&EFK
                United States
                Environmental Protection
                Agency
                           Environmental Monitoring
                           Systems Laboratory
                           Research Triangle Park NC 2771 i
                Research and Development
                           EPA/600/S4-87/007 June 1987
Project Summary
Stability of Parts-Per-Billion
Hazardous Organic Cylinder
Gases and Performance Audit
Results of Source Test and
Ambient Air Measurement
Systems-Status Report #3
                J.M. Allen, C.K. Sokol, R.K.M. Jayanty, C.E. Decker and O.J. von Lehmden
                   An evaluation of 27 gaseous
                 organic compounds at parts-per-
                 billion (ppb) levels  In compressed
                 gas cylinders has been established
                 under a contract with the United
                 States Environmental Protection
                 Agency  (USEPA).  The primary
                 objectives of this on-going project
                 are: (1) to evaluate the quality of
                 measurements made by USEPA,
                 state/local agencies,  or their
                 contractors  by using  ppb  gas
                 cylinders for performance audits to
                 assess the relative accuracy of
                 source measurement  systems
                 during hazardous waste trial burn
                 tests and ambient  air monitoring
                 programs; (2) to verify  the
                 manufacturer's certified analysis of
                 the multi-component gas mixtures;
                 (3) to determine the stability of the
                 gas mixtures with time; and (4) to
                 develop  new  audit materials as
                 requested by USEPA.
                   The cylinder consists of  four
                 mixtures of five, six, eight and  nine
                 organic compounds each. These
                 mixtures were blended  by a
                 commercial  gas supplier in
                 aluminum cylinders in a balance gas
                 of nitrogen. The five-component
                 mixture (Group I) contains carbon
                 tetrachloride, chloroform,  tetra-
                             chloroethylene (perchloroethylene),
                             vinyl chloride and benzene. The
                             nine-component mixture (Group II)
                             includes trichloroethylene, 1,2-
                             dichloroethane    (ethylene
                             dichlorlde), 1,2-dibromoethane
                             (ethylene dibromide), acetonitrile,
                             trlchlorofluoromethane (F-11),
                             dichlorodifluoromethane (F-12),
                             bromomethane (methyl bromide),
                             methyl ethyl  ketone and 1,1,1-
                             trichloroethane.  The eight-
                             component mixture (Group III)
                             includes  pyridine*. vinylldene
                             chloride, 1,1,2-trtchloro-1,2,2-
                             trifluoroethane (F-113), 1,2-
                             dlchloro-l,l,2,2-tetrafluoroethane
                             (F-114), acetone,  1,4-dloxane,
                             toluene, and chlorobenzene. The
                             six-component mixture (Group IV)
                             includes  acrylonitrlle,  1,3-
                             butadiene,  ethylene  oxide,
                             methylene chloride, propylene oxide
                             and o-xylene.  To date, 95
                             performance  audits have been
                             initiated and 76 are complete. The
                             results of these audits and  a
                             description of the  experimental
                             procedures used for analyses and

                             "Although Group III cylinders contain
                             pygdine, the concentrations are not certified
                             due to severe analytical difficulties

-------
available  stability  data  are
presented in  the status  report.
Generally, the results of the audits
show reasonable  agreement (plus
or minus 50 percent) with the audit
material  concentrations measured
by Research Triangle Institute (RTt),
considering the low concentrations
of the organics and the anticipated
uncertainty  associated  with
independent analyses conducted
by an audit laboratory.
    Stability studies for all Group I,
Group II and Group HI  compounds
(except  pyridine)  have  been
performed. Results indicate that  all
the  compounds tested  are
adequately  stable  for  use   as
reliable audit materials. The Group
IV compounds  will not  be available
for audits  until  stability  of the
compounds has  been  established.
If the data indicate that the Group
IV compounds  are stable, Group IV
mixtures  should  be  available  for
audits on or after December  30,
1986.
    This  Project  Summary  was
developed by EPA's Environmental
Monitoring Systems   Laboratory,
Research Triangle Park,  NC,  to
announce  key  findings  of the
research  project that  is fully
documented in a separate report of
the same title, (see Project  Report
ordering information at back).

Introduction

    The   application   of  Quality
Assurance practices is important to the
generation   of   high-quality
environmental  data.  The  Quality
Assurance  Division  of  USEPA's
Environmental  Monitoring  Systems
Laboratory has  initiated  a program to
supply audit materials  for use  during
hazardous waste trial burn tests and
ambient air measurements. RTI, under
contract to the USEPA , has responded
to this need  through development of
gas  cylinders containing 27 gaseous
organic  compounds at ppb  levels in
compressed gas  cylinders.  The
gaseous compounds are  to be used in
performance audits  as designated  by
the  USEPA Project Officer. These
performance audits  are  to assess  the
relative  accuracy   of  source
measurement systems  during
hazardous waste trial burn tests and
ambient air monitoring programs.
    The  audit  materials currently
contain 27 compounds selected on  the
basis of anticipated needs of USEPA's
Office of Solid Waste. Table 1 lists the
four groups of compounds,  the
concentration ranges, and the number
of cylinders in each group. The balance
gas for all gas mixtures is nitrogen and
the cylinder  construction material  is
aluminum.
    The gaseous  compounds  are
acquired from commercial suppliers  in
compressed  gas cylinders.  These
cylinders, in conjunction with  an
appropriate delivery  system, are used
directly  as  sources of  the gaseous
compounds during performance audits.
The accuracy of the supplier-reported
levels of these compounds is  verified
through  measurement  using
commercial   permeation  tubes  or
specially prepared standards supplied
by the National Bureau  of Standards
(NBS) as compressed gas mixtures  in
aluminum cylinders. The permeation
rates  of the  commercially available
tubes are verified gravimetrically  by
RTI before use.
    The accuracy  of  the cylinder
concentrations and  the verification  of
stability of the  compounds  in the
cylinders are important. Along with
acquisition of new compounds  and
verification of their  concentrations, an
extensive stability  study is  being
performed. This study involves periodic
analyses of the contents of each of the
cylinders in the repository.

Procedure

    Once a mixture of compounds  is
chosen,  a  commercial  supplier  is
contacted to  determine  if a cylinder
containing the compounds of  interest
can  be  prepared.   If  so,  the
manufacturer prepares  the cylinder
gases   and  determines   the
concentration  of  the analytes  in the
cylinder at  least  two  times.  The
cylinder  is  sent to RTI where  its
contents are  analyzed, usually within
ten days of its arrival. If the RTI value
varies from the manufacturer's value by
more than 25 percent, reanalysis may
be performed by  a third  party (USEPA
or NBS). The gas mixtures are again
analyzed at  2 months, 6 months,  12
months and on a  yearly basis following
the initial analysis  to determine the
stability of the gas mixtures.
    All analyses for Groups I, II and III
mixtures  are performed using   a
Hewlett-Packard  5880A   gas
chromatograph equipped with  flame
ionization  and  electron  capture
detectors.  The electron  capture
detector  (ECD)  has   been  used
principally  for measurement  of all the
halogenated hydrocarbons except vinyl
chloride.  Vinyl chloride,  benzene,
methyl ethyl ketone, acetonitrile,  all
Group III compounds, and  all of the
Group I  compounds  in  the  high
concentration  range cylinders  are
analyzed with the FID.  The  gaseous
samples are injected onto the column
by  means  of  two Valco  six-port
sampling  valves mounted  near the
injection port. One  valve is equipped
with interchangeable sampling loops (1
cc and 3 cc) to allow the injection of
different  volumes of gas.  The  gas
chromatographic parameters used in
the  measurement  of  individual
compounds in  Group I, Group II and
Group III are described in the status
report.  The gas  chromatographic
parameters  for  the  Group  IV
compounds have not been established.
    Permeation tubes are  generally
used  as  calibration standards for all
Group I  and Group  II compounds. The
permeation rate of each  permeation
tube is determined every 15 to 60 days
by  weight-loss determination of  each
tube.  A compressed  gas  cylinder
standard mixture obtained from NBS is
used  for the calibration  standard  for
Group III  compounds.  A similar NBS
standard will be used for the calibration
of Group IV compounds.
    RTI  supplies  cylinder gases  for
audits upon  request from the  USEPA,
state  or  local  agencies or  their
contractors. When  a  request  is
received, the cylinder is then  shipped
by  a  freight carrier  to the  laboratory
being  audited. A letter is also included
with the  cylinder  which  provides
general instructions for performance of
the audit. The audit concentrations  are
provided  to the requesting  agency
Audit  Coordinator. After the laboratory
being audited  has  analyzed  the
contents of the cylinder,  the  Audit
Coordinator reports the value(s) to RTI,
which in turn reports both the measured
and accepted  values  to  the Project
Officer. There is no charge for the audit
except for the cost of returning  the
audit cylinder.

Results and Discussion

    To  date, 95 performance audits
have  been initiated; 76 are complete.
The results are given in the  status three
report. Generally, the audit results are
within  ±50 percent  of  the  audit
concentrations  measured by RTI.
    Relative accuracies  of the cylindei
gas analyses for Group  I, Group II  and

-------
 Tabto 1. PPB Ural Organic QMM Currently AvaHabto
  Group
Number of Cylinders
Concentration Ranoe of Each Compound (OOP)
  Group I*


  Group II"

  Group Ill-

  Group IV*
      20
      12
      12
      12
       6
       9
       3
      12
       6
               7-90
             90-430
            430-10.000
               7-90
             90-430
               7-90
             90-430
               7-90
            430-10.000
      Group I Compounds: Carbon tetrachtoride. chloroform, tetracNoroethytene (perchtoroetnytene), vinyl chloride and benzene.
      Group II  Compounds: Trichloroethvtene, 1,2-dichtoroethane. 1,2-dibromoethane, acetonitrile, trichlorofluoromethane (F-11),
      dichlorodifluoromethane (F-12). bromomethane, methyl ethyt ketone, and 1,1,1-trichtoroethane.
      Group III Compounds:  Pyridine, VinyWene Chloride, 1,1,2-trichloro-  1,2,2-trifluoroethane (F-113),  1.2-dichloro-1,1.2.2-
      tetrafluoroethane (F-114), acetone, 1,4-dioxane, toluene, and  cNorobenzene.
      Group IV Compounds: Acrytonrtrite, 1,3-butadiene, ethylene oxide, methytene chloride, propytene oxide, and o-xytene. These cylinders
      should be available tor performance audits on or after December 30,1986.
Group  III compounds  have  been
determined  using  NBS  primary
standards. An examination of the data
in the status report  to  assess long-
term stability shows that values for the
compounds in the Group I, Group  II
and Group III repository cylinders vary
by  less  than 10  percent for 3  to  5
analyses over a one-year period. This
variation indicates the imprecision of
the  measurement process.  The
possible sources of experimental error
that could contribute to this variability
include:  (1)  the variability of  the
sampling  injection technique used for
analyses;  and  (2)  the  instrumental
variability in  operating  and detector
parameters. Each of  these  sources of
variability contributes  to the  net
uncertainty  of the resulting stability
data.  Estimates of total  uncertainty
(repeatability) for  Group I compounds
have  been determined to  be in the
range of  2.1-3.2% (coefficient  of
variation) at 95% confidence limits. The
estimate of total uncertainty for Group II
compounds has been determined to be
in the range of 3.4-7.0% (coefficient of
variation) at 95% confidence limits. The
total  uncertainty for the  Group  III
compounds   with  the exception  of
acetone and 1,4-dioxane  has been
determined  to be in the range of 9-
12%  (coefficient of variation) at 95%
confidence  limits.  Acetone and 1,4-
dioxane  initially had  quite high total
uncertainties  in the range of 30-50%
(coefficient   of  variation) at  95%
confidence limits,  due to  difficulties in
the analysis  of these two compounds.
The analytical difficulties from  which
       those high uncertainties  arose have
       been partially  resolved. The total
       uncertainties for  acetone  and  1,4-
       dioxane are presently in the range of
       30-32%  (coefficient of  variation)  at
       95% confidence limits. The stability of
       a compound may be  suspect  if a
       change  in  concentration over time is
       noted that exceeds the 95% confidence
       limits. An examination  of such data
       indicates that the Groups I, II. and III
       compounds in the repository  cylinders
       have continued to remain stable.

       Conclusions

           Compressed  gas  cylinders
       containing  27  gaseous  organic
       compounds at  parts-per-billion levels
       has been used successfully in audits to
       assess  the  relative accuracy  and
       precision  of  analytical systems,
       especially those used during hazardous
       waste trial  bum  tests and ambient air
       monitoring. To  date. 95 performance
       audits have been initiated and 76  are
       complete. Generally the audit results
       are within  ±50 percent of the audit
       concentrations measured by RTI.
           Stability studies for 21  of the 27
       gaseous  organic  compounds included
       in the cylinders have been performed
       to determine the feasibility  of using
       them as audit  materials.   Results
       indicate that all of the organics tested
       are stable enough for use as reliable
       audit  materials.  The  Group  IV
       compounds  will not be  available  for
       audits until  the  stabilities of the
       compounds have been  established. If
       the data indicate  that  the  Group  IV
       compounds  are  stable.  Group IV
       mixtures should be available for audits
       on or after December 30,1986.

-------
 J. M. Allen. C. K. Sokol, R. K. M. Jayanty, and C. E. Decker are with Research
   Triangle Institute. Research Triangle Park, NC 27709; the EPA author Darryl
   J.  Von Lahmden (also  the EPA Project  Officer, see below) is with the
   Environmental Monitoring Systems Laboratory Research Triangle Park, NC
   27711.
 The complete report, entitled "Stability of Parts-Per-Billion Hazardous Organic
   Cylinder Gases and Performance Audit Results of Source Test and Ambient
   Air Measurement Systems—Status Report #3," (Order No. PB 87-168 8037
   AS; Cost: $18.95, subject to change) will be available only from:
         National Technical Information Service
         5285 Port Royal Road
         Springfield, VA 22161
         Telephone: 703-487-4650
 The EPA Project Officer can be contacted at:
         Environmental Monitoring Systems Laboratory
         U.S. Environmental Protection Agency
         Research Triangle Park. NC 27711
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
Official Business
Penalty for Private Use $300

EPA/600/S4-87/007
      0000329   PS

          S
                                       60604

-------