stored in silos.  Liquid spraying of the material before



discharge onto the storage pile is often practiced to reduce the



emission potential.  Telescoping chutes, adjustable stacker con-



veyors, and stone ladders are possible ways to reduce emissions



from loading onto the raw material storage piles.  All of these



devices reduce the free-fall distance and, hence, the fugitive



emissions.



     Emissions from conveying are minimal, but the belts are



sometimes partly covered to reduce any emissions that occur.



Emissions caused by transfer of materials from one conveyor belt




to another are most often controlled by enclosures or water
                               .15-7

-------
sprays,  with an increasing trend toward control by venting the
transfer point to a baghouse.
     Primary crushers and secondary crushers and screens are
often located below grade; this reduces the impact of the emis-
sions.  Suppression of dusts by water sprays at the feed points
of these operations is very common.  Emissions from primary
crushers are sometimes controlled by wet scrubbers or fabric
filters.  An increasing number of plants are venting the dis-
charge points of secondary crushing and screening to a fabric
filter.
     Emissions from kilns are controlled in most plants by pri-
mary collectors, consisting of centrifugal or gravity collectors,
which have,efficiencies between 25 and 80 percent  (70 percent
average).  These collectors are usually followed by secondary
collectors,  such as wet scrubbers  (95 to 99 percent efficient);
electrostatic precipitators  (95 percent efficient); or  fabric
filters  (99  percent efficient).
      Nitrogen oxides,  carbon monoxide, and  sulfur  oxides  are  all
formed  in  the kilns,  but  the last  is  the only  gaseous pollutant
emitted  in significant quantities.  Not all of  the sulfur in  the
kiln fuel  is emitted  as sulfur oxides because  some fraction
reacts  with the materials in the  kiln.   Sulfur oxide  emissions
may be  incidentally reduced by the various equipment  used for
 secondary  particulate control; otherwise,  gaseous emissions are
 uncontrolled.
                               8.15-8

-------
     Some or all of the exhaust from the product cooler is re-



cycled to the kiln as combustion air.  The portion that is not



recycled is typically controlled by a fabric filter, cyclone, or




wet scrubber.



     Emissions from the atmospheric or pressure hydrator are re-



duced by water sprays or wet scrubbers.  The emission rates after



control are 2 Ib/ton and 0.1 Ib/ton of lime produced, respec-




tively.



     Particulates entrained in the air displaced during loading




of the silos are retained by fabric socks on the vents.  In



pneumatic systems the lime silo transport air is often exhausted




through a fabric filter.



     During packaging and processing for bulk shipment, the



emissions that arise are frequently controlled by aspiration



through fabric filters.  Many lime plants are using a gravity-



feed fill spout mechanism that has outer concentric aspiration



ducts to vent the dust to a fabric filter.  This device has been



markedly successful in reducing emissions during packing and




shipping.



     Transfer and conveying of the finished quicklime and slaked



lime can be a considerable fugitive emission problem if these



sources are not properly enclosed and exhausted.  Nearly all



plants completely enclose the conveyor systems, which are most



often belt-type, and many of them also enclose transfer points




and exhaust the emissions to fabric  filters.
                               8.15-9

-------
CODING NEDS FORMS1'8"10

     The emissions sources associated with lime manufacturing

are:

Source
Raw material unloading

Raw material storage piles

Primary crushing

Primary screening
                                  SCC

                              3-05-016-08

                              3-05-016-10

                              3-05-016-01

                              3-05-016-16
Secondary crushing/screening  3-05-016-02

                              3-05-016-07
Raw material transfer and
  conveying

Calcining, vertical kiln

  In-process fuel

Calcining, rotary kiln

  In-process fuel

Product cooler

Hydrator  (atmospheric)

Pressure hydrator

Lime silos

Packing/shipping

Product transfer and
  conveying
                              3-05-016-03

                              3-90-OOX-99

                              3-05-016-04

                              3-90-OOX-99

                              3-05-016-11

                              3-05-016-09

                              3-05-016-12

                              3-05-016-13

                              3-05-016-14

                              3-05-016-15
Pollutant(s)

Particulates

Particulates

Particulates

Particulates

Particulates

Particulates
Particulates, com-
  bustion products
Particulates, com-
  bustion products
Particulates

Particulates

Particulates

Particulates

Particulates

Particulates
     Standard NEDS forms for each of the sources, Figures 8.15-2

through 8.15-15,  show entries for the SCC's and other codes.

Entries in the data fields give information common to lime manu-

factaring plants.  Information pertinent to coding the source is

entered on the margins of the forms and above or below applicable


                              8.15-10

-------
data fields.  Entries for control equipment codes, other optional




codes, emission factors, and required comments minimize the need




to refer to the code lists.



     Typical data values for operating parameters, control equip-



ment efficiencies, and other source information are shown on the



form  (or in the text) only to aid in quick, approximate checks of



data submitted by the plant in a permit application or similar



report.  Data  -ntered in EIS/P&R and NEDS muc. c be actual values



specific to and reported by the plant, rather than typical values.



Contact the plant to validate or correct questionable data and to



obtain unreported information. See Part 1 of  this manual for




general coding instructions.



     The emission source labeled "raw material unloading" in-




cludes emissions released when raw materials  that have been



previously  sized are received from truck, ship, barge, or rail.



Raw materials  that must be crushed and screened are unloaded



directly into  primary crusher hoppers; emissions  from unloading



this unsized material are  included in primary crusher emissions.



There  is no emission factor developed for primary screening.



The emission factor  assigned to  secondary crushing/screening



includes emissions from both operations.



      The emission source labeled "raw material storage piles"



includes loading  onto piles, wind  effects while the materials  are



stored, and retrieval activities.  Raw material transfer  opera-



tions that are not  included  under  unloading,  storage  piles,



primary crushing, primary  screening,  and  secondary  crushing  and







                             8.15-11

-------
screening are grouped under the emission source labeled "raw
material transfer and conveying."  Figures 8.15-2 through 8.15-7
illustrate the standard NEDS forms for these six sources.  When
a plant furnishes emissions data for these sources, code the
values given.  Enter "Emission estimates given by plant" in the
comments field on Card 7.  Where there is no control device or
where water sprays are used, enter zeros in the stack height and
diameter fields, 77 in the temperature field, and zeros in the
common stack field.  Enter appropriate height in the plume height
field.  Where water sprays are used, enter 061 or 062 as a con-
trol equipment code.  In the comments field on Card 6 identify
other equipment used to reduce emissions.  For example, enter
"stone ladders" where these are used during loading onto raw
material storage piles.
     Figure 8.15-8 shows the standard NEDS form for calcining
with the vertical kiln.  The in-process fuel is either oil or
natural gas.
     Figure 8.15-9 shows the standard NEDS form for calcining
with the rotary kiln.  The in-process fuel may be coal, oil, or
natural gas.  AP-421 provides emission factors for control for
primary, and for secondary particulate control.  These numbers
serve as guides; actual plant values must be entered.  Secondary
particulate controls such as venturi scrubbers may reduce sulfur
oxides as well.  When  this  is the case, also enter the scrubber
as  a  secondary  S02  control  device using  053  as the control device
code.

                              8.15-12

-------
     The standard NEDS form for the product cooler used after the



rotary kiln is shown in Figure 8.15-10.  The emission factor from



AP-42  and the control device apply only when the cooler gas is



not completely recycled back to the rotary kiln.  The coder must



determine whether or not this is the case.



     Atmospheric and pressure hydrator emissions are reduced by



water sprays or wet scrubbers; Figures 8.15-11 and 8.15-12 show



standard NELo forms for these sources.



     Particulate emissions from lime silo ventilation air and



packing/shipping are generally vented to fabric filters.  Product



transfer and conveying include all emissions from pneumatic or



mechanical  (conveyor)  transport of the lime from the kiln through



the packing/shipping operation.  These emissions are also usually



controlled by venting to a fabric filter.  See Figures 8.15-13,



8.15-14, and 8.15-15 for standard NEDS forms for these sources.
                             8.15-13

-------
CODING EIS/P&R FORMS



     The BEC's for use in the EIS/P&R forms are:



Source                                       BEC



Raw material unloading                       712



Raw material storage piles                   700



Primary crushing                             650



Primary screening                            575



Secondary crushing/screening              650, 575




Raw material transfer and conveying          700



Calcining, vertical kiln                     229



Calcining, rotary kiln                       229



Product cooler                               330



Hydrator  (atmospheric)                     No code*



Pressure hydrator                          No code*




Lime  silos                                   730



Packing/shipping                          711,  712



Product transfer and  conveying               700
   As of November 1978.
                              8.15-14

-------
                          Figure 8.15-2.   Standard NEDS form for lime manufacturing - raw material unloading.
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                                                           NATIONAL fMISSIONS DATA SYSHM INFOS)
                                                             ENVIRONMLNlftL PROTfCTION AGLNCY
                                                                 IHFICE OF AIR PROGRAMS
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-------
                    Figure  8.15-3.   Standard NEDS  form  for lime manufacturing - raw material  storage piles.
         Ti; irrrvrr vi > i > i«i_i.
                           f MISSIONS DATA SYS I EM (Nf US)
                           MLNI Al PHOTfCTlUN AGENCY

                         OFFICE OF AlBPnOGRAMS
                                                                                                        Input
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                             Figure  8.15-8.  Standard NEDS  form for  lime manufacturing -

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                        Figure 8.15-14.   Standard NEDS form  for  lime manufacturing  - packing'shipping.
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GLOSSARY
Clamshell - A crane with a bucket having two hinged jaws.

Density:
                                        Densities,
     Product                             Ib/ft3

     Lime, hydrated - 200 mesh            20-25

     Lime, quick, lump,
       1-1/2 in. x 0 in.                  70-80

     Lime, quick, lump, 1/2 in. x 0 in.    70

     Lime, quick, ground                  60-65

Stacker conveyor - A belt conveyor that discharges at the storage
     pile.  Use of conveyors that rise and fall with the storage
     pile reduces the distance that the material must drop.

Stone ladder - A fixed column containing a series of steps that
     allow the falling material to cascade in short drops.  As
     the storage pile increases, the material discharges through
     ports progressively higher in the sides of the column so
     that emissions are reduced.

Telescoping chute - A column that can be raised or lowered to
     maintain a constant distance between the coal being dis-
     charged and the top of the storage pile.
                               8.15-29

-------
                   REFERENCES FOR SECTION 8.15
 1.  Compilation of Air Pollutant Emission Factors.  2nd edition.
     U.S.  Environmental Protection Agency, AP-42, February 1976.

 2.  Engineering Science, Inc.   Exhaust Gases from Combustion and
     Industrial Processes.  PB-204-861, Washington, B.C., October
     1971.

 3.  Midwest Research Institute.  Particulate Pollutant System
     Study, Volume III.  Handbook of Emission Properties.  Con-
     tract No. CPA 22-69-104, May 1971.

 4.  Industrial Gas Cleaning Institute, Inc.  Air Pollution
     Control Technology and Costs in Seven Selected Areas.
     Stamford.  PB-231-757, December 1973.

 5.  Technical Guidance for Control of Industrial Process Fugi-
     tive  Particulate Emissions.  EPA-450/3-77-010, March 1977.

 6.  Minnick, L.J.  Control of Particulate Emissions from Lime
     Plants.  In:  63rd Annual Meeting of the Air Pollution
     Control Association, St. Louis, June 1970.

 7.  Vatavuk, W.M.  National Emission Data System  (NEDS) Control
     Device Workbook.  U.S. Environmental Protection Agency,
     APTD-1570, July 1973.

 8.  Aeros Manual Series Volume II:  Aeros User's Manual.  EPA-
     450/2-76-029 (OAQPS No. 1.2-039), December 1976.

 9.  Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA-
     450/2-76-005 (OAQPS No. 1.2-042), April 1976.

10.  Standard Industrial Classification Manual.  Office of
     Management and Budget.  Available from Superintendent of
     Documents, Washington, D.C., 1972.

11.  Loquercio, P. and W.J. Stanley.  Air Pollution Manual of
     Coding.  U.S. Department of Health, Education, and Welfare.
     Public Health Service Publication No. 1956.  1968.
                              8.15-30

-------
         8.19  SAND AND GRAVEL QUARRYING AND PROCESSING



PROCESS DESCRIPTION1"5


     Sand and gravel have many uses in landscaping and construc-


tion, and are also used in concrete aggregate, road base materi-


als, and blacktop.  Figure 8.19-1 shows a typical sand and gravel


operation.


     Sand and gravel deposits are found in banks, pits, and


subterranean beds.  The three methods of excavation are:   (1) dry


pit, in which sand and gravel are removed from above the water


table;  (2) wet pit, in which raw material above or below the


water table is extracted by means of a dragline or by barge-


mounted dredging equipment; and  (3) dredging, in which sand and


gravel are recovered from public waterways, including lakes,


rivers, and estuaries.  Dry pit extraction accounts for 50 per-


cent of the total that is produced; wet pit, for 30 to 40 per-

                                         4
cent; and dredging, for 10 to 20 percent.   Light-charge blasting


is sometimes needed to loosen the deposit.  Before blasting,


holes must be drilled for the explosives.


     The loosened deposit is transported to the plant by earth-


movers, or it is shoveled and loaded into a truck or barge and


transported to the processing plant.  In a wet pit, the material


may be transported by suction pumps.  The processing plant is


usually close to the excavation area.  The material is unloaded



                               8.19-1

-------
PART
                     ' PART
                       G
                                          PART
0
                                                               PART
                                                                       Q
                                                                                                                             3-05-025-03
                                                                                                                    MATERIAL TRANSFER  AND CONVEYING
f f f
\ \ I
EXCAVATING


*
DRILLING AND
BLASTING

f




V—
T"
^^ ^ y
3-05-025-04
HAULING

I ^ 7PART<->
( / ^
m >-x i
^ .^ 1
3-05-025-02 _— — ' L- — "7.DrrM
AGGREGATE r— ' <-^ ^oLKLLH
STORAGE f ~~ 	 —.•'I
    LEGEND:

       EMISSION  FACTOR3
/-\
\-J
       EMISSION  FACTOR NOT DEVELOPED
       FOR THIS  PROCESS
    009 (66.0)  DENOTES CONTROL EQUIP.
              CODE WITH EST. EFF. SHOWN
              IN  ( )
 -

O
              DENOTES FUGITIVE
              EMISSIONS
              DENOTES A STACK
    IN POUNDS PER SCC UNIT
                                                                          OVERSIZE
                                                                                                         PARTICULATES(0.1)
                                                                                                     PRIMARY CRUSHER   3-05^-025-0!
                                                                                                                    CRUSHING AND
                                                                                                                      SCREENING
                                                                                                       SCREEN
                                                                    SECONDARY CRUSHER
                                                                        RECYCLE
                                                                                                   3-05-025-02
                                                                                                AGGREGATE STORAGE
                                                                                                                FINE SAND
                                                                                                                                                    FINES
                                                                                                                                                     TO
                                                                                                                                                  DISPOSAL
                                            Figure  8.19-1.
                                                                      8.
                                                                                gravel  processing.

-------
directly onto the primary screen  (scalping screen), or it is
stockpiled and later transferred to the screen by  a front-ena
loader.
     At the plant, the sand and gravel are crushed and screened
to reduce and segregate the material by size, then it is stored
and loaded.  The sand and gravel are reduced and classified by a
wet or a dry process, many plants use both.
     In the wet process, sand and gravel are washed and screened
for use as concrete aggregate.  The material is first screened
(scalping), and the material passing through the screen is
crushed in a jaw crusher (primary crushing).  Oversize material
from the first screen is removed, reduced in size, and recycled
to the screen.  The output (gravel) from the primary crusher is
again screened (secondary screening).  The oversize material goes
to a secondary crusher  (gyratory or roll crusher) where it is
reduced to a size of 3/4 to 1 inch and recycled to the screen.
The material passing through the screen goes to a washer or
rotary scrubber and is screened a third time to remove unwanted
soil.  Additional screens and classifiers are used to separate
the material further into specified fractions.
     Dry processing prepares sand and gravel that are to be used
for road base, blacktop (bituminous aggregate), or similar pur-
poses.  The dry process is the same as the wet process, with the
exception of the washing steps.  After processing  and classifica-
tion are complete, the material is loaded for shipment or is
stockpiled in storage areas until it is loaded onto trucks for
shipment.
                              8.19-3

-------
     Material is transferred throughout the plant by conveyors



and bucket elevators.




     Individual sand and gravel operations range in size from



less than 1000 tons produced annually to more than 3.5 million



tons.  Plants usually operate 8 hours a day, 5 or 6 days a week.



Many sand and gravel plants operate on a part-time or seasonal



basis to meet fluctuating demands.  During periods of high de-



mand, which is caused by intense construction activity, plants



may operate for longer hours.  The exhaust flow ranges from 500



to 750 scfm per ton/h of aggregate produced  at those plants that



have control devices.






EMISSIONS1"3/6




     Sand and gravel quarrying and processing generate particu-



late emissions,  but since these materials are usually moist when



handled, the emissions are much lower than in crushed stone




plants that use similar operations.  Emission sources are identi-



fied in Figure 8.19-1.  For crushing and screening,  AP-421



provides an emission factor that is listed on the process flow



diagram.  For other sources of emissions,  average emission rates



obtained from other documents are mentioned in the following



source descriptions.



     Particulates are emitted during excavating, drilling,



blasting, and hauling.  When wet pit and dredging methods are



used, the emissions from excavation are minimal.  When the dry



pit method is used, emissions are slightly greater only when the



material is relatively dry.  Drilling and blasting have little




                              8.19-4

-------
impact on overall emissions because they are performed infre-



quently.  Significant amounts of particulate emissions are gen-



erated during hauling when the trucks or earthmovers travel cver



unpaved or dirt-covered paved roads.  The dusts that arise come



mainly from the roads, although the material in the vehicles also



contributes to the emissions, which range from 1.7 to 4.5 lb/



vehicle mile.7  The level of the emissions is affected by the



composition or the road surface, the wetness of the road, and the




volume and speed of the traffic.



     A state agency has estimated that sand and gravel processing



releases overall emissions of 0.06 lb of dust/ton of material.



The primary dust sources listed in the report are the discharge



of the secondary crushers, the transfer of dry material, and the



final screening of dry material.  As much as 75 percent of the



dust was estimated to come from the crushers.  Based on this



information, AP-42  lists an emission factor of 0.1 lb of dust/ton



of product for crushing and screening operations.  Emission rates



may vary, because they are affected by the moisture content of



materials processed, amount of size reduction, and type of equip-




ment used.



     Fugitive emissions arise from outdoor storage.  Most storage



piles are left uncovered, but silos and bins may be used.  Dust



emissions occur at several points in the storage cycle:  during



loading of material onto the pile, during movement of trucks  and



loading equipment in  the storage area, during disturbance by



strong wind currents  (wind erosion), and during  loading  of







                              8.19-5

-------
material from the pile.  An overall emission factor of 0.33/

         2
(P-E/100)  Ib/ton placed in storage has been reported in AP-42


(Section 11.2), where P-E is Thornthwaite's precipitation-evapora-


tion ratio.   Although such factors as age of the pile, moisture


content, and proportion of aggregate fines influence emission


rates, the precipitation-evaporation index is the best guide to


the variability of total emissions from aggregate storage piles.


     Fugitive emissions are generated during material transfer


and conveying, particularly when the material is dry.  The emis-


sions are small when the sand and gravel are moist.


     Particulates are also emitted during loading of the product


for shipment.  Front-end loaders usually transfer the material


into trucks.



CONTROL PRACTICES1"5


     Particulates generated during excavation and drilling are


not controlled.  Emissions from blasting are not amenable to


capture by a hood or similar device and are, therefore, fugitive.


     Emissions from hauling, when controlled, are most commonly


reduced by wet suppression.  Water or water plus chemicals are


applied by trucks to the roads during dry weather.  The frequency


and extent of wet suppression determines its effectiveness.


Emissions  from haul roads can also be reduced by lowering vehicle


speeds,  stabilizing the  soil, and paving the roads.  The material


being hauled  need not  be controlled because  it  is  usually too wet


to generate  significant  amounts of particulate  emissions.





                              8.19-6

-------
     Emissions from crushing and screening, aggregate storage,

and material transfer and conveying are not commonly controlled

because the material is usually wet and emissions are minor.

When the material is dry, emissions can be controlled by wet

suppression.  Initial applications of water are made at the truck

dump and at the outlets of crushers where new surfaces are ex-

posed.   Emissions from dry material processi ig could also be

controlled with low- to medium-efficiency cyclones, wet scrubbers,

and fabric filters; but these devices are seldom used.

     Emissions from aggregate storage can be reduced by wet sup-

pression and by using stone ladders, telescopic chutes, and

hinged-boom stacker conveyors.  A stone ladder is a vertical pipe

with steps inside that reduce the free-fall distance of the sand

and gravel.  The enclosure also protects the material from wind.

A telescopic chute is a retractable chute that is raised or

lowered according to the height of the stockpile.  A stacker

conveyor is equipped with a hinged boom that adjusts the conveyor

height as the level of the stockpile changes.


CODING NEDS FORMS

     The major sources of emissions and their SCC's are:

Source                         SCC           Pollutant(s)

Hauling                    3-05-025-04       Particulates

Crushing and screening     3-05-025-01       Particulates

Aggregate storage          3-05-025-02       Particulates

Material transfer and
 conveying                 3-05-025-03       Particulates



                              8.19-7

-------
     Standard NEDS forms for the sources, Figures 8.19-2 through



8.19-5, show entries for the SCC's and other codes.  Entries in



the data fields give information common to sand and gravel pro-



cessing.  Information pertinent to coding the source is entered



on the margins of the forms and above or below applicable data



fields.  Entries for control equipment codes, other optional



codes, emission factors, and required comments minimize the need



to refer to the code lists.  Typical data values for operating



parameters, control equipment efficiencies, and other source in-



formation are shown on the form (or in the text) only to aid in



rapid, approximate checks of data submitted by the plant in a



permit application or similar report.  Data entered in EIS/P&R



and NEDS must be actual values specific to and reported by the



plant, rather than typical values.  Contact the plant to validate



or correct questionable data and to obtain unreported informa-



tion.  See Part 1 of this manual for general coding information.



     In general, for emission sources that do not discharge



through a stack or vent and are not housed in a building, enter



zeros  in the stack height, diameter, and common stack fields, and



77 in  the temperature field, unless temperature data are fur-



nished.  Enter appropriate plume height.  Where liquid sprays are



used to reduce particulate emissions, enter  061 or 062 as a con-



trol equipment code.  In  the comments field  on  Card 6, identify



other  equipment used to reduce emissions.  For  example, enter



"stone ladders" where they are used.  For  sources  that do not



discharge directly through a stack  and  are not  hooded but are







                              8.19-8

-------
housed in a building, enter the roof vent data in the stack da<
fields.  Enter "roof vents" in the comments field.
     Figure 8.19-2 is a standard NEDS form for hauling.  Wet
suppression by water or water plus chemicals is sometimes used to
reduce emissions.  The SCC unit for this source is expressed in
vehicle miles.
     Crushing and screening are the major sources of particulates
from sand and gravel processing.  The emission factor associated
with all crushing and screening is 0.1 Ib per ton of product.   A
standard NEDS form for crushing and screening is shown in Figure
8.19-3.
     Emissions from aggregate storage include loading onto
piles, wind effects while  the materials are stored, and retrieval
activities from  raw material storage piles and sized product
piles.  A standard NEDS form is shown in Figure 8.19-4.
     Particulate emissions generated during material transfer  and
conveying operations throughout the process are reported under
the source labelled  "material transfer and conveying."  The
emissions are usually not  controlled.  A standard NEDS form  is
shown  in Figure  8.19-5.
     Emission factors for  aggregate storage and for material
transfer have not yet been developed.  When a plant  furnishes
emissions data  for  these  sources,  code the values given.   Enter
"Emission estimates  given  by plant", in the comments  field  on Card
7.
                               8.19-9

-------
     The emission factors assigned to the SCC numbers for sources


other than hauling are expressed as pounds emitted per ton


product.



CODING EIS/P&R FORMS


     The Basic Equipment Codes (EEC's) for use in EIS/P&R forms


are:


     Source                             BEC


     Hauling                          No code*


     Crushing and screening             650


     Aggregate storage                  700


     Material transfer and conveying    700
*
  As of November 1978.
                              8.19-10

-------
                  Figure  8.19-2.    Standard NEDS  form  for  sand  and  gravel  processing  -  hauling.
00
;  i s
                                                             NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                               ENVIRONMfNTAI PROTECTION AGENCY
                                                                   OFFICE OF AIR PROGRAMS
                                                                                       POINT SOURCE
                                                                                        InfMft fotm
                      FORM APPROVED
                      OMB NO IU ROMS
                                    lilt; 20
                         HAULING
                                                     zi :s 10
                                                                                         w     "I"
                          061 or 062

                              \i
                              i,
                                    Dec  M*>  Junr S*oi
                                    fro  M-v  Au«
                                                  00000
                                                                        3) =
                                                                             «t   X
                                                                           II 
                                                                                       JUIi'lioh:
                                                        ALLOWAbLt EMISSIONS (lorn
                                    IS H ?0 .'I !? 21
                                                   2) IS 25 ]0 II
                                                            ;; 33 is Ji H ;: n
                                                                        !' 40 
-------
                            Figure  8.19-3.    Standard  NEDS  form  for  sand  and  gravel  processing  -
                                                                 crushing   and  screening.
00
ACCf I Numn*"
                                                                    NATIONAL EMISSIONS DATA SYSTEM INEOS)
                                                                      ENV RONMENTAI PROTECTION AGENCY
                                                                          OFFICE OF AIR PROGRAMS
                                                                    POINT SOURCE

                                                                      IftfMil Form

                                                                   I Pnion
                                                                   linO, ftU*l
                                                                                                 FORM APPROVED
                                                                                                 OMB NO 1SI ROOK
                                                                                                 0...	
                                          IB 19
                           CRUSHING AND
                            SCREENING
                                               5

                                          Zo«->* >  M (I S? U M (i H » Ji 6» .-0
                                                                                                                                            1
                                                          N C
                                                                                                                                              I N

-------
     Figure  8.19-4.   Standard NEDS  form for  sand and  gravel processing  -
                                        aggregate  storage.
GO
•

M

I

CO
                                       NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                         ENVIRONMENTAl PROTECTION AGENCY
                                            OFFICE OF AIR PROGRAMS
                                                                                                      POINT SOURCE
                                                                                                       Input fotm
                                                                                                    FORM APPROVED
                                                                                                    OMB NO IMROOtt
                                                                                                 N«m« of Pe-s
                                                                                                 Completing f
                                                n/mnt Njmt and A Jrt. «
                                n \n
                              HOHMAi
                              TT|T
                                                                                         Contact P«
                                                                         ESTIMATED CONTROL EFFICIENCY t\\
                                                        EMISSION ESTIMATES l
                                                  nlu
AGGREGATE STORAGE
                                   ALLOWAtLt EMISblONS tllrf.. y«».l




                                           NO.
                      Uil
                                                   40 41
COMPLIANCE
  SIATLJS
  UPDATE
                    XSo+cef
                    y*- I
                                                                                                                 LLU
                                                                                                                   CONTROL REGULATIONS
                                                                                                                         a 2   B« 3
                                     SCC UNIT - TONS  PRODUCT
                                           MOo",      i~ r
                                          ..mumO**.^
                               N C
                                                                                          ElR

-------
                          Figure  8.19-5.    Standard  NEDS  form  for  sand  and  gravel  processing  -
                                                       material  transfer  and  conveying
CO
>£>
 I
                                                               NATIONAL EMISSIONS OATA SYSTEM INEOS)
                                                                 ENVIRONMENTAI PROTECTION AGENCY
                                                                     OFFICE OF AIR PROGRAMS
                                                                      POINT SOURCE
                                                                        Input fotm
                                                                                           OMb KG 1S8 ROO9b
                                      i I! 20 1\ '>
                   MATERIAL TRANSFER
                     AND CONVEYING
                                      1:4
                                             = 0
 Cxuc.i.
10*. BTuf"
                                                  UTM COOHOiNA T
                                                           13 Jl J? » I! 3! 3f
                                                                    S * 3" II 39 40 *1 »? U «
                                                                       r ;i » in In 12 ii
                                                                                   44 15 44 i; 4! w it 51 i7 U S4 SS 54li7 M :i
                                                                                                  TTIsV
                                                     77 II
                                                    0 0 0 OTO
                                                    OPERATING
                                                                              II 4.' 1)141 <', U|«I II !•)
                     ololo|o|olololololololo|o|o|o|oiolo|ololo'to
                                                                                                                • 0000  IF NO COmON STACK         S,
                                                                                                                 XXXX  POINT ID'S IF COWON STACK
                                                                                                    ESTIMATED CONTROL If f IOEMCV IM


                                                                                                              NO.    MC   CO
                                                                                                       i4 5) illil 58 41
                                                      .01 1 10
                                                                                                                  t.'lll (I ii U ('
                                                                                 EMISSION ESTIMATES
                                                               Pj'lrt.,1
                                                              i: :i n
                                                                             SO;
                                      U H 70 !l 72 7) Ii
ALLOWA«Lt EMISSIONS lion* i



         NO.
                                                          !0 Jl
                                                              3.' ]J J« Jl it !' It
                                                                          !' 40111 1? 4] 44
                                                                                      it :.' a\ii so 41 i:
                                                                                                  J, SCHEDULE
                                                                     COMPLIANCE
                                                                      S1-TU5
                                                                      UPDATE
                                                                                                                  (2 U
                                                                                                                            M VI n
                                                                                                                         ESTIMATION
                                                                                                                          METHOD
                                                                                                                                               75 JO
                                                                                                                                  ij 771
                                                                                           I loi  1 i  i
                                                                                                                           CONTROL REGULATIONS

                                                                                                                                R*q
                                                                                                                          «7 U,
                                                                                                                              $9 70 M 72
                                                            SCC UNIT - TONS
                                                                                                              U) (I
                                                      N C

-------
GLOSSARY

Gravel -  Loose,  rounded fragments of rock that are larger and
          coarser than sand.   Also called pebbles.

Sand   -  Separate grains or  particles of rock material,  easily
          distinguishable by  the unaided eye but too small to be
          classified as pebbles or gravel.

Scalping - The removal, by screen or grizzly, of undesirable fine
          material from broken ore, stone, or gravel.

Stacker conveyor - A belt conveyor with a hi-ided boom that dis-
          chrrges at the storage pile.  Use of conveyors  that
          rise and fall with the storage pile reduces the dis-
          tance that the stone must drop.

Stone Ladder - A fixed, rectangular column with a series  of steps
          inside that allow the falling material to cascade in
          short drops.  As the height of storage piles increases,
          the stone discharges through ports in the sides of the
          column and emissions are reduced.

Telescoping chute - A column that can be raised or lowered to
          maintain a constant distance between the stone being
          discharged and the top of the storage pile.

Thornthwaite's precipitation-evaporation ratio - An approximate
          measure of average surface moisture used in estimating
          fugitive emissions from outdoor storage.
                             8.19-15

-------
                   REFERENCES  FOR SECTION 8.19
 1.   Compilation  of  Air  Pollutant  Emission Factors.   2nd edition.
     Environmental Protection  Agency.   AP-42,  February 1976.

 2.   Midwest Research Institute.   Particulate  Pollutant System
     Study.   Volume  III.   Handbook of  Emission Properties.   EPA
     Contract No. CPA 22-69-104.   Kansas City, Mo.,  May 1971.

 3.   PEDCo Environmental,  Inc.   Background Information for  the
     Nonmetallic  Minerals  Industry.  Draft.  EPA Contract No.  68-
     01-1321,  Task No.  44.   Cincinnati, June 1976.

 4.   Newport,  B.D.,  and  J.E. Moyer.  State of  the Art:  Sand and
     Gravel Industry.   EPA-660/2-74-066, June  1974.

 5.   Engineering  Science,  Inc.   Exhaust Gases  from Combustion and
     Industrial Processes.   PB-204-861.  Washington, D.C.,  October
     1971.

 6.   Midwest Research Institute.   Particulate  Pollutant System
     Study.   Volume  I.   Mass Emissions.  EPA Contract No. CPA
     22-69-104.  Kansas  City,  Mo., May 1971.

 7.   Technical Guidance  for Control of Industrial Process Fugitive
     Particulate  Emissions. EPA 450/3- 77-010, March 1977.

 8.   Aeros Manual Series Volume II:  Aeros User's Manual.  EPA
     450/2-76-029 (OAQPS No. 1.2-039), December 1976.

 9.   Aeros Manual Series Volume V:  Aeros Manual of Codes.   EPA
     450/2-76-005 (OAQPS No. 1.2-042), April 1976.

10.   Standard Industrial Classification Manual, 1972 edition.
     Prepared by  Office of Management  and Budget.  Available from
     Superintendent  of Documents,  Washington,  D.C.

11.   Loquercio, P.,  and W.J. Stanley.   Air Pollution Manual of
     Coding.  Public Health Service Publication No. 1956.  U.S.
     Department of  Health, Education and Welfare, 1968.
                              8.19-16

-------
              8.20  STONE QUARRYING AND PROCESSING






PROCESS DESCRIPTION1"



     Crushed and broken stone have many applications, including



uses in road base, concrete aggregate, bituminous aggregate, and




in cement and lime manufacture.  Total production in 1977 was 914




million tons.



     Natural rock deposits are converted into crushed and broken



stone through a series of physical operations.  Drilling and



blasting are quarrying operations; crushing and screening are



among the plant operations.  Figure 8.20-1 gives a process flow



diagram for stone quarrying and processing.



     Stone processing plants are of two types:  stationary and



portable.  Stationary plants are usually located at or very near



the quarry, and the broken rock is hauled to the processing units



by truck.  A portable plant, which is designed to be moved from



one quarry site to another, consists of one or several chassis



upon which processing units are mounted.  The processing steps



are the same at stationary and portable plants; but in the latter,



the units are squeezed into a restricted space.



     The removal of overburden by earthmoving equipment leaves a



large denuded area that is worked into benches or ledges to form



an open quarry  (pit).  Blastholes are drilled into the exposed








                             8.20-1

-------
                                                                                                 PART ( 2
                                                                                                 -\
                                                                                                  I
                                                                                                 3-05-QZO-06
                                                                                        SCREENING/ CONVEYING/ HANDLING
           PART
3-S5-02Q-10
 DRILLING
                   BLASTING
                                   HAULING
                                                                   3-05-020-01
                                                                 PRIMARY CRUSHING
* TYPICAL SPRAY LOCATIONS

* CAPTURE POINTS
  LEGEND:

  (3 EMISSION  FACTOR8

0      EMISSION  FACTOR NOT DEVELOPED
      FOR THIS  PROCESS
  009 (66.0)  DENOTES CONTROL EQUIP.
  ,           CODE WITH EST. EFF.  SHOWN
  O
         IN (  )

         DENOTES  FUGITIVE
         EMISSIONS

         DENOTES  A STACK
                                                                                          A PART 
   a  IN POUNDS PER  SCC UNIT
                                                                                                            FINISHING (TERTIARY)
                                                                                                             SCREENS
                                                                                         SECONDARY
                                                                                          SCREEN
                                                                                       TERTIARY
                                                                                       CRUSHERS
                                                                                            3-05-020-03
                                                                     SECONDARY CRUSHING/
                                                                         SCREENING
                                                                                                                                      COMBUST ION I/
                                                                                                                                       PRODUCTS
 TO STORAGE
OR SHIPMENT
TO STORAG-
OR SHIPMENT
                                       Figure  8.20-1.    Stone  quarrying and  processing  operations.

                                                                                                                                                         TO STORAGE
                                                                                                                                                        OR SHIPMENT
                                                                                                                                       3-05-020-12
                                                                                                                                          DRYING
                                                                                                                                       3-90-006-99 NATURAL GAS
                                                                                                                                       3-90-004-99 RESIDUAL OIL
                                                                                                                                       3-90-005-99 DISTILLATE OIL
                                                                                                                                      IN-PROCESS FUEL
                                                                            8.20-2

-------
rock face, and the rock is blasted out of its deposit with ex-



plosives.  When the fragmentation is insufficient, the rock is



broken a second time, often with drop-ball cranes.  The broken



rock is loaded by loaders or shovelers into trucks (20- to 75-ton



capacity) and hauled to the processing plant.  The haul roads are



usually unpaved.  In portable plants, the rock is fed directly



into a primary-crusher hopper.



     Primary crushing is the first stage in stone processing.



The crusher  (commonly a jaw or cone type) reduces the rock to a



size of 3 to 12 inches.  This material is discharged onto a belt



conveyor that carries it to a surge pile for temporary storage.



     A series of vibrating feeders located under the surge pile



reclaims the stone by placing it on a belt for conveyance to a



scalping screen.  This unit consists of two screens that separate



the material into three fractions before secondary crushing:



oversizes, which are retained on the top screen; undersizes,



which are retained between the screens; and throughs, which pass



through both the screens.  The oversize is discharged to a sec-



ondary crusher for further reduction.  The undersize, which



requires no further reduction at this stage, bypasses the sec-



ondary crushers and thus reduces its load.  The throughs, which



contain unwanted fines and screenings, are removed from the



process flow and stockpiled for sale as a product or disposal as



landfill.  Secondary crushers are usually cone type, but impact



crushers are used at some plants.
                             8.20-3

-------
     After secondary crushing, the product, which is 1 inch or



less in size, is transported to a secondary screen for further



sizing.  Sized material from this screen is conveyed or dis-



charged directly to a tertiary crusher, usually of the cone or



hammer-mill type.   The product from the tertiary crusher is



shuttled back to the secondary screen, the two units forming a



closed circuit with a fixed maximum size, until the material has



been sufficiently reduced to pass through the secondary screen.



The throughs from this screen are discharged to a conveyor and



carried to a screen house or tower containing finishing screens



for final sizing.   Occasionally, fines mills are used to produce



a finer consistency.  After final sizing, end products of the



desired grade are dumped directly into finished-product bins, or



are moved by conveyor or truck to open areas for stockpiling.



The product is usually loaded into open trucks by front-end



loaders.



     Sometimes the stone must be washed to meet particular end-



product specifications, as for concrete aggregate.  The material



falls onto fine mesh screens in washing units, where it is sprayed



heavily with water.  Unwanted fines are discharged to a settling



pond.  Normally dryers are not used, but for some stones, such as



dolomite, drying may be necessary.  The dryers are usually direct-



fired, rotary units.



     Plant capacities range from less than a hundred to several



thcasand tons per hour.
                             8.20-4

-------
EMISSIONS ~5

     Virtually every operation in stone quarrying and processing

is a particulate emission source.  The emission sources are

identified in Figure 8.20-1.  Emission factors, listed on the

process flow diagram, are given in AP-42.   Average emission

rates for other sources were obtained from other documents and  .

are mentioned in the following source descr ptions.

     Unlike emissions from boilers and incinerators, emissions in

this industry have not traditionally been confined and discharged

through stacks or similar outlets.  It is possible for emissions

from drilling, crushing, screening, and conveying to be captured

with enclosures and hoods and collected in a control device.

Emissions from blasting, stockpiling, and hauling, however, are

not amenable to capture by a hood or similar device and are,

therefore, fugitive.

     Emissions at stone quarries and processing operations are

affected by the moisture content of the rock,  type of rock

processed, type of equipment, and operating practices.  Little

information is available on the quantities of  these emissions.

     During drilling operations, emissions arise when cuttings

and dust are removed from the bottom of the hole.  An estimate
                                                                4
for this source for  granite is  0.0008  Ib/ton of stone produced.

Blasting occurs between once a  week and several times a day,  de-

pending on  the plant capacity and  the  size of  individual  shots.

Emissions during blasting are affected by the  size  of shot,  type

of rock, and wetness.   Estimated emissions  from this  source  (for



                              8.20-5

-------
                                           4
granite)  are 0.16 Ib/ton of stone produced.   Emissions from


secondary breakage, usually done by drop-ball cranes, have been

                                                 2
judged by visual observation to be insignificant.   Emissions


from loading are also considered to be minor.


     At most quarries the haul roads are unpaved.  Traffic on


these roads generates a large portion of the fugitive particulate


emissions from quarrying and processing operations.  The amount

                                       2
ranges from 1.7 to 4.5 Ib/vehicle mile.   The level of these


emissions is affected by the composition of the road surface, the


wetness of the road, and the volume and speed of the traffic.


     During crushing, emissions come from the crusher feed and


discharge points.  Sometimes the crusher is housed in an unvented


building, but the degree to which internal settling  (baffling)


reduces the emissions in these cases is not known.  The emission


factors are based on the feed rate to the primary crushers.


Emissions are affected by the moisture content of the rock, the


type of rock processed, and the type of crusher.  Primary crush-


ing releases fewer emissions than secondary, tertiary, or fines


mills processing, because the material itself is less fine.


     Emissions from screening depend on the sizes of the material


screened, the amount of agitation, and the type and moisture


content of the rock.  The emission factors for secondary and


tertiary crushing  include the emissions from secondary and fin-


ishing screens,  respectively.  Emissions from the  scalping screen


are  included in  the  emission  factor  for screening/conveying/han-


dling.  Most of  the  emissions from material  handling occur at





                              8.20-6

-------
transfer points, because transport of material on the conveyor



creates little disturbance of air, and emissions due to wind are



judged to be minimal.   The transfer points include transfers



from one conveyor to another, into a hopper, and onto a storage



pile.  Only those transfer points that are not accounted for



elsewhere are included in screening/conveying/handling.  The



amount of uncontrolled emissions depends on the sizes of the



material handled, the belt speed, and the free-fall distance (the



vertical distance between the belt and the top of the pile or



belt to which the material is transferred).



     Washing generates no emissions.  Particulate emissions from



a dolomite dryer are reported to range from 2 to 50 Ib/ton of



product after a cyclone-type collector.



     Emissions from open storage occur during loading onto the



piles, action of the wind, and retrieval activities.  No data on



emissions during product loading are available.





CONTROL PRACTICES2"4



     Emissions from drilling have not commonly been controlled.



Two methods are available:  liquid injection, and collection by



aspiration to a particulate control device.



     Liquid injection is a wet-control technique in which water,



sometimes with a wetting agent (liquid detergent), is forced into



the compressed air stream that flushes the drill cuttings from



the hole.  The injection of fluid into the air stream produces a
                            8.20-7

-------
mist that dampens the stone particles and causes them to ag-


glomerate.  As particles are blown from the hole, most of them


drop as damp pellets at the drill collar instead of becoming


airborne.


     In the collection systems, a shroud or hood encircles the


drill rod at the collar; and a vacuum pulls the emissions through


a flexible duct into a control device for collection.  Control

                                                          2
devices most commonly used are cyclones or fabric filters.


     No effective method is available for controlling particulate


emissions from blasting.  Good blasting practices can minimize


noise, vibration, and air shock.  Scheduling blasting to occur


during conditions of low wind and low inversion potential can


substantially reduce the local impact of the emissions.  Emis-


sions from the loading of broken rock by loaders or shovels are


difficult to control.  Using water trucks equipped with hoses to


wet down the rock is a potential control technique.


     Watering of the haul roads during dry weather is the most


common method for reducing emissions from hauling.  Water is


applied to the road by water trucks that are equipped with either


gravity-fed spray bars or pressure sprays.  The amount of water


required, frequency of application, and effectiveness of this


method depend on the weather and the conditions of the roadbed.


Other methods for reducing emissions from the roads include soil


stabilization, paving, and lower vehicle speeds.  Paving is


probably  the most effective way to reduce emissions, but it is


very costly.




                             8.20-8

-------
     The plant processes either have water sprays to reduce emis-



sions or, less frequently, hoods to capture and direct them



through a control device.  Combinations of the two methods are



often used at different stages throughout the process.



     Wet suppression is an attempt to prevent fine particles from



becoming airborne.  At critical points, the material is sprayed



with water or water plus wetting agents.  The initial application



is usually made at the truck dump into the primary crusher.



Spray bars are located either on the periphery of the dump hopper



or above it.  Applications of water are also made at the outlet



from the primary crusher and from all subsequent crushers, where



new dry surfaces are exposed by the fracturing of the stone.



Water treatment may also be required at the feeders located under



surge piles.  If the material is properly treated at these points,



further applications of water at screens, conveyor transfer



points, conveyor and screen discharges to bins, and conveyor



discharges to storage piles may not be necessary; sprayed stone



exhibits a carryover effect that permits it to be handled through



a number of operations without significant emissions.  No data on



the effectiveness of wet  suppression have been developed, but a



well designed system can  eliminate visible emissions.



     Collection  systems  consist of enclosures and hoods that



confine  and direct the emissions to a control device.  Good



systems  enclose  the process equipment as completely as practi-



cable, yet allow access  for routine maintenance and inspection.
                              8.20-9

-------
The fabric filter is the most commonly used control device,



although cyclones and scrubbers are sometimes used.  Depending on



the layout of the plant, emission sources may be vented to one



central control device or to units at strategic points.  The



fabric filter is more than 99 percent effective, but the degree



of control depends on the efficiency of the enclosures and hoods.



Fines mills are usually vented to a fabric filter.



     In combination systems, wet suppression is used on the pri-



mary crusher inlet and outlet, screens, and other transfer points,



whereas the outlets of secondary and subsequent crushers are



vented to a control device.



     During conveying, emissions are reduced by the carryover



effect from wet suppression at transfer points.  Conveyor covers



are the most effective measure for controlling these emissions,



but they are not common because of high cost.



     The carryover effect from spraying after final crushing or



screening reduces emissions during loading onto open storage



piles.  Emissions are also reduced by such equipment as stone



ladders, telescopic chutes, and hinged-boom stacker conveyors.  A



stone ladder is a section of vertical pipe with steps inside to



check the fall of the stone.  This ladder reduces the free-fall



distance of the stone and protects it from wind.  The telescopic



chute is a retractable device that receives material from the



conveyor or truck and allows  it to fall freely  to the top of the



pile.  As the  level of  the  stockpile goes up or down, the chute
                              8.20-10

-------
is gradually raised or lowered.  Similarly, the stacker conveyor

is equipped with an adjustable hinged boom that raises or lowers

the conveyor according to the height of the stockpile.

     Watering is the most effective technique for reducing wind-

blown emissions from storage piles.  A water truck equipped with

a hose or other spray device is sometimes used.  One plant uses

spray towers around the stockpiles.  Emissions from washing are

minimal.  Dryers are usually equipped with cyclones.

     Moving the materials from stockpiles into open dump trucks

may generate significant fugitive emissions.  Controls are not

currently used, except for some attempts to wet the material

before loading and to empty the loaded buckets as close to the
                       2
truck beds as possible.   Some plants spray the loaded truck to

reduce emissions during transport.


CODING OF NEDS FORMS3'

     The emission sources associated with stone quarrying and

processing are:

Source                            SCC             Pollutant(s)

Drilling                       3-05-020-10         Particulate

Blasting                       3-05-020-09         Particulate

Hauling                        3-05-020-11         Particulate

Primary                        3-05-020-01         Particulate
  crushing
Secondary                      3-05-020-02         Particulate
  crushing and  screening

Tertiary                       3-05-020-03         Particulate
  crushing and  screening


                              8.20-11

-------
Source                            SCC             Pollutant(s)

Fines mill                    3-05-020-05         Particulate

Screening/conveying/handling  3-05-020-06         Particulate

Open storage                  3-05-020-07         Particulate

Drying                        3-05-020-12         Particulate,
                                                  combustion
                                                  products

(In-process fuel)

     Natural gas              3-90-006-99
     Residual oil             3-90-004-99
     Distillate oil           3-90-005-99

     Standard NEDS forms for each of the sources, Figures 8.20-2

through 8.20-11, show entries for the SCC's and other codes.

Entries in the data fields give information common to stone

quarrying and processing.  Information pertinent to coding the

source is entered on the margins of  the  forms and above or below

applicable data  fields.  Entries for control equipment codes,

other optional codes, emission factors,  and required comments

minimize  the need to refer to the code lists.  Typical data

values for operating parameters, control equipment efficiencies,

and  other source information are shown on  the form  (or in the

text) only  to  aid in rapid, approximate  checks of data submitted

by  the plant  in  a permit application or  similar  report.  Data

entered  in  EIS/P&R  and  NEDS must be  actual values  specific  to and

 reported by the  plant,  rather  than  typical values.   Contact the

 plant to validate  or  correct  questionable data  and to obtain

 unraported information.  See  Part 1 of this manual for general

 coding instructions.


                               8.20-12

-------
     Use appropriate SIC and IPP codes.  SIC Code 1400, which has

been used in the standard NEDS forms included here, is for mining

in general.  The SIC codes are:  1411 for dimension stone  (build-

ing stone); 1422 for limestone; and 1429 for all others.

     Except for a few items, coding of portable plants is simi-

lar.  Follow the special procedures described in Section 3.1.2 of

the Aeros Manual.

     In general, for emission sources that do not discharge

through a stack or vent and are not housed in a building, enter

zeros in the stack height, diameter, and common stack  fields, and

77 in the temperature field, unless temperature data are fur-

nished.  Enter appropriate plume height.  Where liquid sprays are

used to reduce particulate emissions, enter 061 or 062 as a

control equipment code.   In the comments field on Card 6,  identi-

fy other equipment used to reduce emissions.  For example, enter

"stone  ladders" where they are used.  For sources that do  not

directly discharge through a stack and  are not hooded  but  are

housed  in  a building, enter the roof vent data in the  stack  data

fields.  Enter  "roof vents" in the comments field.

     Emissions  from drilling are sometimes controlled.  Code the

operation  when  it  is controlled or when emission data  are  avail-

able.   Use 061  or  062 as  a  control equipment  code  for  liquid

injection  systems  and the appropriate  codes  for  cyclones and

 fabric filters.   Emissions  from blasting are  not controlled.

 Code the source when  emission data are available.   Standard NEDS

 forms  for  drilling and  blasting are  shown in Figures 8.20-2 and

 8.20-3, respectively.
                               8.20-13

-------
     Haul roads are usually watered to reduce the emissions.



Note that the SCC unit for this source is vehicle miles.  A



standard NEDS form is shown in Figure 8.20-4.



     Emission factors for secondary and tertiary crushing include



emissions from associated screening operations.  Other screening



operations are included in the source labeled "screening/con-



veying/handling," which also includes transfer operations not



accounted for in other sources.  Code the primary, secondary, and



tertiary crushing operations as shown in Figures 8.20-5, 8.20-6,



and 8.20-7.  Where combination systems are used, for those units



(usually secondary and subsequent crushers) that use fabric



filters, code the fabric filter as a primary control device and



enter "wet suppression" in the comments field.  For emission



sources equipped only with wet sprays, code 061 or 062 as a



primary control device.  Efficiencies of wet suppression can only



be estimated by plant inspection  (observation) during dry weather.



Where fines mills are used, code them as shown in Figure 8.20-8.



     Wet suppression affords some reduction in emissions from



screening/conveying/handling where the material is sprayed before



these operations.  Assign 061 or 062 as a primary control device



code to wet suppression or combination systems that are designed



to reduce emissions  from screening/conveying/handling.  Figure




8.20-9  shows a standard NEDS form.
                             8.20-14

-------
     A standard NEDS form for open storage is shown in Figure




8.20-10.  In the comments field, identify the equipment that is



used to reduce emissions during loading onto the piles.  Where



the piles are regularly sprayed to reduce emissions from the wind



and during retrieval activities, assign 061 or 062 as the primary



control device code.  Where dryers are used, code them as shown




in Figure 8.20-11.






CODING EIS/P&R FORMS9



     The EEC's for use in EIS/P&R forms are:
     Source



     Drilling



     Blasting



     Hauling



     Primary crushing



     Secondary crushing/screening



     Tertiary crushing/screening




     Fines mill



     Screening/conveying/handling




     Open storage



     Drying
   EEC



No code*



No code*



No code*



  650



  650



  650



651, 654



575, 577



  700



  452
* As of October 1978.
                              8.20-15

-------
      Figure  8.20-2.   Standard  NEDS form  for stone quarrying and processing  - drilling.
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      Figure 8.20-3.   Standard NEDS form  for stone  quarrying and processing - blasting.
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                                          NAIIUNAl (MISSIONS DAT A SYSUMINt OS)
                                           £*VinONMlNlAl PHOTFCTION AtiiNCY
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         Figure 8.20-4.   Standard NEDS  form for  stone  quarrying  and processing  -  hauling.
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-------
      Figure 8.20-5.  Standard NEDS form for stone quarrying  and processing - primary crushing,
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                   Figure  8.20-7.   Standard  NEDS  form for  stone  quarrying and processing -
                                            tertiary  crushing/screening.
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        Figure  8.20-8.    Standard NEDS  form  for  stone quarrying  and processing  -  fines mill.
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-------
                            GLOSSARY


Grizzly - A device used to remove large fragments of rock.  This
     is a form of a scalping screen, except that it has a series
     of heavy steel bars spaced parallel to each other.

Stacker conveyor - A belt conveyor with a hinged boom that dis-
     charges at the storage pile.  Use of conveyors that rise and
     fall with the storage pile reduces the distance that the
     stone must drop.

Stone ladder - A fixed, rectangular column with a series of steps
     inside that allow the falling material to cascade in short
     drops.  As the height of storage pile increases, the stone
     discharges through ports in the sides of the column and
     emissions are reduced.

Telescoping chute - A column that can be raised or lowered to
     maintain a constant distance between the stone being dis-
     charged and the top of the storage pile.
                             8.20-26

-------
                   REFERENCES FOR SECTION 8.20


1.    Pit and Quarry Publications, Inc.  Pit and Quarry Handbook
     and Purchasing Guide.   63rd edition.  Chicago, 1970.

2.    PEDCo Environmental,  Inc.  Control Tech iques for the
     Crushed -.ad Broken Stone Industry (Drafu).  EPA Contract
     Nos. 68-01-4147 and 68-02-2603, Cincinnati, May 1978.

3.    Compilation of Air Pollution Emission Factors.  2nd edition.
     Environmental Protection Agency, AP-42, February 1976.  pp.
     8.6-1 to 8.6-4, C16.

4.    Technical Guidance for Control of Industrial Process Fugi-
     tive Particulate Emissions.  EPA-450/3-77-010, March 1977.

5.    Air Pollutant Emission Factors.  U.S. Department of Health,
     Education and Welfare.  APTD-0923, PB-206924, April 1970.

6.    Aeros Manual Series Volume II:  Aeros User's Manual.  EPA-
     450/2-76-029  (OAQPS No. 1.2-039), December 1976.

7.    Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA-
     450/2-76-005  (OAQPS No. 1.2-042), April 1976.

8.    Standard Industrial Classification Manual.  1972 edition.
     Prepared by Office of Management and Budget.  Available from
     Superintendent of Documents, Washington, D.C.

9.    Loquercio, P., and W.J. Stanley.  Air Pollution Manual of
     Coding.  U.S. Department of Health, Education and Welfare.
     Public Health Service Publication No. 1956.   1968.
                             8.20-27

-------
              10.1.2  SULFATE (KRAFT)  WOOD PULPING






PROCESS DESCRIPTION1'2




     Wood is the most important source of fiber for paper pulp.




The pulp, or cellulose fibers, are extracted from the wood by




dissolving the lignin that binds the cellulose fibers together.




The pulp is used as raw material in the manufacture of paper,




cardboard, tissue, toweling, and related products.




     The kraft process accounts for about 65 percent of all pulp




produced in the United States.  This process, also known as the




sulfate process, is shown in Figure 10.1.2-1.  Wood chips are




cooked  (digested) in an aqueous cooking liquor at high tempera-




ture and pressure.  Regeneration or recovery of the cooking




chemicals is also part of the kraft process.




     The wood that is used as raw material may be purchased as




chips from other forest product manufacturers, or it may be




produced directly from logs or wood at the pulp mill.  "White




wood," from debarked logs, is the preferred material.  The logs




are cut at a 45-degree angle to the grain in a high-speed chipper,




producing a chip that measures about 1 inch by 1 inch by 3/16  inch,




The chips are screened for size and sent to a storage area.




     When they are needed, the chips are conveyed from storage




and placed in a digester.  Cooking liquor, containing sodium




sulfide and sodium hydroxide also known as "white liquor, is





                             10.1.2-1

-------
           I UQlwl
           OXIDATION
i-07-OOI-M   I I(M« J
iiquo> oiim
    TOUCH
                                                                                                      3-90-00«-"9
                                                                                                      4 - RESIWMM OH
                                                                                                      5 - OISIIUHIE OH
                                                                                                      6 - HATIIRM GAS
                                                                                          LCGfMI:

                                                                                          Q EMISSION FACTOK*

0                                                                                             EMISSION FACTOR NOT OEVELOPEO
                                                                                             F0« THIS PROCESS

                                                                                          009 (66.0) DENOTES CONTKH. EQUIP.
                                                                                                  COK KITH EST. EFF. SHOWN
                                                                                                  IN ( )
                                                                                           -

                                                                                          O
                                                                                                  MNOTES FUGITIVE
                                                                                                  EHISSIONS
                                                                                                  OEIIOTES A STACK
                                                                                          IK POUNDS PEK SCC UNIT
              Figure  10.1.2-1.    Sulfate  (kraft)  wood  pulping.
                                        10.1.2-2

-------
added.  The cooking time varies from 2 to 5 hours, at a tempera-
ture of about 350°F and a pressure of 100 to 125 psig.  When cook-
ing is completed, the contents of the digester are forced into
the blow tank, where the gases are relieved and the pulp and liquor
are separated.  Flash steam and gases released from the digester
are vented through a turpentine condenser, where heat is recovered
and the condensable vapors, in the form of t .rpentine, are removed.
Gases from the blow tank are also sent to a separate condenser.
The noncondensable gases, which are a source of malodors, are
primarily reduced sulfur compounds.  They are either confined and
treated or released directly to the atmosphere.  The ususal
treatment, where one is applied, is to carry the gases to the
lime kiln and introduce them with the air for combustion.
     The pulp from the blow tank is separated from the spent
cooking liquor, which is known as black liquor, by screening and
washing.  If the pulp is to be bleached, that operation is done
at this time.  The pulp is sent to the paper machine for futher
processing, or it is stored until needed.
     The black liquor that is removed during washing contains
about 96 percent of the alkali from the chemical solution that
was originally charged to the digester.  In some older kraft
pulping plants, this weak black liquor is conveyed to a liquor
oxidation tower where it is pumped against the flow of flue gas
from the recovery furnace.  This step is designed to oxidize the
reduced sulfur compounds that are a source of malodors.  In newer
plants, the oxidation tower is eliminated, and oxidation is per-
formed at a later stage in the recovery process.
                              10.1.2-3

-------
     The liquor is then pumped to a multiple-effect evaporator,


which uses steam to bring the liquor from a solids concentration


of 15 percent to one of 50 percent.  Using the heat from the


recovery furnace flue gas, the liquor is further concentrated to


between 55 and 70 percent solids in either a direct-contact or a


cascade (closed) evaporator.   The direct-contact evaporator may


include a cyclonic scrubber in older plants, or an ESP in newer


ones.  The concentrated black liquor is then burned in the re-


covery boiler furnace, and the heat from the combustion of the


organic constituents is used to generate steam.  The inorganic


compounds that remain after burning are removed from the recovery


furnace and dissolved in water in a smelt dissolving tank.  The


green liquor that is formed is then passed to a causticizer tank


and treated with slaked lime, to convert the sodium carbonate to


sodium hydroxide that can be recycled back to the digester.  The


lime slurry from the causticizer, after passage through a vacuum


filter, is dewatered and calcined in a lime kiln and stored for


reuse.


     Kraft mills operate continuously for about 350 days a year,


with downtime only for routine maintenance.  Their production


capacities range between 150 and 2700 tons of pulp per day.




EMISSIONS



     Both particulate and gaseous pollutants are emitted from


kraft pulp mills.  The emission  sources are identified in Figure

                                         2
10.1.2-1.  For  some of the  sources, AP-42  provides emission


factors, which  are listed on the process flow diagram.


                               10.1.2-4

-------
     Emissions from debarking, chipping, screening, and storage




are minor.



     The emissions from the digester and blow tank contain re-



duced sulfur compounds that pass through the condensers.



     Small  amounts of sulfur dioxide are emitted during the



washing and screening of the digested pulp.  Section 10.1.2 of



AP-422 lists an emission factor of 0.1 Ib per ton of air-dried,




unbleached  pulp.



     Liquor oxidation towers, when used, are sources of sulfur



dioxide and small amounts of reduced sulfur compounds.  The



multiple-effect evaporator emits small amounts of sulfur dioxide




and reduced sulfur compounds.



     The direct-contact or cascade evaporator receives  flue gas



from the recovery furnace; therefore these two units are con-



sidered one emission source.  This is the major emission source



in kraft pulping mills from which particulates, sulfur  dioxide,



carbon monoixde, and reduced  sulfur compounds are released.  The



particulates are generally less than 1  ym  in diameter.  Sulfur



dixoide emissions result mostly from the oxidation of  reduced



sulfur compounds in the recovery furnace.  Carbon monoxide emis-



sions are considerable.  Sodium sulfide in the black  liquor



reacts with carbon dioxide in the flue  gas to produce  hydrogen



sulfide, which  along with  several other organic sulfur compounds,



is responsible  for the characteristic odor of sulfate  pulping




mills.
                               10.1.2-5

-------
     The smelt dissolving tank and lime kiln are sources of


particulate emissions.  The lime kiln also emits CO and SO-.


The causticizer tank and vacuum filter are not emission sources.


     Some nitrogen oxides are emitted from the recovery furnace


and lime kiln, but the amounts are relatively small.  Nitrogen


oxide emissions from each of these sources are about 1 Ib per

                                     2
air-dried ton  (ADT)  of pulp produced.



CONTROL PRACTICES1'2



     The minor emissions from debarking, chipping, screening, and


storage are not controlled.


     In most cases,  the gases released from the digester are


vented to a condenser for recovery of the crude turpentine.  The


emissions from the blow tank are also sent to a condenser.


Noncondensable, odorous gases from the digester and the blow tank


may be vented to a stack, but are most often sent to the lime


kiln where the reduced sulfur compounds are destroyed by thermal


oxidation.


     The multiple-effect evaporator, which is a source of small


amounts of SO- and reduced sulfur compounds, is usually uncon-


trolled.


     The few emissions from the liquor oxidation tower are


either vented without treatment to a stack, or sent to the


multiple-effect evaporator.


     The reduced sulfur compound and SO- emissions from the


washing and screening operations are not controlled.



                              10.1.2-6

-------
     Several new mills have adopted recovery systems that eliminate


the conventional direct-contact evaporators.  In one system,


preheated combustion air, rather than flue gas, is used for the


evaporation.  In another, the multiple-effect evaporator system


is extended to replace the direct-contact evaporator altogether.


Both systems can reportedly decrease the reduced sulfur emissions


from the recovery furnace by more than 95 percent when compared

                                                          2
with uncontrolled systems using direct-contact evaporators  .


     In conventional systems, flue gas emissions from the re-


covery furnace are vented to the direct-contact or cascade evapo-


rator, and particulates are controlled by the evaporator control


devices.  Particulates are controlled in a variety of ways.


Control is especially important in mills where either a cyclonic


scrubber or a cascade evaporator serves as the final liquor


concentrator, because these devices are only 20 to 50 percent


efficient for particulates.  An electrostatic precipitator  is


most often used after the evaporator to provide an overall parti-


culate control efficiency of 96 to >_99 percent.  In a few mills,


however, a venturi scrubber is used after a direct-contact


evaporator to provide 80 to 90 percent particulate control.  In


either case, auxiliary scrubbers with an average efficiency of  90


percent may be included after the precipitator or the venturi


scrubber to provide additional control of particulates.  Carbon


monoxide and sulfur dioxide emissions are not controlled, al-


though the SO2 is incidentally reduced by the particulate control


devices.



                              10.1.2-7

-------
     Particulate emissions from the lime kiln are controlled by

venturi scrubbers having an efficiency of 99 percent.  Smelt

dissolving tanks use a mesh pad, together with a scrubber, if

needed to remove mists.  The efficiencies of these systems have

been reported as 75 and 80 percent, respectively.

     Although odor control devices are not generally used in kraft

mills, control of the reduced sulfur compounds that produce the

odors can be accomplished by process modifications and by improved

operating conditions.  For example, black liquor oxidation systems

can considerably reduce odorous sulfur emissions from the direct-

contact evaporator.
CODING NEDS FORMS
                 5-8
     The sources of criteria pollutants associated with sulfate

 (kraft) pulping are:
             Source

     Washers/screens

     Liquor oxidation tower

     Multiple effect
      evaporator
    sec

3-07-001-02

3-07-001-09


3-07-001-03
     Recovery furnace/direct-  3-07-001-04
      contact evaporator
     Smelt dissolving tank
     Lime kiln
      In-process fuel
3-07-001-05
3-07-001-06
3-90-OOX-99
  Pollutants
     SO,
     SO,
     so2

Particulates,
   S02, CO

Particulates,
     O \J •-)

Particulates,
   S02, CO
                                10.1.2-8

-------
     Standard NEDS forms for each of the sources, Figures
10.1.2-2 through 10.1.2-7, show entries for the SCO's and other
codes.  Entries in the data fields give information common to
sulfate (kraft) pulping.  Information pertinent to coding the
source is entered on the margins of the forms and above or below
applicable data fields.  Entries for control equipment codes,
other optional codes, emission factors, and required comments
minimize the need to refer to the code lists.  Typical data
values for operating parameters, control equipment efficiencies,
and other source information are shown on the form (or in the
text) only to aid in rapid, approximate checks of data submitted
by the plant in a permit application or similar report.  Data
entered in EIS/P&R and NEDS must be actual values specific to and
reported by the plant, rather than typical values.  Contact the
plant to validate or correct questionable data and to obtain
unreported information.  See Part 1 of this manual for general
coding instructions.
     The digester and blow tank are sources of reduced sulfur
compounds, but a NEDS form is not required for these sources
because no significant amounts of the criteria pollutants are
emitted.
     Emissions from washing and screening and from the liquor
oxidation tower, when used, are usually uncontrolled.  Figures
10.1.2-2 and 10.1.2-3 are standard NEDS forms for these sources.
     The multiple-effect evaporator is a source of SO,, emissions.
These are usually vented through a stack with no control devices.
Figure 10.1.2-4 is a standard NEDS form for this source.
                              10.1.2-9

-------
     The major sources of particulate emissions are the recovery



furnace/direct-contact evaporator, lime kiln, and smelt dis-



solving tank.  In some mills, a cyclonic or a venturi scrubber or



a cascade evaporator serves as the direct-contact evaporator,



with no further controls.  When this is the case, the process is



considered to have no control equipment.  An electrostatic



precipitator, however, is sometimes used after the direct-contact



evaporator, and would be coded as the primary control equipment



for particulates from the furnace.  If an auxiliary scrubber is



used with the ESP, the scrubber would be coded as a secondary



control equipment for particulates.



     The wet scrubber reduces S02 emissions by about 40 percent,



and when it is used it is coded as a secondary control device for



S02 because it is designed to control particulates and only inci-



dentally controls S02.  The CO that is emitted from the furnace



and the evaporator is not controlled, and is unaffected by the



ESP or scrubber control devices.  Figure 10.1.2-5 is a standard



NEDS form for the recovery furnace and direct-contact evaporator.



     A mesh pad or mist eliminator is used on the smelt dissolv-



ing tank as a primary control device for particulates.  This may



be followed by a wet scrubber as a secondary control device.



Figure 10.1.2-6 is a standard NEDS form for this source.



     A standard NEDS form for the lime kiln is shown in Figure



10.1.2-7.  A venturi scrubber is used to reduce particulates from



the kiln.  Emissions of  SO^  and CO are not controlled.  When










                              10.1.2-10

-------
emissions from other sources are vented to the kiln, enter a

comment in the comments field stating this.

     The SCC units are expressed as air-dried tons of unbleached

pulp.


CODING EIS/P&R FORMS9


     The EEC's of the process equipment in a kraft mill are:

               Device                        EEC

     Washers/screens                         450

     Liquor oxidation tower                  292

     Multiple-effect evaporator              308

     Recovery furnace and direct-          206/303
      contact evaporator

     Smelt dissolving tank                   287

     Lime kiln                               231
                              10.1.2-11

-------
 Figure 10.1.2-2.   Standard NEDS  form  for  sulfate  (kraft)  wood pulping -  washers/screens.
to
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-------
 Figure  10.1.2-3.   Standard NEDS  form for  sulfate  (kraft)  wood pulping  -  liquor  oxidation  tower
   APPHOvrO

OMB NO (rjH R0095

0.1!
to
I
M
U)
                                                                                          POINT ;,ouncE
                                                    NATIONAL EMISSIONS OAT A SYSTEM (NEOS)
                                                     ENVIRONMENTAL PROTECTION AGENCY

                                                         OFIICt OF AIR PROGRAMS
                                                                                             ,0000 IF NO COtfON STACK
                                                                                           /XXXX POINT ID'S IF COHON STACK
           LIQUOR  OXIDATION  TOWER '___
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-------
Figure  10.1.2-4.   Standard~NEDS  form  for  sulfate  (kraft)  wood pulping -  multiple-effect  evapprator,
lir
n:
                      intifrHii
NATIONAL EMISSIONS DATA SYSTEM (NCOS)
  ENVIRIHiMrNiAl PHOrFCTION AGENCY
     QFFICl OF AIH PROGRAMS
                                                                                                                  FOH.V, APPROVED
                                                                                                                  OVfc NO 1M K009S
                             ZUilLUJLL-LJ
                                   SSI3L

                                             .iltipflii
                                             J± u
                                           010
                                         ril
                                         OjO
       ;-|.irn
       T±j
                                                                     iiR
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                                                                                                     _
                                                                                                  wjsi .a \iih
                                                                                                  TTTT
                                                                                                   .0000 IF NO COMMON STACK
                                                                                                    XXXX POINT ID'S IF COMMON STACK
                                                                                               COMPOL EFFICIENCY I
                                                                                            --t-i-S
                                                                        Et.tlS'llON fSTl
                                                                    0.01
                                                                    I II  10
                                                                                                ESTIMATION
                                                                                                 METHOD
                                                                                                               63!
                                                                                                                               U
 I
I-1
           MULTIPLE-EFFECT EVAPORATOR
                                         cSCC UNJT-AI*-WY TONS UNBLEACHED PULP,':
                                                                                                 STATUS
                                                                                                             CONTROL REGULATIONS
                                                                                                Hf^i 1  I  fl^q 2
                                                                             H, .,F^.B«, |
                                                                             H1^ fal L- -,tc t
                                                                             T, rrrj^nkl

-------
  Figure 10.1.2-5.    Standard NEDS  form for sulfate (kraft)  wood pulping -


                         recovery furnace/direct-contact evaporator.
                                        NATIONAL EMISSIONS DATA SYSTEM (NEDS)

                                         ENVIRONMENTAL PROTECTION AGENCY

                                              OFFICE OF AIR PROGRAMS
                                                                                       OVf ',0 • ?" F-C09S
                                                                                            0000 IF NO COMMON STACK
                                                                                            XXXX POINT ID'S IF COWON STACK
                       ESP SCRUBBER.

                       Oil   1-002
                                                        CS7.MAT6D CO'iTPOL EFTlC'Er-'CV (M

                                                          EMISSION ESTIVATE5
                                  ALLOWABLE EMISSIONS llcni/y
•§
*!
ji
is"
is
5
333
fM ISI CSI
3
 rf* «
? » " 2
' 5 8
i \r\ —
0 °
«i
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s
8
at
_J M
I
s.g  s
          is ,;
                   sec SCC UNIT-AfrR-ORY TONS UNBLEACHED PULP-C
                       I    I  Furl P.^ri,
                             S. lirt Wji
                                                               ^l^'PsRilsofiilv
                                                               -rrrrrr
                                                               ffi

                                                                                          - ^^-4^  '"'-  I  ,r"';
                                                                                           ^    "
                   .L
     I   S. l.rt Wj-.ir
	  IV I  OP-..'..V, B,ir

ziiiTin0iu»i«i5i«
3Trm»
                               -RECOVERY FURNACE/DIRECT-CONTACT EVAP.

                             CCKWLNIS
                                                                                                UJ_J_
                                                                                  -I-

-------
     9T-Z'T*OT
     UNCONTROLLED

H    MESH PAD
t/>

     WET SCRUBBER
                                                               n
                                                               ro
NJ
 I
                                                                ft
                                                                (V
                                                                0)
                                                                h|
                                                                a
                                                                w
                                                                o
                                                                en

                                                                l-h
                                                                o
                                                                »-!
                                                                3

                                                                HI
                                                                O
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                                                                Hi
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                                                                ft
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                                                                 3
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                                                                 cn
                                                                 01
                                                                 o
                                                                 h-1

-------
Z.T-2'TOT
CONTROL
UNCONTROLLED
SCRUBBER
DEVICE
CODE

001
EFF. ,
X

93
PART.,
LB/TON
45
3
S02.
LB/TON
0.3
0.2
CO.
LB/TON
10
10
                                                    p-
                                                    H
                                                    (D
                                                    ro
                                                    I
                                                    co
                                                    rt
                                                    W
                                                    Hi
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                                                   M
                                                   3

-------
GLOSSARY


Sulfate or kraft process - A chemical process used to convert
     wood to papermaking fibers by using an aqueous solution of
     sodium sulfide and sodium hydroxide as the cooking liquor.

Digester - A device in which wood chips react with chemicals, at a
     specified pressure and temperature, to separate the wood
     fibers by dissolving the lignin.

White liquor - An aqueous solution of sodium sulfide and sodium
     hydroxide, used for cooking wood chips in the digester.

Black liquor - Spent or used solution from the digester.  It
     contains about 15 percent solids as it leaves the digester.

Green liquor - The solution of inorganic compounds generated from
     the recovery furnace.
                               10.1.2-18

-------
                  REFERENCES FOR SECTION 10.1.2
1.    Industrial Gas Cleaning Institute.  Air Pollution Control
     Technology and Costs:  Seven Selected Emission Sources.
     PB-245-065.   Stamford, Conn., December 1974.

2.    Compilation of Air Pollutant Emission Factors, 3rd edition.
     Environmental Protection Agency.  AP-42, August 1977.

3.    Lund,  H.F.,  (ed).   McGraw-Hill Book Company, Industrial
     Pollution Control  Handbook.  New York, 1971. pp. 18.17-
     18.27.

 4.   Standards of Performance For New Stationary Sources.  I^raft
     Pulp Mills.   Federal Register, Volume 43, No. 37, February
     23, 1978.

5.    Vatavuk, W.M.  National Emission Data System  (NEDS) Control
     Device Workbook;  U.S. Environmental Protection Agency
     APTD-1570, July 1973.

6.    Aeros Manual Series Volume II:  Aeros User's Manual.  KPA
     450/2-76-029  (OAQPS No. 1.2-039), December 1976.

7.    Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA
     450/2-76-005  (OAQPS No. 1.2-042),  April 1976.

8.    Standard Industrial Classification Manual, 1972 edition.
     Prepared by Office of Management and Budget.  Available from
     Superintendent of  Documents, Washington, D.C.

9.    Loquercio, P., and W.J. Stanley.  Air Pollution Manual of
     Coding.   U.S. Department of Health, Education, and Welfare.
     Public Health Service Publication No. 1956.  1968.
                              10.1.2-19

-------
                  10.1.3  ACID SULFITE PULPING






PROCESS DESCRIPTION1"3




     About 15 percent of the 35 million tons of paper pulp pro-




duced annual"y in the United States j r manufactured by the sul-




fite pulping process.  The lignin that binds the cellulose fibers




of the wood together is dissolved by an acid sulfite digestion




liquor composed of sulfurous acid and bisulfite salts.  The  pulp




(extracted cellulose fibers) is then used as the raw material for




the manufacture of such products as paper, cardboard, tissue, and




toweling.  The sulfurous digestion or cooking liquor is in solu-




tion with various bisulfites that act as buffers:  calcium,




especially in older mills; ammonium; sodium; or, increasingly,




magnesium.  The lignin is removed from the cellulose as soluble




lignosulfonotes.   Figure 10.1.3-1 is a flow diagram of a sulfite



pulping process using magnesium.




     Wood for raw material may be purchased as chips from other




forest product manufacturers, or may be formed from logs or wood




at tho pulp.ng mill.   "White wood," from debarked logs, is the




prefeired material.   Wood is transported to the mill by rail,




barge,  trucl ,  or ship,  and is stored in piles or in water.  Logs




are washed io remove dirt and are then debarked in drum or hy-




draulic bari ers.   The debarked logs are reduced to chips to










                              10.1.3-1

-------
                                                                                                                              3-U/-002-XX
                                                                                                                            RECOVERT SYSTEM
BASE
«g 0
HH3
Na
XX
21
22
23
1 ®
| S02 (9)
1 FLl
1
1
1
1
1
1
1
1
T
*
1
CONTROL
DEVKF
E GAS f«
WATER/
MAGNESIUM |

"bULFITE '
1
1
1
1
1 SCRUBBER Ut>3
DIRECT
— -p*- ^503 CONTAC
SO^W EVAPORAl

(^ "1 STRONG RED
L. — —1 i iramo
                               S02
                             ABSORBER
                                                                       ACID
                                                                     FORTIFIER
                                                                                              MULTIPLE-
                                                                                               EFFECT
                                                                                             EVAPORATOR
            3-07-002-VV
         DIGESTER  AND PULP
        BLOW PIT OR OUHP TANK


PULP

BASE
HH3
Ra
Ca


tw
31
32
33
HOT t
T
t
IATER )
t
WASHING AND
SCREENING
                                                                          SULFUR
                                                                          BURNER
                                                                                     AIR
                                                                                     MAKEUP
                                                                                     SULFUR
                                                                                  WEAK RED LIQUOR
                                                                                  Hg(OH)2
                                                    RED LIQUOR CONCEN1PATE


                                                    	 WATER
PROCESS  (DIGESTER & BLOW PIT OR DUMP TANK)
ALL BASES EXCEPT Ca
C« BASE
MgO WITH RECOVERY SYSTEM
MgO W/PROCESS CHANGE it SCRUBBER
Nf»3 H/PROCESS CHA06E t SCRUBBER
Na W/PROCESS CHANGE & SCRUBBER
VV
                                         03
                                         12
                                          13
                                         14
                                          15
            3-07-002-34
            WASHING AND
            SCREENING
                                 UNBLEACHED
                                    PULP
*THESE  LINES MAY
 GO DIRECTLY  TO
THE SO? ABSORBER
LEGEND:

(3   EMISSION  FACTOR3

0      EMISSION  FACTOP NOT DEVELOPED
      FOR THIS  PROCESS

009   (66.0) DENOTES  CONTROL EQUIP.
 »          CODE HI Til FST. EFF.  SHOWN
 I          "I ( )

  x,         DENOTE'..  Flit,! TIV'
.-'         EMISSION

Q         DENOTES A STACK
                                                                                                                                             III POUNDS PFP Sfr UNIT
                                      Figure 10.1.3-1.   Magnesium  -  Based Sulfite  Pulping  Process
                                                                                     1.3-2

-------
achieve a uniform size and to allow proper penetration of the



cooking liquor.  The chips are screened, washed, and stored  in



piles.



     Sulfurous acid for the digestion liquor is made by burning



sulfur and dissolving the resulting SO.-, in water.  Some of the



acid is converted to bisulfite (by adding calcium, ammonium,



sodium, or magnesium) to bring the mixture to the desired pH.



The liquor and the wood chips are mixed together in a digester at



high temperature and pressure.  When cooking is complete, the



mixture is discharged into either a blow pit or dump tank, de-



pending on how pressure is released.  The spent sulfite liquor



(red liquor) is separated out and the pulp is washed free of the



remaining liquor with hot water.   The pulp may be bleached during



subsequent papermaking operations.




     Treatment of the spent liquor depends on the base that  is



used.  Figure 10.1.3-1 shows a magnesium system.  Other systems



are similar although some older mills do not practice any chem-



ical recovery.   In a magnesium system, after being separated from



the pulp,  the liquor is partially concentrated in multiple-effect



evaporators.  It is then further  concentrated in a direct-contact



evaporator using hot flue gas from the recovery furnace.  The



concentrated liquor, at 55 to 60  percent solids, is burned in the



recovery furnace (without extra fuel), where the magnesium is



converted to magnesium oxide (MgO) and the sulfur species is oxi-



dized to S02.
                             10.1.3-3

-------
     The magnesium oxide is a solid, occurring in the form of


fine particulates.  It is separated from the flue gas by a me-


chanical collector, usually a cyclone that is part of the process


equipment, and slurried in water to become magnesium hydroxide


[Mg(OH)2l.  It is then sent to the S02 absorber.  The hot flue


gas is also sent to the S02 absorber, after traveling through the


direct-contact evaporator and picking up water vapor.  In the


absorber the gas stream is dissolved in the Mg(OH)_ solution,


regenerating the sulfurous acid and magnesium bisulfite liquor.


Makeup acid, which passes through a sulfur burner and an acid


fortifier, is added as needed.


     In calcium-based systems, the furnace is used for heat


recovery to produce steam.  The solids leaving the furnace are


calcium oxide and calcium sulfate; some SO,, is present in the


flue gas.  The solids are discarded after collection by an ESP or


a cyclone control device, and the cleaned flue gas enters the


atmosphere.  In some cases, the flue gas is sent to the S0~


absorber, which may be a limestone-packed tower or a series of


three or four venturi scrubbers.


     In ammonium-based systems, the products of the liquor com-


bustion in the recovery furnace are SO0  water, and nitrogen.
                                      ~ i

Very few solids are present; they are collected by a mechanical


dust collector and discarded.  The S0« is absorbed from the flue


gas by an ammonia solution to make the digestion liquor.
                              10.1.3-4

-------
     Sodium-based systems are often operated next  to  a  kraft



plant, and the spent liquor is burned with the black  liquor from



the kraft pulping.  In other cases, it  is burned alone  in a



kraft-type furnace and the sodium that  is recovered as  a sulfide



smelt is reused after chemical treatment- or it is shipped to  a


                                 1-4
nearby kraft mill and used there.     The SO2 is absorbed from



the flue gas by sodium carbonate that is recrvered from the



smelt.  Makeup sulfur dioxide is added  to produce  sodium bisul-



fite liquor for digestion.





EMISSIONS1"4



     Particulates and SO2 are the major pollutants from sulfite



pulping.  Emission sources are identified in Figure 10.1.3-1.

                              4

For some of the sources, AP-42  provides emission  factors, which



are listed on the process flow diagram.  For other sources of



emissions, average emission rates obtained from other documents



are mentioned in the following source descriptions.



     No significant emissions are generated by debarking, chip-



ping,  screening, and storage.  The digester and blow pit or dump



tank are a source of S02 emissions as well as acid mists and



water vapor.   The pH of the digestion process affects the SO~



emissions from these operations and from subsequent washing



operations.   Sulfurous acid,  which has a high vapor pressure,  is



present in a greater proportion at low pH.  The high vapor pres-



sure causes S02 to be released from the solution, resulting in



more emissions.  Solutions with higher pH levels have less poten-



tial for S02 emissions.




                               10.1.3-5

-------
     The digester relief and discharge techniques also affect



emissions.  When contents are blown out under high pressure,



large amounts of SO,,, which are difficult to capture and treat




efficiently in scrubbers, are released.  When the pressure in the



digester is relieved and the contents are pumped into a dump tank



the volume of emissions is much less and is more easily captured



and controlled.



     Some sulfur dioxide is emitted from the washing and screen-



ing operations.  When the other emission sources are well con-



trolled, this can be a large percentage of the total S0? emis-



sions from sulfite pulping.



     The multiple-effect evaporator is a source of S02 emissions,



and the recovery furnace is a source of both S02 and particu-



lates.  Particulate emissions are minimal where ammonia is used,



although  some gaseous ammonia may be emitted.  Where magnesium  is



used, magnesium oxide particulates are released from the recovery



furnace.  Where calcium is used, particulates composed of calcium



oxide and calcium sulfate are released.  The calcium is not



reused.   Where sodium is used, some particulates in the form of



sodium carbonate and sodium sulfide are emitted from the recovery



furnace;  however, most of the material is retained in the smelt.



Particulates and S02 from the recovery furnace pass through the



direct-contact evaporator, picking up  additional reduced sulfur



compounds in the evaporator.  These may be  released as  emissions




or  pent to the  S02  absorber.










                              10.1.3-6

-------
     Where chemical and heat recovery are practiced, the sulfur

oxide is scrubbed from the flue gas in the S02 absorber.  The

emissions from the absorber are particulates and SO2.

     The sulfur burner and acid fortifier, which provide makeup

acid for the digester, generate SO2;  however, the exhaust is sent

to the SO« absorber and is not considered an emission source.

     Estimates of S02 emissions from dif ferer c. process equipment,

without controls, are given below:

     Equipment          SO,., emissions, Ib/ton of pulp
                                (dry weight)
     Blow pit                      100-500
     Dump tank                      10-25
     Multiple-effect evaporator      5-10
     S02 absorber                   10-25
     Recovery furnace  (NH3 base)   250-500

Small amounts of nitrogen oxides and carbon monoxide may be

emitted with the flue gas from the recovery furnace.  The gas is

generally sent to the S02 absorber before being vented to the

atmosphere.


CONTROL PRACTICES1"

     Emission factors from various sources, with and without
                                       4
controls, are listed in Table 10,1.3-1.

     Emissions from the digester and blow pit or dump tank are

either sent to a scrubber or to the SO,, absorber for recovery of

SO- to be used as digestion acid.

     Sulfur dioxide generated during washing and screening of the

digested pulp is not controlled.
                              10.1.3-7

-------
    TABLE  10.1.3-1.   EMISSION  FACTORS  FOR SULFITE  PULPING'
Source
Digester blow pit
or dump tankc








Recovery system'


Acid plant?

Other sources1"-
Base
All
MgO
MgO
MgO
MgO

NH..
NH3
Na
Ca
MgO
NH3

Na
NH,
Na
Ca
All
Control
None
Process change6
Scrubber
Process change and scrubber
All exhaust vented through re-
covery system
Process change
Process change and scrubber
Process change and scrubber
Unknown
Multiclone and venturi scrubbers
Ammonia absorption and mist
eliminator
Sodium carbonate scrubber
Scrubber
Unknown*1
Jenssen scrubber
None
Emission factor
Particulates,
Ib/ADUT
Negd
Neg
Neg
Neg
Neg

Neg
Neg
Neg
Neg
2
0.7

4
Neg
Neg
Neg
Neg
Sulfur dioxide,
Ib/ADUT
10-70
2-6
1
0.2
0

25
0.4
2
67
9
7

2
0.3
0.2
8
12
a Data taken from  Reference 4.  All emission factors represent  long-term average
  emissions.
b Factors expressed  in  terms of Ib of pollutant per air dried unbleached ton of pulp (ADUT)

c These factors represent emissions that occur after the cook is  completed and when the
  digester contents  are discharged into the blow pit or dump tank.   Some relief gases
  are vented from  the digester during the cook cycle, but these are  usually trans-
  ferred to pressure a'ccumulators, and the SO2 therein is reabsorbed for use in the
  cooking liquor.  These factors  represent long-term emissions; in some mills, the
  actual emissions will be  intermittent and for short time periods.

  Negligible emissions.
e Process changes  may  include such measures as raising the pH of  the cooking liquor,
  thereby lowering the  free S02;  relieving the pressure in the  digester before the
  contents are discharged;  and pumping out the digester contents  instead of blowing
  them out.
f The recovery system  at most mills is a closed system that includes the recovery
  furnace, direct-contact  evaporator, multiple-effect evaporator, acid fortifier,
  and SO, absorption.   Generally, there will only be one emission point  for the
  entire recovery system.   These  factors are long-term averages and  include the high
  S02 emissions during the periodic purging of the recovery system.
9 Acid plants  are necessary in mills  that have no or insufficient recovery  systems.

h Control  is practiced, but type  of control is unknown.
 1 includes  miscellaneous pulping  operations such as  debarking,  chipping, washing,
  and  screening.
                                          10.1.3-8

-------
     Sulfur dioxide emissions from the multiple-effect evaporator



are controlled by a scrubber or are vented to the SO2 absorber



for reuse in digester acid.



     Particulates generated in the recovery furnace are con-



trolled by an ESP or by mechanical dust collectors, such as



cyclones.  Sometimes these devices are used together.  When the



captured particulates are recycled to the process, as in magne-



sium-based pulping, the cyclone is considered process equipment;



ESP's or scrubbers that follow the cyclone are control devices.



     Calcium oxide, calcium sulfate, and whatever particulates



result from ammonium-based combustion are discarded.  Most of the



particulates in a kraft furnace (which is used for sodium-based



liquor), are removed as molten smelt from the bottom of the



furnace.  Particulates entrained in the flue gas are partly



removed by mechanical means (usually cyclones), and sometimes



also by an ESP or scrubber.  In processes using ammonia, sodium,



and calcium, the cyclone, ESP, and scrubber are considered



control equipment.




     After the particulates have been removed, the exhaust gas



(containing S02) may be sent directly to a stack, or vented to



the direct-contact evaporator for heat recovery and then ex-



hausted through a stack.  The latter is practiced in some older



plants.  Usually, however, the recovery furnace gas is sent



through the direct-contact evaporator to provide heat for



evaporation and is then sent to the S02 absorber to recover SO,,.










                              10.1.3-9

-------
 These absorbers remove most of  the  SC^.   Efficiencies of more

than 95 to 98 percent are reported for  Mg(OH)2  venturi-type

absorber s.


CODING NEDS FORMS

     The sources of emissions  in  a sulfite pulping mill are:

     Source                  SCO                Pollutant(s)


Digester and blow pit or  3_07_002_vv               so
  dump tank                                           L

Washing and screening     3-07-002-34               S02

Recovery System           3-07-002-XX               S02> particulate

     The numbers assigned to the letters in the SCC's vary ac-

cording to the buffering agent  used.   The specific codes are

shown  in Figure 10.1.3-1.

     Standard NEDS  forms for each of the sources, Figures 10.1.3-

2 through  10.1.3-5, show entries for the SCC's  and other codes.

Entries in the data fields  give information common to sulfite

pulping.   Information pertinent to  coding the source is entered

on the margins of the forms and above  or below applicable data

fields.  Entries for control equipment codes, other optional

codes, emission factors, and required  comments minimize the need

to refer to  the code lists. Typical data values for operating

parameters,  control equipment  efficiencies, and  other  source

information  are  shown  on  the form (or in  the text) only  to  aid  in
                         10.1.3-10

-------
 rapid,  approximate checks of data  submitted  by the plant in a




 permit  application or similar report.   Data  entered in EIS/P&R




 and  NEDS  must  be actual values specific  to and reported by the




 plant,  rather  than typical values.  Contact  the plant to validate




 or  correct  questionable data and to obtain unreported informa-




 tion.   See  Part 1 of this manual for general  coding instructions.




      Figure 10.13-2 is a standard NEDs  form  for the digester and




 blow pit  or dump tank.  A different SCC  -lumber is  assigned to the




 blow pit  or dump tank according to the  base  that  is used.   The




 scrubber  on the digester and dump tank  or blow pit,  which  is a




 primary control device for S02,  is coded as  053.   If  the emis-




 sions are sent  to the S02 absorber, it  is the  control device and




 is coded  as 050 or 051.




      Emissions  of SO 2 from washing and  screening are  fugitive.




 A standard  NEDs form for this source is  shown  in Figure  10.1.3-3.




      The  recovery system employed  by sulfite pulp  mills  involves




multiple  pieces of process equipment including  a multiple-effect




 evaporator,   recovery furnace, direct-contact evaporator, and  S02




absorber.    The  controls  applied  to  and procedures  for  venting




 exhaust gases from each  piece of  equipment may  vary  from one  mill




 to another.   In  many mills  the  recovery system  is  a closed  system




 that includes all  of the process  equipment noted above.  As  such,




 there may be only  one  emission  point for the entire system.   Figure




10.1.3-4 is  a standard NEDS  form which treats  the  entire recovery




system as  only  one emission  point.   The emission factors in




Table 10.1.3-1  are also  expressed  on this basis.




     Alternatively,  if each  piece  of equipment  is  separately  vented




to the. atmosphere,  to  a  specific control device or  to  some  other




process it may  be  nore appropriate  to  treat  each piece of





                         10.1.3-11

-------
equipment as a separate emission  point.   In  these cases,  separate




point ID's should be assigned and  a.  NEDS  form coded for each piece




of equipment as necessary.  The SCC  for  the  recovery system,




reflecting the appropriate chemical  base,  should be used  in each




case.  Indicate in a card 6 or card  7  SCC  comment,  the process




equipment that is represented by  the emission point.  If  no




common stack is shared with some  other piece of  equipment in the




recovery system, enter (jxtxfxfr in points  with common stack field.




If a common stack exists, indicate appropriate point ID's in




this field instead.  Code control  equipment  codes as appropriate.




Specific information for each process  is  given below.




     The multiple-effect evaporator  is coded according to the




base used, either Mg, NH-j, or Na.  The wet scrubber control




device is coded as 053.  When the  emissions  are  instead sent to




the S02 absorber, code 050 or 051  as the  control device.   No




NEDS form for the multiple-effect  evaporator need be coded in




this case.  Include a comment with the SC^ absorber point, that




it includes multiple-effect evaporator off-gases.




     The recovery furnace generates  SC^  and  particulate emissions.




Particulates are generally removed from  the  gas  stream by a




mechanical dust collector, usually a cyclone.  For processes




using Ca, NH  , and Na, this cyclone  is a control device;  for




processes using Mg,  the  cyclone  is considered process equipment.
                        10.1.3-12

-------
An ESP, where  used,  is  a control device.  Where  the ESP  follows  a

cyclone in Ca, NH^,  and Na processes, the ESP is a secondary

particulate control  device.   After particulate removal  the  gases

may be vented  to  a  stack,  to the direct-contact  evaporator, cr  to

both the evaporator  and the  SCU absorber.  In the last  two  cases,

the emissions  are included on the NEDS forms for the direct-

contact evaporator  or  the  862 absorber.   The coder need  not include

a point for the recovery furnace in this case.   Indicate  by a

comment ^n the direct-contact evaporator or SC>2  absorber  emission

point, that off-gases  from the recovery  furnace  are included.

     The direct-contact evaporator receives flue gas from the

recovery furnace.   In  some older plants, the gas is vented  to a

stack after passing  through  the evaporator.  In most plants, the

gas is sent to the  862  absorber for SC>2  recovery.  Where  this is

the case, the  emissions from the direct-contact  evaporator  are in-

cluded on the NEDS  form for  the S02 absorber.  The coder  should

include a comment on the SO^ absorber emission point that direct-

contact evaporator  emissions are included.   No emission  point for

the evaporator needs to be defined in this  case.

     For the SC>2  absorber,  the SCC number is assigned according  to

the base used, either Mg,  NHo ,  or Na . No add-on SC>2 controls are

used on the S02 absorber.   A comment should be included  indicating

any other processes  that are vented to the  S02 absorber.

CODING EIS/P&R FORMS

     The BEG numbers for use. in EIS/P&R  forms are:

          Device                          B_EC

Digester and blow pit or dump tank       287
Washing and screening                     575
Multiple-effect evaporator               308
S02 absorber                              350
Recovery furnace                          206
Direct-contact evaporator                 303


                        10,1.3-13

-------
Figure 10.1.3-2.  Standard NEDS form for sulfite pulping - digester and blow pit or dump tank.
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            Figure  10.1.3-3.    Standard  NEDS  form  for  sulfite  pulping  -  Knotters/  Washers/Screens,  etc,
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                                                                 NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                                  ENVIRONMENTAL PROTECTION AGENCY
                                                                       OFFICE OF AIR PROGRAMS

                                                                      Eitjt.Mhmenl Nome and Aifrtren
                                                                            POINT SOURCE
                                                                              Input Form
                   FORM APPROVED
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                                                                       Njme ul Pfiion
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                                                   UTM COORDINATES
                                                                              STACK DATA
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                                       ANNUAL THRUPUT
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                                                                                                              Ilork  x
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      POINT ID'S IF COMMON STACK
                                                                                                        ESTIMATED CONTROL EFFICIENCY i\]
                                                                                                                   NO,
                                                                                   EMISSION ESTIMATES Uont/y«arl
                                                                                            NO,
             WASHING AND SCREENING
                                                           ALLOWABLE EMISSIONS lioni/vll'l


                                                                    NO,
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                                                      fu.l P.oc.ll       Mou.l,
                                                                                                      ^COMPLIANCE
                                                                                                                COMPLIANCE
                                                                                                                               ESTIMATION
                                                                                                                                METHOD
                                                                                           CONTROL REGULATIONS
                                                                                                                                      R'92

-------
Figure 10.1.3-4.  Standard NEDS form for  sulfite  pulping  -  recovery system.
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-------
                Figure 10.1.3-5.   Standard NEDS form for sulfite  pulping -  acid  plant.
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                                                      ENVIRONMENTAL PROTECTION AGENCY
                                                          OFFICE OF AIR PROGRAMS
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                                                                                                             t"Oul Fo»m
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  DEVICE
(PART.)

CYCLONE

ESP

(S02)

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                CODE
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                                                                                                       XXXX POINT ID'S IF COMMON STACK \y\

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-------
GLOSSARY


Lignin -  A group of polymeric molecules which  holds  the  cellulose
          fibers together.

Red liquor -   Spent sulfite digestion  liquor.

Smelt -   Molten sodium salts obtained  from  the sodium based
          recovery furnace.
                             10-1.3-18

-------
                 REFERENCES FOR SECTION 10.1.3
1.  Hendrikson, E.R., J.E. Roberson, and J.B. Koogler.  Control
    of Atmospheric Emissions in the Wood Pulping Industry.  Vol.
    1.  Environmental Engineering, Inc., and J.E. Surine Co.
    Contract No. CPA 22-69-18, U.S. Dept.  of Health, Education,
  •  an£ Welfare.  March 15, 1970.  pp. 3.62-3.71.

2.  Babcock & Wilcox.  Steam-Its Generation and Use.  38th
    edition.  New York, 1972.  pp.  26.11- 26.14.

3.  Kirk-Othmer Encyclopedia of Chemical Technology, Volume 16.
    2nd edition.  John Wiley & Sons, New York, 1963.  pp. 712-
    721.

4.  Compilation of Air Pollutant Emission Factors.  3rd edition.
    Environmental Protection Agency.  AP-42, August 1977.

5.  Aeros Manual Series Volume II:  Aeros User's Manual.  EPA
    450/2-76-029  (OAQPS No. 1.2-039), December 1976.

6.  Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA
    45/2-76-005  (OAQPS No. 1.2-042), April 1976.

7.  Standard Industrial Classification Manual.  1972 edition.
    Prepared by Office of Management and Budget.  Available from
    Superintendent of Documents, Washington, D.C.

8.  Loquercio, P., and W.J. Stanley.  Air Pollution Manual of
    Coding.  U.S. Department of Health, Education, and Welfare.
    Public Health Service Publication No.  1956.  1968.
                             10.1.3-19

-------
       10.1.4  NEUTRAL SULFITE SEMICHEMICAL  (NSSC) PULPING






PROCESS DESCRIPTION1'3



     Wood pulping extracts cellulose from wood chips by dissolving



the lignin that binds the fibers together.  The pulp is then used



as the raw material for the manufacture of paper, cardboard,



tissue, and towel products.  Neutral sulfite semichemical  (NSSC)



pulp is the variety that is produced by the partial chemical



dissolution of the lignin followed by mechanical disintegration.



About 10 percent of the 35 million tons of pulp produced in the



United States annually is made by the NSSC process.



     Figure 10.1.4-1 shows the process flow in an NSSC pulping



mill.   The wood chips used in pulping are purchased from forest



product manufacturing firms and delivered to the mill by truck or



rail,  or they may be produced from logs at the pulp mill.  In



this case, the logs are transported to the mill by rail, barge,



truck,  or ship, and are stored in piles or in water until needed.



The logs are washed to remove dirt and debarked in drum or hydraulic



barkers.   The debarked logs are then reduced to chips to provide



a size that is uniform, easy to handle, and allows even penetration



of cooking liquor during pulping.  The chips are screened to



remove oversized pieces (which are recycled) and slivers; then



the chips are washed to remove dirt and sawdust.  The chips are



then conveyed to storage piles until needed for pulping.




                             10.1.4-1

-------
                                                       9
1 } ' Na SO, r ~ , !
CHIPPING -^ SCREENING/ ^ \ ^ ? "^ ^^ ™) ™T°
J • / i f rnMRUvnnH .n.



(^ ^Y^ 3-07-003-04 r-U INTEGRAL 3-07-003-03
U S02 ABSORPTION TOWER 1 HcYCLONE FLUID-BED
DIGESTER T SOLID \S REACTOR
'SO- O Na,SO., [
i 2 ^^ , £ 4 ^C~T 	 • 	 ~^
3-07-003-01 1 °53 (99-5> 2 r\ 1^
— ' 	 • x SCRUBBER \^y
DIGESTER AND DUMP TANK f } VENTURI SULFUR * 	 <-n ^ CONCENTRATED
OR BLOW PIT /^r-"' BURNER •" 	 SUL1-UK iu2 v^i LIQUOR
| PRESSURE i ! f
DUMP TANK RELIEF*
OR BLOW PIT 3-07-003-02
LJ EVAPORATOR
HOT WATER

— ^
* PRESSURE RELIEF MAY BE 1 | Tn ,FUFR
VENTED DIRECTLY TO SO- I lu itwtl<
ABSORPTION TOWER '
PULP TO
MECHANICAL
DISINTEGRATION
LEGEND:
(^) EMISSION FACTOR3
O EMISSION FACTOR NOT DEVELOPED
FOR THIS PROCESS
009 (66.0) DENOTES CONTROL EQUIP.
CODE WITH EST, EFF. SHOWN
4 IN ( )
N DENOTES FUGITIVE
-' EMISSIONS
O DENOTES A STACK
3 IN POUNDS PER SCC UNIT
Figure 10.1.14-1.   Process flow diagram for NSSC pulping.




                     10.1.4-2

-------
     In the first part of the pulping process,  the wood  chips  are



cooked under pressure in either a batch or a continuous  digester



to partially delignify the wood.  The cooking  liquor  is  sodium



sulfite (Na2SO.,) , mixed with either sodium carbonate  (Na^CO  )  or



bicarbonate (NaHCCK).  The sulfite ion reacts  with the lignin  in



the wood while the sodium carbonate or bicarbonate acts  as a



buffer to maintain a neutral solution  (pH near 7).  The  sodium



sulfite may be purchased, or it may be produc ad at the mill  by



burning sulfur and dissolving the flue gas in  a sodium carbonate



solution in an S02 absorption tower for the reaction.



     Following digestion, the mixture is discharged into a dump



tank or blow pit to bring it to £itmospheric pressure.  A dump



tank is used to receive the mixture when the pressure in the



digester is partially relieved by a pressure relief system;  a



blow pit receives the mixture when the pressure is relieved  as



the material discharges from the digester.




     The material must be washed to remove the liquor from the



pulp.  The cooling liquor is drained and the pulp is washed  with



water,  usually on a multistage drum filter.  The washed  pulp may



then be further disintegrated mechanically by  grinders before



bleaching or manufacture into paper.  Some mechanical disinte-



gration of the pulp is done in the blow pit by blowing the



material onto a plate to break up the fibers.  This combination



of chemical delignification and mechanical disintegration can



yield as much as 60 to 80 percent pulp.  For coarser products,



such as cardboard, the mechanical disintegration is not  necessary.







                             10.1.4-3

-------
     The spent liquor from the washers is sometimes discarded to


the sewer system.  At mills that adjoin kraft pupling mills, the


spent liquor may be combined with the liquor from kraft processing


for chemical recovery.  (See the section on kraft pulping for a


complete description of this chemical recovery process.)  A third


way to dispose of the spent liquor is to concentrate it in an


evaporator and send it to a fluid-bed reactor for combustion.


This particular concentration and combustion process is unique to


NSSC pulp production.  In the fluid-bed reactor, the inorganic


solids are converted to sodium carbonate and sodium sulfate,


which are withdrawn as pellets.  An integral cyclone collects the


entrained solids and returns them to the bed, where any remaining


organic fraction undergoes further combustion.  The solids cannot


be reused in the NSSC process, but they are often sold to a kraft


mill -as process chemicals.



EMISSIONS1"3


     The major pollutants from NSSC pulping are sulfur oxides


 (SCO , hydrogen sulfide  (H2S) , and particulates.  The digester


and dump tank or blow pit, evaporator, fluid-bed reactor, and S02


absorption tower are the  four emission sources.  The fluid-bed


reactor also emits combustion products including CO and NOx/ but

                                      2
these are considered to be negligible.


      Emissions  from  the production of wood  chips  (debarking,


chipping, screening,  and  storage) are insignificant.  Pressure  is


periodically relieved  in  the  digester during  the cooking  cycle  to


maintain  the desired pressure in the vessel,  resulting  in


                              10.1.4-4

-------
intermittent gas release.  Intermittent gases released from the




digester contain SO2 and H2S; however, their quantities are




insignificant compared to those from the dump tank or blow pit.




The main emissions from the digester and dump tank are released




mainly from the digester when the digester and dump tank are




used.  When the digester and blow pit are used, these emissions




are released from the blow pit as shown in Figure 10.1.4-1.




Emissions from the pulp washer and mechanical disintegration are




considered insignificant.




     Mills that purchase sodium sulfite for the digestion liquor




have no SO,, absorber, and therefore no emissions from that




point.  Emissions of S02 and H2S from the SC>2 absorption tower




vary according to the operating conditions and efficiency of the




absorber.



     Mills that send the spent liquor to a sewer have no evap-




orator or fluid-bed reactor exhausts.  Liquor sent to a kraft




mill recovery system contributes to the emissions of that system.




The quantities of these emissions are not known, since they




depend on the operating and process variables at the kraft mill.




It is known that the NSSC effluent lowers the pH of the kraft



black liquor and, as a consequence, can cause generation of




H Q 1'2
ri~ o.



     Because of the scarcity of data on the many variations in




NSSC mills, no emission  factors are currently available.
                              10.1.4-5

-------
CONTROL PRACTICES1 3



     Intermittent emissions from the digester are not controlled.



Emissions from the pressure relief system of the dump tank or



blow pit are usually controlled by a scrubber, usually a venturi



scrubber; or the pressure relief may be vented directly to the


                                                      2
sulfur absorption tower at the mill when it is in use.



     Emissions from the evaporator are relatively small and are



usually uncontrolled.



     A wet scrubber is commonly used to control both the partic-



ulate and gaseous emissions from the fluid-bed reactor.  The



integral cyclone is considered process equipment rather than a



control device because it is a part of the reactor.  Efficiencies



as high as 99 percent can be expected for both the particulate



and S0~ control.  The CO and NO  emissions from the reactor are
      2.                        X


negligible and are not controlled.



     Emissions from the S0_ absorption tower are usually uncon-



trolled.




                 4-6
CODING NEDS FORMS



     The emission sources associated with NSSC pulping are:



Source                        SCC            Pollutant(s)



Digester and dump

 tank or blow pit         3-07-003-01        SO2



Evaporator                3-07-003-02        S02



Fluid-bed reactor         3-07-003-03        Particulates,  S02/

                                              combustion

                                              products
 S02  absorption  tower
3-07-003-04        SO.
                              10.1.4-6

-------
     Standard NEDS forms for each of the sources (Figures 10.1.4-




2 through 10.1.4-5)  show entries for the SCC's and other codes.




Entries in the data fields give information common to NSSC




pulping.   Information pertinent to coding the source is entered




in the margins of the forms and above or below applicable data




fields.  Entries for emission factors, required comments, control




equipment codes, and other optional codes minimize the need to




refer to the code lists.  Typical data values for operating




parameters, control equipment efficiencies, and other source




information are shown on the form  (or in the text) to aid in




rapid, approximate checks of data submitted by the plant in a




permit application or similar report.  Data entered in EIS/P&R




and NEDS must be actual values specific to and reported by the




plant, rather than typical values.  Contact the plant to obtain




unreported information and to validate or correct questionable




data.  See Part 1 of this manual for general coding instructions.




     Emissions from the digester and dump tank or blow pit are




usually vented to a venturi scrubber.  Code this operation as




shown in Figure 10.1.4-2.  When there is a different type of




scrubber, enter the appropriate code.  When the gases are vented




to the SO,, absorption tower, code  the tower as a control device




using code 050 or 051.



     Emissions from the evaporator  are not controlled.   Code  the




evaporator as shown in Figure 10.1.4-3.  The  integral cyclone  on




a fluid-bed reactor is part of the  reactor and not  a control




device.  Emissions from the reactor are  usually controlled with a







                              10.1.4-7

-------
scrubber, which controls both particulates and S02.   Figure



10.1.4-4 shows a standard NEDS form for the fluid-bed reactor



Code 001 in the particulate and S02 primary control device




fields.



     The S09 absorption tower is not controlled.  Code this



source as shown in Figure 10.1.4-5.






CODING EIS/P&R FORMS7



     The EEC's for use in EIS/P&R forms are:



Source                             BEG



Digester and dump tank or blow pit 287



Evaporator                         302



Fluid-bed reactor                  206



S0~ absorption tower               351
                              10.1.4-8

-------
                 Figure 10.1.4-2.    Standard  NEDS  form for NSSC pulping  -
                              digester and dump tank  or  blow pit.
        >,_ \_ TTi lisTa ji_i]ij
                   NATIONAL IMISSIONS DATA SYSItM (NtOSI
                     ENVIMfiNMCNIM PIlOTf CIION AGENCY
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-------
                Figure 10.1.4-3.  Standard NEDS  form for  NSSC pulping - evaporator,
H1
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                 NATION/H EMISSIONS OftTA SYSTEM (NEDS)

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                                                            MIS-jiON tSli'/ATiS IIO/M.V.*-!
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-------
Figure 10.1.4-4.   Standard  NEDS  form for NSSC  pulping -  fluid-bed  reactor,
                                      NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                       ENVIRONMENTAL PROTECTION AGENCY
                                          OFFICE OF AIR PROGRAMS
f~ NT SOURCE
    form
f O«M APPROVED
owe NO
Om
   FLIUD-BED REACTOR

-------
              Figure 10.1.4-5.    Standard NEDS  form for NSSC  pulping -  SO2  absorption  tower,
i
M
NJ
                                                       NATIONAL EMISSIONS DATA SYSTEM (NEDS)
                                                        ENVIRONMENTAL PROTECTION AGENCY
                                                            OFFICE OF AIR PROGRAMS
                           m
                    isse
                                              010!
     0|0
                                                          OToTo
                                                                           00
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                                                                                                                IPI
                                                                                              0000 IF NO COMMON STACK
                                                                                              "XXXX POINT ID'S IF COMMON STACK
                                                                                               l £FF(CIEVCV l\l
                                                                            •.O,
ALt-O-VABLE EMISSIONS 
-------
GLOSSARY

Black liquor - Spent (used) kraft digestion liquor.

Blow pit - The receiving pit for digested pulp released under
     pressure.

Dump tank - The receiving pit for digested pulp released from the
     digester after the pressure in the digestion vessel has been
     reduced by the pressure relief system.

NSSC pulp - Neutral sulfite semichemical pulp.
                             10.1.4-13

-------
                 REFERENCES FOR SECTION 10.1.4


1.   Compilation of Air Pollutant Emission Factors.  2nd edition.
    Environmental Protection Agency, AP-42, February 1976.  pp.
    8.6-1 to 8.6-4, C16.

2.   Hendrikson, E.R., J.E. Roberson, and J.B. Koogler.  Control
    of Atmospheric Emissions in the Wood Pulping Industry.
    Volume 1.  Environmental Engineering, Inc., and J.E. Sirrine
    Co.  Contract No. CPA 22-69-18, U.S. Dept. of Health,
    Education, and Welfare, March 15, 1970.  pp 3.54-3.61.

3.   Environmental Pollution Control—Pulp and Paper Industry,
    Part 1:  Air.  EPA/625/7-76-001, October 1976.

4.   Aeros Manual Series Volume II:  Aeros User's Manual.  EPA-
    450/2-76-029  (OAQPS No. 1.2-039), December 1976.

5.   Aeros Manual Series Volume V:  Aeros Manual of Codes.  EPA-
    450/2-76-005  (OAQPS No. 1.2-042), April  1976.

6.   Standard  Industrial Classification Manual.  1972 edition.
    Prepared  by Office of Management and Budget.  Available  from
    Superintendent of Documents, Washington, D.C.

7.   Loquercio, P., and W.J. Stanley.  Air  Pollution Manual of
    Coding.   U.S. Department of Health, Education, and  Welfare.
    Public Health Service Publication No.  1956.   1968.
                            10.1.4-14

-------
                                  TECHNICAL REPORT DATA
                           (Please read Instructions on the reverse before completing)
1  R'IPCRT NO
  EPA-450/4-80-007
                        J
    LE AND SUBTITLE
    ineering Reference  Manual  for Coding NEDS and
  TTs/P&R Forms:   Volume III
                                                          5. REPORT DATE
                                                       6. PERFORMING ORGANIZATION CODF
7 Al'"HOR(S)
 National Air Data  Branch
                                                          8. PERFORMING ORGANIZATION REPORT NO.
9 PERFORMING ORGANIZATION NAME AND ADDRESS
 U.S. Environmental  Protection Agency
 Office of Air  Quality Planning and Standards
 Monitoring and  Data Analysis Division
 Research Triangle  Park.  NC  27711	
 12. SPONSORING AGENCY NAME AND ADDRESS
 U.S. Environmental  Fiotection Agency
 Office of Air,  Noise and Radiation
 Office of Air  Quality Planning and Standards
 Research Triangle  Park.  NC  27711	
                                                           :. RECIPIENT'S ACCESSION" NO.
                                                           10 PROGRAM ELEMENT NO.
                                                       11 CONTRACT/GRANT NO.
                                                       13. YPE OF REPORT AND PERIOD COVERED
                                                       14 SPONSORING AGENCY CODE
15. SUPPLEMENTARY NOTES
 Associated  Volume  I  is a general
 additional  process  compendiums.
                                introduction to the manual.  Volume  II  presents
16. ABSTRACT
      This manual  provides specific engineering  guidance and background  information
 for the  evaluation and reporting of source/emissions data in NEDS or  EIS/P&R format.
 The manual  is  designed to assist coders  of  NEDS and EIS/P&R data who  may  not be
   imiliar with  a  wide variety of industrial  processes.
      Volume  III  consists of compendiums  of  information about specific  industrial
 processes.   Each compendium presents a process  description and process  flow diagram
 which  identifies the points in the  process  at which pollutants are  emitted, describes
 common  control  measures and presents codes  necessary for preparation of NEDS and
 EIS/P&R forms.   Specific guidance for the coding of process information is  given,
 with example preceded NEDS forms.   Each  compendium also includes a  glossary of
 technical  terms  and a list of pertinent  technical  literature.

      Volume  II  consists of process  compendiums  for additional industries.
17.

a.
                               KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
 NEDS
 CDHS
 EIS/P&R
 Point  Sources
 Air  Pollutants
 Emissions
 Cod-ng forms
                                          b.IDENTIFIERS/OPEN ENDED TERMS
                             COSATI Field/Group
    fl


    ,
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EPA Form 2220-1 (9-73)

-------
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-------