United States
                    Environmental Protection
                    Agency
Air and Energy Engineering
Research Laboratory
Research Triangle Park NC 27711
                   Research and Development
EPA/600/S2-85/106  Jan. 1986
&ER&         Project  Summary
                   Evaluation  of  the  Efficiency of
                   Industrial  Flares:   Flare  Head
                   Design  and  Gas Composition
                   J.H. Pohl and N. R. Soelberg
                     This report documents a continua-
                   tion of Phase 4 of a research program to
                   quantify emissions from, and efficien-
                   cies of, industrial flares. Phases 1 (Ex-
                   perimental Design) and  2 (Design of
                   Test Facilities) were reported in EPA-
                   600/2-83-070 (NTIS  No. PB83-263723).
                   Phase 3 (Development of Test Facilities)
                   and initial work in Phase 4 (Data Collec-
                   tion) were reported in EPA-600/2-84-095
                   (NTIS No. PB84-199371). Further data
                   collection during Phase 4 is reported
                   here.
                     Initial  results were limited  to tests
                   conducted  burning propane/nitrogen
                   mixtures in pipe flares without pilot
                   light stabilization. The work reported
                   here extends the previous results to
                   other flare head designs and other
                   gases and includes a limited investiga-
                   tion of the influence of pilot flames on
                   flare performance.  The following re-
                   sults were obtained:

                     • Flare head design influences the
                       flame stability curve.
                     • Combustion efficiency can be cor-
                       related with flame stability for
                       pressure heads and coanda steam
                       injection heads.
                     • For the limited conditions tested,
                       flame stability and combustion ef-
                       ficiency of air-assisted heads corre-
                       lated with the momentum ratio of
                       air to fuel; the heating value of the
                       gas had only minor influence.
                     • Limited data on an  air-assisted
                       flare show that a pilot light im-
                       proves flame stability.
                     • The destruction efficiency of com-
                       pounds depends on the structure
                       of the compounds.
  • For the compounds tested in this
    program, the destruction efficiency
    of different compounds could be
    correlated with the flame  stability
    curve for each.

  This Project Summary was devel-
oped by EPA's Air and Energy Engineer-
ing Research Laboratory, Research Tri-
angle Park, NC, to announce key
findings of the research project that is
fully documented in a separate report
of the same title (see Project Report or-
dering information at back).

Introduction
  Industrial  flares are commonly used
to safely and economically  destroy
large amounts of industrial waste
gases. Since most of the  gas flared in
the U.S. is from leaks,  purges, and
emergency vents, the amounts and
compositions  of flared gases vary
widely and are difficult  to measure.
Flare emissions are also difficult to mea-
sure. Most  flares are elevated to de-
crease noise and radiation hazards and
to increase  dispersion of combustion
products. Probe collection of plume ma-
terial in such situations is impractical.
Remote sensing of flare emissions is an
alternative to direct sampling, but in-
strumentation and techniques  for this
purpose are still undeveloped.
  To evaluate and control industrial
flare emissions, pilot-scale research is
necessary to obtain direct sampling of
flare emissions. Flare research has been
conducted at Energy and  Environmen-
tal Research Corporation  (EER) since
1980. A pilot-scale flare test facility was
constructed for the U.S. EPA in 1982.

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  Previous results (reported in EPA-600/
2-83-070 and -84-095) showed that flare
combustion  efficiencies are generally
high (i.e., exceeding 98%), but under
some operating conditions (e.g., excess
steam injection) efficiencies can be low.
The results also  showed that, when a
flare flame is stable (i.e., not near blow-
off conditions), combustion is efficient.
However, flares operating with unstable
flames tend  to be  inefficient. Data on
flare gas exit velocity were correlated
with the gas heating value to describe
the region of flame instability. Thus, for
the conditions tested,  the operating
range required for  efficient flare per-
formance can be defined.
  Caution should be used, however, in
applying these results to situations  not
tested. Flare flame  stability and com-
bustion efficiency may vary, depending
on the flare head type, gas composition,
and operating  conditions. Thus, the re-
search was extended to evaluate the ef-
fects of: (1) flare head type on flare com-
bustion efficiency,  and (2)  relief gas
composition On  flare  combustion and
destruction efficiency.

Approach
  The program was divided into four
major tasks:
  • Task 1—Evaluation  of combustion
    efficiency  for different flare head
    types.
  • Task 2—Identification of represen-
    tative,  potentially difficult-to-
    destroy compounds.
  • Task 3—Evaluation  of combustion
    and  destruction efficiency of se-
    lected relief  gas mixtures.
  • Task 4—Data analysis and report-
    ing.
  For Task  1, four commercial flare
heads were  evaluated:  an air-assisted
head, two pressure heads, and a coanda
steam injection head.
  Each head was  tested on the EER
pilot-scale Flare Test  Facility (FTF).
Flame stability  and combustion effi-
ciency were measured as functions of:
(1) relief gas and exit velocity, (2) relief
gas heating value, (3) steam assist flow
rate (for the coanda head), (4) air assist
velocity  (for  the air-assisted  head),
(5) relief gas pressure (for the pressure
head), and (6) with and without pilot
flame (for the air-assisted head).
  The  relief gas for these  tests was
propane, mixed  with  nitrogen  to vary
the heating value. Natural gas was used
for the pilot flame.
  Tasks 2 and 3 were designed  to mea-
sure effects of  flare gas composition on
flame pollutant emissions. A wide vari-
ety of industrial compounds are fre-
quently flared in the U.S. Most often,
they are flared in mixtures containing
several different compounds. Each dif-
ferent mixture may exhibit somewhat
different flaring characteristics. Pilot or
large-scale testing of every conceivable
relief gas mixture would  be expensive
and unending.
  Task 2 involved the testing of com-
pounds  in a  laboratory facility. Al-
though laboratory-scale flare flames are
aerodynamically unlike pilot or large-
scale flare flames, laboratory-scale tests
can be used to economically and swiftly
screen compounds to determine com-
parative potential for destruction in
flares. Compounds which demonstrate
flaring difficulties in the laboratory-
scale Flare Screening Facility (FSF) are
candidates for testing on  the FTF.
  Twenty-one compounds were se-
lected for laboratory-scale testing in the
FSF, representing the following classes:
sulfur compounds,  nitrogen  com-
pounds,  chlorinated compounds, oxy-
genated  compounds,  aliphatic hydro-
carbons, aromatic hydrocarbons, and
compounds with low heating value. Of
the 21 compounds screened, 6 were se-
lected as candidates for testing on the
FTF. Selection criteria included low de-
struction  efficiency, poor ignitability,
and high soot production.
  Three of the six compounds,  along
with hydrogen sulfide, were tested on
the FTF.
  Hydrogen sulfide and ammonia were
tested in mixtures with propane and ni-
trogen. Ethylene oxide and  1, 3-
butadiene were tested  diluted with ni-
trogen to vary the heating value. Flame
stability, combustion  and destruction
efficiency,  soot production, and
byproduct formation from  incomplete
combustion were  measured for each
compound. All tests were conducted
using the 3-in.* open pipe flame, with-
out pilot flame stabilization.
  For Tasks 1  and 3 (conducted on the
FTF), samples were taken at five radial
positions above the flame. These local
samples were analyzed for 02, CO, C02,
hydrocarbon, NOX, and soot concentra-
tion. Where  applicable,  the samples
were also analyzed for H2S, S02, and
NH3 concentration.
  Sampling in the FSF (Task 2) was eas-
ier. In this facility, the flare nozzle was
enclosed in a  reaction chamber, which
 (*) To convert to metric units, please use the equiv-
 alents at the end of this Summary.
isolated the flame from the external en-
vironment. Sampling of the well-mixed
products at the reactor outlet required
only one probe.
  Samples were analyzed during tests
on both the FSF and FTF to evaluate air
dilution, mass balances, combustion ef-
ficiency, and destruction  efficiency.
SO2/ injected during  some of the pilot
tests, was used as a tracer for mass bal-
ances.  Mass balances on the FTF were
more difficult because of product loss,
air dilution in the large exposed flame,
and plume concentration gradients. Lo-
cal mass balances were used to accu-
rately evaluate local mass fluxes, local
combustion efficiency, and destruction
efficiency. Local mass fluxes were radi-
ally integrated to calculate overall com-
bustion and destruction efficiencies.

Results

Flare  Head Design
  The data show that flare head design
influences the flame stability curve (as a
function of gas heating value) as shown
in Figure 1 for the coanda steam injec-
tion  head and the pressure heads. The
flame stability of the air-assisted head
was controlled by the ratio of air to fuel
momentum as shown in Figure 2. The
heating value of the gas had little influ-
ence on flame  stability for the  air-
assisted flare. The  combustion  effi-
ciency of the pressure and  coanda
steam  injection heads correlated with
the gas heating value needed to main-
tain  flame stability, as shown in Figure
3. For  the air-assisted flare, the air to
fuel  momentum ratio was used to de-
velop a correlation with combustion ef-
ficiency. Figure 4 shows this relation-
ship, but caution should be  used in
applying these data due to the limited
number of observations.

Gas Composition
  The  relative destruction efficiency of
different gases was determined in the
FSF. Table 1 gives results of these tests.
Six compounds were identified as po-
tentially difficult to destroy:

  •  1, 3-butadiene yielded large
     amounts of soot.
  •  Carbon monoxide was difficult to
     ignite when pure.
  •  Ethylene oxide yielded low destruc-
     tion efficiency.
  •  Vinyl chloride yielded low destruc-
     tion efficiency.
  •  Hydrogen cyanide yielded low de-
     struction efficiency.

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  • Ammonia  was difficult to ignite
    when pure.
The destruction efficiency (DE) of three
of these compounds and H2S was mea-
sured on the FTP. The flame  stability
curve depended on the compound as
shown in Figure 5. (H2S and NH3 were
tested as  minor constituents in
propane/nitrogen mixtures.) The DE of
the individual compounds depended on
compound type but correlated with the
stability curve  for each compound as
shown in Figure 6.

Conclusions
  • Flare head design influences  the
    flame stability curve.
  • Combustion efficiency can be cor-
    related with flame stability for pres-
    sure heads and coanda steam  in-
    jection heads.
  • For the limited conditions tested,
    flame stability and combustion effi-
    ciency of air-assisted heads corre-
    lated with the momentum ratio of
    air to fuel; the heating value of the
    gas had only minor influence.
  • Limited data on an air-assisted flare
    show that  a pilot light improves
    flame stability.
  • The destruction efficiency of com-
    pounds depends on the structure of
    the compounds.
  • For the  compounds tested in this
    program, the destruction efficiency
    of different compounds could  be
    correlated with the flame stability
    curve for each.

Conversion Factors
  To convert nonmetric units used in
this Summary to their metric  equiva-
lents, please use the following factors:

Nonmetric Multiplied  by  Yields metric
    Btu
    ft
    ft3
    in.
1.055
0.305
0.028
2.54
kJ
m
m3
cm
                           1200
                           1100
                           1000

                        I
                        I
                         <5
                         
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      1000
       100 -

  I
  I
       0.1
                                                           8
                                                    Without Pilot

                                                 O  180-400 Btu/ft3
                                                 D  401-900
                                                 O  901-1400
                                                 A  1401-2350
                                                                  With Pilot
                                                              €  209-400 Btu/ft3
                                                            \
                   0.2       0.4       0.6       0.8       1.0

                                Air-Assist to Gas Momentum Ratio
                                                                     1.2
                                                                  1.4
Figure 2.
Maximum gas exit velocity for stability versus air-assist to gas momentum ratio for
the air-assisted head G. with and without pilot.

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!
u
 .4)
  C
 .o
  1
 1
      100
       98
      96
       QA
      90
      88,
      86
      84
                                  I  N   12 in.   Coanda Steam-Injected
                                  •  u          !./„„_/ n
                                  I
              HeadD
   [j  1.5 in.  Pressure-Assisted Head £
'  Q  3.8 in.  Pressure-Assisted Head F
I  Q    3 in.  Open Pipe Head with Pilot
                                    1
                                   i
Figure 3.
                                  1                        2           2.5
                    Gas Heating Value/Minimum Heating Value for Stability
            Combustion efficiency vs. flame stability for steam-injected and pressure-assisted
            flare heads.

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        99.9 ,
   Uj
   O
    u
   a
    i
   1
    o
   O
        99.0
90.0
                                                                           .0.1
                    C*   Without Pilot

                    £   With Pilot

                  S.R.  =  Air-Assist to Fuel
                         Stoichiometric Ratio
                                                  0.5
       5.0
                                                                            1.0
10.0
                                                                          1
                                                                                   .c
                                                                                   .§>
I
w

I
o
(J
                                                                            100.0
                        0.2          0.4          0.6         0.8


                            Air-Assist to Gas Momentum Ratio
                                                                 1.0
Figure 4.    Combustion efficiency vs. air-assist to gas momentum ratio for commercial air-
             assisted head G.

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  Table 1.    Results of Compound Screening Tests (Gases in Propane/Nitrogen Mixtures)
Compound
Acetylene
Ethylene
Propylene
1, 3-Butadiene
Butane
Propane
Propane
Benzene
Toluene
Chlorobenzene
Carbon Monoxide
Carbon Monoxide
Carbon Monoxide
Acetone
Acetaldehyde
Ethylene Oxide
Carbon Dioxide
Methyl Chloride
Ethylene Dichloride
Vinyl Chloride
Methyl Mercaptan
Acrylonitrile
Hydrogen Cyanide
Ammonia
Ammonia
%
Compound
in Gas
100
100
100
100
100
100
25
1.50
1.50
1.15
100
30
NA
1.43
2.07
1.42
7.58
9.17
1.43
0.11
10.7
1.47
0.013
20
100
%
Nitrogen
in Gas
0
0
0
0
0
0
75
43
43
43
0
44
NA
43
43
43
43
42
43
44
40
43
44
37
0
Heating
Value
Btu/ft3
1475
1580
2300
2780
3321
2350
1763
2370
2381
2350
[C o u 1
1760
1111
2347
2331
2337
2171
2212
2335
2350
2218
2350
2350
1967
}C o u 1

DE"
%
99.99
99.91
99.98
99.93
99.99
99.98
99.97
99.59
99.99
99.49
d No
99.60
NA
99.80
99.99
IS6.92I
NA
99.94
99.70
I9g.79l
99.39
99.99
I85.00I
99.90
d N o

CE"
%
99.97
99.92
99.93
99.93
99.96
98.18
NA»
99.95
99.90
99.95
t 1 g
99.88
99.42
99.96
99.97
99.95
99.93
99.96
99.95
NA
99.82
99.96
NA
NA
t 1 g

Soot
mg/m3
<1.5
<1.5
<1.5
| 75C |
<1.5
<1.5
NA
<1.0
<1.0
<1.0
n i t e\
<1.0
<1.0
<1.0
<1.5
<1.0
<1.0
<1.0
<1.0
<1.0
<1.0
<1.0
<1.0
<1.0
n i t e\

aDE = Destruction Efficiency.
•"CE = Combustion Efficiency.
'Boxes indicate compounds with potential problems.
<
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   59.39

     99.9
 2
 CD
I
 c
 o
99.0
     90.0
                Ethylene Oxide
       1,3-Butadiene
               Propane
                           Q Ammonia, 1.5-4.5 Percent in Propane/Nitrogen

                           Q  1,3-Butadiene in Nitrogen

                           U Ethylene Oxide in Nitrogen

                           ff Propane in Ammonia Tests

                           W Propane in Hydrogen Sulfide Tests
                                                                  0.0)
                                                                       0.1
                                                                         I

                                                                         •Q
                                                                          O

                                                                         .5
                                                                         s^
                                                                          O

                                                                         !
                                                                  1.0
                                                                       10.0
                                                                          1
                                                                          i
                                                                       100.0
Figure 6.
                          1.0                   2.0

             Heating Value/Minimum Heating Value for Stability

       Destruction efficiency of different gases.
   J. Pohl and N. Soelberg are with Energy and Environmental Research Corp.,
     Irvine. CA 92718.
   Bruce A. Tichenor is the EPA Project Officer (see below).
   The complete report, entitled "Evaluation of the Efficiency of Industrial Flares:
     Flare Head Design and Gas Composition, "(Order No. PB86-100 559/AS; Cost:
     $16.95, subject to change) will be available only from:
           National Technical Information Service
           5285 Port Royal Road
           Springfield, VA 22161
           Telephone: 703-487-4650
   The EPA Project Officer can be contacted at:
           Air and Energy Engineering Research Laboratory
           U.S. Environmental Protection Agency
           Research Triangle Park, NC 27711
                                                                                   . S. GOVERNMENT PRINTING OFFICE: 1986/646-116/20747

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