FEBRUARY 1Q86
       EVALUATION OF THE PEM-2 USING THE

1982 PHILADELPHIA AEROSOL FIELD STUDY DATA BASE
  ATMOSPHERIC SCIENCES RESEARCH LABORATORY
     OFFICE OF RESEARCH AND DEVELOPMENT
    U.S. ENVIRONMENTAL PROTECTION AGENCY
RESEARCH TRIANGLE PARK, NORTH CAROLINA 27711

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       EVALUATION OF THE PEM-2 USING THE

1982 PHILADELPHIA AEROSOL FIELD STUDY DATA BASE
                      by
        Jia-Yeong Ku and K. Shankar Rao
 Atmospheric Turbulence and Diffusion Division
National Oceanic and Atmospheric Administration
          Oak Ridge, Tennessee 37830
              IAG-DW13930021-01-2
                Project Officer

              James M. Godowitch
    Meteorology and Assessment Division
  Atmospheric Sciences Research Laboratory
Research Triangle Park, North Carolina 27711
  ATMOSPHERIC SCIENCES RESEARCH LABORATORY
     OFFICE OF RESEARCH AND DEVELOPMENT
    U.S. ENVIRONMENTAL PROTECTION AGENCY
RESEARCH TRIANGLE PARK, NORTH CAROLINA 27711

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                            NOTICE

    The information in this document has been funded in part by
the United States Environmental Protection Agency under Interagency
Agreement IAG-DW13930021 to the Atmospheric Turbulence and Diffusion
Division of the National Oceanic and Atmospheric Administration.
It has been subject to the Agency's peer and adminstrative review,
and it has been approved for publication as an EPA document.
Mention of trade names or commercial products does not constitute
endorsement or recommendation for use.
                               ii

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                               ABSTRACT
    The Pollution Episodic Model Version 2 (PEM-2) is an urban-scale
model capable of predicting short term ground-level concentrations and
deposition fluxes of one or two gaseous or particulate pollutants at
multiple receptors.  The two pollutants may be chemically coupled
through a first-order chemical transformation.  PEM-2 is intended for
urban particulate modeling, and for studies of the atmospheric trans-
port, transformation, and deposition of pollutants to assess the impact
of existing or new sources or source modifications on air quality.

    This report describes an evaluation of the PEM-2 using Phila-
delphia Aerosol Field Study (PAFS) data for 29 days in the summer of
1982.  The model's performance is judged by comparing the calculated
12-hour and 24-hour average concentrations with the corresponding
observed values for four pollutant species, namely, S02, sulfate, fine
and coarse total mass.  The calculated and observed diurnal variations
of hourly SC>2 concentrations at each of the six PAFS stations are
also compared.  A first-order chemical transformation of S02 to sulfate
is considered in the calculations in addition to the direct emission
and dry deposition of all four pollutant species.  The model%domain,
covering 80 km x 80 km with 32 x 32 grid cells, includes 300'point
sources and 289 area sources in the Philadelphia urban area.  Hourly
meteorological and emission data are used as inputs to the model.

    Statistical tests for evaluation of model performance include
standard measures of differences and correlation between observations
and calculations paired in space and time.  For each pollutant, scat-
terplots of calculated 12-hour average concentrations and differences
versus observed concentrations are presented; a linear regression line
is determined and evaluation statistics are tabulated.  Additional
plots and tables, examining the model performance for daytime,
nighttime, and daily mean concentrations (averaged over all PAFS
stations) are given.  The diurnal variations of S02 concentrations
(averaged over the evaluation days) are also compared at each station.

    The emphasis in this evaluation is on particulate species for
which the model performs well; the variations of 12 and 24-hour mean
particulate concentrations over the evaluation period are simulated
closely.  These results, however, should be interpreted with caution
since the background concentrations far exceed the urban source
contributions to the particulate concentrations in Philadelphia.  The
model performance for SC>2 is better during daytime than at nighttime,
and generally better at the suburban stations than at downtown
stations which are impacted heavily by the urban area sources.

    The work described in this report was performed by NOAA's Atmos-
pheric Turbulence and Diffusion Division in partial fulfillment of an
Interagency Agreement with the U.S. Environmental Protection Agency.
This work, covering the period January 1984 to June 1985, was completed
as of June 30, 1985.
                                 iii

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                            CONTENTS
Abstract ................ . ...................................




Figures [[[ vi




Tables [[[ ix




Acknowledgements .............................................  x




1.  INTRODUCTION .............................................  1




2 .  PHILADELPHIA DATA BASE ...................................  3




        Emissions .............. ............ ..................  5




        Concentrations ..... ... ............. .... ..............  7




        Meteorology .......................................... 11




3.  MODEL EVALUATION ......................................... 17




        PEM-2 Runs ........................................... 17




            Calculation Grid ................................. 18




            Emission Data .................................... 20




            Deposition and Transformation Rates .............. 31




            Model Calculations ............................... 32




            Background Concentrations ....... . ....... . ........ 33




        Evaluation Statistics ................................ 34




4.  RESULTS AND DISCUSSION ................................... 39




        Sulfur Dioxide ...... ......... . . ...................... 39




        Sulfate ...................... . ....................... 55




        Fine Total Mass ...................................... 65




        Coarse Total Mass ..... ............................... 70





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                         FIGURES

Number                                                       Page
  1.  Philadelphia area map with locations of monitoring
      stations in PAFS field program	  8

  2.  Average daytime wind distribution during PAFS 	  13

  3.  Average nighttime wind distribution during PAFS 	  14

  4.  Frequencies (No. of hours) of PG stability classes
      during PAFS 	  16

  5.  Calculation grid used for PEM-2 evaluation showing
      the locations of PAFS stations	,	  19

  6.  Variations of daily total (daytime + nighttime) S02
      emissions from point and area sources in Philadel-
      phia for the evaluation period	  21

  7.  Same as in Fig. 6, except for sulfate emissions	  22

  8.  Same as in Fig. 6, except for fine total mass
      emissions	..»..	.......	  24

  9.  Same as in Fig. 6, except for coarse total mass
      emissions	  25

 10.  Diurnal variation of S02 emissions (averaged over
      the evaluation period) from ooint and area sources
      in Philadelphia	  26

 11.  Same as in Fig. 10, except for sulfate emissions 	  27

 12.  Same as in Fig. 10, except for fine total mass
      emissions	 ...,.,.>	>..t.........	  28

 13.  Same as in Fig. 10, except for coarse total mass
      emissions	..<,..<	 < . ..............  29

 14.  Comparison of calculated and observed diurnal
      variations of S02 concentrations (averaged over the
      evaluation period) at Station 5 . c	  40

 15.  Same as in Fig. 14, except at Station 7	  41

 16.  Same as in Fig. 14, except at Station 8  .,,	  42

 17.  Same as in Fig. 14, except at Station 12	  43

 18.  Same as in Fig. 14, except at Station. 28	  44
                           vi

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                    FIGURES (continued)

19.  Same as in Fig. 14, except at Station 34  	 45

20.  Comparison of calculated and observed 12-hour average
     S(>2 concentrations for the evaluation period	 48

21.  SC>2 residuals (D^^ - 0^ - P^ ) versus observed 12-hour
     average SC>2 concentrations for the evaluation period .. 50

22.  Comparison of calculated and observed daily mean
     concentrations of SC>2 (averaged over all  PAFS
     stations) for the evaluation period	 52

23.  Same as in Fig. 22, except for daytime  (12-hour
     average) S02 concentrations 	 53

24.  Same as in Fig. 22, except for nighttime  (12-hour
     average) SC>2 concentrations 	 54

25.  Comparison of calculated and observed 12-hour average
     sulfate concentrations for the evaluation period 	 56

26.  Sulfate residuals (D^ = 0^ - P^ ) versus  observed
     sulfate concentrations for the evaluation period 	 59

27.  Comparison of calculated and observed daily mean
     sulfate concentrations (averaged over all PAFS
     stations) for the evaluation period 	 62

28.  Same as in Fig. 27, except for daytime  (12-hour
     average) sulfate concentrations	 63

29.  Same as in Fig. 27, except for nighttime  (12-hour
     average) sulfate concentrations 	 64

30.  Comparison of calculated and observed 12-hour average
     FP total mass concentrations for the evaluation
     period	 66

31.  FP total mass residuals (Dj_ = 0± - P^ ) versus
     observed 12-hour average FP concentrations for the
     evaluation period	 68

32.  Comparison of calculated and observed daily mean FP
     total mass concentrations (averaged over  all PAFS
     stations) for the evaluation period 	 71

33.  Same as in Fig. 32, except for daytime  (12-hour
     average) FP total mass concentrations 	 72

34.  Same as in Fig. 32, except for nighttime  (12-hour
     average) FP total mass concentrations 	 73
                          vii

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                    FIGURES (continued)
35.  Comparison of calculated and observed 12-hour average
     CP total mass concentrations for the evaluation
     period	74

36.  CP total mass residuals (D^ =• Oj - PA ) versus
     observed 12-hour average CP concentrations over the
     evaluation period	 76

37.  Comparison of calculated and observed daily mean CP
     total mass concentrations (averaged over all PAFS
     stations) for the evaluation period	 79

38.  Same as in Fig. 37, except for daytime (12-hour
     average) CP total mass concentrations 	„	 80

39.  Same as in Fig. 37, except for nighttime (12-hour
     average) CP total mass concentrations ................. 81
                          viii

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                                TABLES
Number
  1.  PEM-2 evaluation days of PAFS data	..	  4

  2.  Average daytime and nighttime total emission rates from
      area and point sources in PAFS inventory	 30

  3.  Summary of PEM-2 evaluation statistics for S02 	 49

  4.  Summary of PEM-2 evaluation statistics for sulfate	 57

  5.  Results of stepwise regression analysis for sulfate 	 61

  6.  Summary of PEM-2 evaluation statistics for fine
      total mass	 67

  7.  Results of stepwise regression analysis for fine
      total mass 	 69

  8.  Summary of PEM-2 evaluation statistics for coarse
      total mass	 75

  9.  Results of stepwise regression analysis for coarse
      total mass	 78

 10.  Comparison of daily average total emission rates from
      area and point sources in Philadelphia and St. Louis ...... 86
                                 ix

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                          ACKNOWLEDGEMENTS
    This report ts prepared for the Office of Research and Development,




Atmospheric Sciences Research Laboratory (ASRL) of the U. S. Environmental




Protection Agency (EPA) to support the needs of the Office of Air Quality




Planning and Standards in urban particulate modeling.  This work is




accomplished under interagency agreements among the U.S. Department of




Energy, the National Oceanic and Atmospheric Administration (NOAA), and




the EPA.






    The authors thank James Godowitch and Jack Shreffler of ASRL for the




guidance and advice during the course of this work, and for their interest




and patience.  One of the authors (JYK) would like to express his




appreciation to the personnel of NOAA's Atmospheric Turbulence and




Diffusion Division (ATDD), especially to Rayford Hosker and Bruce Hicks for




arranging his visit to ATDD to participate in this project.

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                                SECTION  1








                               INTRODUCTION








    The U. S. Environmental Protection Agency (EPA) recently proposed




revisions to the National Ambient Air Quality Standard (NAAQS) for




inhalable particulate (IP) matter which would base the primary,




health-related standard on particles smaller than 10 microns aerodynamic




diameter (PM-10).  As part of the effort to control urban particulate




emissions, EPA sponsored the development and evaluation of an improved




urban scale model capable of simulating the transport, diffusion, and




deposition of particulate matter.






    The Pollution Episodic Model Version 2 (PEM-2) described by Rao (1985)




is an urban scale (10-50 km) model capable of predicting short term (1-24




hr) ground-level concentrations (GLC) and deposition fluxes of one or two




gaseous or particulate reactive pollutants in an urban environment with




multiple point and area sources.  It is intended primarily for particulate




modeling, and also for studies of the atmospheric transport, transfor-




mation, and deposition of acidic, toxic, and other pollutants to assess the




impact of existing or new sources or source modifications on urban air




quality.  The PEM-2 concentration algorithms (Rao, 1983) explicitly account




for the effects of dry deposition, sedimentation, and a first-order




chemical transformation.






    PEM-2 is based on the Pollution Episodic Model (PEM) developed by Rao




and Stevens (1983).   The latter, in turn, is based on the Texas Episodic

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  Model Version 8 (TEM-8)- developed by the Texas Air Control Board (1979) for




  the atmospheric dispersion of non-reactive pollutants over a perfectly




  reflecting (non-depositing) surface.  Rao (1985) discussed the key




  differences between these various models, and gave the algorithms,




  computational techniques,  capabilities, limitations,  and input/ouput




  parameters of PEM-2.   Pendergrass and Rao (1984) described an evaluation of




  PEM using the St.  Louis Regional  Air Pollution Study  (RAPS)  data.






      This  report  describes  an  evaluation of PEM-2 using the data  from EPA's




  1982 Philadelphia  Aerosol  Field Study  (PAFS).   This evaluation is designed




  to  test the performance of  the model by comparing its  concentration  esti-




 mates to  the measured air quality data,  using  appropriate  statistical




 measures of performance.




     Twenty nine days (from July 16 to August 13,  1982) in  the Philadelphia




 data base are utilized for the PEM-2 evaluation.  The model performance is




 judged  by comparing the calculated average concentrations with the




 corresponding observed values  for  the following pollutant species:






      1.  S02                        2.  Sulfate  particles






      3.  Fine  total  mass             4.  Coarse total mass






The  cut-point  size  between  fine particle (FP)  and coarse  particle (CP)




total mass  fractions is 2.5  microns*  A  first-order chemical  transforma-




raation of SC>2 to  fine sulfate  is considered in  the  calculations in addition




to the direct emission and dry deposition of all  four pollutant species.




For each pollutant,  several plots examining the model performance are




given, and the model evaluation statistics are  tabulated.

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                              SECTION  2









                        PHILADELPHIA DATA BASE









    The 1982 Philadelphia Aerosol Field Study has been sponsored by  the EPA




to obtain detailed data bases on emissions and surface air concentrations




of gases and particles, and concurrent meteorological conditions, with




adequate temporal and spatial resolution to evaluate source and receptor




models, including PEM-2, which are capable of predicting short term




concentrations of particles.  The emissions of primary particulate matter,




and pollutants that undergo chemical transformation in the atmosphere to




form secondary particulates are of special interest.  Therefore, the study




was designed to obtain data on total particulate mass, sulfate, and  SC>2.




Philadelphia was chosen for this study because it has a good mix of




industrial emissions, and it was the site of an earlier program for




evaluation of EPA's Urban Airshed photochemical oxidant model.






      The PAFS experiment was conducted from July 14 to August 14, 1982.




From this data base, detailed emission inventories, and meteorology and




concentration measurements for twenty nine days are supplied by the EPA for




PEM-2 evaluation.  The evaluation days are listed in Table 1.  The PAFS




experiment and data base have been described in detail in other publica-




tions referred to below, and will not be discussed here; only the data used




in the evaluation of PEM-2 and other relevant information will be described




in this section.

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                      TABLE  1
           PEM-2 Evaluation Days of PAFS Data.
Pay                       Date               Julian Day
 1                    July 16, 1982             197
 2                         17                   198
 3                         18                   199
 4                         19                   200
 5                         20                   201
 6                         21                   202
 7                         22                   203
 8                         23                   204
 9                         24                   205
10                         25                   206
11                         26                   207
12                         27                   208
13                         28                   209
14                         29                   210
15                         30                   211
16                         31                   212

17                  August  1, 1982             213
18                          2                   214
19                          3                   215
20                          4                   216
21                          5                   217
22                          6                   218
23                          7                   219
24                          8                   220
25                          9                   221
26                         10                   222
27                         11                   223
28                         12                   224
29                         13                   225

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EMISSIONS






    Hourly emission inventories for point and area sources in the




Metropolitan Philadelphia area during the PAFS monitoring period are deve-




loped by Engineering-Science (ES) of Fairfax, Virginia.  The inventories




are listed for FP total mass (diameter < 2.5 microns), CP total mass (2.5 -




10 microns), primary sulfate particles, and sulfur dioxide.  The primary




sulfate data are found from a variety of industrial processes, and its




emission factors are expressed as multipliers of S02 values on a weight




basis or as percent of flyash.  These data are for total sulfates which




include the sulfuric acid aerosol.  No data are found on sulfate particle




sizes.  Because these are thought to be in the lower end of the IP size




range, ES (1984) assumed that all sulfate particles are less than 2.5




microns in diameter.  Therefore, emission data on coarse primary sulfate




particles are not available, and coarse sulfate emissions are assumed to be




zero in this evaluation.







    The emission inventories are supplied on two magnetic tapes, the first




with 300 major point sources, and the second with 289 area sources; the




latter are given on a square grid with 17 x 17 cells each of which is a




square of side 2.5 km.   This emission grid covers the Philadelphia county




and portions of Bucks,  Chester, Delaware, and Montgomery Counties in




Pennsylvania, and Burlington, Camden, and Gloucester Counties in New




Jersey.  Though this area is smaller than the Air Quality Control Region




(AQCR), the grid encompasses the Philadelphia urban area including all of




Philadelphia County to  the North and East, and extends well beyond the




monitoring site locations to the West and South, thus retaining all the




emission data important for model evaluation.

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    In addition, ES provided emission data for minor point sources and




fugitive particulate matter on a third tape, and for mobile sources on a




fourth tape.  These emission data are given on a square grid with 17 x 17




cells each of which is a square of 2.5 km side.  This grid coincides with




the area source grid, so that these emissions can be easily merged with




area sources in the model calculations.  Highway vehicle emissions data are




generated by the Delaware Valley Regional Planning Commission (DVRPC) under




subcontract to ES.  The latter conducted limited source testing and




collected silt loading samples from selected paved roads to provide




site-specific data in Philadelphia for model evaluation.






    The point source emission data contained the stack identification, its




location in UTM (x,y) coordinates, stack parameters such as height,




diameter, plume-exit velocity and temperature, and emission rates of the




four pollutants (S02, sulfate, fine mass, and coarse mass) in g/s.  The




area source emission data included the county code, grid cell number,




location of southwest corner of the source in UTM (x,y) coordinates, and




emission rates (in g/s) of the four species from each grid cell.






    The major point sources in Philadelphia are electric utilities using




oil and coal-fired boilers , municipal incinerators, oil refineries, metal




and chemical industries, grain elevators, etc.  The stack heights are




generally below 100 m.  Outside a 42.5 km x 42.5 km inventory area, ES




selected only about 50 (out of 300) major point sources with SOX or total




mass emissions above a cutoff value of 500 tons per year.  All other point




sources with relatively lower emissions or farther away from the monitoring




sites are classified as minor point sources.  The area sources consist of




residential, commercial, industrial, and agricultural emissions, and

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releases from transportation, incineration, construction, and other

activities.  ES developed procedures to generate hourly emission rates

using data they collected within the framework of the PAFS study.  For a

discussion of these procedures and additional details of the point and area

source inventories, the emissions report by Engineering-Science (1984)

should be consulted.


    It should be noted that these emission data do not represent real time

conditions.  For example, the precipitation events are not taken into

account in developing the hourly emission estimates.  The use of relatively

large (2.5 km square) grid cells in the study complicates model evaluation

since impacts from paved roads very near the monitors are likely to be the

most significant contributions.  Model results should be interpreted keeping

these limitations in mind.
CONCENTRATIONS


    The ambient air monitoring network in the PAFS study was operated by

PEDCO Environmental, Inc. of Cincinnati, Ohio.  The actual period of data

gathering lasted from 6 a.m. Eastern Daylight Time (EOT), July 14 to 6 a.m.,

August 14, 1982.  The locations and characteristics of the six monitoring

sites shown in Fig. 1 are described below:
    Site 5
           Philadelphia, PA
           Community Health Services Building
           500 South Broad Street
           Center City - Commercial

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_   o

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    Site 7
           Philadelphia, PA
           Fire Boat Station
           Alleghany Ave. & Delaware River
           Suburban - Industrial
    Site 8
           Philadelphia, PA
           Water Treatment Plant
           Ford Road & Belmont Ave.
           Suburban - Residential
    Site 12
           Philadelphia, PA
           Philadelphia Northeast Airport
           Grant and Ashton Road
           Suburban - Rural
    Site 28
           Camden, NJ
           Institute for Medical Research
           Copewood and Davis Streets
           Suburban - Residential
    Site 34
           Clarksboro, NJ
           Shady Lane Home
           Cohawkin Road and County House Road
           Suburban - Rural
    The monitors at Site 5 are located on top of a building (11 m above

street level) and are shielded to the south by a 2.5 m high building

extension.  Therefore, these monitors probably are not collecting

representative samples from either the street-level or the building-top

level.  Site 7 is the most impacted by fugitive dust due to nearby truck

terminals and heavy traffic on an adjacent paved road.  The exact location

of the roadway and construction-related emissions are not input to the

model.  Site 8 is affected by particulate emissions from a county

maintenance yard with unpaved roads and aggregate storage piles.  Site 12,

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located near an area used for plane parking, is affected by heavy traffic




on roads in the vicinity as well as airport operations and nearby small




point sources.  Site 28 is expected to be significantly impacted by paved




road emissions, and Site 34 by a number of large point sources in the




vicinity.






    The measurements at the six sites listed above consist of the




following:




1. Continuous gas monitoring of sulfur dioxide (S02), nitric oxide (NO),




   nitrogen dioxide (N02), non-methane organic carbon (NMOC), ozone (03),




   and carbon monoxide (CO), to obtain 1-hour average concentrations.




2. Particulate mass sampling twice daily at each site to obtain two




   12-hour average concentrations, one for daytime (6 a.m. to 6 p.m.)




   and the other for nighttime (6 p.m. to 6 a.m.).




3. Meteorological data  -  wind speed, wind direction, doppler sodar data




   (at Site 28 until August 5, then relocated at Site 8), and minisondes




   (at Site 28 only).






    These measurements are designed to obtain sufficient data to model FP




and CP total mass, and sulfate concentrations on a 12- and 24-hour basis.




S02 is monitored hourly to determine the chemical transformation




contribution to the sulfate concentration.  The other gases, namely, NO,




N02, NMOC, and 03 are monitored to establish sulfate mass formation via




photochemical mechanisms.  The study is conducted 24 hours a day to obtain




data for modeling diurnal variations in sulfate formation.  Sites 28 and 34




are operated by the State of New Jersey, and the other four sites by the




City of Philadelphia.  PEDCO installed and operated additional monitoring




equipment for PAFS to supplement the instrumentation available at each




site.




                                    10

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    The continuous gas analyzers for SC>2 are either Beckman  953  or  TECO




Series 43; the particulate monitors are EPA's high-volume  or dichotomous




filter samplers.  For the duration of PAFS, PEDCO  operated the various




monitors, recorders, and data acquisition  systems, and  performed the




necessary checks, audits, and calibrations called  for in the Quality




Assurance (QA) Project Plan for the field  study.   For details on these




procedures and instrumentation used in PAFS, the reader is referred to the




report by PEDCO (1983).






     For PEM-2 evaluation, the measured concentrations  of  SC>2, fine and




coarse sulfate particles, and FP and CP total mass from the  six  monitoring




sites of PAFS are provided by EPA on a magnetic tape.   All concentrations,




except S02, are 12-hour averages; S02 data are 1-hour averages.











METEOROLOGY






    Each of the monitoring stations is equipped with continuous  wind speed




and direction instruments.  Data from each instrument are  collected on




strip chart recorders and data acquisition system.  Aerovironment,  Inc.




(AV) performed thrice daily (4 a.m., 10 a.m., 4 p.m.) soundings  of  pressure




(height),  temperature, and wet-bulb depression (relative humidity)  at




Site 28 using an airsonde system developed by the Atmospheric




Instrumentation Research (A.I.R.).   Upper air wind data are  obtained by




using a theodolite to track the balloon that lifts the  airsonde.  To




monitor upper air meteorology, a monostatic Doppler acoustic  sounder is




operated by AV to provide 15 minute averages of horizontal wind  speed and




direction at 30 m height increments up to 1 km.
                                    11

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    The wind speed and wind direction data recording systems malfunctioned




during the PAFS experiment; the surface meteorological measurements at the




six sites are either missing or appear to be of dubious quality.  There-




fore, EPA has decided to use the hourly surface winds and temperatures




observed at the Philadelphia International Airport (PHL) National Weather




Service (NWS) Station (see Fig. 1) as input data for PEM-2 evaluation.  A




magnetic tape of these data consisting of hourly values of wind speed and




direction, temperature, stability class, and mixing heights has been




provided by the EPA.  For each hour, the Pasquill-Gifford (PG) stability




class and the two sets of mixing heights are determined by the RAM




preprocessor (RAMMET), following a procedure described by Turner and Novak




(1978).  Morning and afternoon mixing heights required by RAMMET are




derived from the observed airsonde temperature profiles as the base of the




elevated inversion.






    The values of the potential-temperature gradient above the mixing




height are also determined from the temperature profiles for use in the




optional new plume-penetration schemes of PEM-2 (see, Rao, 1985).  The




meteorological data are compiled into data files suitable for input to




PEM-2; for example, stability class 7 (PG class G) in the RAMMET output is




reset as stability class 6 (PG class F) in FEM-2.






    Figure 2 shows the daytime wind distribution from the NWS data at PHL




during the PAFS experiment.  The surface winds during the day are




predominantly from the southwest (WSW to SSW), with speeds ranging mostly




from 2 to 6 m/s.  The nighttime (6 p.m. to 6 a.m.) wind rose presented in




Fig. 3 also shows a dominant southwesterly component.  The major point




sources in the Philadelphia area are distributed along a line oriented
                                     12

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                       TJAY
                                    NNE
                                                 ENE
Figure  2.  Average daytime wind distribution during PAFS.
                         13

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                     "NTURT
                                    NNE
Figure  3.  Average nighttime wind distribution during PAFS.
                          14

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approximately from SW to NE.  Hence, the PAFS station receptors should




receive significant contributions from point sources both day and night.




The nighttime wind rose also shows a strong northerly component; the




nocturnal winds are evenly distributed from WSW to NW.






    The frequencies of the six PG stability classes in the hourly




meteorological data used in model evaluation are shown in Fig. 4.  The




slightly unstable (class C) cases during the day, and moderately stable




(class F) cases during the night, occur frequently.  There are roughly




equal number of daytime and nighttime neutral cases.  The frequencies of




class B (moderately unstable) during day and class E (slightly stable)




during night are also about equal.
                                 15

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                             SECTION  3



                          MODEL EVALUATION



    The details of the PEM-2 computer runs, input parameters, and

statistical procedures of the model evaluation are discussed in this

section.
PEM-2 RUNS


    The PEM-2 concentration predictions are evaluated against the measured

concentrations of four pollutant species:

               1) S02

               2) Fine sulfate particles

               3) FP total mass

               4) CP total mass

The coarse sulfate concentrations could not be evaluated separately since

coarse sulfate emissions are assumed to be zero in the PAFS inventory (see

Section 2).  The four species are calculated in two model runs as follows:


Run       Pollutant-1        Pollutant-2                Note
  I       S02                Fine sulfate       Chemical transformation
                                                of S02 to fine sulfate
                                                is considered.

 II       Fine mass          Coarse mass        No chemical coupling
                                                between the species.
The fine total mass emissions in Run II also include the primary sulfate
                                    17

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particles.  Though the emissions of the latter are assumed to consist only




of fine particles, they obviously include some coarse (2.5 - 10 microns)




sulfate particles as well since, for some point sources in the PAFS




inventory, the primary sulfate emission rates exceed the corresponding fine




total mass emission rates.  Furthermore, the chemical transformation (S02




to fine sulfate) contribution to the calculated fine total mass




concentration is ignored in Run II.  These errors, however, are not




expected to be serious for obtaining the urban-scale 12-hour average




concentration estimates based on the entire inventory in this evaluation.











Calculation Grid






    The calculation grid consists of 32 x 32 cells, each a square of 2.5 km




side.  The southwest corner of the grid is set at XUTM « 444.5 km and YUTM




= 4380 km, and the modeling domain covers 80 km x 80 km to incorporate the




entire PAFS emission data.  The calculation grid cell size is chosen to




agree with the area source grid cell size of 2.5 km, so that emissions can




be directly input to the model from the inventory data files.  Figure 5




shows the calculation grid used for PEM-2 evaluation and the locations of




the six PAFS stations.






    For this evaluation, the maximum capacity of 50 area sources in PEM-2




is increased to accomodate all 289 area sources in the emission Inventory.




The PEM-2 program is also modified such that concentrations from point




sources are calculated only at the four receptors (grid points) surrounding




each PAFS station, and not at the rest of the receptors.  This required




calculation at only 24 out of a total of 1024 receptors, which resulted  in




a significant reduction in the computer run costs.  The area source
                                     18

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           Calculation  grid used for PEM-2 evaluation showing
           the locations  of PAFS stations.
                          19

-------
calculations did not include this modification to the program.  For each of




the area sources, the contributions to the concentrations at the nine




affected receptors located within and immediately downwind of the source




are calculated, as discussed by Rao (1985).  The total concentration at




each PAFS station is then determined as the weighted average of the




corresponding values calculated at the four surrounding receptors.






    A. calculation grid cell size of 5 km side square is also tested in the




evaluation.  The results showed that, for the PAFS emissions inventory, the




calculations are not very sensitive to this change in the grid cell size.
Emission Data






    The hourly emission data are scanned and point sources with emissions




less than 1 g/s of S02 and 0.1 g/s of 804 are eliminated in order  to  reduce




computer run costs. The emissions are analyzed for day-to-day as well as




diurnal variability.






    Figure 6 shows the variations of daily total (daytime + nighttime) S02




emissions from all of the point and area sources in the PAFS inventory




during the evaluation period.  Figure 7 shows a similar plot for daily




total sulfate emissions.  It can be seen that the point-source total




emissions show large day-to-day variability; for example, S(>2 and  sulfate




emissions increase by roughly 50 percent from Day 17 to Day 18, and




decrease by a similar amount from Day 22 to Day 23.  Days 18 to 22 (August




2-6) are characterized by unusually large point-source emissions,  most




probably due to increased power demand for air-conditioning during the hot




summer days.  In contrast, the area-source total S02 and sulfate emissions
                                    20

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are constant during weekdays, and decrease during weekends to  their minimum




values on Sunday.






    Figures 8 and 9 show variations of daily total  (daytime +  nighttime)




emissions of FP and CP total mass, respectively.  The point-source fine




mass emissions show significant day-to-day variability during  the




evaluation period, while the coarse mass emissions  do not vary much.  The




area source emissions of both fine and coarse mass  show periodic




variations, typically increasing slightly during weekdays to a maximum




value on Friday, and decreasing during weekends to  a minimum on Sunday.




These variations are probably dictated by traffic patterns and fugitive




particulate emissions from unpaved highways, and emissions from industrial




and construction activities.







    The diurnal variations of SC>2 and sulfate emissions from point and area




sources in Philadelphia (averaged over the 29-day evaluation period) are




shown in Figs. 10 and 11, respectively.  The point-source emissions




increase sharply after 7 a.m. to their daytime peak values and then




decrease rapidly after 8 p.m.  The area-source emissions also  behave in a




similar manner, though these values are much smaller than the  point-source




emissions.  However, area sources dominate the daytime emissions of fine




and coarse total mass as shown in Figs. 12 and 13, respectively.  The total




particulate emissions increase sharply from  5 a.m. to a daytime peak at




7 a.m., and decrease rapidly from a secondary peak at 4 p.m.   Thus, these




emissions strongly correlate with rush-hour traffic patterns and daytime




industrial activity.
                                       23

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                                      29

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    The total emission rates of the four pollutant species from point and

area sources, averaged over the evaluation period and stratified by day and

night, are shown in Table 2.  It can be seen that point sources dominate

the SC>2 and sulfate emissions.  The area sources dominate the fine and

coarse mass emissions during the day; however, the contributions of point

and area sources are roughly equal at night.
                                 TABLE  2
   Average Daytime and Nighttime Total Emission Rates (kg/s) from
             Area and Point Sources in PAFS Inventory.
   Pollutant
Area Sources
Point Sources
   S02

   Sulfate

   Fine Mass

   Coarse Mass
Daytime (6




Nighttime




:00 a.m. - 6:00 p.m.)
16.665
0.650
7.897
5.133
(6:00 p.m. - 6:00 a.m.)
14.683
0.555
3.021
1.668

56.425
1.797
4.269
1.737

46.697
1.480
3.724
1.536
   S02

   Sulfate

   Fine Mass

   Coarse Mass


Comparing this with a similar tabulation of total emissions for the RAPS

study from Pendergrass and Rao (1984), we note that unlike in St. Louis,
                                    30

-------
area sources in Philadelphia are significant contributors of SC>2 and




sulfate, and point-source contributions to fine and coarse  total mass are




very important.











Deposition and Sedimentation Rates






    Rao (1983) discussed the specification of deposition and gravitational




settling velocities (V
-------
during day.  The sulfate formation rates are smaller at night due to the




absence of photochemical mechanisms.  A constant transformation rate of 3




percent per hour is used for the nighttime runs in this study.











Model Calculations






    The PEM-2 is run with hourly data of meteorology and emissions to




estimate the hourly concentrations.  The output data are stored on a




magnetic tape, and later summed and averaged to obtain 12-hour average (day




and night) values.  The model evaluation runs are made with the following




technical options (see, Rao, 1985) in effect:






1) Wind-profile exponents option: NWPOPT = 0, standard values are used;




2) Stack-tip downwash option: NSTDWN = 0, downwash algorithm is used;




3) New plume-rise equations option: NPRISE = 1, new equations are used




   to estimate maximum rise of buoyancy-dominated plumes from point




   sources in unstable or neutral atmosphere;




4) New plume-penetration schemes option: NINPEN = 1, new schemes are used




   for estimating penetration of an elevated stable layer (capping




   unstable/neutral atmosphere) by buoyancy-dominated plumes from




   point sources.






    The default values of atmospheric potential temperature gradients for E




and F stability classes (0.02 and 0.035°C/m, respectively) are used in the




plume rise equations under stable conditions.  The area source emissions




are assumed to be located at an effective height HAS = 10 m, which is a




typical building height in urban areas.  This value is kept constant for




all area sources and species both day and night.
                                 32

-------
Background Concentrations






    The calculated 12-hour average sulfate,  fine and  coarse  total  mass  con-




centrations, resulting only from the contributions of point  and area  sour-




ces to the receptors, are added to their respective background




concentrations.  The latter are determined as  the lowest  observed  12-hour




average concentrations at one of the four PAFS stations 8, 12, 28,  and  34




located in a generally upwind direction during the averaging period.




Stations 5 and 7, which are located in the downtown urban area and have




higher observed concentrations compared to the other  stations, are not  used




for this background analysis.  The background  concentrations of S02 are




assumed to be zero.






    The method of determining the background concentrations  as described




above is rather subjective due to the small number of monitoring stations




available.  However, the background particulate concentrations play an




important role in evaluating the model performance by comparing the




calculated concentrations to their observed values.  For  example,  the




calculated fine mass concentrations directly attributable to the emissions




in Philadelphia are in the range of 0 - 20 Ug/in3 with an  average of about




5 Vig/m3, while the background fine mass concentrations average about




25 Ug/m3.  The observed coarse mass concentrations at the stations  are  more




variable than for the fine mass; this suggests that local contributions may




be more important for coarse mass.  The calculated average concentration of




coarse mass resulting from local emissions is below 5 Ug/m3, while  its




background concentration is about 10 Ug/m^.







    The station-to-station variations of the observed sulfate concentra-




tions are small,  with the background values averaging about  7







                                    33

-------
On the other hand, the sulfate concentration calculated from direct




emissions and chemical transformation is below 2 yg/m^.  Therefore, the




background concentrations of particulate species play an important role in




this evaluation.
EVALUATION STATISTICS







    The recommendations of two workshops sponsored by the American




Meteorological Society (AMS) to review the statistical approach to air




quality model evaluation and model uncertainty are summarized by Fox (1981,




1984).  Discussions and applications of these statistical methods can also




be found elsewhere in the literature (see, e.g., Ruff, 1983; Rao et al.,




1985).







    The predicted and the corresponding observed concentrations are treated




as pairs in this evaluation.  Two general measures of performance are used




here: (a) measures of difference which include the bias, variance, gross




variability or root mean squared error, average absolute gross error, mean




fractional error, and index of agreement; (b) measures of correlation




including the correlation coefficient, slope, and intercept; estimates  of




the predicted concentrations from the regression analysis allow determin-




ation of the systematic and unsystematic parts of the mean squared error.




The observed and predicted concentrations are analyzed and plotted with a




standard SAS statistical and data-handling package (Ray, 1982).







    In the discussion that follows, the observed concentrations are denoted




by 0± and the corresponding predicted concentrations (paired in space and




time) are denoted by P±<  A11 sums are caicuiated over i = 1,2,	,N,
                                    34

-------
where N is the number of  observations.  The means,  0 and P,  and  standard




deviations (So and Sp)  are  computed as
where               OJ  -  Q± - 0"         I 0^  = 0                      (3)
and                 P   -  P  - 7   ,     I P   = 0                      (4)
                          ±
The mean and standard  deviation of the ratios, PI/O^ ,  between  the



predicted and its  associated observed value are also computed.








(a) Measures of Difference






    Differences (residuals) are based on the observed and  calculated




concentrations such  that






                           DI - Oi - PI                               (5)






A negative residual  indicates model overprediction and  vice  versa.  The



bias D, which is the first moment of the distribution of differences, is



defined as




                           D-TT-P-IXDI                         (6)






This is a measure  of the overall bias of the model in predicting pollutant




concentrations.
                                   35

-------
    The average absolute gross error is defined as
This measure of the absolute size of the error is less affected by the


removal of outliers in the data than the root mean square error


(RMSE).  The estimated variance, which is the second moment of  the distri-


bution of differences, is calculated from







                                                                        (8)


                          D! =• D. — D  ,      l D! = 0




where S^ is the standard deviation.  The variance is a measure  of noise in


the data.  The RMSE, which is a measure of the actual size of the error


produced by the model, is computed from


                                                       2
BMSE
                                   [(TT)
The mean fractional error (MFE), which determines the model's overall bias


to underpredict or overpredict the concentrations, Is given by
                          MFE  =  I I	i	:rT7T               (10)


                                         °i + Pi)/2
                         ']
    For normally distributed variables, the bias has a normal distribution

                    2
while the variance S,  has a chi-squared distribution.  The mean square


error has a compound distribution.  If the distributions of the predicted


and observed concentrations are the same, then it is reasonable to assume


that the differences are normally distributed with a zero mean and a


constant variance.
                                    36

-------
    The index of agreement is a measure of the degree to which the observed




variable is accurately estimated by the calculated variable.  This is not a




measure of correlation, but rather a measure of the degree to which the




model predictions are error-free.  At the same time, it is a standardized




measure so that cross-comparison of its magnitude for different models, or




a model's performance at different receptor locations or under different




atmospheric conditions, can be made.  The index of agreement, d, is




expressed as
Thus, d specifies the degree to which the observed deviations about 0




correspond, both in magnitude and sign, to the predicted deviations from 0.




It is assumed that the parts of the magnitudes of P± and 0± that are




equivalent to 0 are not in error since 0 is considered to be error-free.




All the potential for error is therefore assumed to be contained in the




deviations of P^ and 0^ from 0.








(b) Measures of Correlation






      For each pollutant, a scattergram of predicted (on the ordinate)




versus observed (on the abscissa) concentrations is plotted, and linear




regression analysis is performed to determine a correlation coefficient




(R), slope (b), and intercept (a), as follows:
                               I (OJ • Pp
                                    37

-------
                             I (0! • P!)
                       b =  	==	—   ,      a = P - b 0           (13)
The estimate of the predicted concentration, P^, is then given by
                             Pi  -  a + b 0±                            (14)
    The unsystematic and systematic parts of the mean squared error (MSB)

are computed as follows:


                         MSE(u) -i  I (P± - Pi)2                       (15)




                         MSE(s) - i  I (P^ - Ot)2                       (16)




These new measures illuminating the sources or types of errors can be

helpful in refining a model.  When the MSB is largely systematic, further

refinement in the model may be necessary in order to minimize the MSB so

that the model can predict at its maximum possible accuracy.  On the other

hand, if MSE is largely unsystematic, the model is probably as good as it

can be, and may not require major modifications.  For each species, the

complementary ratios MSE(u)/MSE and MSE(s)/MSE are computed and expressed

as percentages.
                                    38

-------
                             SECTION  4









                       RESULTS AND DISCUSSION









    The PEM-2 is evaluated using 29 days of data from Philadelphia for four




pollutant species: S02> sulfate, fine and coarse mass.  Only S02 concentra-




tions are measured hourly; the particulate data are 12-hour averages.  The




evaluation results comparing the model's concentration estimates to the




corresponding observed values are presented and discussed in this section.
SULFUR DIOXIDE








    The hourly S02 concentration data provide a demanding test of short




term models such as PEM-2, especially since the background S02 concentra-




tions are assumed to be zero.  Figure 14 shows a comparison of the calcu-




lated and observed diurnal variations of S02 concentrations (averaged over




the evaluation period) at Station 5.  Similar plots for the other moni-




toring stations are shown in Figs. 15 to 19.






    At all stations, the calculated and observed concentrations are closer




during daytime than at night.  The model generally overpredicts the hourly




average concentrations at night.






    A significant overestimation of S02 concentrations by the model at




Stations 5 and 7, and also 28 to a somewhat lesser extent, is evident when




compared with the evaluation results at other stations.  The overpredic-
                                    39

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tions at these stations during nighttime are more severe than  during




daytime. The emission sources in Philadelphia area are located roughly




along an axis from southwest corner to northeast corner of the full




calculation grid.  Stations 5, 7, and 28 are located in the region of major




area source emissions, and surrounded by many point sources.  On the other




hand, Stations 8, 12, and 34 are located away from the region of high area




source emissions and may be impacted mostly by the point sources.  At these




stations, the model underestimates the observed concentrations during day,




and overestimates during night.






    From the above, it is clear that the model overprediction results




mostly due to errors in estimating concentrations from the urban area




sources using the narrow plume hypothesis and other simplifying assumptions




(see, Rao, 1983).  Uncertainties in the area-source emission conditions




such as source height, plume rise, and building wake effects also




contribute to these errors.  In general, the isolated point source emission




inventories are better defined and documented than those of the distributed




urban area sources.  The pattern of urban model estimates being highest




under stable (nighttime) conditions and lower under unstable (daytime)




conditions is attributed by Turner and Irwin (1985) to the errors in




modeling low—level sources.






    The plots show that the observed concentration reaches a maximum about




2 to 3 hours after the morning transition when the stratification changes




from stable to neutral or unstable.  The fumigation process which brings




down the elevated plume from above the surface-based inversion may partly




account for the peaks observed soon after sunrise (Rao et al., 1985).




Though PEM-2 does not treat the fumigation process, the model simulates
                                    46

-------
these peaks quite well; this suggests that  the observed peak  concentrations




may be related to the increases in SC>2 emissions  in  the morning  (shown  in




Fig. 10).






    Figure 20 shows a comparison of the calculated and observed  12-hour




average SC>2 concentrations for the 29 evaluation  days.  This  scatterplot is




a composite of all (both day and night) paired comparisons at  the  six PAFS




stations.  The compared range of concentrations extends from  7.8  Wg/m  ,




which approximates the instrument accuracy,  to a  cutoff value  of  57  Vg/ra^




corresponding to 2.5 times the standard deviation, Sp.  A linear




regression fit, with a slope of 0.33 and an  intercept of 17,  is  also shown




in the figure.







    Table 3 summarizes the model evaluation  statistics for S02 for the




total, day, and night paired data comparisons.  The  mean and  standard




deviation of the ratios P±/0± are 1.51 and  1.66,  respectively.   Of




particular interest is the better performance of  the model during  the day




than at night.  The index of agreement (0.43 for  daytime and  0.21  for




nighttime) suggests that PEM-2 calculations  of S02 concentrations  are more




accurate during the daytime than at night.






     The differences D^ between observed and predicted concentrations




are plotted in Fig.  21 against the observed  concentrations.  There is a




tendency for the model to overpredict observed concentrations  less than




25 Ug/m3.  The bias D of -5.71 Ug/m3 indicates that  PEM-2 overpredicts




S02 concentrations on the average.  This overprediction is mostly  due to




the nighttime cases for which the bias is -12.63  Ug/m^; the daytime S02




concentrations are slightly underpredicted.  Because of the smaller




diffusivities and mixing depths,  the nighttime GLC may result mostly from
                                    47

-------
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  20
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    S02 CONCENTRATION ( )iq/s3 )

LtSEND: A = !  OSS, 8 = 2 3SS, ETC.


                         A
                                                         AA
    A A  A   S   4 Aft    A
               A    A
                   Aft              A
   AA  A  3A   C AA   A   A
       3 AAAA  A  ; 4     A
     3  9 AAAAA AA A A            A
   3A    A   AA A   A         A
   A 3AH38M  A  AS A  AA  A   A      A
   C AA BAASAAA A C    A  AA        A      A
   4A  A  A      A AS
   ASAAA   AAB A A A       A  A
   A  A38  AAAA  A   A  A A    A        A
   ASA A CCAD      A A A   A   A
   D AA A AA A AA 3  A    AA
      A          A   A      A
                              20
                              30

                           OBSERVED
40
    Figure  20.   Comparison -of calculated  and observed 12-hour average
                   SC>2 concentrations for the evaluation period.
                                      48

-------
                  TABLE  3
Summary of PEM-2 Evaluation Statistics for


Observations
Range
Mean
S.D.
R
Slope
Intercept
Mean of (Pi/Oi)
S.D. of (Pi/Oi)
Bias
S.D. of Difference
Average Absolute Gross Error
RMSE
Index of Agreement
Mean Fractional Error
MSE(u)
MSE(s)
MSE(u)/MSE
MSE(s)/MSE
Note: The units of Range, Mean,
Total
Obs. Calc.
289
8-46 0-150
16.77 22.48
7.28 22.96
0.10
0.33
17.00
1.51
1.66
-5.71
23.36
15.42
24.00
0.27
-0.46
519.67
56.48
90%
10%
S.D. , Interci
Day
Obs. Calc.
147
8-46 0-91
17.02 16.03
7.85 15.71
0.18
0.35
10.02
1.07
1.46
0.99
16.28
11.45
16.25
0.43
0.75
237.55
26.53
81%
19%
apt, Bias, S.D
Night
Obs. Calc.
142
8-39 0-150
16.52 29.15
6.65 27.07
0.19
0.37
23.12
1.96
1.98
-12.63
27.29
19.53
29.99
0.21
-1.71
721.90
177.31
80%
20%
. of
                       49

-------
                  302 CONCENTRATION i |is/s3 i

             LESEND:  4 = 1  3BS,  3 = 2 G2S. £TC.

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                                      OBSERVED CCNCEHTRATIOS
     Figure  21.    S(>2  residuals  (D^  » 0^_  - P^) versus observed  12-hour
                      average  302 concentrations  for the evaluation period.
                                      50

-------
the surface area source emissions; on  the other hand,  point  sources




contribute significantly during  the daytime.   If more  of  the emissions  were




treated as point sources,  the  result would  be  to increase the daytime




concentrations, and decrease the  concentrations at night.  Thus,  the model




results are sensitive to the characterization  of emissions.   Ruff  (1983),




and Turner and Irwin (1985), identified  the inclusion  of  point sources  in




the RAPS emissions inventory as  area sources as a possible cause  of the




stability bias in the urban model  (RAM)  performance, whereby the  largest




concentrations are often predicted to  occur with stable conditions and  low




wind speeds, in contrast to the  observations.






    Figure 22 shows a comparison  of the  calculated and observed daily




(24 hour average) concentrations  of S02  (averaged over all six stations




for each of the 29 evaluation  days).   In general, the  calculated  daily




concentrations are within  a factor of  two of the corresponding observed




values, except for days 2, 18, and 23.   If  we  plot the daytime and night-




time 12-hour average data  separately (Figs.  23 and 24), we find that the




large differences between  the  calculated and observed  concentrations




occured mostly during the  night.  These  results confirm that  the model




performs much better during the day than at  night, as  noted  above.  Even at




night, however, the major  part of the  error  (about 80  percent)  for SC>2  is




unsystematic.   This means  that, for the  given  data set, PEM-2  is predicting




with a high degree of accuracy, and we cannot  readily  identify  where




further improvements can be made to the  model.






    In order to test whether the optional new plume rise  equations and




plume penetration schemes  of PEM-2 used  in  this evaluation made any




difference,  the model is rerun with the  standard plume rise equations and




the standard "all or none" penetration criterion to calculate  the  hourly
                                    51

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SC>2 GLC for  two days.  Except  for  transition  periods  with  sharp  changes  in




stability and mixing height, no significant differences  are  noticeable in




the calculated values.  This is probably  due  to  the fact that  area sources




are significant contributors to the  SC>2 GLC in Philadelphia.   Furthermore,




the stack heights of point sources in  the inventory are  fairly low (under




100 m) and the plumes are not  very buoyant.   These plume conditions




together with the high mixing  depths input to the model  did  not  give




complete penetration.  This limited  testing of the the new plume rise  and




penetration  schemes in this evaluation, therefore, did not permit a




conclusive assessment of these methods.   We would need a more  suitable and




better-defined data set for this purpose.
SULFATE









    The scatterplot of calculated versus observed  12-hour average  fine




sulfate concentrations is shown in Fig. 25.  The linear  regression fit  is




also shown in the figure.  The statistics for this evaluation are  given in




Table 4.






    The mean of ratios of calculated and observed values, V±/0±, is  1.45;




the correlation coefficient is 0.77 and the slope is 0.84 both day and




night.  Since the background is estimated to be a large  (25% or more) part




the observed GLC, this high correlation suggests that the background




concentrations, arising from long-range transport and regional inflow of




the species across model boundaries, may be decisive in  determining  the




particulate sulfate levels in urban areas.  The high value of 0.87  for  the




index of agreement both day and night suggests that the  background
                                    55

-------
                      S04 CCNCEUfiiATIGH i /iO/a3 i

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40
Figure   25.  Comparison  of calculated and observed  12-hour average
               sulfate concentrations  for  the evaluation  period.
                                  56

-------
                              TABLE  4
         Summary of PEM-2 Evaluation Statistics for Sulfate.


Observations
Range
Mean
S.D.
R
Slope
Intercept
Mean of (PI/OI)
S.D. of (Pi/Oi)
Bias
S.D. of Difference
Average Absolute Gross Error
RMSE
Index of Agreement
Mean Fractional Error
MSE(u)
MSE(s)
MSE(u)/MSE
MSE(s)/MSE
Total
Obs. Calc.
307
0-33 0-36
9.85 11.17
6.91 7.54
0.77
0.84
2.87
1.45
1.89
-1.31
4.91
3.42
5.08
0.87
-0.42
22.87
2.91
89%
11%
Day
Obs. Calc.
152
0-29 1-32
9.19 10.18
6.04 6.58
0.77
0.84
2.48
1.46
2.37
-1.00
4.32
2.86
4.42
0.87
-0.31
17.61
1.94
90%
10%
Night
Obs. Calc.
155
0-33 0-36
10.51 12.13
7.63 8.24
0.77
0.84
3.36
1.44
1.25
-1.62
5.43
3.97
5.65
0.87
-0.52
27.67
4.21
87%
13%
Note; The units of Range, Mean, S.D. ,  Intercept, Bias, S.D. of
      Difference, Average Absolute Gross Error, and RMSE are
                                 57

-------
concentrations determined as described earlier may be appropriate.






    The sulfate residuals are plotted against the observed concentrations




in Fig. 26.  No clear bias in predictions is evident in the results.  The




mean difference over the entire range of concentrations is -1.31  Mg/m^,




i.e., the model slightly overpredicts the sulfate GLC.  The RMSE  is  5.08




Vg/rar, and about 89 percent of the MSE is unsystematic.  This suggests




that PEM-2 performs well in simulating the PAFS sulfate concentrations




resulting from the background contributions and primary emissions of  the




species, and chemical transformation of SC>2.






    In order to investigate the role of background concentrations in  the




correlation between the observed and calculated GLC, a stepwise regression




analysis has been performed.  This consists of fitting regression relations




between the observed GLC values as dependent variables, and the background




and model-calculated concentrations as independent variables in a stepwise




procedure, as follows:






Step  0 :   Y = aL + eL




Step  1 :   Y = a2 + b2 X + e2




Step  2 :   Y = a3 + b_ X + c_ Z + e_






where   Y   = 0^ , the observed ground-level concentrations,




        X   = B£ , the estimated background concentrations,




        Z   = PI - E± , the model-calculated concentrations,




        e.   = the residual errors, (k = 1, 2, 3),






and a^ , b, , and c,  are the regression coefficients.  At each step,  the




residual error, e, and correlation coefficient, R, are calculated to see




if a reduction in the sum of squared errors (SSE) and an  increase in the






                                    58

-------
                  3Qi CONCEHTRATIGK

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                                     OBSERVES C2HCENTRATIOM
   Figure   26.   Sulfate residuals  (Di  = 0^ -  P^)  versus  observed sulfate
                   concentrations for the evaluation period.
                                     59

-------
square of correlation coefficient (RSQ) occurs with the increase in the




number of independent variables in the regression.






    The stepwise regression equations, and the corresponding values of RSQ




and SSE, are determined separately for the total, daytime, and nighttime




observed sulfate GLC data, as shown in Table 5.  The coefficients for the




model-calculated concentrations in the regression equations are smaller




than those for the background concentrations.  This indicates that the




latter account for a larger fraction of the correlation between the




observed and predicted GLC than the local source contributions calculated




by the model.  This is particularly noticeable at nighttime, thus




suggesting that either a major portion of the observed concentrations is




due to the background, or that the model is not geared towards estimating




the GLC at night.  The decrease in SSE from step 0 to step 1 is much larger




than that from step 1 to step 2 in all cases, especially at night.  This




confirms that background concentrations play a more important role at night




for sulfate.






    Figure 27 shows a comparison of the calculated and observed daily mean




concentrations of sulfate (averaged over all six PAFS stations) for each of




the 29 evaluation days.  There is excellent agreement between the calcu-




lated and observed concentrations.  If the results are plotted separately




for 12-hour averages, the differences in model performance between daytime




and nighttime (Figs. 28 and 29) are seen to be small.
                                 60

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                          TABLE  6









   Results of Stepwise Regression Analysis for Sulfate.









                                           RSQ         SSE




Total Data (sample size = 307)







  Step 0 :  Y = 9.85 ,                      -         14608




  Step 1 :  Y = 2.98 + 0.83 X ,            0.59        6056




  Step 2 :  Y = 2.08 + 0.80 X + 0.40 Z ,   0.62        5585







Daytime Data (sample size = 152)






  Step 0 :  Y = 9.19 ,                      -          5506




  Step 1 :  Y = 3.15 + 0.75 X ,            0.51        2703




  Step 2 :  Y = 2.00 + 0.73 X + 0.60 Z ,   0.59        2236






Nighttime Data (sample size = 155)






  Step 0 : Y =* 10.51 ,                      -          8968




  Step 1 : Y = 3.02 + 0.88 X ,             0.64        3249




  Step 2 : Y = 2.52 + 0.86 X + 0.19 Z ,     0.64        3199
                               61

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 FINE TOTAL MASS






    Figure 30 shows a comparison of all of  the calculated and observed




12-hour average fine total mass concentrations for  the model evaluation




days.  The solid line shows the linear regression fit with a slope  of 0.79




and intercept of 10.91 Ug/ra .






    The evaluation statistics of paired comparisons for fine total  mass are




summarized in Table 6.  The high values of  the correlation coefficient




(0.75) and the index of agreement (0.84) indicate that the model performs




well in predicting observed concentrations.  However, the invariance of




these values both day and night suggest that the background concentrations




may be more important than local source contributions in estimating the FP




concentrations in Philadelphia.






    The fine total mass residuals are plotted against the observed  con-




centrations in Fig. 31.  A tendency towards overprediction is evident in




the plot.  The bias over the entire range of comparison is -4.7 yg/m3.  The




nighttime bias (-5.39 Pg/m3) is higher than that during the daytime (-4.01




Mg/m3).  The RMSE is 9.98 ug/m3, and the major part (71 percent) of the MSE




is unsystematic error.  This suggests that PEM-2 performed satisfactorily




in simulating the 12-hour average GLC of FP total mass in the PAFS  data.




In order to investigate the importance of FP background concentrations in




Philadelphia, a stepwise regression analysis (similar to that described for




sulfate) has been performed.  The regression equations, RSQ, and SSE for




each step are shown in Table 7.  These results show that the FP background




concentrations play a major role in correlating to the observed GLC, and




the model-calculated concentrations are only of secondary importance.
                                    65

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                                      OBSERVED
                  Comparison  of  calculated  and  observed  12-hour average
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-------
                       TABLE  6






Summary of PEM-2 Evaluation Statistics for Fine Total Mass.


Observations
Range
Mean
S.D.
R
Slope
Intercept
Mean of (PI/OI)
S.D. of (Pi/Oi)
Bias
S.D. of Difference
Average Absolute Gross Error
RMSE
Index of Agreement
Mean Fractional Error
MSE(u)
MSE(s)
MSE(u)/MSE
MSE(s)/MSE
Note: The unit of Range, Mean,
Total
Obs. Gale.
301
7-65 11-76
29.84 34.54 2
12.15 12.81 1
0.75
0.79
10.91
1.24
0.41
-4.70
8.82
7.43
9.98
0,84
-0.85
71.14
28.49
71%
29%
S.D. , Intercept
Day
Obs. Gale.
150
9-59 11-66
9.34 33.35
1.34 11.83
0.75
0.78
10.46
1.20
0.37
-4.01
8.24
6.49
9.14
0.84
-0.74
61.28
22.27
73%
27%
, Bias, S.D.
Night
Obs. Gale.
151
7-65 11-76
30.33 35.72
12.93 13.65
0.75
0.80
11.56
1.27
0.45
-5.39
9.33
8.37
10.75
0.83
-0.97
79.67
35.93
69%
31%
of
Difference, Average Absolute Gross Error and RMSE are
                           67

-------
            FINE TOTAL 1ASS CGHC3TRATIQSS i  pc/s3 )

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                                     OBSERVED CGNCEHTRATIOH
      Figure  31.   FP  total  mass residuals  (D^  = 0^ -  P^)  versus  observed
                       12-hour average  FP  concentrations for  the  evaluation
                       period.
                                    68

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                            TABLE  7
   Results of Stepwise Regression Analysis for Fine Total Mass,
                                               RSQ
              SSE
Total Data (sample size = 301)







   Step 0 :  Y = 29.84 ,




   Step 1 :  Y = 8.55 + 0.77 X ,




   Step 2 :  Y = 6.03 + 0.78 X + 0.36 Z ,






Daytime Data (sample size = 150)






   Step 0 :  Y = 29.34 ,




   Step 1 :  Y - 9.00 + 0.73 X ,




   Step 2 :  Y = 6.85 + 0.73 X + 0.39 Z ,







Nighttime Data (sample size = 151)






   Step 0 :  Y = 30.33 ,




   Step 1 :  Y = 8.30 + 0.81 X ,




   Step 2 :  Y = 5.69 + 0.81 X + 0.31 Z ,
0.60




0.62
0.66




0.67
44316




17634




16895
—
0.54
0.55
19158
8771
8539
25084




 8602




 8250
                                69

-------
    Figure 32 shows that the model tracks the observed daily mean




concentrations (averaged over the six stations) fairly well for the




evaluation period.  Similar comparisons for the daytime and nighttime




12-hour average concentrations (Figs. 33 and 34, respectively) show no




significant differences in performance.









COARSE TOTAL MASS






     Figure 35 shows a comparison of the calculated and observed 12-hour




average coarse total mass concentrations for the 29 evaluation days.  The




solid line shows the linear regression fit.  The slope is 0.14 and the




intercept is 13.45 Ug/m3.






    The model evaluation statistics for coarse total mass are summarized in




Table 8.  The mean of ratios, Pi/Oi, is 1.29 and the corresponding standard




deviation is 0.81.  The correlation coefficient of 0.25 indicates a large




degree of randomness in the paired comparison of coarse mass concentra-




tions.  The relatively low index of agreement (0.47) suggests that the




predictions of CP contain more error than the results for FP and sulfate.






    The coarse mass residuals are plotted against the observed concentra-




tions in Fig. 36.  The model shows a clear bias to overpredict the observed




concentrations below 20 yg/m3, and underpredict 0^ above this value.  The




mean of differences over the entire range of concentrations is -0.83 pg/m3,




i.e., the model is slightly conservative.  The average absolute gross error




of 5.74 Pg/m3 is much less than the mean of observed concentrations.  The




RMSE is 8.28 Ug/m3, but 73 percent of the MSE is systematic.  This differs




from the results for sulfate and FP for which a major part of the MSE is




unsystematic.  This seems to suggest that there is room for improvement in
                                    70

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    Figure   35.   Comparison of calculated and observed 12-hour average
                    CP  total mass concentrations for the evaluation period.
                                     74

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                           TABLE  8
Summary of PEM-2 Evaluation Statistics for Coarse Total Mass.


Observations
Range
Mean
S.D.
R
Slope
Intercept
Mean of (PI/OI)
S.D. of (Pi/Oj.)
Bias
S.D. of Difference
Average Absolute Gross Error
RMSE
Index of Agreement
Mean Fractional Error
MSE(u)
MSE(s)
MSE(u)/MSE
MSE(s)/MSE
Note: The unit of Range, Mean,
Total
Obs. Calc.
298
1-54 5-31
14.62 15.44 1
8.15 4.46
0.25
0.14
13.45
1.29
0.81
-0.83
8.25
5.74
8.28
0.47
-0.36
18.57
49.99
27%
73%
S.D., Intercept
Day
Obs. Calc.
148
1-47 7-26
3.39 14.89
6.58 3.63
0.25
0.14
13.05
1.35
0.98
-1.50
6.68
4.90
6.82
0.47
-0.52
12.27
34.26
26%
74%
, Bias, S.D.
Night
Obs. Calc.
150
3-54 5-31
15.84 16.00
9.31 5.10
0.23
0.13
14.01
1.22
0.59
-0.16
9.53
6.56
9.50
0.45
-0.20
24.48
65.82
27%
74%
of
  Difference,  Average Absolute Gross Error,  and RMSE are Pg/m3,
                             75

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modeling the CP concentrations, for example, by using a different  set of




values for the deposition and gravitational settling velocities for




particles of size 2.5 to 10 microns.






    In order to investigate the role of background concentrations  in the




comparison between the observed and calculated GLC, a stepwise regression




analysis has been performed for the total, daytime, and nighttime  CP data




separately.  The regression equations, RSQ, and SSE for each step  are shown




in Table 9.  The results show that the correlation coefficients for both




background and model-calculated concentrations are of the same order,




indicating that each accounts for about the same fraction of the




correlation between the observed and predicted GLC.  The decrease  in SSE is




more significant from step 0 to step 1 than from step 1 to step 2.




However, this decrease is not so significant as that for the sulfate or FP




species.






    Figures 37, 38, and 39 show the model performance in predicting daily




mean, daytime and nighttime (12-hour average) coarse total mass concentra-




tions, respectively.  All concentrations are averaged over the six PAFS




stations.  The overall agreement between the calculated and observed




variations is good with no discernable difference between the daytime and




nighttime performance.  Though the local source contributions may  be




relatively more important for the coarse mass than for sulfate and fine




mass, the background plays an important role in determining the overall CP




concentration levels in Philadelphia.
                                    77

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                             TABLE  9
   Results of Stepwise Regression Analysis for Coarse Total Mass.
                                               RSQ
SSE
Total Data (sample size = 298)






   Step  0 :   Y = 14.62 ,




   Step  1 :   Y = 6.38 + 0.70 X,               0.12




   Step  2 :   Y = 3.84 + 0.72 X + 0.67 Z,      0.16






Daytime Data (sample size = 148)






   Step 0 :    Y = 13.39,




   Step 1 :    Y = 6.25 + 0.61 X,               0.11




   Step 2 :    Y - 2.98 + 0.70x + 0.71 Z,       0.15






Nighttime Data (sample size = 150)






   Step 0 :    Y = 15.84,




   Step 1 :    Y = 6.99 + 0.75 X,               0.13




   Step 2 :    Y = 5.23 + 0.73 X + 0.50 Z,      0.15
19723




17264




16595
 6364




 5659




 5383
12908




11166




10950
                                78

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                              SECTION  5









                             CONCLUSIONS









    This report described an evaluation of the Pollution Episodic Model




Version 2 using 29 days of the Philadelphia Aerosol Field Study data.  This




evaluation is designed to test the model performance by comparing its




concentration estimates for four pollutant species (S02, sulfate, fine and




coarse total mass) to the measured air quality data, using appropriate




statistical measures of performance.







    The emphasis in this evaluation is on primary fine and coarse inhalable




urban particulate matter, as well as pollutants that undergo chemical




transformation in the atmosphere to form fine secondary particulates (e.g.,




S02 to sulfate aerosol).  For the evaluation period, PEM-2 predicted




12-hour average concentrations of S02, sulfate, fine and coarse total mass




to within a factor of two, which is the best that may be expected




considering the natural variability in model input data (Hanna, 1981).






    The hourly S02 concentration data are considered to provide a demanding




test of the performance of PEM-2, especially since the background S02




concentrations are assumed to be zero.  The model performance for S02 is




better during daytime than at nighttime, and generally better at the




suburban stations, which are affected mostly by point sources, than at




downtown stations.  The latter are impacted heavily by the urban area




sources, which are thought to be major contributors to the errors in the
                                    82

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concentration estimates.  These errors result from  the difficulty  in




characterizing area source emissions, lack of information on source




conditions such as release height, plume rise, and  building-wake effects,




as well as the narrow plume concept and other simplifying assumptions used




in the concentration algorithms for area sources.






    The calculated and observed SO  concentrations  are closer at all PAFS




stations during daytime than at night.  The model generally overestimates




the hourly concentrations at night, and underpredicts during the day at




rural locations which are not significantly impacted by area sources.  This




stability bias of the model is attributed to the the problems associated




with modeling low-level urban sources, and the model sensitivity to the




characterization and partition of emissions between point and area sources.






    The model performance for the particulate species is good; both the




12-hour and daily mean concentrations (averaged over the six PAFS  stations)




over the evaluation period are predicted well.  For sulfate and fine total




mass, the values of the correlation coefficient and index of agreement are




high, and a large part of the estimated MSE is unsystematic.  For  coarse




total mass, the evaluation statistics are not as good by comparison, and




the large systematic error suggests there is room for model improvement.




On the average, the model estimates of concentrations for the particulate




species are slightly conservative (overpredictions).






    The overall good performance of the model for particulate species




should be interpreted with caution since the background concentrations,




resulting from long-range transport and regional inflow of species across




model boundaries, far exceed the urban source contributions to the surface
                                    83

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concentrations in Philadelphia.  When the wind direction changes




significantly, no particular source contributes longer than one hour to




receptor concentrations in PEM-2 (with the possible exception of receptors




located within area sources).  On the other hand, the determination of




background concentrations from PAFS data is somewhat subjective due to the




small number of monitoring stations available.  Ideally, the background




monitors should be located on the calculation grid boundaries, away from




the influence of sources being modeled.  Nevertheless, judging from the




model performance in this evaluation, the values of background particulate




concentrations estimated from observed GLC at suburban monitors and wind




direction analysis for each 12-hour averaging period seem appropriate.






    It appears that the background particulate concentrations are important




not only in Philadelphia, but in other urban areas as well.  Wolff et al.




(1985) studied the influence of local and regional sources on the




concentrations of inhalable particulate matter at four (urban,




industrialized, suburban, and rural) sites in southeastern Michigan, and




found that FP was dominated by regional influences rather than local




influences at all four sites, while CP was dominated by local sources.  The




regional influences were most pronounced on the sulfate levels which




accounted for the largest fraction (40 - 50%) of the FP in their study.






    It may be possible to establish the relative importance of the local




and regional contributions to the urban FP and CP concentrations from an




analysis of the National Inhalable Particulate Network data.  In a




preliminary interpretation of these data, Pace and Rodes (1981) concluded




that CP and FP concentration levels are substantially different among urban




areas and, on an urban scale, FP averages are generally more homogeneous
                                    84

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indicating a regional pattern; the lower degree of uniformity in CP




(compared to FP) concentrations in urban areas may be due to a larger




contribution of CP from local sources.  The results of the present study




seem to support this conclusion.






    The characteristics of emissions in Philadelphia appear to be




substantially different from those in St. Louis.  This is demonstrated in




Table 10 which compares the daily average emission rates of the species




from point and area sources during the PAFS and the RAPS experiments.




Unlike in St. Louis, the area sources in Philadelphia are significant




contributors of S02 and sulfate, and point source contributions to fine and




coarse total mass are very important.  Because of the differences in




emission characteristics between different urban areas, it is desirable to




evaluate PEM-2 with as many detailed data sets as possible.  In an




evaluation of PEM using St.Louis/RAPS data, Pendergrass and Rao (1984)




attributed the large overpredictions of FP and CP by the model to




overestimation of emission rates of area sources in the inventory and their




incorrect location, among other factors.







    The meteorological data used in this evaluation are surface observa-




tions from NWS station at the Philadelphia Airport (PHL).  These data are




only approximations to real conditions in the Philadelphia urban area.




Errors in wind direction may cause the model to impact particular receptors




which may be completely ignored in reality.  Errors in wind speed and




stability classification may significantly affect the diffusion, plume rise




and penetration calculations.  It is well known that the frequency and




intensity of nocturnal inversions over cities are decreased due to enhanced




thermal and mechanical mixing resulting from urban heat island and
                                    85

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                             TABLE  10
   Comparison of Dally Average Emission Rates (kg/s) from Area and
             Point Sources in Philadelphia and St.  Louis.
Pollutant
  Area Sources
Point Sources
S02

Sulfate

Fine Total Mass

Coarse Total Mass
Philadelphia/PAFS


     15.674

      0.603

      5.459

      3.400
     51.561

      1.639

      3.997

      1.637
S02

Sulfate

Fine Total Mass

Coarse Total Mass
  St. Louis/RAPS


      0.434

      0.008

      2.518

      6.631
     36.018

      0.266

      0.211

      0.921
                                86

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increased roughness effects.  Hence, the diffusion conditions  in  the  lower




atmosphere over cities tend to be of near-neutral type, without the strong




diurnal variations (see Fig. 4) found at airport locations.  The  plume




dispersion parameters used in PEM-2 account for the enhanced turbulence and




mixing over urban areas by using greater sigraa values  (than in the open




country) for given stability class.  However, due to lack or unreliability




of on-site meteorological data, it cannot be ascertained if the actual




dispersion conditions over Philadelphia are adequately simulated  in this




study.






    The effective height of area-source emissions, taken as 10 m  (typical




of building-top releases) in this evaluation, is an approximate value used




to mitigate the large GLC calculated at receptors located within  the area




sources.  Better characterization of area and point source emissions would




be helpful.  The influence of the new plume rise equations and new




plume-penetration schemes used in this evaluation (for buoyancy-dominated




point-source plumes in unstable/neutral atmosphere) could not  be  assessed




since no significant differences are noticeable in the hourly  S02 GLC




calculated for two days from the new schemes and the standard  schemes,




except for transition periods with sharp changes in stability  and mixing




height.  However,  these results are not conclusive, and more tests with




suitable data are necessary to bring out the differences in performance




between the various schemes.






    The primary objective of this study is to evaluate the performance of




PEM-2 with emphasis on estimating concentrations of urban particulate




matter.  Based on the results, we conclude that PEM-2 is able  to  simulate




the observed concentrations of S02, sulfate, FP and CP total mass in PAFS
                                    87

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data fairly well.  The results of stepwlse regression analysis in this




study suggest that the observed GLC of the urban particulate species are




highly correlated to their estimated background concentrations.  The latter




are significantly larger than the local source contributions (as calculated




by the model) in Philadelphia and, therefore, play an important role in




predicting the GLC of particulate matter.  With the PAFS data, we could not




readily identify where further improvements can be made to the model; this




would require a more extensive and better-defined evaluation data set.






    The background concentrations of particulate matter in an urban area




are determined by the primary emissions, chemical transformation, and




transport on scales much larger than the city size.  The background




concentrations in Philadelphia are large because of its proximity to other




densely-populated urban and industrial centers in the eastern U.S.  The




relatively smaller contributions from the local sources of particulate




matter are determined essentially by the given emissions and meteorology.




Therefore, additional effort should be directed towards an examination of




the emissions characterization, input meteorology, and variability of




background concentrations.  An objective methodology to determine the




background particulate concentrations should be evolved and the monitoring




stations in the field programs in future should be located accordingly.
                                 88

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                              REFERENCES
Engineering—Science,  1984: Development  of  an  emission  inventory  for
    urban particle model validation  in  the Philadelphia AQCR.  Contract
    No. 68-02-3509, U.S. Environmental  Protection Agency, Research Triangle
    Park, NC, 613 pp.

Fox, D. G., 1981: Judging air quality model performance.  Bull,  of Amer.
    Meteor. Soc. 62,  599-609.

Fox, D. G., 1984: Accuracy in air quality  modeling.  Bull,  of  Amer. Meteor.
    Soc. j>5_, 27-36.

Hanna, S. R. , 1981: Natural variability of observed hourly  SC>2 and CO
    concentrations in St. Louis.  Atmos. Environ. 16,  1425-1440.

Pace, T. G., and C. E. Rodes, 1981:  Preliminary  interpretation of
    Inhalable Particulate Network data.  Paper No. 81-5.2,  Vol.  I,
    Proc. of 74th Annual Meeting of  APCA,  Philadelphia.

PEDCO Environmental,  Inc., 1983: The 1982  Philadelphia Aerosol Field
    Study.  Data Collection Report.  Contract No. 68-02-3509,  U.S.
    Environmental Protection Agency, Research Triangle Park, NC.

Pendergrass, W. R., and K. S. Rao, 1984: Evaluation of Pollution
    Episodic Model using RAPS data.  EPA-600/3-84-087, U.S.
    Environmental Protection Agency, Research Triangle Park, NC;
    NOAA Tech. Memo. ERL ARL-128. 47 pp.   [NTIS  PB84-232537],

Ray, A. A., 1982: SAS User's Guide:  Statistics,  1982 Ed.
    SAS Institute, Inc., Gary, NC, 584  pp.

Rao, K. S., 1983: Plume concentration algorithms with  deposition,
    sedimentation, and chemical transformation.  EPA-600/3-84-042, U.S.
    Environmental Protection Agency, Research Triangle Park, NC; NOAA
    Tech. Memo. ERL ARL-124, 87 pp.  [NTIS PB84-138742].

Rao, K. S.,  and M. M. Stevens, 1983: Pollution Episodic Model  User's
    Guide.  EPA-600/8-84-008, U.S. Environmental Protection Agency,
    Research Triangle Park, NC;  NOAA. Tech. Memo. ERL  ARL-125, 186 pp.
    [NTIS PB84-164128].

Rao, K. S.,  1985: User's Guide for PEM-2:  Pollution Episodic Model
    (Version 2).  EPA-600/8-85-   , U.S. Environmental Protection Agency,
    Research Triangle Park, NC;  NOAA Tech. Memo.  ERL ARL-137,  128 pp.
    Available from NTIS.

Rao, S. T.,  G. Sistala, V. Pagnotti, W.  B. Petersen, J. S. Irwin, and
    D.  B.  Turner, 1985: Evaluation of the performance  of RAM with  the
    Regional Air Pollution Study data base.  Atmos.  Environ. 19,
    229-245.
                                  89

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Ruff, R. E., 1983: Application of Statistical methods to diagnose
    causes of poor air quality model performance.  Atmos. Environ. 17,
    291-297.

Texas Air Control Board, 1979: User's Guide: Texas Episodic Model.
    Permits Section, Austin, Tx, 215 pp.

Turner, D. B., and J. H. Novak, 1978: User's Guide for RAM.
    EPA-600/8-78-016a, U.S. Environmental Protection Agency, Research
    Triangle Park, NC, Vol. 1, 60 pp.

Turner, D. B., and J. S. Irwin, 1985: The relation of urban model
    performance to stability.  Air Pollution Modeling and Its
    Application IV, C. De Wispelaere, Ed., Plenum Press, New York,
    721-732.

Wolff, G. T., P. E. Korsog, D. P. Stroup, M. S. Ruthkosky, and M. L.
    Morissey, 1985:  The influence of local and regional sources on
    the concentration of inhalable particulate matter in southeastern
    Michigan.  Atmos. Environ. 19, 305-313
                                 90

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