United States Environmental Protection Agency Robert S. Kerr Environmental Research Laboratory Ada, OK 74820 Research and Development EPA/600/S2-89/035 Sept. 1989 &EPA Project Summary Kinematic Modeling of Multiphase Solute Transport in the Vadose Zone R. J. Charbeneau, J. W. Weaver and V. J. Smith The goal of this research was the development of a computationally efficient simulation model for multiphase flow of organic hazardous waste constituents in the shallow soil environment. Such a model is appropriate for investigation of fate and transport of organic chemicals introduced to the soil through spills on the ground surface, leakage from surface impoundments or under- ground storage tanks, or land treat- ment of hazardous wastes. During the initial phases of a site investigation there usually does not exist sufficient data to support the application of comprehensive, computationally ex- pensive numerical models. Simplified physically based models which can address the transport of an organic constituent experiencing volatiliza- tion, multiphase partitioning, biodeg- radation and migration may be preferred. Two models based on the kinematic theory of multiphase flow are developed and presented, along with a number of illustrative examples. The Kinematic Oily Pollutant Transport (KOPT) model assumes steady infiltration of water based on the expected annual infiltration rate; the Kinematic Rainfall and Oily Pollutant Transport (KROPT) model includes transient hydrologic phenomena (evaporation and infiltra- tion) along with a model of stochastic generation of rainfall. The examples presented suggest that the KOPT model may be preferred for most applications. This Project Summary was developed by EPA's Environmental Research Laboratory, Ada, Oklahoma, to announce key findings of the research project that is fully documented in a separate report of the same title (see Project Report ordering information at back). Introduction The focus of this research has been on the fate and transport of organic hazardous waste constituents in the shallow soil environment. Organic hazardous waste constituents may be introduced into the soil by spills on the ground surface, leakage from surface impoundments or underground storage tanks, or land treatment of hazardous wastes. Oftentimes in these circum- stances, an "oil" phase is present in addition to the water, air, and soil of the natural media, and the fate and transport characteristics are determined by the mobility of the water and oil, as well as by multiphase partitioning of the constit- uent between the air, water, oil and soil matrix. The emphasis of the research has been on development of simplified models for fate and transport of organic contaminants which may be appropriate for the initial screening or investigation of a site when the available data base does not warrant the application of more general models. The primary objectives of this cooper- ative agreement have been to support RSKERL in their modeling studies of subsurface contamination from organic wastes, including hazardous waste land treatment operations, and to investigate the application of kinematic models for multiphase processes including the flow of water and oil, as well as multiphase- ------- partitioning, volatilization, and bio- degradation. The Kinematic Oily Pollutant Transport (KOPT) and Kinematic Rainfall and Oily Pollutant Transport (KROPT) programs are implementations of a kinematic multiphase transport model that was developed as a part of this research. The KOPT program is a simplified implementation of the kinematic multi- phase transport model, intended to be used as a screening tool for hydrocarbon spills or near-surface releases. It addresses the questions of how far an oil release might go into the soil and how soon it might get there. In the KOPT implementation, steady water infiltration is assumed to occur, and the specified water saturation is taken as represen- tative of climatic conditions. The KROPT program is the full implementation of the kinematic multiphase transport model and includes modeling of transient hydrologic phenomena (evaporation and infiltration), along with a model for the stochastic generation of rainfall. This model handles multiple loadings or releases of oily wastes at or near the ground surface, multiple rainfall events, potential oil migration, sorption, volatiliza- tion, and biodegradation. Research Background and Scope The objective of this research was to apply kinematic modeling theory to fate and transport of hydrocarbons in the vadose zone for oil spills and land treatment sites. The purpose of the work was to provide a way to estimate the gross movement of pollutants in a multiphase system resulting from spills, leaks and at land treatment sites. In the case of land treatment systems, the long- term behavior of the site is of interest, so computationally efficient simulations are needed. This was the reason for using a simplified approach. When placed in porous media, immiscible pollutants retain their unique properties. Although these pollutants are largely immiscible in water, they are capable of causing ground-water contam- ination by their dissolved constituents. Immiscibility leads to distinct bodies of pollutant in close contact with both air and water, where present. Above the water table, the addition of an immiscible pollutant causes the original two-phase water/air system to become a three- phase water/pollutant/air system. When flowing, the transport and fate of immiscible fluids are governed by a set of relationships which are, basically, expanded forms of the single phase governing equations. The former provides the theoretical framework for solving immiscible (or multiphase) flow problems in general. The specific application of the theory depends on the initial and boundary conditions imposed during pollutant migration as well as other features unique to pollution incidents. Currently available analytic and semi- analytic multiphase flow models share the limitation that they rely on an assumed shape of the oil profile that is not based upon solution of the governing physically based equations. After an oil release ends, the oil is gradually replaced by air as it drains. A drainage profile, similar to those observed for water is expected, since the same forces that act on the water also act on the oil. Other phenomena outside the scope of these models are biodegradation, which also causes variable oil saturations, and simultaneous unsteady flow of the water. The latter is typical of actual time-varying conditions in the field. Only a few numeric solutions of the multiphase flow equations have been presented for the specific problem of shallow aquifer contamination. A limita- tion of the numeric approach is that the models are computationally very inten- sive. To exploit fully their capacity for modeling geologic variability, a large amount of data is required. Because data is usually sparse, the full capacity of a numeric model may never be reached when applied to specific site inves- tigations. The analytic and semi-analytic flow models illustrate that if a constant amount of water is present in the pore space, only the mass conservation equation for the oil needs to be solved. A solution, that has not been used for this purpose, is the kinematic model for soil moisture transport. In addition to a solution for the duration of water application, this model gives a solution for the unsteady flow occurring in soils undergoing drainage (replacement of soil moisture by air). The solution is obtained by solving an approximate governing equation for the water by the method of characteristics (MOC). With the proper constitutive relationships for two-phase flow, the water solution is analytic. Adapting this solution for the oil phase gives a more realistic model than the analytic and semi-analytic models mentioned above, since the oil drainage profile is deter- mined by solution of the governing equation. An analytic solution is not possible for the oil because the relative permeability function is too complicated and depends on the amount of water in the pore space. However, a semi-ana solution for the oil phase can achieved, allowing relatively low c putation times to be achieved. The following assumptions are i for the model formation. The m< equations are solved for one-dimensi flow. This is one of the neces: assumptions to extend kinematic th to multiphase flow. Lateral migra however, reduces the amount pollutants and water that m downward. The one-dimensional forn tion is conservative as it will deten the maximum amount of substances will reach a given depth. A component pollutant is assumed. Th acts as an inert carrier for the dissc pollutant. Various transformations, ( than biodegradation, that the oil undergo are not modeled. Adve< transport is used to model the tran of the constituent by oil and w Equilibrium, linear partitioning rela ships are used for sorption, dissol into the water and for volatilization the air phase. Volatilization is modele applying the wet zone/dry zone m To extend kinematic modeling to tr phase, three more assumptions are i First, the flow of the air does not im the flow of the liquids. Second, the phase transport is dominated by gr Lastly, the medium is assumed t strongly wetted so that water will r in the smallest pores, air in the lai and oil in the intermediate sized pore Under the conditions discussed kinematic model can be applied 1) I unsteady flow of both the oil am water and 2) to the fate and transp the dissolved constituent. If onh advective motion of the constitue modeled, the resulting equation; compatible with the numerical app taken for the oil equations. Two separate implementations created. The first (KOPT) was kinematic model for the oil mig only, with a constant amount of present in the pore space. This me analogous to the simplified analyti semi-analytic flow models noted < but with the capability to sin- degrading oil and the transport ( dissolved constituent. In related re: this model was coupled with a me oil spread along the water table, wl turn supplied input for a model of transport in the saturated zone. He overall model was intended screening tool for oil spills. A Guide for the KOPT model is pre in Appendix A while the listing code is presented in Appendix B. ------- The second implementation (KROPT) vas a model to investigate the nteractions between incoming rainfall and oil moving within the profile. This model is suited for studying the effect of •3 series of rainfall events, irrigations and cultivations on a land treatment site. There are practical limitations to ipplication of the KROPT model, and it is :onsidered a research code at this time. Discussion This work has shown that kinematic heory can be applied to multiphase flow )roblems. Kinematic models have an idvantage over traditional numeric mod- »ls in that the kinematic models are well- tiited for studying the hyperbolic or /ave behavior of the multiphase flow iquations. Inclusion of sharp fronts is atural to the kinematic models, while inite difference or finite element models ncounter difficulties when derivatives in he governing equations tend to become ndefined. Solution of the kinematic lodel shows how the oil and water fronts nteract. Thus, by simplifying the gov- rning equations, some of the funda- lental behavior of the solution is clearly evealed. The effect of the neglected apillary pressure gradients are to crease the infiltration capacity of the oil and smear the fronts. Much of the mportant physics is retained, however, in he kinematic model. Computationally, by reducing the nginal system of coupled partial ifferential equations to a system of rdinary differential equations, the ifficulty of finding a numerical solution is educed greatly. Resulting computer ^odes are well suited to solving problems where there is a constant amount of water in the pore space. Such a situation corresponds to a soil at the so-called field :apacity and can represent typical :onditions of the profile. The best per- ormance of the KOPT model is obtained vhen the oil is nondegrading and the oil iharacteristics are straight. Curving char- ictenstics, due to biodegradation, in- rease the computational effort. The implementation of the more eneral model (KROPT) reveals the iteractions between the oil and water onts. The model is limited to situations 'here the initial water profile is uniform. ince again the best performance is btained when the oil characteristics are raight, since the characteristic equa- Dns are not solved explicitly. Per- imance is degraded where rainfalls cceed the kinematic capacity of the soil. ince the infiltration capacity is infinite initially, very large water fluxes are possible until runoff is produced. During this period small time steps are required. This modeling work enhances understanding of multiphase flow through the results obtained from the example problems presented. Most important is the material concerning the oil banks. If incoming rainfalls displace oil, then the banks are created. Although this is a result of simplified modeling, the notion that incoming water displaces oil into a bank moving ahead of the water front is a more general result. In situations where the flow of the fluids is not kinematic, banks will also exist. In certain cases, the banks may be very pronounced, although short-lived. In others, the banks may persist for longer periods but would be virtually undetectable in the laboratory and the field or by numerical methods that are not based upon the kinematic model. The kinematic model results indicate that the water displaces all of the mobile oil. This result was contrary to what was expected but was established through conservation of mass. Some displace- ment of oil would be expected, along with the creation of an oil bank, but the model result may or may not be confirmed by experiment. The value of the residual oil saturation is critical for the results obtained from the model. This parameter could be easily manipulated to show that oil would spread over a smaller depth. Biodegradation of the oil has only a small effect upon the ultimate depth attained by the oil. It does affect the mobility of the oil (reducing it). An interesting effect on the constituent is caused by biodegradation of the oil. Concentrations increase as the oil degrades because of the loss of solvent. If the constituent is also biodegradable, the shorter half life determines if the concentration will increase or not. As in field cases where constituent concentrations in water are measured, a large mass of constituent may reside in the oil phase and not be detected. In one of the examples, concentrations in the oil are 50 times greater than in the water. If only the water phase concentrations are measured, most of mass in the soil is missed. This is particularly a problem if the oil is immobilized, since the oil cannot flow into an observation well (phenomena akin to end effects may prevent oil flow into wells even at higher saturations). The presence of the oil material is not detected by the observation wells; the core material itself must be analyzed. Using a differential equation solver is well suited to solving the kinematic model, since the model equations can be written as a system of ordinary differential equations. The speed of the solver is degraded as more and more equations are added. For these situations, it might be advantageous to solve the method of characteristics portion of the solution by finite difference techniques instead of tracking the characteristics. The overhead associated with using the Runge-Kutta-Fehlberg solver may be comparable to that for the discretization methods. Also, the necessity to track sets of oil bank characteristics makes the program ex- ceedingly complex Extension of the model may not be practical because of this. Conclusions and Recommendations The results of this research found that kinematic theory was successfully ap- plied to multiphase flow of water and oil. Kinematic models have an advantage over traditional numeric models in that the kinematic models are well-suited foi studying the hyperbolic or wave behavioi of the multiphase flow equations. Inclusion of sharp fronts is natural to the kinematic models, while finite difference or finite element models encounter difficulties when derivatives in the governing equations tend to become undefined. The kinematic model simpli- fies the governing equations revealing some of the fundamental behavior of the solution and showing how the oil and water fronts interact. Solution of the kinematic model indicates that the incoming water must displace all of the mobile oil for mass to be conserved. Another important result is that oil banks are formed when the incoming water displaces the oil that is present. The main limitation to the kinematic model is that displacement of oil by water may be unstable depending on the fluid prop- erties of the oil and the speed of the incoming water. The two computer codes written to implement two versions of the kinematic model, KOPT and KROPT, run in a computationally efficient manner and may be used to estimate the vertical migration of oil and a dissolved con- stituent within the soil profile, including the effects of volatilization and biodegradation. Running these codes showed that the amount of residual oil saturation strongly affects the total depth over which the oil will be predicted to spread. ------- In light of the success of kinematic models for multiphase flow problems, further development of the KOPT and KROPT programs is recommended. Specifically, the following recommenda- tions are suggested: • Generalize KOPT and KROPT models for use in simulation of facilitated transport. Such an application could look at the use of solvents (such as heptane) for flushing a soil profile to remove low mobility organic hazardous wastes and then model the much more rapid volatilization and degradation of the solvent. Development and implementation of user-friendly versions of the KOPT and KROPT programs. Expand KROPT program to handle unstable displacements of oil by water, thereby eliminating the main limitation of the model and enabling the use of randomly generated rainfalls that may exceed the kine- matic rate. This program enhancement would also handle cases where oil is the displacing fluid, instead of water, such as for when the oil loading rate exceeds the kinematic capacity of an initially nonuniform water profile. Expand KROPT to handle lay systems, where the effects of fluids crossing into media of diff< intrinsic permeabilities and pore distributions can have an impo effect on their migration. Modify KROPT to have the optk use other oil relative permea! models, in addition to the Br< Corey approach. Modify KROPT to handle depth time variability in oil resi saturations. R. J. Charbeneau, J. W. Weaver, and V. J. Smith are with the University of Texas at Austin, Austin, TX 78712. John E. Matthews is the EPA Project Officer (see below). The complete report, entitled "Kinematic Modeling of Multiphase Solute Transport in the Vadose Zone," (Order No. PB 89-207 948/AS; Cos?: 527.95, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Robert S. Kerr Environmental Research Laboratory U.S. Environmental Protection Agency Ada, OK 74820 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati OH 45268 Official Business Penalty for Private Use $300 EPA/600/S2-89/035 S00s°!5»§3il UUi....!!..!!,,..!,,}.!,.!! ------- |