United States
                  Environmental Protection
                  Agency          	
Air and Energy Engineering    •
Research Laboratory         "
Research Triangle Park NC 27711
                  Research and Development
EPA/600/S9-88/009 May 1988
&EPA         Project Summary
                   Findings of  the
                   Chlorofluorocarbon  Chemical
                   Substitutes  International
                   Committee
                   Thomas P. Nelson
                    This report presents the findings
                  of a select international committee of
                  experts from industry and  acedemia
                  on  the  subject  of  chemical
                  substitutes  for fully halogenated
                  chlorofluorocarbons (CFCs). This
                  committee,  over the course of two
                  meetings, reviewed  and discussed
                  data and information on  chemical
                  alternatives  for fully halogenated
                  CFCs now in use.  Also, committee
                  members prepared  brief reports
                  highlighting  specific areas  of
                  concern.
                    FC-134a was identified as having
                  the greatest current potential  for
                  replacing CFC-12;  similarly, CFC-
                  123 could  replace  CFC-11. The
                  committee acknowledged that, while
                  there are  many other  possible
                  chemical replacements, there is a
                  dearth  of  information on these
                  compounds with  regard to property
                  data, toxicity,  and  performance in
                  end-use  applications.
                    Investigation of new chemicals to
                  serve  as  backup  candidate
                  substitutes  if FC-134a and  CFC-123
                  fall short  of expectations was
                  strongly  recommended.  Such  in-
                  vestigations  should  include a
                  preliminary  screening of chemical,
                  physical, and thermodynamic prop-
                  erties; acute  toxicity;  and likely
                  atmospheric fate. Finally, several new
                  chemicals  were suggested  for
                  examination.
                      This  Project  Summary was
                  developed by EPA's Air  and Energy
 Engineering Research Laboratory,
 Research Triangle Park, NC, to an-
 nounce key findings of the research
 project that is fully documented in a
 separate report of the same title (see
 Project Report ordering information at
 back).

 Introduction
   A family of chemicals  known  as
 chlorofluorocarbons  (CFCs) has  been
 implicated in the depletion of the earth's
 stratospheric ozone layer. A number of
 adverse health and  ecological effects
 could result from such depletion. For this
 reason a number of strategies or options
 for controlling the atmospheric release of
 these compounds are being evaluated by
 governments and  industries  worldwide
 One promising  approach appears  to be
 the substitution  of new, low-ozone-
 depleting CFCs  for those  currently
 employed in a wide variety of end uses.
 There is  a  need, however,  to better
 define the requirements for  developing
 and  bringing  to  market  these new
 substitutes. To  this end, a committee of
 authorities of CFC  chemistry, production,
 toxicology,  and  marketing  was  as-
 sembled to ascertain  the  degree of
 promise of this  approach and what steps
 must  be  taken by   industry and
 government to achieve  such  substitution
 in the most efficient and timely manner.
   The overall objective  of the committee
 was to  comment  on the commercial-
 ization potential of newer CFC chemical
 substitutes  for the suspect  ozone
 depleting  chemicals: CFC-11 (tri-

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chlorofluoromethane),  -12  (dichloro-
difluoromethane),  and  -113  (1,1,2-
trichloro-1,2,2-tnfluoroethane).  Specific
objectives included:
•  Identify the  most  promising  newer
   CFC chemical substitutes;
•  Estimate cost, quantities of chemicals
   required, and time for toxicity testing,
   application testing,  and commercial-
   ization of these substitutes;
•  Specify necessary  market and price
   preconditions for commercialization;
•  Recommend  research  and develop-
   ment  tasks  to  assist commercial-
   ization; and
•  Suggest  possible  communications
   between CFC producers and potential
   users regarding research activities.
These objectives were to be addressed
by developing consensus opinions of the
committee members.
   The CFC Chemical Substitutes Inter-
national Committee met twice. At the first
meeting  committee members  became
more familiar  with the CFC  environ-
mental issues through  direct discussions
with U.S.  EPA  officials.  Also,  the
committee  formulated their  initial
thoughts  on additional  CFC chemical
substitutes, costs, toxicology, and com-
mercialization potentials.
   The second meeting, a workshop, was
primarily  to complete the definition of the
issues and  organize  an approach  to
addressing  the issues. Based on  results
of the first meeting, the second meeting
also included interactions with CFC users
from industry.  CFC users represented
were automobile  air  conditioning,
refrigeration  and air conditioning,  and
foam  insulation board.  In addition,  F.
Sherwood  Rowland  (University  of
California-Irvine), one  of the originators
of the  ozone depletion  theory,  gave a
presentation of  atmospheric chemistry
that focused on current  knowledge  of
stratospheric  chemistry and  ozone
depletion  potential  of newer CFC
chemical substitutes.
   Deliberations of the committee were
summarized as a formal press  release
and as a joint EPA/Committee Statement.
Also, individual  panel  members  drafted
brief reports on  specific aspects of the
issues.
Accomplishments/Results
(Condensed  from  Executive  Sum-
mary  of Committee  Findings,  by
Richard Lagow,  Committee Chair-
man)
   The  most important findings of this
panel  were that FC-134a  was the
primary replacement  candidate  for
CFC-12,  and  CFC-123  was  the
primary  replacement candidate  for
CFC-11. The  committee advocated
incentives for  increasing the  use  of
CFC-22 in refrigeration  markets  and
other  applications.  Also recommended
was a strong conservation  and recycling
program for CFC-113 which is of key
importance as a  solvent in cleaning
applications in  the electronics  industry
and for metal cleaning applications  The
committee identified many other potential
substitutes  and  recommended further
research on these materials.
   Of  the  many barriers  and potential
barriers to availability of appropriate
quantities of alternative CFC  and fluoro-
carbon compounds, the committee  con-
cluded that the most  basic was the lack
of a worldwide  market for such materials.
Such  a market can only be  created by
government regulations  worldwide  to
create a demand for such materials. Note
that the chemical manufacturing  process
(Swarts reaction and improved versions)
producing  the  currently marketed CFCs
delivers these  products  at such a low
price  ($1.30-$1,75'kg)  that  the  per-
formance/cost  ratio  for  a  variety  of
applications is  among the  highest known
for commercial chemicals. This accounts
for their extraordinarily large market and
widespread use even in applications for
which they are  not unique.
   The essentially nonflammable  and
nontoxic  characteristics at  $1.30-
$1.75/kg, which are primary reasons for
use in many  applications,  cannot be
duplicated  at  that price. This  price
follows  from  the fact that very  in-
expensive  hydrogen fluoride  and chlor-
ocarbons (from petrochemical feedstock
and inexpensive chlorine  gas  derived
through  chloro-alkali  chemistry  of
sodium chloride) are primary feedstocks.
The committee noted that there would be
a very small market or no  market for
performance-effective new materials  at
even  a  price  as  low   as  $2 00/lb
($4.40/kg)
   The committee recommends  that
governments around  the  world  institute
regulations which would make such new
CFC alternative chemicals economically
viable and  establish  a  market  with
suitable  incentive for the chemical
industry worldwide to enter  the market
with  new  compounds   which  have
markedly lower ozone depletion potential
and greenhouse gas effects While some
criticism has been directed toward U.S.
chemical companies along the lines that
it  would be  unlikely that they would
develop and  market such alternatives
without regulatory incentives,  in fact, it is
very unlikely  that  users will,  withoi
regulation, be  unilaterally willing to  pM
higher prices, for they are in competitH
situations and  may  not be  able to sac
rifice to become "better world citizens.
The committee identified the factors  tha
influence the commercialization timescali
for  new compounds as well  as  thi
already  known  substitutes such as  FC
134a and  CFC-123.  Probably the  bes
overview is that commercial quantities o
such new materials could be available ii
a minimum of 5 years and a maximum o
10 years. Analyzing each component o
the timing, the committee found that ever
in view  of the  substantial effort  requirec
for research and development and effor
to design and build commercial facilities
or alter existing commercial  facilities, th«
most time-intensive  part of  the  process
of bringing a new material to the marke
was the chronic inhalation toxicity testing
This  phase requires  up  to  4  years  anc
proceeds in the normal  industrial  en
vironment after initial market analysis foi
the  compound  appears  favorable  anc
after acute and subchronic testing comes
to a favorable conclusion.
  In  view  of  the  time  criticalitv
associated with chronic inhalation studies
and  reproductive toxicity studies,  some
member of  the committee favorec
immediate U.S. government funding oj
tier 3 (chronic)  toxicity testing of "pure!
samples of obvious substitute candidates
such as FC-134a and  CFC-123, noting
that  the $3  million cost was very
acceptable  if it could cut 6-12 months
off the timescale for commercialization.
  It was further noted that such  an early
investment  could be very advantageous
in starting  other new materials down the
path  sooner in  the event of tier 3 toxicity
failure  of  such  materials  as FC-134a
and CFC-123.  However,  after  study, the
consensus of the committee was that tier
3 toxicological  testing  should best be
done by individual companies or groups
of chemical  companies testing  together
(for  example,  through   the  Chemical
Manufacturers  Association in  the  U.S.).
Each chemical company would want full
control of the toxicological  testing,
because they  bear  the financial liability
and  because both the nature and  the
level of impurities in the  product (which
could  also be very  significant  tox-
icologically) vary from chemical company
to chemical company and are sensitive to
their exact  manufacturing process. Rep-
resentatives  of some companies, how-
ever, indicated  that  they  would consider
accepting  government subsidies on the
toxicological  testing  in  exchange  fo|
starting dates earlier  than normally

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 prudent  in their financial  and technical
~ nalysis.
   Most  members of  the  committee
 concluded, with respect to commercial-
 ization  timescales,  that  although
 substantial research  and development
 efforts are in  place  worldwide in the
 chemical industry on alternative materials
 at the present time,  implementation of
 regulations on CFC-11, -12, and  -113
 by governments worldwide would define
 the  zero point on the timescale  Some
 committee  members  felt that  the
 regulatory  strategy and even nuances
 within the regulations would  have  a
 significant effect in determining whether
 the  timescale was more toward the 5 or
 more toward  the 10 year period  for full-
 scale commercialization. Certainly  inter-
 national  agreements  could have major
 impact in either direction.
   With  respect to timing, unfavorable
 toxicological  testing  results  or man-
 ufacturing   problems with  primary
 candidates,  for example  FC-134a  and
 CFC-123,  could  cause  a significant
 delay before  other compounds were in
 place. It  should,  however, be  clearly
 understood that the major reasons the
 committee picked  FC-134a  and CFC-
 123 as  leading candidates is that acute
 testing  for both FC-l34a  and CFC-123
     subchronic (tiers  1 and 2) testing for
FCFC-123 have been completed,  and
 development  work  and several  patents
 for  larger scale (but  not  commercially
 viable)  syntheses  exist  for these
 compounds  This sets them  apart from
 the  bulk of   fluorocarbon, hydrogen-
 containing  fluorocarbon,  and  CFC
 materials considered  by the committee.
 Early analysis  by  the  committee,
 however,  revealed that  the toxicological
 testing  was  such  a time-limiting factor
 that the  increase  in time for selecting a
 material unscreened for toxicology (acute
 and  subchronic) and perhaps  even
 without pilot  plant experience could  be
 as  little as  6-12 months.  As  will  be
 discussed later,  there are almost  no
 toxicological data or technical  per-
 formance property data on many known
 fluorocarbon  materials that would appear
 to  have the  physical  properties  nec-
 essary for use as substitutes.
   A major  contribution  of  this inter-
 national committee has been to identify a
 large number of predominantly fluorine-
 containing  compounds of promise  for
 substitution  in applications of currently
 manufactured CFCs,  particularly CFC-
 11,   -12,  and  -113.  These  com-
 pounds are  listed in  three categories:
I Category A  substitute chemicals are
 primary  candidates chosen  to  facilitate
rapid  implementation  of  alternatives;
Category  B substitute  chemicals are
secondary  candidates  (standby can-
didates),  most of which are hydrogen-
containing  f luoroethanes  and
fluorochloroethanes; and  Category  C
substitute  chemicals are newer,  and  in
some cases novel, compounds. Category
C  has two  subclasses:  a) hydrogen-
containing  fluorocarbons,  and   b)
perfluorocarbons and  their derivatives.
Note that  criteria  for selecting  many  of
the alternative materials were that at least
one hydrogen by  available for attack  by
OH radicals  and/or only  fluorine   be
present as a halogen in the compound. It
was  recognized  that non-hydrogen-
containing materials may  be significant
greenhouse gases.
   Of  primary   importance   is  the
committee finding that  it will be  indeed
possible  to  develop,  at  a moderately
higher to  substantially  higher  cost,
substitutes for  current CFCs if  FC-134a
and CFC-123 fail for  some reason.  As
stated before, these newer materials may
be  only  6-12  months behind  if   all
committee  recommendations  are fol-
lowed. The problem is simply that very
few have been screened even for acute
and subchronic  toxicity  and,  m  most
cases, little more  is  known  of their
physical  properties  than boiling  points
and melting points  Essentially nothing is
known  about, for  example, their refrig-
eration performance or solvent  proper-
ties. In most cases, even basic  thermo-
dynamic  properties  are not known  for
these  new  fluorocarbons.  It should   be
explained that  the  reason that  new
fluorocarbons and CFCs have not been
screened  for application  in the CFC
industry is that producers have known for
years, with respect  to  the   Swarts
technology,  that  their new materials
would not  be  performance-cost  com-
petitive for such applications. Most are
also  manufactured  by processes that
would deliver these  materials at a mini-
mum of $11.00/kg and often up to $45
or  $65/kg
   The committee  listened to   presen-
tations from several user  industry rep-
resentatives and came to the conclusion
that, in most applications, new prices for
substitutes could be borne  effectively  by
the users except  in the very cost-com-
petitive,  flexible, and rigid  foam-blowing
applications where other nonfluorocarbon
materials and  other technology  could
supplant  CFC-11  and -12   It has been
pointed out  that CFC-22 would  be  an
adequate substitute  in rigid foam sheets
but would not have the diffusion  stability
for most  foam  boardstock  applications
The  committee heard from the users  a
strong preference  for FC-134a  (over
CFC-22)  as  a "drop-in"  for  refriger-
ation  applications  (requiring  little
modification of air conditioning  units) for
mobile air  conditioning.  This was  a
particularly  strong  preference of  the
automobile manufacturers. The  commit-
tee  considered  the lack  of a known
lubricating oil (which would probably be a
fluorocarbon in this  instance) compatible
with  FC-134a applications to  be  a
problem likely to find a solution within  6
months by any one of several compa-
nies.
   The committee unanimously  felt that
immediate  strong measures should be
undertaken by all countries to  stimulate
conservation measures  which  lead  to
slower and  lower  volume releases  of
CFCs and believes that accomplishments
can be made in this regard in almost all
applications.
   The committee noted  that the  time-
scale for  implementation  of alternative
chemicals which impact the environment
is 5-8 years,  whereas  significant
reductions  can be  made  immediately
through conservation efforts. In view of
the fact that CFC-113 has application in
a broad spectrum  of  uses and in only
20-30% of these applications is there an
acceptable  alternative,  the committee
favored an approach to continue the use
of CFC-113. Some committee members
felt that industrial  cleaning operations
may  not  make  sufficient  attempts  to
control the emission  of CFC-113
because the price is so low that recovery
is not always economic.  Significant
improvements can be made by upgrad-
ing old cleaning equipment and improv-
ing work practices. Thus, the price could
be  artificially  increased to  make
economically attractive conservation and
recovery  from exhaust systems;  alter-
natively,  one could legislate  against
emissions  (considered less effective).  At
the same time a vigorous  research effort
to synthesize and  develop alternative
chemicals  to replace CFC-113 should
be funded  by the  federal government.
The  committee,  some of  whom  have
consummate knowledge  of  high-per-
formance chemical fittings,  felt that major
advances  could  be made  in  retaining
CFCs  in  mobile  air and other  air
conditioning  applications; and that a cost
for  higher pressure fittings of about
$20-$40  per unit  was very tolerable.
Further, the committee  recommends
strongly economic incentives to expand
the use  of  the  already  commercially
available  CFC-22  (which requires  a
higher operating pressure).

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   The committee  found that  there  is
very little knowledge of the  atmospheric
chemistry of new alternative compounds
other than generalizations which apply to
groups.  The committee has found even
less knowledge concerning  the ultimate
fate in the environment of such species
as  FC-134a. It is  estimated that  hydro-
chloric and  hydrofluoric acids contribute
to acid ram but are orders of magnitude
less significant than sulfunc acid. Little is
known  about the  effect  on  the  at-
mosphere and environment  of  products
such as small concentrations of  tri-
fluoroacetic  acid  or partially fluonnated
acetic  acid  and  if  they   will  be
established, in fact, as breakdown  prod-
ucts.
   The committee  has  determined that it
rs  abso4trtely necessary that  U.S.
government funds  be spent (and funding
encouraged worldwide)  at  a  minimum
level of  $3  million per year to support
research in  the academic, small industry
and industrial sectors  focused   on a
number  of  these  extremely important
problems in areas where knowledge is
essentially  lacking.  Government
         regulations which  were  designed to
         effectively reduce CFC-11  and  -12
         over a period of 10 years will be made at
         very  high risk,  and  "safe"  effective
         alternatives may not be available  on a
         timescale  to meet society's  demands
         without this  relatively  modest funding
         effort   The  most important  research
         needs are.
         • Atmospheric chemistry studies  for
           specific new chemicals  funded  by a
           separate budget within the EPA from
           general atmospheric studies;
         • Synthesizing new  materials to  be
           evaluated for alternative chemical
           applications,
         • Evaluating  properties  of  new
           chemicals for various applications and
           obtaining   basic  thermodynamic
           properties for such materials; and
         • Determining   the     ultimate
           environmental fate of alternative
           fluorocarbon  materials such as  FC-
           134a and CFC-123.
           In general, there is a pressing need to
         evaluate at least 10 or so of the  most
         likely  alternative materials  from  the
         nontraditional areas of CFC   and
             i
             >ri
     Thomas P. Nelson is with Radian Corporation, P.O. Box 9948, Austin TX 78720.
     N. Dean Smith is the EPA Project Officer (see below).
     The  complete report, entitled  "Findings of the  Chlorofluorocarbon Chemical
          Substitutes International  Committee," (Order No.  PB  88-795 664!AS;
          Cost: $19.95, subject to change) will be available only from:
             National Technical Information Service
             5285 Port Royal Road
             Springfield, VA22161
             Telephone: 703-487-4650
     The EPA Project Officer can be contacted at:
             Air and Energy Engineering Research Laboratory
             U.S. Environmental Protection Agency
             Research Triangle Park NC 27711
fluorocarbon chemistry for  application
The  committee  also  strongly  re
ommended that at least 20 of the moi
speculative alternatives be  prepared in
sufficient amounts and purity for acute
and  subchronic  toxicity testing.  It is
further recommended that the committee
replace  yearly any  of those  backup
compounds which fall out of contention
with  others so that a  worldwide pool of
about 10-20 backup  materials  will  be
available.  Overall, the committee  takes
the view that  the level  of knowledge
outside  of  Swarts CFC technology for
production of  materials  for  these
applications critical to societal  needs is
almost nonexistent and certainly no more
than  in the embryonic stage. Therefore,
the need for funding substantial amounts
of research  up  to  the  date  where
important  atmospheric problems  (e.g.,
ozone depletion  and the  greenhouse
effect) are solved  satisfactorily cannot be
overemphasized.
 United States
 Environmental Protection
 Agency
Center for Environmental Research
Information
Cincinnati OH 45268
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