ANALYSIS OF PHOTOCHEMICAL
     OXIDANT AND  PARTICULATE
POLLUTION PATTERNS IN NEW ENGLAND
    USING REMOTE  SENSING DATA
               JUNE 1977
              FINALREPORT
     U.S. ENVIRONMENTAL PROTECTION AGENCY

               REGION I


              AIR BRANCH

-------
     ANALYSIS OF PHOTOCHEMICAL
     OXIDANT AND  PARTICULATE
POLLUTION PATTERNS IN NEW ENGLAND
    USING REMOTE  SENSING DATA
               JUNE 1977
              FINALREPORT
     U.S. ENVIRONMENTAL PROTECTION AGENCY

               REGION I


              AIR BRANCH

-------
                                   TECHNICAL REPORT DATA
                            (Please read Itiztmdions on the reverse before completing)
 1 REPORT NO
  EPA  901/9-77-002
                             2.
 4. TITLE AND SUBTITLE
 \nalysis of photochemical oxidant and particulate  pollu-
 tion patterns  in  New England using remote sensing  data
 7 AUTHOR(S)
 Ilinton  J.  Bowley,  Joseph L. Horowitz, James C.  Barnes
                                         8. PERFORMING ORGANIZATION REPORT NO

                                           P-2273
                                                           3 RECIPIENT'S ACCESSION-NO.
                                                           5 REPORT DATE
                                                      June  1977
                                         6. PERFORMING ORGANIZATION CODE
 9 PERFORMING ORGANIZATION NAME AND ADDRESS
 Environmental  Research £ Technology, Inc.
 696 Virginia Road
 oncord, Massachusetts  01742
                                                           10. PROGRAM ELEMENT NO.
                                         11 CONTRACT/GRANT NO

                                            68-02-2533
 12. SPONSORING AGENCY NAME AND ADDRESS
 Environmental  Protection Agency
 Region  1, Air  Branch
 JFK Federal Building
 Boston. Massachusetts  02203
                                                           13. TYPE OF REPORT AND PERIOD COVERED
                                                  Final Report
                                         14 SPONSORING AGENCY CODE
 15 SUPPLEMENTARY NOTES
                      Abbreviated Title:
                         Analysis of Pollution Patterns  in  New
                         England Using Remote Sensing
 16. ABSTRACT
 Imagery  from  earth surveillance satellites is examined  to  assess the potential useful-
 ness of  satellite  data for monitoring air pollutant patterns  and defining the associa-
 ted meteorological conditions in southern New England.   Three high ozone situations,
 one high total  suspended particulate episode and one high  sulfate episode are studied.
 Imagery  from  one or more of the following satellite systems:   Landsat, NOAA/VHRR, GOES,
 and DMSP, ranging  from the visible to the thermal  infrared portions of the spectrum,
 are visually  interpreted for each case.  Because of the limited data sample, it is
 difficult to  derive firm conclusions for particular imagery types or specified pollu-
 tants.   Nevertheless,  the results of the study indicate that  there is a good correla-
 tion between  certain types of high pollutant load  (including  ozone and sulfates) and
 laze and smoke,  with accompanying reductions in visibility.   There is good evidence
 that satellite  imagery can display differences in  reflectance (visible) or temperature
 (thermal  infrared) due to some combination of haze, smoke  and atmospheric pollutant
 load, on a regional basis.  The greatest promise was shown by the DMSP thermal infrared
 imagery  in application to high sulfate situations.
                               KEY WORDS AND DOCUMENT ANALYSIS
                                             jh.IDENTIFIERS/OPEN ENDED TERMS  C. COSATI F leld/GrOUp
DESCRIPTORS
remote sensing
satellite
 )ollution
regional pollution
ozone
 )articulates
sulfates
 3 DISTRIBUTION STATEMENT
        Release Unlimited
                            19 SECURITY CLASS (Tins Report)
                               Unclassified
21. NO. OF PAGES
    55
                                             20 SECURITY CLASS (This page)
                                                 Unclassified
                                                                        22. PRICE
EPA Form 2220-1 (9-73)

-------
                                      EPA 901/9-77-002
   ANALYSIS OF PHOTOCHEMICAL OXIDANT AND

     PARTICULATE POLLUTION PATTERNS IN
                NEW ENGLAND
         USING REMOTE SENSING DATA
                    By
 Environmental Research S Technology, Inc.
             696 Virginia Road
       Concord, Massachusetts 01742
          CONTRACT NO. 68-02-2533
Mr. Valentine J. Descamps, Project Officer
               FINAL REPORT


               Prepared for
      Environmental Protection Agency
                 Region I
                Air Branch
           JFK Federal Building
        Boston, Massachusetts 02203
                June 1977

-------
     This air pollution report is issued by Region I, Environmental
Protection Agency, to assist state and local air pollution control agencies
in carrying out their program activities.  Copies of this report may be
obtained, for a nominal cost, from the National Technical Information
Service, 5285 Port Royal Road, Springfield, Virginia 22151.
     This report was furnished to the Environmental Protection Agency by
Environmental Research § Technology, Inc., Concord, Massachusetts in
fulfillment of EPA Contract No.  68-02-2533.  This report has been
reviewed by Region I, Air Branch, EPA and approved for publication.
Approval does not signify that the contents necessarily reflect the
views and policies of the Environmental Protection Agency, nor does
mention of trade names or commercial products constitute endorsement or
recommendation for use.
               Region I Publication No.  EPA 901/9-77-002

-------
                                                            ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                                 FOREWORD

     The investigation  described herein was performed by Environmental
Research § Technology,  Inc.  (ERT)  for Region 1,  Air Branch of the Environ-
mental Protection Agency under  Contract No.  68-02-2533.
     The authors acknowledge  the guidance provided by Mr. Valentine J.
Descamps, the EPA Project Officer.   Data from the SAROAD data network
was provided by EPA, Region  1.   The authors are  extremely grateful to
Mr. Eugene Y. Tong of ERT for his  assistance throughout this project and
many helpful suggestions, and for  providing the  regional sulfate data
used in the study.

-------
                                                            ENVIRONMENTAL RESEARCH* TECHNOLOGY, INC
                           TABLE  OF  CONTENTS
                                                                  Page
FOREWORD                                                           v
LIST OF ILLUSTRATIONS                                              i*
1.  INTRODUCTION                                                   1
     1.1  Purpose of Study                                         1
     1.2  Review of Previous  Studies                              1
     1.3  Description of Satellite Data                            2
          1.3.1  Landsat                                           2
          1.3.2  NOAA/VHRR (Very  High  Resolution  Radiometer)       3
          1.3.3  GOES (Geostationary Operational  Environmental
                 Satellite)                                        3
          1.3.4  DMSP (Defense Meteorological  Satellite Program)   4
2.  ANALYSIS PROCEDURES - PHOTOCHEMICAL OXIDANTS/OZONE            5
     2.1  Data Sample                                              5
          2.1.1  Case 1, 20-23 May 1975                            6
          2.1.2  Case 2, 23-24 June  1975                           12
          2.1.3  Case 3,  23  July 1975                             13
3.  ANALYSIS PROCEDURES - TOTAL SUSPENDED  PARTICULATES (TSP)       23
     3.1  Data Sample                                              23
     3.2  Data Analysis for 6 May 1976                             23
4.  ANALYSIS PROCEDURE - SULFATES (S04)                            27
     4.1  Data Sample                                              27
     4.2  Comparison of 8-10  July 1974 High  Sulfate  Episode
          with Correlative Satellite Data  and  Meteorological
          Conditions                                               28
5.  SUMMARY AND CONCLUSIONS                                        37
     5.1  Discussion of Results                                    37
          5.1.1  Photochemical Oxidants/Ozone                      37
          5.1.2  Total Suspended  Particulates  (TSP)                38
          5.1.3  Sulfates (SO.)                                    38
                              4
     5.2  Conclusions and Recommendations                          39
6.  REFERENCES                                                     43
                                   vn

-------
                                                            ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                          LIST  OF  ILLUSTRATIONS

Figure                                                            Page
2-1       Analysis of Ozone  Concentration over Southern
          New England at  1500  GMT,  20 May 1975                    8
2-2       Mosaic of  Landsat-1,  MSS-4  Imagery Viewing
          Southern New England  at  1440 GMT,  20 May 1975           9
2-3       Analysis of Ozone  Concentration over Southern
          New England at  1400  GMT,  23 May 1975                    10
2-4       NOAA/VHRR  Daytime  Visible  Image Viewing the
          Northeastern United  States  at 1401 GMT,
          23 May 1975                                              11
2-5       Map Displaying  the Extent of Reduced Visibilities
          in Haze and Smoke  over the  Northeast at  1600 GMT,
          23 May 1975                                              14
2-6       Analysis o-f Ozone  Concentration over Southern
          New England at  1800 GMT,  23 May 1975                    15
2-7       Map Displaying  the Extent of Reduced Visibilities
          in Haze and Smoke  over the  Northeast at  1600 GMT,
          23 June 1975                                             17
2-8       Map Displaying  the Extent of Reduced Visibilities
          in Haze and Smoke  over the  Northeast at  1600 GMT,
          24 June 1975                                             18
2-9       NOAA/VHRR Daytime  Visible Image  Viewing  the
          Northeastern United States  at  1439 GMT,  24 June
          1975.   A Region of Low Visibility  in Haze  and
          Smoke Located over this Region  is  Easily Detected
          due to Illumination by the  Sun.                          19
2-10      Analysis of Ozone  Concentration  over Southern
          New England at  1500 GMT, 23  July 1975                    20
2-11      Landsat-2,  MSS-4 Image Viewing Connecticut and
          Eastern Long Island Sound at  1455  GMT, 23  July 1975      21
                                   IX

-------
ENVIRONMENTAL RESEARCH & TECHNO LOGY, INC
                            LIST OF ILLUSTRATIONS  (Continued)

         Figure                                                            Page

         3-1       Analysis of 24-Hour Average Values of Total
                   Suspended Particulates over Southern
                   New England on 6 May 1976                                24
         3-2       Landsat-2, MSS-4 Image Viewing  Connecticut and
                   South Central Massachusetts at  1450 GMT,
                   6 May 1976                                               25
         4-1       Analysis of 24-Hour Average Values of Sulfates
                   over the Northeastern United States on
                   8 July 1974                                              30
         4-2       DMSP Daytime Visible-to-Near Infrared Image
                   Viewing the Northeastern United States  on
                   8 July 1974                                              31
         4-3       DMSP Daytime Thermal Infrared Image Viewing  the
                   Northeastern United States on 8 July  1974                32
         4-4       Analysis of 24-Hour Average Values of Sulfates
                   over the Northeastern United States on
                   9 July 1974                                              33
         4-5       Enlargement of Portion of DMSP  Daytime  Visible-
                   to-Near Infrared Image Viewing  the Northeastern
                   United States on 9 July  1974                             34
         4-6       Enlargement of Portion of DMSP  Daytime  Thermal
                   Infrared Image Viewing the Northeastern United
                   States on 9 July 1974, with Sulfate Analysis
                   Superimposed                                             35

-------
                                                          ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                           1.   INTRODUCTION

1.1  Purpose of Study

     The purpose of this investigation was to examine the potential use-
fulness of satellite data for monitoring air pollutant patterns and for
defining the associated meteorological conditions in southern New
England.  The principal objective of Task 1 was to conduct analyses of
Landsat and meteorological satellite data (NOAA/VHRR and GOES) during
three episodes of high photochemical oxidant levels over southern New
England as reported by the EPA's "SAROAD" data network.
     The completion of Task 2 was initially directed toward analyses of
Landsat data during two episodes of high total suspended particulate
(TSP) levels over New England as reported by the "SAROAD" network.
However, problems such as cloud contamination and isolated high TSP
readings suggesting influence of local fugitive dust rather than overall
high TSP events became apparent; therefore, it was mutually agreed (ERT
and EPA Project Officer) that further analyses of TSP episodes would be
replaced by analysis of one or two incidents of high sulfate concentra-
tions over the Northeast utilizing meteorological satellite data.

1.2  Review of Previous Studies

     The ability to detect certain types of air pollution patterns from
satellite imagery has been noted by a number of investigators.  McLellan
(1971) successfully correlated a series of ATS-3 satellite images of
reflected radiation from the City of Los Angeles at 40 minute intervals
on 23 April, 1968 with various ground based meteorological data.  The
analysis of the data indicated the feasibility of satellite monitoring
of short-term atmospheric pollution variation over large urban areas.
Prospero, et al. (1970) showed the feasibility of satellite monitoring
of global scale movements of natural pollution.  In this study, a series
of ATS-3 images were correlated with aircraft and ship sampling data of
dust being transported by air currents from the arid and semi-arid
regions of North Africa across the Atlantic to the Caribbean during the
summer of 1969.

-------
ENVIRONMENTAL MSEARCH & TECHNOLOGY, INC
              Recently,  the utilization of improved satellite imagery as a means
         for monitoring  environmental quality has been further realized.  Lyons
         and Northouse (1973)  showed that the interaction of air pollution and
         meteorological  conditions over the Great Lakes led to inadvertant
         weather modification  detectable in Landsat imagery.   Griggs (1973) found
         that radiance measurements over water could be used successfully to
         calculate the vertical aerosol burden to an accuracy approaching ±10%.
         In a more recent investigation, Brown and Karn (1976) examined the
         usefulness of Landsat imagery for detecting sources of air pollution
         resulting from  coal utilization in the Ohio and Monongahela River
         valleys south of Pittsburgh, Pennsylvania.  This area is heavily indus-
         trialized and includes many coal-fired power-generating stations.  In
         this investigation, large billowy steam plumes from specific point
         sources were identified in Landsat imagery.
              In addition,  Lyons and Husar (1976) reported the likely detection
         of a synoptic-scale sulfate air pollution episode over the central and
         eastern United  States in SMS/GOES visible images.  It was shown that
         image "haziness" correlated well with midday surface visibility reports,
         which in turn appeared to correlate with sulfate aerosol concentrations.
         Unfortunately,  Lyons  and Husar were not able to show the regional extent
         of the high sulfate eposode, probably because the available sulfate
         measurements were only for a limited area.

         1.3  Description of Satellite Data

              The satellite data obtained for the completion of this study
         program included imagery from the Landsat, NOAA/VHRR,  GOES and DMSP
         satellite systems. The wide variety of imagery provided by these
         various experimental  and operational spacecraft are defined in the
         following paragraphs.

              1.3.1  Landsat

              The initial spacecraft in the experimental Landsat series was
         placed into orbit at  a height of 900 km in late July 1972 and was
         called at that  time ERTS-1, the Earth Resources Technology Satellite.
         The second spacecraft, Landsat-2, was placed into operation in January

-------
                                                            ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC

1975.  Each satellite repeats coverage of the  same  area  only  once  every
18 days; however, Landsat-2 was placed into orbit such that coverage  of
the same area was being provided by one of these spacecraft every nine
days.  A recent orbital adjustment has resulted in  repeat  coverage  on a
six- and 12-day cycle.
     The Landsat Multispectral Scanner Subsystem  (MSS) observes  in  four
spectral bands within the visible-to-near infrared  portions of the
spectrum (MSS-4, 0.5-0.6 urn; MSS-5, 0.6-0.7 urn; MSS-6, 0.7-0.8 vim;  and
MSS-7, 0.8-1.1 ym) .  Therefore, Landsat observations  are available  only
during periods of adequate solar illumination.  Landsat  views an area
approximately 185 km on a side, per image frame, as it proceeds  along
its orbital path, and has a resolution of 70-100 meters.   The scale of
the standard Landsat 9 inch x 9 inch prints is 1:1 million.

     1.3.2  NOAA/VHRR (Very High Resolution Radiometer)

     The VHRR sensor has been flown on the NOAA-2, NOAA-3, NOAA-4,  and
NOAA-5 spacecraft, so that the resulting data have been  available on  a
nearly continuous basis (one or two observations per  day)  since  January
1973.  The VHRR is a two-channel radiometer, with one channel sensitive
to reflective solar radiation in the 0.5-0.7 ym wavelengths,  and the
other channel measuring the thermal radiation emitted by clouds  and the
earth's surface in the infrared 10.5-12.5 ym wavelengths.  The spatial
resolution of the VHRR is about 1 km.  The scale of the  standard size
prints is approximately 1:10 million.
     The VHRR is designed primarily for direct readout use as an opera-
tional meteorological satellite.   The area that can be observed  when  the
satellite passes directly overhead is a strip about 2,200 km  wide and
more than 5,000 km long.   This allows broad overall synoptic  weather
patterns to be determined from each individual scene.

     1.3.3  GOES (Geostationary Operational Environmental Satellite)

     Another type of operational meteorological satellite data is
provided by the GOES system.   Launched on 16 May 1974, GOES-1 is sta-
tioned over the equator in an earth synchronous orbit in a position to
view the eastern United States and Atlantic Ocean.   Because of its  earth

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY. INC
         synchronous orbit, GOES provides coverage of the earth's disc on an
         essentially continuous basis, with data being collected every one-half
         hour.  Thus, cloud motions can be tracked and storm development can be
         monitored; using the cloud motions, it is possible to derive low-level
         wind flow.  As with the VHRR, the GOES sensor system carries a thermal
         infrared channel for obtaining nighttime data.  The visible channel
         radiometer operates in the 0.55 to 0.70 ym wavelength at a spatial
         resolution of 1 km, whereas the infrared channel operates-in the 10.5 to
         12.5 ym wavelength at a resolution of 7 km.

              1.3.4  DMSP (Defense Meteorological Satellite Program)

              The Air Force DMSP is an operational satellite system useful for
         providing meteorological and oceanographic data.  These polar orbiting,
         sun synchronous weather satellites are positioned 900 km above the
         earth.  In the operational mode, the DMSP satellites provide imagery
         every 6 hours over any spot on earth.  The imagery includes the visual
         to near infrared and thermal infrared spectral  intervals over a 3,000 km
         wide swath below the satellite.
              Real time meteorological data within the acquisition range of  the
         satellite signal, approximately a radius of 2,800 km of the receiving
         station, are provided to military sites.  These sites are scattered
         around the globe and on board U. S. Navy aircraft carriers.  The Air
         Force Global Weather Center  (AFGWC) at Offutt Air Force Base, Nebraska,
         receives stored data of global coverage; these  data have been available
         to nonmilitary users since 1972, and are archived at the University of
         Wisconsin.  The visible to near infrared wavelength channel has a
         spectral interval of 0.4 to  1.1 ym with a spatial resolution of 0.6 km;
         the thermal infrared channel operates in the  8  to 13 ym wavelength  with
         a spatial resolution of 3 km.  Scale of the standard prints is
         1:10 million.

-------
                                                           ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
        2.  ANALYSIS PROCEDURES  - PHOTOCHEMICAL OXIDANTS/OZONE

2.1  Data Sample

     The three episodes of high photochemical oxidant  levels  over
southern New England selected for analysis were initially  included  on  a
listing of high episodes supplied by the EPA-Region  1, Air Branch.   Each
of the episodes was examined to determine the availability.of useful,
cloud-free Landsat imagery.  A computer listing supplied by the  EROS
Data Center, Sioux Falls, South Dakota, showed that  useful Landsat  data
were available for only two of the episodes.  The correlative satellite
data available for the other episode selected for analysis included only
the NOAA/VHRR and GOES imagery.
     The three episodes of high photochemical oxidant  levels  analyzed  in
this investigation consisted of the following spring and summertime
periods of 1975:  20-23 May; 23-24 June; and 23-24 July.   Correlative
Landsat imagery were available for 20 May and 23 July.  The MSS-4
70 mm positive transparencies for these dates were obtained from the
U. S. Army Corps of Engineers (Waltham, Massachusetts) browse file,  and
standard size, 9 inch x 9 inch (1:1 million scale),  as well as enlarged
(approximately 1:500,000 scale), positive paper prints were processed  in
ERT's photographic laboratory.  The MSS-4 visible band was used  in  each
case because past experience has shown that this is  the most  useful  band
for detecting pollution and haze.  Much of the evidence of this  has come
from investigators of earth surface features who have  found these
features to be more susceptible to obscuration by atmospheric conditions
in Band 4 than in any other band.  Also, all available NOAA/VHRR (visible
and infrared) and GOES (visible) imagery viewing the New England region
during the periods of each episode were obtained from  the  NOAA-Satellite
Data Services Branch, World Weather Building, Camp Springs, Maryland.
     Listings of the EPA's 1975 SAROAD data for Massachusetts, Connecticut
and Rhode Island were obtained from the EPA's facility in  Lexington,
Massachusetts.  The ozone concentrations measured closest  to  the times
of the satellite images were plotted and analyzed on area  base maps.
The comparisons of maximum ozone concentrations with the correlative

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
        satellite  imagery and associated meteorological  conditions  for  each  of
        the episodes are discussed in the  following  sections.

             2.1.1  Case 1, 20-23 May 1975

             Hourly ozone concentrations at times  corresponding  to  the  readout
        times of the correlative Landsat and NOAA/VHRR satellite images  O1500 GMT,
        1000 LSI), generally exceeded the national ambient  air quality  primary
        and secondary standard of 0.080 ppm over broad areas of  southern New
        England.   However, analyses of ozone concentrations during  this  period
        revealed a definite diurnal trend with maximum concentrations occurring
        during the mid to late afternoon hours.  Analysis of the ozone  concen-
        trations over southern New England at 1500 GMT on 20 May is shown in
        Figure 2-1.  Maximum concentrations, exceeding 0.140 ppm, are located in
        extreme southwestern and southeastern Connecticut,  while another rela-
        tively high concentration, exceeding 0.120 ppm,  is  located  immediately
        north and  east of Boston.
             A mosaic of two Landsat, MSS-4, images  viewing this region at
        1440 GMT on this date is shown in Figure 2-2.  In this image, no varia-
        tions in brightness are detectable over the  land area that  could be
        attributed to the high ozone concentrations.  However, in the original
        photographic prints used in the analysis some increased  brightness
        levels [likely associated with reported low  visibilities in haze (less
        than 5 miles) and possibly, high ozone] are  observed over the darker
        water areas of Long Island Sound and to the  east of Boston  and  Cape  Ann.
        Over the land area, any varying degree of  image  brightness  due  to air
        pollution  density is likely obscured by the  varying brightness  levels of
        ground-feature reflectivities (most notably, the dense urban developments
        which appear highly reflective in the images),   No  useful NOAA  or GOES
        imagery was available for this date.
             Isolated high concentrations of ozone at a  somewhat lesser peak
        value (but still >0.080 ppm) remained over portions of the  region during
        21 and 22  May; however, no features were detectable in either the NOAA/
        VHRR or GOES imagery on these dates because  of cloud contamination.
        Analysis of the SAROAD ozone data  for 1400 GMT on 23 May (Figure 2-3)
        showed a broad band of maximum concentration O0.120 ppm) located in
        west central Connecticut, and an isolated  small  pocket  O'O.IOO  ppm)

-------
                                                             ENVIRONMENT*!- RESEARCH & TECHNOLOGY INC
 located  just  to  the west  of Boston.   The  correlative NOAA/VHRR visible
 image  (1401 GMT)  for  this date  is  shown in  Figure  2-4.   Although dense,
 offshore fog  is  observed  surrounding  the  southern  New England coastal
 regions  from  Long Island  Sound  into the southern Gulf of Maine,  no
 features associated with  the maximum  ozone  concentrations are observed
 on the image.  The band of higher  reflectance,  located near the area of
 highest  ozone concentration in  Connecticut,  is  again associated with
 dense urban development in the  Connecticut  River Valley.
     Examination of the meteorological conditions  during this period
 showed a generally light,  southerly flow  of warm,  moist,  tropical air
 associated with  a near stationary  ridge of  high pressure extending from
 well off the  middle Atlantic coastal  region,  southwestward across the
 entire southeastern United States.  The importance of heat and moisture
 becomes  more  apparent when examining  the  late morning surface tempera-
 tures and corresponding dew point  temperature readings.   During  the
 beginning of  the  period (20 and  21 May),  late morning surface tempera-
 tures ranged  between  80°  and 85 °F  across  southern  New England except for
 extreme  southern  coastal  sections  where temperatures remained in the
 mid-70's  due  to  the effect of the  light southerly  wind flow from the
 cooler ocean  waters.  Corresponding dewpoint  temperatures were generally
 in the middle  60°F range  at these  times.
     The  slight  reduction  in peak  ozone concentrations  observed  on
 22 May was likely  the result of  a  weak "back  door" cold front that moved
 westward  across New England into eastern  New  York  State during the
 morning  hours, before retreating eastward again as a warm front  early on
 the 23rd.  During  the early afternoon hours on  23  May,  when the  highest
 ozone concentrations for  the entire period were observed,  surface
 temperatures  ranged between the upper 80's to low  90's,  with dewpoint
 temperatures  ranging from  the upper 60's  to  low 70's.
     Throughout the period,  broadscale haziness resulting in reduced
visibilities accompanied  the high ozone concentrations.   This finding is
 consistent with a report by Husar, et al. (1976),  in which he mentions
that broad areas of haziness and reduced  visibilities  accompanied high
mid-day ozone  concentrations that  exceeded the  national  ambient  air
quality standard in the St.  Louis metropolitan  area  during summertime
periods of 1975.   With this  in mind, area base  maps  of  skycover,  winds,

-------
                                              060
Figure 2-1     Analysis of ozone concentration (ppm) over southern New
               England at 1500 GMT, 20 May 1975

-------
                                                                           ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
            Figure 2-2      Mosaic  of Landsat-1,  MSS-4 imagery viewing  southern New

                            England at 1440 GMT,  20 May 1975
IO
en

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
    .060
   .080
                                                                     . .060
        Figure 2-3      Analysis of  ozone concentration (ppm) over  southern New
                        England at 1400 GMT, 23 May  1975
                                            10

-------
                                   ENVIRONMENTAL RESEARCH & TECHNOLOGY
FiS^e 2-4      NOAA/VHRR  daytime
                 United States at
                         "» -«heastern
11

-------
ENVIRONMENTAL RESEARCH 4 TECHNOLOGY INC
       and visibility were plotted from the weather reports  for the period  of
       18 May through 23 May.  The 1600 GMT hourly reports were chosen to
       reduce the effect on visibilities by early morning fog conditions.
       Analyses of the reported visibilities  suggested an overall  long range
       transport of haziness and smoke into southern New England from the New
       Jersey, Maryland and eastern Pennsylvania area during the period, as
       well as some probable in situ development over southern New York  State
       and western Long Island.  The extent of minimum visibilities of from
       1.5 to 2 statute miles  in haze and  smoke for much of  Connecticut  on
       23 May, shown in Figure 2-5, compares  well with the extent  of maximum
       ozone levels of from 0.150 to 0.205 ppm reported for  this region  at
       1800 GMT on this date (Figure 2-6).

            2.1.2  Case 2, 23-24 June 1975

            The ozone concentrations as reported by the SAROAD data base for
       Massachusetts, Connecticut and Rhode Island at the corresponding  image
       times (NOAA/VHRR - 1438 GMT, and GOES  - 1800 GMT) for the period  of
       23 and 24 June 1975 were plotted on area base maps and analyzed.  No
       Landsat imagery was available for either of these days.  These analyses,
       as in the previous case, showed a marked increase in  ozone  concentration
       at the later time period (1800 GMT), especially on 23 June  when maximum
       levels increased nearly 200%, from  about 0.100 ppm to 0.280 ppm over the
       4-hour period.
            A plot of skycover, winds and  visibility for 1600 GMT  for 22, 23,
       and 24 June suggested some long range  transport of pollutants into
       southern New England from New York  State and Pennsylvania,  as well as
       probable in situ pollution development.  Areas of minimum visibilities
       of 2 to 4 miles in haze reported for much of Connecticut on 23 and
       24 June (Figures 2-7 and 2-8) correlate well with the locations of
       maximum ozone concentrations.
            With one exception, no evidence of the maximum ozone concentrations
       over southern New England was detectable on the NOAA/VHRR or GOES
       imagery of either day.  The exception  is the NOAA-4 visible image of
       24 June, shown in Figure 2-9.  This image was acquired along a satellite
       track positioned far enough to the  west to display a  low sun angle along
       the middle Atlantic coast from about Cape Hatteras to southern New
                                          12

-------
                                                            ENVIRONMENTAL RESEARCH S TECHNOLOGY, INC
England.  Therefore, the area of  low visibility  in  haze  and smoke
(2-4 miles) located over New Jersey, Pennsylvania,  southeastern  New
York State and Connecticut is easily detected due to  illumination  by  the
sun.  The extent of the low visibility area observed  over  Connecticut
agrees well with the location of  the maximum ozone  concentration as
reported by the SAROAD network.   Of all of the satellite imagery examined,
this NOAA image revealed the only detectable evidence of high pollution
concentration associated with peak ozone concentrations  over land  areas.
Sun angle apparently plays an extremely important role in  the ability of
satellites to detect high pollution concentrations  and associated  low
visibilities in the visible portions of the spectrum.
     Examination of the overall synoptic meteorological  pattern  during
this period revealed the•dominance of a warm, humid maritime tropical
air mass throughout the entire region.  A near-stationary  high pressure
system (anticyclone) was positioned just off the middle  Atlantic coastal
region resulting in the flow of warm, moist air  into  New England on
light to moderate  (10-15 knots) southwesterly winds.  Daytime high
temperature readings of from the  upper 80° to low 90°F range were
experienced over southern and central New England on  each  of the days,
and dewpoint temperatures climbed into the low 70°F range.

     2.1.3  Case 3, 23 July 1975

     The hourly ozone concentrations closest to the time of correlative
Landsat imagery (1500 GMT) on this date are shown in  Figure 2-10.  The
analysis of the ozone distribution reveals a band of  maximum concen-
tration (>0.120 ppm) extending from extreme southwestern Connecticut
northward to near Waterbury with  amounts in excess  of 0.080 ppm  extending
as far north as Hartford.   Other  areas of southern  New England reported
amounts generally between 0.050 and 0.070 ppm.
     The Landsat MSS-4 image viewing the area on 23 July is shown  in
Figure 2-11.   Again, as discovered in Case 1, the Landsat  imagery
reveals no indication of the band of maximum ozone  levels  over land
areas; however, evidence of the reduced visibilities  in  haze being
reported from Bridgeport,  Connecticut, eastward to  Block Island, Rhode
Island, is readily detectable (in the original photographic prints) over
the darker water area of Long Island Sound.  Reduced  visibilities  in
haze and smoke have accompanied each of the high photochemical oxidant
episodes being examined.

                                  13

-------
   ENVIRONMENTAL RESEARCH &TECHNOLOGY INC
          Figure 2-5
Map displaying the extent  of reduced visibilities  (statute
miles)  in haze and smoke over the northeast at 1600 GMT,
23 May  1975
o
o
                                               14

-------
                                                                ENVIRONMENTAL RESEARCH &TECHNOLOGY INC
.080
                                                       080
                                                                  .080
                                                                     .060
   Figure 2-6     Analysis of ozone concentration  (ppm)  over southern  New
                  England at 1800 GMT,  23 May 1975
                                       15

-------
                                                                ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
Figure 2-7      Map displaying the extent  of reduced visibilities (statute
                miles) in haze and smoke over the Northeast  at 1600 GMT,
                23 June  1975
                                      17

-------
ENVIRONMENTAL RESEARCH 8.TECHNOLOGY INC
      Figure  2-8     Map displaying the extent of reduced visibilities  (statute
                      miles)  in haze and smoke  over the Northeast at 1600 GMT,
                      24 June 1975
                                            18

-------
                                                                       ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
          Figure 2-9     NOAA/VHRR daytime visible  image  viewing the northeastern
                         United States at 1439 GMT,  24  June 1975.  A region of  low
                         visibility in haze and smoke located over this region  is
                         easily detected due to illumination by the sun.
in
o
                                               19

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                                                                    /080]


                                                                    ft/
                                                                   .060
                                                   060
                                                                           .060
                                                                    .060
        Figure  2-10
Analysis of ozone concentration  (ppm)  over southern New

England at 1500  GMT, 23 July 1975
                                             20

-------
                                                                 ENVIRONMENTAL RESEARCH & TECHNOLOGY IMC
Figure  2-11     Landsat-2,  MSS-4  image viewing Connecticut  and eastern  Lon£
                Island  Sound at 1455  GMT, 23 July 1975
                                       21

-------
ENVIRONMENTAL RESEARCH 4TECHNOLOGY, INC
            The synoptic meteorological conditions associated with this episode
       were also analogous to the previous two cases.  Examination of the
       23  July surface charts showed a nearly stationary ridge of high pressure
       centered well  to the southwest near Virginia.  Therefore, a warm,
       moist flow of  air on light to moderate southwesterly surface winds was
       experienced over southern New England.  Maximum surface temperatures
       reached the low 80's across extreme southern coastal sections and the
       upper 80°F range over northern Connecticut and Massachusetts.  Corres-
       ponding dew point temperatures ranged from the mid to upper 60°F level
       throughout the region.
                                         22

-------
                                                             ENVIRONMENTAL RESEARCH S, TECHNOLOGY, INC

      3.  ANALYSIS PROCEDURES  -  TOTAL  SUSPENDED PARTICULATES (TSP)

3.1  Data Sample

     Examination of correlative  Landsat  coverage during  a number of
periods of high total suspended  particulate  (TSP)  levels over  southern
New England during 1974 and  1975 showed  that no data  were acquired  by
Landsat during any of the episodes.  Therefore,  a computer query search
was requested from the EROS  Data Center,  Sioux  Falls,  South Dakota,  for
a listing of Landsat coverage  of central  and southern  New England for
all dates with less than 50% cloud cover.  A check of  this computer
listing for dates of useful  Landsat coverage showed that correlative
SAROAD TSP data [recorded every  six days) was available  for only two  of
the dates, 4 April and 6 May 1976.  A  check of  the 1976  SAROAD data,
obtained from the EPA facility in Lexington, revealed  low TSP  levels  on
4 April; however, three small  pockets  of  relatively high TSP levels
(exceeding national ambient  air  quality  secondary standard of  150 yg/m
for 24-hour average) were found  to exist  over southern New England  on
6 May 1976.
     Although no Landsat coverage was  available  for two  dates  of reportedly
high TSP concentrations over southern  New England (24  January  and
18 April 1975), NOAA/VHRR and  GOES imagery were  obtained to determine if
the lower resolution of these  satellites  was at  all useful  for detecting
the high TSP events.  Unfortunately, the  imagery was not useful  because
of cloud contamination over  the  region on each  of these  dates.
     The 24-hour average values  of TSP were plotted and  analyzed on area
base maps for 6 May 1976, the  one case for which correlative Landsat
data existed.   A comparison  of the TSP analysis  with the Landsat satellite
data is discussed in the following section.

3.2  Data Analysis for 6 May 1976

     Analysis  of the 24-hour average values of  TSP  as  reported by the
EPA's SAROAD data network is shown in  Figure 3-1.   This  analysis reveals
that the highest concentrations  were confined to  isolated small  areas in
central Connecticut, near Springfield, Massachusetts,  and over Providence,
                                                       3
Rhode Island,  where values generally exceeded 150  yg/m .
                                   23

-------
ENVIRONMENTAL RESEARCH S TECHNOLOGY INC
        Figure 3-1     Analysis of 24-hour  average values  of total suspended
                        particulates (ug/m^)  over southern  New England on  6 May
                        1976
                                            24

-------
                                                                  ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
42° *
    Figure 3-2     Landsat-2,  MSS-4 image viewing  Connecticut and south  cen-
                   tral Massachusetts at 1450 GMT,  6 May 1976
                                        25

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
           The correlative  Landsat  image  (1450  GMT),  shown  in  Figure 3-2,
      views the areas of high TSP levels  located  in central  Connecticut and
      near Springfield, Massachusetts.  This  image shows  a  thin veil of high
      cloudiness  (cirrostratus)  obscuring much  of the area  of  high TSP
                3
      (>200 yg/m  )  located  over  Springfield.  Examination of the 1500 GMT
      hourly weather data revealed  that most  stations in  southern New England
      were reporting high,  thin  clouds.  The  small pocket of high TSP
      (>150 yg/m  )  located  over  central Connecticut lies  under generally clear
      skies; however, no distinct reflectance boundaries  associated with the
      maximum TSP concentration  are observed  in the image.
           Although the isolated pockets of high  TSP  on this date fall within
      a narrow band of relatively high TSP levels O100 yg/m ), which extends
      northward across Connecticut  and then to  the east-northeast across
      Massachusetts  (Figure 3-1), it  is possible  that the high readings
      reflect the actual influence  of local fugitive  dust (such as from roadways
      and gravel  areas) rather than the ambient TSP conditions.  Also, the
      precise times of the  occurrence of high TSP levels  on  this date, which
      contributed to the overall high 24-hour average values,  could have taken
      place much  later in the day,  and not near the time  of  the Landsat image.
           Analysis of the  1500  GMT hourly surface weather data revealed a
      cold front  advancing  slowly southeastward across northern areas of New
      England at  the time of the Landsat  image, with  a moderate (15 to 20  knots)
      south to southwest surface wind flow regime over southern New England.
      This surface  wind flow pattern  agrees remarkably well  with the orienta-
      tion of the band of maximum TSP levels  (>100 yg/m ) observed in Figure 3-1,
      Further examination of the ensuing hourly weather information showed
      that this wind pattern prevailed throughout much of the  remainder of the
      day.
           The correlative  NOAA/VHRR  and  GOES imagery on  this  date revealed no
      features suggesting association with the  locations  of  the maximum TSP
      levels.
                                         26

-------
                                                           ENVIRONMENTAL RESEARCH S TECHNOLOGY, INC
                 4.  ANALYSIS  PROCEDURE  -  SULFATES  (SO ~)

4.1  Data Sample

     Because of  the difficulty  of  identifying  useful  correlative Landsat
imagery, plus possible TSP  sampler  location  problems  affecting the com-
pletion of the Task 2 phase of  this  investigation  (see Section 3), a
modification of  the original  work  statement  was  requested.   It was
subsequently agreed by the  EPA  Project  Officer that  further analysis of
TSP episodes would be deleted.   Instead,  an  analysis  of one or two
incidents of high sulfate concentrations  over  the  Northeast would  be
undertaken with  comparisons being  conducted  with correlative meteoro-
logical satellite imagery.  The  rationale for  examining regional sulfate
episodes with corresponding satellite-observed haze  layers  was provided
by several recent regional air pollution  studies.  Husar, et al.  (1976),
for example, found that  large masses of low-visibility air  can be  tracked
as entities for  several  days, using only  the routine  synoptic observations.
Furthermore, there was evidence  that the  areally extensive  turbidity
reflected the existence  of a  large number of sulfate  aerosols,  whose
particle size distribution shows a peak between  0.05  and 1  pm (see,  for
example, Wilson, et al., 1976).  The correlation between atmospheric
visibility (and  turbidity) and sulfate  concentration,  both  of which
exhibit regional characteristics,  leads therefore  to  the present attempt
to find a qualitative correspondence via  the remotely-sensed medium.
     The case selected for analysis originated from ERT's data base
which is derived from the Electric Power  Research  Institute,  Sulfate
Regional Experiment (EPRI/SURE) program,  several Tennessee  Valley
Authority (TVA)  stations, as well as from the National  Air  Sampling
Network (NASN)  stations.  The sulfate measurements taken at  all  stations
consist of 24-hour average values obtained by  chemical  analysis  of high-
volume particulate filters.   This high  sulfate episode  over  the  north-
eastern United States, for which data existed  in the  ERT data base and
correlative satellite imagery was found to exist,  occurred  during  the
period of 8-10 July 1974.  The comparison of this  high  sulfate  episode
with the corresponding satellite data and associated meteorological
conditions is discussed in the following  section.
                                  27

-------
ENVIRONMENTAL RESEARCH a TECHNO LOGY, INC
         4.2  Comparison of 8-10 July  1974 High  Sulfate Episode with  Correlative
              Satellite Data and Meteorological  Conditions

              Analysis of sulfate  levels during  this period,  as derived  from  the
         ERT data base, showed that this episode, which actually  began about
         4 July  over the Ohio Valley,  reached  a  peak on 8 and 9 July  over  West
         Virginia,  Pennsylvania and New York.  By 10 July,  the geographical peak
         had subsided over the Ohio Valley,  but  a new  episode had developed along
         the middle Atlantic coastal region  northward  into  southern New  England.
              Figure 4-1 shows the analysis  of 24-hour average sulfate levels
         over the region on 8 July.  Concentrations as high as 40 yg/m   are
         observed over southwestern Pennsylvania and the Ohio-West Virginia
         border.  The four statute mile visibility  isopleth is also indicated and
         shows a generally good agreement with the  location of the maximum sul-
         fate levels.
              The DMSP daytime visible-to-near infrared channel image and  cor-
         responding daytime thermal infrared image  of  8 July are  shown in
         Figures 4-2 and 4-3, respectively.   The visible-to-near  infrared  image
         shows mostly cloud-free conditions  over the region of high sulfate
         concentrations but does not indicate any variations in reflectance that
         could be attributed to the high sulfate concentrations.   In  the thermal
         infrared,  however, an overall increase  in  brightness is  observed  over
         the region.  This increase in brightness  (lower  temperatures)  suggests
         that the radiometer is measuring,  at least in part, the  emittance of
         the top of the pollutant/haze/smoke layer  rather  than the surface.   In
         addition,  the daytime  surface temperatures beneath this  layer  averaged
         4°F to  8°F lower  than  in  surrounding, unobscured  areas,  thus con-
         tributing  to the  depressed thermal  response in  the imagery.
              The  analysis of  the  24-hour  average  sulfate  levels  over the region
         on  9 July, shown  in Figure 4-4, reveals an overall increase  in maximum
         concentrations with  levels as high as 75  yg/m  over western  Pennsylvania
                     3
         and 48  yg/m  over West Virginia.   The four statute mile  visibility
         isopleth  is  also  indicated and again shows a generally good  agreement
         with  the  location of  maximum  sulfate concentrations.
                                            28

-------
                                                            ENVIRONMENTAL RESEARCH S TECHNOLOGY. INC
     Enlargements of portions of the DMSP daytime visible-to-near  infrared
band and corresponding daytime thermal infrared  (sulfate analysis  super-
imposed) images of 9 July are shown in Figures 4-5 and 4-6.  The visible-
to-near infrared image displays small areas of scattered to broken
stratocumulus clouds located over portions of New York, Pennsylvania,
West Virginia, Ohio and Kentucky but, again, does not display any  patterns
associated with the area of high sulfates.  These clouds also appear
very bright (cold) in the corresponding thermal  infrared image; in
addition, the entire area of maximum sulfate concentrations appears
somewhat brighter (colder) on this image than the surrouding cloud-free
areas, suggesting once again the presence of high pollution concen-
trations and low visibilities.  In this instance, the brighter pattern
in the thermal infrared and the reduced visibilities (four mile visibility
isopleth, Figure 4-4) both extend into Michigan  and Wisconsin, sug-
gesting that high sulfate concentrations may also have been present in
those areas on this date; corroborative ground sulfate measurements were
unavailable for these two states.
     Analysis of NOAA/VHRR nighttime thermal infrared imagery for  8 and
9 July also showed increased brightness (lower temperatures) within the
areas of maximum sulfate concentrations; however, the extremely high
contrast of these images made them unsuitable for reproduction, and so
they are not shown here.
     The meteorological conditions during this period may be summarized
as the dominance of a warm and humid, maritime tropical air mass through-
out the entire region.   On 8 July, a slow-moving cold front extending
from Quebec to Minnesota was advancing slowly southward.   By 10 July
when the mid-Atlantic coast episode occurred, the cold front was situated
along an east-west line extending from central New England to Minnesota.
     During the early part of the period of 8 and 9 July,  the large-
scale surface wind flow was light southerly or southwesterly, rarely
reaching 10 knots at any reporting station.   The fairly persistent wind
flow from the south and southwest would qualitatively indicate large-
scale transport of pollutants toward the northeast.  However, in this
episode, the time required for northeastward transport of pollutants
would have been so long that pollutant advection alone cannot fully
explain the regionality of the sulfate episode.   There was probably
some in situ pollution development.
                                  29

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
                                                                                                                                                                      ' — ' CTl
                                                                                                                                                                          i — (
                                                                                                                                                                       t/5
                                                                                                                                                                       0>  X
                                                                                                                                                                      4-> i-l
                                                                                                                                                                       OS  p
                                                                                                                                                                           oo
                                                                                                                                                                       to
                                                                                                                                                                       tn  cu
                                                                                                                                                                       CD  -P
                                                                                                                                                                       3  cti
                                                                                                                                                                      i— I  4-1
                                                                                                                                                                       ni  en
                                                                                                                                                                           -P
                                                                                                                                                                          -H
                                                                                                                                                                       f-i  0>
                                                                                                                                                                       3  +->
                                                                                                                                                                       O  t/>
                                                                                                                                                                      f.  rt
                                                                                                                                                                        I   
                                                                                                                                                                           f-l
                                                                                                                                                                      4-1  O
                                                                                                                                                                       O  C
                                                                                                                                                                      •H  X
                                                                                                                                                                       (/>  -P
                                                                                                                                                                       X
                                                                                                                                                                      I-H  fn
                                                                                                                                                                       OJ  0)
                                                                                                                                                                       p:  >
                                                                                                                                                                      <:  o
                                                                                                                                                                       0)
                                                                                                                                                                       fn

                                                                                                                                                                       M
                                                                                   30

-------
                                               ENVIRONMENTAL RESEARCH S TECHNOLOGY INC

                                                                 0

                                                                •M

                                                                 bo

                                                                •H

                                                                 0
                                                                •H
                                                                 >

                                                                 0

                                                                 cd  ^3"

                                                                • H  CTi
                                                                    rH

                                                                 0   X

                                                                 rt  '3

                                                                4-1
                                                                 C  00
                                                                • H

                                                                 r<   O
                                                                 rt
                                                                 0   t/i
                                                                 C   0
                                                                 I  4->
                                                                 O   CTj

                                                                 I  (/)
                                                                 0

                                                                ,0   0
                                                                •H  4->
                                                                 (/)  -H
                                                                •H   C
                                                                 >  3

                                                                 0   C

                                                                • H   0

                                                                 X  w
                                                                 as   n)
                                                                13   0

                                                                CL,  +->

                                                                S   o
                                                                Q   C
                                                                CM
                                                                 I
                                                                n-
31

-------
       ENVIRONMENTAL RESEARCH & TECHNOLOGY INC
                                                                                                                                                      f-l
                                                                                                                                                      o
                                                                                                                                                      0)

                                                                                                                                                     fi
                                                                                                                                                      bO

                                                                                                                                                     •H

                                                                                                                                                      (D
                                                                                                                                                     •H
                                                                                                                                                      0> h-
                                                                                                                                                      M O1
                                                                                                                                                     -O  3
                                                                                                                                                      0) 1-5
                                                                                                                                                      fn
                                                                                                                                                      rt oo
                                                                                                                                                      ^H
                                                                                                                                                     MH  C
                                                                                                                                                      C  O
                                                                                                                                                     • H
                                                                                                                                                      03 4->
                                                                                                                                                      E  rt
                                                                                                                                                      H 4->
                                                                                                                                                      0) CO
                                                                                                                                                      e
                                                                                                                                                     •H
                                                                                                                                                      oj  C
                                                                                                                                                     t3  fn
                                                                                                                                                          
-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY IMC
                                           e

                                           M rf
                                           3  r-~
                                          v — ' CTi
                                              i — l
                                           l/l
                                           
                                           3   rt
                                          T— (  +->
                                           03  CO
                                           >
                                              T3
                                           CD   0)
                                           M 4->
                                           03  -H
                                           fn   C
                                           03
                                               fn
                                               CD
                                          f,  03
                                            l   0)
                                          •* ,fi
                                          CXI 4-1
                                               ^
                                          4n  O
                                           O  C

                                           i/l  
                                           X
                                               >
                                               O
                                           3
                                           tx>
                                          • H
                                          tL,

-------
ENVIRONMENTAL RESEARCH ^TECHNOLOGY INC
                                                                                                                                                                 o
                                                                                                                                                             fn
                                                                                                                                                             oj  t/)
                                                                                                                                                             CD  (L)
                                                                                                                                                             C  4-1
                                                                                                                                                              i   rt
                                                                                                                                                             O  4->
                                                                                                                                                             4-1  CO
                                                                                                                                                              I
                                                                                                                                                             H
                                                                                                                                                             t/>  C
                                                                                                                                                             •H 3

                                                                                                                                                                 c
                                                                                                                                                             0)  fn
                                                                                                                                                             G  CD
                                                                                                                                                             •H 4-1
                                                                                                                                                             4-1  t/)
                                                                                                                                                             X oj
                                                                                                                                                             oj  0
                                                                                                                                                             O,  (H
                                                                                                                                                             co  o
                                                                                                                                                             O

                                                                                                                                                             C
                                                                                                                                                                 C
                                                                                                                                                            •H -H
                                                                                                                                                             4->  S
                                                                                                                                                             fn  CJ
                                                                                                                                                             O -H
                                                                                                                                                             O  M
                                                                                                                                                                 nj
                                                                                                                                                             4,S^

                                                                                                                                                             CD
                                                                                                                                                             S 13
                                                                                                                                                             CD  
                                                                                                                                                            LO
                                                                                                                                                              I
                                                                                                                                                             bo
                                                                                                                                                            •H
                                                                                                                                                            P-,
                                                                               34

-------
                                                             ENVIRONMENTAL RESEARCH &TECHNOLOGY INC
Figure 4-6     Enlargement  of portion of DMSP daytime thermal  infrared
               image viewing  the northeastern United States on 9 July
               1974, with sulfate analysis superimposed
                                   35

-------
ENVIRONMENTAL RESEARCH » TECHNOLOGY INC
            Highest  sulfate  concentrations were, for the most part,  found
       within the warm,  moist air south of the cold front.  On  each  day during
       the period, the dewpoint temperatures reached 70°F as far north as the
       mid-Atlantic  states along the coast and into the upper midwest  region
       west of the Appalachians.   In addition, visibilities were generally less
       than four miles in haze and smoke over much of the region.
                                          36

-------
                                                           ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                      5.  SUMMARY AND CONCLUSIONS

5.1  Discussion of Results

     5.1.1  Photochemical Oxidants/Ozone

     Analysis of three high photochemical oxidant episodes over  southern
New England indicates a definite diurnal trend with the maximum  ozone
concentrations occurring in the mid to late afternoon, and minimum
levels generally confined to the late night and early morning hours.
Unfortunately, the mid-morning readout times of the correlative  Landsat
images did not coincide with these afternoon peak levels; nevertheless,
the ozone concentrations at the time of the satellite passage  (1400-
1500 GMT) generally exceeded the national ambient air quality primary
and secondary standards of 0.080 ppm over much of southern New England.
     Throughout each of the periods examined, broad scale haziness
resulting in reduced visibilities accompanied the high ozone events.
Analyses of the locations of minimum visibilities in haze and smoke
across southern New England were found to compare well with the  loca-
tions of peak ozone concentrations.
     Although, for the most part, the areas of the maximum ozone con-
centrations and haziness were not discernible in the correlative Landsat
imagery, some increased reflectance levels were observed over the darker
water areas of Long Island Sound and to the east of Boston near  coastal
stations that were reporting low visibilities.  Over the land areas, any
varying degree of image reflectance due to air pollution density or low
level haze layer was not discernible due to the highly variable bright-
ness levels associated with various ground-feature reflectances, espe-
cially the higher reflectances associated with dense urban development.
     Examination of the correlative NOAA/VHRR and GOES satellite data
also revealed no features suggesting a relationship to locations of peak
ozone concentrations, with one notable exception.  In this instance, a
NOAA-4 daytime visible image was acquired along a satellite track far
enough to the west to display a low sun angle along the mid-Atlantic
coastal region northward into southern New England.  This resulted in an
area of low visibility in haze and smoke (and possibly high ozone con-
centration) of two to four miles over New Jersey, Pennsylvania,  southern
                                  37

-------
ENVIRONMENTAL RESEARCH S TECHNOLOGY INC
        New York and Connecticut being easily detected on the imagery due to
        illumination by the sun.  Sun angle apparently plays a significant role
        in the capability of satellites to observe high pollutant concentrations
        and associated low visibilities in the visible portions of the spectrum.
             Analysis of the meteorological conditions accompanying each of the
        three high ozone episodes indicates a strong similarity in overall
        synoptic pattern.  In each case, the episode was accompanied by the
        dominance of warm, humid tropical air throughout the region.  In each
        case, a nearly stationary high pressure system (anticyclone) was cen-
        tered over the mid-Atlantic states resulting in the flow of warm, moist
        air into New England on light to moderate south to southwesterly surface
        winds.  Daytime high temperature readings were generally reported in the
        mid-80°F to low 90°F range, while corresponding dew point temperatures
        ranged from the upper 60°F to low 70°F level.

             5.1.2  Total Suspended Particulates  (TSP)

             A lack of correlative Landsat coverage during times of high TSP
        events over southern New England, as well as cloud contamination when
        other satellite coverage was available, together with a lack of con-
        fidence in the representativeness of a number of the important TSP data
        readings severely limited this phase of the investigation.
             Analysis of one correlative Landsat  image that provided coverage
        during a period of isolated high TSP levels reported over southern New
        England revealed no distinct boundaries to suggest any association with
        the location of the maximum TSP concentrations.  NOAA/VHRR and GOES
        imagery for the same period also showed no evidence of high TSP concen-
        trations.  It appears likely, however, that the isolated high levels
        were associated with localized conditions at the location sites of the
        sensors rather than with a widespread pollution episode, and thus no
        real test of the value of satellite imagery for high TSP episodes was
        accomplished in this study program.

             5.1.3  Sulfates (SO )

             The final phase of this investigation involved the detection of
        high sulfate episodes in correlative meteorological satellite imagery.
        Although the areas of high sulfate concentrations could not be detected
                                           38

-------
                                                           ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC

in the DMSP visible-to-near infrared channel imagery at the time  of  a
high sulfate episode over the Northeast  (8-10 July  1974), both the
daytime and nighttime DMSP thermal infrared imagery during this period
showed an overall increase in brightness  (lower temperatures) within
regions of peak sulfate concentrations.  The lower temperatures observed
within the area of high sulfate levels,  as compared to other areas,
suggest that the satellite sensor was viewing, at least in part,  the top
of the pollutant/haze/smoke layer rather than the surface.  In addition,
the daytime surface temperatures beneath this layer averaged 4°F  to
8°F lower than in surrounding, unobscured areas, thus contributing to
the depressed thermal response in the imagery.
     The dominance of a warm, humid, maritime tropical air mass through-
out the region of high sulfate levels was observed throughout the
period.  A persistent, light surface wind flow pattern from the south
and southwest indicated large-scale transport of pollutants toward the
northeast, as well as in situ development of high pollution concentrations.

5.2  Conclusions and Recommendations

     Various types of satellite imagery are capable of detecting the
atmospheric conditions associated with some regionalized air pollutant
concentration situations.   The current study looked at Landsat,
NOAA/VHRR, GOES and DMSP imagery products, including portions of the
visible, near infrared,  and thermal infrared sectors of the spectrum.
The small sample size of each imagery type and differing concentrations
of various pollutants does not allow any definitive conclusion to be
drawn regarding the specific effectiveness of a particular imagery
type for a specified pollutant.   However, some important general observa-
tions may be derived from this study, as follows:

     1)   It is apparent that there is a good correlation between certain
          types of high  pollutant load (including ozone and sulfates) and
          haze and smoke,  with accompanying reductions in visibility.
          There is good  evidence that satellite imagery can display
          differences in reflectance (visible)  or temperature (thermal
          infrared)  due  to some  combination of haze, smoke and atmo-
          spheric pollutant load,  on a regional basis.   It does not
                                  39

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                   appear possible, at this time, to differentiate between
                   pollutant concentrations and haze and/or smoke utilizing
                   only the satellite imagery;
              2)   It has been found that some types of imagery hold more promise
                   than others for helping to delineate the regional extent of
                   pollution-associated conditions.  Landsat visible imagery
                   tends to exhibit so much variability in reflectance  levels
                   over land areas that differences in atmospheric conditions,
                   other than cloudiness, are difficult to observe.  On the other
                   hand, differences among land features are far less pronounced
                   on some of the smaller scale visible and thermal infrared
                   imagery (NOAA/VHRR and DMSP), due to significantly lower
                   resolutions.  These image types provide much better  backgrounds
                   on which to detect reflectance and thermal differences resulting
                   from high atmospheric pollution episodes.  In addition, sun
                   angle seems to play a significant role in the detectability  of
                   pollutant-associated conditions in the visible portions of
                   the spectrum.  Of the various combinations of type of episode
                   and imagery analyzed during this project, the greatest
                   promise was shown by the DMSP thermal infrared imagery in
                   application to high sulfate situations;
              3)   The value of  satellite systems for monitoring the regional
                   transport of  pollutants ultimately depends on their  capability
                   for at least  daily repetitive observation, as well as the
                   ability of these systems to temporally coincide their obser-
                   vations with  the usual time of day of highest pollutant
                   levels.

              It  is  suggested that further study be made to allow additional
          specificity and quantification of these conclusions.   Since the  current
          investigation was heavily Landsat-oriented, ERT recommends that  a
          further  in-depth investigation be made of the  smaller  scale types  of
          imagery  (>1 km resolution and less)  such as NOAA/VHRR,  DMSP and  GOES for
          which  much  greater promise has been  shown in the detection and moni-
          toring of pollution-associated  situations.  A  suggested approach  to  such
                                            40

-------
                                                           ENVIRONMENTAL RESEARCH S TECHNOLOGY, INC
a study would be to take several high sulfate episodes over the eastern
United States and determine the relative capability of each specific
satellite system for delineating and monitoring the movement of the
pollutant-laden air.  ERT would utilize its extensive and unique data
base which is derived from the EPRI/SURE program, several Tennessee
Valley Authority (TVA) stations, and the National Air Sampling Network
(NASN) stations.  As part of this study, a further investigation of the
influence of factors such as sun angle upon detection of pollutants
within the visible bands of satellite sensors could be undertaken.  For
this, it would be possible to utilize the GOES imagery, which is available
on a half-hourly basis throughout the day.  It is also suggested to
combine with this program a theoretical analysis of the physics of
detecting pollutants from space, to help substantiate the findings of
the imagery/field data oriented studies.
     An additional topic for investigation could include analysis of
selected digitized, computer-compatible data from the NOAA/VHRR and
Landsat sensors.  This would allow much finer separation of reflec-
tance and thermal levels on the imagery than by visual interpretation.
No analysis of digitized data was possible under the scope of the
current study.   Some further means of extracting more useful information
from the Landsat imagery could also be assessed, such as comparing
imagery from different MSS spectral bands, perhaps using ratioing
techniques, or processing the Landsat imagery photographically in such a
way as to subdue earth surface features and enhance atmospheric features.
     Since only a very limited sample was available in this study,
further investigation should be carried out to assess the utility of
satellite observations to detect high TSP episodes.  As one possible
study, correlative meteorological satellite imagery (NOAA/VHRR and GOES)
and available Landsat data obtained during the recent, severe dust
storms originating over the widespread drought areas of the southwestern
United States (late February 1977) would be analyzed to determine the
extent to which the high TSP levels are detectable in the various satellite
data.  ERT already has seen significant evidence of the dust clouds on
both NOAA/VHRR and GOES imagery of this period.   Attempts would be made
                                  41

-------
ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
         to obtain sufficient ground truth TSP measurements for comparison  with
         the imagery.  An investigation of this type would allow  identification
         of the levels and distribution of TSP necessary for detection by earth
         observational satellites, as well as determination of to what extent
         the advection and dispersion characteristics can be monitored by
         satellite imagery viewing land areas.
              The conclusions of the current study demonstrate the vast  potential
         that exists in the realm of satellite remote sensing for detection and
         monitoring of regional pollutant concentrations.  Sufficient evidence
         has been accumulated here to suggest that the Environmental Protection
         Agency (EPA) continue to maintain interest, and play a significant
         role, in the development of the specifications for the use of present
         and future earth surveillance satellite systems.  Only by such  con-
         tinued awareness and involvement will EPA ensure that the potential of
         these systems will be available in the proper modes and  further
         developed, as appropriate, for EPA operational purposes.
                                           42

-------
                                                           ENVIRONMENTAL RESEARCH & TECHNOLOGY, INC
                             6.   REFERENCES
Brown, F. R., and F. S. Karn,  1976:   "Air  Pollution  from the Ohio River
     and Monongahela River Valleys,"   ERTS-1,  A  New  Window on our Planet,
     U. S. Geological Survey,  Professional  Paper 929,  pp.  261-265.

Griggs, M.,  1973:  "A Method to Measure  the  Atmospheric  Aerosol  Content
     Using ERTS Data,"  Third  ERTS Symposium,  Paper  E2,  pp.  1505-1518.

Husar, R. B., N. V. Gillani, J. D. Husar,  C. C.  Paley, and P.  N.  Turcu,
     1976:   "Long Range Transport of  Pollutants  Observed Through Visibility
     Contour Maps, Weather Maps and Trajectory Analysis," Proc.  Third
     Symposium on Atmospheric  Turbulence,  Diffusion  and  Air  Quality,
     October 19-22, 1976, Raleigh, North Carolina, American  Meteorological
     Society, pp. 344-347.

Lyons, W. A., and R. A. Northouse, 1973:   "Use of ERTS-1  Imagery in Air
     Pollution and Mesometeorological  Studies  Around the Great  Lakes,"
     Third ERTS Symoposium, Paper El,  pp.  1491-1504.

Lyons, W. A., and R. B. Husar, 1976:   "SMS/GOES  Visible  Images  Detect a
     Synoptic-Scale Air Pollution Episode,"  Monthly  Weather  Review,
     Vol. 104, pp. 1623-1626.

McClellan, A., IV, 1971:  "Satellite  Remote  Sensing  of Large Scale  Atmo-
     spheric Pollution," Proc. Second  International  Clean  Air  Congress,
     Academic Press, New York, p.  1408.

Prospero, J. M., E. Bernatti,  C. Schubert, and T. N. Carlson,  1970:   "Dust
     in the Caribbean Atmosphere Traced to an  African  Dust Storm,"
     Earth and Planetary Science Ltrs., Vol. 9,  p. 287.

Tong, E.  Y., G.  Battel, and R. B.  Batchelder,  1976:  "Case Studies  of
     Atmospheric Sulfate Distribution  over the Eastern United  States,"
     Proc. Fifteenth Purdue Air Quality Conference,  November 8-9,  1976,
     Indianapolis, Indiana.

Wilson, W. E., R. J. Charlson, R.  B. Husar,  K. T. Whitby,  and  D.  Blumenthal,
     1976:  "Su_lfates in the Atmosphere",  Paper  76-30-06,  69th Annual
     Meeting, Air Pollut. Control  Assoc.,  Portland,  Ore.,  20 pp.
                                  43

-------