v°/EPA
                                   United States
                                   Environmental Protection
                                   Agency
                                  Health Effects Research
                                  Laboratory
                                  Research Triangle Park NC 27711
                                   Research and Development
                                  EPA-600/S1-81-017 Apr. 1981
Project  Summary
                                   Mutagenesis  Screening  of
                                   Pesticides  Using  Drosophila
                                   Ruby Valencia
                                    Drosophila melanogaster males
                                   were exposed by feeding (plus contact
                                   and  possibly inhalation). The genetic
                                   test  found most sensitive and appro-
                                   priate was the sex-linked recessive
                                   lethal test. For this, males of the
                                   Canton-S wild type stock were ex-
                                   posed. They were mated  individually
                                   and  brooded to sample the entire
                                   range of germ cell developmental
                                   stages. A very large number of tests
                                   (over 7000) were accumulated for
                                   each compound in two or more repli-
                                   cate experiments. Concurrent negative
                                   controls were done with each, and
                                   positive controls were run occasionally.
                                   Thirty  pesticides and seven  other
                                   miscellaneous compounds were tested
                                   and four reference mutagens were run
                                   through the system, some of the latter
                                   at a series of "doses" (exposure
                                   concentrations). Table 1 lists them all,
                                   with the results.
                                    Of the 15 pesticides (listed first in
                                   the table) which could be  tested at
                                   adequate concentrations, four (captan,
                                   folpet, bromacil, and simazine) were
                                   found to be weak mutagens. One
                                   (cacodylic acid) was questionable but
                                   called negative. The rest  of the pes-
                                   ticides were so toxic that only very low
                                   concentrations (0.1-5 ppm) could be
                                   used (usually for a reduced exposure
                                   time), and those are not considered
                                   adequately tested, in view of results
                                   obtained with reference mutagens at
                                   these concentrations.
                                    Two of the miscellaneous compounds
                                   (Tris and PtCU) were found to be
                                   potent mutagens. The rest were nega-
                                   tive.
                                    This Project Summary was devel-
                                  oped by EPA's Health Effects Research
                                  Laboratory. Research Triangle Park,
                                  NC, to announce key findings of the
                                  research project which is fully docu-
                                  mented in a separate report of the
                                  same title (see Project Report ordering
                                  information at back).

                                  Introduction
                                    The mutagenicity tests carried out in
                                  this laboratory using Drosophila  were
                                  part of a larger program  involving
                                  several test systems in several labora-
                                  tories. It was not known how Drosophila
                                  systems would compare with others in
                                  terms of sensitivity to detect mutagenic-
                                  ity. Neither was it known which genetic
                                  endpoints (in Drosophila) would be most
                                  adequate in a screening test. It was
                                  recognized that pesticides (especially
                                  the insecticides) would pose special
                                  problems for  genetic tests with fruit
                                  flies. The Drosophila screening system
                                  itself was therefore undergoing defini-
                                  tion and simplification during the course
                                  of these studies.
                                    The original plan was to test  each
                                  compound in  a stepwise manner, as
                                  follows:
                                    1. Dominant lethal test (the fastest).
                                      Stop if positive.
                                    2. Chromosomal alteration test (a
                                      one-generation test). Stop if posi-
                                      tive.
                                    3. Sex-linked recessive lethal test.
                                    It became clear, however, that the
                                  first two tests were not highly sensitive,
                                  and were not easy to do, thus, the lethal
                                  test had to be  done in all cases. At the
                                  same  time, evidence was founding

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(especially Vogel and Sobels, 1976) that
the sex-linked recessive lethal test is by
far the most sensitive Drosophila test.
This type of mutation isfrequent, involv-
ing some 800 genes on the X chromo-
some, and varied in nature, including
both "point" mutations  and chromo-
somal alterations. We feel that the sex-
linked recessive lethal test alone should
be an adequate probe for mutagenesis.
  Many people have  been  hesitant to
accept results with an insect as relative
         to man.  It was thought that insect
         metabolism was probably too different.
         These objectives have been consider-
         ably reduced  by  the discovery that
         Drosophila has enzymes which carry
         out metabolic activation similar to that
         effected by mammalian enzyme extracts
         (Vogel and Sobels, 1976).
           The toxicity of many of the com-
         pounds did cause serious problems, and
         resulted in  a "no  test" conclusion  for
         some of  the compounds. For those
Table 1.    Summary of Compounds Tested
                              Concentration (ppm)
           Pesticide           in feeding solution
                               Mutagenesis
                                  result
  Bromacil
  Captan
  Folpet
  Simazine
  Cacodylic acid
  Dicamba
  DMSA
  Methoxychlor
  Monuron
  MSMA
  Quintozene (PCNB)
  Trifuluralin
  Siduron
  Acephate
  Carbofuran
  Dimethoate
  Methomyl
  Aspon
  Azinphos-methyl (Guthion)
  Chlorpyrifos (DursbanJ
  Demeton
  Dinoseb
  Disulfoton
  Ethyl parathion
  Fenthion
  Malathion
  Monocrotophos (Azodrin)
  Phorate (Thimet)
  Trichlorfon
Miscellaneous  Compounds
  Safrole
  1 'Hydroxy Safrole
  1 'Hydroxy Safrole
    -2,3 epoxide
  Direct Black 38
  Tris (2,3-dibromopropyl
    phosphate)
  Benzidine dihydrochloride
  PtC/4
Reference Mutagens
  EMS (Ethyl methanesulfonate
  El (ethylenimine)
  TMP (trimethyl phosphate)
  TMP (trimethyl phosphate)
  DBE (1,2-dibromoethane)
2, 3, 5, 2000
2, 3. 2000
2, 3, 2000
3. 5, 2000
3. 500, WO
3, 2000
3, 1500
1000
4. 1000. 2000
2, 3, 4, 1500, 2000
3. 4, 8. 2000
2, 3, 1000
100
10
10
1. 5, (10)
4. (10)
5
0.25-1.0
0.1
1
0.5, 1.4
1
0.25. 0.5
0.1,0.25
0.25. 0.5
2. 3
0.5-3
1

100
1000

1000
2000

4,  10. 100, 1000
1000
100, 500


2, 4, 10, 100, 200, 400
2, 4, 10. 30, 50
1000
100, 300
5,  10, 50
+
+
-t-

-?
which could be adequately tested, the
Drosophila results compared quite
favorably with the other systems, pick-
ing up four weak mutagens and one
questionable mutagen. All of these
except one were picked by at least one
other system. Two were found positive
in all systems.

Exposure Methods
  Initial trials  were made of several
other exposure methods (aerosol spray,
contact, injection), but the method
chosen as most appropriate was feeding.
Since flies walk on their food, contact is
always involved; and when vaporization
occurs, the test substance is also inhaled.
The method thus seemed more complete
and exposure more certain, and it better
mimicked human exposure routes.
  It was shown several years ago by
Lesid and Backer (1968) that feeding of
mutagens in glucose solution is effec-
tive. They fed flies in vials with a bit of
soaked tissue (such as Chem-Wipes).
We chose to feed in small disposable
petri plates with a disc of glass fiber
filter m the  bottom. This permitted easy
observation and counting of dead flies
for toxicity information.
  At first, flies  were exposed (toxicity
permitting) for 48 hours. Later, to make
ingestion more certain, the time was
extended to 72 hours.  Flies cannot
survive for more than 24-36 hours
without drinking, but in 72 hours, they
should be obliged to ingest more. Con-
tact and inhalation were also thus
extended.
   Compounds were dissolved, when
possible, in 1 % glucose. During the first
year,  DMSO was  used for compounds
not water soluble. At that time, a deci-
sion was taken (after warnings voiced at
the Fredericksburg meeting) to avoid
DMSO if possible. As a result,  many
compounds were used in suspension
rather than in solution.
   The concentrations were chosen  by
the following criteria. If toxic at 2000
ppm or below, a concentration giving as
near as possible to 50% mortality at 72
hours was  chosen. For very toxic com-
pounds, the duration of exposure was
reduced  as well as the concentration.
For non-toxic  compounds, 2000 ppm
was chosen as a reasonable upper limit.

Sex-linked  Recessive Lethal
Test
   Canton-S wild type  males were ex-
posed. "CS" stock was used because it
has had a low spontaneous frequency

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 >ver many years of use. The frequency
 iverages about 0.15%, with variations
 arely exceeding 0.1% and 0.3%.
  Treated males were mated to "FM6"
 emales.  The X-chromosome of this is
 narked with yellow, white and Bar and
 :arries a  complex of stock inversions.
  Heterozygous Fi females were mated
 ndividually to  FM6 males (brothers or
 stock males) and the Fa of each was
 observed for the presence or absence of
 '+" males. Any culture having no or less
 han 5% of the expected  number of
 males was considered a lethal case and
 i/vas confirmed by  repeating the test
 with four individual heterozygous F2
 emales mated to FM6 males.
  Each treated or  control  male was
 ransferred to new sets of FM6 females
 at intervals of 4, 3, 3,  and 4 days to
 produce 4 broods of progeny. The differ-
 ent broods sample germ cells in gradually
 earlier stages of development at  the
 ime of exposure.  Mature sperm  are
 sampled in Brood 1, spermatids in Brood
 2, spermatocytes in  Brood 3, and sperm-
 atogonia in Brood 4. These  are  not
 "clean," but rather "rough" samples,
 due to the  length of the mating  times
 and that fact that chemicals may remain
 in the body beyond the external exposure
 ime.

 "Cluster" detection and
 handling
  Treated and control males were num-
 aered, mated, and transferred individu-
 ally and the F,  daughters of each were
 mated  as a "family." This is  done in
 order to detect cases where more than
 one  lethal  is produced by one  male.
 These  cases  will  be referred  to as
 "multiples" (as opposed to "singles"
 and "nulls"). A multiple can be due to
 multiple individual  mutations (MIM) or
 o a  single  mutation event in a gonial
 cell,  which  then reduplicates and pro-
 duces two or more sperm cells carrying
 he same lethal (a "cluster"). The
 distinction (if possible) between  these
 wo circumstances is very  important
 when attempting to detect low-level
 mutagenicity.  With potent mutagens,
the contribution of clusters is insignifi-
cant, and mass matmgs of treated and
control males  are the rule.  When  ex-
posure is  simple (as with radiation), and
 many flies  can be  exposed, the pro-
cedure is often  to test only one daughter
of each treated or control fly, this
avoiding both  MIMs and clusters.  Ex-
posure is not simple with chemicals,
  id other precautions must be taken.
  The following procedure was applied
to this data regardless of the recognized
pitfalls. Whenever a multiple was found,
a statistical method (devised by Seymour
Abrahamson) was applied, which yields
the probability (binomial expectation) of
that number of mutations arising inde-
pendently in a single male given (a) the
number  of males in that particular
treated or control group which produced
progeny,  (b) the average number of  FI
females tested per Pi male, and (c) the
mutation frequency.
  If the number of lethals in the multiple
greatly exceeded probability, we con-
sidered it a  cluster and did not count
these lethals.
  In addition,  however, it was often
necessary to make some subjective
judgments on particular compounds.
When the lethals in the replicate treated
groups occurred in multiples, while
those in  the concurrent control group
did not,  this might have indicated
"spotty"  exposure.

Number of chromosomes tested
  The  number of tests needed per
compound of "compound equivalent,"
which would be any variant on a com-
pound, such as dose level, germ cell
stage, or exposure method depends
mostly upon (a) mutagenicity—the more
mutable, the fewer tests needed  to
prove it—and (b) the increment  in
frequency desired to detect.
  When the control rate is 0.15%, and
when it is desired to detect (and prove
statistically) an equal induced frequency
(a doubling of background), then about
8000 treated and 8000 control chromo-
somes should be tested.

Dominant Lethals
  Methodology was developed for dom-
inant lethal screening and tests were
performed on simazine and dicamba,
using very low concentrations. Simazine
gave possibly positive results. This test,
however, was abandoned since it was
time-consuming and would probably
rarely help avoid future testing.

Chromosome Loss, Replace-
ment and Non-disjunction
  The test is  relatively  fast, requiring
only one  generation, and appears to be
simple. In  use,  however,  very  large
numbers are required and interpretation
of results are difficult, due to the several
different  types of variants and their
quite different meanings in terms  of
cytogenetic events. Since the recessive
lethal test also picks up chromosomal
rearrangements, it was  decided that
this separate test was not worth the
time and effort required.
Results and Conclusions
  The pesticide results fall into three
categories:
  (a) Those which were tested at con-
centrations above 10 ppm for at least 24
hours and which yielded results indicat-
ing a weak  mutagenic effect.  These
were captan, folpet, bromacil, and
simazine, plus possibly, cacodylic acid.
  (b) Those  which were presumably
tested adequately (as above) but which
yielded negative results. These were
dicamba through carbofuran in Table 1.
  (c) Those which may not have been
adequately  tested, since they were
highly toxic, were  used at very low
concentrations,  and gave negative
results.
  For the four compounds called positive,
the conclusion was based upon the
experiments with 2000 ppm. Captan,
simazine, and bromacil were tested
simultaneously in  Run No. 37.  Folpet
was tested in Run No. 38. Both runs had
controls with quite low frequencies, but
this appeared to be a true low period for
the stock. Run 37 was done with a
newly prepared stock and the control
was the first of a series giving low
values. In all four cases, there were
several multiples in the treated  series,
but none in the controls. These multiples
were:
  Captan—5 males with 2,2 males with
    3, 1 male with 6
  Folpet—4 males with 2,1 male with 3
  Bromacil—3 males with 2, 1  male
    with 3, 1 male with 4, 1 male with 5
  Simazine—4 males with 2, 2 males
    with 3.
  When the Kastenbaum and Bowman
statistical test (Mut. Res. 9 [1970] 527-
549) is applied to the data for these
compounds (using the sum of Controls
37 and  38 to provide approximately
equivalent numbers of treated and
control tests), the result is as follows.
  Captan is significant at the .01  level if
the multiple of 6 is  included. Without
the multiple, it is significant at the .05
level.
  Bromacil is significant at the .01 level
if the multiples (one of 4 and one of 5)
are included. It barely misses signifi-
cance at .05  without them.
  Simazine had no  multiples greater
than 3 and is significant at the .01 level.
 i US GOVERNMENT PRINTING OFFICE 1981-757-012/7031

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     Folpet also had no correction factor,
   but is significant only at the .05 level.
   Using the Chi2 test, which is somewhat
   less conservative than the Kastenbaum-
   Bowmantest, P=<.02. More importantly
   the folpet data shows a peak of mutage-
   nicity in Broods 2 and 3. Using these
   broods, only, the result is highly signifi-
   cant (Chi2 = 15, P = <.01).
     In  all these cases, the deduction of
   multiples of 4, 5, and 6 is questionable,
   since there are also several multiples of
   2 and 3, while the controls have almost
   none.
     It is possible that exposure may have
   been "spotty"—i.e., some males may
   have ingested, contacted, or inhaled
   more than others, in which case the
   compounds  may be more mutagenic
   than the averaged results indicate.
     Cacodylic acid caused marked sterility
   of treated males, especially in Brood 3,
   indicating a cytotoxic effect on  peri-
   meiotic cells. Unfortunately, it is not
   possible  to  know from  these experi-
   ments whether or not the damage is
   genetic. The recessive lethal frequency
   obtained in  the one adequate experi-
   ment (Run 52) was actually 3 times the
   concurrent control value. The latter,
   however, was exceptionally low, and in
   this case it was not part of consistently
   low control  period. (Controls were, in
   fact, somewhat erratic during thattime.)
   There were no multiples in Control 52
   and only one multiple of 3 in the treated
   males. The result was, thus, considered
   negative but questionable.
           In the tests of miscellaneous com-
         pounds, Tris and PtCU were clearly
         mutagenic, with peak effects in Brood 2,
         indicating  an effect primarily on sper-
         matids. All others were clearly negative.

           The reference mutagens EMS, El, and
         TMP were positive when tested  at
         adequate concentrations. EMS, a very
         potent mutagen, surprisingly gave fre-
quencies very near control level wh«
tested at very low concentrations (2 ar
4 ppm). TMP was negative at 100 pp
and 300 ppm. DBE was tested only ,
low concentrations and was negative <
questionable. It is probable that a
exposure technique was inappropria
for this volatile compound, In all thes
cases,  however,  there were multiple
indicating possible "spotty" exposure
            Ruby Valencia is with the WARF Institute, Inc., Madison, I/I// 53706.
            Michael D. Waters is the EPA Project Officer (see below).
            The complete report, entitled "Mutagenesis Screening of Pesticides Using
              Drosophila," (Order No. PB 81-160 848; Cost: $9.50, subject to change) will
              be available only from:
                   National Technical Information Service
                   5285 Port Royal Road
                   Springfield, VA 22161
                    Telephone: 703-487-4650
            The EPA Project Officer can be contacted at:
                   Health Effects Research Laboratory
                   U.S. Environmental Protection Agency
                   Research Triangle Park, NC 27711
United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
                  Postage and
                  Fees Paid
                  Environmental
                  Protection
                  Agency
                  EPA 335
Official Business
Penalty for Private Use $300
                          000032*

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