United States
                  Environmental Protection
                  Agency	    	
                       Air and Energy Engineering
                       Research Laboratory
                       Research Triangle Park. NC 27711
                  Research and Development
                       EPA/600/S7-89/006b Feb. 1990
x°/EPA         Project Summary
                   Evaluation  of FGD  Injection
                   Sorbents and Additives:
                   Volume 2. Pilot Plant
                   Evaluation  of High Reactivity
                   Sorbents
                  John C. S. Chang and Claus Jorgensen
                    A mini-pilot test  program  was
                  undertaken to investigate potential
                  new sorbents and processes for dry
                  SO2 removal. Initial testing showed
                  that the 85 m3/h pilot  plant could be
                  used successfully to  evaluate  both
                  spray  dryer  and dry  injection
                  processes using traditional calcium
                  or sodium based sorbents. The major
                  part of the test program Investigated
                  the use of flyash or  diatomaceous
                  earth for  enhancement of lime  with
                  respect to SO2  removal in a dry
                  infection process. This part of the
                  test program verified the silica
                  enhancement of Ca(OH)2 which
                  previously has  been extensively
                  studied on a  bench-scale reactor.
                  The pilot program showed that 50 to
                  90% SO2 removal can be achieved for
                  a stolchiom
                  injection of
                  when usin
                  + cyclone
                  recycle. TC
itric ratio of 1 to 2 by dry
the silica enhanced lime
)  a duct +  baghouse
                  configuration or when using a duct
configuration including
e  sorbent preparation
                  procedure was developed throughout
                  the test program, and  an important
                  result was that the silica enhanced
                  lime can be prepared as a  semidry
                  sorbent  containing  20 to 30%
                  moisture, suitable for duct injection.
                  This allows evaporative cooling of the
                  flue gas as a  result of the  sorbent
                  injection,  thereby lowering  the
                  approach  to  saturation and
                  increasing the SO2 removal.
                         This  Project  Summary was
                       developed by EPA's Air and  Energy
                       Engineering  Research  Laboratory,
                       Research  Triangle Park,  NC,  to
                       announce key findings of the research
                       project that is fully documented in a
                       separate report of the same title (see
                       Project Report ordering Information at
                       back).
Introduction
  A research program to evaluate an
emerging dry flue gas desulfurization
(FGD) technology was undertaken at the
Environmental Protection Agency/Air and
Energy Engineering Research Laboratory
(EPA/AEERL) in  Research Triangle Park,
North  Carolina. This research was
conducted on a recently  installed mini-
pilot plant, with an 85 m3/h simulated flue
gas flow. The pilot plant features a spray
dryer, a duct section, and a cyclone
separator or a  baghouse as  its  main
components  for controlling sulfur dioxide
(SO2) and particulates from a simulated
flue gas stream (see Figure 1).
  The initial goal of the program was to
start up the pilot facility and to evaluate
the S02 removal efficiency which can be
achieved in a spray dryer/baghouse test
configuration, using lime as sorbent. The
test  results  related well  to  previous
results, reported by other researchers,
which were generated on the  basis of
pilot  or  larger scale  testing. The

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                               Flue Gas Duct (2.0 SEC)
                       L.
                                           •11
              Water
              Tank
        SO2 Gas Supply —»»

               Sorbent Injection Point



         Figure 1.  Schematic of duct injection pilot plant facility.
                                                        Flue Gas Duct (0.8 SEC)
                                                   Spray Dryer
                                                . (Gas Humidifier)
                                            Clean-Side
                                             Gas Duct %


                                           n/
                                                                                                    Exhaust Duct
                                                                                                     (To Stack)
                                                                                       4
                 Temperature
                Control Panel
adequacy  of  the  mini-pilot  plant  as  a
suitable  test facility  for preliminary
evaluation  of new  processes  and
sorbents therefore seems justified.

Pilot Plant  Tests
   Testing using the pilot plant for dry
injection studies in combination with flue
gas humidification was  accomplished by
spraying water from the rotary atomizer
in  the spray  dryer, then  injecting dry
sorbent in the  duct  section  located
downstream. Specifically,  calcium
hydroxide  [Ca(OH)2]  and sodium
bicarbonate   (NaHCOa)  have  been
injected into the humidified flue gas and
entrained to the fabric filter baghouse for
collection. The normal sorbent residence
time in the gas stream provided  by this
equipment configuration ranged from 10
to  30 minutes. The results, specifically in
terms of  SO2 removal  and  sorbent
utilization, can be related to previously
performed bench-scale  testing  in  a
packed bed reactor. These results clearly
demonstrate  the  limited  potential  of a
totally dry Ca(OH)2  injection  process, as
compared to a spray drying process.
   Consequently,  the major  part of the
test  program  uses a recently developed
method which enhances lime with  silica
in  order to promote its reactivity toward
S02. This method, extensively tested in
bench-scale  packed bed reactors used
flyash or diatomaceous earth as the silica
source. Under the present pilot program,
lime was  slurried with  either flyash or
diatomaceous  earth  at   elevated
temperatures of 85 to 95°C for prolonged
periods of time  (8 to  16  h). The lime
slurry was  then dewatered  and  the
resulting  filter  cake dried to  produce a
powder.  Injection  of this  "silica
enhanced"  lime  into  the simulated  flue
gas stream  and  its entrainment to  the
baghouse  for   collection   clearly
demonstrated an  increased S02  removal,
compared  to using  pure  Ca(OH)2.
Parametric testing was  undertaken to
evaluate  the effect  of  varying  sorbent
preparation  procedures  (e.g., changing
the silica/lime  ration, the  slurrying
temperature, and time  period  used  for
slurrying; or  using potential additives like
sodium hydroxide (NaOH) to increase the
solubility  of silica). Also  investigated were
the effects on the S02 removal efficiency
of changing  various operating  conditions,
e.g., the  approach  to  saturation (At,),
stoichiometric  ratio  (SR),  S02
concentration in the inlet gas.
   Most of these pilot plant results seem
to confirm the effects  which had been
anticipated from  the bench-scale testing.
The most significant evidence obtained,
however, is the relationship between S02
removal efficiency and SR, which  could
not have been determined  from bench-
scale testing.
   Both the baghouse and the cyclone
separator have been used for particulate
collection  of silica-enhanced  lime
sorbent. The cyclone separator simulates
the relatively short  residence  time
provided by an electrostatic precipitator
(ESP)  for the sorbent in the flue gas
stream. The  highest  SO2 removal and
sorbent utilization  are  achieved  when
using  a  baghouse  for  particulate
collection, obviously relating to the longer
sorbent residence time in the baghouse.
However,  as most  of  the existing  coal
fired  utility  boilers in the  U.S. are
equipped with ESPs, the main goal of the
present work is to study retrofit options
for S02  control  for  those  facilities.
Continued work focused on the use of a
cyclone  separator  for  particulate
collection in the pilot plant.
   The concept of recycling the product
collected in the cyclone separator  back
into the  makeup sorbent consisting  of
silica-enhanced lime was now introduced.
Normally, the collected product is only
partly  reacted, and therefore  contains
unutilized sorbent.  The advantages  of
reintroducing it into the flue gas streaml
thereby increasing  its overall  residence

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time, seem obvious. The success of this
approach  is  also explained  by  its
t/ersatility  as a means of "dewatering"
the makeup slurry (or paste). Dewatering
converts the silica-enhanced lime sorbent
into a semidry, manageable powder, with
20 to 30% moisture, which is suitable for
dry injection. Injecting  this semidry
sorbent into the flue gas duct at an At, of
up  to  55 °C demonstrates the effect of
flyash  drying the sorbent throughout the
duct section, thereby lowering the Ats to
10 to 20° C and achieving significant S02
removal across the short  residence  time
(2s) duct section prior to collection of dry
product (about 5% residual moisture) in
the cyclone.  Finally, the  direct  use of
recycle solids, rather than pure flyash, as
the silica  source for lime enhancement
was also successfully tested.
   An  overall flow   sheet  for  the
developed  process is  being  proposed
(Figure 2).  Based on  these  mini-pilot
plant  results, this  particular process is
expected to result in about 50% sorbent
utilization when used in combination with
an ESP for particulate  collection.  About
50% S02 removal is expected for an SR
of 1.  Based  on  mini-pilot plant results
only,  a utilization  of  at  least 80% is
expected if a fabric filter baghouse is
used, which provides  a longer sorbent
residence time in the gas stream.
   Testing in the immediate future should
undertake  the pilot  development of
pressure hydration  to enhance lime with
flyash/recycle  solids during the  slaking
process.  Bench-scale  and preliminary
pilot plant tests have demonstrated that
the increased temperature provided by a
pressure hydrator  (up  to  150°C) will
significantly reduce the time requirement
of the  lime-silica reaction. Eventually the
process should be evaluated on a  large
pilot facility, such as AEERL's 3,400 m3/h
pilot  plant.  This  facility should  be
operated preferably in a continuous mode
where key  operational  parameters  (e.g.,
SO2 concentration,  recycle  ratios,  Ats,
SR) and their  impact on overall SO2
removal could be evaluated.

Conclusions
   Conclusions from the present work on
the mini-pilot plant include:

•   The mini-pilot  plant  is an  efficient
    and effective tool  for evaluating dry
    FGD processes, including both spray
    drying and dry sorbent injection.
•   In-duct injection of dry Ca(OH)2 into
    a humidified SOg-laden  flue  gas
    stream results in  significantly less
    S02 removal in the  duct/baghouse
    system that in a  lime spray drying
    system.
•   In-duct injection of dry NaHC03 at
    low temperature (49  to  93°C)  and
    high relative humidity (up to 60%)
    results in very high S02 removal, if
    the  injected sorbent  has a  particle
    size sufficiently small (less than 10
    jam)  to   allow  effective  gas
    entrainment of the particles and their
    deposition on the fabric filter bags. At
    low temperature (49°C), the  thermal
    decomposition  of   NaHC03  to
    NagCOs   may not   occur to  a
    significant extent, so that only 1 mole
    of NaHCOa is required to react with 1
    mole of S02 at a low stoichiometry.
•   The reactivity of  Ca(OH)2  with
    respect to dry  S02 removal  can be
    enhanced by  slurrying lime with
    silica,  such   as   flyash   or
    diatomaceous  earth, at  elevated
    temperatures   (85 to 95°C) for
    prolonged periods  (12 to 16 h).
•   Slurrying flyash with Ca(OH)2  at  a
    weight ratio of 3:1  and injecting the
    resultant dry sorbent into humidified
    flue  gas  (Ats  =   11  to  17°C)
    containing  1,500 ppm S02 resulted
    in an S02 removal of 50 to 80% over
    the SR range of 1  to 1.8, in the 0.8s
    gas retention  time  duct-baghouse
    system (Figure 3).
•   Without    product    recycle,
    approximately   50%  Ca(OH)2
    utilization occurred  in the tests cited
    above. With  product recycle  the
    utilization increased to at least 70 to
    80% at the same conditions.
•   Tests  using the  same  silica-
    enhanced sorbents injected into the
    2s gas  retention time duct/cyclone
    system  without recycle,  at similar
    test  conditions,  provided  S02
    removal efficiencies  of  only about
    30% of those above.
•   Introducing  recycle  of the  sorbents
    by mixing the cyclone catch solids
    into the prepared  slurry of silica-
    enhanced  Ca(OH)2  prior  to  duct
    injection avoided  the  need  for
    separate drying/dewatering of  the
    enhanced sorbent slurry. The overall
    Ca(OH)2 utilization also increased.
•   The recycle solids provided the silica
    for Ca(OH)2  enhancement in lieu of
    flyash during slurrying at elevated
    temperatures.
•   When  using  sorbent recycle,  the
    duct injection/cyclone system (2.0 s
    retention  time) resulted  in  S02
    removals of about 50% at an SR of
    1, and 50 to 90% at SRs in the range
    of 1 to 2 (Figure 4).
•   The  results  suggest that a  dry
    injection  process  using  silica-
    enhanced lime sorbents  may be an
    attractive retrofit option for controlling
    S02 emissions from an existing coal-
    fired  power plant equipped with an
    ESP.

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   Raw Flue Gas: 40 scfm
   0.6 Ib/h S02 ^—-—
   2.1 Ib/h Ash ———
Water
Discharge
3.3 Ib/h
  Make up
  Water
  9.0 Ib/h
                              Sorbent: 28.5 Ib/h
                                        Slurry Solids
                                        3.11b/h
                                                                Recycle Solids
                                                                14 Ib/h
                                                                 NOTE:    1 Ib = 0.454 kg
                                                                           1 scfm =  1.70 sm3/h
                                                                                                                  Cleaned Flue Gas
                                                                                                                  0.5 Ib/h SO2
Disposal
3.1 Ib/h
                    0.70 Ib/h
 Figure 2.  Continuous mini-pilot process using lime enhanced by recycle solids.

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IUV

90
SO
*. 70
|60
•58 50
30

20
10
n
I I I I I
S02 Inlet: 1500 ppm O
4f,= 11-17°C D,*x'
Flyash/Ca(OH)2 Ratio: O D
O 3:1 XX DO^^**
4fs= 11"C(200F)/ &»
X° A A Pure Hy*a^t
x ^»**^
~4f, = 17°C(3B°F) ^^ 	 l->"
.-•—•'"""""**"
— -"*"T i i i i


-
-
-
„.-—""**

—
_
i
                  0.5         r.O          J.5        2.0          2.5         3.0

                                        Stoichiometric Ratio
Figure 3.  Removal of S02 in duct injecfon/baghouse pilot plant facility. Ftyash enhanced lime
           used as dry sorbent.
IOU
90
80
70
geo
Iso
f
0 40
9)
«30
20
10
0
i i i ID
A xx
>'"
O XXX A
° X
n ° .4 -
' ° 4f, = 5-J7°C
O O J0~* v O Flyash/Ca(OH)2 = 3:1
fS Recycle/Cake = 2:1
9'' O Recycle/Ca(OH)2 = 4.5:1
j* . Recycle Cake = 2:1
A A Recycle/Ca(OH)2 = 4.5:1
O Recycle/ Slurry = 2:1
1 1 I 1
-
                      0.5             7.0              J.5             2.0             2.

                                      Stoichiometric Ratio

Figure 4.  Removal of SO2 in duct injection/cyclone pilot plant facility (2.0 s retention time);
           flyash-enhanced lime used as dry sorbent with recycle.

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  John  C.  S.  Chang and  Claus Jorgensen  are with Acurex Corp., Research
        Triangle  Park. NC 27709.
  Charles B. Sedman is the EPA Project Officer (see below).
  The complete report,  entitled "Evaluation of FGD Dry Injection Sorbents and
        Additives: Volume 2. Pilot Plant Evaluation  of High Reactivity Sorbents,"
        (Order No. PB  89-214 134/AS;  Cost: $21.95, subject to change) will be
        available only from:
           National Technical Information Service
           5285 Port Royal Road
           Springfield.  VA  22161
           Telephone:  703-487-4650
  The EPA Project Officer can be contacted at:
           Air and Energy  Engineering Research Laboratory
           U.S. Environmental Protection Agency
           Research Triangle Park, NC 27711
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
Official Business
Penalty for Private Use $300

EPA/600/S7-89/006b
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