vvEPA
                                United States
                                Environmental Protection
                                Agency
                                Industrial Environmental Research
                                Laboratory
                                Research Triangle Park NC 27711
                                Research and Development
                                EPA-600/S7-82-029 Oct. 1982
Project Summary
                                Effects  of  Fuel  Properties and
                                Atomization  Parameters  on
                                NOX Control  for  Heavy Liquid
                                Fuel Fired  Package  Boilers

                                G. C. England, D. W. Pershing, M. P. Heap, and J. E. Cichanowicz
                                 Experimental  studies were con-
                                ducted to (1) relate the formation of
                                NO* in  liquid fuel flames  to the
                                chemical/physical fuel properties and
                                to the atomizer design, and (2)
                                investigate the interaction between
                                liquid sprays and airflow pattern for
                                conditions typical of package boilers.
                                These experiments were conducted in
                                an 880 kW firetube boiler simulator
                                and in a 21 kW tunnel furnace, under
                                both normal and staged combustion
                                conditions.
                                 The fuels studied were primarily
                                conventional heavy residual fuel oils
                                covering a wide  range of properties;
                                however, shale- and coal-derived
                                liquids were also tested. Fuel nitrogen
                                content of the liquid fuels was found
                                to be the only first order parameter
                                affecting NOx emissions for a given
                                spray/flow field  configuration under
                                excess air conditions.  The tunnel
                                furnace results indicated, however,
                                that (during staged combustion) fuel
                                nitrogen speciation has a second-
                                order effect on the minimum achiev-
                                able NOx level.
                                 The boiler simulator studies showed
                                that atomizer design, spray/flow field
                                configuration, and fuel composition
                                are significant dependent parameters
                                affecting NOx emissions. Cold-flow
                                spray characterization  using laser
                                diffraction showed that, in general,
                                drop size information  alone was
                                insufficient to predict NOX emissions
                                in complex flow fields under normal
                                combustion; however, staged  com-
                                bustion was found to be more effective
                                with atomizers which produced smaller
                                droplets.
                                 Staged combustion was an effective
                                NOx control for all liquid fuels tested.
                                Optimization of staging parameters
                                (e.g., mixing and primary zone time/
                                temperature history) is indicated to
                                achieve maximum NOX reduction
                                using staged combustion.
                                 This Project Summary was developed
                                by  EPA's Industrial Environmental
                                Research  Laboratory. Research Tri-
                                angle  Park, NC. to announce key
                                findings of the research project that is
                                fully documented in a separate report
                                of the same title (see Project Report
                                ordering information at back).

                                Introduction
                                 Although increased coal use partially
                                solves the U.S. energy crisis,  many
                                industrial users will continue to burn
                                liquid fuels. However, the composition
                                of these fuels will change as premium
                                fuels are  reserved  for  transportation
                                and domestic use. Industrial users will
                                be required to burn  heavy petroleum-,
                                coal-, and shale-derived residual oils, all
                                of which have relatively high nitrogen
                                contents  and low hydrogen-to-carbon
                                ratios. Unless appropriate pollution
                                controls are applied, use of these fuels
                                will increase NOx or paniculate  emis-
                                sions from stationary combustors firing

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these fuels. The production of N0xand
participate in turbulent diffusion flames
depends on the fuel composition and
the fuel/air contacting process.  The
latter depends on the complex interaction
of the  liquid  fuel  spray from the
combustion air flow field.
  The overall goal of this study was to
provide  the information  necessary to
develop  and generalize low NOX oil
burner  technology for application to
package firetube boilers. Specific objec-
tives of the research were:
  • To relate the formation of NOX in
    liquid fuel flames to the chemical
    and  physical fuel  characteristics
    and to the atomizer design.
  • To investigate the  interaction be-
    tween liquid sprays and the airflow
    pattern for conditions typical of
    package boilers under normal and
    staged conditions.
  Two combustors (Figure 1) of different
scales were used to provide information
to assess the  impact  of liquid spray
characteristics on NOX formation and to
relate the formation  of NOX  under
normal  excess air and staged heat
release  conditions to  the liquid  fuel
properties.

Experimental Systems

Tunnel Furnace
  The down-fired tunnel  furnace was
designed to allow utilization of commer-
cially available atomizers and to be fired
with both artificial oxidants and air. The
small-scale combustor was 2.1 m long
with  an I.D. of 0.2 m. The walls were
insulating and high temperature castable
refractory,  and  the  nominal  full-load
heat  release was 70,000 Btu/hr (21
kW).  In  certain  investigations  the
combustion air was enriched or replaced
with  varying amounts of CO2, Ar, and
02, all of which were supplied from high
pressure cylinders.  The furnace was
fired with  a commercial air-assisted
ultrasonic atomizer  which was  used
because  it provided adequate atomiza-
tion of the viscous liquid fuels at these
low flow rates.

Boiler Simulator
  Experiments at  larger scale were
carried out in  an axisymmetric calori-
metric combustor with a nominal firing
rate of 3 x 106 Btu/hr (880 kW). This
pilot-scale combustor was divided into
calorimetric sections cooled by heat
transfer fluid and had a length of 3.2m
and  an  I.D. of approximately 0.58m.
The double-concentric burner  could
accept a wide range of commercially
available fuel  nozzles.  The unheated
combustion air was supplied through an
annular duct with an axial velocity of
30m/sec. Swirl level could be varied by
interchangeable fixed-vane  annular
swirl generators.

Analytical System
  Identical  sampling  and analysis
systems,  used for both combustors,
     Viewing
      port
          allowed for continuous monitoring of
          NO, NOX, CO, C02, 02, and SOz using
          commercially available  instruments
          Flue  gases were withdrawn  from the
          appropriate combustor exhaust through
          a water-cooled stainless steel probe

          Fuel Effects
            The work  focused primarily  on  13
          petroleum-derived heavy fuel oils, but
          also considered three distillate oils, four
    Oil heater
   connection
Combustion
    air
 air
__O/7 Pressure
       Tap
 Oil inlet
                                       Tunnel furnace
                               Flue
   Recycled flue products
                       To atmosphere

                     Stac,1'
                 To A ux.
                  heat
               exchanger
                          Connective heat exchanger
Fuel
                                                               Observation
                                                                 window
                                                              Access
                                                               port
                         Modular calorimetric
                           cooled sections
Figure 1.  Combustors used in experiments.
                                                 Boiler simulator

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 shale oil  blends, and one coal-derived
 liquid (Figure 2).

 Excess  Air Combustion
   Figure  3  is a composite plot of total
 and fuel NOx emissions from the tunnel
 furnace for a wide range of petroleum-,
 coal-, and  shale-derived  liquid fuels.
 Fuel NOx was defined by  replacing
 combustion air with a synthetic oxidant
 mixture containing 21 percent Oa, 20
 percent C02, and 59 percent Ar.  C02
 was added  to the mixture  to  match
 theoretical  flame temperature for the
 air  and  artificial  oxidant cases. Both
 total and fuel NOx emissions increase
 with increasing fuel nitrogen content.
 These data are representative of a high
 mixing intensity  burner with a finely
 atomized spray. Fuel NOX emissions
 increase  by approximately 95 ppm per
 0.1  percent nitrogen. Experiments were
      Legend

O Alaskan diesel

A W. Texas diesel
9 California diesel

O Essex County
k Middle east
O Low sulfur #6
A Indo/Malaysian
Q Desulfurized
  Venezuelan
b Pennsylvania

O Gu/f Coasf

O Venezuelan
O Alaskan
 V California #1
 O California #2
 0 California #3

 O California #4
 • Cructe s/?a/e and
  blends with o

<1 Shale-derived DFM
• S/?C //

• Synthoil blends
   with 9

• CM + /V//3
  2.0

  7.S

  /.6
*
gO.5

  0.5

  0.4

  0.2
                    A. I
                                 
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Staged Combustion

  Staged combustion, a cost-effective
control for the  reduction of NOX,
involves operating the combustor to
ensure  that the fuel originally  burns
under oxygen-deficient conditions.
Second stage air is  then added to
complete the oxidation process. Figure
6 shows data  obtained from both the
boiler simulator and the tunnel furnace
                                   using the ultrasonic atomizer and
                                   operated at  3 percent  overall  excess
                                   oxygen.  The  data  is presented as a
                                   function of the stoichiometric ratio of
                                   the primary zone, defined as the fraction
                                   of the theoretical air required  for
                                   complete combustion. Since distillate
                                   oil is essentially nitrogen-free, these
                                   results represent the influence of  the
                                   primary  zone  oxygen on NOx produced
                                   from molecular nitrogen. The data for
     700
      600
     500
 I
     400
300
     200
     100
              4% Excess 62
              Son/core 2507 Atomizer
            [/VOx] = 174 + 572 (%Nj
            (fit - 0.99>
                                                          30° Swirl
                                                          45° Swirl
                                     [/VOx] = 158 + 305 I%N)
                                     (fit = 0.99)
                                 1
                                  I
                    0.2
                           0.4          0.6

                            Wt%N in Fuel
0.8
1.0
Figure 4.  Effect of fuel nitrogen content -- boiler simulator.

                                 4
                      the three residual oils indicate that, as
                      the primary zone becomes progressively
                      more fuel-rich, the ultimate NOx emis-
                      sions decrease dramatically to a mini-
                      mum and  then increase  again. This
                      upturn in emissions at very low stoi-
                      chiometric ratios is probably due to an
                      increase in the concentration of oxidiz-
                      able fuel nitrogen species at the exit of
                      the primary zone. Minimum NOX emis-
                      sions achievable under staged combus-
                      tion conditions for a range of liquid fuels
                      are compared  in Figure 7 Minimum
                      emissions from the boiler simulatorare,
                      in general,  higher than those from the
                      tunnel  furnace,  indicating that  the
                      small-scale furnace provides more
                      optimum conditions for the minimization
                      of NOx production than does the boiler
                      simulator; e.g., time and temperature in
                      the fuel-rich zone. However, the general
                      trends for  both combustors  are  the
                      same. Minimum NOX emissions increase
                      strongly with fuel nitrogen content up to
                      fuel nitrogen levels of approximately 0.5
                      percent, and then show only a  minor
                      increase as the  nitrogen content is
                      increased above 2 percent by weight.
                      The volatility of the nitrogen compounds
                      in the liquid fuel appears to be  the
                      limiting factor in NOx control by staged
                      combustion. Experiments  involving a
                      residual fuel and  a distillate oil doped
                      with pyridine and thiophene to give the
                      same  nitrogen and  sulfur  content
                      showed  minimum  emission levels
                      under staged  conditions  30 percent
                      lower for the doped distillate  than  for
                      the residual fuel.
                                                                                s
                                                                              .270
                                                                          §60

                                                                          S?

                                                                           50
                               0.4    0.8   1.2   1.6

                                   Wt%N in Fuel
                                                                                                               2.0
                      Figure 5.   Composite fuel nitrogen
                                conversion to NOx as a
                                function of fuel nitrogen
                                content -- tunnel furnace.

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Atomizer Effects
  A goal of this program was to assess
the impact of atomizer characteristics
on  pollutant production under both
excess air and staged  combustion
conditions. Commercial atomizers were
selected for use in the boiler simulator
and the characteristics of six  of these
atomizers were determined in a cold-
flow test  rig  using  a  laser diffraction
droplet size analyzer.
                                        Flow Field Interaction
                                          In a given flow field, NOX formation
                                        depends on the atomizer type. Figure 8
                                        shows  data  for several commercial
                                        atomizers, four of which  were char-
                                        acterized by the laser diffraction analy-
                                        zer. The Peabody and Todd nozzles pro-
                                        duced similar drop-size distributions
                                        (mean diameter approximately 40/urn).
                                        The largest mean drop size (90/urn) was
                                        produced by the Monarch nozzle; the
  700
£600
Q

O
S?
  500
  400
S
§;300
  700

    0
        O Residual 0.51 %N
        O Residual 0. 36% N
        & Residual 0.24% N
        * Distillate 0.007% N
                           T.unnel
                           rurnace
  I     i    i     i    i
Package boiler simulator
      0.6      0.8       1.0                0.6       0.8

                           Primary zone stoichiometry ratio
                                                                1.0
Figure 6.  The effect of fuel composition on NOxemissions under staged-combustion
          conditions.
 £  500
 £  200
 i
    100
                    Boiler simulator  _+ +
                                                   Liquid Fuel
                                            Petroleum Shale   Coal
                                Boiler simulator   •      *
                                 Tunnel furnace   o      a      O
             _L
                    i
                                      j
                                                  I
                                                        i
                                                                    i
        0    0.2  0.4    0.6    0.8   1.0    1.2    1.4   1.6   1.8   2.0
                                  Wt % in Fuel

Figure 7. Minimum NOx achievable under staged conditions.
Sonicore produced the smallest (21 //m).
Thus,  emissions do not  correlate
directly with drop size. Figure 9 shows
that the impact of nozzle design also
depends'on flow field characteristics.
The effect of increasing swirl is seen to
be different for each atomizer. Varia-
tions  in  swirl level  produce  a large
change in  NOX  emissions with  the
Monarch nozzle, and relatively mild
change with the Delavan atomizer. The
data in Figure 9b illustratethatdropsize
information alone  is not sufficient to
correlate emissions and that the flow
field characteristics can have a signifi-
cant effect with some atomizers.

Staged Combustion
  Increasing the  mean drop size under
staged combustion conditions effectively
decreases  the gas-phase  residence
time  in the fuel-rich primary  zone
because it  increases droplet lifetimes.
Table  1 shows the effect of increasing
mean  drop size  on staged  NOX emis-
sions  measured  in the tunnel furnace
for a given  primary zone stoichiometry
ratio and overall  excess air level. As
drop size increases, the final emission
level  also  increases. However,  this
increase is  less apparent for high nitro-
gen fuels.  Figure 10 compares  NOX
emissions obtained in the boiler simu-
lator under staged combustion condi-
tions with the Sonicore and the Monarch
nozzles for  two different fuels. In both
instances the Sonicore nozzle gives
higher NOX  emissions under excess air
conditions,  but lower emissions under
staged combustion conditions. Smoke
emissions  increased dramatically as
NOX emissions decreased when burning
petroleum-derived residual fuel,  and
nozzle design has the most significant
impact on  exhaust smoke number in
this case. However, with shale-derived
fuel, the smoke emissions are accept-
able with both nozzles under all primary
zone stoichiometries,  but less NO* is
produced when using the  nozzle with
the smaller dropsize distribution.

Summary
  The results of these small -and pilot-
scale studies  of the influence of fuel
properties and spray/flow field interac-
tion indicate that:
  1. With  liquid  fuels,  fuel  nitrogen
     content is the primary fuel com-
     position variable affecting fuel NO
     formation.  NOx emissions in-
     crease with increasing fuel nitro-
     gen content for petroleum-, shale-,
     and coal-derived  liquid  fuels.

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                                                                                       Atomizers
£   260
O
 §:   220
i
     180
                 2.0         3.0         4.0
                            Percent Excess O2
Figure 8.   The effect of spray/flow field interactions.
5.0
                         Monarch
                                                                             Peabody
                                                                       Industrial combustion
                                                                            Delavan
                                                                                                   Son/core
                                             T/#///y%g>^' '-
                                                 Todd
                                                          O
                                                   Delavan
  320
  300
  280
  260

§240
i
  220
  200
      0.2             0.4             0.6
                       Swirl number (SJ
                             fa)
Figure 9.  NOx emissions as a function of drop size.

                                 6
0.8
             O Sonicore
             Q Monarch 30 gph
             A Todd "CDS"
            280
         ^.
         Q
          CN-
         o
         I 240
         O
                                                               200
                 Peabody
                 Delavan "Swirl air"
40          60          80
     Mean drop size, jum
               (b)
100

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Table 1.     Influence of Mean Drop Size on Staged NOt Emissions3
                                         NO* ppm (O% Oa Dry)
Fuel Nitrogen, %
0007
0 16
0.24
0.51
20 fjm
48
85
no
165
180 pm
75
105
140
170
3Tunnel furnace, primary zone stoichiometry is 0.70.
   1400
   1200
   WOO
             Atomizer
       • Son/core  Monarch     f
          o a Petroleum N= 0.5,1%
          • • Shale N , 2.08%/
 Q
 S
 fi

•8
 <0
•5
   800
I
IS'
O
p 600
 I
 *
O
400


200


  0

  8

  6

  4

  2
         0.6    0.8     1.0    1.2

     Primary zone stoichiometric ratio

Figure 10.   Influence of atomizer type
            on staged NOx and smoke
            emissions for the shale
            and petroleum fuels --
            boiler simulation.
   Staged combustion as a control
   technique is effective for all three
   fuels, and minimum levels achiev-
   able with high nitrogen alternate
   fuels approximate those of petro-
   leum fuels with much lower nitro-
   gen contents.
2.  Decreasing  droplet diameter re-
   duces both NOx and smoke emis-
   sions  under staged combustion
   conditions.
3.  Fuel  nitrogen speciation has an
   impact on the effectiveness of
   staged combustion as a control for
   minimizing  NOX  emissions pro-
   duced with high nitrogen fuels.
                                          G. C. England, D.  W.  Pershing, and M. P. Heap are with Energy and Envi-
                                            ronmental Research Corporation, Santa Ana, CA 92705; J. E. Cichanowicz is
                                            with Electric Power Research Institute, Palo Alto. CA 94304.
                                          W. Steven Lanier is the EPA Project Officer (see below).
                                          The  complete report,  entitled "Effects of Fuel Properties and Atomization
                                            Parameters on /VOX Control for Heavy Liquid Fuel Fired Package Boilers,"
                                            (Order No. PBS 2-230 715; Cost: $31.50, subject to change) will be available
                                            only from:
                                                  National Technical Information Service
                                                  5285 Port  Royal Road
                                                  Springfield, VA22161
                                                  Telephone: 703-487-4650
                                          The EPA Project Officer can be contacted at:
                                                  Industrial Environmental Research Laboratory
                                                  U.S. Environmental Protection Agency
                                                  Research Triangle Park. NC 27711
                                                                                                  •USGPO:1982-659-095-537-

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