xvEPA United States Environmental Protection Agency Municipal Environmental Research Laboratory Cincinnati OH 45268 Research and Development EPA-600/S2-81-214 Oct. 1981 Project Summary Modification of Spill Factors Affecting Air Pollution: Volume I. An Evaluation of Cooling as a Vapor Mitigation Procedure for Spilled Volatile Chemicals J. S. Greer, S. S. Gross, R. H. Hiltz, and M. J. McGoff Spilled chemicals that pose a hazard to the land and water ecosystem can also provide a significant vapor hazard. Although the vapors released by such chemicals may ultimately be dispersed in the environment with few long- term effects, they do pose a hazard to life and property downwind of the spill. Among the vapor amelioration tech- niques that have been considered is the use of a coolant to lower the temperature of a spill and reduce its equilibrium vapor pressure. This pro- gram was conducted as a feasibility study of that mechanism. Four potential coolants were exam- ined: water ice, dry ice, liquid carbon dioxide, and liquid nitrogen. Further evaluation based on laboratory studies and limited scaled-up tests established dry ice as the most versatile coolant choice. Water ice does not cool suf- ficiently. Liquid nitrogen and carbon dioxide require large quantities of material and produce a dense obscur- ing cloud that has some adverse impli- cations. Dry ice avoids these problems and is readily available at a reasonable cost, but some method is required for crushing and distributing the dry ice on the spill. A prototype unit was thus developed consisting of a crusher and a pneumatic conveyor to perform these functions. A pool of diethyl ether with 2.23 m2 (250 ft2) of surface was cooled to -60°C (-76°F) using 408 kg (900 Ib) of dry ice fed at a rate of 13.6 kg/min (30 Ib/min). A measurable reduction in downwind vapor concentration was realized. Pool temperature was still below -10°C (14°F) 2 hr after dry ice discharge was terminated. This program has established the feasibility of the mechanism, but additional work is necessary to estab- lish practicality, define materials to which cooling is applicable, and opti- mize the dispensing equipment. This Project Summary was devel- oped by EPA's Municipal Environmen- tal Research Laboratory, Cincinnati, OH, to announce key findings of the research project that is fully docu- mented in a separate report of the same title (see Project Report ordering information at back). Introduction Many of the chemicals that pose a hazard to the land and water ecosystem when spilled can also provide a signifi- cant vapor hazard. Although the vapors ------- released by such chemicals may ulti- mately disperse into the environment with little long term effect, they do pose an immediate hazard to life and property downwind of the spill. In addition, a hazard exists to those responding to the spill who must remain in the area for the duration of the incident. The vapor hazard from spilled chemi- cals takes two forms: the release of toxic fumes that pose a life hazard even at low concentrations (parts per million), and the release of flammable vapors where minimum dangerous concentrations are usually above 1%. Some chemicals may exhibit both hazards, but toxicity, with its lower allowable concentration, will be the controlling feature. The great difference in minimum hazard levels creates two distinct prob- lems. In the case of flammable vapors, small increments of reduction can be meaningful. For toxic materials, the ability to provide meaningful mitigation of the hazard may lie only with reduction of the equilibrium vapor pressure. A number of vapor amelioration tech- niques have received consideration. A review of the techniques conducted under U.S. Coast Guard sponsorship shows that most are ineffective. The techniques of mechanical covers, in- duced air movement, vapor scrubbing, and vapor phase reaction are in this category. The techniques of foam blan- keting and liquid phase modification are the only ones that in their present state of development have had any practical demonstration and can pass the criteria of cost, availability, deployment, and application. The degree of vapor control that can be achieved with these two techniques is beneficial where flam- mable vapors are the hazard. But where the vapor hazard is one of toxicity and hazardous vapor concentrations are in the parts per million range, such tech- niques are not adequate. Maintenance of vapor levels in the parts-per-million range appears to require a mechanism to reduce the equilibrium vapor pressure. One poten- tial mechanism of vapor control may achieve that end: the use of a coolant. Reducing the temperature of the spill reduces the equilibrium vapor pressure and the rate of vapor release per unit of time. This technique has been addressed in two programs, but no systematic inves- tigation has been conducted. Based on these studies, EPA inaugurated a de- tailed program to evaluate the potential of cooling and, if warranted, to conduct a simulated spill scenario to define feasibility. Discussion of Results This study establishes the basic feasibility of the cooling concept. A literature search and data evaluation delineated an extensive list of potential coolants. Practical considerations of cost, availability, safety, and field handling reduced the candidate list to four materials: wet ice (solid water), dry ice (solid CO2), liquid C02, and liquid nitrogen. All four materials are readily available from many sources on short notice and at a reasonable cost. The liquefied gases, N2 and C02, can achieve signifi- cant reductions in the temperature of the spill, but they are attended by certain disadvantages. These gases require continuous application, and the effect does not persist if application is discontinued. The boiling of the liquid exaggerates the vapor release from the spilled material, negating some of the benefits of cooling. Both materials produce a dense obscuring cloud above the spill surface. This cloud provides a nonflammable atmosphere, but it is also nonbreathable. Liquid CO2 can be released to form solid C02, identified as COa snow. But conversion is only 15 percent with current technology, an obscuring cloud is still generated. Wet ice has certain advantages, but its capability is limited to 0°C (32°F). Ice can react with some materials and will cause a volume increase because of its nonvolatility. Dry ice, crushed and applied as a particulate, initially showed the best potential for effective, persistent cooling with small material losses and minimal cloud formation. Further evaluation supported by laboratory studies and limited scaled-up tests were able to establish dry ice as the best coolant choice. The bases for this selection are detailed in Table 1. The main comparison was the difference of the temperatures achieved and the rate of rise after coolant application was stopped. A comparison using ethyl ether is shown in Figure 1. Results The laboratory results were encour- aging, but they were not sophisticated enough to establish the feasibility for field use. Field application necessitated a mechanism to convert the standard form of dry ice blocks (10x10x1 in.; 25 x 25 x 2.5 cm) to a particulate form and a means for dispensing the particulates to the spill surface. A review of commer- cial equipment revealed several types ol applicable equipment. After a limited testing program, a commercial shredder/ crusher was selected. The shredder operation was modified in terms of the speed of rotation and the configuration of the tines to achieve a reasonable yield of particles within an acceptable size range. The distribution covered fine particulates to coarse material of 0.635 to 1.27 cm (1 /4 to 1 /2 in.). Because of the problem of sublimation, a true size range could not be measured. Efficiency in terms of material out versus material in was in the range of 75%. Several concepts were evaluated for dispensing the crushed dry ice. A snow blower was originally selected, but its operation reduced the effective discharge to 65%. The combination of snow blower/crusher was a poor selection in real time. The discharge distance was not sufficient to allow operation from a restricted location, and the machine was difficult to manipulate around the spill. A change was made to a pneumatic conveyor, which was made up of an auger feeding the particulate into an air stream with forced discharge through a hose. * The combination unit was mounted on a wheeled frame to provide mobility, but the hose discharge allowed an extended discharge pattern from a single location. Some additional mate- rial losses were encountered, reducing efficiency to about 50%. Field tests were conducted using diethyl ether as a spill simulant: 757 L (200 gal) was spilled into a 7.62- by 6.1 - m (25- by 20-ft) impoundment. Dry ice was charged at a rate of 13.61 kg/min (30 Ib/min) for 30 min with an effective application of 6.80 kg/min (15 Ib/min). The spill temperature was reduced in that time to an averge of -60°C (-76°F), which resulted in a decrease of the equilibrium vapor pressure from 440 to 4.0 mm of Hg. An absolute measure of vapor reduction could not be obtained because of wind effects. The available data show the effective reduction in the vicinity of the spill to be at least 75% of the free spill value. Typical values show a free spill vapor concentration of 10,000 ppm, which was reduced to 180 ppm by the dry ice application. Conclusions The results of this program show that dry ice can significantly reduce th ------- fable 1. Cryogen Comparisons Cryogen Advantages Disadvantages Liquefied Nitrogen Liquefied Carbon Dioxide Solid Carbon Dioxide Ice 1. Cheaper than COz on a per-pound basis 2. Extremely low temperatures possible 1. No storage losses 2. Reasonable temperature reduction of spill 1. Better cost advantage than liquid COz or liquefied Nz 2. Less application loss than with LNZ or liquid COz 3. Rapid cooling of spill 4. No problems with COz cloud 5. Can be projected over distances 6. Readily available 7. Safer than liquefied /V2 or liquefied COz to handle 1. Safest to use 2. Most readily available 3. Can be projected 1. Vapor losses occur on storage 2. Nz cloud significantly reduces visibility and oxygen levels in vicinity of spill 3. Larger quantities needed to cool spill than with solid COz 4. Not as cost effective as solid COz 5. Hazardous liquid may be entrained by Nz vapors 1. Higher liquid COz losses occur upon application to the spill 2. COz cloud significantly reduces visibility and oxygen levels in vicinity of spill 3. More expensive than solid COz based on the amount actually applied to the spill 1. Storage losses occur 2. Grinding necessary before application 1. Temperature of the spill is not reduced sufficiently 2. Increases the liquid volume of the spill when the ice melts Liquefied Nitrogen 1. Cheaper than COz on per pound basis 2. Extremely low temperatures possible Liquefied Carbon Dioxide Solid Carbon Dioxide Ice 1. No storage losses 2. Reasonable temperature reduction of spill 1. Better cost advantage than liquid COz or liquefied Nz 2. Less application losses than with LNz or liquid COz 3. Rapid cooling of spill 4. No problems with COz cloud 5. Can be projected over distances 6. Readily available 7. Safer than liquefied NZ or liquefied C02 to handle 1, Safest to use 2. Most readily available 3. Can be projected 1. Vapor losses on storage 2. Nz cloud significantly reduces visibility and oxygen levels in vicinity of spill 3. Larger quantities needed to cool spill than solid COz 4. Not as cost effective as solid COz 5. Possible entrainment of hazardous liquid by Nz vapors 1. Higher liquid COz losses upon application to the spill 2. COz cloud significantly reduces visibility and oxygen levels in vicinity of spill 3. More expensive than solid COz on the basis of amount actually applied to the spill 1. Storage losses 2. Grinding necessary before application 1. Temperature of the spill is not reduced sufficiently 2. Increases the liquid volume of spill when the ice melts ------- 20 -20 -40 2 Cb | -60 -80 -100 -120 9.3 m2 (100 ft2) pond 208 I (55 gal) diethyl ether -40 -20 20 40 60 Time, min. 80 WO 120 Figure 1. Subscale field test results with ethyl ether—temperature versus time (9.3 m2(100-ft2) pond, 208 L (55 gal) diethyl ether). temperature of a spilled liquid with a concomitant reduction in the vapor release rate. Crushing the dry ice to an acceptable particulate level and dis- tributing it over the spill surface can be achieved by state-of-the-art techniques. The equipment evolved in this pro- gram required further optimization. Further study must be done on opera- tion, configuration, and materials of construction. The tests that have been conducted are not sufficiently extensive to show clearly a practical, efficient operation in a real-time spill scenario. But they do support continued investi- gation and evaluation of the cooling concept. The cooling concept is primarily suited for use with materials that pose a toxic vapor hazard rather than a flammable or explosive vapor hazard. In most cases, aqueous foams provide effective mitiga- tion for such materials. Foams are a well developed technol- ogy in common use by emergency organizations, but they cannot provide the degree of vapor control necessary where toxic levels are in the parts per million range. This study provides a basic guideline for further evaluation of coolants. The full report was submitted in partial fulfillment of Contract No. 68- 03-2648, Task 9A. by MSA Research Corporation under subcontract to Rock- well International under sponsorship of the U.S. Environmental Protection Agency. ------- J. S. Greer. S. S. Gross, P. H. Hiltz, and M. J. McGoff are with MSA Research Corporation, Evans City, PA 16033. John E. Brugger is the EPA Project Officer (see below). The complete report, entitled "Modification of Spill Factors Affecting Air Pollution: Volume I. An Evaluation of Cooling as a Vapor Mitigation Procedure for Spilled Volatile Chemicals," (Order No. PB 82-108 382; Cost: $9.50, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Oil and Hazardous Materials Spills Branch Municipal Environmental Research Laboratory—Cincinnati U.S. Environmental Protection Agency Edison, NJ 08837 ------- United States Environmental Protection Agency Center for Environmental Research Information Cincinnati OH 45268 Postage and Fees Paid Environmental Protection Agency EPA 335 Official Business Penalty for Private Use $300 RETURN POSTAGE GUARANTEED PS 0000329 U S ENVIR PPOTKC1IUN AGENCX REGION 5 LIBRAK* 230 S UEAR80RN STREET CHICAGO IL 606U4 *U.S. GOVERNMENT PRIMING OFFICE : 1981--559-092/ ------- |