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                   United States
                   EnvironmlWWProtection
                   Agency	
Air and Energy Engineering    *^M^>>
Research Laboratory          x  V \N
Research Triangle Park NC 27711  "
                                                      EPA/600/S2-89/009  June 1989
v°/EPA         Project Summary
                   Evaluation  of  Refrigerant from
                   Mobile Air  Conditioners
                   Leo Weitzman
                     This project was initiated to provide
                   a scientific  basis for choosing a
                   reasonable standard  of purity for
                   recycled  chloroflurocarbon (CFC)
                   refrigerant in operating automobile
                   air conditioners. It evaluated  the
                   quality of the  refrigerant from air
                   conditioners in automobiles of
                   different makes, ages,  and mileages,
                   from  different parts of the country,
                   and with both  failed  and properly
                   working  air conditioners.  The
                   refrigerant, CFC-12,  was tested for
                   water content,  acidity,  residue
                   quantity, refrigerant purity,  residue
                   purity, inorganic  chloride,  and
                   inorganic fluoride. This work will be
                   the basis for programs  to reduce CFC
                   emissions from  the  servicing of
                   automotive air conditioners.
                     Of the 227 cars sampled, neither
                   the compressor oil nor  the refrigerant
                   showed  any measurable levels of
                   acid (to 1 ppm), inorganic chlorides
                   (to 0.1 ppm), or inorganic fluorides
                   (to 0.1 ppm). The gaseous refrigerant,
                   in all but two samples  was of higher
                   purity than the specification for new
                   CFC-12.
                     The amount of residue measured in
                   the  CFC-12 was  simply the  com-
                   pressor oil which was carried  over
                   into the  sampling container by  the
                   refrigerant The amount of residue in
                   each  sample  depended on the
                   amount of refrigerant in the air condi-
                   tioner, the rate at which the sample
                   was removed (the sampling rate), and
                   on how soon after the air conditioner
                   was used the sample was taken.
                     The  residue (compressor oil) was
                   also tested for purity. It was found to
                   be very pure (>99% in  all but one or
                   two samples).  That impurity  was
found  to  consist of very  small
amounts (< 1 ppm) of a large number
of different organic compounds.
There was no statistically significant
correlation between residue  purity
and car mileage, whether the car's
compressor was functioning, or with
the area of the U.S. where the sample
was taken.
  Traces of water were found  In the
refrigerant The mean for all of the
samples was found to be 56 ppm. No
statistical correlation was  found
between the water content  of  the
refrigerant and  whether  the  com-
pressor was  working or  failed  nor
with the area where the sample was
taken; however, a statistically signif-
icant correlation was found between
the odometer reading of the car and
the water content The mean  water
content for odometers registering up
to 18,000 mi (29,000 km) was 34 ppm.
At higher mileage ranges, the mean
moisture content of the refrigerant
was In the 56- to 94-ppm range.
  This Project Summary  was {level-
oped  by EPA's  Air and Energy
Engineering Research Laboratory, Re-
search Triangle Park, NC, to announce
key findings of the  research project
that is fully documented In a separate
report of the same title (see Project
Report ordering Information at back).

Introduction
  Approximately 25% of all domestically
consumed  chlorofluorocarbons (CFC or
CFCs)  are currently used in automobile
air conditioners, the single largest use of
these  chemicals.  Moreover, current
servicing practices  result in substantial
but unnecessary emissions  of CFC-12
(dichlorodifluoromethane). During typical

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 servicing, any CFC-12 remaining  in the
 automobile air conditioner is first vented
 to the air, a new charge of  CFC-12  is
 sometimes used to test the system and
 locate the leak, and finally the system  is
 recharged with CFC-12 after repair. The
 release of CFC to the atmosphere  could
 be reduced by requiring the recovery and
 reuse  of  the  refrigerant  from all
 automobile  air  conditioners serviced;
 however, there has been little  information
 available on the  level of contamination  in
 operating automobile air conditioners and
 the  ability of equipment  to satisfactorily
i clean the CFC for reuse.
   This project to evaluate CFC refrigerant
 from automobile  air conditioners was
 initiated in response to these questions.
 The quality  of  refrigerant  present  in
 vehicles of  different makes,  ages, and
 mileages and  from  different parts of the
 country  has  now  been assessed. The
 refrigerant from  227 vehicles with  both
 failed  and  properly  working air
 conditioners was collected and  tested.
 The results of the program have provided
 an understanding of not only  the quality
 of the  refrigerant  found  in automobiles
 but  also  of  how  failure  of  the
 compressors and other equipment affects
 its contamination.
   The  work  was guided  by   and
 performed in cooperation with an ad hoc
 industry group comprised  of represent-
 atives of interested parties. The  ad hoc
 industry group agreed that the following
 parameters would fully describe possible
 refrigerant  contaminants: water  content,
 acidity, residue, chloride ion, purity  of the
 liquid phase, purity of the gas phase
   The group  also  determined that the
 recycled refrigerant would be  considered
 satisfactory  for   reuse if  recycling
 equipment could achieve a standard  of
 purity  comparable to  that   of the
 refrigerant  in  properly  working air
 conditioners  in  automobiles that have
 been driven for  15,000  ± 3,000  miles
 (25,000 ± 5,000 km). Thus, the two main
 aims  of the  program  were:  (1)  to
 determine the purity of CFC using the six
 parameters  listed  above  for properly
 working air conditioners in cars at 15,000
 ± 3,000 miles,  and (2) to determine the
 maximum  CFC  contamination for cars
 that will seek  service  due to   major
 component failure.
   In response  to  the  objectives,
 refrigerant in 227 vehicles from different
 parts  of the U.S. with a  variety  of
 mileages and automobile air conditioners
 was evaluated.
Sampling Procedure
  The equipment used for sampling the
automobile air conditioners consisted of a
sampling cylinder, sampling  line, and a
manifold  gauge  set and  vacuum  pump
(furnished by the shop at the sampling
site).
  Three  hundred  sampling  containers
that were manufactured specifically  for
this purpose were used for this program.
Each container  is an  (approximately) 1-
gal. (3.8 L) steel vessel equipped with a
2-way valve suitable  for CFC-12. One
sampling line  was  made  for  each
container and  packed  with  it.  Before
being shipped to the  sampling sites, all
sampling containers and  sampling  lines
were cleaned, dried and tested to ensure
that they  were  clean and  capable of
holding pressure.
  At the  sampling site, the sampling
containers  were  filled with  refrigerant
from the  automobiles by  placing  the
sampling container into a pan of dry  ice
and evacuating the line  and container.
The sample was then  drawn from the air
conditioning system at the high pressure
side so that lubricant would be withdrawn
with  the  refrigerant. Once the sampling
was  completed,  the air conditioning
system was serviced, if needed, and then
recharged by  service center personnel
following normal  procedures. For each
vehicle,  the model, year,  type of engine
and air conditioner, and other  information
were recorded on a Vehicle  Information
Form prepared for the  purpose.

Analytical Procedures
   The contents of each sample container
were  analyzed  as  received  by  the
method indicated for the following:
1.  Moisture  content:  Karl Fischer
    titration
2.  Acidity or acid number: KOH titration
3.  High boiling  residue or  oil content:
    Gravimetric analysis
4.  Cleanliness  or  purity  of  the
    refrigerant: GC/FID.
5.  Purity of the residue: GC/FID.
6.  Free halides: Ion chromatography

Results
  This sampling and  analytical program
showed that the  refrigerant in operating
air conditioners is very pure. Acids do not
accumulate  in  the  refrigerant.  Any
impurities that accumulate in the air con-
ditioning system are concentrated in the
compressor oil.  They are dissolved by
the liquid phase of the refrigerant but d
not get carried  over into  the gas phase
The gas phase proved  to  be  free  <
contaminants and equivalent in purity 1
new CFC-12.
  Water content was the  only  parametc
which was  highly dependent on vehicl
mileage.  In more than 95%  of th
samples analyzed, moisture was presei
at above the specification for  new CFC
12. Table 1 summarizes the results fc
water as well as for  residue purity. Th
water content of the refrigerant tended t
be greater  in  vehicles with  highe
mileage.  However,  even  refrigerant  i
new vehicles had a moisture level greate
than the 10-ppm specification on  nei
CFC-12. This may be due to  the sma
amount of moisture that is present on a
manufactured  parts  (e.g.,  as  th
compressor, expansion valve, and hose;
and to the  migration of moisture throug
hose  material. As illustrated  by th
relatively  small  standard  deviation
shown in  Table 1,  the moisture in th
lower mileage ranges does  not  vary a
much as it does in  the  higher  mileag
ranges.  The moisture  level  in th
refrigerant  did not show  any correlatio
with geographic location or vehicle make
  The mean for all of the samples wa
found to  be 56 ppm.  No  correlation wa
found between  the water content of th
refrigerant and the area of the U.S. wher
the  sample was taken;  however,
correlation was  found  between th
odometer reading of the car and th
water content.  The mean water conter
for cars up to 18,000 mi (29,000 km) wa
34 ppm. Above this mileage,  the mea
moisture content of  the refrigerant i
different mileage ranges remained in th
56- to 94-ppm range.
   Contamination  of   the  CFC-12  wit
HCFC-22  is  not  widespread.  Only tw
cars  out  of  more   than  200 teste
contained  more than the limit for ne<
CFC-12 of 0.5%.  Even if it occurs,  il
effect is limited since  it quickly leaks 01
of the system through the hoses and ha
a  very  limited  effect on  the ai
conditioner's performance.
   Neither the refrigerant  nor the residu
(compressor oil)  which  came with
during  the sampling  showed  an
measurable level  of  acid  (to 1 ppm
inorganic  chlorides   (to  0.1  ppm),  c
inorganic  fluorides (to 0.1  ppm). Th
refrigerant  in all the  samples  was bett<
than the purity requirement for new  CFC
12 by these criteria.

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  Table  1,   Summary of Results (ppm)
     Good Compressors
          (miles)*
 •t mi = 1.6km
 Standard deviation
                                            Moisture
                                                           Residue Purity
No.
Maximum
Mean
SO"
No.
Maximum
Mean
SD»
0-12,000
12,000-18,000
18,000-40,000
40,000-60,000
60,000-90,000
> 90,000
15
49
39
25
41
23
207
127
1,002
413
224
755
34
34
73
56
49
94
50
28
189
77
36
147
16
47
39
23
41
22
7,600
9,900
10,600
6,600
9,700
4,700
1,841
1,969
1,656
1,246
1,230
785
2,300
2,353
2,327
1,558
2,277
1,232
Subtotal
Failed Compressors
Total
Blanks
192
24
216
21
188
515 58 100 26 5,700
214
65 15 16 20 2,100

852 1.208

313 504
  One  possible explanation  of  the
absence of acid is that an automobile air
conditioner is a relatively  benign environ-
ment for a material  as chemically stable
as CFC-12. A second'explanation is that
the  acids  that  might form  are fully
contained in  the  lubricant or  are
neutralized by the metal content of the air
conditioner  components.  There  was
evidence that free acid reacted with the
material of the sampling system.  This
chemical  reaction  would result in
deterioration  of  metal,  but  would not
degrade refrigerant.
  The finding on  the lack  of acid  is good
news for  the program.   Because the
sampling system was selected to closely
duplicate the recovery system that will be
used to recycle  the refrigerant, there is
every reason to believe that no significant
quantity of acid will be removed from the
unit  during recycling/servicing.  Further-
more, any acid  present  during  normal
capture  and  recycling  of the refrigerant
can  be removed  by  the  recycling
equipment. Laboratory tests indicate that
acid  can be  neutralized by contact  with
special  metal  compounds that can be
incorporated in the recycling equipment.
The  acid  is  neutralized  within  a  few
minutes of contact. Based on this labora-
tory  analysis,  acidity in recycled refriger-
ants  will not  be  a  problem  if recycling
equipment is properly designed.
  The level of residue in each  sample
depended on  the amount  of refrigerant in
the air conditioner, the rate at which the
 ample was removed (the sampling rate),
            and on how soon after the air conditioner
            was used before the sample was taken.
            The residue detected in the samples is
            primarily the  compressor oil which was
            carried over into the sampling  container
            by the refrigerant. No significant contam-
            ination,  other than  oil, was  found in the
            CFC.
              The residue (compressor  oil) was also
            tested  for purity.  The results are sum-
            marized in Table  1. It was  found to  be
            very pure (>99%  in all but one or two
            samples). The impurity  was found  to
            consist of very small amounts (< 1 ppm)
            of a large number of different organic
            compounds. The  concentration  of any
            one compound was too low  to allow
            identification.  The residue turned out to
            be a reasonably good quality compressor
            oil. Attempts were made to  correlate the
            residue purity  with  car  mileage, with
            whether the compressor had failed or not,
            and with the part of the country where the
            sample  was taken.  No correlation was
            found with any of these three parameters.
              The purity of the refrigerant itself was
            tested  by withdrawing a  sample of the
            gas phase from the  sampling container
            and analyzing it with a gas chromato-
            graph/flame ionization detector. The pur-
            pose  of this  test  was  to determine
            whether any of the refrigerant samples
            had been  contaminated with other CFCs
            such as  HCFC-22. The  test could also
            identify  any  gaseous  products  of
            decomposition of the refrigerant or of the
            compressor oil. Except for  two samples
            that showed some HCFC-22, no measur-
                                            able extraneous materials were found in
                                            the gas phase of the refrigerant.
                                             Trace quantities of  other  CFCs and
                                            HCFCs  are  common  contaminants  in
                                            CFC-12  and  are allowed by the speci-
                                            fications for new CFC-12 to compose up
                                            to 0.5% of the  product. Samples of new
                                            CFC-12 from  several  suppliers  were
                                            analyzed  as  part  of this program and
                                            were found to contain up to 0.1% HCFC-
                                            22  as well as  of  other  volatile  compo-
                                            nents. HCFC-22 contamination in opera-
                                            ting automobile air conditioners cannot
                                            remain very high because it quickly leaks
                                            out through the  rubber hose materials.
                                             Only  two samples of refrigerant out of
                                            the 227 automobiles tested were found to
                                            contain more than 0.5%  HCFC-22 in the
                                            CFC-12;  one contained 2% and the
                                            second 5% HCFC-22. In neither case did
                                            the level of contamination make  that air
                                            conditioner's  performance deteriorate  to
                                            the point where the owner chose to have
                                            it repaired.

                                            Conclusion
                                             This sampling and analytical program
                                            showed that  the refrigerant in operating
                                            air conditioners  is very pure. Acids do not
                                            accumulate  in the refrigerant.   Any
                                            impurities  that  accumulate  in the  air
                                            conditioning system are  concentrated in
                                            the compressor oil. They are dissolved
                                            by the liquid  phase of the refrigerant but
                                            do  not  get  carried  over into the gas
                                            phase. The gas phase proved to  be free
                                            of contaminants and  equivalent in purity
                                            (as measured by  a gas chromatograph

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with  a flame  ionization detector) to  new
CFC-12. The  moisture  level  in  the
refrigerant did not show  any correlation
with geographic location or vehicle make.
  The finding on the lack of acid is good
news for  the program.  Because  the
sampling system was selected to closely
duplicate the recovery system that will be
used to recycle  the refrigerant, there  is
every reason to believe that no significant
quantity of acid will be removed from the
unit  during recycling/servicing.  Further-
more, any  acid  present  during normal
capture and recycling of the refrigerant
can  be  removed  by  the  recycling
equipment. Laboratory tests indicate that
acid  can be neutralized by  contact with
         special metal compounds that can be in-
         corporated  in  the  recycling equipment.
         The  acid is neutralized  within  a  few
         minutes  of  contact.  Based  on  this
         laboratory analysis, acidity in recycled
         refrigerants will not be a problem if re-
         cycling equipment is properly designed.
           The lack of chloride or fluoride ions in
         the samples further reinforces the above
         conclusion. These ions would typically
         form by hydrolysis of the CFC-12, form-
         ing hydrochloric or hydrofluoric acid. The
         lack of these ions, coupled  with the  high
         purity seen in the CFC-12 itself, indicates
         that refrigerant breakdown does not occur
         under the conditions encountered in an
         automobile air conditioner.
  In  summary, the data gathered  he
indicate that the CFC-12 refrigerant  do
not  degrade  significantly  with  us
Furthermore, while small amounts of cc
taminant are removed with the refrigers
during  servicing,  the  bulk  of  tl
contaminants remain with the compress
oil.  Current  servicing practices do r
require that  the compressor  oil I
changed unless the  compressor is i
placed.  The presence  of  HCFC-22
concentrations above the specification 1
new  CFC-12 is rare, less than 1% of t
cars  tested. HCFC-22 contaminant quic
ly leaks out of the automotive air com
tioner  through hoses  and,  does n
appear  to cause  operational  probler
while in the system.
 L Weitzman is with Acurex Corp., Research Triangle Park, NC 27709.
 Dale L Harmon is the EPA Project Officer (see below).
 The complete report,  entitled "Evaluation of  Refrigerant  from  Mobile  Air
    Conditioners," (Order No. PB 89-169 8821 AS; Cost: $15.95, subject to change)
    will be available only from:
         National Technical Information Service
         5285 Port Royal Road
         Springfield, VA 22161
         Telephone: 703-487-4650
 The EPA Project Officer can be contacted at:
         Air and Energy Engineering Research Laboratory
         U.S. Environmental Protection Agency
         Research Triangle Park, NC 27711
 United States
 Environmental Protection
 Agency
Center for Environmental Research
Information
Cincinnati OH 45268
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