United States Environmental Protection Agency Hazardous Waste Engineering Research Laboratory Cincinnati OH 45268 Research and Development EPA/600/S2-85/029 July 1985 &EPA Project Summary Test Methods for Determining the Chemical Waste Compatibil- ity of Synthetic Liners Joseph Tratnyek, Peter Costas, and Warren Lyman Flexible membrane liners (geomem- branes) used to contain liquid chemi- cals and leachate at waste containment sites are required to be chemically re- sistant (compatible) to the liquid. In order to select a liner for use as well as judge its long-term reliability, its chem- ical resistance against the liquid(s) to be contained must be known. The mea- surement of compatibility is a complex matter, because a variety of physical and chemical interactions can occur, and compatibility failure of a mem- brane has never been adequately defined for this application. A search was made for test methods that would ascertain the compatibility performance of liners. Disclosed methods and procedures were exam- ined and compared. Two tests being promoted for general acceptance are NSF Standard No. 54 (a voluntary industry-generated test) and the pro- posed EPA Test Method 9090. Several other tests developed by liner manufac- turers and researchers were found, as well as those methods generally applied to pipes, bottles, film, plastics, rubber sheeting and the like. Although details of tests vary, all are laboratory tests in which selected phys- ical properties of the membrane are compared and evaluated after contact with the liquid for specified periods of time. All are tedious, time-consuming, and potentially costly. Useful data for product specification and application are derived from these tests, but none adequately addresses all issues and questions raised, especially with regard to liner life-time prediction. Nor is any one test universally accepted for use. A combination of compatibility tests (e.g., immersion, stress-crack, and per- meation) may be necessary to fully characterize chemical resistance in specific cases. A superior test(s) based on a comprehensive understanding of liner compatibility remains to be developed. Two levels of effort (immediately prac- tical, and long-term) directed at evalu- ating membrane compatibility are proposed. In the first, a test methodol- ogy based on current protocols and methods would be developed to provide three kinds of required infor- mation: short-term (testing up to 30 days' exposure), intermediate (testing up to 4 months' exposure), and long- term (greater than 4 months' exposure). In the second, research and test method development would be pursued with the purpose of exploring new methods, techniques, apparatus, etc., for better compatibility characterization. This Project Summary was devel- oped by EPA's Hazardous Waste Engi- neering Research Laboratory, Cincinnati. OH, to announce key find- ings of the research project that is fully documented in a separate report of the same title (see Project Report ordering information at back}. Introduction Liners fabricated from synthetic poly- mer materials (often referred to as flexi- ble membrane liners, - FML*) will be used at a large number of the waste sites to contain leachate and other waste liquids. Since the primary function of a liner is to contain waste liquids, a priori, a liner must be resistant to the liquid. A key issue in the use of an FML is its compati- ------- bility (chemical resistance)* with the waste liquid it will hold. The criteria for evaluating chemical resistance and the choice of test methods are part of that issue. Field test information is preferred because it reflects "real" exposure. Ade- quate field data have not been generated because the use of FML for waste con- tainment is too new a technology (in the order of 20 years of experience). Although field information is currently being generated, field testing is a slow process. To expedite the evaluation and selection of an FML, data are obtained from laboratory tests in which an FML is exposed to a chemical challenge under set conditions, and then properties- usu- ally physical - of the exposed FML are measured. Laboratory tests serve as the primary screening approach to FML chemical compatibility evaluation. There are problems with current methodology. Most tests produce only indirect indication of FML chemical re- sistance, and important parameters are neglected or minimized in FML product evaluation. No actual determination of chemical change is made in routine test- ing. In the absence of true long-term data from field or laboratory (the FMLtechnol- ogy is too new), current compatibility data, in conjunction with industrial expe- rience, must be used to judge future behavior of FML. Lack of correlation with field performance remains a present issue. For the benefit of regulators, planners, and designers, the current test methodol- ogy requires review and assessment so that uncertainties about data can be min- imized. Chemical resistance data are needed for FML product development, screening purposes, site liner-waste matching, and liner life prediction. The purpose of this projectwasto com- pile, review, and evaluate available test methods for measuring and/or estimat- ing the chemical compatibility of poly- meric flexible membrane liners with liquid wastes for use at hazardous waste treatment, storage, and disposal facili- ties. The intention was not to write a test method for FML/waste compatibility, but to assess the current state of affairs and direct the thinking of all those concerned toward routes that might lead to a satis- factory, comprehensive, and reliable *The currently used term "geomembrane" includes FML. In FML technology, a "compatible" liner is gen- erally accepted as one that is "resistant" to chemical attack as judged by its changes in physical properties upon exposure to liquid waste chemical compatibility measurement technique. General Technical Considerations General technical considerations rele- vant to FML compatibility testing include the nature of liner products, the nature of chemical and leachate which a liner is to contain, the nature of chemical compati- bility, the compatibility measurement features and test requirements. Although the behavior of an FML prod- uct will depend upon its total composi- tion, the fundamental behavioral element will be the polymer phase. Therefore, the polymer has to be selected for its chemical resistance in a specific application. Chemical resistance will depend not only upon the chemical makeup of the polymer, but also on other factors, such as degree of polymerization or molecular weight, degree of crosslink- ing, crystallinity, morphology, and the like. The nature and composition of the waste liquid challenging the liner may be infinite in variation. While water and selected organic liquids can be chosen to challenge the membrane alone, combi- nations of liquids and other waste mate- rial may also be used. Dissolved salts and other materials may be found in the chal- lenge liquid. In the field, actual leachate/ waste at a site is usually a complex mix- ture of many components. It may be diffi- cult to analyze and characterize because of multiphase components or immiscible material. In any case, mixtures frequently do not behave in a manner predicted from components. Within the FML industry,^! "compati- ble" FML material is generally accepted as one that is resistant to chemical attack as judged by its changes in physical prop- erties after exposure to the waste. How- ever, the chemical attack can take place via several routes, all of which can be mutually interactive. They are' • Chemical reaction, • Hydrolysis, • Solvation/plasticization, and • Environmental response (heat, light, ozone, bio-organism, etc.). It is important to remember that although we are dealing specifically with tests for chemical compatibility, FML chemical resistance is influenced or altered by all factors capable of producing polymer degradation. A variety of properties has been pro- posed and used for evaluating mem- branes. Chemical resistance or compatibility is usually based on physical test data gathered after exposure to a chemical or leachate. Physical test data may include tensile properties such as tensile strength, yield strength, elonga- tion at break, elongation at yield, and some others. These are one-dimen- sional, short-term, simple tests that are easily accomplished in the laboratory, and that are preferred by the industry as service indicators. Additional physical tests may include tear and puncture re- sistance of the membrane, hardness, and, in the case of a reinforced mem- brane, ply adhesion tests. Stress- cracking is measured in testing polyethylene-type plastics, and permea- tion is presently being considered as a property to be measured for FMLs. Present Compatibility Tests The search for compatibility test methods included not only tests strictly intended to determine the chemical re- sistance of rubber and plastic mem- branes such as FMLs, but also allied tests (e.g., for pipe, packaging, and film). All types of tests that were relevant to chem- ical resistance and the transfer of liquids through membranes were considered and reviewed. Levels of information sources are categorized as follows: I. International standards and tests; II. National standards and tests; III. Industrial standards and tests; IV. Project tests; and V. Academic/literature tests. Tests (27) applicable to the subject are described and discussed in detail. Infor- mation is presented in tabular form, in descriptive text, and in schematic diagrams. A general feature of the tests is com- monality of approach. This is evidenced by the cross-referencing of key tests (e.g., ASTM D543, ASTM 471, ISO 175, ISO 1817, DIN 53 521, BS 4618). The approach to testing appears to be based on assimilating test methods for rubber sheet and plastic sheet into a test useful for FMLs. It is worth noting that a "caveat" is generally found in each method, warning that the test may not correspond with the service condition and that data are only comparative in nature. Absolute values or criteria for compatibility are not established in the tests. At the present time, two specific test methods for evaluating FML perfor- mance in a chemical environment have evolved - NSF Standard No. 54 and EPA ------- Method 9090. The latter was designed specifically as a compatibility test for membrane liners in the presence of waste. In the NSF standard, chemical compatibility testing is described in the document which deals with other aspects of FML specifications. The NSF method is a voluntary approach to indus- try standardization; the EPA method may be promulgated as a national standard having regulatory authority. The NSF test is primarily short-term, although provi- sion is made for longer testing. Both tests rely on measurement of sim- ilar physical property changes. Criteria for failure are not specified by the NSF test, nor the EPA test, although the EPA test refers to RCRA guidance documents for evaluation of data. The NSF document deals with stress-cracking phenomena in a separate test; the EPA test does not at all. Both employ similar test tempera- tures (23°C and 50°C). Importantly, in Method 9090 samples are subjected to one-side exposure; in NSF 54, individual test specimens are immersed in a rea- gent. Both recommend FML contact with actual waste liquid or leachate. Other FML industry test methods depend primarily upon immersion in fluid, although one-side contact in a sim- ulated ponding arrangement (heated dish or tub) is sometimes used. Attempts are made to simulate real experience, but the merit of the exposure methods is still being debated. Physical and mechanical features are generally monitored for change. Information on industry test results is scarce because results tend to be proprietary. Industry does retain its own concept as to what constitutes fail- ure in products. Tests are static in nature and single property measurements (e.g., tensile strength, elongation, hardness, and tear strength) suffice for characterization. In summary, the test reviewed exhibit the following characteristic features: • Test by immersion or one-side exposure; • Test without stress, except for the polyethylene-type plastics, which are a special case; • Test at ambient temperature and some elevated temperature; • Test with varying time (short to long), or to equilibrium; • Test in laboratory; • Test with reagents or waste; and • Measurement of mechanical properties and evaluation of appearance as the preferred indi- cators of compatibility. No one test satisfies all needs for a chemical compatibility test, and test pro- tocols and experimental details are sub- jects for discussion and re-evaluation. Consensus Meeting As part of the need to elucidate and understand compatibility test methods and FML requirements, a meeting with experts in FML technology and applica- tions was held at Arthur D. Little, Inc., Cambridge, Massachusetts, in January 1984. In attendance were several manu- facturers' representatives, an independ- ent FML researcher, EPA representatives, and members of the Arthur D. Little staff. This meeting provided an opportunity to discuss the current test methodology and recommendations for improvements in tests for FML compatibility. The discus- sions identified areas of concern, issues, and means for resolution. This meeting was most useful in bringing to light practi- cal aspects of testing not dealt with in the published test methods. General Approach to Compati- bility Testing Compatibility testing of FML is made complex by a number of factors and inter- actions. Although apparatus and protocol may differ, current test methods apply simple, familiar technological tests to evaluate those FML materials being used in a demanding, new application. Each of the tests described appears to be useful for screening and evaluation, but all are inadequate for predicting behavior patt- erns on a truly long-term basis. Evalua- tion of test results is based on limited experience, mostly from membrane manufacturers. Because of a recognized need for better information, the subject f FML compatibility testing requires further development. Test methodology must be matched to performance requirements. The scope of compatibility testing, FML material versus liquid chal- lenge, test parameters, measurement and observation, and test details are sub- jects that require rethinking. New methods, which include stress- relaxation measurement and dynamic mechanical analysis, are described and suggested for further study and development. Aside from refining present test methodology to meet immediate demands, and for building a technologi- cal and historical baseline, research is required in several areas if chemical compatibility is to be fully understood and measured. The result of current and future investigations into FML perfor- mance in a chemical environment will be a better understanding and a test(s) satis- factory to all. Conclusions 1. Presently there is no generally accepted test method that fully meets the needs of industry or regulatory agency for the chemi- cal compatibility assessment of FML in the presence of waste liquid. 2. Two general test methods specifi- cally promoted for compatibility testing of FMLs are NSF Standard 54 and EPA Method 9090. Sev- eral manufacturers' tests are used for evaluating liners; and some standard material tests have been applied to liners. 3. Chemical compatibility testing is conducted primarily in the labora- tory with actual leachate, waste, or reagent. Field data are scarce because liner technology for waste containment is too new. Reagent testing is preferred for screening, but all current methods specify exposing the test specimen to actual waste sam- ples or leachate. Exposing test specimens in an actual waste containment facility is recom- mended, and provision for inclu- sion of membrane coupons at the site for periodic examination for compatibility appears to be an obvious prerequisite for obtaining real data over the long term. Chemical class lists versus the FML type developed by industry and investigators for tests appear to be adequate for the initial stages of selecting an FML for a specific site. 4. FML chemical compatibility test- ing is made complex because of a large variety of possible interac- tions among components of the process. 5. Compatibility testing is tedious, time-consuming, costly, and potentially dangerous due to the need for handling toxic substan- ces. The ideal route to testing has not yet been established, and long-term prediction is tenuous because of incomplete knowledge. ------- 6. Current tests, including those dis- cussed, deal with only part of the compatibility problem. Broader issues include questions about practicability, cost, time span, sig- nificance, and reliability. 7. It appears that there will be no immediate and ideal resolution of the FML chemical compatibility test issue. It is obvious that NSF 54 and Method 9090 are the current contenders for a standard test method, since other tests have not been developed sufficiently for FML evaluation. However, whether NSF 54 is followed. Method 9090 is imposed, other methods surface, or industry goes its own way, the problems are too diffuse and complex to rely on a simple set of rules as presently conceived. The crux of the problem is related to the need for good long- term data in what is essentially a new industry, and the fact that chemical compatibility indicators remain undefined. Truly reliable compatibility data will be gener- ated with time, but continuous action is required by industry, regu- latory agencies, and the research community to define the requisite parameters for evaluation, and then to develop the appropriate tests. Recommendations Effort on two levels is needed to evalu- ate FMLs for waste liquid containment. The first level of effort deals with the immediate practical issue of ascertaining FML compatibility for a particular appli- cation. The second - of long-term nature -focuseson understanding FMLcompat- ibility in the chemical/physical context, and then devising test methods for meas- uring the identified parameters. The first relies on maximizing application of cur- rent tests. The second explores new or untested methods. For the first approach, it is recom- mended that test protocol be developed that would provide three kinds of infor- mation which might satisfy industry and regulatory body needs to the different degrees required: I. Short-term tests (up to 30 days' exposure), II. Intermediate tests (up to 4 months' exposure), and III. Long-term tests (greater than £ months' exposure). In the second approach to establishing the chemical resistance of FML, an exploratory course is called for in which FML properties are evaluated with tech- niques not now employed for compatibil- ity measurement. Information about visco-elastic behavior and permeability obviously should be included. Methods for measurement of dynamic stress- strain properties, dynamic mechanical analysis, torsional stress, and thermal properties, especially under stress or load, are examples of techniques that might be explored further. ^~ Joseph Tratnyek, Peter Costas, and Warren Lyman are with Arthur D. Little, Inc., Cambridge. MA 02140. Robert Hartley is the EPA Project Officer (see below). The complete report, entitled "Test Methods for Determining the Chemical Waste Compatibility of Synthetic Liners," (Order No. PB 85-182 970/AS; Cost $73.00, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Hazardous Waste Engineering Laboratory U.S. Environmental Protection Agency Cincinnati, OH 45268 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati OH 45268 Official Business Penalty for Private Use $300 EPA/600/S2-85/029 OCQQSe* PS U $ ENVIR PROTECTION ASENCY RcGION 3 LIBRARY 230 S DEARBORN STREET CHICAGO IL «0*C4 ill,,,,l.,i.,,li,i,l,!i,,,,i,i,,f,i ------- |