5551
905R85112
                  Method 680.   Determination of Pesticides and PCBs
                            in Water  and Soil/Sediment
                      by Gas Chromatography/Mass Spectrometry
                                  November 1985
                                 Ann Alford-Stevens
                                  Thomas A. Bellar
                               James W. Eichelberger
                                  William L. Budde
                        Physical and Chemical Methods  Branch
                   Environmental Monitoring and Support Laboratory
                         Office of Research and Development
                       U. S. Environmental Protection  Agency
                               Cincinnati, Ohio 45268
                                            US. Environmental  Protection Agency
                                            Region V, Library
                                            230 South  Dearborn  Street
                                            Chicago, HHnois  60604

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U,S. Environmental Protection Agency^

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                                    INDEX

Section
Number            Subject

  1         Scope and Application
  2         Summary of Method
  3         Definitions
  4         Interferences
  5         Safety
  6         Apparatus and Equipment
  7         Reagents and Consumable Materials
  8         Sample Collection, Preservation and Handling
  9         Calibration
 10         Quality Control
 11         Procedures
 12         Calculations
 13         Automated Identification and Measurement
 14         Method Perforamnce              •
 15         References

Tables
  1
  2
  3
  4

  5a

  5b

  6
  7a

  7b

  7c
  8
  9

 10

 11
 12

 13
 14
 15
Recommended GC Operating Conditions
PCS Congeners Used as Calibration Standards
Scheme for Preparation of PCB Stock Solution
Composition and Approximate Concentrations of Calibration Solutions
for Full-Range Data Acquisition
Composition and Approximate Concentrations of Calibration Solutions
for SIM Data Acquisition for PCB Determinations
Composition and Approximate Concentrations of Calibration Solutions
for SIM Data Acquisition for Pesticide Determinations
Criteria for DFTPP Spectrum
Ions for Selected Ion Monitoring to Determine PCBs by Acquiring
Data for Four Sets of £35 Ions Each
Ions for Selected Ion Monitoring to Determine PCBs by Acquiring
Data for Five Sets of £20 Ions Each
Five Ion Sets of £20 Ions Each for Selected Ion Monitoring of PCBs
Retention Time Data For PCB Isomer Groups and Calibration Congeners
Ions for Selected Ion Monitoring Data Acquisition for Pesticide
Analytes, Internal Standards and Surrogate Compounds
Ion Sets for Selected Ion Monitoring of Pesticide Analytes,
Internal Standards, and Surrogate Compounds
Known Relative Abundances of Ions in PCB Molecular Ion Clusters
Quantitation, Confirmation, and Interference Check Ions for
PCB Analytes, Internal Standards, and Surrogate Compounds
Correction for Interference of PCB Containing Two Additional Chlorines
Correction for Interference of PCB Containing One Additional Chlorine
Accuracy and Precision of Automated Measurements of PCBs and Pesticides
in Fortified Water Extracts
Figures

  1

  2
Total ion current profile of PCB calibration congeners and
pesticide Analytes
Diagram indicating approximate relative retention times of PCB
isomer groups and retention time congeners.

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1.  SCOPE AND APPLICATION
   1.1.  This method provides procedures for mass spectrometric determination
         of polychlorinated biphenyls (PCBs) and the listed pesticides in water,
         soil, or sediment.  This method is applicable to samples containing PCBs
         as single congeners or as complex mixtures, such as commercial Arodors.
         PCBs are identified and measured as isomer groups (i.e., by level of
         chlorination).  The existence of 209 possible PCS congeners makes
         impractical the listing of the Chemical Abstracts Service Registry
         Number (CASRN) for each potential method analyte.  Because PCBs are
         identified and measured as isomer groups, the non-specific CASRN for
         each level of  chlorination is used to describe method analytes.
Analyte(s)

Aldrin
BHCs
   alpha isomer
   beta  isomer
   delta isomer
   gamma isomer (lindane)
Chlordane ( technical )
   alpha-chlordane
   gamma-chlordane
   trans-nonachlor
4,4'-DDD
4, 4 '-DDE
4, 4 '-DDT
Dieldrin
Endosulfan I
Endosulfan II
Endosulfan sulfate
Endrin
Endrin aldehyde
Endrin ketone
Heptachlor
Heptachlor epoxide
Methoxychlor
PCBs
   Monochlorobiphenyls
   Dichlorobiphenyls
   Trichlorobiphenyls
   Tetrachlorobiphenyls
   Pentachlorobiphenyls
   Hexachlorobiphenyls
   Heptachlorobiphenyls
   Octachlorobiphenyls
   Nonachlorobiphenyls
   Decachlorobiphenyl
                                     Formula

                                     C12H8C16

                                     CgHgClg
                                     CgHgClg
                                     CgHgClg
                                     C14H10C14
                                     C14H8C14
                                     C14H9C15
                                     C12H8C160
                                     CgHgClgO3S
                                     C8HgClgO3S
                                     CgH4Clg04S
                                     C12H8ClgO
                                     C-]2H8ClgO
                                     C-|2H8C12
                                     C-|2H7Cl3
                                     C12HgCl4
                                     C^2H5Cl5
                                     Ci2H4Clg
   CASRN

  309-00-2

  319-84-6
  319-85-7
  319-86-8
   58-89-9
   57-74-9
 5103-71-9
 5103-74-2
19765-80-5.
   72-54-8
   72-55-9
   50-29-3
   60-57-1
  959-98-8
33213-65-9
 1031-07-8
   72-20-8
 7421-93-4
53494-70-5
   76-44-8
 1024-57-3
   72-43-5
                                     C-|2H2C18
                                     Ci2HClg
27323-
25512-
25323-
26914-
25429-
26601-
28655-
31472-
53742-
 2051-
•18-8
•42-9
68-6
33-0
•29-2
•64-9
•71-2
83-0
•07-7
•24-3

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                                        -2-
   1.2  Detection Limits vary among method analytes and with sample matrix, sample
        preparation procedures, condition of the GC/MS system, type of data
        acquisition, and individual samples.  The calculated method detection
        limit (MDL) for each pesticide in fortified reagent water extracts analyzed
        with full-range data acquisition is presented in Sect. 14.  Analysis of
        calibration solutions indicated that the calculated MDLs do not accurately
        reflect instrumental detection limits.  The following guidance is based on
        numerous analyses of calibration solutions with one instrument over a period
        of approximately six months.  Pesticide analytes other than endosulfans
        I and II can be identified and accurately measured when the injected
        aliquot contains 2 ng of each analyte; the endosulfans require about 4 ng
        each.  With selected-ion-monitoring (SIM) data acquisition, pesticide
        analyte detection limits are lowered by at least a factor of five.  Detection
        limits for individual PCS congeners increase with increasing number of
        chlorine atoms, with the detection limit for decachlorobiphenyl being
        about 5-10 times higher than that of a monochlorobiphenyl.  A monochloro-
        biphenyl can be identified and accurately measured when the injected
        extract aliquot contains 1 ng and full-range data are acquired.  The
        detection limit for total PCBs will depend on the number of individual
        PCS congeners present.  SIM data acquisition procedures reduce the detection
        limit for PCBs by at least a factor of three.

2. SUMMARY OP METHOD

   A 1-L water sample is placed in a separatory funnel and extracted with methylene
   chloride.  Appropriate extraction procedures for soil/sediment samples will be
   added when results are obtained from ongoing experiments. The extract is dried
   and exchanged to hexane during concentration to a final volume of 1 mL or less.
   Sample extract components are separated with capillary column gas chromatography
   (GC) and identified and measured with low resolution, electron ionization mass
   spectrometry (MS).  An interfaced data system (DS) to control data acquisition
   and to store, retrieve, and manipulate mass spectral data is essential.  Either
   full-range or selected-ion-monitoring (SIM) data are acquired, depending on the
   concentration range of concern.  If full-range data are acquired, all method
   analytes can be identified and measured with one GC/MS analysis.  If all pesti-
   cides and PCBs must be determined and if SIM data are necessary to meet required
   detection limits, two GC/MS analyses are necessary, one to detect and measure
   pesticides and one to detect and measure PCBs.

   Two surrogate compounds are added to each sample before sample preparation;
   these compounds are   C12~4»4'~DDT and  3Cg-gamma-BHC.  Two internal standards,
   chrysene-d-) 2 **& phenanthrene-d^ g / are added to each sample extract before GC/MS
   analysis and are used to calibrate MS response.  Each concentration measurement
   is based on an integrated ion abundance of one characteristic ion.  All pesticides
   are identified as individual compounds, and a concentration is calculated by
   relating the MS response of each compound to the MS response of the internal
   standard with GC retention time nearer that of the pesticide analyte.  The
   extent of sample contamination with technical chlordane is indicated by identi-
   fication and measurement of the two most persistent components, gamma-chlordane
   and nonachlor.  (Alpha-chlordane and heptachlor, other major components of
   technical chlordane, may also be present and will be detected and measured
   with this method.)

   PCBs are identified and measured as isomer groups (i.e., by level of chlorination).
   A concentration is measured for each PCB isomer group; total PCB concentration
   in each sample extract is obtained by summing isomer group concentrations.

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                                         -3-


    Nine selected PCS congeners are used as calibration standards/ and one internal
    standard, chrysene-d-^/ is used to calibrate MS response to PCBs, unless sample
    conditions require the use of the second internal standard, phenanthrene-dig.


3.  DEFINITIONS

    3.1  CONCENTRATION CALIBRATION SOLUTION (CAL) — A solution of method analytes
         used to calibrate the mass spectrometer response.

    3.2  CONGENER NUMBER -- Throughout this method, individual PCBs are described
         with the number assigned by Ballschmiter and Zell (2).  (This number is
         also used to describe PCS congeners in catalogs produced by Ultra Scientific,
         Rope, RI.)

    3.3  INTERNAL STANDARD -- A pure compound added to a sample extract in known
         amounts and used to calibrate concentration measurements of other compounds
         that are sample components.  The internal standard must be a compound
         that is not a sample component.

    3.4  LABORATORY DUPLICATES (LD1 and LD2) —Two sample aliquots taken in the
         analytical laboratory are analyzed with identical procedures.  Analysis
         of laboratory duplicates indicates precision associated with laboratory
         procedures but not with sample collection, preservation or storage procedures.

    3.5  LABORATORY PERFORMANCE CHECK SOLUTION (LPC) — A solution of method analytes,
         surrogate compounds, and internal standards used to evaluate the performance
         of the GC/MS/DS with respect to a defined set of method criteria.

    3.6  LABORATORY REAGENT BLANK (LRB) —  An aliquot of reagent water or neutral
         solid reference material that is treated as a sample.  It is exposed to
         all glassware and apparatus, and all method solvents, reagents, internal
         standards, and surrogate compounds are used.  The extract is concentrated
         to the final volume used for samples and is analyzed the same as a sample
         extract.

    3.7  LABORATORY SPIKE DUPLICATE SAMPLE — One aliquot (LSD) of a sample is
         analyzed before fortification with any method analytes.  In the laboratory,
         a known quantity of method analytes (LSA) is added to two independent
         aliquots of the same sample, and final analyte concentrations (LF1 and
         LF2) are measured with the same analytical procedures used to measure LSD.

    3.8  LABORATORY SURROGATE SPIKE

         3.S.1  Measured Value (LS1) — Surrogate compound concentration measured
                with the same procedures  used to measure sample components.

         3.8.2  Theoretical Value (LS2) ~ The concentration of surrogate compound
                added to a sample aliquot before extraction.   This value is determined
                from standard gravimetric and volumetric techniques used during
                sample fortification.

    3.9  METHOD DETECTION LIMIT (MDL) — A statistically determined value (1)
         indicating the minimum concentration of an analyte that can be identified
         and measured in a sample matrix  with 99% confidence that the analyte
         concentration is greater than zero.  This value varies with the precision
         of the replicate measurements used for the calculation.

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   3.10 PERFORMANCE EVALUATION SAMPLE — A sample containing known concentrations
        of method analytes that has been analyzed by multiple laboratories to
        determine statistically the accuracy and precision that can be expected
        when a method is performed by a competent analyst.  Analyte concentrations
        are unknown to the analyst.
                                                             •'
   3.11 QUALITY CONTROL (QC) CHECK SAMPLE —  A sample containing known concentra-
        tions of analytes that is analyzed by a laboratory,to demonstrate that it
        can obtain acceptable identifications and measurements with procedures to
        be used to analyze environmental samples containing the same or similar
        analytes•  Analyte concentrations are known by the analyst.  Preparation
        of the QC check sample by a laboratory other than the laboratory performing
        the analysis is highly desirable.

   3.12 SURROGATE COMPOUND — A compound not expected to be found in the sample
        is added to a sample aliquot before extraction and is measured with the
        same procedures used to measure sample components.  Associated with the
        surrogate compound are two values, laboratory surrogate spike- measured
        value (LS1) and laboratory surrogate spike - theoretical value (LS2).
        The purpose of a surrogate compound is to monitor method performance
        with each sample.

4. INTERFERENCES

   4.1  Interferences may be caused by contaminants in solvents/ reagents, glassware,
        and other sample processing equipment.  Laboratory reagent blanks (LRBs)
        are analyzed routinely to demonstrate that these materials are free of
        interferences under the analytical conditions used for samples.

   4.2  To minimize interferences, glassware (including sample bottles) should
        be meticulously cleaned.  As soon as possible after use, rinse glassware
        with the last solvent used.  Then wash with detergent in hot water and
        rinse with tap water followed by distilled water.  Drain dry and heat in  a
        muffle furnace at 450°C for a few hours.  After cooling, store glassware
        inverted or covered with aluminum foil.  Before using, rinse each piece
        with an appropriate solvent.  Volumetric glassware should not be heated
        in a muffle furnace.

   4.3  For both pesticides and PCBs, interference can be caused by the presence
        of much greater quantities of other sample components that overload the
        capillary column; additional sample extract preparation procedures must
        then be used to eliminate interferences.  Capillary column GC retention
        times and the compound-specific characteristics of mass spectra eliminate
        many interferences that formerly were of concern with pesticide/PCB
        determinations with electron capture detection.  The approach and identi-
        fication criteria used in this method for PCBs eliminate interference by
        most chlorinated compounds other than other PCBs.  With the isomer group
        approach, coeluting PCBs that contain the same number of chlorines are
        identified and measured together.  Therefore, coeluting PCBs are a problem
        only if they contain a different number of chlorine atoms.  This interference
        problem is obviated by rigorous application of the identification criteria
        described in this method.

   4.4  For SIM identification and measurement of pesticides, other chlorinated
        sample components that produce the same quantitation and confirmation
        ions may interfere, but only if retention times are nearly equivalent.

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                                         -5-
5. SAFETY

   5.1  The toxlcity or carcinogenicity of each chemical used in this method
        has not been precisely defined.  Therefore, each should be treated as a
        potential health hazard, and exposure should be reduced to the lowest
        feasible level.  Each laboratory is responsible for safely disposing
        materials and for maintaining awareness of OSHA regulations regarding
        safe handling of the chemicals used in this method.  A reference file of
        material data handling sheets should be made available to all personnel
        involved in analyses.  Additional information on laboratory safety is
        available (3-5).

   5.2  The following method analytes have been classified as known or suspected
        human or mammalian carcinogens:  BHCs, 4,4'-ODD, 4,4'-DDT, and PCBs.
        Primary standards of these compounds should be prepared in a hood.  A
        toxic gas respirator should be worn when the analyst handles solutions
        containing high concentrations of these compounds.
  t

6. APPARATUS AND EQUIPMENT

   6.1  SAMPLING EQUIPMENT

        6.1.1  Water Sample Bottles — Meticulously cleaned (Sect. 4.2) 1-L or
               1-qt amber glass fitted with a. Teflon-lined screw cap.  (Bottles in
               which high purity solvents were received can be used as sample
               bottles without additional cleaning if they have been handled
               carefully to avoid contamination during and after use of original
               contents.)

        6.1.2  Soil/Sediment Sample Bottles — Appropriate containers will be
               specified when appropriate extraction procedures are determined.

   6.2  GLASSWARE

        6.2.1  Separatory Funnel ~ 2-L with Teflon stopcock.

        6.2.2  Drying Column — glass column approximately 400 mm long X 19 mm ID
               with coarse frit filter disc.

        6.2.3  Chromatography Column — glass column approximately 400 mm long
               X 19 mm ID with coarse frit filter disc and Teflon stopcock.

        6.2.4  Concentrator Tube —- 10-mL graduated Kuderna-Danish design
               with ground-glass stopper.

        6.2.5  Evaporative Flask — 500-mL Kuderna-Danish design that is
               attached to concentrator tube with springs.

        6.2.6  Snyder Column — three-ball macro Kuderna-Danish design.

        6.2.7  Vials — 10- to 15-mL amber glass with Teflon-lined screw caps.

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                                      -6-
6.3  COMPUTERIZED GC/MS SYSTEM

    6*3.1  The GC must be capable of temperature programming and be equipped
           with all required accessories, such as syringes, gases, and a capillary
           column.  The GC injection port must be designed for capillary columns.
           Manual splitless injections were used to acquire data used as the basis
           for quality control requirements.  An automatic injector, however, is
           desirable, because it should provide more precise retention times and
           areas.  On-column injection with an uncoated precolumn is encouraged,
           because high mass descrimination and analyte degradation problems
           are minimized with this technique.  With some GCs, however, the
           irreproducibility of the low initial column temperature required for
           on-column injections will cause irreproducible retention times (RTs)
           and relative retention times (RRTs).  That can result in an inability
           to distinguish between two closely-eluting pesticide isomers and may
           cause ion sets to be changed at inappropriate times during SIM data
           acquistion.  Splitting injections are not recommended.

    6.3.2  Either full range or SIM mass spectral data are obtained with electron
           ionization at a nominal electron energy of 70 eV.  To ensure sufficient
           precision of mass spectral data, the required MS scan rate must
           allow acquisition of at least five full-range mass spectra or five
           data points for each monitored ion while a sample component elutes
           from the GC.  The MS must produce a mass spectrum meeting all criteria
           for £20 ng of decafluorotriphenylphosphine (DFTPP) introduced through
           the GC inlet.

    6.3.3  An interfaced data system (OS) is required to acquire, store, reduce,
           and output mass spectral data.  The OS must be capable of searching
           a data file for specific ions and plotting ion abundances versus time
           or spectrum number to produce selected ion current profiles (SICPs)
           and extracted ion current profiles (EICPs).  Also required is the
           capability to obtain chromatographic peak areas between specified
           times or spectrum numbers in SICPs or EICPs.  Total data acquisition
           time per cycle should be £0.5 s and must not exceed 1.5 s.

   6.3.4   SIM Option — For SIM data acquisition, the DS must be equipped with
           software capable of acquiring data for multiple groups of ions,
           and the DS must allow automated and rapid changes of the set of ions
           being monitored.  To acquire all PCS data needed for implementation
           of two currently-available automated interpretation procedures, the
           SIM program must be capable of acquiring data for four groups (or
           mass ranges) each consisting of £35 ions or for five groups of £20
           ions each.  The times spent monitoring ions during sample analyses
           must be the same as the times used when calibration solutions were
           analyzed.

6.4  GC COLUMN —  A 30 m X 0.32 mm ID fused silica capillary column coated with
     a 0.25 urn or thicker film crosslinked phenyl methyl silicone (such as
     Durabond-5 (DB-5), J and W Scientific, Rancho Cordova, CA) or polydiphenyl
     vinyl dimethyl siloxane (such as SE-54, Alltech Associates,  Deerfield,  IL)
     is required.  Operating conditions known to produce acceptable results with
     these columns are shown in Table 1; separation of pesticide analytes and PCS
     calibration congeners with a DB-5 column and those operating conditions is
     shown in Figure 1.  Retention times have been reported (6) for all 209 PCS

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        congeners with am SE-54 column/ which provides the same retention order for
        PCBs and essentially the same separation capabilities as a DB-5 column.

   6.5  MISCELLANEOUS EQUIPMENT

        6.5.1  Volumetric flasks - 2-inL, 5-mL, 10-mL, 25-mL, and 50-mL with
               ground glass stoppers.

        6.5.2  Microsyringes - various standard sizes.

        6.5.3  Boiling Chips — approximately 10/40 mesh.  Heat at 400°C for
               30 min or extract with methylene chloride in a Soxhlet apparatus.

        6.5.4  Water Bath — heated, with concentric ring cover, capable of tempera-
               ture control within ^ 2°C.

        6.5.5  Analytical Balance — capable of accurately weighing to 0.0001 g.


7. REAGENTS AND CONSUMABLE MATERIALS

   7.1  SOLVENTS —  High purity, distilled-in-glass hexane and methylene chloride.
        For precise injections with aplitless injectors and capillary columns, all
        samples and standards should be contained in the same solvent.  Effects of
       . minor variations in solvent composition (i.e., small percentage of another
        solvent remaining in hexane extracts) are minimized with the use of internal
        standards.  (External standard calibration is not acceptable.)

   7.2  SODIUM SULFATE — ACS, granular, anhydrous.  Purify by heating at 400°C
        for 4 h in a shallow tray.

   7.3  SODIUM THIOSULFATE — ACS, granular.

   7.4  TETRABUTYLAMMONIUM SULFITE REAGENT — Dissove 3.39 g of tetrabutyl-
        ammonium hydrogen sulfate in 100 mL distilled water.  To remove impurities
        extract solution three times with 20-mL portions of hexane.  Discard the
        hexane extracts, and add 25 g sodium sulfite to the water solution.  Store
        the resulting solution in an amber bottle with a Teflon-lined screw cap.
        The solution can be stored at room temperature for at least one month.

   7.5. MS PERFORMANCE CHECK SOLUTION — Prepare a 10 ng/uL solution of decafluoro-
        triphenylphosphine (DFTPP) in an appropriate solvent.

   7.6  INTERNAL STANDARDS — Chrysene-d-)2 and phenanthrene-d^o are used as internal
        standards.  They are added to each sample extract just before analysis and are
       'contained in all calibration/performance check solutions.

   7.7  SURROGATE COMPOUNDS — 13C12~4,4'-DDT and 13Cg-gamma-BHC are added to every
        sample before extraction and are included in every calibration/performance
        check solution.

   7.8  PCS CONCENTRATION CALIBRATION CONGENERS — The nine individual PCS congeners
        listed in Table  2 are used as concentration calibration compounds for PCB
        determinations.   One isomer at each level of chlorination is used as the
        concentration calibration standard for all other isomers at that level of
        chlorination, except that decachlorobiphenyl (Clig) is used for both Clg

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                                      -8-
     and C1-|Q isomer groups.  The basis for selection of these calibration
     congeners has been reported (7).

7.9  PCB RETENTION TIME CONGENERS FOR SIM DATA ACQUISITION OPTION — Knowledge
     of the retention times of certain congeners is necessary to determine
     when to acquire data with each ion set.  Two concentration calibration
     congeners also serve as retention time congeners; the first eluting
     Cli-PCB indicates the time when data acquisition must have been initiated
     for ion set #1, and the Cl^Q-PCB indicates when all PCBs have eluted.
     Two or three additional PCB congeners are used to establish times to
     initiate data acquisition with other ion sets (Sect. 9.4).

7.10  PESTICIDE SOLUTIONS

    7.10.1  Pesticide Stock Solutions —  Prepare from pure standard materials.
            Weigh approximately 25.0 mg (with accuracy of 0.1 mg) of each
            surrogate compound and each pure pesticide analyte, except
            Endosulfan I and Endosulfan II.  For those two pesticides, prepare
            a stock solution twice as concentrated as that prepared for other
            pesticide analytes.  Dissolve each compound in hexane and dilute to
            volume in a 10-mL (5-mL for the two Endosulfans) volumetric flask.
            (Concentration of each component = 2.5 mg/mL, except Endosulfans,
            which should be 5 mg/mL.)  Smaller or larger volumes of stock solution
            may be used if desired.  If compound purity is certified at 2.96%,
            the weight can be used without correction to calculate the concen-
            tration of the stock standard solution.  Commercially prepared
            stock standards in hexane can be used at any concentration if they
            are traceable to USEPA-supplied standards.

    7.10.2  Pesticide Primary Dilution Solutions —- A convenient approach to
            solution preparation is to prepare two pesticide primary dilution
            solutions that are twice the concentration of the highest concentration
            calibration solution required.  These solutions can then be diluted
            as necessary to prepare all needed calibration solutions.  One solution
            contains endrin aldehyde and one does not, because the medium level
            calibration solution does not contain endrin aldehyde.  Place 1 mL
            of each pesticide analyte/surrogate compound stock solution in a
            25-mL volumetric flask.  (Total volume for all 22 pesticide analytes
            and 2 surrogate compounds a 24 mL.) Make to volume with hexane and
            mix well.  (Concentration of endosulfan sufate, endosulfan I and
            endosulfan II » 200 ng/uL; concentration of each other component »
            100 ng/uL.)

7.11  PCB SOLUTIONS

    7.11.1  Stock Solutions of PCB Calibration Congeners ~ Prepare a stock
            solution of each of the nine PCB concentration calibration congeners
            at a concentration of 1 ug/uL in hexane.  (If SIM data are to be
            acquired, prepare a 1 ug/uL stock solution of each of the three
            retention time congeners also.)  Place each solution in a clean
            glass vial with a Teflon-lined screw cap and store at 4°C if solutions
            are not to be used right away.  Solutions are stable indefinitely
            if solvent evaporation is prevented.
            CADTION:  Each time a vial containing small volumes of solutions is
            warmed to room temperature and opened, a small volume of solvent in
            the vial headspace evaporates, significantly affecting concentration.

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            Solutions should be stored with the smallest possible volume of
            headspace, and opening vials should be minimized.

    7.11.2  PCS Primary Dilution Standard --  Take aliquots of the stock
            solutions of the nine PCS concentration calibration congeners and
            mix together in the proportions of one part of each solution of the
            Clf (#1), Cl2 (#5), and Cl3 (#29) congeners/ two parts of each solution
            of the C14 (#50), els (#87), and Clg (#154) congeners, three parts
            of each solution-of the 017 (#188) and Clg (#200) congeners, and five
            parts of the C110 (#209) congener solution.  (Note:  The retention
            time congeners described in Sect. 7.9 are not included in the PCB
            primary dilution standard because th'ey are not needed for full-range
            data acquisition.) This will provide a primary dilution standard
            solution of the composition shown in Table 3.  Calculate the concen-
*           tration in ug/uL? use three significant figures.  Place each solution
            in a clean glass vial with a Teflon-lined screw cap and store at
            4°C.  Mark the meniscus on the vial wall to monitor solution volume
            during storage; solutions are stable indefinitely if solvent evapo-
            ration is prevented.

7.12  INTERNAL STANDARD (IS) SOLOTIONS — Two solutions are needed to prepare
      concentration calibration solutions (CALs).

     7.12.1  IS.solution #1 (for full-range CALS) — Weigh 7.5 mg + 0.1 mg
             each of phenanthrene-d-jg and chrysene-d^? dissolve-in hexane and
             dilute to 10 mL in a volumetric flask.  (Concentration of each
             IS = 750 ng/uL)

     7.12.2  IS solution #2 (for SIM CALS) — Take 1 mL of IS solution #1 and
             dilute to 10 mL in a volumetric flask.  (Concentration of each
             IS - 75 ng/uL)

7.13  CALS FOR. FULL-RANGE DATA ACQUISITION —  Five hexane solutions are required.
      The solutions contain constant concentrations of the ISs (chrysene-d^
      and phenanthrene-d^) and varying concentrations of individual pesticide
      analytes, the nine PCB calibration compounds, and the two surrogate compounds
      (  C-2~4»4'-DDT and   Ce-gamma-BHC). (Composition and approximate concen-
      trations are given in Table 4.) Four solutions (high and low concentrations)
      contain both ISs, both surrogate compounds, the nine PCB concentration
      calibration congeners, and each of the single-compound pesticide analytes.
      The fifth solution, the medium level concentration solution, contains all
      the above compounds except endrin aldehyde, which is not present for reasons
      described in Sect.  8.  The lowest concentration solution contains each
      individual pesticide analyte and each PCB calibration congener at a concen-
      tration near but greater than its anticipated detection limit.  (Because
      MS response to PCBs decreases with increasing level of chlorination, PCB
      congener concentrations in CALs increase with level of chlorination.)
      Components of the highest concentration solution (High CAL)  are present at
      a concentration that allow injections of 2-uL aliquots without MS saturation
      or GC column overloading.

      7.13.1  The Full-Range High CAL can be prepared by mixing equal portions
              of the PCB primary dilution solution and the pesticide primary
              dilution solution that contains endrin aldehyde and then adding an
              appropriate volume of IS solution #1. For example,  1 mL of each

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                                        -10-


                 primary dilution solution and 20 uL of IS solution #1 provide the
                 appropriate concentration for High CAL.

         7.13.2  Other full-range CALS are prepared by diluting the primary dilution
                 standard solutions and adding the appropriate amount of IS solution
                 #1.  CADTION:  The pesticide primary dilution standard that does
                 not contain endrin aldehyde must be used for the medium level
                 full-range CAL.

   7.14  CALS FOR SIM DATA ACQUISITION OPTION — Two sets of solutions are needed,
         one set of five solutions for determinations of pesticide analytes, and
         one set of five solutions for PCB determinations.  Appropriate concen-
         trations of SIM CALs are given in Tables 5a and 5b.  Solutions are
         prepared by diluting appropriate primary dilution standards and adding
         an appropriate volume of IS solution #2.
         CAOTION: The Pesticide SIM Medium CAL does not contain endrin aldehyde;
         the PCS SIM CALS must include the three PCB retention time congeners.
         that are used to establish conditions for SIM data acquisition.

   7.15  Prepare a solution of surrogate compounds in a water miscible solvent
         to provide a concentration in the sample/blank extract that is near
         the concentration anticipated for analytes when an aliquot of >20 uL is
         added to the sample before extraction.

   7.15  Calculate the concentration (two significant figures if <100 and three
         significant figures if £100 ng/uL) of each component in each solution.
         Note:  Concentrations presented in tables are only approximate.

   7.16  LABORATORY PERFORMANCE CHECK SOLUTION - For both full-range data acquisition,
         and the SIM data acquisition option, the Medium CAL is used as the laboratory
         performance check solution (LPC) to verify response factors and to demonstrate
         adequate GC resolution and MS performance.


8- SAMPLE COLLECTION, PRESERVATION AND STORAGE

   8.1  WATER SAMPLES

        8.1.1  Samples must be collected in clean (Sect. 4.2) glass containers.
               Note:  When samples are anticipated to contain low concentrations
               of method analytes, a sample larger than 1-L may be needed.  An
               effective sample collection procedure to minimize losses of hydro-
               phobic analytes is to add a portion of extracting solvent to each
               sample container when the sample is collected.  When a 1-gal sample
               is collected, an appropriate solvent volume is approximately 100 mL.
               (The entire sample must be used as one sample aliquot, and blank
               sample/solvent volumes must be adjusted also.)

        8.1.2  Samples must be iced or refrigerated at 4°C from time of collection
               until extraction.  If samples will not be extracted within 72 h after
               collection,  use either sodium hydroxide or sulfuric acid to adjust
               sample pH to within a range of 5 to 9.  Record the volume of acid
               or base used.  If aldrin is to be determined, add sodium thiosulfate
               when residual chlorine is present.  Field test kits are available
               for measurement of residual chlorine.

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                                         -11-


        8.1.3  Samples should be extracted within 7 days after collection and analyzed
               within 40 days after extraction.

   8.2  SOIL/SEDIMENT SAMPLES  —  Appropriate procedures will "be specified when
        results are obtained from ongoing experiments.

9. CALIBRATION

   Demonstration and documentation of acceptable initial calibration is required
   before any samples are analyzed and is required intermittently throughout
   sample analyses as dictated by results of continuing calibration checks.
   After initial calibration is successfully performed, a continuing calibration
   check is required at the beginning and end of each 12-h period during which
   analyses are performed.  The Medium CALs for pesticide determinations do not
   include endrin aldehyde.  This allows the Medium CAL to be used for continuing
   calibration checks, including a check to ensure that endrin decomposition is
   £10%.  During initial calibration a separate Medium CAL containing endrin
   aldehyde and the internal standard is analyzed to determine the response factor
   for endrin aldehyde.  Thereafter, if endrin aldehyde is a component of any
   sample and endrin decomposition is not a problem, the response factor for
   endrin aldehyde is verified by analyzing a calibration solution containing it.

   9.1  DATA ACQUISITION OPTIONS — Either full-range or SIM data acquisition may
        be used.

        9.1.1  Full-range data acquisition is recommended if sample extract
               components are anticipated to be at sufficiently high concentrations.

        9.1.2  SIM data acquisition will provide an increase in sensitivity by
               at least a factor of five for pesticide determinations and by at
               least a factor of three for PCB determinations.

   9.2. INITIAL CALIBRATION

        9.2.1  Calibrate and tune the MS with standards and procedures prescribed
               by the manufacturer with any necessary modifications to meet USEPA
               r equi rements•

        9.2.2  Inject a 1- uL or 2-uL aliquot of the 10 ng/uL DFTPP solution and
               acquire a mass spectrum that includes data for m/z 45-450.  If the
               spectrum does not meet all criteria (Table 6), the MS must be
               hardware tuned to meet all criteria before proceeding with calibration.

        9.2.3  Full-Range Calibration — Inject a 1- or 2-uL aliquot of the Medium
               CAL and acquire data from m/z 45 to 510.  Acquire >5 spectra during
               elution of each GC peak.  Total cycle time should be >0.5 s and <,1*5 s.
               Notes  Either a 1- or 2-uL aliquot should be used consistently for
               CALs and sample/blank extracts.

        9.2.4  SIM Calibration -- Acquire at least five data points for each ion
               during elution of each GC peak.  Total cycle time should be >0.5 s
               and £1«5 s.
               CADTION:   When acquiring SIM data, GC operating conditions must be
               carefully reproduced for each analysis to provide reproducible
               retention times; if not, ions will not be monitored at the appropriate
               times•

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                                     -12-
            9.2.4.1  SIM Calibration for PCB determinations

                 9.2.4.1.1  Two options for SIM data acquisition are provided.
                            Data can be acquired with four sets of 60% of the
                           peak height of methoxychlor, which may partially coelute
                           with the Clg-PCB congener.

                9.2.5.1.2  MS sensitivity — Signal/noise ratio of >5 for
                           m/z 499 of PCB congener #209, C110-PCB.

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                              -13-
        9.2.5.1.3  MS calibration —  Abundance of >40% and <60% of
                   m/z 502 relative to m/z 498 for PCB congener #209.

        9.2.5.1.4  Lack of degradation of endrin.  Examine an extracted
                   ion current profile (EICP) for m/z 67 in the retention
                   time window between 4,4'-DDE and endosulfan sulfate;
                   confirm that the abundance of m/z 67 at the retention
                   time of endrin aldehyde is <10% of the abundance of
                   m/z 67 produced by endrin.

        9.2.5.1.5  Lack of degradation of   C12-4,4'-DDT.  Examine EICPs
                   for m/z 258 and m/z 247 in the retention time window
                   that includes 4,4'-DDD, 4,4'-DDE and 4,4'-DDT; m/z
                   258 would be produced by   C12-4,4'DDE, and m/z 247 by
                     C.j2-4,4'-DDD.  Confirm that the total abundance of
                   both ions is <5% of m/z 247 produced by 13C12-4,4'-DDT.

9.2.5.2  SIM PCS Data

         9.2.5.2.1  GC separation -- Baseline separation of PCB congener
                    #87 from congeners #154 and #77, which may coelute.

         9.2.5.2.2  MS sensitivity — Signal/noise ratio of £5 for m/z
                    499 of PCB congener #209, C110-PCB, and for m/z 241
                    of chrysene-d-|2-

         9.2.5*2.3  MS calibration — Abundance of >70% and <95% of m/z
                    500 relative to m/z 498 for congener #209, C110-PCB-.

9.2.5.3  SIM Pesticide Data

         9.2.5.3.1  GC separation —  Baseline separation of endrin
                    ketone and chrysene-d12; baseline separation of
                    beta-BHC and gamma-BBC;  baseline separation of endrin
                    ketone and chrysene-d12; height of chrysene-d12 peak
                    j>60% of methoxychlor peak height.

         9.2.5.3.2  MS sensitivity — Signal/noise ratio of >5 for m/z
                    241 of chrysene-d-|2.

         9.2.5.3.3  MS calibration —  Abundance of m/z 241 relative
                    to that of m/z 240 produced by chrysene-di2 is >15%
                    and <25%.

         9.2.5.3.4  Lack of degradation of endrin.  Examine an SICP for
                    m/z 67 in the retention time window between 4,4'-DDE
                    and endosulfan sulfate;  confirm that the abundance
                    of m/z 67 at the retention time of endrin aldehyde
                    is <10% that of m/z 67 produced by endrin.

         9.2.5.3.5  Lack of degradation of 13C12-4,4'-DDT.  Examine SICPs
                    for m/z 258 and m/z 247 in the retention time window
                    that includes 4,4'-ODD,  4,4'-DDE, and 4,4'-DDT; m/z
                    258 would be produced by   C12-4,4'-DDE, and m/z 247
                    by 13C12-4,4'-DDD.  Confirm that the total abundance
                    of both ions is <5% of m/z 247 produced by 13C12-4,4'-DDT.

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                                 -14-
9.2.6 Replicate Analyses of CALs -- If all performance criteria are met,
      analyze one 1- or 2-uL aliquot of each of the other four CALs.

9.2.7 Response Factor Calculation

      9.2.7.1 Calculate five response factors (RFs) for each pesticide
              analyte, PCB calibration congener/ and surrogate compound
              relative to both ISs (See Sect. 12.3.2), phenanthrene-dig and
                                    Ais
              where   AJJ  *  integrated ion abundance of quantitation
                             ion for a pesticide, a PCB calibration
                             congener or a surrogate compound,

                             integrated ion abundance of m/z 240, the  '
                             quantitation ion when chrysene-d-j2 is used
                             as the internal standard or m/z 188, the
                             quantitation ion when phenanthrene-d-jg
                             is used as the internal standard,

                             injected quantity of chrysene-d^ or
                             phenanthrene-djQ,

                      Qx  »  injected quantity of pesticide analyte, PCB
                             calibration congener or surrogate compound.

              RF is a unitless number, units used to express quantities
              must be equivalent.  Note:  The Cl2~PCB calibration congener
              may not be resolved from alpha-BHC.  If not, alpha-BHC will
              contribute to the ion abundance measured for C12-PCB.  To
              correct for this contribution, subtract 6.7% of the ion
              abundance of m/z 219 measured for alpha-BHC from the ion
              abundance measured for m/z 222 for
9.2.8  Response Factor Reproducibility --  For each pesticide analyte, PCB
       calibration congener and surrogate compound, calculate the mean RF
       from analyses of each of the five CALS.  When the RSD exceeds 20%,
       analyze additional aliquots of appropriate CALS to obtain an acceptable
       RSD of RFs over the entire concentration range, or take action to
       improve GC/MS performance.

9.2.9  SIM Analyte Retention Time Reproducibility

       9.2.9.1  PCB determinations - Absolute retention times of PCB congeners
                f77 and #104 should not vary by more than ;MO s from one
                analysis to the next.  (Retention time reproducibility is
                not as critical for congeners #1 and #209 as for #77 and
                #104, which are used to determine when ion sets are changed.)

       9.2.9.2  Pesticide determinations — Absolute retention times of
                gamma-chlordane, endosulfan I, and endosulfan II should not
                vary by more than +10 s from one analysis to the next.

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                                     -15-
      9.2.10  Record a spectrum of each CAL component.

9.3. CONTINUING CALIBRATION CHECK

     9.3.1  With the following procedures,  verify initial calibration at the
            beginning and end of each 12-h  period during which analyses are to
            be performed.
                                           *
     9.3.2  Calibrate and tune the MS with  standards and procedures prescribed
            by the manufacturer.

     9.3.3  Analyze a 1-uL or 2-uL aliquot  of the DFTPP solution and ensure
            acceptable MS calibration and performance (Table 6).

     9.3.4  Inject a 1-uL or 2-uL aliquot of the Medium CAL and analyze with the
            same conditions used during Initial Calibration.

     9.3.5  Demonstrate acceptable performance for criteria described in Sect.
            9.2.5.

     9.3.6  Determine that neither the area measured for m/z 240 for chrysene-d-) 2
            nor that for m/z 188 for phenanthrene-d-) g has decreased by more than 30%
            from the area measured in the most recent previous analysis of a
            calibration solution or by more than 50% from the mean area measured
            during initial calibration.

     9.3.7  Response Factor Reproducibility —  For an acceptable Continuing Cali-
            bration Check, the measured RF  for each analyte/surrogate compound
            must be within +20% of the mean value calculated (Sect. 9.2.7)
            during Initial Calibration.  If not, remedial action must be taken;
            recalibration may be necessary.

     9.3.8  SIM Analyte Retention Time Reproducibility  — Demonstrate and
            document acceptable (Sect. 9.2.9) reproducibility of absolute retention
            times of appropriate pesticide  analytes and PCS retention time congeners.

     9.3.9  Remedial actions must be taken  if criteria  are not met; possible
            remedies are:

            9.3.9.1   Check and adjust GC and/or MS operating conditions.

            9.3.9.2   Clean or replace injector liner.

            9.3.9.3   Flush column with solvent according to manufacturers
                      instructions.

            9.3.9.4   Break off a short portion (approximately 0.33 m)  of the
                      column;  check column  performance  by analysis of performance
                      check solution.

            9.3.9.5   Replace GC column;  performance of all initial calibration
                      procedures then required.

            9.3.9.6   Adjust MS for greater or lesser resolution.

            9.3.9.7   Calibrate MS mass scale.

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                                          -16-


                9.3.9.8   Prepare and analyze new concentration calibration/
                          performance check solution.

                9.3.9.9   Prepare new concentration calibration "curve(s).

10.  QUALITY CONTROL

    10.1   LABORATORY REAGENT BLANK (LRB)  — Perform all steps in the analytical
          procedure (Section 11)'using all reagents, standards/ surrogate  compounds,
          equipment, apparatus,  glassware, and solvents that would be used for a
          sample analysis, but omit an aliquot of sample (water or soil/sediment).
          For water samples, substitute 1 L of reagent water.  If available,
          substitute EPA-provided reagent blank solid material for an aliquot of
          soil/sediment.

          10.1.1  An LRB  must contain the same amount of surrogate compounds and
                  internal standards that is added to each sample.  This amount
                  will vary with sample type and with the type of data acquisition
                  (full-range or SIM).

          10.1.2  Analyze an LRB before any samples are extracted and analyzed.

          10.1.3  Before  a new batch of solvents or reagents is used for sample
                  extraction or for'column chroraatographic procedures,  analyze
                 'an LRB.  In addition, analyze a laboratory solvent blank (LSB),
                  which is the same as  -an LRB except that no surrogate compounds or
                  internal standards are  added;  this demonstrates that reagents
                  contain no impurities producing an ion current above the level of
                  background noise for  quantitation ions for those compounds.

          10.1.4  Analyze an LRB along  with each batch of £20 samples.

          10.1.5  An acceptable LRB contains no method analyte at a concentration
                  greater than one half of its MDL and contains no additional  compounds
                  with elution characteristics and mass spectral features  that would
                  interfere with identification and measurement of a method analyte
                  at its  MDL.  If the LRB that was extracted along with a  batch of
                  samples is contaminated, the entire  batch of samples must be
                  reextracted and reanalyzed.

          10.1.6  Corrective action for unacceptable LRB ~ Check solvents,  reagents,
                  apparatus and glassware to locate and eliminate the source of
                  contamination before  any samples are extracted and analyzed.
                  Purify  or discard contaminated reagents and solvents.

    10.2   CALIBRATION —  Included among initial and continuing calibration procedures
          are numerous quality control  checks to ensure that valid data are acquired
          (See Sect. 9).   Continuing calibration checks are accomplished with  results
          from analysis of one solution,  the medium level calibration solution for
          the appropriate type of data  acquisition,  either full-range or SIM.

          10.2.1  If some criteria are  not met for a Continuing Calibration Check
                  after a 12-h period during which samples were analyzed,  those
                  samples must be reanalyzed.  Those criteria are:   GC performance
                  (Sect.  9.2.5),  MS calibration as indicated by DFTPP spectrum, and
                  MS sensitivity as indicated by area  of internal standards.

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                                     -17-
      10.2.2  When other criteria in Sect. 9.2 are not met, results for affected
              analytes must be labeled as suspect to alert the data user of the
              observed problem.  Included among those criteria are: response
              factor check for each analyte or PCS calibration congener, degra-
              dation of DDT and endrin, and retention time reproducibility for
              SIM data acquisition.

10.3  INITIAL DEMONSTRATION OF LABORATORY CAPABILITY FOR WATER ANALYSES
      (Insufficient information is currently available for demonstration for
      soil/ sediment analyses.)

      10.3.1  Until appropriate Quality Control Check Samples are available,
              each laboratory should prepare one or more solutions containing
              each method analyte at a concentration corresponding to that antici-
              pated in samples.  Until accuracy and precision limits have been
              established for PCS isomer groups in appropriate samples, a solution
              containing an Aroclor mixture may be used; compare total measured
              PCB concentration to the total Aroclor concentration.  Report
              Aroclor concentration and measured concentrations of PCS isomer
              groups and total measured PCS concentration.

      10.3.2  Add an appropriate volume of a solution of method analytes
              to each of four 1-L aliquots of reagent water.  Extract and
              analyze according to procedures in Sect. 11.

      10.3.2  For each analyte, calculate measured concentrations, relative
              standard deviation of the four measurements, and method bias
              (Sect. 12.6).  .

tO.4  LABORATORY PERFORMANCE CHECK SOLUTION — In this method, the medium level
      concentration calibration solution also serves the purpose of a laboratory
      performance check solution.

10.5  LABORATORY SURROGATE SPIKE

      10.5.1  Measure the concentration of both surrogate compounds in
              every sample and blank.

      10.5.2  Until performance based acceptance limits have been established for
              surrogate compounds, the following guidelines are provided:
              measured bias with LRB =• -30% to +10%; measured bias with
              water or soil/sediment extract » -50% to +25%.

10.6  QUALITY CONTROL CHECK SAMPLE — Not yet available; anticipate need for
      analysis of one for each batch of £20 samples.  If full-range data are
      acquired,  both pesticide and PCS analytes can be determined with one
      analysis.   If SIM data are acquired, one extraction and two GC/MS analyses
      will be needed to determine both PCBs and pesticides.

10.7  LABORATORY SPIKED DUPLICATE SAMPLE — Select one sample from each batch of
      £20 samples of similar type and fortify (spike) two aliquots of that sample
      with a solution containing appropriate concentrations of pesticide analytes
      and at least one Aroclor mixture.  After addition of surrogate compounds,
      extract and analyze (Sect.  11) these two fortified aliquots along with
      an additional unfortified sample aliquot.  Relative difference (RD) of
      duplicate results for surrogate compound concentrations should be £40%.

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                                          -18-
          (RD - [C-! - C2 / 0.5 (CT + C2)]  100 )  Calculate bias (Sect. 12.6) for
          each analyte and surrogate compound.  Insufficient data are currently
          available to provide guidance for acceptable bias and RD of -measured
          analyte concentrations.

    10.8  PERFORMANCE EVALUATION SAMPLE — Not yet available; to be analyzed
          periodically when available.

11. PROCEDURES

    11.1  SAMPLE EXTRACTION

          11.1.1  Water Samples

                  11.1.1.1  Mark the water meniscus on the side of the sample bottle
                            for later determination of sample volume.  Pour entire
                            sample into a 2-L separatory funnel.  (If a sample larger
                            than 1-L or 1-
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                                       -19-
                        and the water temperature as required to complete the
                        concentration in 15-20 min.   At the proper rate of
                        distillation the balls of the column will actively chatter
                        but the chambers will not flood with condensed solvent.
                        When the apparent volume of  liquid reaches 1 mL, remove
                        the K-D apparatus from the water bath and allow it to
                        drain and cool for at least  10 min.

              11.1.1.6  Momentarily remove the Snyder column, add 50 mL of hexane
                        and a new boiling chip, and  reattach the Snyder column.
                        Increase the temperature of  the hot water bath to about
                        80 °C.  Concentrate the extract to approximately 10 mL
                        as in Sect. 11.1.1.5, except use hexane to prewet the
                        column.  Elapsed time of concentration should be 5-10
                        min.

              11.1.1.7  Remove the Snyder column and rinse the flask and its
                        lower joint into the concentrator tube with 1-2 mL of
                        hexane.  'A 5-mL syringe is recommended for this operation.
                        Stopper the concentrator tube and store refrigerated if
                        further processing will not  be performed within a few
                        hours.  If the extract will  be stored longer than two
                        days, transfer it to a Teflon-sealed screw-cap vial.

              11.1.1.8  Determine the original sample volume by refilling the
                        sample bottle to the mark and transferring the liquid
                        to a 1000-mL graduated cylinder.  Record the sample
                        volume to the nearest 5 mL.

      11.1.2  Soil/Sediment Samples — Appropriate extraction procedures to be
              specified when results of ongoing experiments are obtained.

11.2  Sulfur Removal — Elemental sulfur can be removed by the procedure described
      below.  (Sulfur is not expected to be a problem in water sample extracts but
      sulfur removal is recommended for soil/sediment sample extracts.)

      11.2.1  Transfer the extract to a 50-mL clear  glass bottle or vial with a
              Teflon-lined screw cap.  Rinse the extract container wtih 1.0 mL of
              hexane, adding the rinse to the 50-mL  bottle.

      11.2.2  Add 1  mL of Tetrabutylammonium-sulfite reagent and 1 mL 2-propanol,
              cap the bottle, and shake for at least 1 min.  If the sample is
              colorless or if the initial color is unchanged, and if clear crystals
              (precipitated sodium sulfite)  are observed, sufficient sodium
              sulfite is present.  If the precipitated sodium sulfite disappears,
              add more crystalline sodium sulfite in approximately 100-mg portions
              until  a solid residue remains after repeated shaking.

      11.2.3  Add 5  mL of distilled water and shake  for at least 1 min.   Allow
              the sample to stand for 5-10 min and remove the hexane layer (top)
              for analysis.  Dry the extract by passing it through a 10-cm
              column containing hexane-washed sodium sulfate.  Rinse the sodium
              sulfate with about 30 mL of hexane and add this hexane to the
              extract.  Concentrate the extract to approximately 10 mL with a
              K-D apparatus.   Store in a refrigerator if GC/MS analysis is not to
              be  performed within a few hours.

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                                         -20-


  11.3 GC/MS ANALYSIS

      11.3.1   Remove the sample extract or blank from storage and allow it to warm
               to ambient laboratory temperature if necessary.  With a stream of
               dry, filtered nitrogen, reduce the extract/blank volume to the
               appropriate volume, depending on anticipated analyte concentrations.
               Add an appropriate volume of the appropriate internal standard stock
               solution.

              11.3.1.1  Internal standard concentration for full-range
                        data acquisition =« 7.5 ng/uL of extract.

              11.3*1.2  Internal standard concentration for SIM data
                        acquisition - 0.75 ng/uL of extract.

     11.3.2   Inject a 1-uL or 2-uL aliquot of the blank/sample extract into the GC
              operated under conditions used to produce acceptable results during
              calibration.'

     11.3.3   Acquire mass spectral data with either full-range data acquisition
              conditions or SIM conditions, as appropriate.  Use the same data
              acquisition time and MS operating conditions previously used to
              determine response factors.

     11.3.4   Examine data for saturated ions in mass spectra of target compounds,
              if saturation occurred, dilute and reanalyze the extract after the
              quantity of the internal standards is adjusted appropriately.

     11.3.5   For each internal standard, determine that the area measured in the
              sample extract has not decreased by >30% from the area measured
              during the most recent previous analysis of a calibration solution
              or by >50% from the mean area measured during initial calibration.
              If either criterion is not met, remedial action must be taken to
              improve sensitivity, and the sample extract must 'be reanalyzed.


11.4  IDENTIFICATION PROCEDURES

      11.4.1  Using the ions shown in Tables 7a-7c for PCBs or Table 9 for
              pesticides, examine ion current profiles (ICPs)  to locate internal
              standards, surrogate compounds, pesticide analytes, and PCBs for each
              isomer group.   Use the RRT data in Table 9 as guidelines for location
              of pesticide analytes and the RRT window data in Table 3 as guidelines
              for location of PCS isomers.  (A reverse search software routine
              can be used to locate compounds of concern.)

      11.4.2  Full-Range Data

             11.4.2.1  Examine.each pesticide and PCS candidate spectrum after
                       background correction routines have been applied.   Compare
                       the candidate spectrum with the appropriate standard spectrum
                       measured during calibration.  Verify the absence of any ions
                       with mass greater than the highest mass possible for the
                       compound of concern.  (Ions in PCS M+ ion clusters are shown
                       in Table 12.)

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                                   -21-
       11.4.2.2  Obtain integrated abundance areas for quantitation and
                 confirmation ions.

11.4.3  SIM Data — Obtain appropriate selected ion current profiles (SICPs)
        for IS quantitation and confirmation ions, for each ion monitored
        to detect pesticides and the surrogate compounds (Table 9), and for
        the quantitation and confirmation ions for each PCB isomer group.

11.4.4  PCB Analytes

      11.4.4.1  For all PCB candidates, confirm the presence of an (M-?!))*
                ion cluster by examining ICPs or spectra for at least one of
                the most intense ions in the appropriate ion cluster.

      11.4.4.2  For Cl^-Cl7 isomer groups, examine ICPs or spectra for intense
                (M+70)* ions that would indicate a coeluting PCB containing two
                additional chlorines.  (GC retention time data show that
                this is not a potential problem for other PCB isomer groups;
                see Figure 2.) If this interference occurs, a correction can
                be made.  Obtain and record the area for the appropriate ion
                (Table 12) for the candidate PCB isomer group.  Use the
                information in Table 13 to correct the measured abundance of
                M .  For example, if a Cl^-PCB and a Clg-PCB candidate coelute,
                the Cly-PCB will contribute to the ion measured for m/z 326 and
                m/z 324, the quantitation and confirmation ions, respectively,
                for a C15-PCB.  Obtain and record the area for m/z 322 (the
                lowest mass ion in the (M+-70)  ion cluster of a Cl^-PCB
                fragment produced by a Cl7-PCB)t.  To determine the m/z 326 and
                m/z 324 areas produced by the Cls PCB, calculate the C17-PCB
                contribution to each and subtract it from the measured area.
                In this example, 164% of the area measured for m/z 322 should
                be subtracted from the area measured for m/z 324,  and 108% of
                the m/z 322 area should be subtracted from the area measured
                for m/z 326 (Table 13).

      11.4.4.3  For Cl2-Clg-PCB  candidates, examine ICPs or spectra for
                intense (M+35)+ ions that would indicate a coeluting PCB
                containing one additional chlorine.  This coelution causes
                interferences because of the natural abundance of  13C.
                (This interference will be small and can be neglected except
                when measuring the area of a small amount of a PCB coeluting
                with a large amount of another PCB containing one  more
                chlorine.) To correct for this interference, obtain and
                record the area for the appropriate ion (Table 14)  from
                the (M-1)+ ion cluster, and subtract 13.5% of the  area
                measured for the CM-1)"*" ion from the measured area of the
                quantitation ion.  For example, for Cls-PCB candidates,
                obtain and record the area for m/z 325;  subtract 13.5% of
                that area from the measured area of m/z 326.

11.4.5  All Analytes — Use ICP data to calculate the ratio of the measured
        peak areas of the quantitation ion and confirmation ion(s), and
        compare to the acceptable ratio (Table 9 for pesticides and Table 12
        for PCBs).  If acceptable ratios are not obtained, a coeluting or
        partially coeluting compound may be interfering.  Examination of data
        from several scans may provide information that will allow application
        of additional background corrections to improve the ion ratio.

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                                        -22-


11.5.  IDENTIFICATION CRITERIA

      11.5.1   Internal  Standards

            11.5.1.1 Chrysene-d12 — the abundance of m/z 241  relative  to m/z
                     240 must be XI5% and £25%,  and these ions must maximize
                     simultaneously.   The area measured for m/z 240 must  be
                     within 30%  of the area  measured during the most  recent
                     calibration.

            11.5.1.2 Phenanthrene-d-jQ ~ the abundance  of m/z  189  relative to m/z
                     188 must be _>10% and £22%,  and these ions must maximize
                     simultaneously.   The area measured for m/z 188 must  be
                     within 30%  of the area  measured during the most  recent
                     acceptable  calibration.

            11.5.1.3 Retention time must be  within £10  s of that observed
                     during the  most recent  acceptable  calibration.

     11.5.2   Full-Range Data for  Pesticide Analytes and  Surrogate Compounds

            11.5.2.1 Retention time  of the sample  component must be within t s
                     of the time observed for that same compound when a calibration
                     solution was analyzed.   Calculate  the value of t with the
                     equation, t = (RT)V^»  where  RT =  observed retention time
                     (in seconds) of  the compound  during the last  previous acceptable
                     calibration.      '                              .

            11.5.2.2 All ions with relative  abundance >10% in  the  mass  spectrum
                     must be present  in the  mass spectrum of the candidate sample
                     component;  a molecular  ion  with relative  abundance >2% in
                     the standard spectrum must  be present in  the  candidate
                     spectrum.

            11.5.2.3 The ion that was the most abundant (base  peak) in  the standard
                     spectrum must also be the base peak in the candidate spectrum.

            11.5.2.4 For all ions with relative  abundance >20%  in  the standard
                     spectrum, the relative  abundance in the candidate  spectrum
                     must not vary by more than  £15% in percentage units  (i.e.,
                     if 50% in standard,  must be £35% and £65%).

            11.5.2.5 Ions with relative abundance  >10%  in the  candidate spectrum
                     but not present  in the  standard spectrum  must be considered
                     and accounted for by the analyst.   When data  processing
                     software is used to obtain  candidate spectra, both processed
                     and unprocessed  spectra must  be evaluated.

     11.5.3   SIM Data for Pesticide Analytes  and  Surrogate Compounds

            11.5.3.1 Absolute retention time of  each surrogate  compound and
                     pesticide candidate must be within 10 s of  that  measured
                     during the  last  previous acceptable calibration.

            11.5.3.2 All ions monitored for  each compound (Table 9) must  be
                     present and must maximize simultaneously.

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                                          -23-
              11.5.3.3  In a spectrum averaged across a GC peak and with background
                        correction, if necessary/ the most abundant ion must correlate
                        with Table 9 data.

              11.5.3.4  Observed relative abundances of the monitored ions must
                        meet the following criteria:
                          Aldrin — m/z 263 =- >20% and m/z 265 = >13%
                          BBC (each isomer) — m/z 183 » 70-95% of m/z 181
                          13C6-gamma-BHC — m/z 189 = 75-90% of m/z 187
                          Chlordane (alpha and gamma) — m/z 375 » 75-99%
                          4,4'-DDE — m/z 248 = 45-85%
                          4,4'-ODD and 4,4'-DDT — m/z 237 - 45-85%
                          13C12-4,4'-DDT — m/z 249 - 45-85%
                          Dieldrin —  m/z 263 = >3% and m/z 108 » >8%
                          Endosulfan I and II ~ m/z 339 = >30% and m/z 341 =• >20%
                          Endosulfan sulfate — m/z 274 = 60-95%
                         ' Endrin — m/z 263 = >50%
                          Endrin aldehyde —• m/z 345 = _>m
                          Endrin ketone — m/z 317 = 2.30%
                          Heptachlor — m/z 272 » >30% and m/z 274 = >20%
                          Heptachlor epoxide ~ m/z 353 = >60%
                          Methoxychlor — m/z 228 «  3-30%
                          Nonachlor — m/z 407 = 65-95%

      11.5.4  Full-Range and SIM Data for PCBs

             11.5.4.1   Absolute retention times of surrogate compounds must be
                        within vt 0 s of that measured during the last previous
                        continuing calibration check.

             11.5.4.2   Quantitation and confirmation ions for each PCB isomer group
                        must maximize within ^1 scan of each other.

             11.5.4.3   The integrated ion current for each quantitation and confir-
                        mation ion must be at least three times background noise and
                        must not have saturated the detector.

             11.5.4.4   For each PCB isomer group candidate, the ratio of the quanti-
                        tation ion area to the confirmation ion area must be within
                        limits shown in Table 12; at least one ion in the (M-70)+
                        ion cluster must be present.


12. CaLCOIATIONS

    12.1  From appropriate ICPs of quantitation ions, obtain and record the spectrum
          number of the chromatographic peak apex and the area of the entire
          chromatographic peak.

    12.2  For PCBs, sum the areas for all isomers identified at each level of
          chlorination (e.g., sum all quantitation ion areas for Cl^PCBs).

    12.3  Calculate the concentration of each surrogate compound, pesticide
          candidate, and PCB isomer group using the formula:

-------
                                     -24-


                  Cx - /(Ais '«*•»)

          where  Cx  =  concentration (micrograms per kilogram or micrograms
                        per liter) of surrogate compound, individual pesticide
                        or a PCB isomer group,

                 AX  =  the area of the quantitation ion for each pesticide
                        analyte/surrogate compound or the sum of quantitation
                        ion areas for all PCB isomers at a particular level
                        of chlorination,

                        the area of the internal standard quantitation ion,
                        m/z 240 for chrysene-d^ °r m/z 188 for phenanthrene-d^ g,

                        quantity (micrograms) of internal standard added to
                        the extract before GC/MS analysis,

                 RF  =  calculated response factor for the surrogate compound,
                        the pesticide standard, or the PCB calibration compound
                        for the isomer group (level of chlorination), and

                 W   =•  weight (kilograms) of sample extracted.  If a liquid
                        sample was extracted, W becomes V, the volume (liters)
                        of water extracted, and concentration units become
                        micrograms per liter.

      12.3.1  Use the grand mean RF calculated during Initial Calibration.
              CAOTION:  For PCB analyses with automated data interpretation
              a linear fit algorithm will produce erroneous concentration
              data.

      12.3.2  For pesticides eluting before heptachlor epoxide, use the RF
              relative to phenanthrene-d-jg; for heptachlor expoxide and later
              eluting pesticides, use the RF relative to chrysene-d-)2'  For
              PCBs, use the RF relative to chrysene-d^ unless an interference
              makes the use of the RF relative to phenanthrene-d-jg necessary.

12.4  Estimation of the Concentration of Technical Chlordane.  Technical chlordane
      is a mixture that contains alpha-chlordane (about 13% by weight), gamma-
      chlordane (about 18% by weight), heptachlor (about 8%), chlordene (three
      isomers; about 19%) and a variety of side reaction products (including
      nonachlor isomers)  from chlorination of chlordene.  Alpha-chlordane is
      readily converted to gamma-chlordane, which is persistent in environmental
      samples.  Another persistent component is trans-nonachlor.  The presence
      of gamma-chlordane and trans-nonachlor, with or without alpha-chlordane
      and heptachlor) indicates that technical chlordane was once present in
      the sample.  Therefore the sum of measured concentrations of alpha-chlordane
      and gamma-chlordane can be used to estimate the original concentration of
      technical chlordane.

               ctc  =  
-------
                                         -25-
   12.5  Report calculated values to two significant figures.

   12.6  When samples of known composition or fortified samples are analyzed,
         calculate the percent method bias using the equation:"

                     B - 100 (Cs - Ct)/ Ct

             where  Cg  ™  measured concentration (in micrograms per kilogram
                           or micrograms per liter),
                    Ct  »  theoretical concentration (i.e., the
                           quantity added to the sample aliquot/weight or volume
                           of sample aliquot)•

             Note:  The bias value retains a positive or negative sign.
  *

13.  AUTOMATED IDENTIFICATION AND MEASUREMENT

    Special software can be used for automated identification and measurement of
    PCBs (8) and pesticides.  Unprocessed GC/MS data are handled without human
    interaction with the software operating on the dedicated computer.  A concen-
    tration for each pesticide and each PCB isomer group is calculated automatically.
    Contact EMSL-Cincinnati for further information.
14. METHOD PERFORMANCE

    To obtain single laboratory accuracy and precision data for method analytes,
    replicate 1-L aliquots of reagent water and river water fortified with known
    amounts of analytes were extracted and analyzed.  Automated procedures were used
    to identify and measure method analytes in 2-uL aliquots of 1-mL extracts.
    Because a sufficient quantity of individual PCB congeners was not available,
    Aroclor mixtures were used to fortify water samples.   This is not desirable,
    because individual PCBs in Aroclors vary in concentration.  As Aroclor concen-
    trations decrease in a sample extract, an increasing number of components
    will fall below the detection limit and will not be identified and measured.
    In addition, insufficient data are available about Aroclor composition to assess
    accuracy of isomer group measurements or to assess MDLs for PCBs when Aroclors
    are used to fortify samples.

    14.1 Medium Level Reagent Water Extracts —• Five aliquots of reagent water
         fortified with each individual pesticide at a concentration of 10 ug/L and
         Aroclors 1221, 1242, 1254, and 1268 at concentrations of 5 ug/L, 50 ug/L,
         50"ug/L and 25 ug/L, respectively, were extracted and analyzed.  Method
         bias for individual pesticides ranged from -10%  to +18% with a mean method
         bias of +2% for all 21 pesticides (Table 15).  For individual pesticides,
         RSDs of measured concentration ranged from 0.61% for endrin ketone to
         9.8% for endrin aldehyde.  No true values are known for concentrations of
         PCB isomer groups in Aroclors, but the mean measured total PCB concentration
         was 110 ug/L (RSD 2.9%), which indicated a method bias of -15%.  For
         individual isomer groups, RSDs of mean measured concentrations ranged
         from 3.9% to 16%.

    14.2 Low Level Reagent Water Extract -- Reagent water was fortified with each
         pesticide at a concentration of 3 ug/L and a total PCB concentration of
         27 ug/L (Aroclors 1221, 1 ug/L; 1242,  10 ug/L;  1254, 10 ug/L; and 1268,

-------
                                         -26-


         6 ug/L).  When seven replicate extracts were analyzed, method bias for
         individual pesticides ranged from -17% to +20% with a mean method bias of
         -2% (Table 15).  An MDL was calculated for each pesticide using the equation
         relating the standard deviation of the seven replicate measurement and
         Student's t value for a one-tailed test at the 99% confidence level with n-1
         degrees of freedom (1).  With this calculation, MDL is defined as the
         minimum concentration that can be measured and reported with 99% confidence
         that the value is above zero.  The excellent precision achieved with these
         measurements resulted in unrealistically low MOLs ranging from 0.2 to 0.8
         ug/L for pesticide analytes (Table 15).  A PCS MDL is an individual congener
         characteristic and cannot be determined with samples fortif-ied with Aroclor
         mixtures.  Estimates of MDLs for individual components of PCS isomer groups
         were obtained by proportioning the total quantity measured for each isomer
         group among individual measured isomers.  The estimated MDL values for
         individual PCBs also were unrealistically low (0.01-0.1 ug/L) because of
         the excellent precision of measurements.  A more realistic statement of
         detection limits for pesticides and PCBs can be found in Sect. 1.2.

   14.3   River Water Extracts ~ Five aliquots of river water fortified with
          each pesticide at a concentration of 5 ug/L and total PCB concentration
          of 70 ug/L (Aroclors 1221, 2 ug/L; 1242, 30 ug/L; 1254, 30 ug/L; and
          1268, 8 ug/L) were extracted and analyzed.  Method bias for individual
          pesticides ranged from -30% to +8% with a mean of -8% (Table 15).  The
          excellent precision of measured pesticide PCS isomer group concentrations
          was indicated by RSDs ranging from 1.6% to 7.5%.  The mean measured total
          PCS concentration of 51 ug/L (RSD 2.5%) indicated a method bias of -27%.


15.  REFERENCES

     1.  Glaser, J. A., D. L. Foerst, G. D. McKee, S. A. Quave, and W. L. Budde,
         "Trace Analyses for Wastewaters", Environ. Sci. Technol. 15, 1426, 1981.

     2.  Ballschmiter, K. and M. Zell, Fresenius Z. Anal. Ghent., 302, 20, 1980.

     3.  "Carcinogens — Working with Carcinogens", Department of Health Service,
         Center for Disease Control, National Institute for Occupational Safety
         and Health, Publication No. 77-206, August 1977.

     4.  "OSHA Safety and Health Standards, General Industry", 29 CFR 1910,
         Occupational Safety and Health Administration, OSHA 2206, Revised
         January 1976.

     5.  "Safety in Academic Chemistry Laboratories",  American Chemical Society
         Publication, Committee on Chemical Safety, 3rd Edition, 1979.

     6.  Mullin, M. D., C. Pochini, S. McCrindle, M. Romkes, S. H. Safe, and
         L. M. Safe, "High Resolution PCS Analysis:  Synthesis and Chromatographic
         Properties of All 209 PCS Congeners", Environ. Sci. Technol. 18, 466,  1984.

     7.  Gebhart, J. E., Hayes, T. L., Alford-Stevens, A. L., and W. L. Budde,
         "Mass Spectrometric Determination of Polychlorinated Biphenyls as
         Isomer Groups", Anal. Ghent. 57, 2458, 1985.

-------
                                     -27-
  8.  Slivon, L. E., J. E. Gebhart, T. L. Hayes, A. L. Alford-Stevens/
      W. L.-Budde, "Automated Procedures for Mass Spectrometric Determi-
      nation of Polychlorinated Biphenyls as Isomer Groups", Anal. Chem.
      £7, 2464, 1985.

  9. . Rote, .&• W. and W. J. Morris, "Use of Isotopic Abundance Ratios in
      Identification of Polychlorinated Biphenyls by Mass Spectrometry",
      J. Assoc. Offic. Anal." Chem. 56(1), 188, 1973.
            Table 1.  Recommended GC Operating Conditions
Column Type:

Film Thickness:

Column Dimensions:

Helium Linear Velocity:


Temperature Program for Splitless Injection:

o Full-range data acquisition for PCBs
  and pesticides
  (Analysis time = approx. 50 min)
o SIM data acquisition for PCBs
  (Analysis time = approx. 25 min)
o SIM data acquisition for pesticides
  (Analysis time - approx. 30 min)
   SE-54 or DB-5

      0.25 urn

   30 m X 0.32 mm

    28-29 cm/sec
     at 250°C
Inject at 80°C and hold 1 min;
increase at 30°/min to 160°C and
hold 1 min? increase at 3°/min to
310«C.
            or

Inject at 80°C and hold 1 min; heat
rapidly to 160°C and hold 1 min;
increase at 3°/min to 310°C.

Inject at 45°C and hold 1 min; increase
at 20°/min to 150«C and hold 1 min;
increase at 10°/min to 310°C.

Inject at 80 °C and hold 1 min; increase
at 30°/min to 160°C and hold 1 min;
increase at 3°/min to 250°C; hold
past elution time of methoxychlor.

-------
                                     -28-
     Table 2.  PCS Congeners Used as Calibration Standards
                         Congener           Chlorine
  PCS Isomer Group       Number3          Substitution
Concentration Calibration Standard

  Monochlorobiphenyl         1        2

  Dichlorobiphenyl           5        2,3

  Trichlorobiphenyl         29        2,4,5

  Tetrachlorobiphenyl       50        2,2',4,6

 . Pentachlorobiphenyl       87        2,2',3,4,5'

  Hexachlorobiphenyl       154        2,2',4,4',5,6'

  Hepta-chlorobiphenyl      188        2,2',3,4',5,6,6'

  Octachlorobiphenyl       200        2,2'',3,3',4,5',6,6'

  Nonachlorobiphenyl*5       -         -—

  Decachlorobiphenyl       209        2,2',3,3',4,4',5,5',6,6'


Retention Time Calibration Standards

  Tetrachlorobiphenyl       77        3,3',4,4'

  Pentachlorobiphenyl      104        2,2',4,6,6'

  Nonachlorobiphenyl       208        2,2',3,3',4,5,5',6,7'




a Numbered according to the system of Ballschmiter and Zell (2).

b Decachlorobiphenyl is used as the calibration congener for both nona-
  and decachlorobiphenyl isomer groups.

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                             -29-
Table 3.  Scheme for Preparation of PCB Primary Dilution Standard
PCB
Cong.
#1
#5
#29
#50
#87
#154
#188
#200
#209
Isomer
Group
Cl,
C12
C13
C14
C15
<*6
C17
Clg
d10
Stock Sol.
Cone.
mg/mL
1.0
1.0
1.0
1.0
1.0
1.0
1.0
1.0
1.0
Proportion
for Primary
Oil. Sol.
1 part
1 part
1 part
2 parts
2 parts
2 parts
3 parts
3 parts
5 parts
Primary Oil.
Std. Cone.
ng/uL
50
50
50
100
100
100
150
150
250
                           Total  20 parts

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                                     -30-
Table 4.  Composition and Approximate Concentrations of Calibration Solutions
           for Pull-Range Data Acquisition
Analyte/Int. Std./
Surrogate Compound
CAL 1
                                     Concentration (ng/uL)
CAL 2   CAL 3   CAL 4   CAL 5
PCS Cal. Congeners
 Cl! (#1)
 C12 (#5)
 C13 (#29)
 C14 (#50)
 C15 (#87)
 C16 (#154)
 C17 (#188)
 C18 (#200)
 C110 (#209)

Pesticides
 Aldrin
 BHC, each isomer
 Chlordane, each isomer
 4, 4 '-ODD
 4, 4 '-DDE
 4, 4 '-DDT
 Dieldrin
 Endosulfan I
 Endosulfan II
 Endosulfan sulfate
 Endrin
 Endrin aldehyde
 Endrin ketone
 Heptachlor
 Heptachlor epoxide
 Methoxychlor
 Nonachlor, each isomer

Internal Standards
 Phenanthrene-d-j Q

Surrogate Compounds
 13C6-gamma BHC
0.5
0.5
0.5
1
1
1
1.5
1.5
2.5
2.5
2.5
2.5
5
5
5
7.5
7.5
12.5
5
5
5
10
10
10
15
15
25
10
10
10
20
20
20
30
30
50
25
25
25
50
50
50
75
75
125
1
1
1
1
1
1
1
2
2
2
1
1
1
1
1
1
1
5
5
5.
5
5-.
5
5
10
10
10
5
5
5
5
5
5
5
10
10
10
10
10
10
10
20
20
20
10
—
10
10
10
10
10
20
20
20
20
20
20
20
40
40
40
20,
20
20
20
20
20
20
50
50
50
50
50
50
50
100
100
100
50
50
50
50
50
50
50
 13
   C12-4,4'-DDT
  7.5
  7.5
  7.5
  7.5
           5
           5
7.5
7.5
         10
         10
7.5
7.5
       20
       20
7.5
7.5
       50
       50

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                                     -31-
Table 5a.  Composition and Approximate Concentrations of Calibration Solutions
           for SIM Data Acquisition for PCS Determinations
                                      Concentration (ng/uL)
Compound
Cal. Congeners
C1-, (#1)
C12 (#5)
C13 (#29)
C14 (#50)
C15 (#87)
C16 (#154)
C17 (#188)
Clg (#200)
C110 (#209)
RT Congeners
C14 (#77)
C15 (#104)
C19 (#208)
Internal Standards
Chrysene-di 2
Phenanthr ene-df g
CAL 1 CAL 2

0.1 0.5
0.1 0.5
0.1 0.5
0.2 1.0
0.2 1
0.2 1
0.3 1.5
0.3 1.5
0.5 2.5

0.2 1
0.2 1
0.4 2

0.75 0.75
0.75 0.75
CAL 3

1
1
1
2
2
2
3
3
5

2
2
4

0.75
0.75
CAL 4

2
2
2
4
4
4
6
6
10

4
4
8

0.75
0.75
CAL 5

5
5
' 5
10
10
10
15
15
25

10
10
20

0.75
0.75
Surrogate Compounds

  ^Cg-gamma-BHC
 13
   C12-4,4'-DDT
0.2

0.2
2

2
4

4
10

10

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                                     -32-
Table 5b.  Composition and Approximate Concentrations of Calibration Solutions
           for SIM Data Acquisition for Pesticide Determinations
                                           Concentration (ng/uL)
Analyte/Internal Std/
Surrogate Compound
Pesticide Analytes
Aldrin
BHC, each isomer
Chlordane, each isomer
4, 4 '-ODD
4, 4 '-DDE
4,4'-DDT
Dieldrin
Endosulfan I
Endosulfan II
Endosulfan sulfate
Endrin
Endrin aldehyde
Endrin ketone
Heptachlor
Heptachlor epoxide
Methoxychlor
Nonachlor, each isomer
Internal Standards
Chrysene-d-|2
Phenanthrene-di g
Surrogate Compounds
Cg-gamma-BHC
13C-,-4,4'-DOT
CAL 1

0.2
0.2
0.2
0.2
0.2
0.2
0.2
0.4
0.4
0.2
0.2
0.2
0.2
0.2
0.2
0.2
0.2

0.75
0.75

0.2
0.2
CAL 2

1
1
1
1
1
1
1
2
2 '
1
1
1
1
1
1
1
1

0.75
0.75

1
1
CAL 3

2
2
2
2
2
2
2
4
4
2
2
-
2
2
2
2
2

0.75
0.75

2
2
CAL 4

5
5
5
5
5
5
5
'10
10
5
5
5
5
5
5
5
5

0.75
0.75

5
5
CAL 5

10
10
10
10
10
10
10
20
20
10
10
10
10
10
10
10
10

0.75
0.75

10
10

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                    -33-
Table 6.  Criteria for DFTPP Spectrum









 m/z       "    Relative Abundance




 127           40-60%




 197           <1%




 198           100%  (Base Peak)




 199           5-9%




 275           10-30%




 365           >1%




 441         '  Present and 40%




 443   .        17-23% of m/z 442

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                                     -34-
Table 7a.  Ions for Selected Ion Monitoring to Determine PCBs by Acquiring
           Data for Four Sets of <35 Ions Each
PCS Isomer Group/
Int.Std./Surr.Cmpd.
Monochlorobiphenyls
Dichlorobiphenyls
Trichlorobipheny Is
Tetrachlorobiphenyls
Pentachlorobiphenyls
Hexachlorobiphenyls
Hept a chlor obipheny Is
*
Octachlorobiphenyls
No nach 1 or obi pheny Is
Decachlorobiphenyl
Chrysene-d-j 2
Phenanthr ene-d^ g
1 3Cg-gamma-BHC
13C1--4/4'-DOT
Nominal
Mol. Wt.
188
222
256
290
324
358
392
426
460
494
240
188
294
364
Mass or Range
to be Monitored
152; 186-190
220-224
254-260
288-294
322-328
356-362
390-396
424-430
460-466
496-500
240-241
188-189
187,189
247; 249
No. of
Ions
6
5
7
7
7
7
7
7
7
5
2
2
2
2
Ion Sets
#1 #2 #3 #4
6
5
7 7 1a
7 7 1b
7 7
6C 7 7
6d 7
7
7
5
2
2e
2f
2
                                                Total # ions    25   27   24   35
Monitor m/z 254 to confirm presence of (M-70)  for Clg-PCBs.

Monitor m/z 288 to confirm presence of (M-70)+ for Clg-PCBs..

GBegin range at m/z 357 in Ion Set #2.

^Begin range at m/z 391 in Ion Set #3.

eM/z 188 and 189 included among ions used to detect and measure monochlorobiphenyIs<

     187 and 189 included among ions used to detect and measure monochlorobiphenyls.

-------
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-------
                                       -36-
Table 7c.  Ions for Selected Ion Monitoring to Determine PCBs by Acquiring
           Data for Five Ion Sets of <20 Ions
Ion Set          Ion Set          Ion Set          Ion Set         Ion Set
 No. 1a           No. 2b           No. 3C           No. 4d          No. 5e

 "152              186      -        247              240             356
  153              188              249              241             358
  186              220              254              288             360
  187              222              256              290             390
  188              254              288              322             392
  189              255              290              324             394
  190              256              322              326             424
  220              258              323              356             425
  221              288              324              357             426
  222              289   *           326              358             428
  224              290              328              360             430
  255              292              357              362             432
  256              294              358              391             462
  258              323              360              392             464
  290              324              362              394             466
  292              326              392              396             496
  294      .        328              394              398             498
                   358              396              428             499
                   360              398              430             500
                   362             .                  432             502

17 ions          20 ions          19 ions          20 ions         20 ions
a Ions to identify and measure Cl..-Cly-PCBs, phenanthrene-d,.-, and
    Cg—gamna—BHC.

  Ions to identify and measure Clg-Clg-PCBs.

c Ions to identify and measure Clg-Cl^-PCBs and   C^-^'^

  Ions to identify and measure Clg-Clg-PCBs and chrysene-d^*

e Ions to identify and measure Clg-Cl^Q-PCBs.

-------
                                     -37-
Table 8.  Retention Time Data for PCS Isomer Groups and Calibration Congeners
Isomer Group
Monochlorobiphenyls
Dichlorobiphenyls
Trichlorobiphenyls
TetrachlorohLphenyls
Pentachlorobiphenyls
Hexachlorobiphenyls
Heptachlorobiphenyls
Octachlorobiphenyls
Nonachlorobiphenyls
Decachlorobiphenyl •
Approximate
RRT Range*
0.30-0.35
0.38-0.50
0.46-0.64
0.55-0.82
0.64-0.92
0.75-1.1
0.88-1.2
0.99-1.21
1.16-1.28
1.3
Cal . Cong .
Number
1
5
29
50
87
154
188
200
-
209
Cal • Cong
RRTa
0.30
0.43
0.54
0.56
0.80
0.82
0.88
1.03
-
1.3
a Retention time relative to chrysene-d.., with a 30 mX 0.31 mm ID SE-54 fused
  silica capillary column and the following GC conditions: splitless injection
  at 80°C; hold for 1 min; heat rapidly to 160°C and hold 1 min; increase at
  3*C/min to 310«C.

-------
                                     -38-
Table 9.  Ions for Selected Ion Monitoring Data Accpiisition for Pesticide Analytes,
          Internal Standards and Surrogate Compounds  (Ordered by Retention Time)
Ion     Analyte/Internal Std/   Approx.   Quant.
Set   Surrogate Compound (MW)    RRT      Ion
      Alpha-BHC

      Beta-BHC

        .mma-BHi

        Cg-gaanna-BHC    (294)

      Phenanthr ene-d-j Q  (188)

      Delta-BHC

      Heptachlor

      Aldrin
Gannna—BHC

13
      Heptachlor epoxide (386)

      Gamma-chlordane   (406)

      Endosulfan I

      Alpha-chlorda ne   (406)

      Trans-nonachlor   (440)

      Dieldrin

      4,4'-DDE

      Endrin

      Endosulfan II


      4,4'-DDD

      Endrin aldehyde   (378)

      Endosulfan sulfate(420)

      4,4'-DDT

      13C12-4,4'-DDT

      Endrin ketone

      Chrysene-d-|2

      Methoxychlor
(288)
(288)
(288)
(294)
(188)
(288)
(370)
(362)
(386)
(406)
(404)
(406)
(440)
(378)
(316)
(378)
(404)
(318)
(378)
(420)
(352)
(364)
(378)
(240)
(344)
0.43
0.47
0.48
0.48
0.49
0.51
0.5$
0.64
0.70
0.74
0.76
0.76
0.77
0.80
0.81
0.83
0.35
0.87
0.88
0.92
0.93
0.93
0.99
1.00
1.03
219
219
219
225
188
219
272
263
353
373
195
373
409
79
246
81
195
235
67
272
235
247
67
240
227
                                               Ions  (Approximate
                                              Relative Abundance)
181 (100), 183  (90), 219  (70)

181 (100), 183  (90), 219  (70)

181 (100), 183  (90), 219  (75)

187 (100), 189  (90) 225 (80), 227  (40)

188 (100), 189  (15)

181 (100), 183  (90), 219  (70)

100 (100), 272  (60), 274  (40)

66 (100), 263 (40), 265 (25)


81 (100), 353 (80), 355 (65)

373 (100), 375  (.95)

195 (100), 339  (50), 341  (35)

373 (100), 375  (95)

409 (100), 407  (85)

79 (100), 263 (10), 108 (15)

246 (100), 248  (65)

81 (100), 263 (75)

195 (100), 339  (50), 341  (35)


235 (100), 237  (65), 165  (65)

67 (100), 345 (30)

272 (100), 274  (80), 387  (50)

235 (100), 237  (65), 165  (65)

247 (100), 249  (65)

67 (100), 317 (50)

240 (100), 241  (20)

227 (100), 228  (15)

-------
                                     -39-
Table 10.  Ion Sets for Selected Ion Monitoring of Pesticide Analytes, Internal
           Standards and Surrogate Compounds (Ordered by Retention Time)
Ion Set
No, 1
66
100
181
183
187
188
189
219
225
227
263
265
272
274

Monitored
Compounds
Alpha-BHC
Beta-BHC
Delta-BHC
Gamma— BHC
Cg-gamma-BHC
Phenanthrene-d-j Q
Heptachlor
Aldrin







Ion Set
No. 2
79
81
108
195
246
248
263
339
341
353
355
373
375
407
409
Monitored
Compounds
Heptachlor
epoxide
Alpha-chlordane
Gamma-chlordane
Endosulfan I
Trans-nonachlor
Dieldrin
4, 4 '-DDE
Endrin
Endosulfan II





Ion Set Monitored
No. 3 Compounds
67 4 ,4 '-ODD
165 Endrin aldehyde
227 Endosulfan sulfate
228 4,4'-DDT
235 13C12-4,4'-DDT
237 Endrin fcetone
240 Chrysene-di2
241 Methoxychlor
247
249
272
274
317
345
387
14 ions, 8 compounds
15 ions, 9 compounds
15 ions   3 compounds

-------
                                     -40-
Table 11. Known Relative Abundances of Ions in PCS Molecular  Ion Clusters*
  m/z
Relative
Intensity
Monochlorobiphenyls
  188        100
 '189         13.5
  190         33.4
  192          4.41

Dichlorobiphenyls
  222        100
  223         13.5
  224         66.0
  225          8.82
  226         11.2
  227          1.44

Trichlorobiphenyls
  256        100
  257         13.5
  258         98.6
  259         13.2
  260         32.7
  261   .      4.31
  262          3.73
  263          0.47

Tetrachlorobiphenyls
  290         76.2
  291         10.3
  292        100
  293         13.4
  294         49.4
  295          6.57
  296         11.0
  297          1.43
  298          0.95

Penta chlorobiphenyIs
  324         61.0
  325          8.26
  326        100
  327         13.5
  328         65.7
  329          8.78
  330         21.7
  331          2.86
  332          3.62
  333          0.47
  334          0.25
m/z
Relative
Intensity
                   Hexachlorobiphenyls
                     358         50.9
                     359          6.89
                     360   •     100
                     361         13.5
                     362         82.0
                     363         11.0
                     364      .  36.0
                     365          4.77
                     366          8.92
                     367          1.17
                     368          1.20
                     369          0.15

                   HeptachlorobiphenyIs
                     392         43.7
                     393          5.91
                     394        100
                     395         13.5
                     396         98.3
                     397        ' 13.2
                     398         53.8
                     399          7.16
                     400         17.7
                     401          2.34
                     402          3.52
                     403          0.46
                     404'         0.40

                   Octachlorobiphenyls
                     426         33.4
                     427          4.51
                     428         87.3
                     429         11.8
                     430        100
                     431         13.4
                     432         65.6
                     433          8.76
                     434         26.9
                     435          3.57
                     436          7.10
                     437          0.93
                     438          1.18
                     439          0.15
                     440          0.11
m/z
Relative
Intensity
                          Nonachlorobiphenyls
                            460         26.0
                            461          3.51
                            462         76.4
                            463         10.3
                            464         100
                            465         13.4
                            466         76.4
                            467         10.2
                            468         37.6
                            469          5.00
                            470         12.4
                            471          1.63
                            472          2.72
                            473          0.35
                            474          0.39

                          Decachlorobipheny1
                            494         20.8
                            495          2.81
                            496         68.0
                            497          9.17
                            498         100
                            499         13.4
                            500         87.3
                            501         11.7
                            502         50.0
                            503          6.67
                            504         19.7
                            505          2.61
                            506          5.40
                            507          0.71
                            508          1.02
                            509          0.13
Source:  Rote and Morris (9)

-------
                                     -41-
Table 12.  Quantitation, Confirmation, and Interference Check Ions  for PCBs,
           Internal Standards, and Surrogate Compounds
Analyte/
               Norn.   Quant.  Confirm.   Expected
                                      M-70  Interference
                           Accept.  Confirm. Check Ions
Internal Std.
PCB I some r Group
C11
C12
C13
C14
C15
Cl6
C17
Clg
C19
Clin
. MW

188
222
256
290
324
358
392
426
460
494
Ion

188
222
256
292
326
360
394
430
464
498
Ion

190
224
258
290
324
362
396
428
466
500
Ratioa

3.0
1.5
1.0
1.3
1.6
1.2
1.0
*
1.1
1.3
1.1
Ratio*

2.5-3.5
1.3-1.7
0.8-1.2
1.1-1.5
1.4-1.8
1.0-1.4
0.8-1.2
0.9-1.3
1.1-1.5
0.9-1.3
Ion

152b
152
186
220
254
288
322
356
390
424
M+70

256
292
326
360
394
430
464
498
-
.
M+35

222
256
290
326
360
394
430
464
498
_
Internal standards

  Chrysene-d|2      240

  Phenanthrene-dfQ  188

Surrogate compounds

  13
Cg-gamma-BHC    294

'C-j^^'-DOT    364
240

188



187

247
 241


 189

»


 189


 249
5.1

6.6




1.0

1.5
4.3-5.9

6.0-7.2




0.8-1.2

1.3-1.7
a Ratio of quantitation ion-to confirmation ion

^ Monodichlorobiphenyls lose HC1 to produce an ion at m/z 152.

-------
                                    -42-
Table 13.  Correction for Interference of PCS Containing Two Additional Chlorines
Candidate
                Ion Measured
Quant. Confirm, to Determine
% of Meas. Ion Area to
 be Subtracted from
Isomer Group
Trichlorobiphenyls
Tetrachlorobiphenyls "
Pentachlorobiphenyls
Hexachlorobiphenyls
Heptachlorobiphenyls
Ion
256
292
326
360
394
Ion
258
290
324
362
396
Interference
254
288
322
356
390
Quant
Ion Area
99%
65%
108%
161%
225%
Confirm.
Ion Area
33%
131%
164%
71%
123%
Table 14. Correction for Interference of PCS Containing One Additional Chlorine
Candidate
Isomer Group
Dichlorobiphenyls
Trichlorobiphenyls
Te tr achlorobipheny Is
Pentachlorobipheny Is
Hexachlorobiphenyls
Heptachlorobipheny Is
Oct achlorobipheny Is
Quant.
Ion
222
256
292
326
360
394
430
to Determine
Interference
221
255
289
323
357
391
425
to be Subtracted
from Quant. Ion Area
13.5%
13.5%
17.4%
22.0%
26.5%
30.9%
40.0%








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