United States
                     Environmental  Protection
                     Agency
 Water Engineering
 Research Laboratory
 Cincinnati OH 45268
                     Research and Development
 EPA/600/S2-86/099  Feb. 1987
4>EPA          Project  Summary
                     Limestone  Bed  Contactors  for
                     Control   of  Corrosion  at
                     Small   Water   Utilities
                     Raymond D. Letterman, Charles T. Driscoll, Jr., Marwan Haddad,
                     and H. Alan Hsu
                       A study was conducted to investigate
                     the use of limestone contactors for miti-
                     gating corrosion in small water  supply
                     systems that use dilute acidic (corrosive)
                     water. As water is transported through a
                     packed bed of crushed limestone, calcium
                     carbonate dissolves and the pH, calcium
                     concentration, and alkalinity increase.
                       A mathematical model was derived for
                     use in contactor design.  The  model is
                     based on the interfacial  transport of
                     calcium ion and relates the depth of lime-
                     stone required in the contactor  to the
                     desired effluent water chemistry, influent
                     water chemistry, limestone particle size
                     and shape, limestone bed porosity, water
                     temperature, and superficial velocity. The
                     model was calibrated and tested using
                     laboratory column experiments.
                       In a field contactor monitored for 2.5
                     years, the water quality following treat-
                     ment (except for the initial few months)
                     was  essentially constant. No gradual,
                     long-term degradation in performance was
                     noted. After several months of operation,
                     however, the rate of CaCO3 dissolution
                     was not as high as that observed in the
                     laboratory using fresh limestone. The rate
                     of dissolution was possibly reduced by an
                     alumino-silicate  residue  that  remained
                     after the CaCO3 was dissolved from the
                     limestone matrix. A microbiological film
                     may also have been a limiting factor.
                       Field studies indicated that limestone
                     contactors can effectively reduce the
                     tendency of  water to take up  corrosion
                     byproducts (copper, lead, and zinc) from
                     surfaces in  piping systems. First-flush
                     samples of cottage tap water  receiving
                     untreated spring water showed copper and
                     lead concentrations that were significantly
higher than those in contactor-treated cot-
tage tap water (1.9 ± 0.31 mg Cu/L and
0.046 ± 0.004 mg Pb/L as opposed to
0.030 ± 0.037 mg Cu/L and 0.0084 ±
0.0084 mg Pb/L, respectively).
  This Project Summary was developed
by EPA's Water Engineering Research Lab-
oratory, Cincinnati, OH, to announce key
findings of the research project that is futty
documented in a separate report of the
same title (see Project Report ordering in-
formation at back).

Introduction
  In many areas of the United  States,
homeowners and small public and private
water supply systems use water that is
potentially corrosive to metallic materials
used in the distribution system. Corrosion
is a concern to the owners and users of
small water supply systems because of
the potential health problems associated
with the ingestion of corrosion byprod-
ucts, the  degradation of the aesthetic
quality of the water,  and the significant
economic consequences of piping  system
deterioration.
  Corrosion  and contamination  of the
water by corrosion byproducts may be
caused by the use of dilute (low-ionic-
strength) acidic waters that generally have
low pH, alkalinity,  and concentrations of
dissolved  solids.  Dilute acidic ground-
waters and surface waters are found in  a
number of regions of the country, particu-
larly in regions underlain by siliceous bed-
rock. The waters naturally have low buffer-
ing capacity and are corrosive. They are
also prone to acidification by atmospheric
deposition of strong acids (acid precipita-
tion) or other factors such as changes in

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 land use. In some areas (for example, the
 Adirondack region of New York State); it is
 possible that the corrosivity of water has
 been increased by acid precipitation.  In
 any event, until recent concern developed
 about acid precipitation and the resulting
 deterioration of water quality, residents
 and visitors tolerated or ignored the prob-
 lems caused by corrosive water. Now this
 indifference has changed to a significant
 concern, and many home and resort own-
 ers as well as those responsible for village
 water supplies have begun to adopt tech-
 niques designed to mitigate drinking water
 corrosivity.
   Low cost is a very important criterion in
 establishing the feasibility of any corrosion
 mitigation technique for a small water  sup-
 ply system. Also, the  maintenance re-
 quired should be minimal, and the tech-
 nique should present a  low potential for
 public health  hazard resulting from im-
 proper  construction,  installation, or
 maintenance.  Limestone contactors are
 water treatment devices that generally
 meet these requirements.
   In a limestone contactor, water is closed
 to the atmosphere and flows through and
 dissolves a packed bed of crushed lime-
 stone. The chemistry of the water  is
 altered as the limestone dissolves. Sources
 of  CaCO3 other  than high-calcium
 limestone (e.g., seashells) are sometimes
 used. Limestone contactors are simple but
 effective devices with low capital cost and
 minimum maintenance requirements. They
 have been used to neutralize acid mine
 drainage,  acidic  industrial  wastes,  and
 dilute acidic surface waters.
  The overall objective of this project was
to investigate the use of limestone contac-
tors for mitigating corrosion in small water
supply systems  that use  dilute acidic
water. The research plan  included  the
development and testing of  a rational
method for contactor design and the eval-
uation of the field operation of a contactor
with respect to corrosion control and oper-
ation  and  maintenance  problems.   The
study had  the  following   specific
objectives:

  0)~to derive and test  a mathematical
      model for limestone contactor de-
      sign, using laboratory, column-type
      reactors,
  (2) to develop design objectives by ex-
      perimentally determining the rela-
     tionship between contactor-treated
     water quality and metal release from
     pipes, and
  (3) to evaluate the  practical application
     of the design equations and objec-
     tives by monitoring the field per-
      formance of full-scale contactors
      and to determine the feasibility of
      long-term operation and the type
      and  frequency of  maintenance
      required.
Results
  As dilute acidic water is transported
through a packed bed of crushed lime-
stone, calcium carbonate in the limestone
dissolves, the pH, calcium ion concentra-
tion,  and  alkalinity increase, and  these
characteristics generally tend to mitigate
the dissolution of corrosion byproducts
from surfaces in piping systems.
  A laboratory study was conducted using
packed-column contactors (Figures 1 and
2).  Results were used to develop and test
a numerical model for contactor design.
  The design equations are based on the
interfacial transport of calcium ion. Limited
axial dispersion was also considered. Ac-
cording to the model, the  depth of lime-
stone, L, required to achieve a given level
of treatment is given by
   L =
        1n[(Ceq - CbL)/(Ceq  - 0^)]
          Us
                 - 2 d
where a is the interfacial area of limestone
per unit volume of interstitial water, t is the
bed porosity, Us is the superficial velocity,
d is the effective diameter of the limestone
particles, and K0 is the overall CaC03
dissolution  rate constant. Cbo is the in-
Figure  1.    Laboratory columns with water supply and flow control system. Insert is a drawing
            of a typical through-the-watl sampling tube.

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fluent calcium concentration. The quantity      The results of this study indicate that
a is calculated using d and the particle    K0 can be estimated using a correlation of
sphericity.                                dimensionless mass transfer parameters.
                                         Plan
                                      Limestone
                                      Contactor
                                      Chamber
                                                       Limestone
                                                       Contactor
                                                        Chamber
Figure 2.    Diagram showing the installation of the baffled-box contactor in the spring at
            Covewood.
For low values of a modified Reynolds
number (1< MRe < 30)
  K0 =  5.70 
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bon dioxide can have a significant effect
on the pH of the solution and hence on the
tendency of the water to dissolve corro-
sion byproducts. When the influent D1C is
high  (e.g.,  greater  than   10  mg  C/U.
equilibration of the effluent with the at-
mosphere causes the pH to  increase.
When the influent DIG concentration is
less than several mg  C/L, the pH tends to
decrease.
   Results of the study suggest that dilute
acidic waters  facilitate the  release of
elevated concentrations of trace metals
from metal piping systems. Passivation
films  of  most  significance  include
Cu2
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