United States
 Environmental Protection
 Agency
 Industrial Environmental Research
 Laboratory
 Cincinnati OH 45268
 Research and Development
 EPA-600/S2-82-063  Sept. 1982
Project Summary
Chemical Stabilizers for  the
Control of  Fugitive Asbestos
Emissions  from  Open Sources

Paul K. Ase, Roger Koch, and George Yamate
  Quarried serpentinite, recently
found to contain asbestos, is used as
aggregate  for surfacing secondary
roads. Emission concentrations of
0.6 x 106 to 8 x 10* fibers/m3 were
collected 20m downwind from a
serpentinite surfaced roadway. These
levels correspond to emission factors
of 34x1010 to 370x1010 fibers/km-
vehicle at vehicular traffic speed of
13.4 m/sec (30 mph).
  Chemical treatments were tested
for controlling these asbestos emis-
sions. Laboratory tests were developed
for screening  51 candidate commer-
cial materials. Four of the most
promising were field tested. Asbestos
emission reductions of up to 90%
were achieved with  chemical treat-
ments at application rates  ranging
from $0.08/m2 to $0.25/m2. Similar
emission reductions were observed
with traffic speeds reduced  to 6.7
m/sec (15 mph).
  This Project Summary was devel-
oped by EPA's Industrial Environ-
mental Research Laboratory, Cincin-
nati. OH. to announce key findings of
the research project that is fully
documented in a separate report of the
same title (see Project Report ordering
information at back).

Introduction
  Quarried serpentinite crushed stone
is the major source of crushed stone
where it is readily available  and in
localities where access to limestone is
limited. Limestone is preferred because
it  is a sedimentary  material, and
therefore has better weathering prop-
erties. Serpentinite is used as road
aggregate material for parking lots,
driveways, and country roads. It is also
used as base course for highways, as
concrete aggregate, and as binder filler
for  asphalt paving.  Serpentinite rock
formations occur at or near the earth's
surface in  many regions of eastern
United States. Belts of  serpentinite
extend from Maine to Alabama, covering
much of the  Appalachian Moutains.
Serpentinite is native to extensive
regions of the western United States
also.
  The bulk  of serpentinite quarried in
the United States for crushed stone is
made up of antigorite. However, chryso-
tile, tremolite, deweylite, talc, antho-
phyllite, and  other silicate minerals
have been reported to occur in serpen-
tinite. Dustfall collected along roads and
trails in a  western recreational area
located over a  serpentinite massif
contained 90 percent chrysotile. On the
other hand,  the average concentrations
of asbestos in quarried  serpentinite
crushed stone ranged from 10 * 1010
fibers/g to 100 * 10'° fibers/g, repre-
senting roughly  0.1 to 1% by weight
asbestos in  the quarried stone.
  The erosive action of vehicular
passage is much more  intensive than
the action of wind alone. The large dust
plume in the wake of an automobile on a
dirt road gives visible demonstration to
the intense dust generating forces that
accompany vehicular traffic on unpaved

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roadways (See Figure 1). The mechan-
ical  action of the tires on the road
surface  kicks up  dust particles  and
places them  directly into  suspension.
The  simultaneous turbulence of vehic-
ular  movement adds more suspension
in the wake.  Large  dust  plumes are
formed which are  easily dispersed by
the faintest air currents.
  On unpaved crushed stone roadways,
the pressure of vehicular  tires on the
road surface applies an intense grinding
action on  the unbound  rock  which
replenishes the fines lost to suspension.
Since the effect of vehicular traffic is
much more  severe than the action of
wind alone, the amount  of stabilizer
material needed to control roadway
emissions is also  much greater than
that  required to control wind erosion.
  The present program was undertaken
to determine the extent to which dust
control  agents might provide control
over asbestos emissions from the use of
crushed  serpentinite rock  on  unpaved
roadways. Laboratory tests were devel-
oped to screen control agents and levels
of their application. In all, 69 materials
were considered.  Of these, 51 were
screened in  the laboratory tests. Three
levels of application, based on cost of
control agents, were tested. Transmis-
sion electron microscope (TEM) analysis
of air samples collected near  the
roadway were used to evaluate the
effectiveness  of  four of the most
promising control agents in field appli-
cations.

Conclusions

  Serpentinite is native to many parts of
eastern  and western United States.
Serpentinite rock  in some of  these
regions is quarried and is used locally as
aggregate for surfacing  material on
secondary  roads.  The quarried ser-
pentinite is known  to contain asbestos.
  Chemical stabilizers were tested for
controlling  asbestos emission from
unpaved roadways surfaced with crushed
serpentinite. Significant asbestos emis-
sions over  background  levels were
measured on the  untreated roadway.
Emission factors of 34 x 1010  to 370 x
1010  fibers/km-vehicle were  reached
for a vehicular traffic  speed of 13.4
m/sec  (30 mph). These emission
generation  levels corresponded to
ambient concentrations of 0.6 x 106 to 8
x 106 f/m3 at 20 m downwind from the
road. Fiber emission reductions of 80 to
90 percent were achieved with chemical
treatment. Similar  reductions were
Figure 1.  Large dust plume in the
          wake of an automobile on a
          serpentinite crushed stone
          road.

achieved with reduction in traffic speed
to 6.7 m/sec (15 mph).
  The asbestos emissions were essen-
tially all  chrysotile  asbestos. The
observed fibers were all in the respirable
range and averaged <0.1 fjm indiameter
and  <2 //m in length.  The emission
fibers were classified  in terms of four
structural  forms: individual fibers,
matrices, bundles, and clusters. The
fiber structures found in the  roadway
emissions were mostly either  single
fibers or fibers attached to rock matrix
material. Very few bundles or clusters of
fibers were found.  Fiber structures
found in the emission from the untreated
roadway section and the treated roadway
sections were indistinguishable.
  Respirable  emission levels  were
much lower than projected from the
concentration of asbestos fibers in the
dust from fresh quarry crushed aggre-
gates. This may be due, in part, to the
manner in which the serpentinite  tends
to break up  along asbestos-containing
seams during crushing.  It may also be
due, in  part, to the  presence  of larger
aggregates in which the fibers are still
bound and not released.
  The field-tested treatments showed
that they were each capable of control-
ling asbestos emissions. The treatment
choice would depend on a number of
factors  including: availability  of  treat-
ment, equipment on  hand, and local
climatic conditions.  More extensive
testing could be used to refine application
strategies. These  should be tailored to
the  physical nature of the  individual
treatments and anticipated local condi-
tions. Under the most severe weather
conditions, traffic  controls could also be
used to hold down emissions. Alterna-
tively, significant  emissions reductions
might  be achieved  by removing the
initial fines  from  the freshly produced
aggregates.
Methodology
  There is no data on the comparative
effectiveness of stabilizers for the
present application,  i.  e., to control
emission  of  asbestos from crushed
stone roadways. Stabilizers were se-
lected from those which showed prom-
ise  in other applications such as soil
stabilizers,  as palliatives for treatment
of unpaved roadways, and for application
on asbestos waste piles, as well as other
more recent commercial materials. Of
69 chemical agents originally selected,
51 were laboratory tested.
  A  number of desirable properties for
chemical agents are needed for them to
act as effective stabilizers including low
application cost,  water solubility, high
bondability to the particles, long life and
stability, resistant  to heat and cold,
nonphytotoxicity, biodegradability, no
drainage  water pollution problems,
ease of  cleaning  from  application
devices, and effectiveness at  low
dilutions. In addition, for  roadway use it
would be useful for the chemical agents
to have a regenerative capacity in order
to maintain control action in spite of the
continual generation of  fresh particu-
lates from the pulverization of surface
materials.
  The stabilizer cost was used as a basis
for comparing stabilizer effectiveness in
the laboratory tests. Application rates of
$0.01/m2, $0.05/m2, and $0.25/m2
were selected. These rates were based
on bulk material prices and the amount
of each  material required for a 1 m2 x
2.54 cm (1  in.) deep application.

Laboratory Tests
  In the laboratory screening tests, the
main emphasis was placed  on the
measurements  of  treatment  control
effectiveness. Ball milling was selected
to simulate the wear action of vehicular
traffic over crushed stone road beds,
and  the  fine fractions, measured by
sieve analysis, were used to determine
stabilizer  effectiveness. The  overall
laboratory test procedure used a series
of six consecutive steps:
  1. Sample Preparation — Weighing
     and Drying,
  2. Initial Sieve Analysis,
  3. Treatment Application,
  4. Rain Cycling,
  5. Traffic Simulation,  and
  6. Final Sieve Analysis.
  The treatment effectiveness of each
stabilizer treatment was calculated as
the weight fraction of fines <140 mesh
found in each sample after the traffic
simulation compared to the  weight

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fraction of fines <140 mesh  found
initially in each sample. The treatment
effectiveness  is referred to here as the
Treatment Score (TS):
TS _   Final Wt % <140 mesh
       Initial  Wt % <140 mesh
where the Wt % is based on the total dry
sample weight.  The treatment effec-
tiveness,  TS  (treatment),  is further
normalized by comparison  with the
treatment effectiveness of the control,
TS  (control),  treated with  water only.
The value for  the normalized treatment
effectiveness  is referred to as Relative
Treatment Score (RTS):
           TS (treatment)
                                                                                           Wind
            TS (control)
The  RTS is the ratio of the treatment
effectiveness for a particular stabilizer
at a  selected  treatment level (e.g.,
$0.01 /m2, $0.25m2) compared to the
effectiveness with only water (control).
The value for TS (control) was calculated
from the average of randomly selected
control samples.

Field Tests
  Four  of the most highly ranked
laboratory treatments were selected for
field testing: Coherex (oil byproduct
emulsion), SS-1H (asphalt emulsion),
Liquidow (aqueous  calcium chloride),
and  Orzan  GL-50 (ammonium  liquo-
sulfonate). These  treatments were
applied on the roadway and upwind and
downwind high volume  air  sampling
stations were  positioned to  collect
emissions. The collected high volume
filter samples were  analyzed by trans-
mission electron  microscope (TEM)
methods for ambient air asbestos.
  A public secondary road in Maryland,
surfaced with  crushed serpentinite,
was selected  for field testing.  The
crushed serpentinite rock used on the
road was produced locally. This aggre-
gate material is used on approximately
60 miles of  unpaved secondary roads
throughout the country. Fresh crushed
serpentinite, crusher No. 6 (~<7.5 cm)
was applied during the summer along a
5OO-m field test section.
  The field treatments were applied
in the fall. A section of roadway  was
prepared for each of the four treatments
and a fifth was used as a control section
with no treatment, as shown in Figure
2. Applications were made with readily
available road  working  equipment:  a
water sprinkler truck and a road grader.
The grader was used to serape the road
surface to a depth of 2.5 cm (1 in.), and
this was done just before each treatment
                 UpwindSamp/ing Sites D-
              --D
                6
N
t





5.
-+ j I\|\\\N t,

Test Sections
4. 3.
\v\\N_-
Holy Cross Road Ammonium Coherex
Lignosulfonate 20m
twnwind Sampling Sites d
5
-D--
30m

2.
-i\\\\TLi\\\\s/ _
QJI Calcium
EmulsionChloride
--D 	 D--
432


1.
fs ^ x \ \N
Control
--D
'
                                                 Weather O  ' <
                                                 Station

Figure 2.  Field test sections on crushed serpentinite roadway, each   5.5m x 67.5m.

Table 1.    Comparison of Laboratory and Field Application Rates.

                                             Application Rate
Laboratory
Treatment
Coherex (oil byproduct emulsion)
SS-1H (asphalt emulsion)
Liquidow (calcium chloride)
Orzan GL-50 (lignosulfonate)
1/m2
1.8
2.3
7.2
7.2
(gal. /yd2)
(0.4)
(0.5)
(1.6)
(1.6)
Field
1/m2*
1.5
2.3
2.3
2.3
(gal. /yd2)
(0.33)
(0.5)
(0.5)
(0.5)
*Treatments were diluted for ease of application and applied at the rate of 4.5 1/m2 (1
 gal./yd2) of the diluted treatment.

application. The treatment and their
application rates are shown in Table 1.
  The test sections, each 67.5 m (220ft)
long and  5.6 m (18.5  ft)  wide, were
separated  by 23 m (75 ft) long inhibited
sections on which the emulsion oil was
applied to minimize "cross talk" between
the sections. (Figure 3.)
  All  treatments, except  the SS-1H,
emulsion  oil, were  applied  from  the
water truck. All treatments were made
as  single  applications. The amount
needed for a 2.5 cm (1 inch) depth was
mixed for each test area in the sprinkler
truck  and applied through a sprinkler
bar. Between 6 to 10 passes of each
treatment were  used to get uniform
application and to permit the treatments
to soak in. (Figure 4).
  After each treatment application, the
grader was used to mix the treatment
into surface layer by blading. (Figure 5).
In this operation the wetted,  treated
aggregates were bladed to the center of
the road  from each side. Then  the
central pile was spread out and a crown
formed in the middle of the road. (Figure
6). This procedure was used to provide
intimate mixing of the aggregates with
the treatment. Several additional passes    Figure 4.  Application of a treatment
were then made by the grader to roll out               from the water truck to a test
the surface.                                       section.
Figure 3.  Emulsion oil application to
          minimize "cross talk"
          between test sections.

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Figure 5.   Grader used to mix the treat-
           ment into surface layer by
           blading.
 Figure 6.  Central pile spread out to
           provide intimate mixing of
           the aggregates with the
           treatment.

  Upwind/downwind air samples were
collected immediately after application
of treatments and six months later, in
the spring. These ambient air samples
were collected with high volume sam-
plers on 20.3 cm x 25.4 cm membrane
filters. The downwind  high volume
samplers were located 20 m downwind
of the road centerline and aligned with
the average wind direction through the
middle of each roadway test section.
Two upwind stations were located 30 m
upwind of the roadway, 150 m apart. At
the beginning and end of each run high
volume sampler flow rates were verified
with a magnehelic gauge  calibrated
with a high volume air sample calibrator.
Meterological information was obtained
continuously from a recording weather
station which was located in  an open
field 40 m south  of the control section.
The instrument  readout was used to
align the sampling stations with the test
sites  and the current average  wind
direction.  Tests  were conducted only
when the average wind direction was
perpendicular to  the roadway.
   Ambient air samples were  collected
 on membrane filters. The bulk of the
samples were collected on 0.4 /um pore
diameter polycarbonate membrane
filters. In addition, 0.8 fjm pore size
cellulose mixed ester membrane filters
were used to collect emission from the
control section in parallel with  the
polycarbonate filter samplers. A What-
man 41 cellulose filter was used as a
backup support filter for each membrane
filter. At  the  end of each  run, filter
sections were stored in 150 mm  petri
dishes and returned to the laboratory for
analysis.
  The filter samples were prepared and
analyzed  in  accordance  with EPA's
provisional methodology for ambient air
asbestos.  The EM grid samples were
examined with a JEOL 100C analytical
electron microscope in the Transmission
Electron Microscope  (TEM) mode. Grid
samples were screened initially under
low magnification by TEM to determine
suitability for further examination. In this
inspection the grid was examined for
loading, uniformity, lack of processing
contamination, adequacy of clearing,
and damage. Inadequate grids were
either reprocessed or discarded and
reprepared from another filter section.
  Acceptable  prepared samples were
examined at  a 20.000X magnification
for chrysotile  and  amphibole asbestos
fibers. Fibers with length to width ratios
of greater than 3:1  and substantially
parallel sides were recorded. The fibers
were classified as:
  • chrysotile asbestos
  • amphibole asbestos
  • ambiguous (incomplete spot pat-
     tern)
  • non-asbestos (definitely some
     other mineral)
  • no pattern (unknown, no  spot
     pattern).
Fibers were classified based on mor-
phology and recognition of selected area
electron  diffraction  (SAED) pattern.
TEM  morphology  and SAED patterns
from  standard samples were used as
guides for fiber identification.  Fibers
showing the tubular structure of chry-
sotile are tentatively classified as
chrysotile  but morphological features
alone are not sufficient to distinguish
chrysotile  and  amphibole from other
fibrous minerals. A recognizable SAED
pattern is used to confirm identification.
Pattern recognition is not always easy
for ambient  air samples which  can
include interference from nearby part-
icles and attached aggregates.  Due to
the very light fiber loading encountered
in the field samples, the procedures for
counting at low  loading  levels were
followed. The entire grid opening was
scanned  and the entire grid openinc
was considered as a single field. Each
grid opening was scanned in a series ol
parallel  scans across  the grid until a
total of  10 grid openings or 100  total
fibers were counted, whichever occurred
first. In the roadway emission samples,
fibers were identified in several contexts
with other particulates,  not currently
considered under the provisional meth-
odology.
  These were characterized as asbestos
structures. The effective concentration
and desposition pattern in the respiratory
system will be affected by the asbestos
content and on the aerodynamic size of
individual asbestos  structures. The
individual "fiber" is a  form of asbestos
structure which  is isolated from all
other particulates. The other structural
forms are  "bundles", "clusters", and
"matrices", by themselves or in com-
binations. A bundle is a single entity
composed  of  fibers  in  a parallel ar-
rangement with  each fiber  closer
together  than one fiber diameter. A
cluster is a single entity composed of
numerous fibers in random orientation
with all  other  fibers  intermixed  in a
single group. A matrix is a fiber with one
end free and the other  end embedded in
some other material. Each  of these
asbestos structures were included  as
single asbestos entities  in the analysis
for asbestos fibers, provided it met the
test for asbestos by  morphology and
SAED pattern.

Results
  The transmission electron microscope
was used as the principal analytical tool
for the field sample measurements. In
general, the filter loadings were all very
light. The asbestos fiber concentrations
on a count basis were mainly all
chrysotile. The overall amphibole  fiber
concentration  was <3 percent. While
the amphiboles found were all single
fibers, chrysotile occurred about equally
as  single  fibers and as matrix  fibers.
Bundles and clusters  were only occa-
sionally observed.
  The asbestos emissions concentra-
tions from the road were determined as
the  difference between upwind and
downwind concentrations based on the
TEM fiber counts. These observed levels
of asbestos concentrations were used to
estimate emission factors. In the control
section,  the emission  factor (f/km-
vehicle) varied from 32 x 10'° to 370 x
1010 fibers/km-vehicle corresponding
to net emission concentrations of 0.6 x

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10e to 7.7 x io» fibers/m2. The lowest
levels were collected in mid-fall just
after  treatment application while the
highest levels were collected during the
following spring. With chemical treat-
ment, overall fiber emission reductions
of 80 to 90 percent were achieved.
  Two stabilizer mechanisms for asbes-
tos emission control were identified:
   1) Stabilizer  which  forms a solid,
     water resistant surface coating
     and binds road aggregates togeth-
     er — This type is represented by
     SS-1H and Coherex, both of which
     are petroleum byproducts. After 6
     months, they still retained better
     than 80 percent emission reduction
     when  applied at the level of
     $0.20/m2 to $0.25/m2.
   2) Stabilizer  which forms a water
     soluble surface  matrix which
     binds surface particles together —
     This type may not control aggregate
     wear as well as the first, but is
     able to rewet new particulates and
     repair worn surfaces to minimize
     emission. This type is represented
     by Liquidow (calcium chloride) and
     Orzan GL-50 (ligno-sulfonate).
     The first is hygroscopic and main-
     tains a high moisture presence in
     the road surface. The second fills
     the voids and can be redispersed
     by precipitation. These showed
     little  emission control after 6
     months when applied at the rate of
     $0.08/m2, but periodic reapplica-
     tion can be used to  maintain
     emission control.
   Essentially all of the asbestos found in
the downwind air samples were within
the  respirable  range, (<3.5 /urn  in
aerodynamic diameter). A large fraction
of the fibers were still attached to matrix
particulates. This suggests  that the
fibers in serpentinite, which occur  in
thin veins and bundles, are in intimate
association with the matrix rock but are
easily separated into small, thin fibers
which are then emitted.
  However, the concentration of asbes-
tos  collected from the  control section
emissions were  much lower than
expected based on the level of fines  in
the road surface aggregates and the on
average concentration of  asbestos
found in fresh  quarried crushed stone.
Several  factors may contribute to this
reduced  level  of asbestos emissions
found.
  When fresh  aggregate is  laid on the
road, the fiber release may be relatively
high. However, the original free fibers
may soon be depleted by being emitted
into  the air or  by being washed away.
When subsequent grinding of the larger
aggregates replaces the original fines
with others which  contain  reduced
concentrations of  asbestos,  the long-
term asbestos emissions from the road
will be reduced correspondingly.
  Those fibers  buried in the aggregates
could not be identified  and were not
counted. Thus, the presence of these
fibers would not be evident under EM
analysis. Also, much of the fugitive dust
ejected from an unpaved road are large
particulates, which deposit close to the
edge of the road. Fibers bound in such
large particles did not reach  the
samplers and thus were also excluded
from analysis.
   Paul K. Ase, Roger Koch, and George Yamate are with IIT Research Institute.
     Chicago, IL 60616.
   Mary K. Stinson is the EPA Project Officer (see below).
   The complete report, entitled "Chemical Stabilizers for the Control of Fugitive
     Asbestos Emissions from Open Sources," (Order No. PB 82-249 905; Cost:
     $9.00. subject to change) wilt be available only from:
           National Technical Information Service
           5285 Port Royal Road
           Springfield, VA 22161
           Telephone: 703-487-4650
   The EPA Project Officer can be contacted at:
          Industrial Pollution Control Division
          Industrial Environmental Research Laboratory—Cincinnati
          U.S. Environmental Protection Agency
          Edison, NJ 08837
                                                                                . S. GOVERNMENT PRINTING OFFICE: 1982/659-095/539

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