United States Environmental Protection Agency Hazardous Waste Engineering Research Laboratory Cincinnati OH 45268 * Research and Development EPA/600/S2-87/071 Nov. 1987 Project Summary Sensitivity Analysis for Application of the Inhalation Exposure Methodology (IEM) to Studies of Hazardous Waste Management Facilities F. R. O'Donnell and C. C. Gilmore This study investigated the uncer- tainties associated with using the Inhalation Exposure Methodology (IEM) to determine human exposures to hazardous waste management facility air emissions. The Inhalation Exposure Methodology is an integrated system of computer programs that simulates the atmospheric transport of and the result- ing human exposures to pollutants released from one or more sources at an industrial complex. The full report illustrates the sensitivity of IEM pre- dictions to (1) variations of important user-supplied source, meteorological, and pollutant parameter values and (2) use of three IEM source modeling options to represent emission sources found at hazardous waste management facilities. This Project Summary was developed by EPA's Hazardous Waste Engineering Research Laboratory, Cincinnati, OH, to announce key findings of the research project that Is fully documented In a separate report of the same title (see Project Report ordering Information at back). Introduction The Inhalation Exposure Methodology (IEM) is an integrated system of computer programs that simulates the atmospheric transport of and the resulting human exposures to pollutants released from one or more sources at an industrial complex. This study was undertaken to determine the sensitivity of IEM predic- tions of pollutant concentrations and population exposures to (1) variations of selected, user-supplied source, meteoro- logical, climatological, and pollutant pa- rameter values and (2) use of the three available source modeling options to represent emission sources found at hazardous waste management facilities (HWMFs). These sources include incin- erators and associated structures, storage and treatment tanks, drum stacks, process buildings, surface impoundments, land- fills, waste piles, and land treatment areas. Several sources may be found at one HWMF. The study only determined the sen- sitivity of IEM predictions to the above factors. It did not validate the model by comparing IEM predictions with actual field data. Modeling the sources found at an HWMF could present problems because they may be located close together or near buildings and structures that could influence pollutant dispersion, and they may have ill-defined pollutant release rates. In some cases, source-specific pol- lutant release rates may be unavailable, thus forcing the modeler to represent several sources at a single source. The IEM uses a Garissian-plume atmospheric dispersion model, the Inhala- tion Source Complex Long Term Model (ISCLTM), to calculate annual-average, sector-averaged, centerline, ground-level, air concentrations of released pollutants at user-selected receptor points. It uses these concentrations to calculate average ------- concentrations over each sector segment of a user-specified polar grid. Finally, it multiplies the sector-segment-averaged concentrations and their corresponding sector-segment populations to give esti- mates of human exposures to the released pollutants. Although applicable to a variety of problems, the IEM was devel- oped as a tool for estimating pollutant concentrations and associated human exposures in the vicinity of hazardous waste management facilities (HWMFs). Approach Emission sources found at HWMFs have relatively low pollutant release heights, may be located near structures that in- fluence pollutant dispersion, and, except for incinerator stacks, may have es- sentially no associated plume rise. Pre- vious studies have examined the sen- sitivity of ISCLTM predictions to typical hazardous waste incinerator stack pa- rameters (e.g. stack height, gas tempera- tures). Based on these studies and the fact that all stack parameters except the physical stack height affect only plume rise, these parameters were not studied in detail. The remaining, important, user- supplied input parameters include mete- orological parameters (wind speed, wind direction, and stability class), source parameters (release height, source area, and adjacent building cross sections), pollutant parameters (decay coefficient, settling velocity, and reflection coeffici- ent), and the array of receptor grid points chosen. The study report documents the effects of varying these parameters on ambient pollution concentrations and population exposures. In addition, the effects of using three different source representation options (point, area or volume representa- tions) on pollution concentrations are investigated. Several typical HWMF sources were selected for detailed study; a stack with essentially no plume rise, a 14.1 -m square (200 m2) area, an 80.6-m square (6500 m2) area, a 316.2-m square (100,000 m2) area, and a 2236.1 -m square (5,000,000 m2) area. Since the ISCLTM algorithm will not accept zero values for a stack diameter or gas exit velocity, our stack source was assumed to have a diameter of 1.0 m and a gas exit velocity of 1 x 10 5 m/s, the ISCLTM default value. Source (release) heights of 0,5,10,15, and 20 m were considered for these sources. Limited evaluations were made of the effects of representing a 200-m2 process building with a release hefght of either 5 or 10 m by one stack source, by two area sources, and by two volume sources. Similar evaluations were made for a 200-m2 tank farm containing four tanks with release heights of either 3 or 6 m that were represented by four point sources, with and without building wake effects; by ^ne area source; by four area sources; by one volume source; and by four volume sources. In order to investigate the sensitivity of different IEM input parameters and pro- gramming options, the following computer outputs were generated: 1. Plots of the exceptor grid-point con- centrations directly downwind of the source. (These are defined as pri- mary grid-point concentrations). 2. Value and location of the maximum primary grid-point concentration. 3. The exposure to all individuals living directly downwind of the source. (The area directly downwind of the source is defined as the "primary sector," which lies within ± 11.25° of the wind direction.) 4. Plots of the sum of the pollution concentrations for all grid points at a given distance from the source, which indicates total exposure as a function of distance from the source. 5. The magnitude and distance from the source of the maximum con- centration for each profile generated in Item 4. 6. The total potential exposure to the population based on summing the exposure potentials over all direc- tions and distances from the source out to 50Km. The analyses specified in Items 4-6 were included because the dimensions of some of the area sources were large enough to cause substantial air concen- trations to occur at grid points that lie outside the primary sector. Ignoring these concentrations would give a false impres- sion of the importance of area size. These measures also give a better picture of IEM predictions under real meteorological conditions. Differences in concentration and ex- posure potential predictions due to the choice of source representation option were also investigated. Two typical HWMF sources were chosen, a process building and a small tank farm. The process building was assumed to be 10-m high, to cover 2 m2, and to release pollutants either from a rooftop or a midheight vent. The building was modeled as one stack source, as one 14.1 -m square area source, as two 10-m square area sources, and as two volume sources having standard deviations of 2.33 for their crosswind source distribu- tions and 4.65 for their vertical source distributions. The tank farm was assumed to contain four 6.1-m high tanks, to cover 200 m2, and to release pollutants from vents located on top of the tanks. The tanks were modeled as four stack sources, as four stack sources with adjacent 6.0-m2 high structures, as one 14.1-m square area source, as four 7.07-m square area sources, as one volume source having standard deviations of 3.29 for its cross- wind source distribution and 2.84 for its vertical source distribution, and as four volume sources having standard devia- tions of 1.64 for their crosswind source distributions and 2.84 for their vertical source distributions. Midheight (3.05-m) releases were considered only for the single area and volume source repre- sentations. Results and Conclusions Based on the analysis of variations in user-supplied input parameters and of the use of several modeling options for representing emissions sources, the study made the following findings: 1. Predicted ground-level air concen- trations are probably accurate to within a factor of 2, if the IEM is applied under well-behaved mete- orological conditions over flat terrain. 2. The IEM method for estimating the total exposed population is as ac- curate as any other general method. However, the accuracy of the method used to link exposed per- sons to specific pollutant concen- trations (i.e., to calculate exposures) is unknown, but likely is compar- able to the accuracy of other exist- ing methods. 3. For the sources considered in this study, wind speed acted as a linear scaling factor, except when pol- lutant decay and decomposition were considered. This relationship also would not hold for stacks that have an associated plume rise. 4. The effects on predicted pollutant concentrations due to variations in atmospheric stability, pollutant release height, and source area are interdependent. All three pa- rameters are strongly influenced by predicted concentrations, and every effort should be made to use accurate values for them. ------- 5. Increasing atmospheric stability increased exposure estimates, but it may either increase or decrease maximum concentration predic- tions, depending largely on the release height. 6. Increasing release height de- creased both exposure and con- centration estimates. 7. Increasing source area had little effect on exposure estimates for the same receptor array. Maximum concentration predictions varied by as much as 60% for the source areas considered in this study. 8. Use of the building wake effects option increased concentration predictions within 200 m of the source center, but had little effect on more distant concentration pre- dictions and on exposure estimates. 9. For pollutants that have half-lives of a few days or less, pollutant decay could significantly reduce airborne concentrations at recep- tors beyond 1 km. For longer-lived pollutants, decay is unimportant. 10. Pollutant disposition significantly affected both concentration and exposure predictions, especially at sites characterized by stable atmo- spheric conditions and low wind speeds. The pollutant deposition option in IEM should be used if the emitted pollutants are particles or can form particles that can be characterized. 11. The choice of a receptor array can bias predictions significantly. An array with receptors concentrated between the minimum allowed- radial receptor distance and 2 km should produce the most accurate estimates of maximum concentra- tions and exposures. 12. The various available emissions source modeling options produced essentially the same exposure esti- mates and airborne concentrations at receptors beyond approximately one kilometer. At the closer recep- tors, the stack and the area source representations produced very similar results. Volume source representations predicted close-in concentrations higher than those predicted using stack and area source representations for the more stable atmospheric conditions. For the less stable conditions, volume sources tended to predict the close-in concentrations which were lower than for the other two options. References 1. O'Donnell, F. R., P. M. Mason, J. E. Pierce, G. A. Holton, and E. Dixon, User's Guide for the Automated Inhalation Exposure Methodology (IEM), EPA-600/2-83-029(1983). F. R. O'Donnell and C. C. Gilmore are with Oak Ridge National Laboratory, Oak Ridge. TN 37830. Benjamin L Blaney is the EPA Project Officer (see below). The complete report, entitled "Sensitivity Analysis for Application of the Inhalation Exposure Methodology (IEM) to Studies of Hazardous Waste Management Facilities, "(Order No. PB87-232 641/AS; Cost: $18.95, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Hazardous Waste Engineering Research Laboratory U.S. Environmental Protection Agency Cincinnati, OH 45268 ------- United States Environmental Protection Agency Official Business Penalty for Private Use $300 EPA/600/S2-87/071 Center for Environmental Research Information Cincinnati OH 45268 CICAGO ------- |