United States
                    Environmental Protection
                    Agency
Hazardous Waste Engineering
Research Laboratory
Cincinnati OH 45268
                    Research and Development
EPA/600/S2-85/029 July 1985
&EPA          Project  Summary
                    Test   Methods  for   Determining
                    the Chemical Waste  Compatibil-
                    ity  of  Synthetic  Liners

                    Joseph Tratnyek, Peter Costas, and Warren Lyman
                     Flexible membrane liners (geomem-
                    branes) used to contain liquid chemi-
                    cals and leachate at waste containment
                    sites are required to be chemically re-
                    sistant (compatible) to the liquid. In
                    order to select a liner for use as well as
                    judge its long-term reliability, its chem-
                    ical resistance against the liquid(s) to be
                    contained must be known. The mea-
                    surement of compatibility is a complex
                    matter, because a variety of physical
                    and chemical interactions can  occur,
                    and compatibility failure of a mem-
                    brane  has  never  been adequately
                    defined for this application.
                     A search was made for test methods
                    that would ascertain the compatibility
                    performance of  liners.  Disclosed
                    methods and procedures were exam-
                    ined and compared. Two tests being
                    promoted for general acceptance are
                    NSF Standard No.  54 (a voluntary
                    industry-generated test) and the pro-
                    posed EPA Test Method 9090. Several
                    other tests developed by liner manufac-
                    turers and researchers were found, as
                    well as those methods generally applied
                    to pipes, bottles, film, plastics, rubber
                    sheeting and the like.
                     Although details of tests vary, all are
                    laboratory tests in which selected phys-
                    ical properties of  the  membrane are
                    compared and evaluated after contact
                    with the liquid for specified periods of
                    time. All are tedious, time-consuming,
                    and potentially costly. Useful data for
                    product specification and application
                    are derived from these tests, but none
                    adequately addresses  all issues and
                    questions raised, especially with regard
                    to liner life-time prediction. Nor is any
                    one test universally accepted for use. A
                    combination  of compatibility tests
(e.g., immersion, stress-crack, and per-
meation) may be necessary to fully
characterize  chemical resistance  in
specific cases. A superior test(s) based
on a comprehensive understanding of
liner compatibility remains to  be
developed.
  Two levels of effort (immediately prac-
tical, and long-term) directed at evalu-
ating  membrane  compatibility  are
proposed. In the first, a test methodol-
ogy based on current protocols and
methods would be developed to provide
three  kinds of  required  infor-
mation: short-term  (testing up to 30
days' exposure),  intermediate (testing
up to 4 months' exposure), and long-
term (greater than 4 months' exposure).
In the second, research and test method
development would be pursued with the
purpose  of  exploring  new  methods,
techniques, apparatus, etc., for  better
compatibility characterization.
  This Project Summary was  devel-
oped by EPA's Hazardous Waste Engi-
neering  Research  Laboratory,
Cincinnati. OH, to announce key find-
ings of the research project that is fully
documented in a separate report of the
same title (see Project Report ordering
information at back}.


Introduction
  Liners fabricated from synthetic poly-
mer materials (often referred to as flexi-
ble membrane liners, - FML*) will be used
at a large number of the waste sites to
contain leachate and other waste liquids.
Since the primary function of a liner is to
contain  waste liquids,  a priori, a liner
must be resistant to the liquid.  A key
issue in the use of an FML is its compati-

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 bility (chemical  resistance)*  with  the
 waste liquid it will  hold. The criteria for
 evaluating chemical resistance and the
 choice of test  methods are  part of that
 issue.
   Field  test  information is  preferred
 because it reflects "real" exposure. Ade-
 quate field data have not been generated
 because the use of FML for waste con-
 tainment is too new a technology (in the
 order of  20  years  of experience).
 Although field information  is currently
 being generated, field testing is a slow
 process. To expedite the evaluation and
 selection of an FML, data are obtained
 from laboratory tests in which an FML is
 exposed to  a chemical challenge under
 set conditions, and then properties- usu-
 ally physical - of the exposed FML are
 measured. Laboratory tests serve as the
 primary  screening   approach to  FML
 chemical compatibility evaluation.
   There   are   problems with  current
 methodology.  Most tests  produce only
 indirect indication of  FML chemical re-
 sistance, and important parameters are
 neglected or minimized in FML product
 evaluation.  No actual  determination of
 chemical change is made in routine test-
 ing. In the absence of true long-term data
 from field or laboratory (the FMLtechnol-
 ogy is too  new), current compatibility
 data, in conjunction with industrial expe-
 rience,  must  be used to judge future
 behavior of FML. Lack of correlation with
 field  performance  remains a  present
 issue.
   For the benefit of regulators, planners,
 and designers, the current test methodol-
 ogy requires review and assessment so
 that uncertainties about data can be min-
 imized.  Chemical  resistance  data  are
 needed for  FML product development,
 screening  purposes,   site   liner-waste
 matching, and liner  life prediction.
  The purpose of this projectwasto com-
 pile, review, and evaluate available test
 methods for measuring and/or estimat-
 ing the chemical compatibility of poly-
 meric  flexible  membrane  liners with
 liquid wastes for use at hazardous waste
treatment, storage,  and disposal facili-
ties. The intention was not to write a test
 method for FML/waste compatibility, but
to assess the current state of affairs and
direct the thinking of all those concerned
toward routes that might lead to a satis-
factory,  comprehensive,  and  reliable
*The currently used term "geomembrane" includes
FML. In FML technology, a "compatible" liner is gen-
erally accepted as one that is "resistant" to chemical
attack as judged by its changes in physical properties
upon exposure to liquid waste
 chemical compatibility  measurement
 technique.

 General Technical
 Considerations
   General technical considerations rele-
 vant to FML compatibility testing include
 the nature of liner products, the nature of
 chemical and leachate which a liner is to
 contain,  the nature of chemical compati-
 bility,  the compatibility measurement
 features and test requirements.
   Although the behavior of an FML prod-
 uct will  depend upon its total composi-
 tion,  the  fundamental   behavioral
 element will  be  the polymer  phase.
 Therefore, the polymer has to be selected
 for its chemical resistance in a specific
 application.  Chemical  resistance will
 depend  not  only  upon the  chemical
 makeup of the polymer, but also on other
 factors, such as degree of polymerization
 or molecular weight, degree of crosslink-
 ing, crystallinity, morphology, and the
 like.
   The nature and composition of the
 waste liquid challenging the liner may be
 infinite in  variation.  While water and
 selected organic liquids can be chosen to
 challenge the membrane alone, combi-
 nations of liquids and  other waste mate-
 rial may also be used. Dissolved salts and
 other materials may be found in the chal-
 lenge liquid. In the field, actual leachate/
 waste at a site is usually a complex mix-
 ture of many components. It may be diffi-
 cult to analyze and characterize because
 of multiphase components or immiscible
 material. In any case, mixtures frequently
 do not behave in a manner predicted from
 components.
  Within the FML  industry,^! "compati-
 ble" FML material  is  generally accepted
 as one that is resistant to chemical attack
 as judged by its changes in physical prop-
 erties after exposure to the waste. How-
 ever, the chemical  attack can take place
 via several routes, all of which can  be
 mutually interactive. They are'

   •  Chemical reaction,
   •  Hydrolysis,
   •  Solvation/plasticization, and
   •  Environmental  response  (heat,
      light, ozone, bio-organism, etc.).

  It  is  important to remember that
 although we are dealing specifically with
tests  for  chemical compatibility,  FML
chemical  resistance   is  influenced  or
altered by all factors capable of producing
polymer degradation.
  A variety of properties has been pro-
posed  and used for  evaluating  mem-
branes.  Chemical  resistance  or
compatibility is usually based on physical
test data  gathered  after exposure to a
chemical or leachate. Physical test data
may include tensile properties such as
tensile strength, yield strength, elonga-
tion at  break, elongation at yield,  and
some  others.  These  are one-dimen-
sional, short-term, simple tests that are
easily  accomplished in the laboratory,
and that are preferred by the industry as
service  indicators.  Additional physical
tests may include tear and puncture re-
sistance of the membrane, hardness,
and, in the case of a reinforced mem-
brane,  ply adhesion  tests.  Stress-
cracking   is  measured  in  testing
polyethylene-type plastics, and permea-
tion is presently being considered as a
property to be measured for FMLs.

Present Compatibility Tests
  The   search  for  compatibility  test
methods included not only tests strictly
intended to determine the chemical re-
sistance of rubber  and  plastic  mem-
branes such as FMLs, but also allied tests
(e.g., for pipe, packaging, and film). All
types of tests that were relevant to chem-
ical resistance and the transfer of liquids
through  membranes were considered
and reviewed.
  Levels  of  information  sources  are
categorized as follows:
     I.   International  standards and
       tests;
    II.   National standards and tests;
   III.   Industrial standards and tests;
   IV.  Project tests; and
    V.  Academic/literature tests.
  Tests (27) applicable to the subject are
described  and discussed in detail. Infor-
mation is  presented in tabular form, in
descriptive text,  and   in  schematic
diagrams.
  A general feature of the tests is com-
monality of approach. This is evidenced
by the cross-referencing of key tests (e.g.,
ASTM  D543, ASTM 471,  ISO 175,  ISO
1817,  DIN 53  521,  BS  4618). The
approach to testing appears to be based
on assimilating test methods for rubber
sheet and  plastic sheet into a test useful
for  FMLs. It  is worth noting  that  a
"caveat"  is generally  found in each
method, warning that the test may not
correspond with the service  condition
and that  data are only comparative in
nature.  Absolute values or criteria for
compatibility are not established  in the
tests.
  At the present time, two specific  test
methods  for  evaluating  FML  perfor-
mance in  a chemical environment have
evolved -  NSF Standard No. 54 and EPA

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 Method 9090. The latter was designed
 specifically as a compatibility test for
 membrane liners in the  presence  of
 waste.  In  the  NSF standard,  chemical
 compatibility testing is described in the
 document  which  deals  with  other
 aspects of FML specifications. The NSF
 method is a voluntary approach to indus-
 try standardization; the EPA method may
 be promulgated as a national standard
 having  regulatory authority. The NSF test
 is primarily short-term, although provi-
 sion is  made for longer testing.
   Both  tests rely on measurement of sim-
 ilar physical property changes. Criteria
 for failure  are not specified by the NSF
 test, nor the EPA test, although the EPA
 test refers to RCRA guidance documents
 for evaluation of data. The NSF document
 deals with stress-cracking phenomena in
 a separate test; the EPA test does not at
 all. Both employ similar test  tempera-
 tures (23°C and  50°C). Importantly,  in
 Method 9090 samples are subjected  to
 one-side exposure; in NSF 54, individual
 test specimens are immersed  in a rea-
 gent.  Both  recommend FML contact with
 actual waste liquid or leachate.
  Other FML  industry  test  methods
 depend   primarily  upon  immersion  in
 fluid, although one-side contact in a sim-
 ulated ponding arrangement (heated dish
 or tub) is sometimes used. Attempts are
 made to simulate real experience, but the
 merit of the exposure methods is still
 being debated. Physical and mechanical
 features are  generally monitored for
 change.  Information  on industry  test
 results is scarce because results tend to
 be  proprietary.  Industry does retain its
 own concept as to what constitutes fail-
 ure in products. Tests are static in nature
 and single property measurements (e.g.,
 tensile  strength, elongation, hardness,
 and  tear  strength)  suffice  for
 characterization.
  In summary, the test reviewed exhibit
the following characteristic features:
    •  Test by immersion  or  one-side
        exposure;
    •  Test without stress, except for
       the  polyethylene-type  plastics,
       which are a  special case;
    •  Test at ambient temperature and
       some elevated temperature;
    •  Test with varying time (short to
       long), or to equilibrium;
    • Test in laboratory;
    •  Test with reagents or waste; and
    •   Measurement of  mechanical
      properties   and  evaluation  of
      appearance as the preferred indi-
      cators of compatibility.
   No one test satisfies all needs for a
 chemical compatibility test, and test pro-
 tocols and experimental details are sub-
 jects for discussion and re-evaluation.


 Consensus Meeting
   As part of the need to  elucidate and
 understand compatibility  test  methods
 and FML requirements, a meeting with
 experts in FML technology and applica-
 tions was held at Arthur  D. Little, Inc.,
 Cambridge, Massachusetts, in January
 1984. In attendance were several manu-
 facturers' representatives, an independ-
 ent FML researcher, EPA representatives,
 and members of the Arthur D. Little staff.
 This meeting provided an opportunity  to
 discuss the current test methodology and
 recommendations for improvements  in
 tests for  FML compatibility. The discus-
 sions identified areas of concern, issues,
 and means for resolution. This meeting
 was most useful in bringing to light practi-
 cal aspects of testing not dealt with in the
 published test methods.
 General Approach to Compati-
 bility Testing
   Compatibility testing of  FML is made
 complex by a number of factors and inter-
 actions. Although apparatus and protocol
 may differ,  current test methods apply
 simple, familiar technological tests  to
 evaluate those FML materials being used
 in a demanding, new application. Each of
 the tests described appears to be useful
 for screening and evaluation, but all are
 inadequate for predicting behavior patt-
 erns on a truly long-term basis. Evalua-
 tion of test  results is based on limited
 experience,  mostly from membrane
 manufacturers. Because of a recognized
 need for better information, the subject  f
 FML  compatibility  testing   requires
 further development. Test methodology
 must  be  matched  to   performance
 requirements. The scope of compatibility
 testing, FML material versus liquid chal-
 lenge,  test  parameters,  measurement
 and observation, and test details are sub-
 jects  that  require  rethinking.  New
 methods,   which   include  stress-
 relaxation measurement and  dynamic
 mechanical  analysis, are described and
 suggested  for   further  study  and
development.
  Aside  from  refining  present  test
 methodology  to  meet  immediate
demands, and for building a technologi-
cal and historical baseline, research  is
required  in  several areas  if chemical
compatibility is to be fully understood and
measured.  The  result of current and
future investigations  into FML perfor-
mance in a chemical environment will be
a better understanding and a test(s) satis-
factory to all.

Conclusions
    1. Presently  there is no generally
      accepted test method that fully
      meets the needs of industry or
      regulatory agency for the chemi-
      cal compatibility assessment of
      FML  in the  presence of waste
      liquid.

    2. Two general test methods specifi-
      cally  promoted for compatibility
      testing of FMLs are NSF Standard
      54 and EPA Method 9090. Sev-
      eral   manufacturers'  tests  are
      used  for evaluating  liners;  and
      some  standard material  tests
      have been applied to liners.

    3. Chemical compatibility testing is
      conducted primarily in the labora-
      tory with actual leachate, waste,
      or reagent. Field data are scarce
      because  liner technology for
      waste containment is too  new.
      Reagent testing is preferred for
      screening,  but  all current
      methods specify exposing the test
      specimen  to actual waste sam-
      ples  or leachate. Exposing  test
      specimens  in  an  actual waste
      containment facility  is  recom-
      mended, and provision for inclu-
      sion of membrane coupons at the
      site for periodic examination for
      compatibility appears  to be an
      obvious prerequisite for obtaining
      real  data  over the  long term.
      Chemical  class lists versus the
      FML type  developed  by industry
      and investigators for tests appear
      to be adequate for  the  initial
      stages of selecting an FML for a
      specific site.

    4. FML chemical compatibility test-
      ing is made complex because of a
      large  variety of possible interac-
      tions  among components of the
      process.

    5. Compatibility testing  is tedious,
      time-consuming,  costly,  and
      potentially dangerous  due to the
      need for handling toxic substan-
      ces. The ideal route to testing has
      not yet been  established,  and
      long-term  prediction  is tenuous
      because of incomplete knowledge.

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      6. Current tests, including those dis-
        cussed, deal with only part of the
        compatibility  problem.  Broader
        issues  include questions about
        practicability, cost, time span, sig-
        nificance, and reliability.

      7. It appears  that there will be no
        immediate  and ideal  resolution of
        the  FML  chemical  compatibility
        test issue. It is obvious that NSF 54
        and Method 9090 are the current
        contenders  for  a standard  test
        method, since other tests have not
        been   developed  sufficiently  for
        FML  evaluation.   However,
        whether NSF  54   is followed.
        Method 9090 is imposed,  other
        methods surface, or industry goes
     	  its own way, the problems are too
        diffuse and complex  to rely on  a
        simple  set  of rules  as presently
        conceived. The crux of the problem
        is related to the need for good long-
        term data in what is  essentially a
        new  industry, and the fact that
        chemical compatibility indicators
        remain undefined. Truly reliable
        compatibility data will be gener-
        ated  with  time,  but continuous
        action is required by industry, regu-
        latory  agencies, and  the research
        community to define  the requisite
        parameters for   evaluation,  and
        then  to develop  the appropriate
        tests.

  Recommendations
    Effort on two levels is needed to evalu-
  ate FMLs for waste liquid containment.
  The first level of effort deals with the
  immediate practical issue of ascertaining
  FML compatibility for a  particular appli-
  cation. The second - of long-term nature
      -focuseson understanding FMLcompat-
      ibility in the chemical/physical context,
      and then devising test methods for meas-
      uring the identified parameters. The first
      relies on maximizing application of cur-
      rent tests.  The second explores new or
      untested methods.
        For the  first approach, it is  recom-
      mended that test protocol be developed
      that would provide three kinds of infor-
      mation which might satisfy industry and
      regulatory  body needs to the different
      degrees required:

          I.   Short-term tests (up to 30 days'
              exposure),
          II.   Intermediate   tests  (up  to   4
              months' exposure), and
   III.  Long-term tests (greater than £
       months' exposure).

  In the second approach to establishing
the chemical  resistance of  FML, an
exploratory course is called for in which
FML properties are evaluated with tech-
niques not now employed for compatibil-
ity  measurement.  Information about
visco-elastic behavior and permeability
obviously  should be included. Methods
for  measurement  of dynamic stress-
strain  properties, dynamic mechanical
analysis, torsional  stress, and thermal
properties, especially under stress or
load, are  examples of techniques that
might be explored further.
        	                           ^~

         Joseph Tratnyek, Peter Costas, and Warren Lyman are with Arthur D. Little, Inc.,
           Cambridge. MA 02140.
         Robert Hartley is the EPA Project Officer (see below).

         The complete report, entitled "Test Methods for Determining the Chemical Waste
           Compatibility of Synthetic Liners," (Order No. PB 85-182 970/AS; Cost $73.00,
           subject to change) will be available only from:
                 National Technical Information Service
                 5285 Port Royal Road
                 Springfield, VA 22161
                 Telephone: 703-487-4650
         The EPA Project Officer can be contacted at:
                 Hazardous Waste Engineering Laboratory
                 U.S. Environmental Protection Agency
                 Cincinnati, OH 45268
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
Official Business
Penalty for Private Use $300
EPA/600/S2-85/029
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