United States
                    Environmental Protection
                    Agency
Water Engineering
Research Laboratory
Cincinnati OH 45268
                    Research and Development
EPA/600/S2-88/039 Sept. 1988
vvEPA          Project  Summary
                    Radium  Removal  for  a  Small
                    Community  Water  Supply  System
                    Kenneth A. Mangelson
                      In 1984, a radium removal treatment
                    plant was constructed tor the small com-
                    munity of Redhlll Forest, located In the
                    central mountains of  Colorado.  The
                    treatment plant consists of a process for
                    removing iron and manganese ahead of
                    an Ion exchange process tor the removal
                    of radium. The raw water comes from
                    deep wells and has naturally occurring
                    radium and iron concentrations of about
                    30 to 40 pCi/L and 7 to 10 mg/L, respec-
                    tively. Before the raw water enters the
                    main treatment plant, the raw water is
                    aerated to remove radon gas and carbon
                    dioxide.
                      The unique features of the Redhill
                    Forest Treatment Plant are related to the
                    ways In which the radium removed from
                    the raw water Is further treated and even-
                    tually  disposed of as treatment plant
                    waste. A separate system removes only
                    radium from the backwash/regeneration
                    water of the ion exchange process, and
                    the radium Is permanently complexed on
                    a Radium Selective Complexer* (RSC)
                    resin made by Dow Chemical. The  RSC
                    resin containing radium Is replaced with
                    virgin  resin  as needed and the resin
                    waste transported to a permanent  final
                    disposal site in Beatty, NV.
                      The aeration system reduces  the
                    radon gas by about 85% based upon the
                    data obtained. Typically, the radon gas
                    is reduced from 23,000 pCi/L to about
                    3,400  in  the raw  water after passing
                    through the  aerator.
                      The water quality data on the opera-
                    tion of the  ion exchange system In-
                    dicates that the radium In the inflow to
                    the ion exchange tanks is reduced from
                    about 22 to 35 pCI/L to 0.0 to 4 pCI/L in
                    the outflow from the treatment system.
                    •Mention of trade names or commercial products does
                    not constitute endorsement or recommendation for use.
  The RSC system has been very effec-
tive in the removal of radium from the ion
exchange system wastewater by remov-
ing an average of over 99% of the radium
in the inflow to the  RSC system. The
average inflow radium concentration was
about 1,180  pCi/L  with the average ef-
fluent at about 9.0 pCi/L.
  This report  presents  a detailed
description of the Redhlll Forest treat-
ment system and the results of in-depth
monitoring of the  processes and other
factors relating to the overall operation
of the radium removal system. Included
are descriptions of modifications made
in the plant operation to improve the
overall system operation and of the pro-
cedures for  final disposal of the RSC
resin containing radium.
  This Project Summary was developed
by ERA'S Wafer Engineering Research
Laboratory, Cincinnati, OH, to announce
key findings of the research project that
is fully documented in a separate report
of the same title  (see Project Report
ordering information at back).

Introduction
  A 21-month project  was initiated to
monitor and evaluate the full-scale opera-
tion of the treatment plant processes
designed and constructed to remove iron,
manganes, and radium and to determine
appropriate methods for disposal of plant
wastewater and complexed radium waste.
  In October 1985, the U.S. Environmental
Protection Agency in cooperation with the
Redhill Forest Property Owners Association
undertook a study  of the Redhill Forest
water treatment system.
  The following summarizes the processes
that make up the treatment plant and iden-
tify the areas where in-depth monitoring
was performed:

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  1. Aeration for radon and carbon dioxide
    gas removal.
  2. Chemical clarification, including set-
    tling  and  filtration  for  iron  and,
    manganese removal.
  3. Ion exchange for radium and hard-
    ness removal.
  4. Chlorination and water stabilization.
  5. Removal of radium from ion exchange
    regeneration water by RSC resin.
  6. Infiltration/evaporation (I/E) disposal
    pond for  plant wastewaters.
  The problem of radium in groundwater,
which serves as the  raw water supply for
the development, is common for  many
communities in the  United States.  If the
development of new water sources that do
not have a radium problem is not possible
or economically feasible, then a treatment
process for radium removal needs to be
considered. This report concerns itself with
one treatment alternative  and not with
locating new raw water sources that are
free of radium.
  The  treatment of  well water  for the
removal of radium is not practiced to any
great extent in the water treatment  field.
However, the ion  exchange process using
standard water softening type resins for
radium removal is well documented. The
Redhill Forest water treatment system in-
corporates a new process for concentrating
the radium removed by the ion exchange
process to simplify the final radium disposal
problem. The regeneration water from the
ion exchange process passes through  a
bed of RSC resin to remove the high levels
of radium  before the wastewater is dis-
charged to the I/E pond for final disposal.
There  are  no  known  water treatment
systems like the Redhill system. The RSC
resin has been used on a trial basis at
several locations primarily in Texas and one
site in  Wyoming. In  all  these cases, raw
water from the wells was passed directly
through the RSC bed with radium levels up
to about 100 Ci/L.

Experimental Procedures
  Raw water  from two wells is pumped
through a countercurrent  flow aeration
tower located at the  booster pump house.
The purpose of the aeration process is to
remove dissolved gases, specifically radon
and carbon dioxide, from the raw water. The
water is pumped to the  treatment plant at
a rate of about 90 to 100 gpm for further
water treatment  to remove iron, manga-
nese,  radium,  and hardness prior  to
Chlorination and discharge to the water
distribution system.
  As the raw water  enters the treatment
plant, alum, potassium permanganate, and
a polyelectrolyte are added to remove iron
and manganese by chemical precipitation.
The treatment unit is a prefabricated self-
contained unit that includes a mixing and
flocculation chamber, tube settlers, and
multi-media filtration. The effluent from the
iron and  manganese  removal process is
further treated to remove radium and hard-
ness in a ion exchange system that  uses
a cation resin.  The effluent from the ion
exchange system is chlorinated and zinc
hexame taphosphate added to control cor-
rosion  and sequester any residual iron
before being pumped  to the treated water
storage tank. The radium removed from the
water supply in the ion exchange process
is removed from the regeneration brine by
passing the brine through a separate treat-
ment process in which the radium is per-
manently complexed on the RSC material.
The wastewater from  this process along
with the backwash wastewater from the iron
removal process is pumped to the  final
disposal I/E pond.  Figure 1 is a schematic
diagram of the processes presented above.

Ultimate Disposal of Wastewater
and Radium Removal from Water
Supply
  The  original concept and design ap-
proved  by the Colorado  State  Health
Department for ultimate disposal of waste
generated at the  treatment plant are as
follows:

Plant Wastewater
  All wastewater from the plant operation
is discharged into an  I/E pond. The  main
purpose of the  pond is to allow for rapid in-
filtration of plant wastewater into a geologic
formation, which dips steeply to the east
and is located beneath the geologic forma-
tion in the area of the raw water supply
wells. The deep wells  obtain the raw water
from  this formation to  supply  the
development.

Radium Waste
  Most of the radium removed from the raw
water entering the treatment plant is even-
tually complexed  on  the RSC  resin.  As
needed,  RSC resin is  replaced  and
transported  to  an  approved  hazar-
dous/radiological waste disposal facility for
final disposal.
Sampling and Analyses
  The  project  generally consisted of  in-
depth monitoring of the operation of the full-
scale Redhill Forest water treatment plant
over a 21-month period from October 1985
through  June  1987.  All water  quality
parameter concentrations were determined
according to Standard Methods for the Ex-
amination of Water and Wastewater (15th
Edition).
  Most of the water quality analysis work
was performed  by Hazen  Research
Laboratory, a commercial lab  in Golden,
CO. Some analysis work was performed by
the EPA Laboratory in Cincinnati, OH, and
some radon gas analyses were performed
by Lowry Engineering in Maine.
  In-depth monitoring included water quali-
ty sample  collection  and   laboratory
analyses,  field  measurements,  flow
measurement, and detailed plant operation
and was performed to evaluate the follow-
ing components of the  treatment  plant
operation:
  1. Aeration system for radon  removal.
    Water  samples were collected and
    analyzed for radon concentration in
    the  raw  water before  and  after
    aeration.
  2. Treatment  system  for  iron  and
    manganese removal. Samples were
    collected and analyzed on the raw
    water inflow to the process and the ef-
    fluent from the system to assess the
    efficiency of operation.  The water
    samples were typically analyzed for
    iron, manganese, gross alpha, gross
    beta, and radium 226. The process
    wastewater from backwash operations
    was also analyzed on several occa-
    sions to determine the composition of
    the wastewater discharged to the I/E
    pond for final disposal. Parameters of
    primary interest for the wastewater in-
    cluded total iron, manganese, solids,
    and radium 226.
  3. Ion exchange process for radium and
    hardness removal.  Water  samples
    were collected  for  the  inflow and
    outflow to  the  unit process.  The
    samples typically were analyzed for
    iron, manganese, sodium, hardness,
    gross alpha, gross beta, and radium
    226. Water samples were collected
    from the backwash, regeneration, and
    quick  rinse  water on  several
    occasions.
  4. Radium Selective Complexer process
    for radium removal. This process was
    monitored frequently to determine the
    efficiency of radium removal from the
    ion exchange process wastewater and
    the buildup of radium in the complex-
    er  resin.  Environmental  radiation
     monitoring of the  area  outside the
     RSC tank surface was done to deter-
     mine the exposure and to relate the
     exposure to radium buildup on the
    complexer resin.

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                Booster Pump House
              Radon Gas
              Carbon Dioxide Gas
                Radon-
                3.400 pd/L
                        Concrete Sump
                       'Under Pump ^
                        House - 4.
Notes
                   Raw Water
                    Q= 10,000 gal
                    Iron = 4-7 mg/L
                    Na = 7 mg/L
                    TDS = 300 mg/L
                /-^"Hardness = 200-300 mg/L
               We/f Radium = 35-40 pd/L
               N° 2 pH =6.5
                V— Radon - 25.000 pd/L
1
1
1
1
np \
\

«Jffa/(
1
Chemica
(Alum., 1
nd Potassii
r»
Ac
aoly
im
Iron and Mant
and Filtrat
J
§
v
Idition
electrolyte.
Permanganate) \
janese
>cess
ion
Partii
+- Iron
Na =
TDS
Radi
Hard
, pH>
i Housea in
Backwash Wastewater \ Plant Build
Q = 350 gat
lron= 100-1 10 mg/L
Na = 700 mg/L
illy Treated Water TS = 570 mg/L
= 0.1 -1.0 mg/L Hardness = 0-10 mg/L
1 0 mg/L Radium = 60 pCi/L
= 300 mg/L
um =30 pd/L
ness = 200-300 mg/L Backwash Wa
f
ste water - 40C
''"^^^ 	 Iron « 76 mg/L I
1.  Ion exchange tanks  are assumed to  be back-
   washed after 40,000 gal  of water have been
   treated.

2.  Flows shown are average flows for every 10,000
   gal of ra w water processed through the plant from
   the wells.

3.  The treatment processes include:

   a. Aeration for carbon dioxide (pH adjustment) and
      radon gas removal.

   b. Chemical precipitation of iron and manganese
      in the Neptune  Microfloc flocculator/settler/
      filter unit.

   c. Ion exchange for radium removal and softening.

   d. Radium removal process using Radium Selec-
      tive Complexer  (RSC). Removes radium from
      the ion exchange  backwash  wastewater and
      concentrates radium on comp/exer resin.

4.   The normal treatment plant flowrate is about WO
   gpm The water from the ion exchange process
   for radium removal and softening is discharged
   into the wastewater holding tank from which the
   wastewater is pumped  through  the RSC at  a
   constant rate for radium removal
      650.
  Ion Exchange
    Process
(Radium Removal
 and Softening)
           Radium Removal
                 'sing Radiun
                 Selective
                 Complexer
Regeneration Wastewater
Holding Tank
Na °* 44 mg/L   I
Hardness *• 175 mg/L
TS « 736 mg/L
Radium = 42 pd/L
                                            Treated Backwash
                                         250 gal Constant Rate
                                                         Final Disposal of   j
                                                     Backwash Wastewater in
                                                      Infiltration/Evaporation
                                                             Pond        I
                    Chemical Addition
                 +- Chlorine and Zinc
                    Hexametaphosphate
                    Iron = 9.6 mg/L
                    Na = 10,300 mg/L
                    TS "37,600 mg/L
                    Hardness = 8,600 mg/L
                    Radium =7.0 pCi/L
                             To Morrison Formation -  1,000 gal
                   	_—I  Iron = 70 mg/L
                          To Distribution System
                          Iron 0.3
                          Na = 110 mg/L
                          TDS = 300 mg/L
                          Radium < 3 pci/L
                          Hardness = 5 mg/L
                                                     Hardness = 2,220
                                                     Radium = 40 pCi/L
Figure  1.    Flow diagram of'water treatment plant processes.
    5. I/E pond monitoring of the sand and
      soils was done to determine the extent
      of radium buildup due to the disposal
      of plant wastewater containing small
      amounts of radium.
    General plant monitoring of plant  flow
  rates,  volumes  of water processed,
  wastewater volumes, etc., was performed
  for use along with water quality data  in
  determining  plant  process efficiencies,
  plant operation and maintenance costs, etc.
    Some radon gas measurements were
  conducted  on site using a  RDA-200
Radon/Radon  Daughter  Detector unit
manufactured by EDA Instruments, Inc.
Also, some samples were collected and
sent to Lowry Engineering for additional
radon gas analysis.

Results and Conclusions
  Figure 1 shows the flow volumes for each
part of the total system operation for an
assumed raw water flow volume of 10,000
gal into the plant. Also presented are the
average water quality data for each com-
ponent that makes up the treatment plant.
                                   The aeration system has been proven to
                                 effectively remove radon and carbon diox-
                                 ide gases from the raw water supplied by
                                 the deep wells.  Carbon dioxide gas has
                                 been typically reduced from about 125 to
                                 25 mg/L in the aeration system. The reduc-
                                 tion of radon gas has been about 85% from
                                 about 23,000 pCi/L in the raw water to about
                                 3,400 pCi/L in the effluent from the aera-
                                 tion system. Additional measurements have
                                 indicated that the radon gas concentration
                                 in the treated water from the main treatment
                                 plant is about 600 pCi/L. The iron remov-

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ed about 13% of the radium from the inflow
to this process. When the  iron removal
system  was  backwashed,  the  radium
removed was wasted in  the I/E  final
disposal pond. Based  upon  the results of
the monitoring of the backwash water, the
average concentration of radium in the
wastewater was about 60 pCi/L.
  The ion exchange system removes  ra-
dium, hardness, and  residual iron and
manganese through the use of a standard
cation exchange resin. The process has
been very  effective  in removing radium,
hardness, and residual iron,  and in polish-
ing the effluent from the iron removal pro-
cess as long as the ion exchange capacity
is not exceeded. The monitoring results
generally indicate radium 226 levels of less
than 3 pCi/L and iron levels of less than the
recommended maximum level of 0.3 mg/L.
Frequent monitoring of the system opera-
tion has  indicated  that  the  radium
breakthrough occurs between 40,000 and
45,000  gal (i.e., 178  to 200  resin  bed
volumes). The quality of the influent to and
effluent from the ion exchange process has
generally been as given in Table  1.
  The   RSC  system  is  designed  and
operated to remove radium from the ion ex-
change process wastewater and to per-
manently concentrate  the radium on the
complexer  resin. On July 10,  1986, new
RSC resin  was placed in the complexer
tank and a detailed program of monitoring
the flow rate and the water  quality of the
inflow and  outflow was initiated.  Table 2
presents a summary of some of the results
of the monitoring from July 10, 1986, up
through June 1987. It should be noted that
the flow rate through the column has been
about 22 gpm, which is equivalent to the
surface loading rate of about  10 gpm/ft2.
The RSC resin  bed  depth is 2 ft.
  It can be seen in Table 2  that the RSC
resin  is highly  radium  selective  with
generally over 99% removal of radium from
the influent wastewater. Average data for
the water quality parameters included in
Table 2 are shown on the bottom of the
Table. The average inflow and outflow water
quality data indicate that iron,  sodium,
hardness, and total solids are virtually un-
changed in passing through the  resm
whereas over 99% of the radium in the in-
fluent is removed and concentrated on the
RSC resin. Also shown on the bottom of
Table 2 is  the  total quantity of  radium
removed and concentrated on the  resin
from July 10,1986, to June 10,1987. Based
upon the operation of the plant during this
time, the rate of radium buildup on the RSC
resin is about 347 /tCi/yr (347 X 106 pCi/yr).
  Further, it has been determined  that the
rate of radium removed from the raw  water
and permanently complexed on the RSC
resin is about 9.6 /*Ci (9.6 X 106  pCi) per
100,000 gal of water treated at the plant.
After some period of operation, the RSC
resin containing radium  will  be removed
from the RSC tank and replaced with new
resin and the old resin will be disposed of
at a  Nevada waste disposal site.  It is an-
ticipated that the RSC resin will be replaced
when the radium on the complexer  reaches
about 3,080 MCi (3,080 X 106 pCi). The 4 ft3
of RSC resin will then be placed in  a 55-gal
drum, 3.35 ft3 of concrete will be added, and
the entire  drum  will be transported to
Nevada for final disposal. This method of
handling the radium waste will ensure that
the total radium content of the container to
be buried will  not exceed 10 nCi/g (i.e.,
10,000 pCi/g).
  Finally, plant operating costs have been
determined and  estimated in Table  3.
  The full report was submitted  in  fulfill-
ment  of  Cooperative  Agreement No.
CR-812691-01-0  by the  Redhill  Forest
Property Owners Association under  the
sponsorship of the U.S. Environmental Pro-
tection Agency.
Table 1. Summary of Quality of
Parameter
Flow rate, gpm
Iron, mg/L
Manganese, mg/L
Sodium, mg/L
Hardness, mg/L as CaCO3
Radium 226, pd/L
Water to and from Ion Exchange Process
Influent
90 to 100
0.15 to 2.7
0.4 to 1.3
7.4 to 12.5
212 to 350
22 to 35
Effluent
90 to 100
0.03 to 0.5
0.01 to 0 15
40 to 150
5 to 70
0 to 4

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Table 2. Summary of Water Quality Data for Regeneration Wastewater from Ion Exchange Regeneration Through RSC Resin' (Effluent Discharged
to I/E Pond)
Accumulated Parameters Tofa/
Volume
Treated Bed
Date gal Volumes Sample
7/10/86 0
7/30/86 2,400
8/31/86 9,460
9/29/86 14,600
10/30/86 22,600
11/26/86 27,700
1/14/87 39,550
2/21/87 49,700
3/18/87 57,700
6/10/87 71,700
Averages
0
Inflow
Outflow
77
Inflow
Outflow
305
Inflow
Outflow
471
Inflow
Outflow
729
Inflow
Outflow
894
Inflow
Outflow
1,276
Inflow
Outflow
1,603
Inflow
Outflow
1,861
Inflow
Outflow
2,313
Inflow
Outflow
Inflow
Outflow
Iron
mg/L
2.48
0.98
2.03
1.56
9.0
8.5
7.21
7.15
2.79
2.07
7.17
6.30
31.4
27.8
61.3
62.2
93.4
92.0
8.08
3.76
19.8
18.5
Manganese
mg/L
23.8
16.7
31.8
32.2
33.1
33.1
30.5
31.5
33.1
33.5
28.2
26.9
19.2
18.1
30.5
32.4
31.2
31.9
17.4
15.8
29.9
27.7
Sodium
mg/L
11,600
13,300
11,000
11,000
12,600
12,700
11,400
11,500
8,170
8,640
13,400
13,300
9,350
9,000
12,300
12,100
13,500
12,400
8,070
8,460
10,850
10,760
Hardness
mg/L
476
245
9,850
10,200
11,500
11,600
8,350
8,420
9,380
10,100
9,620
9,520
7,260
7,740
10,900
11,400
11,600
12,600
5,580
4,940
8,890
9,030
Total
Solids
mg/L
34,900
34,600
41,700
41,800
54,200
55,200
37,600
37,600
35,000
35,300
45,400
45,500
31,300
30,400
49,800
50,400
53,200
53,300
28,100
28,300
40,590
40,550
Radium
226
pCi/L
860 ±30
16±11
1280 ±40
1.6.±3.2
1400 ±40
9.4 ±3.5
920 ±30
4.1 ±2.4
860 ±50
5.3 ±2.8
1040 ±30
8.1 ±3.3
1070 ±60
8.4 ±2.3
1 780 ±80
7.2 ±7
2000 ±80
18±9
650 ±20
9.2 ±2.4
1181
9.0
%
Radium
Removal
98.1
99.9
99.3
99.6
99.4
99.1
99.2
99.6
99.1
98.6
99.2
Note: From 7/10/86 to 6/10/87 (i.e., 355 days), 71,700 gal of plant wastewater was treated In RSC tank. The following is the amount of radium removed and deposited in the resin.

Radium removed  = 71,700 gal (3.785  L/gal) (1181-9.0 pCi/L)
                 = 318.1  X 106  pCi
                 = 318.1  ^Ci about 0.949 ^Ci/day
Estimate for year  = 347 pCi

"Resin bed volume  = 4.15 ft3 (31.0 gal)

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Table 3.     Summary Treatment Plant Operating Costs
                                                                  Cost/1,000 gal
                         Item                                    of Water Treated
        1.   Plant Chemicals, Alum,
            Permangante, Chtorine, etc.                                 $0.137

            Salt                                                       $0.475

        2.   Energy Costs                                              $0.206

        3.   RSC Resin Disposal
            (includes disposal and new resin)                            $0.088

	Total	$0.906*
'Operator cost not included.

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    Kenneth A. Mangelson is with Rocky Mountain Consultants, Inc., Englewood,
      CO, 80111.
    Richard P. Lauch is the EPA Project Officer (see below).
    The complete report, entitled "Radium Removal for a Small Community Water
      Supply System." (Order No. PB 88-235 551/AS; Cost: $14.95, subject to
      change) will be available only from:
            National Technical Information Service
            5285 Port Royal Road
            Springfield, VA 22161
            Telephone: 703-487-4650
    The EPA Project Officer can be contacted at:
            Water Engineering Research Laboratory
            U.S. Environmental Protection Agency
            Cincinnati, OH 45268
United States                        Center for Environmental Research
Environmental Protection               Information
Agency                             Cincinnati OH 45268
Official Business
Penalty for Private Use $300

EPA/600/S2-88/039
         H
          CHICAGO

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