vVEPA United States Environmental Protection Agency Industrial Environmental Research Laboratory Cincinnati OH 45268 Research and Development EPA-600/S2-81-043 Apr 1981 Project Summary Removal of Phenolic Compounds From Wood Preserving Wastewaters Bruce K. Wallin, Arthur J. Condren, and Roy L. Walden Laboratory and pilot-scale studies were undertaken to develop economically feasible technologies for the treatment of wastewaters from wood preserving operations. Of prime concern was the removal of phenol and its chlorinated derivatives, in particular, pentachlorophenol. Screening analysis of the wastewater indicated that pentachlorophenol was the only chlorinated derivative con- sistently present in concentrations of approximately 100 mg/l. Treatment technologies investi- gated for the treatment of these wastewaters included: 1. adsorption; 2. biological oxidation; 3. chemical oxidation; 4. coagulation; 5. extraction; and 6. pH adjustment. Each of the above, alone or in combination, was capable of yielding a measurable reduction in the concen- tration of total phenols and penta- chlorophenol in the untreated waste- water. Two technologies yielded consis- tently high levels of treatment: pH adjustment of the waste- water, followed by adsorption with bentonite clay and final polishing by the polymeric adsorbant, XAD-4; and 2. pH adjustment of the waste- water, followed by extraction with a mixture of #2 fuel oil and a co-solvent such as still bottoms from amyl alcohol production. Total annual operating costs for systems treating a typical 10,000 gpd of wastewater were calculated to be $40,000 and $23,600, respectively, for the two aforementioned technol- ogies. This report was submitted in fulfill- ment of Contract No. 68-03-2605, Work Directive No. 2, Parts 1 and 5, by the Edward C. Jordan Co., Inc., under the sponsorship of the U.S. Environmental Protection Agency. This report covers the period Novem- ber 20, 1978 to May 20, 1980, and work was completed as of May 20, 1980. This Project Summary was develop- ed by EPA's Industrial Environmental Research Laboratory. Cincinnati, OH. to announce key findings of the research report that is fully docu- mented in a separate report of the same title (see Project Report ordering at back). Introduction The U.S. Environmental Protection Agency has been involved in extensive investigations of toxic compounds being discharged from industrial facilities. Primary emphasis has been on the 65 "priority" pollutants, which are con- tained in the Settlement Agreement of ------- 1976 and in the Clean Water K 1977 (PL 95-217). Phenolics and U, chlorinated derivatives are a part of thiL group and are commonly found in the wood products industry's wastewater streams. The initial objective of this study was to evaluate the treatability of 2,4,6- trichlorophenol, parachlorometacresol, 2-chlorophenol, 2,4-dichlorophenol, and pentachlorophenol in the wood products industry's wastewater The wood preserving industry was selected for this program because wastewater from wood preserving facilities is usually low in volume but high in con- centrations of chlorinated phenolics. A chemical screening of the wastewater revealed that it had a high organic con- tent, but more significantly, it contained pentachlorophenol in concentrations exceeding 100 mg/l. The program's focus then shifted primarily to penta- chlorophenol to the virtual exclusion of all else, since only trace levels of other chlorinated phenolics were found. In conjunction with the treatability aspect, the program was intended also to explore atypical pretreatment schemes that would reduce chlorinated phenolics, namely pentachlorophenol, in typical wood preserving wastewater to levels at which the wastewater could be discharged to a POTW without causing an upset Owing to constraints imposed by time and financial resources, it was not the objective of this program to investigate all aspects of each treat- ment scheme (e g., residual catalyst after PCP removal, toxicity of the removal concentration, adsorptive capacity of the regenerated resin). The objective here was also not to improve the phenol-contaminated wastewater to drinking water quality, nor was it within the bounds of the study to make any conclusions concerning the toxicity of the residual pentachlorophenol con- centration in the wastewater that would be discharged to the POTW. The physical/chemical properties of pentachlorophenol, as distinguished from those of phenol, were important in considering the pretreatment systems which would be capable of reducing concentrations to an acceptable level. Pentachlorophenol consists of a ben- zene ring (CeH6) with all six hydrogen sites substituted by one hydroxyl group (OH) and five chlorine atoms (CU). The resulting compounds, CeCUOH, is mildly acidic, boils at 309°C, and is soluble in 50°C water at 30 mg/l Oils or emul- c .o •8 .0 CU (J to ID Oc t3 tb i/i <0 5) b ol 2,4-Dichlorophenol a 2,4,6-Trichlorophenol 0 Pentachlorophenol Figure 1. Phenolic resistance to biodegradation (2). sions in wastewater can provide a "carrier" effect, allowing pentachloro- phenol to far exceed its normal solubility in water. Table 1 summarizes the physical properties of several phenolic compounds. Figure 1 presents phenolic structures for several compounds. A review of available literature assisted the investigators in identifying treatment techniques foi investigation. Investigations were divided into two phases, preliminary bench-scale treat- ability studies and an evaluation of batch treatment techniques. Unlike phenol, which is quite unstable and easily oxidized either chemically or biologically, pentachloro- phenol is stable and resistant to oxida- tion In some instances, though, when wastewater containing pentachloro- phenol in concentrations which a biomass can tolerate is run through a biological treatment system, pentachlo- rophenol is adsorped onto the biofloc. Disposal of the sludge, now laden with pentachlorophenol, then presents a hazardous waste problem. Alkyliniza- tion of the sludge, a relatively common practice, would more than likely release the pentachlorophenol intotheenviron- ment If the sludge were incinerated, 2,3,7,8-tetrachlorodibenzo-p-dioxm, a thermal degradation product of penta- chlorophenol, could be released into the atmosphere. These rather ominous prospects make such treatment techniques as solvent extraction and batch polymeric resin adsorption, two schemes investi- gated during this study, more appealing from the standpoint of avoiding the creation of a hazardous waste problem while improving water quality In the preliminary bench-scale studies the investigators traveled to a wood preserving facility on the west coast to evaluate treatment technol- ogies, described m the literature, designed to lower pentachlorophenol concentrations Treatment schemes tested included pH reduction, acid cracking, chemical coagulation, chemi- cal oxidation, ultrafiltration, resin adsorption, and solvent extraction After conducting the preliminary bench-scale studies, the investigators reported to representatives of the EPA. Table 1. Physical Properties of Several Phenolic Compounds Compound Phenol o-Chlorophenol m-Chlorophenol p-Chlorophenol 2,4-Dichlorophenol 2,4,6-Trichlorophenol Pentachlorophenol o-Cresol m-Cresol p-Cresol p-Chloro-m-Cresol 2. 4, 6- Trichloro-m-Cresol Boiling Point °C 182 173 214 220 210 246 309 191 201 202 196 265 Solubility in H2O mg/l @ 25° C 93,000 28.000 26.000 27,000 4,500 900 30(50°C) 25.000 26,000 23,000 insol. si. sol. Ka x 10'° 1.1 77.0 16.0 6.3 Large Very Large Very Large 0.63 0.98 0.67 Unknown Unknown Ka = thermodynamic acid dissociation constant ------- At this time, mid-course corrections were suggested It was suggested that the program emphasis be shifted to focus on only those pretreatment systems that would both lower pervta- chlorophenol concentrations to levels acceptable for discharge to a POTW and be economically feasible for wood pre- servers To meet the revised criteria, pretreat- ment schemes had to be both efficient and economically feasible, which essentially eliminated from considera- tion the more elaborate treatment technologies (e.g., reductive degrada- tion, electrochemical oxidation, ion exchange, rotary vacuum filtration with activated carbon) The effectiveness of these cannot be denied, but the cost of installing and operating any one of them makes it economically impractical for wood preservers. Batch treatment systems were set up at the southern facility to provide some indication of which methods were cost effective. Technologies tested at the southern facility included batch biolog- ical treatment, chemical and polymeric coagulation, resin adsorption, acid cracking, bentonite clay, solvent extrac- tion, and filtration. As at the west coast facility, a combination of these were tested The size of the batch treatment reactors ranged from several litersto 50 gallons, depending on the pretreatment system being tested. Summary and Conclusions Processes for the treatment of waste- waters from two wood preserving facilities were investigated at the laboratory and pilot scale levels In- cluded were various chemical, physical, and biological operations selected specifically for the removal of phenol and its chlorinated derivatives. Of the treatment technologies investigated, two systems consistently lowered the concentrations of pentachlorophenol in the wastewater from 100 mg/l to less than 1 mg/l. In the first system, the wastewater was first acidified to a pH of 4.0 ± 0.1, then bentonite clay was added. A polymeric adsorbant, amberlite XAD-4 was used in the final polishing process. In the second system a mixture of No. 2 fuel oil and a cosolvent (amyl alcohol still bottoms) was used to extract penta- chlorophenol from the waste stream. Reductions were consistently in excess of 99 percent. Since No. 2 fuel oil is used often in the preserving process, as it was at this facility, it is conceivable that a facility could operate this extraction process without incurring any additional chemical expense, except possibly for the cosolvent. Trials with No. 2 fuel oil alone yielded removal ef- ficiencies in the vicinity of 97 percent, which may be high enough to allow the wastewater to be discharged to a POTW. For both systems to function consistently, the wastewater first had to be subjected to free oil separation and flow equalization.The following summarizes the findings of other inves- tigations, based on reductions in total phenol and/or pentachlorophenol con- centrations. pH Adjustment Lowering the pH of the wastewater with sulfuric acid was found to induce the formation of colloidal material. Sub- sequent removal of this colloidal mate- rial resulted in slight reductions in total phenol concentrations as measured by the modified lowry procedure described in the Project Report. Pentachloro- phenol concentrations, however, were consistently reduced from approxi- mately 100 mg/l to less than 20 mg/l. Biological Oxidation Biological oxidation was not found to be an effective treatment technique be- cause bioadsorption rather than bio- transformation was found to be the primary removal mechanism. Removal rates continued to diminish as the adsorptive capacity of the biomass was approached Chemical Oxidation At high doses, chlorine yielded sub- stantial reductions in the compounds of concern. Hydrogen peroxide, on the other hand, had little effect. The high chemical demand observed precludes the use of chemical oxidation as a viable treatment alternative Coagulation Coagulation with alum, ferric chloride, and/or polymers resulted in modest pollutant reductions. These reductions were not deemed sufficient to justify coagulation as a sole treat- ment technology. Applicability of Technologies In turning now to the applicability of the programs' findings to the wood pre- serving industry as a whole, it should be understood that the utility of any single pretreatment option is contingent upon both the volume and chemical make-up of the waste stream. Because wood preserving processes are so variant, each facility must be evaluated in terms of its preserving process, its waste stream, and the capital available for investing in a pretreatment system The systems devised for wood preservers in connection with this study would prob- ably not be transferable to the leather tanning industry or to the paper indus- try, not because a No. 2 fuel oil - cosol- vent mixture would not remove penta- chlorophenol from leather tanning or paper industry effluent just as effectively as it would from wood pre- serving wastewater, but because neither of these industries uses No. 2 fuel oil in its production process (non- combustion) as do some members of the wood preserving industry The advantage of the fuel oil extraction process is that the pentachlorophenol can be removed from the wastewater without creating an additional waste and without bringing large capital and operating expense to bear on the wood preserver. Recommendations If results obtained during these investigations are to be verified, a continuously flowing pilot-scale system must be established. Because this study was done on a quick response basis with limited financial resources, researchers could not investigate all aspects of each pretreatment scheme (e.g., residual catalyst after pentachlo- rophenol removal, toxicity of removal concentrations, utility or necessity of catalysts other than amyl alcohol still bottoms). Instead, the project provided an overview of the many economically achievable approaches to removing pentachlorophenol from wastewater and identified two systems especially successful in lowering pentachloro- phenol concentrations in wood pre- servers' wastewater to levels that would allow it to be discharged to the POTW without causing an upset. : US GOVERNMENT PRINTING OFFICE 1981 757-012/7060 ------- Bruce K Walhn, Arthur J Condren, and Roy L Wa/den are w/th the Edward C Jordan Co , Inc , Portland, ME 0417 2 Donald L. Wilson and Brian West fall are the EPA Project Officers (see below) The complete report, entitled "Removal of Phenolic Compounds from Wood Preserving Wastewaters, "(Order No PB81 -172637, Cost $12 50,subjectto change) will be available only from National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone 703-487-4650 The EPA Project Officers can be contacted at Industrial Environmental Research Laboratory U S Environmental Protect/on Agency Cincinnati, OH 45268 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati OH 45268 Postage and Fees Paid Environmental Protection Agency EPA 335 Official Business Penalty for Private Use $300 RETURN POSTAGE GUARANTEED ------- |