United States
                    Environmental Protection
                    Agency
                    Research and Development
                    Atmospheric Sciences Research
                    Laboratory
                    Research Triangle Park NC 27711
                    EPA/600/S3-85/039  May 1985
&ERA         Project  Summary
                                   i
                    Temporal  and  Spatial
                    Variabi ity of  the  Visual
                    Effects
of Stack Plumes
                    Christian Seigneur, A. Belle Hudischewskyj, and Henry Hogo
                      Temporal and ipatial variabilities of
                    stack plumes are analyzed by means of
                    field data analysii and computer simu-
                    lations.  In this investigation,  photo-
                    graphs from field p rograms of the study.
                    Visibility Impairment Due to Sulfur
                    Transport and Transformation in  the
                    Atmosphere went analyzed via sensi-
                    tometry, and PLUVUE II model simula-
                    tions were conducted for a case study.
                    Analysis of the temporal variability of
                    plume visibility led to documentation of
                    the fact that the vi tual effects of plumes
                    vary with time because of (1) turbulent
                    fluctuations, (2) changes in atmospheric
                    stability, and (3) cr> anges in the observer-
                    plume-sun scattering angle. Likewise,
                    the analysis of thu spatial variability of
                    plume visibility led to the fact that the
                    visual effects oF plumes  vary with
                    downwind  distance from the stacks
                    because of  (1) turbulent fluctuations,
                    (2) dilution of the plume and/or a
                    change in the obsurver-plume distance,
                    and (3) changes in the observer-plume-
                    sun scattering angle.
                      This Project Summary was developed
                    by EPA's Atmospheric Sciences Re-
                    search Laboratory, Research Triangle
                    Park. NC. to announce key  findings of
                    the research project that  is fully docu-
                    mented in a separate report of the same
                    title (see Project Report ordering infor-
                    mation at back).


                    Introduction
                      The impact of stack plumes on atmos-
                    pheric visibility has been the subject of
                    extensive  experimental and  theoretical
                    studies over the past 5 years. Of these
                    studies, the Visibility Impairment Due to
                    Sulfur Transport and Transformation in
                    the Atmosphere (VISTTA) program was
                    comprised of four field programs con-
                    ducted in 1979 and 1981, as well as an
                    evaluation of the EPA plume visibility
                    models PLUVUE and PLUVUE H.
                     An important conclusion of these
                    plume-visibility studies is that there is a
                    major discrepancy between the nature of
                    the measurements of plume visibility and
                    computer simulations of plume visibility.
                    Measurements of plume visibility were
                    taken over a given time interval (about 15
                    to 30 minutes for teleradiometer meas-
                    urements, and instantaneous measure-
                    ments for the sensitometry of color slides)
                    and at a given location. Fluctuations of
                    atmospheric turbulence led to plume-
                    visibility effects that varied with time and
                    location. Simulations of plume visibility,
                    on the other hand, were conducted with
                    mathematical  models that assumed
                    steady-state conditions, a given atmos-
                    pheric stability class, and time-averaged
                    dispersion coefficients. The discrepancy
                    between the time- and location-specific
                    nature of experimental measurements
                    and the time-averaged (e.g., dispersion
                    coefficient) and conditions-averaged (e.g.,
                    atmospheric stability) nature of model
                    simulations necessarily results in differ-
                    ences between experimental measure-
                    ments and model simulations.
                     In this study, we investigated the tem-
                    poral and spatial variability of plume vis-
                    ibility in a systematic fashion. We ana-
                    lyzed a series of color slides  from the
                    1979 and 1981 VISTTA field programs by
                    means of sensitometry to determine the
                    temporal  and spatial variability of plume
                    visual effects. Conclusions can thus be
                    drawn about the uncertainties that will

-------
result when using atmospheric data on
plume  visibility for model evaluation or
when using a plume-visibility model in
regulatory applications.

Experimental Procedure
  The data base utilized in this study con-
sisted  of color slides of power  plant
plumes that were  selected from the
December 1979 program at the Navajo
power plant and from the February 1981
program at the  Kincaid power  plant.
These slides offered the best time series
of the visual effects of stack plumes col-
lected during the four VISTTA field pro-
grams. A total of 46 slides were chosen
for sensitometry (i.e., digitization). These
slides were digitized at Perkin-Elmer in
Garden Grove, California.
  For the temporal  variability analysis,
each slide was processed at a given loca-
tion. The section of the photograph to be
digitized corresponded to an imaginary
vertical line across the plume so that both
the background below and above the
plume andthe plume itself were digitized.
The procedure is therefore similar to the
vertical scan taken with a teleradiometer.
For the spatial variability analysis, 10 ver-
tical scans were performed on the select-
ed slides at equal horizontal intervals that
covered the entire  slide  range.  These
scans thus corresponded to plume visibil-
ity measurements conducted at different
downwind distances from the same ob-
servation site (i.e., the site where the pho-
tograph was taken).
  The slide digitization was conducted at
three wavelengths by using narrow-band
filters with peaktransmittance at 450 nm
(blue filter),  540  nm (green filter), and
above 700 nm (red filter). The sensitometry
provided pixel densities for each scan at
three wavelengths.  The pixel densities
obtained from sensitometric curves were
then converted to normalized exposures
by means of  characteristic curves that
were constructed from sensitometry of
reference slides.  The exposure results
were then analyzed in a standard fashion
to calculate the ratio of plume radiance to
sky radiance.
  After the digitized data were processed,
the digitization scans were reviewed to
select the scans that could be analyzed,
i.e., those for which a plume was discern-
ible above the noise of the measure-
ments. The list of slides selected for tem-
poral variability analysis was reduced to
32. These 32 slides included sights of the
Navajo power plant plume on December 7
and 15, 1979, and of the Kincaid  power
plant plume on February 20  and 24,
1981.
Temporal Variability of Plume
Visibility
  The ratios of plume  radiance to sky
radiance were calculated by the sensito-
metric  technique  and plotted for  each
case study as a function of time. The case
studies  considered included the Navajo
power plant plume observed from two dif-
ferent sites on December 7, 1979, and
from one site on December 15,1979, and
the Kincaid power plant plume observed
on February 20, 1981, and on February
24, 1981. The later Kincaid power  plant
plume was dark on the left side and bright
on the right side of the slide; the analysis
was therefore conducted at two locations
on the slide.
  The study of the temporal variability of
plume visibility has shown that notable
variations  in the  plume  visual effects
occur as a function of time. These varia-
tions, which exceed the uncertainties of
the sensitometric measurements,  may
represent:
  1.  An evolution of atmospheric stabil-
     ity toward more unstable conditions
     that lead to a more dispersed and
     less discernible plume; this effect
     was observed for the Navajo power
     plant plume on December 15,1979,
     and the Kincaid power plant plume
     on February 20, 1981.
  2.  A  variation in plume visual effects
     that  results from a change in the
     scattering angle andthe associated
     varying effects of particulate  scat-
     tering; this phenomenon  was ob-
     served in measurements and model
     simulations of the Kincaid power
     plant plume on February 24, 1984.
  3.  Turbulent fluctuations that occur in
     a random manner and are reflected
     in nonstationary characteristics of
     the plume; this phenomenon was
     observed for the Navajo power plant
     plume on December 7, 1979.

Spatial Variability of Plume
Visibility
  The ratios of plume  radiance to sky
radiance were calculated by the sensito-
metric technique and plotted for each of
the four analyzed case studies as a  func-
tion of theobserved azimuth angle, i.e., as
a function of the horizontal distance  along
the color slide. The four case studies con-
sidered were the  Navajo power  plant
plume on December 7 and 15,1979, and
the Kincaid power plant plume on Febru-
ary 20 and 24, 1981.
  The study of the spatial variability of
plume visibility showed that variations in
the plume visual effects occur as the
muth of the observer's  line  of  s
changes. These  variations  exceed
uncertainties of the sensitometric mi
urements and may occur in a monoti
form, representing any of the  follov
conditions:
  1.  A decrease in plume visual eff
     due to dilution of the plume anc
     an increase in the observer-pli
     distance; this phenomenon '
     observed for the Navajo power p
     plume on December 7 and 15,1 £
  2.  A variation in plume visual off
     (e.g., from bright to dark plume)
     results from a change in the seal
     ing angle and the associated v
     ing effects of particulate scatter
     this effect was observed and,
     certain extent,  simulated for
     Kincaid power plant plume on F
     ruary 24, 1981.
  3.  Turbulent fluctuations that lea-
     nonhomogeneous characteris
     of the plume; this phenomenon \
     more evident in observations of
     Kincaid power plant plume on F
     ruary 20, 1981.

Conclusions
  This investigation demonstrates I
the visual  effects of plumes  vary v
time because of several factors.

  1.  Turbulent fluctuations lead to r
     dom temporal and spatial variati
     in plume visibility.
  2.  Evolution of atmospheric stab
     toward more unstable conditi
     leads to a  temporal  variation
     plume visibility dueto a moredil
     plume.
  3.  Dilution of the plume and/or
     crease in the observer-plume i
     tance lead  to a spatial variatior
     plume visibility.
  4.  A change in the observer-plur
     sun  scattering angle may leac
     temporal and spatial variations
     plume visual  effects (e.g.,  fr
     bright to dark); these temporal <
     spatial variabilities in plume visi
      ity were documented in our am
     sis of power plant plumes. Preli
      nary simulations of the power pi
      plume visual  effects  with
      PLUVUE  II  model tend to supp
      our experimental results.

-------
      Christian Seigneur.  A.  B.  Hudischewskyj, and H.  Hogo are  with  Systems
       Applications, Inc.. San Rafael, CA 94903.
      William Conner is the EPA Project Officer (see below).
      The complete report,  entitled "Temporal and Spatial Variability of the Visual
       Effects of Stack Plumes," (Order No. PB 85-200 020/AS; Cost: $8.50, subject to
       change) will be available only from:
             National Technical Information Service
             5285 Port Royal Road
             Springfield, VA 22161
              Telephone: 703-487-4650
      The EPA Project Officer can be  contacted at:
             Atmospheric Sciences Research Laboratory
              U.S. Environmental Protection Agency
             Research Triangle Park, NC 27711
                                      a U.S. GOVERNMENT PRINTING OFFICE: 1985-55M16/27074
United States
Environmental Protection
Agency
                           Center for Environmental Research
                           Information
                           Cincinnati OH 45268
Official Business
Penalty for Private Use $300
OCOC329

   S
                      PS
                        PROTECTION  AGENCY

-------