United States
                    Environmental Protection
                    Agency
Health Effects Research
Laboratory
Research Triangle Park NC 27711
                    Research and Development
EPA/600/S1-85/008 July 1985
oEPA         Project  Summary
                    Morphometric  Studies  of the
                    Effects  of Ozone  on  Rodent
                    Lungs

                    J. D. Crapo, B. E. Barry, and R. R. Mercer
                     The degree of lung injury caused by
                    prolonged inhalation of low  levels of
                    ozone is relevant because a number of
                    urban environments periodically reach
                    levels of 0.2 - 0.3 ppm ozone. Morpho-
                    metric methods were used to evaluate
                    the effects of 0.25 ppm ozone on lung
                    tissue of both young adult and juvenile
                    rats.  Three regions of the lung were
                    examined, the distal alveolar region, the
                    proximal alveolar region, and the termi-
                    nal bronchioles. In addition, the effects
                    of  inhalation of 0.12  ppm O3 on the
                    proximal alveolar region of young adult
                    rats were also evaluated.
                     The results showed that ozone in
                    these low concentrations reacts mainly
                    in  the  terminal bronchioles and the
                    proximal alveolar region. After 6 weeks
                    of inhaling 0.25 ppm ozone the number
                    of type I epithelial cells in the proximal
                    alveolar region doubled in the animals
                    exposed from 1 day of age. The mean
                    surface area of type I epithelial cells
                    decreased 38% and their mean thick-
                    ness  increased  24%.  The number of
                    alveolar type II epithelial cells  also
                    increased  and the  number of alveolar
                    macrophages doubled. Young adult
                    animals exposed to 0.25 ppm ozone
                    showed similar changes in the epithe-
                    lium  of the proximal  alveolar region,
                    moreover,  these animals showed  a
                    doubling of interstitial macrophages
                    indicating a mile inflammatory stimulus
                    in the interstitium. In the terminal bron-
                    chioles, exposure to 0.25 ppm ozone
                    produced a significant 14-16% decrease
                    (p< 0.05) in the average luminal surface
                    area  of clara cells. Inhalation of 0.12
                    ppm  ozone for 6 weeks also caused
                    measureable changes in the  proximal
alveolar region of young adult rats. Type
I cell number increased 36% (p< 0.05)
and the mean surface area of both the
air side and the basement membrane
side of the cell decreased 23%. These
results suggest that 0.25  ppm ozone
causes epithelial injury in the proximal
alveolar region and  in the terminal
bronchioles of both juvenile and young
adult rats. Exposure to 0.12 ppm ozone
causes a detectable but less extensive
injury to the type I epithelium in the
proximal alveolar region.
  This Project Summary was developed
by EPA's Health Effects Research Lab-
oratory. Research Triangle Park, NC, to
announce key findings of the research
project that is fully documented in a
separate report of the same title (see
Project Report ordering information at
back).

Introduction
  Ozone is an atmospheric pollutant
occurring as a photochemical oxidant in
ambient air. The concentration of ozone
in ambient air depends on the concentra-
tion of the primary pollutants as well as
local environmental conditions such as
temperature, air stagnation, and sunlight
intensity. For several years oxidant con-
centrations have been measured by state
and local control agency monitoring sta-
tions. These data are gathered and ana-
lyzed by the U.S. Environmental Protec-
tion Agency (EPA). Most urban centers
have intermittently exceeded the current
national  air quality standard for ozone
(0.12  ppm),  and several  cities (Los
Angeles, Denver, Philadelphia, Houston,
and New York) have had high hourly lev-
els in excess of 0.20 to 0.30 ppm. The

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chronic effects of such ozone concentra-
tions are unknown.
  Currently there is a scientific agree-
ment that ozone concentrations in excess
of one ppm are  hazardous to  human
health. Experiments on  laboratory ani-
mals (rats, mice, guinea pigs, rabbits, and
monkeys) at ozone concentrations of 0.2
to 1.0 ppm for short exposures have dem-
onstrated qualitative histopathologic chang-
es in conducting airways and alveolar
spaces. Various investigations have des-
cribed: (1) damage to ciliated cells in the
terminal  bronchioles  with nonciliated
progenitor cell division  for bronchiolar
epithelial  cell  renewal; '(2) hyperplasia
and  hypertrophy of  nonciliated bronch-
iolar epithelial cells in respiratory bronch-
ioles and intrabronchial accumulation of
alveolar  macrophages;  (3) significant
cellular damage at the alveolar duct level;
(4) swelling and desquamation of type I
alveolar  lining  cells with  subsequent
proliferation of type  II  cells to  cover
denuded  areas;  and (5)  ultrastructural
evidence of damage to endothelial cells
and the basement membrane. However,
there are currently no  qualitative  or
quantitative  morphologic studies  of an-
imals exposed to ozone concentrations
less than 0.2 ppm. Such experiments are
obviously vital to our understanding of
possible  damage to the human lung in
urban areas, where low level exposures
occur intermittently in the range of 0.20
ppm or less.


Materials and Methods
  Specific  pathogen-free male,  Fisher
344 rats that were either 1 day or 6 weeks
old were exposed to 0.12 ppm or 0.25
ppm ozone. Rats that breathed filtered
room air served as controls. After 6 weeks
of exposure,  rats were sacrificed and
their lungs fixed by intratracheal instilla-
tion of 2% glutaraldehyde. The procedure
used to isolate terminal bronchioles and
proximal alveolar tissue from slices of the
left lung is illustrated in Figure 1.
  Ultrathin  sections of terminal bronchi-
oles and  proximal alveolar regions were
obtained and EM micrographs taken from
them. Morphometric analysis was applied
to study  structural  changes caused by
inhalation of ozone. Randomly selected
blocks of distal alveolar tissue were also
studied.
Results

Effects of Inhalation ofO.25
ppm O3 on the Distal Alveolar
Region of Juvenile and Young
Adult Rats
  Morphometric methods  were used to
evaluate the effects of 0.25 ppm ozone on
lung tissue randomly selected from the
alveolar region of mature and neonatal
rats. For this study this area is defined as
the distal alveolar region and it includes
all alveoli beyond the terminal bronchi-
oles. The results indicate that few struc-
tural changes occur in the distal alveolar
region as a consequence of this level of
Os exposure. There were  reductions in
the body weight gained by mature anim-
als exposed to ozone for 6 weeks (p=0.05)
and  by neonates  exposed for  1  week
(p=0.06).  Previous investigators  have
reported this difference in rats exposed to
1 ppm or less of ozone. The arithmetic
mean thicknesses of the epithelium and
endothelium increased 10%(p=0.08)and
16% (p=0.08), respectively, in mature rats.
The volume density of air in the alveolar
region was significantly smaller in neo-
                 Sharpened Canula
 Terminal Bronchioles
   In Cross-section
                                                           Terminal Bronchiole
                                                             In Cross-section
                                                    Embed
                                                   Oriented
                                                   Tissue
                                                   Plug In
                                                   Capsule,
                                                 ii-—v-TWC'-r/1^- ^!
                                                  *_>-    r*.  '  &r*r+*A
                                                                   I  Serial Section To
                                                                   \ First Duct Bifurcation
                                                                                          , * 1
                                                                                                 T/rt   rX.
                                                                                                                r>-
 Figure 1.    Schematic of the microdissection procedure used to isolate lung tissue containing terminal bronchiole and proximal
            alveolar region.

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natal rats exposed to ozone for 1 week,
but this change may have been caused by
variations in fixed lung volumes of these
small rat lungs. In neonatal rats exposed
to ozone for 6 weeks, the average base-
ment membrane surface area covered by
type I cells decreased 20% (p=0.06). There
were no significant  increases in  the
arithmetic mean thickness of epithelium
or endothelium. No  other  significant
changes were found in the morphometric
characteristics of the  distal alveolar re-
gion of the adult or neonatal rats.

Effects of Inhalation of 0.25
ppm Oa on the Proximal Alveolar
Region of Juvenile and Young
Adult Rats
  Since the alveolar region most adjacent
to terminal bronchioles has been reported
as one of the major sites of injury due to
ozone inhalation, this specific lung region
was  studied  using ultrastructural mor-
phometric analysis. After 6  weeks of
exposure to  0.25  ppm  03,  qualitative
examination  of the tissue revealed  no
observable damage to the terminal bron-
chioles or the adjacent proximal alveolar
tissues. However, by morphometric anal-
ysis, significant changes occurred in the
alveolar epithelium of the proximal alve-
olar region. In the animals exposed from 1
day of age (juvenile animals) the number
of type I epithelial cells doubled, their
mean surface area decreased 38%, and
their mean thickness increased 24%. The
number of alveolar type II epithelial cells
increased and the number of alveolar
macrophages doubled. Young adult ani-
mals exposed to ozone  showed similar
changes in the epithelium of the proximal
alveolar reigon. The changes in type I and
type II cells are illustrated in Figures 2 and
3 respectively. Compared to the juvenile
animals, the young adult, ozone exposed
animals  showed more  interstitial  cell
reaction  with a doubling of interstitial-
macrophages suggesting a mile inflam-
matory stimulus in the interstitium. The
change in number and size of type I cells
is consistent with an increased cell turn-
over rate due to prolonged ozone inhala-
tion. These results suggest that 0.25 ppm
ozone causes a chronic epithelial injury in
the proximal alveolar region of both juve-
nile and young adult rats.

Effects of Inhalation of 0.12
ppm Oa on the Proximal Alveolar
Region of Young Adult Rats
  Morphometric analysis was carried out
on lung tissue of the  proximal alveolar
                              Proximal Alveolar Region
                                Type I Epithelial Cells
     + 100
  I   +5°
  Cj
  6
  I
      -50
                Cell
              Number
               Mean Cell
                 Volume
                   Mean Cell
              Basement Membrane
                  Surface Area
   Mean Cell
   Thickness
     f urn)
  *p < .05

  §|  Juvenile flats

  I  Young Adult flats
Figure 2.    Effects of inhalation of 0.25 ppm ozone on the characteristics of type I epithelial cells
           in the proximal alveolar region of juvenile and young adult rats.
                           Proximal Alveolar Region
                             Type II Epithelial Cells
      +50
      +25
   I
   OS

   O
      -25 L
  Cell
Number
(>#/mm2)
Mean Cell
 Volume
 (urn3)
                                         Mean Alveolar
                                          Surface Area
Mean Celt
Thickness
  (umj
     *p<.05

         Juvenile flats


         Young Adult Rats
Figure 3.    Effects of inhalation of 0.25 ppm ozone on the characteristics of type II epithelial
            cells in the proximal alveolar region of juvenile and young adult rats

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region isolated from young adult rats that
were exposed to 0.12 ppm, the current air
quality standard for ozone. This investiga-
tion is therefore of fundamental impor-
tance  in evaluating the effectiveness of
present air quality control standards. The
results of morphometric  analysis indi-
cated that after 6 weeks of ozone inhala-
tion, significant changes occurred in the
type I epithelium of the proximal alveolar
region. Type I cell  number increased 36%
(p < 0.05) and  both their  mean surface
area and mean basement membranesur-
face area decreased 23% (p <  0.05).
While  the  average  type  I cell volume
decreased 11%, this change was not sta-
tistically significant. The volume of type I
epithelium increased 13% and the thick-
ness of type II epithelium increased 29%.
No significant changes were found in the
mean cell volume or surface area of type II
cells. The  changes observed with the
inhalation of 0.12 ppm ozone were found
to be similar to, but of lesser magnitude
than, those occurring with exposure to
0.25 ppm ozone (see Figure 4).
  The higher concentration of ozone pro-
duced both a greater and a broader degree
of injury. In addition to increases in type I
epithelium, the volumes of type II epithe-
lium, alveolar macrophage, and cellular
interstitium were  found to increase after
6 weeks of exposure to 0.25 ppm ozone.
This study demonstrates that the expo-
sures to ozone  concentrations near cur-
rent air quality standard of 0.12 ppm
ozone  can cause  measurable structural
changes in the alveolar epithelium. The
degree of tissue injury caused by ozone
can  be  rigorously  quantified and in-
creased with exposure to higher concen-
trations of ozone.

Effects of Inhalation of 0.25
ppm Oa on the Terminal
Bronchioles of Juvenile and
Young Adult Rats
  Terminal bronchioles comprise the final
portion of the conducting airway in the
lung. It has been shown to be particularly
sensitive to the effects of ozone exposure.
Morphometric methods were developed
to evaluate the effects  of inhalation of
0.25 ppm ozone on the terminal bronchi-
oles of rats. This concentration of ozone is
near the current  air quality  standard of
0.12 ppm and is below the level at which
changes can  be  reliably documented
qualitatively. The  results of the morpho-
metric analysis indicated that ciliated
cells composed 48% (juvenile) or 53%
(young adult) of the total  population of
terminal bronchiolar cells and clara cells
were 33% (juvenile) or 29% (young adult).
The average terminal bronchiolar diam-
eter (210 fjm) and the average thickness
of the bronchiolar epithelium  (7.5 fjm)
was  not significantly changed by  the
exposure to ozone. Exposure to 0.25 ppm
ozone for 6 weeks produced a significant
14-16% decrease (p < 0.05) in the aver-
age luminal surface  area of clara cells in
the terminal bronchioles of both juvenile
and young adult  rats. No changes oc-
curred in mean clara cell volume or in
average clara cell basement  membrane
                             surface area. The changes found in cil-
                             iated cells are illustrated in Figure 5.
                               The effect of ozone on terminal bron-
                             chiolar cells are subtle, especially when
                             compared with changes induced  in the
                             epithelium of the proximal alveolar region
                             after exposure to the same concentra-
                             tions of ozone. These differences may be
                             due to the terminal bronchiolar epithelial
                             cells being less susceptible to this con-
                             centration of ozone than are the cells of
                             the alveolar epithelium. Alternatively, it
                             may be due to the fact that the epithelium
                     Total Volumes of Alveolar Tissue Compartments
    +50
  £+25
  §
  o
  I
  I
  
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in the terminal bronchiole is covered by a
mucous/serous coat which  may  react
with the low concentrations of Oa and
thereby prevent the Oa from reaching the
underlying cells.

Conclusions and
Recommendations
  EM morphometry is extremely sensi-
tive and particularly suited as a tool to
evaluate health effects of air pollutants
such as ozone at low concentrations. By
the combined use of microdissection and
EM morphometry, we demonstrated in
this study that subchronic exposure to
0.25  ppm  ozone  produced  significant
structural changes in the cells of the ter-
minal  bronchioles  and  their adjacent
alveolar tissues. In addition, inhalation of
0.12 ppm 03, the  current ambient air
quality standard, caused structural chang-
es to occur in the alveolar epithelium
immediately peripheral  to the terminal
bronchioles.
  A wide array of effects have previously
been reported as a result of subchronic
exposure to ozone. These investigations,
although mostly at higher concentrations
of Oa, were essentially in agreement with
the results of the present study  in the
location and nature of the injury invoked
by ozone. The major impact of the current
study is that by using quantitative tech-
niques subchronic exposure to ozone at
extremely  low levels can be shown to
cause structural changes in lung cells
which  are  suggestive of injury.  These
changes can be detected at the current air
quality standard of 0.12 ppm Oa. Because
the long-term effects of lung cell injury
caused by low levels of 03 are not known,
chronic exposure to Oa at near ambient
levels should be performed and adverse
health  effects carefully defined.
   J. D. Crapo, B. E. Barry, andR. R. Mercer are with Duke University Medical Center,
     Durham, NC 27710.
   Jean Wiester is the EPA Project Officer (see below).
   The complete report, entitled "Morphometric Studies of the Effects of Ozone on
     Rodent Lungs, "(Order No. PB 85-207 470/AS; Cost: $8.50, subject to change)
     will be available only from:
          National Technical Information Service
          5285 Port Royal Road
          Springfield. VA2216J
          Telephone: 703-487-4650
   The EPA Project Officer can be contacted at:
          Health Effects Research Laboratory
          U.S. Environmental Protection Agency
          Research Triangle Park, NC27711
                                                                                 RnutPWMCWTDDiMTiur:ncLirt iooc/cm in

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