&EPA
                                   United States
                                   Environmental Protection
                                   Agency
                                   Industrial Environmental Researc
                                   Laboratory
                                   Research Triangle Park NC 2771"
                                   Research and Development
                                  EPA-600/S7-81-025  July 1981
Project  Summary
                                   Environmental  Aspects  of
                                   Synfuel  Utilization
                                  M. Ghassemi and R. Iyer
                                    This study reviews the environ-
                                  mental concerns relating to the distri-
                                  bution, handling, and end use of
                                  synfuel products likely to enter the
                                  marketplace by the year 2000, and
                                  assigns priority rankings to these
                                  products  based on environmental
                                  concerns to aid EPA in focusing its
                                  regulatory and research activities.
                                  Major products and by-products from
                                  oil shale, coal liquefaction, and  coal
                                  gasification technologies are consid-
                                  ered.
                                    Based on current developmental
                                  activities, three likely scenarios for
                                  shale- and coal-based synfuel plant
                                  buildup  are projected. The type and
                                  quantity of synfuel products and by-
                                  products likely to enter the market are
                                  identified  and their regional market
                                  penetration is estimated. The environ-
                                  mental analysis consists of a review of
                                  the available data on the  physical,
                                  chemical, and health effects charac-
                                  teristics of synfuel products and envi-
                                  ronmental significance of their char-
                                  acteristics; an analysis of the potential
                                  environmental impacts and regional
                                  implications associated with the  pro-
                                  duction and use scenarios considered;
                                  and a ranking of the products from the
                                  standpoint of environmental concerns
                                  and mitigation requirements.
                                   The results indicate that: (1) signifi-
                                  cant quantities of synfuel products are
                                  expected to enter the marketplace
                                  during the next 20 years; (2) large-
                                  scale transportation, distribution, and
                                  end use of pertain synfuel products
                                  can present significiant threats to the
                                  environment and the public health; (3)
                                  based on gross characteristics, synfuel
                                  products appear to be similar to petro-
                                  leum products, but detailed character-
                                  ization data are not available with
                                  which to judge  their relative safety;
                                  and (4) synfuel test and evaluation
                                  programs currently underway or plan-
                                  ned provide excellent opportunities
                                  for collecting some of the required
                                  environmental data.
                                    This Project Summary was devel-
                                  oped by EPA's Industrial Environmen-
                                  tal Research Laboratory, Research Tri
                                  angle Park, NC, to announce key
                                  findings of the research project that is
                                  fully documented in a separate report
                                  of the same title (see Project Report
                                  ordering information at back).

                                  Introduction
                                    The present study consists of: (1) a
                                  projection of synfuel production and
                                  product utilization over the next 20
                                  years, and (2) a ranking of products from
                                  the standpoint of environmental con-
                                  cerns. The data base used consists of
                                  information obtained from major process
                                  developers, potential product users, and
                                  published literature.

                                  Candidate Technologies and
                                  Products
                                    Synfuel technologies likely to be used
                                  in commercial plants over the next 20
                                  years are oil shale,  coal, gasification
                                  (low-/medium-Btu and SNG) and coal
                                  liquefaction (direct and indirect). Brief
                                  descriptions of these technologies and
                                  their development status are presented

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in Table 1. Major products and by-products
of these technologies and their antici-
pated general uses are indicated in
Figure 1.

Synfuel Energy Buildup
Scenarios
  Three scenarios or forecasts for synf uel
industry buildup to the year 2000 were
developed. These scenarios are:
  • National goal scenario driven by
     federal incentives (Scenario I;
     medium buildup rate).
  • Nominal production scenario (Sce-
     nario II; low buildup rate).
  • Accelerated production scenario
     representing an  upper bound for
     industry buildup (Scenario III; high
     buildup rate).
  The scenarios project the total quanti-
ties of shale oil, low-/medium-Btu gas,
high-btu gas, and liquids from coal that
would be expected to enter the market
under the assumed sets of conditions.
Based on discussions with major synfuel
suppliers and  users and  industry  and
government planners. Scenario II was
selected  as the most realistic of the
three scenarios and was used for anal-
ysis of regional  impacts and  environ-
mental issues. This scenario is consist-
ent with the general consensus among
technical experts and potential major
suppliers that  shale oil is most nearly
cost competitive and closest  to com-
                          mercialization than high-Btu gasifica-
                          tion or coal liquefaction, and that com-
                          mercial coal liquefaction facilities will
                          not probably come on-line before the
                          early 1990's.
                            Table 2 presents the product/by-
                          product estimates of synfuel utilization
                          in the U.S.
                            Note that, even though on a national
                          scale, projected synfuel utilization would
                          account for small fractions of the total
                          product usage, in some regions a very
                          high fraction  of the  currently used
                          products are expected to be replaced by
                          synfuel products.

                          Synfuel Product Utilization and
                          EPA Regions of Maximum
                          Impact
                            EPA regions where synfuel products
                          would most likely be utilized are identi-
                          fied in Figure 2. Except for oil shale in
                          the  1988-1992 and 1993-2000 time
                          frames and for direct coal liquefaction in
                          the 1993-2000 time period, the trans-
                          portation, distribution, and use of prod-
                          ucts are expected to be confined to the
                          regions where each synfuel is produced.
                          Consequently, environmental impacts
                          associated with  product utilization are
                          expected to be  confined primarily to the
                          production regions, except for impacts
                          associated with the natural transporta-
                          tion  of pollutants across regional
                          boundaries (for example, transportation
Table 1.     Candidate Synfuel Technologies and Their Status of Development

  Technology                            Description
                 of air pollutants emitted from combustion
                 sources). The  projections indicate that
                 up to the year 2000 under Scenario II,
                 the environmental impacts of synfuel
                 product utilization would be expected to
                 be largely limited to EPA Regions V and
                 VIII for oil shale; to EPA Regions IV, VI,
                 and VIII for medium-Btu gas; to EPA
                 Regions III, IV, and VIII for indirect coal
                 liquefaction products; and to EPA Regions
                 III,  IV,  and V for  direct liquefaction
                 products.

                 Environmentally Significant
                 Characteristics of Synfuel
                 Products
                   The current product characterization
                 data base is  a collection of  results  of
                 sampling, analysis and performance
                 testing  conducted  by different investi-
                 gators using samples/batches of products
                 obtained from pilot plants operated under
                 varying  conditions.  Accordingly, sig-
                 nificant inconsistencies exist in the
                 reported results, which further hamper
                 assessment of the environmental safety
                 of synfuel product utilization. This
                 assessment is also hindered by a lack of
                 data on  analogous petroleum and nat-
                 ural gas products that the synfuel
                 products will  replace and that, because
                 of their large-scale and widespread
                 utilization, have generally come to be
                 viewed by the public as environmentally
                 innocuous.
                                                                      Development Status
 Oil Shale
 Direct Coal
 Liquefaction
 Indirect Coal
 Liquefaction
 Coal
 Gasification
• Heating oil shale to about 480° C to extract shale oil
• Heating by surface retorting, in-situ retorting.
  or modified in-situ retorting
• Crude shale oil can be upgraded to produce syncrude for
  use as refinery feed stocks or boiler fuel

• Coal, hydrogen, and a coal-derived liquid mixed at high
  temperature and pressure to produce additional coal-derived
  oil, which is separated and refined to liquid fuels
• Three major processes under development: SCR II, H-coal,
  and Exxon Donor Solvent (EDS). Processes differ in the way
  hydrogen is made to react with coal
• Coal reacted with oxygen and steam in a gasifier to produce
  a synthesis gas; after removal of COt and other impurities,
  CO and Hi in the gas reacted catatytica/ly to produce several
  products ranging from lightweight gases to heavy fuel oil
  (Fischer-Tropschprocessj or to methanol which is then con-
  verted to gasoline (Mobile-M process)
• Closest to commercialization of all synfuel technologies
  for production of large volumes of liquid fuels
• Surface retorting more advanced than in-situ retorting
• All technologies demonstrated at pilot scale or larger
• Several production facilities planned for operation in 1980's

• SRC II: Pilot plant under operation; 6700-ton/day of coal
  demonstration unit under design and scheduled for operation
  in 1984-85
• H-Coal; 600-ton/day of coal pilot plant under construction;
  testing to begin soon
• EDS: 250-ton/day of coal pilot unit under construction;
  testing to begin soon

• Fischer- Tropsch: 8000-ton/day of coal plant (SASOL I) produc-
  ing over 10.000 bbl/day of liquids in commercial operation
  since 1956 in South Africa; a 40,OOO-ton/day of coal unit
  (SASOL-H) will begin operation soon
• Mobil-M: Commercial plant to produce 12.500 bbl/day of gasoline
  from reformed natural gas planned for New Zealand in 1984-85
  Reacting coal, steam, and air/oxygen to produce low-Btu (80-150 • Low-Btu gas: Extensive commercial experience in U.S. with
  Btu/scfl or medium-Btu (300-500 Btu/scf) gas; medium-Btu gas    gasifiers operating near atmospheric pressure; applications are
                                                       small-scale operations producing gas for captive use in
                                                       industrial and process heating
                                                     • Medium-Btu gas: extensive commercial experience exists for
                                                       Lurgi fixed-bed process; several projects using the Texaco
                                                       process for captive applications (chemical feedstocks and
                                                       on-site power generation) in planning and design stages
                                                     • High-Btu gas: plans for SNG production using Lurgi technology
                                                       announced by pipeline and gas utility companies	
                   purified and upgraded to SNG (-1000 Btu/scf)
                  > Gasifiers differ in design and operation, depending on type
                   of coal used and products desired

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                             Oil Shale
                             Products
          Major Synfuel Products/
                By-Products

                      Indirect Coal
                      Liquefaction
                        Products
Coal Gasification
    Products
       Coal
   Liquefaction
     (Direct &
     Indirect
    Processes)
                                                Directo Coal
                                                Liquefaction
                                                  Products
Transportation
   Sector
                                                          • Gasoline
                                                          • Middle
                                                            Distillates
                                                            (e.g.. Jet Fuel,
                                                            Diesel,
                                                            Kerosene)
                                                          • SNG
                                                          • Methanol
                                                          • Petro-
                                                            chemicals
                                     • Middle
                                       Distillates (e.g..
                                       Jet Fuel, Diesel,
                                       Kerosene}
                                     • Residuals
                                       (e.g.. Marine
                                       Fuels,
                                       Lubricants)
                                     • Naphtha
                                     • LPG
                                     • Petro-
                                       chemicals
                                                             Industrial
                                                               Sector
• Gasoline
• Middle
  Distillates
  (e.g.. Jet Fuel,
  Diesel,
  Kerosene,
  Light Fuel Oil)
• Residuals
  (e.g.. Marine
  Fuels,
  Lubricants)
 • SNG
 • Low and
   Medium
   Btu Gas
Penetration of Shale Oil into the Utilities and
Commercial and Residential sector is expected
to be minimal and therefore not highlighted.
                                                            Commercial
                                                             Residential
                                                               Sector
 Figure 1.    Synfuel utilization during 1985-2000.
  Table 3 identifies the differences in
chemical, combustion, and health effects
characteristics of synfuel products and
their petroleum analogs, based on the
reported characterization data. These
differences primarily relate to the higher
content of aromatics and fuel bound
nitrogen (FBN) and greater emissions of
NOx during combustion. Although no
test data for synfuel products are avail-
able, high concentrations of aromatics
in fuels have been shown to enhance
production of PNA's during combustion.
In the case of fuels, high aromaticity has
been generally implicated in an increase
in smoke  production; the limited com-
bustion data which are currently avail-
able, however, do not  indicate that all
aromatic synfuels have higher smoke
levels.  High FBN content can raise the
    level of NO. emissions; the excess NO,
    emissions of synfuels are believed to be
    correctable by combustion modifications.
    The nitrogen content of the synfuels can
    also be lowered to meet appropriate fuel
    specifications by the use of certain
    refining processes.
      The data in Table 3  identify two
    products as highly hazardous because
    of mutagenic, tumorigenic, and cytotoxic
    properties. These are crude shale oil
    and fuel oils  from coal liquefaction
    processes. These hazardous properties,
    which are characteristic of high boiling
    and tarry coal and petroleum materials,
    are caused by the presence of substances
    or classes of substances such as poly-
    cyclic aromatic hydrocarbons,  hetero-
    and carbonyl-polycyclic compounds,
    aromatic amines, and certain inorganics
                                         (for example, arsenic in crude shale oil).
                                           In general, synfuel product charact-
                                         eristics that cause environmental con-
                                         cern in any wide-scale  utilization sce-
                                         nario relate to  the known or potential
                                         presence of toxic substances (including
                                         carcinogenic compounds associated
                                         with crude shale oil and heavy distillates
                                         from coal liquefaction and hazardous aro-
                                         matics), fuel-bound nitrogen, volatile
                                         components, and minor and trace ele-
                                         ments. Potential environmental concerns
                                         relating to anticipated product uses
                                         generally fall  into  three  categories:
                                         occupational exposure, public exposure,
                                         and  general environmental pollution.
                                         The occupational hazards affect workers
                                         manufacturing  and  using the products
                                         and personnel involved in facility main-
                                         tenance and  product distribution

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Table 2. Estimated Quantity of Synfuel Products used in the U.S. Under Scenario II
1980-1987 1988-1992
Product Amount % of total Amount % of total
(10*bpd) in U. S. (W6 bpd) in U. S.
Crude shale oil (fuel)
Shale oil refinery feed
Shale jet fuel
Shale diesel fuel
Shale residuals
Shale gasoline
Medium-Btu gas (coal)
SNG (coal)
Gasifier tars, oils
Gasifier phenol
F-TLPG
F-T medium-Btu gas
F-T SNG
F-T heavy fuel oil
F-T gasoline
Mobil-gasoline
F-T diesel fuel
Fuel methanol
SRC II fuel oil
SRC II naphtha
SRC II LPG
EDS fuel oil
EDS naphtha
EDS LPG
H-coal fuel oil
H-coal naphtha
H-coal LPG
0.0008
0.07
0.015
0.042
0.007
0.13
0.09
0.042
0.004
0.004
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0.05
0.45
1.2
1.2
0.2
0.2
0.9
0.4
0.04
0.04
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0.41
0.09
0.23
0.04
0.07
0.27
0.17
0.01
0.01
0.01
0.01
0.03
0.001
0.02
0.05
0.002
0.14
0.03
0.02
0.006
0
0
0
0
0
0
0
0.24
6.5
6.5
1.3
0.9
2.8
1.8
0.1
0.1
0.06
0.06
0.33
0.02
0.2
0.66
0.04
1.8
0.3
0.2
0.4
0
0
0
0
0
0
1993-2000
Amount % of total
(106bpd) in U.S.
0
0.43
0.09
0.23
0.04
0
0.45
0.25
0.01
0.02
0.01
0.01
0.07
0.001
0.03
0.1
0.01
0.23
0.09
0.05
0.02
0.06
0.03
0.01
0.06
0.03
0.01
0
2.4
6.8
6.8
1.3
0
4.7
2.6
0.1
0.2
0.06
0.1
0.7
0.03
0.4
1.3
0.1
3.0
1.3
0.8
1.6
1.0
0.6
0.9
0.4
0.2
0.1
services.  Public exposure primarily
relates to air pollution resulting from
product uses such as the use of gasoline
in automobilies, hazardous fugitive
emissions from storage tanks and prod-
uct transfer points,  and accidental
spills. In the general category of envi-
ronmental pollution, major contributors
would include accidental spills, sludges
from product storage tanks and spill
cleanup, and solid,  liquid,  and gaseous
wastes associated with combustion and
combustion-related  air pollution control.

Basis for Priority Ranking of
Synfuel Products
  As noted previously, the objective of
the study was to provide input to the
EPA effort for: (1) assessing the envi-
ronmental implications  of a mature
synfuel industry and of large-scale
utilization of synfuel products; and (2)
planning and prioritizing regulatory and
research and development programs.
Accordingly, a system was developed
and used to rank the synfuel products
from the standpoint of environmental
concerns and to identify those products
and areas of concern that should receive
more immediate and greater regulatory
and R&D attention. The ranking is
subject to the limitations of the existing
product characterization data and the
assumptions used in developing the
productions and use scenarios; the
product rankings will most likely change
as more data become available, especially
for those products for which little or no
data are currently available. It should
also be noted that the specific approach
used  represents only one of many
approaches that could be used to rank
synfuel products from the standpoint of
environmental concerns.
  Two approaches were examined for
ranking the synfuel products, based on:
(1) the limited product characterization
data currently available (Table 3) sup-
plemented by engineering judgement
where appropriate; and (2) the premise
that, in the absence of detailed charac-
terization data, and unless the available
data indicate otherwise, it would be
reasonable to assume that a synfuel
product would be more hazardous than
its petroleum analog. The first approach
was selected and used to develop prod-
uct rankings.
  Under this approach, a synfuel prod-
uct would necessarily be considered
more hazardus because of the mere lack
of detailed characterization data. Instead,
assignment of a more positive ranking
to a product is supported by actual data
or is based on strong indications of
greater potential  hazards. Under the
first scenario, prioritization of regulatory
and R&D activities does not have to
await  collection of additional data,
which should proceed concurrently as a
separate effort.

Attribute Rating Procedure
  Table 4 presents the assessment of
the environmental concerns for various
synfuel products relative to their petro-
leum analogs on a "barrel-per-barrel"
basis. As indicated by the headings in

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                                 Shale Oil
                                 Low-/Medium-Btu Gas
                                 Indirect Coal Liquefaction
                             Shale Oil
                             Indirect Coal Liquefaction
                             Direct Coal Liquefaction
                                                                                             Indirect Coal Liquefaction
                                                                                                    Coal Liquefaction

                                                                                                 Region II
                                                                                           Puerto Rico
       Low-/Medium-Btu Gas
       Direct Coal Liquefaction
       Indirect Coal Liquefaction
                                                          Virgin Islands

                                                ,Low-/Medium-Btu Gas
                                                Direct Coal Liquefaction
Figure 2.    EPA Regions of synfuel products utilization (1990'sj.
the table, the relative ranking considers
potential for  exposure, emission, toxic
hazard, cost of control, and adequacy of
existing regulations. A(+) ranking is
assigned to a product for .an environ-
mental attribute if the product is judged
to present greater environmental con-
cern than the petroleum analog;  a
ranking of (0) indicates that the environ-
mental concern would be similar to or
less than that of the petroleum product.

Product Ranking
  Table 5 presents the results of synfuel
product ranking. The  results generally
indicate the greatest  level of environ-
mental concern  and regulatory  re-
quirements for shale  oil refinery feed
and  coal liquids. These liquids have
been demonstrated to be more hazard-
ous than petroleum crude and fuels oils
(a major factor in assigning a "1"
ranking). This and the fact that shale oil
products will  be the synfuels that  are
expected to first enter the market on a
large scale, are the major factors that
flag near-term environmental concerns
for shale oil-products  in general and
shale oil  fuel and refinery feed  in
particular.

Data Limitations and Related
Programs
  As noted  previously, a number  of
major gaps in the existing data base
preclude accurate analysis of the envi-
ronmental concerns associated with a
future large-scale utilization  of synfuel
products in the U.S. These gaps relate
to: (1) present uncertainties regarding
the size of the industry, specific synfuel
technologies that will be used, product
slates that will be produced, locations of
production facilities and product distri-
bution systems, and the specific areas
of synfuel  use; and (2) lack of adequate
characterization data on synfuel prod-
ucts  and on the analogous petroleum
products that they will partially or totally
replace.
  At present, the first category of data
gaps can only be partially filled. Many of
the gaps in the second category, how-
ever, can and  should be filled through
testing and evaluation of synfuel products
obtained from  existing U.S. pilot plants
and commercial facilities abroad.

Conclusions
  • In the next 20  years  significant
    quantities of synfuel products are
    expected to enter the marketplace
    and in certain regions a very high
    percent of the currently used prod-
    ucts will be replaced by their synfuel-
    derived analogs.
  • Based on gross characteristics,
    synfuel products appear to be simi-
    lar to  petroleum products,  but
    detailed characterization data are
    not available for many of the synfuel
    and petroleum products with which

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Table 3.    Reported Known Differences in Chemical, Combustion, and Health Effects Characteristics of Synfuel Products and
            Their Petroleum Analogs
 Product                       Chemical Characteristics       Combustion Characteristics      Health Effects Characteristics
 Shale oil
  Crude

  Gasoline
  Jet fuels

  DFM

  Residuals
 Direct Liquefaction
  Syncrude (H-Coal,
  SRC II. EDS)
  SRC II fuel oil
 H-Coal fuel oil

 EDS fuel oil
 SRC II naphtha

 H-Coal naphtha
 EDS naphtha
 SRC II gasoline
 H-Coal gasoline
 EDS gasoline
Indirect Liquefaction
 FT gasoline
 FT by-product
 chemical
 Mobile-M gasoline

 Methanol
Gasification
 SNG

 Low/medium-Btu gas
  Gasifier tars, oils
  phenols
Higher aromatics, FBNAs, Hg. Mn   Higher emissions of NO* paniculate, and    More mutagenic, tumorigenic, cytotoxic
Higher aromatics
Higher aromatics

Higher aromatics

Higher aromatics

Higher aromatics and nitrogen

Higher aromatics and nitrogen
Higher nitrogen content
Higher nitrogen, aromatics

Higher nitrogen, aromatics
Higher nitrogen, aromatics
Higher aromatics
Higher aromatics
Higher aromatics

Lower aromatics; N and S nil
(Gross characteristics similar
to petroleum gasoline)
Traces of metal carbonyls
and higher CO
(Composition varies with coal
type and gasifier design/
operation)
(Composition varies with coal
and gasifier types; highly
aromatic materials)
(possibly) certain trace elements
Slightly higher No, and smoke emissions
Slightly higher No* and smoke emissions

Slightly higher NO, and smoke emissions
                                                            Higher NO, emissions
Higher No, emissions

Higher No, emissions
                               N/A
                               Higher aldehyde emissions
(Emissions of a wide range of trace and
minor elements and heterocyclic organics)
Eye/skin irritation, skin sensitization
same as for petroleum fuel
Eye/skin irritation, skin sensitization
same as for petroleum fuel
Middle distillates: non-mutagenic; cytotoxi-
city similar to but toxicity greater than
No. 2 diesel fuel; burns skin.
Heavy distillate: considerable skin carcin-
ogenicity, cytotoxicity, mutagenicity, and
cell transformation
Severely hydrotreated: non-mutagenic, non-
tumorigenic; low cytotoxicity

Non-mutagenic, extremely low tumorigeni-
city, cytotoxicity, and fetotoxicity
Non-mutagenic
                                     Non-carcinogenic
                                                                   Affects optic nerve
Non-mutagenic, moderately cytotoxic
     to assess and compare their safety.
     Large-scale  transportation,  distri-
     bution,  and end use of certain
     synfuel products (for example,
     heavy distillates derived from coal
     liquids and shale oil) can present
     significant threats to the environ-
     ment and the public health.
    ' Essentially all synfuel-related envi-
     ronmental projects that are planned
     or currently underway relate to the
     design and  operation of synfuel
     plants and not to the subsequent
                     distribution and utilization of prod-
                     ucts. The present study constitutes
                     the first attempt to focus attention
                     on the potentially broad and far-
                     reaching environmental implica-
                     tions of large-scale marketing and
                     utilization of synfuel  products.
                     A number of major test and evalua-
                     tion programs are planned or cur-
                     rently underway to assess the
                     combustion characteristics and
                     general performance of synfuels
                     relative to those of petroleum prod-
                                    ucts. These  programs provide ex-
                                    cellent opportunities for collecting
                                    the environmental data needed for
                                    assessing the relative safety of
                                    synfuel products, determining the
                                    adequacy of the existing control
                                    technologies, and identifying regu-
                                    latory needs.
                               Recommendations
                                 Based on the results and conclusions
                               of the study, the following recommenda-
                               tions are offered:

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Table 4. Relative Assessment of the Environmental Hazards Associated with Synfuel Products and Petroleum Analogs
Emission Toxic Adequacy of
Product Exposure Factor Hazard Existing Regulations
Transport
&
Storage End Use
Crude shale oil (fuel)
Shale oil refinery feed
Shale jet fuel
Shale diesel fuel
Shale residuals
Shale gasoline
0
0
0
0
Low-/Medium-Btu gas (coal) 0
SNG (coal)
Gasifier tars and oil
Gasifier phenol
F-T LPG
F-T medium-Btu gas
F-T SNG
F- T heavy fuel oil
F-T gasoline
M-gasoline
F-T diesel fuel
Fuel methanol
SRC II fuel oil
SRC II naphtha
SRC II LPG
EDS fuel oil
EDS naphtha
EDS LPG
H-coal fuel oil
H-coal naphtha
H-coal LPG
0
0
0
0
0
0
0
0
0
0

+
0
0
+
0
0
+
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
Transport
&
Storage End Use
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
+
0
+
+
0
0
0
0
0
0
0
+
+
0
0
+
0
0
+
0
0
Transport
&
Storage End Use
0
0
0
+
0
+
+
0
0
0
0
0
0
0
0
+
+
0
+
+
0
+
+
0
1
+
0
+
+
0
0
0
0
0
0
0
0
+
+
0
+
+
0
+
+
0
Cosf of
Control
0
+
0
+
0
0
0
0
+
0
0
0
0
+
0
0
+
0
0
+
0
0
c/w
0
+
0
+
0
0
0
0
0
0
0
0
+
+
0
0
+
0
0
+
0
0
CWA
0
0
0
0
0
+
0
0
0
0
0
0
0
0
0
+
+
0
+
+
0
+
+
0
RCRA
+
+
0
+
0
0
0
0
+
+
+
+
+
+
+
0
+
+
0
+
+
0
TSCA
0
0
0
0
0
0
0
0
o
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
> More  systematic approach to
 product characterization and
 testing.Better coordination among
 various on-going and planned stud-
 ies (perhaps through establishing a
 "test tracking" system that would
 promote exchanges of information
 among various studies) is recom-
 mended to avoid duplication of
 effort and to ensure generation of
 appropriate environmental data in
 a most cost-effective manner.
 Collection of environmental data in
 conjunction with planned perform-
 ance testing programs. Collection
 of environmental data, which can
 be correlated with performance,
 which  can  be correlated in con-
 junction with product performance,
 in conjunction with a systematic
 product characterization effort can
 provide valuable timely inputs to
 the evolution of the synfuel industry
and would ensure that: (1) envi-
ronmental  considerations  are in-
cluded in the selection of processes,
equipment, and product slates for
commercial facilities;  and (2) the
drafting of specifications for synfuel
products, new source performance
standards for synfuel  plants,  and
emissions standards for facilities
using synfuel products is based on
the best available technical  and
engineering data.
Consideration of end-use environ-
mental implications in the selection
of the product  slates and in the
development of the synfuel industry.
By proper selection of the refining
steps (and the operating mode for
some synfuel processes), the prod-
uct slate can be altered to favor the
production  of those products that
present fewer and more controllable
end-use  environmental impacts.
 Studies should be undertaken to
 define the engineering and eco-
 nomics of selecting environmentally
 acceptable product slate possibili-
 ties for various synfuel technologies.
i Compilation of characterization/
 performance data on analogous
 petroleum products. Very little data
 are available on potential pollutants
 and  toxicological and  ecological
 properites of many of the petro-
 leum products to provide a baseline
 for assessing  the safety of synfuel
 products. It is recommended that
 the potential sources of data on
 petroleum products be contacted in
 an effort to compile all available
 data and identify data gaps. Also,
 synfuel product testing and char-
 acterization efforts should include
 parallel testing  of  petroleum-
 derived analogs.

-------
Table 5. Priority Ranking of Synfuel Products
Environmental Concerns*
Product 1980-1987
Crude shale oil (fuel)
Shale oil refinery feed
Shale jet fuel
Shale diesel fuel
Shale residuals
Shale gasoline
Medium-Btu gas (coal)
SNG (coal)
Gasifier tars & oils
Gasifier phenol
F-TLPG
F- T medium-Btu gas
F-TSNG
F-T heavy fuel oil
F-T gasoline
Mobile -M gasoline
F-T diesel fuel
Fuel methanol
SRC II fuel oil
SRC II naphtha
SRC II LPG
EDS fuel oil
EDS naphtha
EDS LPG
H-coal fuel oil
H-coal naphtha
H-coal LPG
2
1
2
2
2
2
2
3
—
2
—
—
—
—
—
—
—
—
—
—
—
—
—
—
—
—
—
from the Standpoint of
1988-1992 1993-2000
—
/
2
2
2
2
2
3
;
2
3
3
3
3
3
3
3
/
7
2
3
—
—
—
—
—
—
—
7
2
2
2
2
/
3
7
2
3
3
3
3
3
3
3
/
7
2
2
/
2
3
7
2
3
*Degree of concern: most = 7, modest= 2, and low- 3;—indicates product not produced
 or not used as indicated
                                          M. Ghassemi and R. Iyer are with TRW, Inc., Redondo Beach, CA 90278.
                                          J. McSorley is the EPA  Project Officer (see below).
                                          The complete report, entitled "Environmental Aspects of Synfuel Utilization,"
                                            (Order No. PB 81-175 937; Cost: $29.00, subject to change) will be available
                                            only from:
                                                  National Technical Information Service
                                                  5285 Port Royal Road
                                                  Springfield. VA 22161
                                                  Telephone:  703-487-4650
                                          The EPA Project Officer can be contacted at:
                                                  Industrial Environmental Research Laboratory
                                                  U.S. Environmental Protection Agency
                                                  Research Triangle Park, NC 27711
                                                                                   IU. OOVBmMCMr FHHTMO Omce m-797'0 U/7219

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