United States
Environmental Protection
Agency
Office of Air Quality
Planning and Standards
Research Triangle Park MC 27711
EPA-450/4-84-015
July 1984
Air
Compilation of Air
Toxic ajad Trace
Metal Summary
Statistics
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EPA-450/4-84-015
Compilation of Air Toxic and Trace Metal
Summary Statistics
William F Hunt, Jr , Robert B Faoro
and
George M. Duggan
U.S. ENVIRONMENTAL PROTECTION AGENCY
Office of Air and Radiation
Office of Air Quality Planning and Standards
Research Triangle Park, NC 27711
July 1984
•
O, EnvTrorwenfaT Pr?fec+Ton Sgemcy
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DISCLAIMER
This report has been reviewed by the Office of Air Quality Planning
and Standards, Environmental Protection Agency, and approved for publication,
Mention of trade names or commercial products is not intended to constitute
endorsement or recommendation for use.
-------
CONTENTS
Page
LIST OF FIGURES ii 1
LIST OF TABLES iv
1. INTRODUCTION 1
2. OBJECTIVE 1
3. DATA BASE AND COMPLETENESS CRITERIA 1
4. STATISTICS 4
5. DATA QUALITY 4
6. RES ULTS 6
7. POLLUTANT SPECIFIC DATA SUMMARIES 6
7.1 Volatile Organic Chemical (VOC) Pollutant Summaries 9
7.2 Trace Metal Pollutant Summary 10
8. REFERENCES 12
Tables A-l through A-20 14-45
Figures A-l through A-20 46-65
Tables A-21 through A-25 66-95
Figures A-21 through A-25 96-100
Tables B-l through B-13 101-114
Figures B-l through B-13 115-127
Tables B-14 through B-17 128-151
Fi gures B-14 through B-17 152-155
APPENDIX A. SUPPLEMENTAL POLLUTANTS 156
Table 1 and 2 157-164
Figures 1 and 2 165-166
ii
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FIGURES
A-l.
A-2.
A-3.
A-4.
A-5.
A-6.
A-7.
A-8.
A-9.
A-10.
A-ll.
A-12.
A-13.
A-14.
A-15.
A-16.
A-17.
A-18
A-19.
A-20.
A-21.
A-22.
A-2 3.
A-24.
A-25.
B-l.
B-2.
B-3.
B-4.
B-5.
B-6.
B-7.
B-8.
B-9.
B-10.
B-ll.
B-12.
B-13.
B-14.
B-15.
B-16.
B-17.
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(317)
(303)
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(329)
(321)
(306)
(104)
Acetal dehyde
Acrol ei n
Acryl oni tril e
Carbon Tetrachloride
Chloroform
Chloroprene
o-Cresol
p-Di chl orobenzene
Dimethyl Nitrosamine
Formal dehyde
Methyl ene Chl oride
Ni trobenzene
Phenol
Phosgene
Methyl Chloroform
Tol uene
Trie hi o roe thy! ene
Vinyl idene Chloride..
o-Xylene
m/p-Xyl ene
) Beryl 1 i um - Any Data
) Benzo( a)Pyrene - Any Data..
) Cadmi um - Any Data
) Manganese - Any Data.......
) Nickel - Any Data
1 ,3 Butadiene
Carbon Disulfide
Carbonyl Sulfide
Ethyl Chloride
1,2 Dibromomethane
c-1,2 Dichloroethylene
Ethyl benzene
Ethyl ene
Methyl Chloride
Methyl Ethyl Ketone
Naphtha! ene
Propene
Styrene
(42604 ) Ammoni a - Any Data
(12112
(12114
(12167
) Chromium - Any Data
) Copper - Any Data
) Zi nc - Any Data
Pag
46
47
48
49
50
51
52
53
54
55
56
57
58
59
60
61
62
63
64
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97
98
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...116
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...118
...119
.. .120
...121
. . .122
...123
...124
...125
.. .126
...127
.. .152
...153
.. .154
...155
Appendix A
1 Air Quality Sites for (001) Benzene...
2. Air Quality Sites for (12103) Arsenic
165
- Any Data 166
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TABLES
Page
1. Summary of Information Available for List of 37 Priority
Chemicals (Defined as Type A Pollutants) 2
2. Summary of Information Available for 50 Additional Chemicals
Under Assessment (Designated as Type B Pollutants) 3
3. Summary of Sites with Quarterly and Annual Averages for the
Volatile Organic Chemical Data Available on the Singh
Data Base 7
4. Summary of Cities with One or More Sites of Annual Averages
for the Trace Metal Data on SAROAD 8
A-l. Summary of Quarterly and Annual Average Statistics for
Acetal dehyde 14
A-2. Summary of Quarterly and Annual Average Statistics for
Acrolein 15
A-3. Summary of Quarterly and Annual Average Statistics for
Acrylonitrile 16
A-4. Summary of Quarterly and Annual Average Statistics for
Carbon Tetrachloride 17
A-5. Summary of Quarterly and Annual Average Statistics for
Chloroform 20
A-6. Summary of Quarterly and Annual Average Statistics for
Chloroprene 23
A-7. Summary of Quarterly and Annual Average Statistics for
o-Cresol 24
A-8. Summary of Quarterly and Annual Average Statistics for
p-Dichlorobenzene 25
A-9. Summary of Quarterly and Annual Average Statistics for
Dimethyl Nitrosamine 26
A-10. Summary of Quarterly and Annual Average Statistics for
Formaldehyde 27
A-ll . Summary of Quarterly and Annual Average Statistics for
Methyl ene Chi or ide 28
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TABLES (Continued)
Page
A-12. Summary of Quarterly and Annual Average Statistics for
Ni trobenzene 30
A-13. Summary of Quarterly and Annual Average Statistics for
Phenol 31
A-14. Summary of Quarterly and Annual Average Statistics for
Phosgene 32
•
A-15. Summary of Quarterly and Annual Average Statistics for
1,1 ,1 , Trichloroethane 33
A-16. Summary of Quarterly and Annual Average Statistics for
Tol uene 36
A-17. Summary of Quarterly and Annual Average Statistics for
Tri chl oroethyl ene 38
A-18. Summary of Quarterly and Annual Average Statistics for
Vinyledene Chloride 41
A-19. Summary of Quarterly and Annual Average Statistics for
o-Xyl ene 42
A-20. Summary of Quarterly and Annual Average Statistics for
m/p-Xyl ene 44
A-21. Toxic Air Data Summary - Four Highest Annual Averages for
Beryl 1 ium 66
A-22. Toxic Air Data Summary - Four Highest Annual Averages for
Benzo(a)Pyrene 71
A-23. Toxic Air Data Summary - Four Highest Annual Averages for
Cadmium .- 73
A-24. Toxic Ai r Data Summary - Four Highest Annual Averages for
Manganese 81
A-25. Toxic Air Data Summary - Four Highest Annual Averages for
Nickel 89
B-l. Summary of Quarterly and Annual Average Statistics for
1 ,3 Butadiene 101
B-2. Summary of Quarterly and Annual Average Statistics for
Carbon Disul fide 102
B-3. Summary of Quarterly and Annual Average Statistics for
Carbonyl Sul fide 103
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TABLES (Continued)
B-4. Summary of Quarterly and Annual Average Statistics for
Ethyl Chloride 104
B-5. Summary of Quarterly and Annual Average Statistics for
1 ,2 Dibromoethane 105
B-6. Summary of Quarterly and Annual Average Statistics for
c-1,2 Dichloroethylene 107
B-7. Summary of Quarterly and Annual Average Statistics for
Ethyl benzene 108
B-8. Summary of Quarterly and Annual Average Statistics for
Ethyl ene 109
B-9. Summary of Quarterly and Annual Average Statistics for
Methyl Chi ori de 110
B-10. Summary of Quarterly and Annual'Average Statistics for
Methyl -ethyl Ketone Ill
B-ll. Summary of Quarterly and Annual Average Statistics for
Naphthalene 112
B-12. Summary of Quarterly and Annual Average Statistics for
Propene 113
B-13. Summary of Quarterly and Annual Average Statistics for
Styrene 114
B-14. Toxic Air Data Summary - Four Highest Annual Averages for
Ammonia 128
B-15. Toxic Air Data Summary - Four Highest Annual Averages for
Ch romi urn 130
B-16. Toxic Air Data Summary - Four Highest Annual Averages for
Copper 136
B-17. Toxic Air Data Summary - Four Highest Annual Averages for
Zi nc 144
APPENDIX A
1. Summary of Quarterly and Annual Average Statistics for
Benzene 157
2. Toxic Air Data Summary - Four Highest Annual Averages for
Arsenic 159
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COMPILATION OF AIR TOXIC AND TRACE METAL SUMMARY STATISTICS
1. INTRODUCTION!
This report summarizes both air toxic data compiled by Dr. Hanwant
B. Singh of SRI International * and selected trace metal and benzo(a)-
pyrene data contained on the National Aerometric Data Bank's (NADB)
Storage and Retrieval of Aerometric Data (SAROAD).^ The pollutants,
that are summarized, are listed in Tables 1 and 2. Table 1 is a list
of 37 priority chemicals under assessment as potential carcinogens
(Type A Pollutants), while Table 2 lists 50 additional chemicals that
are under assessment (Type B Pollutants). Of the 37 pollutants listed
in Table 1, data were obtained on 24 pollutants. This compares with
finding information on only 17 of the 50 additional chemicals. In
addition to the above pollutants, arsenic and benzene are summarized in
Attachment A.
Emphasis has been placed on obtaining long term averages to match
the concern with chronic long-term exposure of human populations to
these pollutants. A long-term averaging time may be appropriate for
known and suspected carcinogens depending on the compounds ability to
induce significant health impacts.
2. OBJECTIVE
The principal objective of this report is to summarize the existing
data by calculating long-term annual averages. In the case of the air
toxic data compiled by Dr. Singh in his report, Volatile Organic
Chemicals in the Atmosphere: An Assessment of Available Data, the
information is generally spotty with few locations having sufficient
data to calculate an annual mean. In order to achieve the maximum
utilization of the available data on the Singh Data Base, quarterly
arithmetic means were computed, as well as annual arithmetic means.
The information on trace metals, and benzo(a)pyrene (B(a)P) available on
SAROAD, is far more complete with sufficient data available to calculate
annual means in many locations. With respect to B(a)P, it should be pointed
out there is a problem in underestimating its concentration, because part
of the sample is destroyed during the collection probably by conversion into
the epoxide. Although the product remains on the filter it is not detected
in the analysis.3>4
3. DATA BASE AND COMPLETENESS CRITERIA
Both quarterly averages and annual means were calculated for the
volatile organic chemical data available on the Singh Data Base. All
available data are summarized in the tables which follow. While quarterly
arithmetic means are listed with only one observation, the minimum
criteria that we recommend is five observations per quarter. This is
generally consistent with the existing NADB validity criteria, however,
no stratification of the five observations among the months of the
quarter is imposed. In order for a site to have a valid annual average,
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Table 1. Summary of Information Available for List of 37 Priority
Chemicals (Defined as Type A Pollutants)
Pollutant
Acetaldehyde
Acrolein
Acrylonitrile
Ally! Chloride
Benzyl Chloride
Beryl 1 i urn
Cadmium
Carbon Tetrachloride
Chlorobenzene
Chloroform
Chloroprene
Coke Oven Emissions
o-,m-,p- Cresol
p-Dichlorobenzene
Dimethyl Nitrosamine
Dioxin
Epichlorohydrin
Ethylene Dichloride
Ethylene Oxide
Formaldehyde
Hexachiorocyclopentadiene
Maleic Anhydride
Manganese
Methyl Chloroform (1,1,1 trichloroethane)
Methylene Chloride (dichloromethane)
Nickel
Nitrobenzene
Nitrosomorpholine
Perchloroethylene
Phenol
Phosgene
Polychlorinated Biphenyls
Propylene Oxide
Toluene
Trichloroethylene
Vinyl idene Chloride
o-,m,p-Xylene
Data Source
Singh Data Base
ii ii ii
Singh Data Base
N/A*
N/A
SAROAD
SAROAD
Si ngh Data Bas e
N/A
Singh Data Base
11 M 11
SAROAD
Singh Data Base
N/A
N/A
N/A
N/A
Si ngh Data Base
N/A
N/A
SAROAD
Singh Data Base
it ii II
SAROAD
Singh Data Base
N/A
N/A
Singh Data Base
n 11 n
N/A
N/A
Singh Data Base
*N/A - No data available
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Table 2. Summary of Information Available for 50 Additional Chemicals
Under Assessment (Designated as Type B Pollutants)
Pollutant
Acetic acid
Acetonitrile
Acrylamide
Ammonia
Barium carbonate
1,3 Butadiene
Carbon Disul fide
Carbonyl sulfide
Chlorine
Chloroacetic acid
Chloroethane (Ethyl chloride)
Chromium
Copper
Cumene
Cyclohexane
Dibenzofuran
1,2 Dibromoethane (Ethylene dibromide)
1 ,2 Dichloroethylene
Diethanolamine
Dioctyl phthal ate
Ethyl benzene
Ethyl ester acrylic acid (Ethyl acryl ate)
Ethylene
Ethylene glycol
Ethylene glycol monoethyl ether
Hexahydro-2H-Azepin-l-One (E-Caprolactam)
Isobutyraldehyde
Isopropyl alcohol
4,4 Isopropyl idenediphenol
Melamine
Methanol
Methyl chloride
Methyl ethyl ketone
Methyl methacryl ate
4,4 Methylenediani 1 ine
Molybdenum trioxide
Napthaiene
Pentachi orophenol
Phthal ic anhydride
Propene (Propylene)
Propional dehyde
Propylene dichloride
Styrene
Terephthal ic acid
Tert-butyl alcohol
Titanium dioxide
1 ,2 Toluene diisocyanate
Vinyl acetate
Zinc
Zinc oxide
Data Source
N/A*
N/A
N/A
SAROAD
N/A
Si ngh Data
Base
N/A
N/A
Singh Data Base
SAROAD
SAROAD
N/A
N/A
N/A
Si ngh Data Base
it it ii
N/A
N/A
Si ngh Data Base
N/A
Singh Data Base
N/A
N/A
N/A
N/A
N/A
N/A
N/A
N/A
Singh Data Base
II H H
N/A
N/A
N/A
Singh Data Base
N/A
N/A
Singh Data Base
N/A
N/A
Singh Data Base
N/A
N/A
N/A
N/A
N/A
SAROAD
N/A
*N/A - No data available
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it had to contain at least one winter quarter [quarter 1 (January - March)
or quarter 4 (October - December)] and one summer quarter [quarter 2
(April - June) or quarter 3 (July - September)]. This requirement was made,
because of the work of Paul J. Lioy, et. al. 5 which found seasonal
differences in ambient volatile organic chemical between the summer and
winter with winter averages higher than summer averages. Therefore, in
calculating an annual arithmetic mean at least one summer and one
winter quarter should be available in order to minimize bias. If a
site had valid quarterly arithmetic means for any 3 quarters, an annual
arithmetic mean would also be calculated. Ideally, four "valid" quarterly
arithmetic means are preferred. This occurred only 34 times for a
total of 8 volatile organic chemicals. Finally, in calculating the
annual arithmetic means each quarter is weighted equally.
The trace metal, ammonia and benzo(a)pyrene data were taken from
SAROAD. In order for a site to be listed it had to satisfy either the
NADB validity criteria or contain at least 20 daily observations per
year. In the event of chemical composite data, which are either monthly
or quarterly, an annual arithmetic mean would be computed if it had at
least 9 out of 12 monthly chemical composites or 3 out of 4 quarterly
chemical composites.
4. STATISTICS
Arithmetic mean statistics were calculated for both quarterly
and annual means for the volatile organic chemical (VOC) data. It
is recognized that other measures of central location may be more
appropriate depending upon the statistical distribution of the (VOC)
pollutants. Since the data, however, is so spotty, it is difficult to
examine the underlying statistical distributions of the VOC data. The
spotty nature of the VOC data is complicated by the fact that the data
consist of instantaneous data, data collected over several hours within
a day, data collected for one 24-hour period or one measurement
representing several days.
The number of observations associated with the quarterly and annual
means are the number of 24-hour measurements or their equivalents. An
equivalent 24-hour measurement is defined as either a single instantaneous
reading in a day, an average of multiple readings within a day or one
of several 24-hour periods contained in a long-term measurement lasting
several days. All the VOC data have been summarized in terms of micrograms
per cubic meter (ug/nP).
In contrast to the VOC data, the trace metal data are collected
using a high volume sampler. Only 24 hour measurements are made. Most
of the trace metal data consist of annual arithmetic means of the individual
24-hour measurements. In some cases, the annual arithmetic mean may be based
on either monthly or quarterly composites.
5. DATA QUALITY
Dr. H. Singh has assigned a data quality code to the volatile organic
chemical data listed in Tables A-l to A-20 and B-l to B-13. The code
can be sumarized as follows:
-------
1:
2:
3:
4:
Z:
= 1
= 1
= 2
> 2
Unable
.25
.50
.00
.00
to
5
(Excellent)
(Good)
( Acceptabl e)
(Questionable)
assign quality
Dr. Singh states in his report1, that in many cases, the information
that was available to make a quantitative assessment was lacking, and
the authors relied on their own experience and judgment. Where enough
information was available, the factor was used to establish the error
limits of the data, such that the "true" concentration is within a
factor of from the measured concentration (e.g. a measurement of 100
with quality code 2, =1.5, means that the "true" concentration lies
between 66.7 and 150). Their assignment of quality codes included
consideration of the comments of the original researcher, the
appropriateness of analytic techniques, the known limits of techniques,
accuracy and magnitude of reported concentrations. It should be noted,
however, that no probability is specified for the implied confidence
interval, which in the above example says the true concentration lies
between 66.7 and 150.
In addition to the data quality code assigned by Dr. Singh, the
volatile organic chemical data in most cases is collected using the
adsorbent tenax, which has recently become a cause for concern in
itself. Tenax has been discovered to suffer from a number of serious
problems as do other collection systems designed to collect many
chemicals in the air at the same time. Anong the most serious
problems uncovered are:
1 . chemicals in the sampled air can be transformed into other
chemicals (artifact formation).
2. the collection of certain chemicals like chloroform has been
found to have difficulties because of its instability in the absorbent.1
3. the collection of chemicals has been shown to vary with the
flow rate.
4. the desorbtion of certain chemicals collected can be difficult.
5. the breakthrough (overloading) of certain chemicals on the
tenax trap cannot be predicted.
Given the problems identified above, it is important to note that
the system utilizing tenax is the best system available at this time.
Improvements are being made to the collection system, such as distributed
air volumes which give reproducible results. In addition to tenax,
other absorbents are being considered which may be more reliable for
more compounds than tenax.
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6. RESULTS
Table 3 summarizes the number of sites with one or more 24-hour
observations or equivalent, one or more valid quarters, and "valid"
annual means for the 32 volatile organic chemicals, 19 of which are
from the original list of 37 pollutants (designated Type A Pollutants)
and 13 of which are from the supplemental list of 50 pollutants
(designated Type B Pollutants). From the tables it can be seen
that a total of 1206 sites had one or more observations, while only 498
sites had one or more "valid" quarters with considerably fewer sites, 96,
having "valid" annual means. Of the total of 32 volatile organic
chemicals only 14 pollutants have one or more sites with valid annual
means. In summary, the data are extremely spotty.
About one third (31) of the 96 sites with valid annual means had
means of zero meaning that all of the sampled values for the year were
below the minimum detectable limit for the analysis method. The chemicals
having the most non-zero annual means were toluene, trichloroethylene, and
o,m,p-xylene. Toluene, an aromatic hydrocarbon, trichloroethylene,
and o,m,p-xylene are very widely used chemical solvents having national
annual emissions of over 1 million tons for toluene, 100,000 tons
for trichloroethylene and 500,000 tons for o,m5p-xylene. The non-zero
annual means reported represent, for the most part, locations in California
and New Jersey. The highest annual mean reported for trichloroethylene
was 6.34 ug/m^ at Rutherford, N.J. in 1979. Background concentrations
of this chemical are reported to be about 0.16 ug/m^. The highest reported
annual mean for toluene was 82.64 ug/nP at a site in Brooklyn, N.Y., while
o-xylene reported an average of 8.26 ug/rn^ at Upland, California and m/p-
xylene an average of 23.30 ug/nP at again Upland, California.
In sharp contrast to the volatile organic data, is the summary
information available for trace metals, benzo(a)pyrene and'ammonia.
Table 4 summarizes the number of sites satisfying the NADB validity
criteria for an annual mean or those having at least 20 daily observations,
or 9 out of 12 monthly composites or 3 out of 4 quarterly composites.
The number of cities represented for the trace metals, ammonia,
and benzo( a)pyrene (BaP) with at least one site having an annual arithmetic
mean vary from a high of 312 cities for cadmium to a low of 46 cities
with BaP data. Cities with 2 or more sites vary from 57 for copper to
1 for BaP. About one-half of the cities having 2 or more sites are
located in the State of Texas since that state monitors extensively for
trace metals.
7. POLLUTANT SPECIFIC DATA SUMMARIES
The pollutant specific data summaries which follow, are divided
into the Type A Pollutants (the subset of the 37 priority chemicals
under assessment for which data is available) and the Type B Pollutants
(the subset of the 50 additional chemicals that are under assessment
for which data is available). Tables A-l through A-20 are the Type A
-------
Table 3.
Summary of Sites
Volatile Organic
with Quarterly and Annual Averages for the
Chemical Data Available on the Singh Data Base
Pollutants Volatile Organic Chemicals
No. of Sites
Type A
One or More One or More Valid
Obsn(s) Valid Quarters Annual Means
Acetaldehyde 9
Acrolein 2
Acrylonitrile 34
Carbon Tetrachloride 121
Chloroform 105
Chloroprene 1
o-,m-,p- Cresol 6
p-Dichlorobenzene 28
Dimethyl Nitrosamine 29
Formaldehyde 14
Methyl Chloroform
(1,1,1 trichloroethane) 115
Methylene Chloride
(dichloromethane) 49
Nitrobenzene 21
Phenol 9
Phosgene 10
Toluene 77
Trichloroethylene 113
Vinyl idene Chloride 41
o-,m,p-Xylene 131
0
1
0
44
39
0
6
6
1
36
19
9
6
9
45
43
12
82
0
0
0
8(6)*
8(6)
0
0
1
0
4
0
7(6)
0
0
12
8
6(6)
16
Type B
1,3 Butadiene 15
Carbon Disulfide 2
Carbonyl Sulfide 4
Chloroethane
(ethyl chloride) 7
1 ,2 Dibromoethane
(ethylene dibromide) 55
1,2 Dichloroethylene 32
Ethyl benzene 40
Ethylene 30
Methyl chloride 20
Methyl ethyl ketone 9
Napthalene 13
Propene (Propylene) 32
Styrene 32
23
10
20
12
20
6
10
14
10
0
0
0
6(1)
0
6
0
6(6)
0
6
0
1 (N) - Number of sites whose annual average was below minimum detectable limit.
-------
Table 4. Summary of Cities with One or More Sites of Annual Averages for
the Trace Metal Data on SAROAD
Pollutants
Trace Metal
No. of Cities
Type A
Beryllium
Cadmium
Coke Oven Emissions
(Benzo( a)pyrene)
Manganese
Nickel
One Site With
Annual Mean
186
312
46
301
258
Two or More
Sites with
Annual Mean
37
49
1
51
43
Type B
Ammonia
Chromium
Copper
Zinc
48
200
284
292
13
32
57
47
-------
volatile organic chemical pollutants for which there are data, while
Tables A-21 through A-25 are the Type A trace metal data. Similarly,
Tables B-l through B-13 are the Type B volatile organic chemical
pollutants for which there are data, while Tables B-14 through B-17
are the Type B trace metal data.
A map of the contiguous 48 states is provided for each of the
Type A and B Pollutants, showing the location of each monitoring
site having data. In the case of the VOC data, sites are indicated for
any monitor collecting one or more observations over the period, 1970
to 1980. The trace metal data represent sites operating over the
period, 1979 to 1982.
7.1 Volatile Organic Chemical (VOC) Pollutant Summaries
The VOC data are summarized in Tables A-l through A-20 and B-l
through B-13. They are summarized according to the following format:
SI DA S A --QTR 1 QTR 2 QTR 3 QTR 4 Annual--
City TE TA M M QUAL YR CNT AVERAGE CNT AVERAGE CNT AVERAGE CNT AVERAGE QTRS AVERAGE
The individual terms are defined as follows:
City = the state and city location of the site.
SI= the site type (UR = urban, RE = remote, SU = suburban,
TE RU = rural, and SR = source related)
DA= the data type [IN = instantaneous, HR = hourly avg.
TA DA = daily avg; IA = integrated avg. (1 to 7 days)
and LT = long-term avg. (>7 days)]
S= Sampling Method— Method by which the samples were collected, coded
M. as follows:
A = Di rect
B = Pressurized canisters
C = Absorbing resin
D = Absorbing cartridge (Tenax)
E = Bag samples
F = Cold trap
G = Bubbler
H = High volume sampler
-------
10
A= Analytic Method--Method by which the samples were analyzed, coded
M as follows:
A = GC-ECD (gas chromatography - electron capture
detection)
B = GC-FID or GC-FPD (flame ionization or photometric
detection)
C = GC-EC/coul (electron capture/coulometric)
D = Chemil uninescence
E = GLC-TEA (gas liquid chromatography - thermal
electron activation)
F = FTIR (Fourier transform infrared)
G = Total hydrocarbon analyzer
H = GC-PID (photoionization detection)
I = Bioassay
J = GC/MS
K = GC-MPD (microwave plasma detection)
L = Wet chemical techniques.
QUAL = Singh quality code (defined in Section 5)
YR = Year
QTR 1 , 2, 3, and 4 = Quarter 1 (January - March), Quarter 2 (April - June)
Quarter 3 (July - September) and Quarter 4 (October -
December)
CNT = no of 24-hour measurements or equivalents there are in the
quarterly average
AVERAGE = the arithmetic mean quarterly average
ANNUAL = the number of quarterly averages contained in the
QTRS AVERAGE annual arithmetic mean, followed by the annual mean,
which is weighted equally by quarter for those quarters
with at least 5 or more observations.
7.2 Trace Metal Pollutant Summary
The trace metal data are summarized in Tables A-21 through A-25
and B-14 through B-17. They are summarized according to the following
format:
ST CITY NAME SITE CODE MTD INT UNT YR OBS 1ST 2ND 3RD 4TH
-------
11
The individual terms are defined as follows:
ST - State abbreviation
City Name - The name of the city, county, or area where the sampling
took place.
The following six items refer to the site reporting the highest
annual average.
Site Code - the SAROAD site code which identifies the location of
the monitor within the city
Mtd - the method of sampling6
Int - the time interval over which the sampling took place^
Unt - the units of measurement (1-micrograms per cubic meter
3-nanograms per cubic meter)
Yr - the year of sampling with the highest annual average
OBS - the number of observations reported for this year
1st - the highest reported annual average
2nd - the second highest reported annual average
3rd - the third highest reported annual average
4th - the fourth highest reported annual average
The use of the heading "city name" is a slight misnomer since in some
cases the air quality information does not represent sites located in a
city but instead sites in counties or even in national parks. The
SAROAD area code (the 3rd through the 6th digits in site code) was used
to geographically arrange the sites into these groups. The first two
digits of the site code identifies the state6 e.g. 01-Alabama, 02-Alaska
etc., etc. The years 1979 to 1982 were used to obtain the most recent
and reliable estimates of annual averages with the exception of
Benzo(a)pyrene, where 1977 and 1978 were included to increase the annual
averages reported, since very few averages for BaP were found in the
1979-82 time period. Averages were reported which had at least 20 24-
hour observations, 3 quarterly composites, or 9 monthly composites
reported for the year. The four highest annual averages are presented
in order to define the highest annual averages reported in a given area.
-------
12
8. REFERENCES
1. R. Brodzinsky and H. Singh, Volatile Organic Chemicals in the Atmosphere:
An Assessment of Available Data. Final Report. Prepared for Larry
T. Cupitt, U. S. Environmental Protection Agency, Environmental Sciences
Research Laboratory, Research Triangle Park, N.C. Publication No.
EPA-600/3-83-027 (A). 1983.
2. D. H. Fair, SAROAD Station Coding Manual for Aerometric Sampling
Networks, U. S. Environmental Protection Agency, Office of Air Programs,
Research Triangle Park, N.C., EPA Publication No. APTD-0907. June 1972.
3. J. Peters and B. Seifert "Losses of Benzo(a)pyrene Under the Conditions
of Hi Vol Sampling" Atmos. Environ., ]£, 117-119 (1980).
4. J. N. Pitts, Jr., D. M. Lokensgard, P. S. Ripley, K. A. Van Cauwenberghe,
L. Van Vaeck, S. D. Shaffer, A. J. Thill and W. L. Belser, Jr.,
"Atmospheric Epoxidation of Benzo(a)pyrene by Ozone: Formation of the
Metabolite Benzo(a)pyrene-4,5-oxide" Science 210. 1347-1349 (1980).
5. P. J. Lioy, J. M. Daisey, T. Atherholt, J. Bozzelli, F. Darack,
R. Fisher, A. Greenberg, R. Harkov, B. Kebbekus, T. Kneip, J. Louis,
G. McGarrity, L. McGeorge, and N. Reiss, "The New Jersey Project on
Airborne Toxic Elements and Organic Substances (ATEOS): A Summary of the
1981 Summer and 1982 Winter Studies." J. Air Poll. Control Assoc.,
Vol . 33, No. 7, July 1983.
6. AEROS Manual Series Volume V: AEROS Manual of Codes (2nd Edition)
U. S. Environmental Protection Agency, Office of Air Quality Planning
and Standards. Research Triangle Park, N.C. Publication No.
EPA-450/2-76-005a. June 1983.
-------
13
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Appendix A SUPPLEMENTAL POLLUTANTS
This attachment summarizes arsenic and benzene data. The arsenic
data is taken from the National Aerometric Data Bank's (NADB) Storage
and Retrieval of Aerometric Data (SAROAD). It is summarized according
to the format specified in Section 7.2 of the main body of this report.
The location of the sites are shown on Figure 1. One hundered and
thirty-nine cities have at least one site with an annual arithmetic mean
and 20 cities have at least two sites with annual arithmetic means
(Table 1).
The benzene data is taken from the air toxic data base, consisting
of volatile organic chemicals, compiled by Dr. Hanwant B. Singh. The
data is summarized according to the format specified in Section 7.1 of
the main body of the report. The location of the sites are shown in
Figure 2. Of the 94 sites reporting one or more 24-hour observations,
41 sites have at least one valid quarter and 9 have a valid annual
average (Table 2).
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