EPA TECHNOLOGY TRANS REQOJNG ZINC IN VISCOSE RAYON PLANTS BY TWO STAGE PRECIPITATION U.S. ENVIRONMENTAL PROTEC~~ .. flAL DEMONSTRATDN GRANT ------- EPA TECHNOLOGY TRANSFK RECYOJNG ZINC IN VISCOSE RAYON PLANTS BY TWO STAGE PRECIPITATION ENTAL ., __ .„ . .\lr\L DEMONSTRATION GRANT ------- *». Densator Reactor ------- Over 50 million Ibs. of zinc sulfate are used annually in the United States for the manufacture of approximately one billion pounds of viscose rayon. Zinc is used as a regeneration retardant in the acid spinning bath. Since it is not consumed in any of the viscose reactions, these 50 million pounds of zinc represent process losses, through dragout by the filaments to the subsequent wash streams, filter backwashing, splashes, leaks and the washing of equipment. The effects of zinc as a pollutant are well documented. Concentrations as low as 1.0 ppm have been shown to be harmful to fish. In addition, there is some evidence indicating that zinc has a synergistic property when associated with copper. Although it has been known that zinc can be precipitated from the acid waste streams by the use of lime, the resultant sludge has been of low zinc assay, contaminated with other compounds, and with very poor settling characteristics. In commercial operations, the sludge presented a disposal problem and recovery of zinc suitable for recycle was impossible. In this EPA demonstration grant with the American Enka Company, a process for precipitating a dense sludge of high zinc assay was proven. The zinc in the sludge was recovered and recycled to the rayon manufacturing plant. This recycling of zinc was shown to have no ill effects on the rayon yarn. There are 10 viscose rayon manufacturing plants in the United States, all of which are believed to use zinc sulfate in their spinning bath. This process greatly enhances the economics of removing this source of zinc pollution, allowing neutralization of the acid stream and recovery of the zinc of a good profit for industrial yarns and at a moderate cost for textile yarns. ------- American Enka Waste Treatment Facilities The key to this zinc recovery process is a two-stage precipitation with the second precipitation taking place under careful pH control, using sodium hydroxide, in contact with a circulating slurry of zinc hydroxide crystals. All of the zinc precipitates in the second step, most of the impurities in the first. Referring to the flow sheet, Figure 1, the elements of the process are as follows: Acid and alkaline waste streams are collected in a neutralization tank (T-l). Here sufficient lime is added to raise the pH to 6.0. At this point, no zinc hydroxide will precipitate but a portion of the iron, calcium sulfate, and other impurities will form a light precipitate. With a coagulant aid, the mixture is sent to a clarifier (C-l) where a clear overflow containing the dissolved zinc is obtained. This clear overflow is contacted in a reactor (R-l) with a circulating stream of previously precipitated sludge containing zinc hydroxide. The pH is raised subsequently to 9.5 —10.0 with sodium hydroxide. The bulk of the zinc precipitates onto the existing crystals in the circulating slurry. At steady state conditions, a withdrawal of the circulating slurry stream is made equivalent to the zinc being added. This dense sludge is then settled (T-2). The settled sludge of 4-7% zinc assay is converted back to zinc sulfate with sulfuric acid (T-3) and sent back to the spinning bath. If desired, the sludge can be filtered or centrifuged to 18% solids before dissolving with acid. The zinc content of the overflow water from the densator-reactor is set by the pH-solubility relationship of zinc in water and results in a zinc content of 0.5 — 1 ppm atpH = 10. Once the precipitated zinc is removed from the wastewater, the pH can be readjusted to a lower value. ------- ------- Typical Influent vs. the Treated Effluent at American Enka's North Carolina Plant (Basically Textile Yarn Nominally 50 Million Ibs. Per Year) Ibs./lOOO Ibs. yarn unless otherwise noted IN OUT Flow pH Zn H2SO4 Na2SO4 CaSO4 MgSO4 BOD COD 131,000 (1500 GPM) 1.5-3.0 12.5 (95 ppm) 184 (1400 ppm) 288 (2200 ppm) 13.8 (105 ppm) 3.1 (24 ppm) 7.0 (53 ppm) 131,000 (1500 GPM) 8.0 (after final pH adjustment) 0.13(1 ppm) 320 (2440 ppm) 256 (1940 ppm) 13.8 (105 ppm) 3.1 (24 ppm) 7.0 (53 ppm) ------- The conventional technique for removing zinc from the spinning acid waste stream has been direct lime precipitation to a pH of about 10, with no zinc recovery. The economics of this approach are compared to the American Enka Zinc Recycle Process. In order to protect proprietary spinning information relating to acid/zinc ratios for a given product mix of yarns, it has been necessary to choose a hypothetical product mix and acid ratio which, although reasonable for economic evaluation, does not correspond to an actual production situation of the American Enka Plant. The economics of recovery are a very strong function of the amount of zinc used in the preparation of the yarn and the ratio of acid to zinc in the spinning bath. In manufacturing industrial yarns and tire cords, it is common to use 4.5 — 7.5 pounds of zinc per 100 pounds of yarn. This high concentration of zinc makes recovery extremely attractive. Textile yarns use less zinc and although recovery is still the most economic solution, it offers less of a return. These two cases are presented as extremes, with many plants falling between the two values. For the 50 MM Ibs./yr plant considered, the use of two stage precipitation combined with zinc recycle offers a savings of $383.000 over neutralization for a plant producing industrial yarns and a savings of $68,000 for textile yarns. Many plants produce a mix of the two and results would be between these values. The costs associated with the more extensive sludge handling and storage in neutralization and precipitation only aren't included. The cost of installing the complete neutralization and zinc recycle system would Lime Slaking System ------- 50MM/LBS./YR. OF TEXTILE YARN (Acid/Zn SO4 = 5.5) Ibs./Zn 100 Ibs. yarn = 1.5 Total Investment (including engineering) Operating Costs (all costs in $/yr.) I Wages II Electric Power @ 8 mils III Maintenance (3% on Invest./yr.) IV Laboratory V General Plant Overhead VI Raw Materials Lime ($20/ton) NaOH ($40/ton) Polyelectrolyte Total Materials Total Operating Cost Fixed Charges Depreciation @ 15 yrs. Taxes, Insurance Total Fixed Charges Zinc Credit (@ 15.5/lb.) Conventional Lime Neutralization Precipitation $425,000 Two Stage Precipitation With Zinc Recycle $625,000 5,000 10,000 7,000 9,300 12,800 18,800 All on-site, included in wages 8,000 10,000 72,900 72,900 105,700 28,300 2,000 30,300 0 64,800 20,800 5.500 91,100 139,200 41,600 3,000 44,600 [116,000] Net Yearly Cost Total 136,000 67,800 Net Yearly Advantage (Recycle over Conventional Neutralization) 68,200 Pretax Return on Differential Investment $ 68.200 = 34.1% $200,000 ------- 50 MM IBS./ YR. OF INDUSTRIAL YARN (Acid/Zn SO4 - 2.0) Ibs. Zn 100 Ibs. yarn - 6.0 Total Investment {including engineering) Operating Costs (all costs in $/yr.) I Wages J/2, 1 man @ $10,000/yr. II Electric Power @ 8 mils HI Maintenance {3% on Invest/yr.) IV Laboratory V General Plant Overhead VI Raw Materials Lime ($20/ton) NaOH ($40/ton) Polyelectrolyte Total Materials Total Operating Cost Fixed Charges Depreciation @ 15 yrs. Taxes, Insurance Total Fixed Charges Zinc Credit (@ 15.5/Ib.) Conventional Lime Neutralization Precipitation $425,000 Two Stage Precipitation With Zinc Recycle $625,000 5,000 7,000 12,800 All on-site, included in wages 8,000 123,500 123,500 156,300 28,300 2.000 30,300 0 10,000 9,300 18,800 10,000 94,000 76,000 5.500 175,500 223,600 41.600 3.000 44.600 [465.0001 Net Yearly Cost Total 186,000 Net Yearly Advantage (Recycle over Conventional Neutralization) Pretax Return on Differential Investment 383,600 383.600 200,000 192% Pretax Return on Total Zn Pollution $197,000 = 31.5% Control Facility $625,000 [197,000] Credit ------- Sludge Settling and Sludge Dissolving Tanks have negligible economic impact on the rayon industry, running from $.40/100 Ibs. profit to a $.13/100 Ibs. cost compared to selling prices of $30-35/100 Ibs. of staple, $70-80/100 Ibs. of tire yarn, and $100-150/100 Ibs. of filament. Zinc oxide manufacturers face the loss of the bulk of a 50 million Ib./year market as this product is reused rather than wasted. At the present rate of consumption, the known world zinc reserves are estimated to last 23 years. Allowing for an estimated yearly increase in consumption of 2.9%, these reserves would last only 18 years. Thus, the recycling of zinc in the rayon industry is desirable to extend the domestic supply. ------- This technology, with only small modifications to conform with local plant conditions, could have immediate application in any viscose rayon plant with soluble zinc in the plant waste stream. The techniques of initially precipitating the impurities which would prohibit zinc recycle as well as the use of a sludge recirculation process to obtain a dense sludge are excellent examples of good process engineering being applied to a waste problem. In a broader sense this technology could have application to any waste stream containing soluble zinc in a form which can be precipitated by lime or caustic addition. The possibility of recycling the Pump Room ------- precipitated zinc would depend upon the nature of the process considered and may require further work. Examples of other areas with zinc containing wastes are ground-wood pulp, metal plating, zinc refining, and recirculating water systems. To our knowledge, no R&D activity to demonstrate the economics and effectiveness of this technology in these applications is in evidence to date. For further information: Detailed information on this project, including equipment list, is available from the Superintendent of Documents as EPA Report 12090 ESG "Zinc Precipitation and Recovery from Viscose Rayon Wastewater". Or write: Technology Transfer Environmental Protection Agency Washington, D.C. 20460 * U. S. GOVERNMENT PRINTING OFFICE : 1974 O - 534- 948 ------- |