\ V
                 United States
                 Environmental Protection
                 Agency
Atmospheric Research and Exposure•>",.
Assessment Laboratory         ^-'
Research Triangle Park NC 27711   ',
                 Research and Development
 EPA/600/S3-89/012  June 1989
&EPA        Project Summary
                 Interim  Report:  Quality
                 Assurance  Support  for the
                 National  Atmospheric  Deposition
                 Program and  National Trends
                 Network  Monitoring  Activities:
                 1987-1990
                 David S. Bigelow
                  The full report  summarizes the
                 quality assurance activities of the
                 NADP/NTN  Quality Assurance
                 Manager from mid-1987 through mid-
                 1988. The report presents  some
                 accomplishments and makes recom-
                 mendations for the network.
                  The report  discusses data quality
                 issues relating  to site representa-
                 tiveness, field  versus laboratory
                 measurements of  pH, site operator
                 turnover rates and various monitoring
                 network reviews.  The report also
                 contains  the previously released
                 "NADP/NTN Instruction Manual for
                 Site Operation" and the "Quality
                 Assurance Report of NADP/NTN
                 Deposition Monitoring for Laboratory
                 Operations" as well as an NADP/NTN
                 quality assurance bibliography.
                  Recommendations emphasize the
                 quality assurance  manager's role in
                 coordinating quality  assurance
                 activities, the need for more inte-
                 grated quality assurance evaluations,
                 the  need  to standardize quality
                 assurance data reporting formats and
                 data transfer protocols in the network
                 and the need  for establishing  a
                 method for estimating  overall
                 precision and accuracy in spatial and
                 temporal data summary statistics.
  This Project Summary was  devel-
oped by ERA'S Atmospheric Research
and Exposure Assessment Laboratory,
Research Triangle Park, NC,  to
announce key findings of the research
protect that Is fully documented In a
separate report of the same title (see
Project Report ordering Information at
back).

Introduction
  The National  Atmospheric Deposition
Program (NADP) monitoring network
began operations in July of 1978. The
Network  uses  cooperating local, state,
and federal agencies  as well as  private
industry to operate a network of sites
according to a single set of protocols. In
1983, NADP assumed responsibility  for
managing the  day-to-day operations  of
the National Acid Precipitation Assess-
ment Program's National Trends Network
(NTN).  This action  resulted in the
combined, cooperative monitoring pro-
gram now  known as the NADP/NTN
monitoring  network.  The NADP/NTN
monitoring network  serves both the
National  Atmospheric Deposition Pro-
gram and the National Acid Precipitation
Assessment Program.
  Because  the NADP/NTN monitoring
program  both  represents and relies  on

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many  different  public  and private
agencies  to  accomplish its  goals, it  is
unique in its  structure  and  mode of
operation. For quality assurance, this has
meant that  responsibility for  the
development of  quality  assurance
programs has been and continues to be a
voluntary  effort assumed by each of the
agencies who have  responsibility for
managing  specific network  operations
(i.e.,  Field  Sites, Central  Analytical
Laboratory,  Coordination  Office, U.S.
Geological Survey, U.S.  Environmental
Protection  Agency).  These quality
assurance procedures are  then reviewed
and  accepted by the various  NADP
committees who  have responsibility for
overseeing each network function.  This
practice has been strongly  encouraged
since it would require considerable effort
and expertise to  centralize this function
within a single organization.
  A  decentralized approach  to  quality
assurance,  however, creates  its own
problems.  Many  of the network quality
assurance procedures are  innovative
adaptations  of   recognized  quality
assurance practices,  and  as  such  are
reported in the scientific literature, at
professional and technical  meetings or  in
various agency reports rather than in  a
standard network document or operating
procedure  publication.  This  lack of
centralized quality assurance reporting
makes  documenting the achievement of
network data quality goals  and objectives
difficult and  also  makes  it  difficult to
continue  some key  quality  assurance
programs once scientific recognition for
the techniques has been  achieved.  The
likelihood that those  quality  assurance
activities that cannot be maintained by a
single agency, either because of financial
or  cooperative  restraints,  will be
overlooked is also increased.  Finally,
decentralized reporting  can  lead to
situations where  results from one effort
may conflict  with another such  that no
clear picture  of 'true' data  quality  can
emerge.
  Recognizing the  need  for  a more
coordinated  and thorough  quality
assurance program,  NADP  formed  a
study committee  in 1982 to address this
issue.  The  work of this  committee
resulted in the development of a Quality
Assurance Plan to cover  all  aspects  of
network operation and the recommenda-
tion  that  a full time  Quality Assurance
Manager  be appointed to  administer this
quality  assurance  program.  The
desirability  of a coordinated  quality
assurance program was again recognized
in  the NAPAP Peer  Review  held in
Boulder, Colorado in 1985.

Accomplishments

Coordination of NADP/NTN
Quality Assurance Plan
Implementation
  The primary coordination efforts have
involved attending the frequent  NADP
Technical and Subcommittee meetings;
writing, revising and  reviewing  NADP/
NTN documentation;  reviewing  agency
reports and  proposals  that  utilize
NADP/NTN  data or documentation; and
disseminating quality assurance informa-
tion to the various NADP committees and
scientists. Each of these activities serves
as a vehicle for obtaining and document-
ing the quality assurance activities of the
network and for promoting the evaluation
and reporting of quality assurance data.
  An additional part of the coordination
effort has involved overseeing the  Site
Visitation program and providing admin-
istrative assistance  to the program's
auditors. The Quality Assurance Manager
is  responsible for distributing the  results
of  the site  audits  and  for  initiating
corrective  action  to  correct any  dis-
covered deficiencies.  As with all of the
external quality  assurance programs,
results are reported separately by each
sponsoring agency.

Review and Revision of the
NADP/NTN Quality Assurance
Plan
  During October of  1986, the  NADP
Quality Assurance Steering Committee
began the task of reviewing and  revising
the NADP Quality Assurance  Plan. As
part  of this  process,  external  reviewers
were asked  to make  suggestions to
improve the  plan. By 1987  reviewer
comments  had  been  received  and
assignments  made   for revising  all
portions of  the  Plan.  This process
continues  with the  Quality Assurance
Manager taking  a lead  role  in the
development  of the Data Management
portion of the Plan. A first revised  working
draft was completed in August of 1988.
  As part of this revision and in response
to  reviewer comments, a Remedial Action
Plan (RAP) was developed for correcting
instances of  non-compliance detected
during network operations. The RAP was
completed and approved in  November
1987. It outlines for  the  first time the
responsibilities of the subcommittees and
program managers for resolving netwoi
deficiencies.


Review and Evaluation of
NADP/NTN Network Operations
  Four areas of Network operations wer
targeted for review during the past ye<
by the Quality Assurance Manager. Th
reviews covered  regional  represents
tiveness of NADP/NTN monitoring dab
differences between NADP/NTN labors
tory  and field  data, turnover rates  c
NADP/NTN site operators and  the revie'
and  revision  of  the  site operator'
instruction manual.


Future Needs of the NADP/NTN
Monitoring Network

Precision and Bias Estimates
  A proposal for establishing NADP/NTf
network precision and accuracy wa
developed and  submitted for  funding it
September 1987. The proposal outlined .
duplicate sampling program to determim
the precision and  accuracy  of NADP
NTN weekly  data, seasonal  summarie
and  regional estimates of depositioi
based  upon  monitoring network  data
Estimates  of  precisions were  to com*
from a proposed within network colocatet
sampling program.  Bias and accurac;
were to be  estimated  using  data fron
existing  between  network colocate<
sampling programs and the  propose<
colocated sampling  program. Th<
proposal  was accepted but not funded
Unfortunately  this leaves  the  networl
without the  means to establish  the
precision and accuracy estimates callec
for in the NADP Quality Assurance Plan
Data from which estimates  of precisior
can  be made  are available at only twc
locations and for  limited  time periods
One location in North Carolina producec
data only for  one year.  The  seconc
location in Wisconsin has only  18 month;
of  data.  Neither  location  can  be
considered as representative of the entire
network and  neither can  be  used  foi
estimates of bias.
  In addition  to duplicate sampling,  the
proposal described a second program fpi
determining  precision  and bias of rair
gauge measurements. In  this seconc
program,  precision would  have  beer
determined by the rain gauge's ability tc
weigh a  known amount of  sand at  twc
reference  points within the instruments
working range. The reproducibility of the
difference between the known sand bottle

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 weight  and  that  measured  by  the
instrument at the reference points  would
have been a measure of the precision or
random error.  The magnitude of  the
difference would have been a measure of
bias or systematic  error. The  lack of
funding of  this portion of the proposal
leaves the  network with no  means to
establish rain gauge performance  in the
network. Similar rain gauge performance
tests were  discontinued in 1983 due to
lack of funding.
  Overall seasonal and  regional  esti-
mates of precision  and accuracy of
NAOP/NTN rain and chemistry data will
have to be inferred from other monitoring
network  data  (e.g.,   Electric Power
Research Institute's daily  Operational
Evaluation  Network, National Weather
Service's  climate  center, etc.) or be
computed piece-meal from the volume of
agency information  specific  to  each
network related study.  The  quality  and
completeness of this latter approach has
never been assessed. Even if this latter
approach were successful,  it is antici-
pated that  much of the error estimates
used in computing overall error estimates
will have to  come from 'related studies.'

Addition of a Second Laboratory
to the NADP/NTN Monitoring
Program
  One of the more time consuming tasks
of the past  contract period has been the
addition of  a second  laboratory to  the
NADP/NTN monitoring program. Because
of contracting requirements,  site liaison
and the chemical analysis  of samples
from  18 NADP/NTN  monitoring  sites
administered by  the  National  Park
Service were performed by  a second
laboratory  from  March  24  through
September  29.  1987.  During this  time
period, the Quality Assurance Manager
was required to provide additional  SOP
and QA documentation to  the second
laboratory as  well as coordinate  the start
up of  internal and external quality assur-
ance  programs  that  would eventually
allow the  evaluation of the  second
laboratory's data in  relation to the data
from  the  original  laboratory.  At  the
request of the National Park Service, two
audits of  the  new  laboratory  were
conducted, one prior to  the start  of
operations and  one approximately four
months into the contract. Completed data
and   some  documentation became
available in the early summer of 1988.
  A  number  of  inconsistencies  with
previous NADP practices have prevented
a full evaluation of the data. Work is
currently  scheduled, subject to  funding,
for the fall of 1988 to reevaluate field data
in a  manner consistent with  prior
NADP/NTN practice. Chemistry data will
require more  documentation before an
evaluation of comparability  can be
initiated.  Audit  reports  are  available
through the National Park Service's Acid
Rain Coordinator in Washington, DC.
  Briefly, no  serious deficiencies were
found in the laboratory's operations.
Many of the 'problems' noted in the audit
were  associated  with data management
and  site  liaison  activities. Most were
correctable. Some  of the noted  defi-
ciencies might have been more easily
correctable if better documentation  of
NADP/NTN standard  operating  proce-
dures in these areas was available. The
quality of chemistry results simply lacked
documentation. This  does not necessarily
indicate a lack of quality, only that quality
is undefined.
  The NADP/NTN  quality  assurance
activities  and  their sponsoring agencies
are listed  in Table 1.

Recommendations
• The Quality  Assurance  Manager's
  participation in auditing,  document
  reviews and scientific meetings should
  continue to be supported. These are
  the windows through which  the  QA
  Manager can view the network opera-
  tions.
• Standard formats and transfer protocols
  for  external quality  assurance  data
  needs to be  established  to  eliminate
  redundant data entry and to enable the
  timely transfer  of  quality assurance
  data  from  the  agencies  to  the
  NADP/NTN Coordination Office.

• Continue to evaluate  and document
  network data quality and  network
  procedures through  the publication of
  integrated  quality assurance  reports.
  These reports should be inclusive  of all
  years of operation through current  time.

• Studies  like the field versus laboratory
  pH  evaluation should be  increased to
  further  document the  limitations and
  strengths of the NADP/NTN data set.

• Establish the  Quality Assurance  Man-
  ager and quality assurance  technician
  roles as full time  positions. This should
  help increase the frequency  of  inte-
  grated  quality  assurance  reports and
  allow for continuity in the tracking of
  network  quality  assurance  activities.
  The current three-quarter  time staffing
  level provides only enough resources
  to manage the  NADP/NTN quality
  assurance program on a topical basis.

• The network should continue  to
  organize and gather information which
  profiles each of its monitoring stations.
  This information should be maintained
  and organized in such a way as  to
  facilitate the  selection  of  sites for
  regional and topical data analysis.

• A quality assurance program specif-
  ically designed to estimate  network
  precision  and  bias  should  be
  developed  and implemented as  soon
  as  possible. Emphasis should be
  placed  on  comparisons within NADP/
  NTN and between peer network data.

• The comparability of NADP/NTN  data
  to that  of other major  networks
  operating in North America should be
  established.

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Table 1.    NADP/NTN Monitoring Network Quality Assurance Activities and Their Sponsoring Agencies
         Task No.                       Task Name                  Operating Agency"
                                                                        Program Name
 Field Site Operations:
            1.
            2.
            3.

            4.
Quality Control of Field Operations        CAL
Quality Assurance of Field Operations     CSU
Systems and Performance Audit of Field   EPA (RTI)
Operations
Quality Assurance of Site Chemical       USGS
Analysis
                       CAL Site Interactions
                       Across Site Network Analysis
                       NADPINTN Site Visitation Program

                       Intersite Comparisons
 Laboratory Operations:
            5.
            6.
            7.
Laboratory Quality Control
Laboratory Quality Assurance
Laboratory Systems Audit
CAL
CAL
NADP Subcommittee 2
CAL QA Program
Interlaboratory Comparisons
 Data Management:
            8.

            8.

            9.

           10.
Quality Control of Site/Chemical Analysis
Data through Data Management
Quality Control of Site/Chemical Analysis
Data through Data Management
Quality Control of Data Management

Quality Assurance of Network Data
Management
CAL
CSU
PNL
QA Steering Committee
Data Screening and Coding

Data Screening, Coding and
Summary Reporting
Acid Deposition System (ADS)
for Statistical Reporting
Systems and Performance Audit
of (he Data Management Program
 Network Operations:
           11.

           12.
           13.

           14.

           15.

           15.
Performance Audit of Field and
Laboratory Chemical Analysis
Laboratory Quality Assurance
Performance Audit of the Network

Special Studies which Assess Various
Components of Network Performance
Systems Review of the Deposition
Monitoring Network
Systems Review of the Deposition
Monitoring Network
USGS

USGS
CSU

ALL

TASK GROUP 4

QA Steering Committee
Blind Audit Program

Interlaboratory Comparisons
Network Intercomparison's
with CANSAP/CAPMoN
Published Scientific Research Results

NAPAP Annual Review

IR-7 Annual Review
•CAL-Central Analytical Laboratory, Illinois State Water Survey
 CSU-Natural Resource Ecology Laboratory, Colorado State University
 EPA-Environmental Monitoring Systems Laboratory, Environmental Protection Agency
 PNL-Battelle's Pacific Northwest Laboratory
 RTI—Research Triangle Institute, Research Triangle Park, NC
 USGS-National Water Quality Laboratory, U.S. Geological Survey
 Task Group 4—National Acid Precipitation Assessment Program (NAPAP)
 QA Steering Committee—National Atmospheric Deposition Program

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David S.  Bigelow is with the Colorado State University, Fort Collins, CO.
Berne I. Bennett is the EPA Project Officer (see below).
The complete report, entitled "Interim Report: Quality Assurance Support for the
  National Atmospheric  Deposition  Program  and National Trends  Network
  Monitoring Activities: 1987-1990" (Order No. PB 89-155 220/AS; Cost: $36.95,
  subject to change) will be available only from:
        National Technical Information Service
        5285 Port Royal Road
        Springfield, VA 22161
        Telephone: 703-487-4650
The EPA Project Officer can be contacted at:
        Atmospheric Research and Exposure Assessment Laboratory
        U.S. Environmental Protection Agency
        Research Triangle Park, NC 27711
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
Official Business
Penalty for Private Use $300

EPA/600/S3-89/012
          0000329    PS

          U  S  *ȴIR PROTECTION  AGENCY
          CHlCftSO
                                    *»-   60604

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