United States
                   Environmental Protection
                   Agency
 Hazardous Waste Engineering
 Research Laboratory
 Cincinnati OH 45268
                   Research and Development
 EPA/600/S2-86/098  Jan. 1987
\>EPA         Project Summary
                   Preliminary Assessment  of Air
                   Emissions  from  Aerated
                   Waste  Treatment  Systems  at
                   TSDFs

                   C. C. Allen, D. A. Green, J. B. White, and J. B. Coburn
                    Aerated wastewater treatmet unit
                   operations are used for the removal of
                   organic compounds from hazardous
                   waste and other industrial wastewater
                   streams. Some operations use aeration
                   to supply oxygen for aerobic decompo-
                   sition of organics; in other operations,
                   incidental air/water contact occurs to
                   varying degrees. Methods for estimat-
                   ing emissions resulting from air strip-
                   ping of volatile organic compounds
                   that may accompany aerated treatment
                   are applied to full scale and pilot plant
                   wastewater treatment plants.

                    Treatment plant examples are inves-
                   tigated for aerated industrial waste
                   treatment systems employing trickling
                   filters, activated sludge and aerated la-
                   goons. The size and configuration of full
                   size treatment plants are highly vari-
                   able, corresponding to the highly vari-
                   able volume and strength of industrial
                   wastewater. Typical size and residence
                   time specifications for unit operations
                   within these plants are discussed.

                    The recommended mathematical
                   models are used to generate predic-
                   tions of the fate of volatile organic com-
                   pounds in wastewater treatment sys-
                   tems. Where full scale plant data are
                   available, predictions generally agree
                   with measurements (within the limits
                   of accuracy which result from varia-
                   tions in sampling and chemical analy-
                   sis). For this reason, the mathematical
                   models can be used to estimate emis-
                   sions for those systems where no field
                   data are available.
  This Project Summary was devel-
 oped for the EPA's Hazardous Waste
 Engineering Research  Laboratory,
 Cincinnati, OH, to announce key find-
 ings of the research project that is fully
 documented in a separate report of the
 same title (see Project Report ordering
 information at back).


 Introduction
  The EPA Office of Air Quality Planning
 and Standards (OAQPS) is developing
 regulations under the 1976 Resource
 Conservation and Recovery Act (RCRA)
 to control air emissions from hazardous
 treatment, storage, and disposal facili-
 ties (TSDFs). The purpose of the air
 emissions regulations is to protect
 human  health and  the .environment
 from emissions of volatile organic com-
 pounds (VOCs), particulates, and aero-
 sols.
  The sources of TSDF emissions in-
 clude storage tanks, treatment proc-
 esses, surface impoundments, lagoons,
 landfills, land treatment, and drum stor-
 age and handling facilities. Those proc-
 esses involving the use of air (biological
 treatment and cooling) or subject to the
 introduction of air (stirred equalization
 and neutralization) may emit VOCs as a
 consequence of air stripping.
  To further understand and better esti-
 mate the sources and extent of  VOC
 emissions from TSDFs, typical aerated
 treatment facilities  are investigated.
 Various mathematical models are
presented to predict the mechanism
and extent of VOC emissions during the

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different process conditions encoun-
tered. The models include a methodol-
ogy for estimating the  relative impor-
tance of competing removal pathways
(i.e., adsorption and  biological oxida-
tion). The study is limited to those bio-
logical processes or physical chemical
processes with potential to vent VOC to
the air.
  The basic problem in evaluating air
emissions from aerated waste treat-
ment processes is determining  the im-
portance of competing mechanisms. In
an activated sludge biological treatment
process, for example, the major mecha-
nisms for removal of dissolved contam-
inants from the aqueous waste are bio-
logical oxidation, adsorption on
biomass, and mass transfer into the air.
In a  rough analysis of "removal effi-
ciency" concentrations  of the contami-
nants in the aqueous influent and efflu-
ent are measured and the fraction of the
contaminant which disappears in the
process is  reported as an  efficiency.
This procedure gives no information
about the relative importance of com-
peting removal mechanisms.
  Where one or more  of the  removal
mechanisms is destructive of the con-
taminants (chemical or biological oxida-
tion) and  others  non-destructive (air
stripping or aerosol dispersal), measur-
ing the relative importance of the com-
peting mechanisms becomes compli-
cated. In such  a case, the contaminant
removed by the non-destructive mecha-
nism  must be recovered and the bal-
ance assumed to have been destroyed.
Errors in chemical analyses, and partic-
ularly sampling errors, have a great im-
pact on calculations of the fraction of
the destroyed contaminant.
  Alternatively, data may be obtained
under controlled laboratory conditions
and adapted to provide  reasonable esti-
mates of  emissions expected under
field conditions. One approach is to con-
duct experiments in covered vessels to
permit accurate sampling of vent gases
and accurate metering of vent gas flow
rates. Another approach involves  in-
hibiting the destructive removal mecha-
nisms by taking steps to chemically
sterilize the system or to substitute an
inert gas such as nitrogen for air. In this
latter case, the mass transfer to the gas
phase continues to occur and all of the
destructive mechanisms are eliminated.
Influent and effluent aqueous phase
sampling are used to determine the ex-
tent of removal resulting from stripping.
Vapor phase sampling of such a labora-
tory system should close the mass bal-
ance for the system. The extent to which
under-recovery or over-recovery of con-
taminants is found can be used to evalu-
ate the adequacy of laboratory vapor
phase sampling techniques.
  One approach to the air  stripping
problem is to measure the total disap-
pearance in the field and then apply
mathematical  models obtained from
laboratory data to simultaneously esti-
mate the rate of stripping and  biological
oxidation. When these models account
for significantly more or significantly
less contaminant removal than the ob-
served total removal, several steps may
be taken. The simplest approach  is to
assume that the mass transfer model is
more accurate than the biological  oxi-
dation model and account for  biological
oxidation (and other destructive  re-
moval mechanisms) by difference. Be-
cause they are less affected by changes
in operating conditions and influent
wastewater composition, the mass
transfer models are in fact more accu-
rate predictors than are  the  biological
oxidation models. In some cases, how-
ever, air sampling must be conducted to
verify the prediction of stripping mod-
els. The interpretation of such data ob-
tained under field conditions is, how-
ever, subject to considerable  error.
  The objectives of this study are to
present and evaluate the various kinetic
and predictive fate models that are ap-
plicable to aerated wastewater treat-
ment systems. Four different waste
treatment systems will be  considered:
(1) trickling filters, (2) activated sludge,
(3) aerated lagoons, and (4) spray
ponds. When possible, model  predic-
tions will be compared with experimen-
tal data.
  This study investigated mathematical
models and correlations available in the
literature for mass  transfer in systems
similar to wastewater treatment units.
Classical engineering approaches to
strippers and absorbers, packed bed de-
sign, and  stream and lake reaeration
were considered and adapted as neces-
sary to wastewater treatment systems.

Procedure
  Pretreatment was modeled as a plug
flow system with the gas phase mass
transfer coefficient  calculated from a
"wind speed" correlation and the liquid
phase mass transfer coefficient calcu-
lated using a stream reaeration correla-
tion. Primary and secondary clarifiers
were  modeled  as  plug  flow systems
using the same methods as  described
above to calculate mass transfer coeffi-
cients. Surface  aeration systems (e.g.
some activated sludge units) were mod-
eled using a correlation with applied
aerator horsepower.  Biological  oxida-
tion was incorporated using a pseudo-
first order rate constant to be calculated
from the best available zero-order data
and an assumption as to steady state
composition.
  Diffused aeration systems (e.g. some
activated  sludge systems with sub-
merged aerators) were modeled with
stripping based  on the attainment of
equilibrium during the time of bubble
rise, which is combined with surface dif-
fusion calculated as for clarifiers. Bio-
logical decay is treated in the same
manner regardless of the means of
aeration. Suggested procedures for cal-
culating mass transfer coefficients ap-
propriate for equalization  ponds, dis-
solved air flotation units, spray ponds
and cooling towers are also given.
  As a step in verifying the accuracy of
the suggested  mathematical models,
data from an extensive sampling pro-
gram at a well  characterized (with re-
spect to  residence time,  dimensions
and  influent and effluent concentra-
tions) wastewater treatment  system
were  used to test the models. In addi-
tion,  pilot  scale data from well con-
trolled experiments and some less  ex-
tensive industrial wastewater treatment
system data from EPA  plant surveys
were  also  used.
  A list of input specifications which de-
scribe the system to be  modeled is
given in Table 1; values given are from
a wastewater treatment system at a
Union Carbide chemical manufacturing
plant. For cases where units of a particu-
lar type are not used in a particular sys-
tem  (e.g. dissolved air flotation in  the
example given), a specification of zero
for area, number, or  air flow eliminate
the inappropriate part of the model.

Results and Discussion
  The results of the calculations on  the
sample plant specification  are given in
Table 2. The rate of loss of volatiles
from the plant as predicted  by the math-
ematical  models agreed well with
measured results, with the  exception o1
the UNOX biological treatment unit
The  rate of removal  in the UNOX sys
tern was overpredicted by the  model
particularly  in the case  of tetralin. Al
though the loss in the aeration basir
was overpredicted by the model foi
tetralin and naphthalene (89% was the
observed loss in both cases), the abso
lute errors were still only 5-10%.

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Table 1.   Model Input Data for Union Carbide Plant (Alsop, et al., 1984)*

Water Temperature (Deg C)                                               25
Wind Velocity (cm/S)                                                    200
Concentration of Benzene (Mole Fract)                                        .001
Concentration of Naphthalene (Mole Fract)                                     .005
'Concentration of Ethylbenzene (Mole Fract)                                    .001
Concentration of Methylcellosolve (Mole Fract)                                 .001
Concentration of Tetralin (Mole Fract)                                         .0002
Biorate of Benzene (Hours)                                               400
Biorate of Naphthalene (Hours)                                           400
Biorate of Ethylbenzene (Hours)                                           400
Biorate of Methylcellosolve (Hours)                                        800
Biorate of Tetralin (Hours)                                                200
Waste Flow Rate (M3/Sec)                                                   .07
Area of Pretreatment Basin (M2)                                           50
Depth of Pretreatment Basin (M)                                            3
Diameter of Clarifier (M)                                                  19.4
Depth of Clarifier (M)                                                      2.4
Number of Clarifiers                                                      1
Length of Aeration Basin (M)                                             170
Width of Aeration Basin (M)                                              170
Depth of Aeration Basin (M)                                                3.6
Area of Agitators (Each) (M2)                                              96
Number of Agitators                                                     30
Power of Agitation (Each) (HP)                                             75
Impeller Diameter (cm)                                                   30
Impeller Rotation (rpm)                                                 2000
Number of Secondary Clarifiers                                             1
Diameter of Secondary Clarifiers (M)                                        37
Depth of Secondary Clarifiers (M)                                            3
Area of Equalization Basin (M2)                                          5185
Depth of Equalization Basin (M2)                                            3
Air Flow in DAF (Pretreat) (SM3/S)                                           0
Flow of Submerged Air (M3/Sec)                                             .4
Power of Sub-Agitation, Each (HP)                                          50
Length of Sub. Aeration Basin (M)                                          33.5
Width of Sub. Aeration Basin (M)                                            8.4
Depth of Sub. Aeration Basin (M)                                            8.5
Area of Sub. Agitators (Each) (M2)                                          70.1
Number of Sub. Units in Series                                             3
Impeller Rotation (rpm)                                                   70
Impeller Diameter (cm)                                                  243
Weir Height (cm)                                                        30
Thickness of Weir Flow (cm)                                                1
Enter {1} for Covered Subm. Agit.                                            1

*Fate of Specific Organics in an Industrial Biological Wastewater Treatment Plant, EPA Draft
 Report (June 29, 1984).
  In an EPA pilot investigation, a num-
 ber of VOCs were processed in a clari-
 fier before entering an aerated biologi-
 cal oxidation  unit. Enough data were
 provided to specify the input parame-
 ters of the model. Although the treat-
 ment plant was not directly exposed to
 the atmosphere, air was circulated and
 the mass transfer is considered  to  be
 liquid phase controlled. For both the
 clarifier and the aerator, the model pre-
 dicted VOC losses in close agreement
 with the pilot data. The model predicted
 that most of the VOCs were lost to the
 circulating air.

  The fractional loss of VOCs to the air
was estimated for the du Pont Belle, WV
plant. The model predictions for
methanol, acetone, and chloroform
were within a factor of 5 for the primary
process, but did not agree with the esti-
mated losses of butanol. The secondary
treatment  estimations did  not agree
with model predictions. Not enough in-
formation was provided to  determine
the source of the  difference. At the
Union Carbide Sisterville plant, the pre-
dicted fractional loss was within a factor
of 5 of the estimated values. Only pri-
mary  treatment was assumed; except
for the flow rate, no information  was
provided about the  source characteris-
tics.
Conclusions and Recommenda-
tions
  The available theoretical  and semi-
empirical methods for predicting the
rates of mass transfer of volatile organic
compounds from dilute solution into air
can be used to accurately predict emis-
sions from aerated wastewater treat-
ment processes in the absence of com-
peting removal mechanisms. Where
liquid phase  concentration  data  and
system operating conditions are well-
characterized,  VOC emissions from  aer-
ated  lagoons, activated sludge proc-
esses, trikckling filters,  and Clarifiers
associated with wastewater treatment
systems  may  be estimated  within the
accuracy of sampling and  chemical
analysis results.
  The presence of competing removal
mechanisms,  of which biooxidation  is
the most  important, reduces the accu-
racy of emissions predictions based on
plant influent concentration data. If bulk
wastewater  concentrations are known
for individual treatment units, then  rea-
sonably  accurate predictions may be
made. However, when only the concen-
tration of the influent to the entire plant
is known, accurate rate data  for biooxi-
dation become more  important,  and
their absence has a greater influence on
the accuracy of emissions estimation.
  Biooxidation rate data  is available  in
the literature for various organic com-
pounds which  may be present in indus-
trial wastewater. The data are highly de-
pendent on the conditions under which
they were obtained and  are not easily
adapted  to  real systems which may
have different initial  concentrations,
biomass loadings, nutrient and inhibitor
concentrations, etc. A table of bioxida-
tion  rate  data  obtained from the litera-
ture is included in the final report to pro-
vide a starting point for calculations.
  Industrial  waste  treatment systems
vary widely in design reflecting the wide
variation  in the waste streams to be
treated. The recommended predictive
mathematical  models are adapatable  to
widely varying volumetric flow rates.
Residence time, which  in actual system
designs accounts for the concentration
and  increases  with  the difficulty of re-
moval of organic compounds and sus-
pended solids, must be specified from
actual system designs  or  estimated
(less accurately) from  removal rate
data.  Model plant designs are given  in
the report which fit within  the wide
range of suitable  designs.  The best
mathematical  models, as determined

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Table 2. A Comparison of the Experimental Loss of Volatiles from the Union Carbide Plant by this Study, were compared with ex-
Field Test to the Predicted Loss from Mathematical Models perimental measurements of full-scale
Fractional Loss Fractional Loss to Air and P»ot-*cale wastewater treatment
UniWolatile (experimental) (predicted) systems. Sample calculations are in-
/Nlnrl
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       C. C. Allen, et a/., are with Research Triangle Institute, Research Triangle Park,
        NC 27709.
       Ronald J. Turner is the EPA Project Officer, see below.
       The complete report, entitled "Preliminary Assessment of Air Emissions from
        Aerated Waste Treatment Systems at Hazardous Waste  Treatment Storage
        and Disposal Facilities," (Order No. PB87-113 783/AS; Cost: $18.95, subject
        to change) will be available only from:
              National Technical Information Service
              5285 Port Royal Road
              Springfield,  VA 22161
              Telephone: 703-487-4650
       The EPA Project Officer can be contacted at:
              Hazardous Waste Engineering Research Laboratory
              U.S. Environmental Protection Agency
              Cincinnati, OH 45268
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
Official Business
Penalty for Private Use $300

EPA/600/S2-86/098
         0000329   PS

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