United States Environmental Protection Agency Environmental Monitoring Systems Laboratory Research Triangle Park NC 27711 Research and Development EPA/600/S4-86/042 March 1987 v>EPA Project Summary Investigation of Source Emission PM10 Particulate Matter Field Studies of Candidate Methods William E. Farthing, Ashley D. Williamson, Sherry S. Dawes, Randal S. Martin, and James W. Ragland The full report describes the field evaluation of two candidate methods for source PM-10 measurement. The two techniques are a new sampling train design using emission gas recycle (EGR) and a Simulated Method 5 (SIM- SI approach using existing hardware with a specific traversing protocol. Four field tests were performed. At each test site, the EGR and SIM-5 measurements were compared with reference mea- surements of PM10 and/or total par- ticulate mass measurements. At two sites, the EGR and SIM-5 measure- ments were run simultaneously and compared to each other. The test results are presented, and the conclusions derived from these results are discussed. Also, recommendations are made for procedural and hardware refinements of each method. Tn/s Pro/ecf Summary was developed by EPA's Environmental Monitoring Systems Laboratory, Research Triangle Park, NC, to announce key findings of the research project that Is fully docu- mented In a separate report of the same title (see Project Report ordering In- formation at back). Introduction A size-specific PM,0 ambient-air par- ticulate standard has been proposed and promulgation is expected. The introduc- tion of size into the definition of sus- pended paniculate matter in the ambient air suggests the need for measurement of size-specific emissions from stationary sources. Technology related to such mea- surements has been developed in con- nection with evaluation of control devices on process streams. Inertia! impactors and cyclones can separate or classify aerosol particles in situ but are more complex to operate than total paniculate mass trains. Furthermore, operation of these devices for typical engineering evaluations does not require the docu- mented accuracy and reproducibility desired for established sampling methodology. The technical difficulties in size-specific (i.e., PM,0) paniculate sampling are greater than, but similar to, those of total paniculate sampling by EPA Reference Methods 5 or 17. Potential sampling biases exist due to variations in the spatial distribution of paniculate concentrations across the sampling plane defined by the duct cross-section. Likewise, temporal variations in paniculate concentrations due to process variations can cause in- accurate or unrepresentative emissions measurements. EPA Reference Methods for paniculate sampling (Methods 5 and 17) deal with these problems by specifi- cations on the sampling location to minimize stratification (Method 1) and by spatial and temporal averaging using a traversing protocol which collects a weighted average of the paniculate emis- sions at an array of points spanning the sample plane. Method 5 specifications also require at least 3 separate mea- surements, allowing further temporal averaging. A second potential error in paniculate measurements is duct/nozzle sampling bias. Unless the gas velocity entering the sampling nozzle equals the local duct velocity, paniculate matter will be selectively depleted or enriched in the sample gas stream due to inertial separa- ------- tion at the nozzle entrance. For total paniculate sampling, this bias may be restricted by specifying isokinetic sam- pling (within a 10% tolerance) at each point. This tolerance is easily attained in sampling that is not size specific by vary- ing the sample flowrate so that nozzle is within 10% of stream velocity. These potential problems are made more severe in PM10 sampling by the fact that inertia! size segregation must be performed. Any inaccuracies in the in- ertial cutoff diameter, which is determined by sample flowrate, will lead to errors in the PM,0 measurement by misclassifica- tion of paniculate matter in the size range near 10 jum. Inertial sizing devices (im- pactors and cyclones) are available which have a sufficiently sharp collection effici- ency cut at 10/um, but only for specified flowrates which are dependent on gas temperature and composition. Without a sampling nozzle of continuously variable cross-sectional area, this fixed flowrate requirement makes isokinetic sampling in the manner of Method 5 impossible. Since an isokinetic sampling bias can be significant for particles near 10/im. this effect cannot be ignored. Previous work on this problem at Southern Research Institute has led to the development of two potential sampling methods the Emission Gas Recycle (EGR) sampling train, and the Simulated Method 5 (SIM-5) traversing protocol. The Emission Gas Recycle (EGR) Train in principle eliminates the problem of anisokinetic sampling bias by simulta- neously allowing isokinetic sampling by the nozzle and fixed flow operation at the inertia! sizing device(s). The train design allows the isokinetic flow of gas into the sampling nozzle to be augmented by an adjustable amount of filtered, recycled stack gas upstream of the inertia! sizing device. The SIM-5 protocol is an alternate candidate PM10 method in which existing sampling equipment (cyclones or cascade impactors without special gas recycle adaptations) are used. The objective of the protocol is to reduce anisokinetic sampling errors to the approximate range expected from spatial and temporal varia- tion of emissions. Anisokinetic sampling bias is kept in this range by synthesizing a full duct traverse from partial traverses at constant sample flowrate. Points for each partial traverse are selected that have duct velocities in the range to keep anisokinetic sampling errors for 10 /im particles below ±20% at each point. Procedure Emission Gas Recycle (EGR) Train A block diagram of the prototype field EGR train is shown in Figure 1. Stack gas is isokinetically extracted through the sample portion of the EGR mixing nozzle into the inertia! sizing component of the sample train. After passing the inertia! sizing device and instack sample filter, the sample gas passes through the probe and condenser or impinger train and into the EGR flow control module. As in con- ventional Method 5 control modules, the gas flowrate entering the control module is controlled by coarse and fine control values (V, and V2, respectively) at the entrance of the sealed pump. At the exit of the pump and absolute filter, the total flow is measured using a laminar flow element (LFE). The gas stream is then split into the recycle and sample flow lines. The sample flow is monitored in the normal manner using a dry gas meter and a calibrated orifice. The recycle gas flowrate is measured using a second LFE. The partitioning between sample and recycle gas is controlled by a valve (V3) located downstream of the LFE. Valve V4 was added to the system to extend the range of control to higher recycle per- centages by adding back pressure to the sample flow line. The recycle gas line, along with the sample and pitot lines, passes through the heated probe in which the recirculated gas is reheated to the duct temperature. Power to the heater is regulated by a proportional temperature controller using a thermocouple reference sensor located in the gas stream downstream of the heater. In the course of this field measurement program, size specific paniculate mea- surements were made with two types of inertia! sizing devices. Direct PM10 size fractionation was performed using the first cyclone of the SoRI/EPA Five Stage Series Cyclone sampling train. This cyclone was used for all EGR testing and much of the SIM-5 testing. The remainder of the SIM-5 testing and other reference size distribution measurements were performed using University of Washington Mark V Cascade Impactors. EGR Test 1 The first field test of the (EGR) system at a stationary source took place at one of two twin 56 MW coal-fired boilers at a utility generating station. The test plan consisted of two subtests. Subtest A in- volved the comparison of traverses per- formed with the EGR train and a standard Method 17 train. To eliminate spatial bias, a two-probe setup was configured. One probe was configured with a cyclone set using an EGR nozzle. Colocated with the cyclone set was a Method 17 probe with a 47mm filter. Three traverse points were selected which represented the maximum point-to-point velocity change accessible to the EGR probe through one of three six-inch ports. The recycle rate was adjusted to achieve isokinetic sam- pling at each point while maintaining the chosen constant flowrate through the cyclone set. The flowrate through the colocated 47mm filter was adjusted ai each point to sample isokinetically. Tota paniculate mass concentrations mea sured by the two trains were compared In Subtest B, the EGR-Method 17 hard ware previously described was usec without modification. A third probe with a cyclone using a non-recycle nozzle was used for a "near-colocated" reference Sampling for this subtest took place at i single point. The nozzle for the non recycle cyclone was chosen to provide t 10jum cut at the isokinetic sample flow rate. The EGR cyclone was fitted with < smaller nozzle. The recycle rate was ther adjusted to provide the flowrate require* through the cyclone for a 10/im size cu as well. The gas flowrate in the Methoi 17 sampler was adjusted in the usua fashion to maintain isokinetic conditions Total mass concentrations measured b all three trains and PM-10 concentration obtained from the two cyclone trains wen compared. SIM-5 Test 1 The first field test of the SIM-5 samplin protocol took place at the same 56 MV coal-fired boiler used for the EGR shake down. The test plan consisted of thre subtests. In all subtests the SIM-5 sizin devices were modified University c Washington Mark V cascade impacton In Subtest A, three probes were usec Both a Method 17 and a SIM-5 impactc were used in a twelve point traverse c the duct area using the SIM-5 samplin protocol. The impactor was operated at constant flowrate while the flowrat through the Method 17 was changed s as to be isokinetic at each of the travers points. A simultaneous 50 point travers of the duct was made with the thir probe operated according to EPA Refe ence Method 17. The total particulal mass determined by each device w£ compared. For Subtest B, three identic ------- EGR Probe Assembly Recycle Line Sample Inlet V3 Recycle Flow LFE ! ! Sealed Pump Sample Orifice Exhaust Dry Gas Meter Figure 1. Schematic of the emission gas recycle train. impactors sampled simultaneously at the same point. To quantify the magnitude of error in PM,0 determinations resulting from anisokinetic sampling error, one impactor sampled isokinetically while the remaining two operated at the upper and lower limits of acceptability according to the SIM-5 protocol. The PM-10 masses obtained from each were then compared. For Subtest C, three points in the sample plane were chosen with widely differing velocities. Identical impactors were op- erated simultaneously, one at each point while another identical sampler traversed the same points in one sampling run according to the SIM-5 traversing proce- dure. The single point impactors sampled isokinetically. Again, the PM10 masses obtained by each impactor were compared. EGR/SIM-5 Test 2 The major purpose of the third field test was to provide a direct comparison of the SIM-5 and EGR techniques. Indepen- dent reference measurements were ob- tained with single point isokinetic impactors. The site, a 500 MW coal-fired power plant, was selected to access a duct with velocities near 60 ft/sec, with substantial velocity spread, and with an aerosol mass median diameter in the 7 to 14/im range. The test consisted of three subtests. For Subtest A, a simultaneous three- point traverse of the duct was performed with both the SIM-5 and EGR samplers. Both of these PM-10 sampling trains used Cyclones I and IV of the SoRI/EPA five stage cyclone set followed by a 47 mm filter. For Subtest B, three University of Washington Mark V impactors were run simultaneously as near in time as practical to each set of Subtest A. Each impactor was operated isokinetically at one of the three traverse points used for Subtest A. Subtest C consisted of a single twelve point traverse of the duct with both the EGR and the SIM-5 samplers. The main purpose of this subtest was to determine the problems associated with a nozzle change during the SIM-5 run. EGR/SIM-5 Test 3 The site for the fourth and final test was a 221 MW pulverized coal-fired utility boiler. The test plan was designed to evaluate the EGR and SIM-5 protocols in high and low particulate mass concentra- tions. In the high concentration tests each of the dual inlets of the control device was sampled. Sampling was also done at the outlet of the exhaust stack. This test consisted of five subtests. Subtest A involved a simultaneous twelve point traverse of the duct with the EGR and SIM-5 samplers. Subtest B deter- mined reference size distributions using University of Washington Mark V impac- tors. The cascade impactors were op- erated over the same twelve point traverse used for Subtest A. The traverse was subdivided into four subtraverses, each subtraverse corresponding to a different sample port. Each subtraverse was sampled with a different impactor, using SIM-5 protocol with the flowrate fixed so that the nozzle velocity equaled the mean measured velocity for the three points. Subtest C consisted of Method 17 mass train samples at the inlet to both units of the control device. Subtest D involved simultaneous impactor traverses in the exhaust stack at the outlet of the control device. For Subtest E, Method 17 mass train samples were taken at the outlet sampling site. ------- Results and Discussion As described previously, the EGR and SIM-5 techniques were tested at four sampling locations at three coal fired utility boilers. The sites were selected to provide a range of particulate concentra- tions (15-4000 mg/dnm3) and duct veloc- ities (15-100 ft/sec), significant fractions of particulate larger than 10 micrometers aerodynamic diameter (50-80%), and substantial velocity non-uniformity. At each site the EGR and SIM-5 measure- ments were compared with reference measurements of PM10 and/or total particulate concentrations, and at two sites the EGR and SIM-5 measurements were run simultaneously and compared to each other. Table 1 contains a summary of these comparisons for the field tests in the full report. Several conclusions may be drawn from the field data in Table 1. First,, in every case, the average concentrations mea- sured using different techniques agreed within the combined 95% confidence intervals. Since these intervals for some tests reflect a substantial degree of vari- ation presumably due to source fluctua- tions, a more meaningful comparison can be drawn from paired-run analysis of the simultaneous measurements indicated in Table 1. Since source fluctuations cancel to first order in the comparisons, the confidence intervals are smaller and some observed differences are found to be statistically significant. Thus, for example, the EGR concentrations for both total mass and PM10 are significantly lower than the SIM-5 concentrations at Site 2. Likewise, the EGR concentrations are higher than the SIM-5 values at Site 3. Such differences, even when significant at the 95% confidence level, are not consistent in direction from site to site, and are typically on the order of 10%. These differences may only reflect dif- ferences in operating conditions. We conclude that PM10 measurements using each technique can be expected to com- pare well with the other and with those using other reference techniques. Like- wise, EGR measurements of total mass concentration may be expected to com- pare well with Method 17 measurements were particulate catches are sufficient to allow good recovery from the EGR sampler. Although SIM-5 was not de- signed for total particulate mass concen- trations, in the present test series SIM-5 total mass measurements fell within 15% of values from the EGR and other iso- kinetic samplers. Table 1. Percentage Differences and Confidence Intervals in Particulate Concentrations Measured During Test Series" Number of Replications PMn Total Concentration EGR Initial Test Site 1 EGR Cyclone Isokinetic Cycloneb EGR Method 17" SIM-5 Initial Test Site 1 4 8 -8.3±27% 9.O±29% -11.5±8.3% SIM-5 Method 17± SIM-5 Isokinetic Impactor^ EGR/ SIM-5 Comparison Test Site 2 EGR Cyclone - SIM-5 Cyclone* EGR Isokinetic Impactors SIM-5 Isokinetic Impactors EGR/ SIM-5 Comparison Test Site 3 EGR-SIM-5* EGR Impactor SIM-5 Impactor SIM-5 Impactor Method 1 7 3 4 5 5-6° 7-6f Inlet 6 6-5= 6-5= Outlet 6-7 -1.8±22% -15.5±6.5% -11±31% 3.8±25% 11 ±9.8% 27±16% 16±16% -16±32% -14.0±65% -9.2±8.5% 1.3±38% 14±31% 1.7±21% -9.8±16% -11±14% -7.4±23% " All differences and confidence intervals expressed as percentages of the mean value. Confidence intervals represent 95% significance level. * These comparisons were analyzed as pairs since the measurements were simultaneous. c Where two numbers of replications are given, the first number corresponds to the first listed device and the second to the second device. Recommendations We have several recommendations for further study. First, we feel that both techniques are sufficiently advanced that they should be documented in detail for potential use as sampling methods if source PM10 regulations are issued. Second, they should be subjected to more extensive validation and collaborative testing than was possible during this project in order to further define precision, reproducibility, comparability with other measurements, and possible sources of interference of bias using each technique. It is also recommended that further development of both techniques continue to refine procedural details and investigate hardware improvements. These include development of an EGR impactor train, further characterization of impactor pre- cutters and the existing PM10 Cyclone (SoRI-l), investigation of an alternate geometry Cyclone I, and investigation of the optimum use of S-type pitot tubes with instack PM10 samplers. ------- William E. Farthing, Ashley D. Williamson. Sherry S. Dawes. Randal S. Martin, and James W. Raglandare with the Southern Research Institute, Birmingham, AL 35255-5305. Alice C. Gagnon is the EPA Project Officer (see below). The complete report, entitled "Investigation of Source Emission PM^P articulate Matter Field Studies of Candidate Methods," (Order No. PB 87-132 841 / AS; Cost: $18.95, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at: Environmental Monitoring Systems Laboratory U.S. Environmental Protection Agency Research Triangle Park, NC 27711 United States Center for Environmental Research Environmental Protection Information Agency Cincinnati OH 45268 Official Business Penalty for Private Use $300 EPA/600/S4-86/042 0000329 PS ------- |