United States
Environmental Protection
Agency
Municipal Environmental Research
Laboratory
Cincinnati OH 45268
EPA-600/2-80-? 1 7
August 1980
Research and Development
Phosphorus
Removal in  Lower
Great Lakes
Municipal Treatment
Plants

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                RESEARCH REPORTING SERIES

Research reports of the Office of Research and Development, U.S. Environmental
Protection'Agency, have been grouped into nine series. These nine broad cate-
gories were established to facilitate further development and application of en-
vironmental technology. Elimination of traditional grouping was consciously
planned to foster technology transfer and a maximum interface in related fields.
The nine series are:  „
      1.  Environmental Health  Effects Research
      2.  Environmental Protection Technology
      3.  Ecological Research
      4.  Environmental Monitoring
      5.  Socioeconomic  Environmental Studies
      6.  Scientific and Technical Assessment Reports (STAR)
      7.  Interagency-Energy-Environment Research and Development
      8.  "Special"  Reports
      9.  Miscellaneous Reports

 This report has been assigned to the ENVIRONMENTAL PROTECTION TECH-
 NOLOGY series. This series describes research performed to develop and dem-
 onstrate instrumentation, equipment,  and methodology to repair or prevent en-
 vironmental degradation from point and non-point sources of pollution. This work
 provides the new or improved technology required for the control and treatment
 of pollution-sources to meet environmental quality standards.
 This document is available to the public through the National Technical Informa-
 tion Service, Springfield, Virginia  22161.

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                                             EPA-600/2-80-11 7
                                             August  1980
               PHOSPHORUS REMOVAL
              IN LOWER GREAT LAKES
           MUNICIPAL TREATMENT PLANTS
            .by

                Joseph V. DePinto
                James K. Edzwald
             Michael  S.  Switzenbaum
                 Thomas  C.  Young
Department of Civil  and  Environmental  Engineering
         Clarkson College of Technology
            Potsdam,  New York  13676
              Grant No,  R806817-01
                 Project Officer

                 Edwin  F.  Barth
         Wastewater  Research  Division
      Municipal  Environmental  Research  Lab
             Cincinnati, Ohio  45268
  MUNICIPAL  ENVIRONMENTAL  RESEARCH LABORATORY
      OFFICE OF RESEARCH AMD  DEVELOPMENT
     U.S. ENVIRONMENTAL PROTECTION AGENCY
             CINCINNATI, OHIO  45268

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                                DISCLAIMER
     This report has been reviewed by the Municipal Environmental Research
Laboratory, U.S. Environmental Protection Agency, and approved for
publication.  Approval does not signify that the contents necessarily reflect
the views and policies of the U.S. Environmental Protection Agency, nor does
mention of trade names or commerical products constitute endorsement or
recommendation for use.
                                     ii

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                                 FOREWORD
     The Environmental Protection Agency was created because of increasing
public and government concern about the dangers of pollution to the health
and welfare of the American people.  The complexity of that environment and
the interplay between its components require a concentrated and integrated
attach on the problem.

     Research and development is that necessary first step in problem solu-
tion and it involves defining the problem, measuring its impact, and
searching for solutions.  The Municipal Environmental Research Laboratory
develops new and improved technology and systems for the prevention, treat-
ment, and management of wastewater and solid and hazardous waste pollutant
discharges from municipal and community sources, for the preservation and
treatment of public drinking water supplies, and to minimize the adverse
economic, social, health, and aesthetic efforts of pollution.  This publica-
tion is one of the products of that research; a most vital communications
link .between the researcher and the user community.

     This report addresses the efficacy and desirability of employing a
0.5 mg/L total phosphorus effluent standard for municipal treatment plants
in the lower Great Lakes basins.
                                     Francis To  Mayo
                                     Director
                                     Municipal  Environmental  Research
                                     Laboratory
                                    iii

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                                   PREFACE


     The North American Great Lakes contain about 20 percent of the world's
supply of surface freshwater and, as such, are indispensible resources worthy
of every effort possible to protect and preserve their quality.  Over the
past ten years the United States and Canada have spent a tremendous amount
of time and money in this pursuit.  Knowledge has been gained, decisions have
been made, goals have been set, and most importantly, significant progress
has been made.

     With respect to eutrophication control, it has been determined that
reducing and restricting phosphorus inputs is the best approach for the Great
Lakes.  While we feel strongly that there is little question that phosphorus
load reductions are necessary for the lower Great Lakes, there is still a
debate over the most efficient and economical means to achieve the target
loads.  This study was conceived to provide some of the data and other
information needed to answer several of these questions.  The eighteen month
review period for the November, 1978 -IJC Great Lakes Water Quality Agreement,
imposed a definite time constraint on this project.  Therefore, based on
consultation with our project officer and others in the wastewater research
division at MERL, a survey and field study were designed to provide as much
useful information on phosphorus removal in the lower Great Lakes municipal
treatment plants as possible within the available time-frame and resources
at our disposal.  As a result this report should not be viewed as supplying
definitive answers to the questions addressed,  but should be used as a
source of necessary information in coming to a  decision on a phosphorus ,
standard for lower Great Lakes municipal treatment plants.

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                                 ABSTRACT
      The  Great  Lakes  Water  Quality Agreement  of  1978, established  by  the
 International Joint Commission  of Canada  and  the United  States called for,
 among other things, the  achievement  of  0.5 mg/L  total phosphorus as the
 maximum effluent  level in all Lake Erie and Ontario municipal treatment
 plants discharging greater  than one  million gallons per  day.  In order to
 provide information necessary to review and evaluate the a.bove objective, a
 study composed  of three  parts was undertaken:  1) a survey of phosphorus
 treatment approaches  and accomplishments  for  all  lower Great Lakes basin
.plants with flows greater than  1 mgd; 2)  field operation monitoring studies
 to evaluate the performance of  four  municipal treatment  plants practicing
 phosphorus removal, including a determination of the bioavailability  of the   ,
 wastewater phosphorus; and  3) an analysis of  costs at each of the  four plants'
 monitored, including  incremental costs  to achieve a 0.5  mg/L standard.

      Of the 229 plants in our survey 52 percent  are achieving an effluent
 total phosphorus  concentration  <_1.0 mg/L, while only 8.3 percent  .(19 plants)
 are meeting a 0.5 mg/L standard.  If all  plants  in the Lake Erie basin not
 currently achieving a 1.0 mg/L  standard were  to  do so, the municipal  load
 would' be  reduced  by 2165 MT/yr. A standard of 0.5 mg/L  met in the Lake Erie
 basin would reduce the current  load  by  3264 Mt/yr. Similar standards
 achieved  in the Lake  Ontario basin would  reduce  municipal loads by 1450 and
 2085 Mt/yr, respectively.

      Most of the  plants  practicing phosphorus removal add either aluminum or
 iron as a precipitation  cation  at some  point  in.  the conventional secondary
 operation.  The field studies indicated that  a conservatively operated plant
 using one of the  above approaches could achieve  an effluent level  of  <_ 0.75
 mg/L, and in some cases  lower,  without  filtration.

      Combining  all bioavailability assays run on samples from the  four plants
 revealed  an average of 72  percent of the  total P - 55 percent of  the
 particulate fraction  and 82 percent  of  the  total soluble fraction  -  was
 available for uptake  by  Scenedesmus  sp.  Comparison of available P fractions
 within and among  plants  suggested that  the  methods of treatment examined
 were not  selective for available P to the exclusion of non-available  P
 fractions.

      This report  was  submitted  in fulfillment of grant number R-806817 by the
 environmental engineering  group at Clarkson  College of Technology  under the
 sponsorship of  the U.S.  Environmental Protection Agency. This report covers.
 a period  from June 21, 1979 to  March 20,  1980, and work  was completed as of
 April 14, 1980.

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                                   CONTENTS,

Foreword	•.	.  ,  .  .        HI
Preface  	 .....  	         IV
Abstract .	.*	          V
Figures	       VIII
Tables	         XI
Acknowledgments	•  •  •  •       Aili

   1.  Introduction	•  •  •          ^
   2.  Conclusions	„	          5
   3.  Recommendations	          '
   4.  Methods of Investigation  .... 	  .....          8
   5.  Results of Survey and Phosphorus Loadings to Lower Lakes  .         22
   6.  Results of Field Studies  .	         49
   7.  Studies on Biological Availability of Wastewater
       Phosphorus	'.....	         74
   8.  Cost Analysis  .........	         99

References . .	•        132
Appendices

   A.  Questionnaire  and Survey Work Sheet .	        135
   B.  Wastewater plant performance data	        "138
   C.  Data from field monitoring studies	        139
                                    vn

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                                  FIGURES
Number
   1  '  Periods of composite sampling at the Gates-Chili-Ogden
           wastewater treatment plant, Rochester,  NY;  July 3-11,
           1979	      12
   2    Periods of composite sampling at the Big Sister Creek
           wastewater treatment plant, Angola,  NY; July 30 -
           August 9, 1979	      13
   3    Periods of composite sampling at the Ely wastewater
           treatment plant,  Ely, MN;  August 13  - 22, 1979  .....      14
   4    Flow diagram of analytical  work on wastewater  samples  ...      15
   5    Dual culture diffusion apparatus for particulate phosphorus
           bioassay tests	      17
   6    Flowchart of available phosphorus bioassay  ........      18
   7    Histogram of effluent phosphorus concentration in  lower
           Great Lakes plants	      40
   8    Histogram of phosphorus percentage removals  in lower
           Great Lakes plants	.      44
   9    Comparison of point  to non-point source loading of
           phosphorus at present conditions and at effluent limita-
           tions of 1.0 and  0.5 mg  P/L for municipal point source
           dischargers		      48
  10    Process schematic for Gates-Chili-Ogden plant,  NY  .....      50
  11     Process schematic for Frank Van  Lare plant, NY  ......      51
  12    Process schematic for Big Sister Creek  plant,  NY   .....      53
  13    Process schematic for Ely plant,  MN	„  .      54
  14    Mean concentrations  of total  phosphorus  and phosphorus    ' .   , '
           fractions  at the  Gates-Chili-Ogden plant	 ,      62
  15    Distribution  of phosphorus  fractions at  the Gates-Chili-
           Ogden  plant	      63
                                   vi i i

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Number

   16


   17


   18


   19


   20


   21

   22


   23



,   24
Mean concentrations of total phosphorus arid phosphorus
   fractions at the Frank Van Lare plant ........
Distribution of phosphorus fractions at the Frank Van Lare
   plant	

Mean concentrations total of phosphorus and phosphorus
   fractions at the Big Sister Creek plant	
Distribution of phosphorus fractions at the Big Sister Creek
   plant	

Mean concentrations total of phosphorus and phosphorus
   fractions at the Ely plant	.  .  .  .  .

Distribution of phosphorus fractions at the Ely plant  ,

Algal growth and phosphorus uptake during a bioassay to
   determine available soluble  phosphorus   	  .  .
 Biologically available and non-available fractions- of
    phosphorus in wastewater  samples from the Gates-Chili-
    Ogden  plant	••  <

 Biologically available and non-available fractions of
    phosphorus in wastewater  samples from the Frank Van
Page


  64


  66


;.  67


  68


  70

  71


  75



  81



  82
25
26
27
28
29
30
31.
Biologically available and non-available fractions of
phosphorus in wastewater samples from the Big Sister
Biologically available and non-available fractions of
phosphorus in wastewater samples from the Ely plant ....
Biologically available soluble phosphorus as a function of
Biologically available soluble phosphorus as a function of
Biologically available particulate phosphorus as a function
of total particulate phosphorus in wastewater samples . . .
Biologically available particulate phosphorus as a function
of NaOH extractable particulate phosphorus in wastewater
Total biologically available phosphorus as a function of
total nhnc;nhnni<; in wastewater samoles . 	 	
83
84
89
91
92
94
95
                                      ix

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Number
                                                               Page
  32

  33
  34
  35
  36
  37
  38

  39
  40
  41
  42
  43
  44
  45

  46
  47
Total  biologically  available  phosphorus as a function of
    soluble  reactive plus NaOH extractable particulate
    phosphorus  in wastewater samples  	
Summary of  phosphorus data and line schematic - GCO  .  . .
Phosphorus  concentration of secondary effluent versus
   overflow rate of final sedimentation basin - GCO  ... .
Summary of  phosphorus data and line schematic - Ely  .  . .
Jar test results (unadjusted pH) - Ely	.  .  . .
Jar test results (pH adjusted to 6) - Ely . 	
Phosphorus concentration of secondary effluent versus
   overflow rate of secondary sedimentation basin - Ely .,
Secondary effluent and dual media filtered effluent
   phosphorus concentrations - Ely	 . ... .
Summary of phosphorus data and line schematic - Big Sister
   Creek  	
Jar test results - Big Sister Creek
Phosphorus concentrations of secondary and solids contact
   effluents versus overflow rate - Big Sister Creek  .  .
Granular media filter performance - Big Sister Creek  .  .
Summary of phosphorus data and line schematic - Frank Van
   Lare . . "	
Phosphorus concentrations versus overflow rate of primary
   sedimentation unit - Frank Van Lare  .	
Jar test results (unadjusted pH) - Frank Van Lare .  .  .  .
Jar test results (pH adjusted to 6) - Frank Van Lare  .  .
 96
100

105
108
112
113

114

116

117
120

121
122

124

128
129
130

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TABLES
Number
1
2
•3
4
K
6
7
8
9
10
n
12
13
14
15
16

Base year and target phosphorus loads to Great Lakes 	
Pertinent information on intensively monitored plants ....
Phv^iral anrl rhpmiral methods of analysis 	


Treatment approaches by chemical (precipitation cation) and
Frequency of precipitation cation metered usage (%)' 	
Summary of location of phosphorus removal treatment in the
treatment plant process (%) . 	
Frequency of 30-day average effluent phosphorus concentra-
tions - mg/L as total P 	 	
Distribution of plants by size and basin reaching 1.0 and
0.5 mg P/L total phosphorus effluent concentrations ....
Frequency of % phosphorus removal achieved (based on total
nhn^nhnvii^ • Hnta "fynm niip^t'ionnai re ) 	
Present and projected municipal point source phosphorus
loadings to the lower Great Lakes - in metric tons/year . .
Phosphorus loading to Lakes Erie and Ontario (in metric
Sampling locations within monitored treatment plants 	
Performance of intensively monitored waste treatment plants .
Concentration of phosphorus fractions and removal percentages
•t.hrnijah intensi vel v monitored wastewater plants 	 	
Page
2
10
20
?3
36
38
38
38
39
42
43
45
47
55
57
60
   XI

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Number                                                                  Page
                                                                         i
  17    Concentration of priority pollutants in wastewater
           samples from monitored treatment plants 	 	    72
  18    Results of phosphorus availability bioassays on wastewater
           samples from Gates-Chili-Ogden plant	    76
  19    Results of phosphorus availability bioassays on wastewater
           samples from Frank Van Lare plant	    77
  20    Results of phosphorus availability bioassays on wastewater
           samples from Big Sister Creek plant	    78
  21    Results of phosphorus availability bioassays on wastewater
           samples from Ely plant	    79
  22    Available: total  phosphorus ratios and available phosphorus
           removal percentages through intensively monitored
           wastewater plants		    86
  23    Summary statistical parameters and correlation coefficients
           for chemically and biologically assayed phosphorus in
           wastewater samples	  .    88
  24    GCO - total  O&M costs	   101
  25    Associated O&M costs for phosphorus removal   	 ...   101
  26    Sludge and chemical costs at GCO	   103
  27    Summary of incremental  costs at GCO	   106
  28    Ely - total  O&M costs	   106
  29    Associated O&M costs for phosphorus removal  - Ely  ......   HO
  30    Sludge production - Ely  .	   110
  31    Big Sister Creek  - total O&M costs	   110
  32    Associated O&M costs for phosphorus removal  - Big Sister
           Creek	   118
  33    Sludge Production - Big Sister Creek	,	   118
  34    Van Lare - total  O&M costs	   118
  35    Associated O&M costs for phosphorus removal  - Van Lare  ....   126
 36     Sludge production - Van Lare	    126
                                    xii

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                              ACKNOWLEDGMENTS

     The cooperation and assistance of a great many individuals and agencies
were necessary to complete this study.  Although they are too numerous to
mention individually we would like to thank the treatment plant supervisors
and operators who took the time to respond to our rather probing survey
questionnaire.  Special acknowledgment is due to the gentlemen at the four
treatment plants that were highlighted in this study for their total
cooperation and hospitality throughout.  Mr. Joe Catone, chief operator at
the Gates-Chili-Ogden plant; Mr. Mike Schifano, chemist at the Frank Van
Lare plant, Mr. Glenn Absolom, Jr., chief supervisor and Mr.  Mark Fitzgerald
of the Big Sister Creek plant, Mr. James Pastica, plant superintendent and
Mr. Terry Jackson at the Ely plant were our major contacts.  Of course, the
help of all the staff at these plants is greatly appreciated.

     A good deal,of advice and information was provided by individuals
throughout the Great Lakes community, Dr. Edwin Tifft, Jr. and Mr. David
Hill, lab supervisor, of O'Brien and Gere Engineers, Inc. conducted the
analysis of trace organics in our samples; Mr. Donald Schwinn, Stearns and
Wheler, provided valuable assistance on our cost analysis; Dr. William
Sonzogni, Great Lakes Basin Commission, Mr. John Archer, Ontario Ministry of
Environment,-Mr. Ron Drynan, International Joint Commission,  Mr. Thomas
Quinn and Mr. John Chase of the Monroe County Division of Pure Waters, and
Mr. Joe DiMura of the New York Department of Environmental Conservation  .
provided advice and essential information for the study.

     Special thanks and acknowledgment is due those students  who devoted
much time and effort in field and lab analysis to make this project a
success; Mr. Kent McManus and Mr. Shawn Veltman spent nearly three months in
the field monitoring the four treatment plants; Mr. Steven Flint conducted
all the bioavailability work; and Mr. Edward Seger and Mr. Greg Comstock
assisted in the heavy metal analysis.

     Finally, because of the valuable guidance and active support of certain
individuals in the Wastewater Research Division of the Municipal Environ-
mental Research Lab in Cincinnati this project was truly a cooperative
agreement.  Our special thanks goes to Mr. Edwin F. Barth, Project Officer,
for his enthusiasm and insight in planning this project, for his attention
to details in our conducting the study and for his thorough review of this
manuscript.  We also acknowledge the great interest taken in this project by
Mr. John J. Convery, Director of the Wastewater Research Division, whose
-upport and advice were invaluable.
                                    xm

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                                 SECTfON 1

                              " INTRODUCTION


     On November 22, 1978 the International Joint Commission (IOC) of Canada
and the United States effected the Great Lakes Water Quality Agreement of
1978.  Among the many aspects of water quality addressed in the Agreement,
the IJC recognized that control  of phosphorus in the Great Lakes system was
necessary to minimize eutrophication problems.  The Agreement denotes a
specific objective with respect to phosphorus:

        "The concentration should be limtted to the extent
         necessary to prevent nuisance growths of algae,
         weeds and slimes that are or may become injurious
         to any beneficial water use."  (IJC, 1978).

     Pursuant to the above objective the IJC Agreement established a program
to reduce the input of phosphorus to the Great Lakes.  The removal of
phosphorus from municipal waste treatment discharges was considered an
important part of the overall program.  In  this regard the Agreement called
for the achievement by all plants discharging more than one million gallons
per day of "effluent concentrations of 1.0  milligram per litre total
phosphorus maximum for plants in the basins of Lakes Superior, Michigan, and
Huron, and. 0.5 milligram per litre total phosphorus maximum for plants .in
the basins of Lakes Ontario and Erie."  (IJC, 1978).

     Because of more severe demographic pressure, the lower Great Lakes were
considered subject to more severe loading limitations, and hence greater
emphasis was placed on control of point sources of phosphorus.  Table 1 is a
reproduction from the IJC Agreement of the  base year (1976) phosphorus loads
to the Great Lakes along with target loads  recommended by Task Group III
(Vallentyne and Thomas, 1978) to meet the Agreement's eutrophication-related
water quality objectives.  The 1978 Agreement also provided for an eighteen
month review to confirm the target loads in Table 1, followed by the
establishment of load allocations and compliance schedules.  The purpose of
this study was to provide information necessary to make recommendations
regarding phosphorus load reduction requirements for municipal treatment
plants in the lower Great Lakes basins.

     It must be noted at this point that the target loads of phosphorus for
Saginaw Bay, Lake Erie and Lake Ontario cannot be met by only reducing
municipal point source total phosphorus (TP) to 0.5 mg/L.  According to the
Task Group III report, a 1 mg/L municipal total phosphorus effluent standard
for the Erie and Ontario basins would require a concurrent 50 percent
reduction in diffuse sources to meet the target loads.  A 0.5 mg/L TP

                                      1

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TABLE 1.

Basin
Lake Superior
Lake Michigan
Main Lake Huron
Georgian Bay
North Channel
Saginaw Bay
Lake Erie
Lake Ontario
BASE YEAR AND TARGET PHOSPHORUS

Base Year (1976) Phosphorus
Load (Metric Tons/Yr)
3,600
6,700
3,000
630
550
870
20,000
11,000
LOADS TO GREAT LAKES*

Target Phosphorus Load
(Metric Tons/Yr)
3,400+
5,600+
2,800+
600+
520+
440+"
11,000+"
7,000+"
* From IJC (1978)

+ These loadings would result if all  municipal  plants over one mgcl (3,785
  nvVd) achieved an effluent total  phosphorus of 1  mg/L

+ The loadings are required to meet water quality objectives

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standard would require a 30 percent reduction in diffuse sources.  Assuming
the target loads are not changed, a decision must be made regarding the
efficacy and cost desirability of the 0.5 mg/L recommended municipal effluent
standard for the lower lakes.

     There are several questions related to the municipal treatment plant
phosphorus standard which were addressed in this study.  The current status
of municipal treatment plant activities in the lower lakes with respect .to
phosphorus removal has been evaluated.  Such questions as "what are the
prevalent approaches being taken to reduce phosphorus effluent concentra-
tions to 1.0 mg/L" and "what technological needs would the treatment plants
have to reduce total phosphorus effluent levels to 0.5 mg/L or any point
below 1.0 mg/L" have been addressed.  Also, there is a need to know the
reliability with which full scale treatment operation can operate at the
various phosphorus reduction performance levels.

     In addition to the technological aspect of establishing a phosphorus
treatment regulation for the lower lakes treatment plants, prudent use of
the taxpayer's money requires systematic evaluation of the relationship
between costs incurred and effluent phosphorus residuals.  These costs could
then be weighed against the economic and environmental benefits of various
phosphorus effluent limitations below 1.0 mg/L.  This type of cost analysis
at the individual treatment plant level is examined in this study.  Costs
data gathered in this study can provide crucial information and confirmation
of assumptions necessary to make basin-wide cost projections for various
municipal phosphorus management programs.

     Another important consideration, which is receiving much attention in
Great Lakes management and the scientific community, is the question of
"phosphorus availability" for the various sources of this material.  For  -
virtually every type of phosphorus source there is a certain fraction that
is immediately available for algal uptake.  The remainder of the total
phosphorus  in that source contains phosphorus that may be unlikely to ever
become available and/or, depending upon its chemical character and the
conditions  in the receiving water body, will be transformed to a usable form
at a certain rate.  Projections of lake dynamics in response to phosphorus
loads from  various sources need to consider, among many other things, the
form of the phosphorus in those sources and the rate at which and extent to
which each  form becomes available for algal uptake.  This need applies just
as much to  municipal point sources as to  any other phosphorus source to the
Great Lakes.  Of particular  concern  for municipal treatment plant phosphorus
is the question of the variability of phosphorus availability with wastewater
influent  source, conventional treatment approach and specific phosphorus
removal measures.  This project utilized  techniques to bioassay the fraction
of phosphorus in municipal treatment plants that can be taken up by algae in
a fixed length of time.   It  should be noted that the results in this phase
of the  project are only preliminary,  and  because :0f time and resources
available,  could  not answer  definitively  all the questions regarding phos-
phorus  availability in municipal effluents.

      In order to  address,  the questions posed in the above discussion, this
study contained the following objectives:

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1)  A desk survey was made of all municipal treatment plants in the
    lower Great Lakes basins with effluent flows/greater than 1 MGD.
    The purpose of the survey was to evaluate the phosphorus treatment
    approaches and plant performance and to confirm municipal phos-
    phorus loads.

2)  A detailed field operation monitoring program was conducted at four
    treatment plants practicing phosphorus removal processes representa-
    tive of lower Great Lakes basin plants.  The performance of these
    plants was evaluated in terms of removal  of various phosphorus
    fractions, reduction of certain priority pollutants, and the
    overall effluent quality as a function of the phosphorus removal
    process employed.

3)  A detailed analysis of costs incurred at the four selected treatment
    plants was made for the existing level of treatment.  With the
    existing treatment level costs as a base, estimates were made of
    costs associated with reducing total  phosphorus concentrations to
    0.5 mg/L.

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                                 SECTION 2

                                CONCLUSIONS
1.   There are 229 municipal  treatment plants with discharge greater than 1
    mgd (3785 rri3/d) in the two lower Great Lakes basins,  representing
    municipal total phosphorus loads of 4555 metric tons/year to Lake Erie
    and 2858 metric tons/year to Lake Ontario.   Currently 52 percent of the
    plants in both basins are achieving an effluent total phosphorus con-
    centration <. 1.0 mg P/L.

2.   Of the 229 plants in the lower lakes information on treatment approach
    was obtained for 134.  One hundred and four of the 134 plants responding
    indicated that they practiced phosphorus removal.  Of the plants
    practicing phosphorus removal 48 percent used aluminum as the precipita-
    tion cation while 50 percent used iron.  Only two plants practiced
    phosphorus removal with lime addition.  Only 5 percent of the plants
    utilized some form of tertiary treatment beyond precipitation.

3.   Currently 19 treatment plants have been identified as achieving a 0.5
    mg P/L effluent concentration.  The treatment approach information
    available on 14 of these plants indicates that only 2 are employing any
    tertiary processes.

4.   The mean influent total phosphorus concentration for 117 municipal
    plants reporting this value was 6.3 mg P/L.  Therefore, on the average
    84 percent TP reduction through the plant would be required to achieve
    1.0 mg P/L.  Of course, these calculations could vary considerably for
    individual plants.  For example, states with phosphate detergent bans
    (such as New York) tended to have lower influent P concentrations.

5.  Based on the results of our survey, if all treatment plants in the Lake
    Erie basin not currently achieving a 1.0 mg P/L effluent concentration
    were to  do so, the total load to Lake Erie would be  reduced by 2165
    metric tons/year  (13 percent of the current total).  A standard of 0.5
    mg P/L in Lake Erie would reduce the municipal load  by 3264 metric
    tons/year (19  percent of the current total).

6.  'For  Lake Ontario  total  load reductions of  11 percent (1450 metric tons/
    year) and 15 percent  (2085 metric tons/year) would be  achieved  if treat-
    ment plants  in the basin achieved 1.0 mg P/L and 0.5 mg  P/L effluent
    levels,  respectively.   These  load reductions are conservative in that
    they do  not  account  for the reduction  in the load of phosphorus  to  Lake
    Ontario  from Lake Erie  which  would  likely  result from  common  standards oi
    phosphorus removal being met  simultaneously  by wastewater plants  in  both

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      basins.
  7.
 8.
 9.
10.
11.
12.
13.
 Data on phosphorus removal from the four plants which were sampled
 during this investigation indicate that a final effluent total   phos-
 phorus standard of 1.0 mg P/L can be attained with reliability and
 without filtration, provided that conservative overflow rates are
 employed during clarification.  Though achievement of final  total phos-
 phorus concentrations which would meet a 0.5 mg P/L standard appeared
 to be possible without filtration, as shown by data collected at the
 Big Sister Creek plant, the reliability with which that standard could
 be met was uncertain, due to insufficient data.  Filtration, as
 practiced at the Ely plant did appear to provide a reliable  technique
 to attain a 0.5 mg P/L standard.

 For a specific wastewater the ratio of biologically available phosphorus
.to total  phosphorus remains relatively constant regardless of methods
'employed for treatment, including phosphorus removal.   Thus, the pro-
 portionate availability of phosphorus in the raw wastewater  determines
 the fraction of available phosphorus concentration of a wastewater
 results in a proportionate reduction in the available phosphorus during
 treatment.

 Soluble phosphorus  is proportionately more  available (82 percent)  than
 particulate phosphorus (55 percent)  in wastewater.   Thus,  efforts  to
 control  the ecological  effects of phosphorus in wastewater effluents
 should  focus,  preferentially,  on  minimizing the soluble phosphorus.

 It was  noted that an  effluent  level  of 0.5  mg/L could  be met with  the
 addition  of liquid  alum to the effluent of  the  aeration basin of a
 conventional  activated sludge  process  provided  that  a  conservative
 operation  of the final  sedimentation  basin,  approximately  400 gpd/ft2
 (16.3 m-YmZ-d), was used.

 It was  noted the alum addition to  the  primary sedimentation  basin was
 not an  effective use  of the precipitation cation  due to competing
 reactions with  the aluminum.

At a tertiary plant,  with  a well operated solids  contact clarifier with
FeCl3 and polymer addition, an  effluent  level of  0.5 mg/L was met
without filtration.

The operation and maintenance  costs associated with phosphorus removal
varied significantly  for the four treatment plants studied (from $0.007
to  0.107 per 1000 gallons  (3.78 m3) treated) with higher costs at the
plants with  tertiary  treatment.  Chemical costs, as opposed to power
and labor costs, were the most significant" items.  The costs  associated
with sludge production attributed to phosphorus removal were  in general
not too significant.

-------
                                 SECTION 3

                              RECOMMENDATIONS

     The survey of phosphorus removal performance at wastewater plants in
the Lower Great Lakes Basin (L.GLB) indicated that average final effluent
concentrations of 0.5 mg/L of total phosphorus may be achieved without
resort to filtration.  It is recommended, therefore, that should a 0.5 mg
P/L final effluent standard be placed on municipal treatment plants, then a
careful evaluation of less costly, alternative treatment approaches to meet
the standard should be performed before resorting to a more expensive
filtration process.

     The survey showed that the basic approach employed most frequently at
wastewater plants in the LGLB to remove phosphorus, in order to comply with
present effluent restrictions, amounted to the addition of iron or aluminum
salts to the wastewater at some point in a conventional secondary treatment
system.  Consequently, it is. recommended that full-scale studies be under-
taken to optimize this approach in terms of the main operational parameters,
such as, point of chemical addition and dosage, and further, its integration
with standard operating conditions, such as clarifier overflow rates and
biological treatment parameters.

     With regard to the biological availability of wastewater phosphorus it
is recommended that further work be directed toward extensive quantification
of availability for wastewaters of differing raw wastewater characteristics,
for differing stages of treatment within plants, and among plants which
employ different treatment approaches for removal of phosphorus as well as
other'pollutants.  Studies on biological availability should include an
analysis of the kinetics of conversion of wastewater phosphorus to available
phosphorus, a determination of the fraction of total wastewater phosphorus
which ultimately may become available in natural waters, and an examination
of the relationship between biologically available phosphorus and chemical
measurements of phosphorus.

-------
                                 SECTION 4

                         METHODS OF INVESTIGATION
GENERAL

     This study involved three phases of investigation.   The first phase was
a desk survey of all municipal treatment plants in the lower Great Lakes
basins (Erie and Ontario) with effluent flows greater than 1 mgd (3785 m3/d).
The main objective of this survey was to obtain phosphorus removal  process
information and to confirm the current phosphorus removal performance at
these plants.  Concurrently with this phase, a second line of investigation
was to conduct field sampling studies at four selected municipal treatment
plants.  Approximately two weeks were spent at each plant gathering
operational data, historical data and cost information.   Subsequent to the
first two phases of the project, a detailed cost analysis related to the
question of phosphorus removal in municipal treatment plants was conducted.

SURVEY METHODS

     In order to meet the objectives of the project, it was felt that
several important pieces of information had to be gathered on every treat-
ment plant in the Lake Erie and Lake Ontario basins with a discharge flow
greater than 1 mgd (3785 m3/d).  Therefore, the following information was
obtained for the plants in question:                          ,   •,.

     •  Identification of the location of the treatment plant in terms of.
        lake basin, regulatory unit, county, city and receiving water body.

     •  Identification of type of treatment plant {eg. conventional
        activated sludge, extended aeration, trickling filter, primary
        treatment only, etc.)

     •  Identification of method of phosphorus removal, including point of
        chemical additions and any tertiary processes associated with P
        removal  (such as filtration, sedimentation, etc.).

     •  Identification of annual average daily flow and design flow as well
        as total P concentrations in the raw and plant effluent.

     Although much of the above information could be obtained from previous
studies, it was  felt that certain information could only be reliably obtained
directly from the plants.  As a result a questionnaire (Appendix A) designed
to obtain the above information was sent to a list of 263 municipal treatment
                                      8

-------
 plants  in the lower  lakes  basins.
 following sources:
The list of plants was compiled from the
      1.   International Joint Commission  (Julyjl978),
      2.   NYS Dept. of Environmental Conservation  (January, 1979),
      3.   Ontario Ministry of the Environment  (December 31, 1977),
      4.   Great Lakes Basin Commission, Personal Communication  (1979).

 In addition to providing such otherwise  unavailable information as phosphorus
 removal approach and chemical dosage, the questionnaire provided a current
 update and confirmation of plant flow and effluent P concentration.

      On the basis of the questionnaire,  and from other sources of informa-
 tion  (see Section 5) when the questionnaire was not.answered, a survey work
 sheet (Appendix A) was prepared for each plant.  These work sheets provided
 the basis for the survey results presented in Section 5.  Of the 263 plants
 sent  the questionnaire, 154 returned it with the information requested.
 Subsequent to mailing the questionnaire, it was determined for a variety of
 reasons that the actual survey should include only 229 plants.  A final list
 of the survey plants is presented in Section 5.

      A special effort was made to obtain the desired information, by tele-
 phone if necessary, from all plants with discharge flow greater than 10 mgd
 (37850 ,m3/d).  Plants with discharge flow less than 10 mgd (37850 m3/d) and
 greater than 1 mgd (3785 m3/d) which did not answer the questionnaire are
 not included in certain aspects of the survey results.   However, a flow and
 effluent phosphorus concentration has been assigned to each of the 229
 plants, either from questionnaire data or from an independent IJC survey
 (July, 1979).  This was necessary in order to calculate total  municipal
 phosphorus loads to the lower lakes.

MUNICIPAL TREATMENT PLANT MONITORING PROCEDURES

 Treatment Plant Section

      Four different treatment plants were intensively monitored during the
 field study phase of this project.   The primary criterion for plant selection
was that they represented a variety of P removal  approaches,  including P
 removal  in a primary, a secondary and a tertiary system.   Of secondary
concern was the logistics of monitoring four different plants for two weeks
each, over a period of about two months.  It was felt that at least two weeks
of data were necessary to smooth out the typical  day-to-day fluctuations
encountered in the' operation of a wastewater treatment plant.   It should be
noted, however, that the results obtained in this field study represent
operational  data during summer seasonal  conditions.   Appendix B contains
historical data obtained from each of the four plants so that a perspective
can be obtained on seasonal  and long-range fluctuations in plant operation.

     A brief description of the four intensively monitored treatment plants
is presented in Table 2.   A more detailed description of each  plant,
including  a  process schematic,  is given in Section 6.

-------
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Field Monitoring Procedures

     The on-site monitoring phase of the project was performed during July
and August of 1979.  For the three plants in western New York the field team
worked out of a 24 foot (7.3 m) Mobile Environmental Lab (MEL); however,
available bench space was used at the Ely plant.  During the visit to each
plant the following tasks were performed: sample collection; analysis of
many parameters on site; shipment of samples for bioassay work and priority
pollutant analysis (see below); assessment of plant operation and procurement
of historical data on P removal with associated costs; and the gathering of
sludge production data for the existing operating mode.

     The sample collection involved approximately a 10-12 day period wherein
eight-hour composite samples (except for the Van Lare Plant where '24-hour
composites were used) were collected from three key locations within each
plant, the location of which depended on whether phosphorus removal was a
discrete treatment step or integrated with other treatment processes.   In all
cases the sampling points were selected in order to isolate the effect  of the
phosphorus removal procedure.  The periods of composite sampling at each
treatment plant where 8-hour composites were used are'presented in Figures 1
through 3.

     A flow  chart  of the analyses performed on  the  composite samples is
presented in Figure 4.  Each composite  sample was analyzed on-site for
chemical oxygen demand  (COD),  suspended  solids  (SS), pH, alkalinity, soluble
reactive phosphorus  (SRP), total phosphorus  (TP), total particulate phos-
phorus  (TPP),  and  the total particulate  phosphorus  extractable by 0.1 N NaOH
 (NaOH-P).  Less frequently, on-site analyses were performed to determine
total Kjeldahl  nitrogen  (TKN), nitrate  and nitrite  nitrogen  (NOX), and  five-
day  biochemical oxygen  demand  (BOD5).   Phosphorus precipitation cations
 (A13+ and Fe3+) were measured  off-site  on subsamples taken  in  connection
with the less frequent  series  of on-site analyses.

     A  final group of analyses were performed off-site  on two  or three
 samples from each  sampling location at  each  plant.  Analytical determinations
 in this group include those for  priority pollutants and bioassay of  phos-
 phorus  availability.  The  priority  pollutants to be measured  include both
 organics and heavy metals  (Cd, Zn,  Ni).  A  subcontract  to an  outside
 consultant  (O'Brien  and Gere  Consulting Engineers,  Syracuse,  N.Y.) was  used
 to obtain analyses for  organics, while  samples  for  metals were analyzed by
 project personnel  at Clarkson.  Bioassay studies of phosphorus availability
 were performed at  Clarkson (procedure described below).

 Available  Phosphorus Bioassay Procedures

      As a  verification  of the chemical  analysis of  phosphorus availability
 in the  plant samples,  a bioassay of algal-available phosphorus was  conducted
 on selected samples  from each plant.  While some work has  been done  on
 correlating chemical  procedures  with  bioassay measurements  of available phos-
 phorus  in  river water,  urban  runoff,  lake  sediments and atmospheric  inputs
 (Cowen  and Lee, 1976;  Dorich  and Nelson, 1978;  Fitzgerald,  1970;  Goltermann,
 et a-T., 1969; Logan, et al.,  1979,  among others) no such  correlations  have

                                      11

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                        GATES-CHILI-OGDEN
                                 HOUR
 Date


 3 July


 4 July


 5 July


 6 July


 7 July

 8 July


 9 July


10 July


II  July
             MN
&OOAM
>£/
                                          N
                            6:QOPM
                                                                   J2J/IN
 Figure 1. Periods of composite  sampling at the Gates-Chili-Ogden
           wastewater treatment  plant, Rochester, NY; July 3-11,
           1979
                                  12

-------
        I2MN
Date

30 July

31  July

 i  Aug.

 2 Aug.

 3 Augl

 4Augr

 5 Aug.

 6 Aug.

 7 Aug.

 8 Aug.

 9 Aug.
                           BIG SISTER CREEK
                                HOUR
6=OQAM
I2N
6-OOPM
                                                                   12MN
  Figure 2. Periods of composite sampling at the Big Sister  Creek
            wastewater treatment plant, Angola, NY; July 30-
            August 9,  1979
                                    13

-------
         I2MN
Date

13 Aug.

14 Aug.

15 Aug.

16 Aug.

17 Aug.

18 Aug.

19 Aug.

20 Aug.

21 Aug.

22 Aug.
                                  ELY
                                 HOUR
6:00 AM
I2N
6=00 RM
I2MN
   Figure 3. Periods of composite sampling at the Ely wastewater
            treatment plant,  Ely, MM; August 13 -22, 1979
                                  14

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been published for municipal treatment plants effluents.  We, therefore,
endeavored to determine what fraction of a plant effluent phosphorus actually
has the potential to contribute to algal growth.  This information should be
valuable in the determination of benefits to be derived from a lower total
phosphorus standard for municipal treatment plants.

     While it is generally accepted that only a bioassay can be used to
measure available phosphorus, the details of the experimental procedures
vary widely (DePinto, 1978a).  We have selected an approach which employs a
direct measurement of phosphorus taken up by a test algal species, thus over-
coming the problems associated with indirect estimates relating algal growth
to phosphorus uptake.  Furthermore, our approach provides for the separation
of the assay algae from the particulate material in the plant effluent,
which is a prerequisite for direct measurement of algal phosphorus.

     Given the above considerations it was determined a dual culture
approach similar to that currently being used in our laboratory (DePinto,
1978b) would circumvent many of the problems associated with bioassay
determination of available phosphorus from particulates.  The apparatus
employed (hereafter referred to as a Dual Culture Diffusion Apparatus - DCDA)
allows a suspension of particulate matter from plant effluent in a given
water medium to be placed in one culture vessel (regeneration vessel) and
the placement of a unialgal assay culture (with a known P content) in a
separate assay vessel.  The two vessels are clamped together but the contents
are separated by a 0.4 ym membrane filter (Figure 5).  This set-up permits
repeated, routine sampling of the algae in the assay vessel without dis-
turbing the particle-water system in the regeneration vessel.  The membrane
between the two vessels would prevent cross-contamination of particulates
but would allow cross-diffusion of soluble material (including P released
from the particle-water suspension).  Any available phosphorus released by
the material in the regeneration vessel  will  have a tendency to diffuse
across the membrane to the assay vessel  where it will be rapidly incorporated
by'the P-starved algae.  By periodically sampling the phosphorus content of
the assay vessel and performing a mass balance on the system one can
determine the extent to which phosphorus is being released by. the particu-
lates.  Details of DCDA operation and data analysis can be found in McKosky
(1978).

     A typical bioassay experiment to measure the rate of release of
available P from plant effluent particulates  is illustrated in Figure 6 and
consisted of the following general  steps:

     1.  An aliquot of an 8-hour composite was collected from the treatment
         plant in question, and a sample of Lake Ontario water was collected
         from the water intake system at Sackets Harbor,  NY (Lake Ontario).

     2.  The particulate matter in the composite sample was separated from
         the water by 0.45 ym membrane filtration.   The Lake Ontario water
         sample was also filtered through a 0.45 ym membrane filter.

     3.  A complete chemical  characterization was performed on the treatment
         plant sample as describedi in the previous  section.
                                     16

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  Raw Influent
  Biological  Effluent
  Final. Effluent
                    Filtration /Residue
Algae \ _ Harvest
Algae  \ (0.45jj)
\ Filtration  /  \ Filtration ~7
A (0.4511)  /'   \(0.45u) /
                       Rltrate  Residue
                               Algae
       Figure 6. Flowchart  of available phosphorus  bioassay

                                   18

-------
     4.  The sample participate matter, suspended in P-free synthetic algal
         medium, was placed in the darkened regeneration vessel  of the DCDA.
         The lighted assay vessel contained a P-starved Scenedesmus culture
         in the filtered lake water.

     5.  The contents of each vessel were continuously stirred and the assay
         vessel was periodically sampled for phosphorus to determine the
         accumulation of released available P in the algae.

     6.  After a suitable incubation period (two weeks to a month) the run
         was terminated and both sides of the DCDA were reanalyzed for the
         same parameters as the initial characterization.

     In addition to the above analysis on the suspended solids in the plant
effluent, a bioassay of algal available P was performed on the "soluble"
fraction of the effluent collected in step. 2 above.  A number of authors
have pointed out possible discrepancies between chemical methods (such as
the soluble reactive P test) and actual algal available phosphorus
(Chamberlain and Shapiro, 1969; Peters, 1977).  To bioassay the fraction of
total "soluble" (less than 0.45 pm) phosphorus in these samples that is    /
available for algal uptake, a simple sequential batch uptake experiment was
performed according to the following general procedure:

     1.  The 0.45 pm filtrate of a treatment plant sample was diluted with
         P-free synthetic algal medium to a total soluble phosphorus con-
         centration of 300 pg P/L.  The diluted sample was inoculated with a
         P-starved test algae inoculum (of known P content) and incubated in
         a lighted environment with continuous stirring.

     2.  After a suitable incubation period (2-5 days), a separation of the
         test algae from the water sample was obtained by differential
         centrifugation, which left colloidal and soluble material in the
         supernatant.  An analysis was made of the new total P content of
         the separated algae.

     3.  A new inoculum of P-starved test algae was added to'the supernatant
         sample and step 2 was repeated.

     4.  Steps 2 and 3 were repeated until no increase in test algal cell
         phosphorus content was noted..

     5.  The total available phosphorus in the original sample was then the
         summation of the phosphorus taken up in each sequential incubation.

ANALYTICAL METHODS

     For the most part the analytical methods used in this study are
described in Standard Methods (APHA, 1975) and/or recommended by EPA (1976).
The routine analytical methods are described and referenced in Table 3.
Additionally, the determination of total NaOH-extractable phosphorus
fraction of non-filterable residue was made by an extraction method similar
to that of Sagher, et al. (1971) followed by total phosphorus determination
                                     19

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            TABLE 3.  PHYSICAL AND CHEMICAL METHODS OF ANALYSIS
        Parameter
    Method
 Reference
         pH



Alkalinity

Suspended Solids


Chemical Oxygen Demand




Phosphorus


Total Kjeldahl Nitrogen
N03+N02-N
Biochemical Oxygen Demand
Iron
Aluminum
Cadmium, Nickel and Zinc
Electrometric,
combination
electrode

Electrometric
titration

Gavimetric @
103°C

Standard ampule
method, acid-
dichromate
oxidation

Ascorbic acid
col crimetrie
Acid Digestion;
distillation;
phenate col cri-
me trie

Cadmium reduction;
chromatropic acid
colorimetric

Dilution bottle
test; pplaro-
graphic oxygen
measurement

Nitric acid
digestion; flame
atomic absorption

Nitric acid
digestion; erio-
chrome cyanine-R
colorimetric

Nitric acid
digestion; carbon
rod atomic
absorption	
APHA (1975)
Part 424


APHA (1975)
Part 403   ,

APHA (1975)
Part 208D

Oceanography
International
  (1978)


APHA (1975)
Part 425F

Scheiner (1975)
HACH Cheimical Co.
  (1975)


APHA (1975)
Part 507
EPA (1976)
APHA (1975)
Part 302B
EPA (1976)
                                     20

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of the filtered extract.

     The forms of particulate phosphorus which are extractable by a variety
of solutions including 0.1 N NaOH have been discussed by several workers;
for example, Armstrong et al. (1971), Cowen and Lee (1976), and Williams
et al. (1971).  These investigators have indicated that the phosphorus
removed from particulate matter by 0.1 N NaOH consists of inorganic and
organic phosphorus which is bound by a gelatinous matrix consisting of
colloidal organics a-nd amorphous oxides and hydroxides of iron and aluminum
which coat the surfaces of the particulate.  Studies by Sagher (1976) and
Wildung et al. (1977).have indicated the inorganic component of the NaOH-
extractable particulate phosphorus to be that which is most readily available
to algae.  Inasmuch as the particulates of interest in the present investi-
gation were from municipal wastewaters and, thus, contained relatively
labile organic phosphorus, it was decided to measure the total particulate
phosphorus extractable by NaOH for comparison with bioassay tests of
particulate phosphorus availability to algae.

     Organic contaminants (PCB's and chlorinated pesticides) measured by
O'Brien and Sere were determined by hexane extraction followed by gas
chromatography with electron capture detection.
                                      21

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                                  SECTION 5

          RESULTS OF SURVEY AND PHOSPHORUS LOADINGS  TO  LOWER  LAKES
 INTRODUCTION

      In  order to  evaulate  present  conditions  regarding phosphorus loadings
 and treatment removal  strategies in  the  lower Great Lakes Basins, a survey
 was conducted of  all municipal  treatment plants with flows greater than 1
 mgd (3785 nr/day)  in the drainage  basins of Lakes Erie and Ontario.
 Originally,  a list of  plants was put together as a mailing list for a
 questionnaire.  The mailing list for the questionnaire was compiled from
 lists  provided  by  the  following agencies: 1)  IJC, 2) Ontario Ministry of the
 Environment,  3) Great  Lakes Basin  Commission  and 4) New York State Department
 of  Environmental Conservation.  The  following information was requested from
 each of  the wastewater treatment plants:
     1)
     2)
     3)
     5
     6)
treatment plant name and address
type of plant
average daily flow and design flow
method of phosphorus removal
influent and effluent phosphorus concentrations
chemical dosages for phosphorus removal
A copy of the questionnaire and cover letter is presented in Appendix A.

     The questionnaire information was checked and supplemented with
additional data from the same agencies used for compiling the mailing list.
Finally, the data were transferred to work sheets, a copy of which is shown
in Appendix A.

     The questionnaires served as the major source of information for the
survey.  Originally 268 were mailed to plants in the lower lakes basins.
Five turned out to be duplicates, thus 263 plants were covered in the
mailing.  The number of responses received was 154.  Supplemental information
was then collected for the plants which did not respond, as well as for
verification of the respondents.   A recent IJC report (July 1979) and other
sources (NYS Dept. of EnCon, 1979; IJC, 1977; Ontario Ministry of the
Environment, 1977) were used for verification and augmentation of question-
naire data.

     A master list of the treatment plants in the lower Great Lakes Basins
is presented in Table 4.   The breakdown of the number of plants by drainage
basin and country is detailed in  Table 5.   Note that 229 plants are included
in the master list.  The  final  number is less than the 263 questionnaires

                                     22                               '

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TABLE 5.  NUMBER OF PLANTS IN SURVEY

Lake Ontario
New York
Ontario
Lake Erie
New York
Pennsylvania
Indiana
Michigan
Ohio
Ontario
48
43
91
10
1
3
23
69
32
138
U.S. 48
Canada 43
U.S. 106
Canada 32




                       Totals:   U.S.
154
                                Canada    75
                                      .  229
                  36

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mailed out.  A number of plants, 48, were removed from the list for one of
several reasons.  Among these were: 1) the plants were abandoned; 2) the
plants were not actually in the lower lakes basins (i.e. were discharging
into the St. Lawrence River or Huron basin); and 3) the flows were less than
1 mgd (3785,m3/d).  Data from questionnaires received from plants with actual
flows less than the 1 mgd limit were not discarded, and the plants were
included on the master list.  This was done in order to keep the information
regarding phosphorus removal strategies for subsequent analysis.  Finally,
14 plants were later added to the list after the initial mailing.  Thus, 229
plants are included on the master list.

     Where more than one source of data existed for one plant, priority was
given to the questionnaire data.  The 1979 UC report was then used for
plants with no questionnaire data, if the data were available from the
report.  Finally for plants on-the .list for which neither the questionnaire
nor the IJC report contained data, the other sources listed above were used.

TREATMENT APPROACHES FOR PHOSPHORUS REMOVAL

     Based on the results of the questionnaire, the treatment approaches for
phosphorus removal at wastewater plants in the Great., Lakes vicinity can be
listed.  One hundred and four plants indicated that phosphorus removal was
being practiced at the present time, while 30 indicated that phosphorus
removal was not practiced.  An additional 20 plants were eliminated from
those who responded due to their location or abandonment.  Thus, from the
questionnaire responses approximately 80 percent of the plants used for the
survey practiced phosphorus removal.

     A summary of the major chemicals used for phosphorus removal and their
point of addition in the treatment process (i.e. primary, secondary or
tertiary) is shown in Table 6.  Of the 104 plants practicing phosphorus
removal, 53 used an iron salt (one more than shown in Table 6 as one
respondent listed iron but did not specify where), 49 used an aluminum salt,
and only two used lime.  One plant used both iron and alum.  A comparison of
frequency of the precipitation cation used (aluminum or iron) by country is
shown in Table 7.  In comparison, Fe or Al are used with about the same
frequency.  Lime is now seldom used based on our survey.  In regard to point
of treatment, the data are summarized in Table 8.

     From Table 6, it can be seen that approaches for phosphorus removal
include aluminum addition to the secondary process, iron addition to primary,
and iron addition to secondary processes, in order of decreasing frequency
of use.

PHOSPHORUS REMOVAL'DATA

Frequency of Phosphorus Effluent Concentrations

     Based on the master list developed from our survey (Table 4), a
frequency distribution was developed for 30-day average effluent phosphorus
concentrations in the lower lakes basins.  This distribution is summarized
in Table 9 and illustrated in Figure 7.  Of the plants in Table 4 that
                                     37

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           TABLE 6.  TREATMENT APPROACHES BY CHEMICAL
                     (PRECIPITATION CATION) AND LOCATION

Number of Plants

Primary
Secondary
Tertiary
Total

Al
1
26
2
29
U.S
Fe
16
6
2
24
Canada
Total
17
32
4
53
Al
2 -
17
1
20
Fe.
20
8
0
28
Total
22
25
1
48
Al
3
43
3
49
Total
Fe
36
14
2
52
Total
39
57
5
101

      TABLE 7.  FREQUENCY OF PRECIPITATION CATION USAGE


Metal
Al
Fe
Lime

U.S.
54
44
2
Percent
Canada
41
57
2'

Total
48
1 50
2

TABLE 8.  SUMMARY OF LOCATION OF PHOSPHORUS REMOVAL TREATMENT
          IN THE TREATMENT PLANT PROCESS

Process
Locati on
Primary
Secondary
Tertiary

U.S.
32
60
8
Percent
Canada
46
52
2

Total
39
56
5
                               38

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       TABLE  9.   FREQUENCY OF  30-DAY AVERAGE  EFFLUENT  PHOSPHORUS
                 CONCENTRATIONS  - mg/L AS  TOTAL  P
Range of TP,
mg. P/L
06.0

U.S.
14
39
21
10
6
TO.
6
2
6
6
3
4
12
Number of Plants"
Canada
5
54
8
4
2
0
1
0
0
0
1
0
0

Total
19
93
29
14
8
10
7
2
6
6
4
4
12
214

*Phosphorus effluent data were not available for 7 plants in the
 Erie basin and 8 plants in the Ontario basin
                                    39

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listed effluent P, 9 percent have an effluent TP concentration _< 0.5 mg P/L
and 52 percent are <. 1.0 mg P/L.  The distribution of these plants by size
and lake basin is given in Table 10.  Currently, 62 plants in the Lake Erie
basins (47 percent) do not meet a 1.0 mg P/L effluent phosphorus standard,
while 40 plants in the Lake Ontario basin (48 percent) are failing to meet
the standard.  There does not appear to be any major trends by plants size
in the fraction meeting a 1.0 mg P/L standard; however, plants in the 10 to
50 range seem to be doing comparatively better than the others.

     Whether required or not, there are 19 plants in the basins currently
meeting a 0.5 mg P/L standard.  We received a questionnaire response, and
therefore have treatment approach information, on 14 of these 19 plants.  It
is especially interesting to note that only 2 of the 14 plants are currently
employing any tertiary treatment processes.  Seven of the plants use FeCls
(some also use a polymer) or pickle liquor at some point in the treatment
process; four of the plants use alum; and three plants claim to achieve
0.5 mg P/L with no chemical addition simply because the influent phosphorus
is low (1-2 mg P/L).

Frequency of Percentage Removal Achieved

     In order to get some feel for what percentage removals are currently
needed to meet todays effluent phosphorus standards, a frequency distri-
bution of removal percentage was prepared from our questionnaire data.  These
results are presented in Table 11 and in Figure 8.  Note that only 117 plants
made up the sample for this distribution, since both influent and effluent
data were necessary to compile removal percentages.  Recall that approxi-
mately 80 percent of the respondents to the survey were practicing phosphorus
removal, yet only 63 percent of those reporting influent and effluent
phosphorus levels were achieving 80 percent removal of total phosphorus
through the plant.  Virtually all (96 percent) of the plants which reported
removals of 80 percent or more of influent phosphorus were using iron or
aluminum for precipitation during treatment.  Only 68 percent of all the
plants which employed chemicals for phosphorus removal, however, were
achieving percent removals of 80 or better.  This result suggests two possi-
bilities: either the treatment plants do not generally have to remove 80
percent of the phosphorus to meet 1.0 mg P/L effluent concentration, or there
is room for  improvement in many plants as far as phosphorus removal
efficiency is concerned.  Since 47  percent of the plants are failing to meet
1.0 mg P/L,  it seems likely that the latter case is most prevalent.

     According to our questionnaire the mean  influent phosphorus concen-
tration to plants  in the  lower  lakes is 6.3 mg  P/L.  This means that on the
average 84 percent TP reduction through plant would be necessary to achieve
a  1.0 mg P/L effluent standard and  92 percent TP reduction would be necessary
to achieve a 0.5 mg P/L effluent concentration.

PHOSPHORUS LOADING TO THE LOWER LAKES     ,

      Based on the  survey  results, current loadings of total phosphorus  from
municipal point  sources are presented in Table  12.  Additionally, Table 12
contains projected  phosphorus  loadings which would result  if all plants
                                     41

-------
        TABLE  30.   DISTRIBUTION  OF  PLANTS  BY SIZE AND BASIN REACHING
                   1.0  and  0.5 mg P/L TOTAL PHOSPHORUS EFFLUENT
                   CONCENTRATIONS
Plant Size
(mgd)*

<1
1-<10
10-<50
50-<100
>100

1
1-<10
10-<50
50-<100
>100
No. of Plants
in Size Range**

12
94
18
5
2
Total 1ST

5
60
11
4
3
Total 83
Plants Meeting
1.0 mg P/L Standard
Lake Erie
6
47
14
1
1
69
Lake Ontario
3
29
8
1
2
43
Plants Meeting
; 0.5 mg P/L Standard

0
8
, 3
0
0
TT
.
2
5
1
0
0
B
*  1.0 mgd = 3,785 m/d

** Phosphorus effluent data were not available for 7 plants in the Erie
   basin and 8 plants in the Ontario basin
                                    42

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TABLE 11.  FREQUENCY OF PERCENT PHOSPHORUS REMOVAL
           ACHIEVED (BASED ON TOTAL PHOSPHORUS;
           DATA FROM QUESTIONNAIRE)
Range, Percent
0-<10
10-<20
20-<30 .
30-<40
40-<50
50-<60
60-<70
70-<80
80-<90
90-100

U.S.
6
1
1
3 '
4
10
8
7
17
9
Number of Plants
Canada
0
0
0
0
0
3
2
, 4
28
14

Total
6
1
1
3
4
13
10,
11
45
23
                                                         117
                          43

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   TABLE  12.   PRESENT AND  PROJECTED MUNICIPAL  POINT SOURCE PHOSPHORUS
               LOADINGS TO  THE  LOWER GREAT  LAKES  -  IN METRIC TONS/YEAR
Lake Ontario
New York
Ontario
Lake Erie
New York
Pennsylvania
Ohio
Indiana
Michigan
Ontario
Total
Present Loading*
1973
885
2858
64
112
1812
23
2312
232
4555
7413
Projected
1.0 mg/L
783
625
1408
33
80
705
23
1356
193
2390
3798
Loadings
0.5 mg/L
406
367
773
18
40
395
23
701
114
1 991
2064
* For all plants above 1  mgd (3,785 m /d)
                                     45

-------
 which presently exceed 1.0 or 0.5  mg  P/L  effluent  concentrations were to
 achieve the respective levels.   All calculations were  based on  loads reported
 on the master list,  Table 4,  and assume that  phosphorus acts conservatively
 between the points of effluent  discharge  and  entry to  the  lakes.  The data
 in Table 12 indicate that should all  plants larger than 1  mgd  (3785 m3/d)
 achieve the level of 1.0  mg P/L, the  municipal  loads would be reduced to 52
 and 49 percent of their present values for Lakes Erie  and  Ontario,
 respectively.   Achievement of 0.5  mg  P/L  in final  effluents for these plants
 would reduce municipal  loads  to 28 and 27 percent  of present values for the
 two lakes.

      The magnitude of municipal  load  reductions may be placed in perspective
 by comparison  to other sources  of  phosphorus  to the lower  Great Lakes.  The
 present municipal loading data  are presented  with  data on  loads from other
 sources of  phosphorus  to  Lakes  Erie and Ontario and combined to give total
 phosphorus  loads to  the lakes in Table 13.  These  data indicate that
 municiapl point sources account for 27 and 21 percent of the present total
 phosphorus  load to Lakes  Erie and  Ontario, respectively.   The effect of
 municipal load reductions  on total phosphorus loads, as a  result of all
 wastewater  treatment plants larger than 1  mgd (3785 m3/d)  achieving 1.0 and
 0.5 mg  P/L  in  the basins  of the two lakes, is illustrated  in Figure 9.
 Effluent standards of  1.0  and 0.5  mg  P/L would represent total load
 reductions  of  13 and 19 percent, while for Lake Ontario, the same standards
 would represent reductions  in the  total phosphorus load of 11  and 15 percent.

      It should  be noted that the load reductions shown in Figure 9 for Lake
 Ontario  do  not  account for reductions in the load from Lake Erie to Lake
 Ontario  by  way  of the Niagara River.   Such a load reduction would be a
 likely  result  should all wastewater plants in the Lake Erie basin achieve
 1.0 or  0.5  mg P/L effluent levels.   Therefore, the above Lake  Ontario load
 reductions  are minimum values and would probably be larger as  a result of
 reductions  in the relatively large phosphorus load from the Niagara River.
 In any event, a major conclusion derived from Figure 9 is  that a .0.5 mg  P/L
 effluent standard alone will not allow the attainment of IJC target loads of
 11,000 and  7,000 metric tons/year for Lakes Erie and Ontario,  respectively.
The total load to Lake Erie under a 0.5 mg P/L standard would  be reduced to
approximately 13,670 metric tons/year.  The total  load to  Lake Ontario would
be reduced at least to 11,515 metric  tons/year;  however,  it is  unlikely  that
a 4000 metric ton/year reduction (70  percent)  would occur  in the Niagara
River to bring the Lake Ontario load  down  to  7000 metric  tons/year.
                                     46

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          TABLE 13.  PHOSPHORUS LOADING JO LAKES ERIE AND
                     ONTARIO, IN METRIC TONS/YEAR

Lake Erie

Point Sources
Municipal
2
Industrial
U.S.

4323
211
Canada

232
38
Total

4555
249
Lake Ontario
U.S.

1973
81
Canada

885
120
Total

2858
201
Upper Lake


Niagara River
 (Lake Erie)3


Detroit River
 (Lake Huron)3


Non-Point Sources


Di ffuse/Tri butary"

             3
Direct Runoff

           4
Atmospheric
 6156


 1576
1804


 740
1080





7960


2315


 744
2123


 975
1131


 261
                                        5613
3254


1236


 438
Total
12266
2814  ,16934   5152
               2937   13600
1
 Present loading conditions as computed from survey master list

'Computed from IJC - (1979).

 Computed from Vallentyne and Thomas (1978).
i
 Computed from Gregor and Johnson (1979).
                                 47

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                                 SECTION 6

                         RESULTS OF FIELD STUDIES
WASTEWATER TREATMENT PLANT DESCRIPTIONS

     Given below are general descriptions of the treatment methods employed
at the four wastewater plants which were .studied intensively on-site during
this investigation.  Included in the descriptions are the approaches used
for preliminary, primary, secondary, and tertiary wastewater treatment, and
sludge treatment and" disposal.

Gates-Chili-Ogden, 15 -mgd (56775 m3/d)

     At the Gates-Chili-Ogden facility, located near Rochester, NY, raw
municipal wastewater was given preliminary and primary treatment prior to
biological treatment by a conventional activated sludge process.  To remove
phosphorus, alum was added in liquid form to the effluent of the aeration
basin, upstream from the final clarifiers as illustrated in the process
schematic (Figure 10).  The secondary sludge, which consisted of biological
and aluminum-phosphorus solids1, was partially recycled to the aeration basin
and partially wasted.  By recycling alum with the return activated sludge,
the contact period between alum and phosphorus in the wastewater was
increased, which would permit kinetically-limited precipitation reactions to
approach equilibrium more closely than could occur without alum recycle.
Waste secondary sludge was conditioned for flotation thickening with a
polymer and combined after thickening with primary sludge.  The combined
sludges were dewatered by vacuum filtration and incinerated or composted
on-site.               -

Frank Van Lare.,! 100 mgd (378500 m3/d)

     Municipal wastewater treatment, at the Frank Van Lare plant, located
near Rochester, NY, consisted of two main treatment streams, as shown in the
process schematic,-;Figure 11.  Raw wastewater received preliminary screening
and degritting and was then split for primary sedimentation and further
treatment.  To 20 percent of the total flow, liquid alum and a polymer was
added just upstream from the primary clarifiers to enhance phosphorus
removal during primary sedimentation.  The remainder of the flow was given
primary treatment, without alum addition, and biological treatment by
conventional activated sludge.  The clarified secondary effluent and alum-
treated primary effluent were combined for chlorination prior to discharge.
The primary sludges from both treatment streams were combined with wasted
biological sludge for treatment by gravity thickening, vacuum filtration,
and incineration.

                                     49

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Big Sister Creek, 3 mgd (11355 m3/d)

     The Big Sister Creek wastewater treatment plant, located near Angola,
NY, was upgraded in 1978 from a primary treatment facility to a.tertiary
treatment system.  As shown in the process schematic for the Big Sister
Creek plant, Figure 12, screened and degritted raw wastewater was sent with-
out primary sedimentation to an aeration basin for biological treatment by
an extended aeration activated sludge process.  Effluent from the aeration
basin is clarified by sedimentation and then dosed with ferric chloride and
a polymer for phosphorus removal in a solids contact clarifies  Effluent
from the solids contact clarifier is applied to a sand filter after which
the filtrate is chlorinated for discharge.  A portion of the iron-phosphorus
sludge from the solids contact clarifier is recycled back to the clarifier
influent.  The sludge recycle provides an increased contact period between
iron and wastewater phosphorus, which permits a closer approach to precipi-
tation equilibria, than would occur in the absence of solids recycle.  Both
secondary and iron-phosphorus sludges were thickened by flotation and
combined for storage in an aerobic digester.  Centrifugation and sand bed
drying were employed for sludge dewatering.  Dewatered sludge was trucked to
an adjacent land fill for disposal.,

Ely. 1 mgd (3785 m3/d)                                                 ,

     As illustrated in the process schematic for the Ely, MN wastewater
treatment plant, Figure 13, screened and degritted raw wastewater was given
primary settling before biological treatment, which consisted of a single-
stage trickling filter.  Liquid alum and a polymer were added to the trick-
ling filter effluent to enhance phosphorus removal during secondary
clarification.  All biological solids and alum-phosphate sludge which
collected in the final clarifiers was recycled to the influent of the primary
sedimentation tanks, which served to increase the time of contact between the
alum, wastewater solids, and phosphorus.  The secondary effluent was
chlorinated, held briefly in non-functional solids contact tanks, and passed
through a dual media filter prior to discharge from the plant.  Sludge from
the primary clarifier was thickened by gravity and conditioned with lime
prior to vacuum filtration.  A landfill was used for disposal of the vacuum
filter cake.

TREATMENT PLANT MONITORING

     The performance of the four wastewater plants was determined by repeated
sampling at fixed points along the treatment stream at each plant and
characterizing the progress of treatment at each selected point.  Presented
in Table 14 is a listing of the sampling locations which were selected at
each wastewater plant.  A brief description of each location is included to
specify the exact sampling point.

     Though several treatment parameters were determined on the samples taken
from each sampling location, special focus was given to the analysis of
phosphorus and various fractions of phosphorus through the treatment plants.
Additionally, a subset of samples from each plant was analyzed for selected
heavy metal and organic priority pollutants, in order to assess the

                                     52

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      TABLE 14.   SAMPLING LOCATIONS WITHIN MONITORED TREATMENT PLANTS
   Plant Name
Sampling Location Name    Location Characteristics
Gates-Chi1i-Ogden
Frank Van Lare
Big Sister Creek
Ely
  Raw Influent

  Primary Effluent

  Secondary Effluent


  Raw Influent

  Alum Effluent


  Biological Effluent


  Raw Influent

  Secondary Effluent

  Filtered Effluent


  Raw Effluent

  Secondary Effluent

  Filtered Effluent
Sample taken from aerated grit
chamber
Sample taken from weir of
primary clarifier
Sample taken from weir of
final clarifier

Sample taken from aerated grit
chamber
Sample taken from weir of
primary clarifier after alum
treatment
Sample taken from weir of
final clarifier

Sample taken from post-
screening wet well
Sample taken from weir of
secondary clarifier
Sample taken from sand
filter effluent channel

Sample taken from aerated grit
chamber
Sample taken from weir of
secondary clarifier
Sample taken from dual media
filter effluent channel
                                     55

-------
 effectiveness of the differing treatment methods  of the wastewater plants  on
 such pollutants.

 Overall  Treatment Performance

      Presented in Table 15  is a summary of data collected  at  the  four  treat-
 ment plants  on biochemical  oxygen  demand (BODs),  chemical  oxygen  demand
 (COD),  suspended  solids (SS), total  phosphorus  (Total  P),  total Kjeldahl
 nitrogen (TKN),  and total nitrogen (Total  N), the latter of which was
 estimated from the sum of TKN and  nitrate  plus nitrite nitrogen.   A complete
 listing  of the data summarized in  Table 15 is given  in Appendix C.   Also
 given in Table 15 are figures for  overall  percent removals of the listed
 parameters for each wastewater,, pi ant.

      At  the  Gates-Chili-Ogden plant  sampling focused on the raw influent and
 final effluent.   Data on three samples  of  primary effluent are included in
 Appendix C.   The  data in Table 15  demonstrate removal  percentages  on the
 order of 90  percent for conventional treatment parameters  including Total  P,
 during the periods of sampling,  and  indicate a well designed  and  operated
 wastewater plant.

      The Frank Van Lare plant,  during the  monitoring period for this investi-
 gation,  was  less  efficient  than  the  other  plants  at removing  common waste-
 water pollutants,  as  indicated  by  the data in Table 15.  Removal  of BODs .and
 COD  through  the biological  treatment stream averaged over 80  percent, while
 through  the  primary by-pass stream,  removal of the two  pollutants  averaged
 29 and 47 percent,  respectively.   Removal  of total P and suspended  solids "
 appeared equally  effective  through either  biological or primary +  alum
 treatment, with approximately 60 and 70  percent removal of the two pollutants
 by either method.   The  effectiveness of  the Frank Van  Lare plant  for
 pollutant removal  is  indicated by  the overall percentages given in  Table 15.
 The  overall  percentage  removals were calculated on the  basis  of an  80/20
 percent  split  of  the  raw influent  between  biological and primary +  alum
 treatment.

      Performance  data for the Big Sister Creek wastewater plant, Table 15,
 show excellent treatment efficiency for  BOD, COD,  and suspended solids, with
 greater  than 93 percent reductions in each pollutant through  the plant.
 Additionally,  the  total N concentration was reduced by nearly 60 percent
 through  the  plant  and the final effluent total  N was predominately nitrate
 (approximately 97  percent), an expected  benefit of the extended aeration
 process.  The  total P content of the wastewater was reduced by an  average of
 86 percent during  treatment, though at intermediate stages of treatment the
 removal   of total  P was significantly greater than  this figure.  A  more
 detailed assessment of phosphorus removal performance will  be given in the
 next section.

     As   the data  in Table 15 indicate,  the Ely wastewater treatment plant
 performed well for removal  of BOD,  total P, -and suspended solids,  each of
which was reduced by greater than 85 percent during treatment.  Removal of
 COD was   less effective at 75 percent, than removal of BOD,  and the final
 effluent from  the plant was not nitrified with  approximately 63 percent of

                                     56

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 the influent TKN remaining.

 Phosphorus Removal

      Presented i.n Table 16 is a summary of the data collected on phosphorus
 during the investigation.   A more detailed presentation of phosphorus data
 may be found in Appendix C.   Given in Table 16 is a listing,  by plant and
 sampling locations within each plant, of the average total phosphorus con-
 centration and concentration of several fractions of the total phosphorus in
 the wastewater.  Statistical distribution parameters for each group of
 samples are given, also.

 Gates-Chili-Ogden--

      Removal of phosphorus at the Gates-Chili-Ogden plant is  illustrated in
 Figure 14, which gives the concentrations of total phosphorus and several
 fractions of particulate and soluble phosphorus in the raw wastewater and in
 the final effluent before chlorination.  As the data in Figure 14 indicate,
 addition of alum to the biological effluent before secondary  clarification,
 as practiced at the Gates-Chili-Ogden plant, resulted in a reduction in the
 concentration of all the fractions of phosphorus for which samples of final
 effluent were analyzed.  However, the relative amount of particulate
 phosphorus  increased during treatment, as shown in Figure 15.,  This change
 in the relative distribution of the phosphorus fractions illustrates that
 soluble phosphorus was  removed more efficiently (greater than 90 percent
 removal) than particulate phosphorus (approximately 80 percent removal), by
 the treatment approach  employed at the Gates-Chili-Ogden plant.  In'addition
 to the increased level  of particulate phosphorus, as a fraction of the total
 phosphorus  which remained after treatment, an increase was noted in the
 relative contribution of NaOH  extractable phosphorus to the total particulate
 phosphorus  which remained,  as  shown  in Figure 15.

 Frank Van Lare--

      Removal of phosphorus  at  the Frank Van Lare wastewater plant is
 illustrated in  Figure  16, which shows  concentrations of total phosphorus and
 phosphorus  fractions  in the raw wastewater, the alum-treated  effluent, and
 the biologically-treated effluent.   It is apparent from the data that
 biological  and  physical-chemical treatment with alum were nearly equal in
 reducing  the total  phosphorus  content  of  the wastewater during the sampling
 periods  of  this  investigation.  The  figures given  in Table 16  indicate that
 both  biological  and "physical-chemical  treatment reduced the total phosphorus
 content  of  the  wastewater  by similar amounts  , 60  and  66  percent,
 respectively.   Additionally,  both treatment streams were  more effective  at
 reducing the  soluble  phosphorus  fraction  than that of  particulate phosphorus.
 Approximately  70  percent  of the  total  soluble phosphorus  of the  raw  influent
 was removed through the biological treatment  stream while nearly 90  percent
 of that  fraction  was  removed during  alum  treatment.  Thus, alum  was  more
 effective than biological  treatment  for  reducing  the soluble  phosphorus  of
 the wastewater.   Particulate phosphorus  removal was similar through  the  two
 treatment streams  and averaged approximately  50  percent of the  raw waste-
* water particulate phosphorus.   The  levels of  total  NaOH extractable

                                      59

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                    GATES-CHILI-OGDEN
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        TP  TPR NaOH-P TSP  SRP

           RAW INFLUENT
TP  TPP NaOH-P TSP SRP

   FINAL EFFLUENT
       Figure 14. Mean  concentrations; of total  phosphorus  and
                 phosphorus fractions at the Gates-Chili-Ogden
                 plant
                              6/ 2

-------
                 GATES-CHILI -OGDEN
i PARTICIPATE



NaOH
Extractable
h SOLUBLE


Soluble
Reactive
Raw Influent, Total P* 6,28 mg P/L



, NaOH
Extractable
L OUUUDUt.
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Soluble
Reactive
Final Effluent, Total P=0.75/mgP/L
           20         40          60          80

             Percent of  Total Phosphorus
100
Figure 15. Distribution of phosphorus fractions  at the Gates-
          Chili -Ogden plant
                           63

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particulate phosphorus followed closely those of total participate phosphorus
in both treatment systems.
                                               /
     As indicated previously, soluble phosphorus was removed more effectively
than particulate phosphorus in the Frank Van Lare plant.  The differential
removal of these two fractions resulted in the phosphorus fraction distri-
butions shown in Figure 17 for the raw influent, alum and biological ,
effluents at the Van Lare wastewater plant.  It is -apparent from Figure 16
that particulate phosphorus, predominantly the total NaOH extractable
fraction, was the main component of the phosphorus which remained in the
treated wastewater, whether treatment was given through the biological or
alum-treated stream.  Moreover, a greater portion of the total particulate
phosphorus which remained after alum treatment could be extracted with NaOH,
as compared to the particulate phosphorus in the biological effluent.

Big' Sister Creek--

     The performance of the Big Sister Creek wastewater plant for removal of
phosphorus is presented in Table 16 and illustrated in Figure 18 for fixed
sampling points along the treatment stream.  Figure 18 shows a large
reduction in total raw wastewater phosphorus from biological treatment alorie,
due almost exclusively to removal of particulate phosphorus.  The effluent
from the secondary clarifier averaged 0.17 mg P/L of total particulate
pho,sphorus, compared with 4.40 mg P/L in the raw wastewater, while the total
soluble phosphorus concentration averaged 2.13 and 2.15 mg P/L on samples J'?
taken from the two locations.  The effectiveness.of iron for further
phosphorus removal can be seen from the data in Figure 18 for the phosphorus
in the effluent of the solids contact clarifier.  The data indicate that  vr
iron precipitation reduced the total soluble phosphorus from 2.13 mg P/L in :
the secondary effluent, to 0.16 mg P/L, a reduction of 92 percent.  The   -*
increased concentration of phosphorus observed in the filtered effluent,
after iron precipitation, was due to routing of a portion of the secondary
effluent around the,sol ids contact clarifier for mixing with the iron
treated effluent downstream from the clarifier and application to the sand
filters.

     As illustrated in Figure 19 the distribution of the phosphorus
fractions relative to the total phosphorus changes dramatically during
treatment.  In the raw wastewater, particulate phosphorus, predominately
extractable by NaOH, represented nearly 65 percent of the total phosphorus,
while the remaining soluble phosphorus was principally soluble reactive
phosphorus.  However, after biological treatment and clarification, the
particulate phosphorus fraction was reduced greatly, and soluble reactive
phosphorus comprised approximately 80 percent of the total phosphorus whi^ch
remained.  After iron treatment, the low concentration of phosphorus which
remained occurred mainly as NaOH extractable particulate and soluble re-   •
active phosphorus.  Finally, as the flows were recombined and sent to the
sand filters, the filtered effluent contained phosphorus fractions which-
were similar to the clarified biological effluent, with soluble reactive
phosphorus as the main component.
                                     65

-------
                   FRANK  VAN  LARE
             PARTICULATE
                      SOLUBLE

NaOH
Extractable

Soluble
Reactive
Raw  Influent,  Total P = 3.81 mg P/L
                PARTICULATE
                        SOLUBLE

NaOH
Extractable

Soluble
Reactive
Biological Effluent, Total P= 1.52 mg P/L
                    PARTICULATE
Alum Effluent, Total P= l.3lmgP/L
                                               SOLUBLE

NaOH
Extractable

          20
4O
60
80
100
             Percent  of Total  Phosphorus
 Figure 17.  Distribution of phosphorus  fractions  at the Frank
           Van Lare plant
                          66

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BIG SISTER CREEK
PARTICULATE . .. SOLUBLE _


NaOH
Extractable


Soluble
Reactive
Raw Influent, Total P = 6.81 mg P/L

 V-PARTICULATE
                            SOLUBLE

X
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.Soluble Reative
Secondary Effluent, Total P=2.27 mg P/L
PARTICULATE M

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Extractable
SOLUBLE



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Solids Contact, Total P= 0.35 mg P/L


 v-PARTICULATE            	„,
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Soluble Reative

Final Effluent, Total P= 0.94 mg P/L
 1
20
60
                                              80
100
               Percent  of Total  Phosphorus
 Figure 19.  Distribution of phosphorus  fractions at the Big
            Sister  Creek plant

                             68

-------
 Ely--                                   '

      Data  on  phosphorus  removal  through .the Ely,wastewater treatment plant
 are  presented in  Table  16  and illustrated  in Figure  20.   Figure  20 indicates
 significant reduction of total wastewater  phosphorus occurred  both as a
 result of  alum addition  to the trickling filter effluent,  and  as a result of
 dual  media filtration.   As Figure  20 illustrates,  alum precipitation was
 much  more  efficient at  reducing  the soluble rather than the particulate
 fraction of the total ^aw  wastewater phosphorus.   Removal  of the total
 particulate fraction averaged 33 percent from the  raw influent to  the clari-
 fied,  alum-treated biological effluent, compared to  98 percent removal for
 the total soluble  fraction.  Through the dual  media filter, the extremly  low
 concentrations of soluble  phosphorus did not change, while the'total  partial--
 late  fraction was reduced  to 20  percent of the raw wastewater  particulate
 phosphorus.                            	"    ""	" '

      An examination of  the distribution of fractions of total  phosphorus
 .through the plant shows  the approach to treatment  at Ely favored removal  of
 phosphorus from the soluble fraction to the extent that over 90  percent  of
 the  total  phosphorus which remained in the wastewater after.alum treatment
 or filtration occurred  as  particulate phosphorus "(Figure 21).'  'Additionally,
 the  NaOH extractable fraction of the total-"parti cul ate' phosphorus  was an
 increasingly  predominant component of that fraction, relative  to the total
 phosphorus that remained in the  wastewater at the  stages of treatment which
 were  sampled.           :          -  ,->

 Priority Pollutants  .

      During the investigation infrequent samples were taken from the1
 locations  given in Table 14 for  analysis of the priority pollutants: nickel,
,zinc,  cadmium, total polychlorinated biphenyl (PCB), and total chlorinated
 hydrocarbon pesticides  (CHP). The results, of these  analyses.are presented
 in Table 17.   These determinations were made to gauge the possibility that
 removal techniques for  control of phosphorus to defined levels might offer
 side  benefits of  enhanced  removal  of other pollutants.

 Toxic Heavy Metals--

      No trend was noted  to suggest removal  of nickel or cadmium through  the
 four treatment plants which were monitored.  However, as indicated by the
 data  in Table 17, reductions in  total zinc concentrations from the levels
 found .in the  raw  influent  samples  were noted at all  four plants, and the
 lowest concentrations of total zinc were found in  samples taken from
 filtered effluents.

 Organic Pollutants--

      None  of  the  samples which were analyzed for organic pollutants contained
 measurable concentrations  of PCB.   However, samples  from three of the four
 plants contained  quantifiable levels of  CHP.  The  pesticide, p-p-DDT, was
 determined at 0.2 yg/L  in  the raw influent to the  Gates-Chili-Ogden plant.
 Additionally, aldrin was found at 0.09 yg/L in the filtered effluent from

                                      69

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                             ELY



NaOH
Extractable



Soluble
Reactive
 Raw  Influent, Total P = 3.77 mg P/L
                       PARTICULATE
 Secondary Effluent, Total P = 1.72  mg P/L
                      PARTICULATE
                                                    SOLUBLE

NaOH
Extractable

                                                    SOLUBLE-
                          NaOH
                       Extractable
  Final Effluent, Total P=0.56 mg P/L
; o
IOO
             20         40         60          80
                Percent of Total  Phosphorus

Figure  21. Distribution of  phosphorus fractions  at the Ely plant
                              71

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        TABLE  17.   CONCENTRATIONS  OF  PRIORITY  POLLUTANTS  IN WASTEWATER
                   SAMPLES  FROM  MONITORED  TREATMENT  PLANTS
Plant Name and
Sampling Location
Gates-Chili-Ogden
Raw Influent
Primary Effluent
Secondary Effluent
Heavy Metals*
Ni
(mg/L)
0.09(2)
0.08(2)
0.08(2)
In
(mg/L)
0.11(2)
0.05(2)
0.05(2)
Cd
'(yg/L)
2.2(2)
2.8(2)
<0.5(2)
Organics**
PCB
(yg/L)
<0.1
<0.01
CHP
(yg/L)
0.2(p-p-DDT)
<0.01
 Frank Van Lare
 Raw Influent
 Alum Effluent
 Biological  Effluent

 Big Sister Creek
 Raw Influent
 Secondary Effluent
 Filtered Effluent

 Ely
 Raw Influent
 Secondary Effluent
 Filtered Effluent
0.02(3)   0.15(3)      2.1(3)   <0.03
0.02(3)   0.09(3)       ***     <0.01
0.02(3)   0.06(3)      3.3(3)   <0.01
0.06(2)   0.21(2)     <0.5(2)   <0.01
0.06(2)   0.02(2)     <0.5(2)   <0.01
0.07(2)  <0.018(2)    <0.5(2)   <0.01
0.04(3)   0,08(3)     <0.5(3)   <0.01
0.02(3)   0.03(3)     <0.5(3)   <0.01
0.02(3)   0.02(3)     <0.5(3)   <0.01
 0.26(Aldrin)
 0.14(Aldrin)
<0.01
<0.01
<0.01
<0.01
<0.01
<0.01
 0.09(Aldrin)
  * Number in parentheses indicates the number of samples analyzed.
    Detection limits for the metals were: 0.02 mg Ni/L, 0.5 yg-Cd/L,
    and 0.018 mg In/I.

 ** Concentration of organics which were too low for quantification are
    reported as less than (<) the analytical limit for the methods used.
    Specifically quantified pesticides are given in parentheses.

*** Samples lost
                                      72

-------
the Ely plant and in both the raw and alum-treated primary effluent at the
Frank Van Lare plant.  The relative magnitude of the concentrations measured
in the Van Lare samples., 0.26 ug/L in the raw influent, 0.14 yg/L in the
primary effluent, and < 0.01 yg/L in the biological effluent, suggests that
aldrin was removed during both physical-chemical and biological  treatment of
wastewater.  However, the number of samples which contained measurable
concentrations of any anal ate pesticide was inadequate to permit substantive
conclusions regarding removal during treatment at the plants investigated.
                                     73

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                                 SECTION 7

                    STUDIES ON BIOLOGICAL AVAILABILITY
                         OF WASTEWATER PHOSPHORUS


 RESULTS OF BIOASSAY STUDIES

     To illustrate algal growth and phosphorus uptake during a typical bio-
 assay, Figure 22 shows the response of Scenedesmus sp., in terms of cell
 volume concentration and algal phosphorus, during a batch bioassay experi-
 ment to determine the concentration of biologically available soluble
 phosphorus in a wastewater sample from the raw influent to the Ely plant.
 As indicated in Figure 22, the algae in the batch system were harvested and
 replaced with phosphorus-starved algae on days 4 and 8.  The growth of test
 culture between harvest periods is shown on the left axis of Figure 22 as
 the logarithm of the cell volume concentration during growth.  From the cell
 volume concentration data it is apparent that significant algal growth
 occurred only during the first 4-day incubation period.  The phosphorus up-
 take data show that approximately 91 percent of the algal phosphorus uptake
 which was measured in the bioassay, occurred during the first four day
 period.  However, as shown in Figure 22, additional phosphorus uptake
 occurred during succeeding incubation periods, even though the algal biomass
 failed to increase or actually decreased.  Also shown in Figure 22 is the
 total soluble phosphorus concentration of the bioassay medium, which was
 approximately 200 yg P/L.  Not shown in the figure is the soluble reactive
 phosphorus concentration which was 127 yg P/L or approximately 64 percent of
 the total soluble phosphorus.  However, as Figure 22 shows, the algal uptake
 of soluble phosphorus amounted to 158 yg P/L during the initial 4-day
 incubation period, or approximately 80 percent of the total soluble waste-
 water phosphorus which was present initially.  Clearly short-term uptake
 amounted to more phosphorus than the initial  soluble reactive phosphorus.

     Phosphorus taken up by the algae during the first 4-day incubation
 amounted to nearly 91  percent of the 173 yg P/L which had become available
 to the algae by the termination of the bioassay.   As for the soluble phos-
 phorus bioavailability assay presented in Figure 22, it was generally true
 for all bioassays, for both soluble and particulate, that the majority of
 the phosphorus which became available, did so during the first 3-5 days of
 incubation.

     Presented in Tables 18 through 21 are the results of the phosphorus
 availability bioassays for available particulate and soluble phosphorus in
wastewater samples taken from each of the four monitored wastewater plants.
Additionally, Tables 18 through 21  contain a  detailed chemical  characteri-
zation of the phosphorus in the wastewater samples as determined at the

                                     74

-------
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                             '   ELY  '
                           AUGUST 22, 1979
                           RAW INFLUENT
                         Algal Harvest
                              and
                          Reinoculdtion
                                                           -0
            TOTAL  SOLUBLE PHOSPHORUS CONCENTRATION
                                          im Incremental
                                             P Uptake

                                          I—I Cumulative
                                             P Uptake
                     \
                                                               200
                                                               150
                                                               100
                                                               50
                                                                    o>
                                                                   g
                                                              CO.
                                                              a:
                                                              o
                                                              a.
                                                              CO
                                                              I

                                                              i.
                                     8
                                             10
                                               12
14
                               DAYS
      Figure 22.  Algal growth and phosphorus  uptake during a bioassay
                 to determine available soluble  phosphorus
                                 75

-------
     TABLE 18.  RESULTS OF PHOSPHORUS AVAILABILITY-BIOASSAYS ON WASTE-
                WATER SAMPLES FROM GATES-CHILI-OGDEN PLANT

Sampling Date**
July 3, 1979
Measured Raw Primary Final Raw
Parameter* Influent Effluent Effluent Influent
(1) (2)
Chemical Assay
TP 6.60 0.92 5,76
TPP 2.60 0.55 2.16
NaOH-P 2.30 0.54 0.37
TSP 4.00 0.37 3.60
SRP 2.56 0.08 2.48
Biological Assay
Parti cul ate
BAPP 1.60 0.34
Error*** 1 13
Soluble
BASP 2.36 0.13
Error 8 1 0
TBAP 3.96 0.47

July 12, 1979
Primary
Effluent
(1)
4.95
1.20
0.41
3.75
2.36
0.82
9
2.14
7
2.96


Final
Effluent
(2)
1.28
0.66
0.55
0.62
0.08
0.58
6
0.27
24 .
0.85

* Phosphorus concentrations given in mg P/L:
Tp = total phosphorus
TPP = total parti cul ate phosphorus
NaOH-P = total NaOH extractable phosphorus
TSP = total soluble phosphorus
SRP = soluble reactive phosphorus .
BAPP = biologically available particulate phosphorus
BASP = biologically available soluble phosphorus
TBAP = biologically available phosphorus
TBAP = BAPP + BASP
** Replication of BAPP bioassays is indicated by the number in parentheses;
   BASP bioassays were not replicated.
*** Error = percent error in mass balance.

                                     76

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        TABLE 19.  RESULTS OF PHOSPHORUS AVAILABILITY BIOASSAYS ON
                   WASTEWATER SAMPLES FROM FRANK VAN LARE PLANT*

Measured
Parameter
Sampling Date
July 17, 1979 Julv 27, 1979
Raw
Influent
(1)
Bio-
logical
(1)
Secondary
Effluent
(1)
Raw
Influent
(2)
Bio-
logical
(1)
Secondary
Effluent
(2)
Chemical Assay -
TP
TPP
NaOH-P
TSP
SRP
Biological
Parti cul ate
BAPP
Error
Soluble
BASP
Error
TBAP
2.72
0.88
0.55
1.84
1.63
Assay
0.32
8
1.83
13
2.15
2.34
0.96
0.76
1.38
0.89

0.56
6
.1.00
6
1.56
2.42
0.84
0.10
1.58
1.38

0.51
19
1.26
15
1.77
3.28 .
1.18
0.15
2.10
1.58

0.63
6
1.62
9
2,24
2.17
1.03
0.56
1.14
0.97

0.68
5
1.03
11
1.71
0.58
0.36
0.22
0.22
0.14

0.16
4
0.20
18
0.36
* See Legend, Table 18
                                     77

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   TABLE 20.   RESULTS OF PHOSPHORUS AVAILABILITY  BIOASSAYS  ON  WASTEWATER
              SAMPLES FROM BIG SISTER CREEK PLANT*
Sampling Date
Measured
Parameter
Jul
Raw
Influent
(2)
y 31, 1979
Secondary
Ef f 1 uent
(1)

Final
Ef f 1 uent
(2)


August 10, 1979
Raw
Influent
(2)
Secondary
Effluent
(1)
Final
Effluent
(1)
Chemical Assay
TP
TPP
NaOH-P
TSP
SRP
Biological
Parti cul ate
BAPP
Error
Soluble
BASP
Error
TBAP
7.03
1.95
1.37
5.08
4.77
Assay
0.97
4
5.08 '
24
6.04
2.46
0.08
0.01
2.37
2.11

0.05
1
2.29
12
2.34
1.03
0.04 ,
0.03
0.99
0.86

0.02
.14
0.85
5
0.87
4.77
1.17
1.04
3.60
1.49

0.37
-8
3.15
9
3.52
2.02
0.17
0.09
1.86
1.15

0.05
25
z.
1.58
9
1.63
0.86
0.07
0.94
0.79
0,41

0.02
20
0.57
21
0.59
* See Legend, Table 18
                                     78

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   TABLE 21.  RESULTS OF PHOSPHORUS AVAILABILITY BIOASSAYS ON WASTEWATER
              SAMPLES FROM ELY PLANT*,

Sampling Date
August 14, 1979
Measured
Parameter
Raw
Influent
(2)
Secondary
Effluent
(2)
Final
Ef f 1 uent
(2)
August 22, 1979
Raw
Influent
(2)
Secondary
Effluent
(2)
Final
Effluent
(2)
Chemical Assay
TP
TPP
NaOH-P
TSP
SRP
Biological
Parti cul ate
BAPP
Error
Soluble
BASP
Error
TBAP .
4.78
2.62
1.06
2.16
1.13
Assay
1.34
27
1.73
12
3.07
1.38
1.26
0.71
0.12
0.00

0.76
21
0.11
17
0.87
0.27
0.24
0.19
0.02
0.00

0.12
31
0.02
33 '
0.13
2.36
1.03
0.09
1.33
0.85

0.69
6
1.16
10
1.84
1.17
1.05
0.62
0.12
0.00

0.70
18
0.11
6
0.81
0.71
0.62
0.25
0.08
0.01

0.47
12
0.08
25
0.55 .

* See Legend, Table 18
                                     79

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beginning of each bioassay.  Bioassay replication was generally as duplicates
on each sample for particulate phosphorus for the dates indicated in the
tables.  Soluble phosphorus bioassays were not replicated.  Lastly, Tables
18 through 21 contain values for the error in the phosphorus, mass balances
which were required for calculation of the biologically available particulate
phosphorus and biologically available soluble phosphorus from the bioassay
data.

     Mass balance errors were calculated according to the relationship:

                     - s(Algal P) - A(Wastewater P)   ,nno/
                     	(Initial Wastewater P)    XIUU/0

where:  E(%) = Mass balance error, percent;

        z(Algal P) = Mass of algal phosphorus harvested from assay
               vessel during the algal bioassay, corrected for
               phosphorus in phosphorus-starved assay cultures and
               inocula, yg P.           •                                  ,

        A(Wastewater P) = Change in the mass of phosphorus fraction
               in the decay vessel from initiation to termination,
               yg P.

The error in the mass balances ranged from -8 to 31 percent with an average
error of 11 percent for the particulate phosphorus bioassays and ranged from
5 to 33 percent with an average error of 14 percent for the soluble
phosphorus bioassays.

     The results given in Tables 18 through 21 are illustrated in Figures 23
through 26 as bar diagrams which show the biologically available and non-
available portions of total phosphorus, total particulate phosphorus, and
total soluble phosphorus in samples taken through the four wastewater plants.
It is clear from the data in Figures 23 through 26 that biologically
available phosphorus in the raw wastewater influent to each plant was
reduced in concentration during treatment.

Effects of Treatment on Biologically-Available Phosphorus

     To facilitate an examination of the effects of wastewater treatment on
the biologically available fraction of wastewater phosphorus, the chemical
and biological phosphorus data in Tables 18 through 21 were used to calculate
average amounts of biologically available phosphorus relative to the soluble,
particulate, and total phosphorus in the wastewater during various stages
of treatment.  This required calculation of the ratios:TBAP/TP, BAPP/TPP,
and BASP/TSP,

where:  BAPP = Biologically available particulate phosphorus, yg P/L;

        BASP = Biologically available soluble phosphorus, yg P/L;
                                     80

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       TBAP = Total biologically available phosphorus, BAPP +
              BASP, ug P/L;

        TP  = Total phosphorus, ug P/L;

        TPP = Total particulate phosphorus, ug P/L;

        TSP = Total soluble phosphorus, ug P/L
                '\                     '                                     '
Additionally, the data were used to calculate estimates of the percentage
reduction of raw wastewater TBAP, BAPP, and BASP at the sampling locations
in each treatment plant.  The ratios and removal data are given in Table 22.

     The data on the amount of available phosphorus in the soluble, particu-
late, and total phosphorus fractions of wastewater shows little variation in
available phosphorus as a proportionate component during treatment.  The lack
of variation is particularly evident in the amount of TBAP (BAPP + BASP)
relative to the total phosphorus during treatment.  The ratio, TBAP/TP, in
raw wastewater varied from 0.6 to 0.8 among the wastewater plants.  However,
within any particular plant the ratio varied over a considerably smaller
range through the treatment stream.  Thus it appears that raw wastewater
characteristics, as yet unidentified, play a greater role in determining the
overall extent of biological availability of phosphorus in treated effluents
than the methods employed during wastewater treatment, at least with a
respect to the methods encountered during this investigation.  Similarly, the
proportions: BAPP/TPP and BASP/TSP in wastewater were more variable among
plants than between stages of treatment within any particular plant.  The
only exception to the apparent lack of in-plant variation in available phos-
phorus as a component of the wastewater phosphorus occurred at the Frank Van
Lare plant, where the amount of BAPP relative to TPP was quite variable.
However, the BASP relative to TSP through the Van Lare plant showed little
change.

Removal of Biologically Available Phosphorus

     A comparison of data on the removal of total phosphorus and the phos-
phorus fractions, given in Table 16, with the removal of biologically,
available phosphorus, set forth in Table 22, shows similar percentage
removals for available fractions and corresponding, analytically-defined
chemical fractions of wastewater phosphorus, with the exception of the Frank
Van Lare plant.  Available phosphorus in the raw influent at the Van Lare
plant was removed less efficiently than the analytically-defined components
of phosphorus.  Among the three other wastewater plants, the percentage
removals of total phosphorus ranged from 85 to 88 percent (Table 16), while
total available phosphorus removal (TBAP) ranged from 83 to 88 percent
(Table 22).  Percent removals of biologically-available and total quantities
of soluble and particulate wastewater phosphorus were similar..

CHEMICAL FRACTIONS AND BIOLOGICALLY AVAILABLE PHOSPHORUS     	':   '*

     A major objective of this investigation was to determine the extent to
which available phosphorus, as determined by algal bioassay, may be related

                                     85

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      TABLE 22.  PERCENTAGES OF BIOLOGICALLY AVAILABLE PHOSPHORUS AND
                 REDUCTION IN BIOLOGICALLY AVAILABLE PHOSPHORUS AT
                 MONITORED WASTEWATER PLANTS

Percent
Biologically Avai


Plant Name and
Sampling Location*
Gates-Chili-Ogden
Raw Influent (1)






Primary Effluent (1)
Secondary Effluent
Frank Van Lare
Raw Influent (2)
Alum Effluent (2)
(2)



Biological Effluent (2)
Big Sister Creek
Raw Influent (2)
Secondary Effluent
Filtered Effluent
Ely
Raw Influent (2)
Secondary Effluent
Filtered Effluent


(2)
(2)


(2)
(2)


TBAP
TP

60
60
58

72
68
73

80
88
76

71
66
64
Phosphorus

BAPP
TPP

62
68
74

44
52
62

40
48
40

59
63
62
Table


BASP
TSP

59
57
40

88
86
82

94
91
79'

82
92
86
Reduction
Available
Compared

TBAP

,-
-
88

_
51
26

-
58
85

-
64
83
of Biologically
Phosphorus
to Raw

BAPP

-
-
79

._
12
38

-
90
96

-
21
62
Influent

BASP


-
94

_
59
41

-
53
83

_
92
96

* Number of samples assayed is given in parentheses.
                                     86

-------
to and predicted from chemical assays of phosphorus in wastewater.  The
approach taken toward achieving this objective focused on examining the
biological availability data, from the wastewater samples collected at the
treatment plants, for correlations with the different chemical fractions of
wastewater phosphorus which were measured at the time each bioassay was
initiated.

     Given in Table 23 are zero-order correlation coefficients between
biologically assayed available phosphorus and chemically assayed fractions
of phosphorus for all the wastewater samples for which bioassays were
performed.  Thus, the correlation coefficients listed in Table 23 represent
the extent of relationship between available and chemical fractions of phos-
phorus which occur in wastewater samples from different wastewater plants
and differing stages of treatment.

Available Soluble Phosphorus

     Biologically available soluble phosphorus correlated strongly and
nearly equally (r > 0.95, a < 0.01) with both total soluble phosphorus and
soluble reactive phosphorus.  Such a result is not unexpected as soluble
reactive phosphorus is considered widely to be the phosphorus form used
directly for algal growth.  Since soluble reactive phosphorus was a major
component of the soluble phosphorus in the wastewaters employed in this
investigation, any correlation between biologically available soluble phos-
phorus and soluble reactive phosphorus would be reflected in a coincident
correlation with total soluble phosphorus.  However, biologically available
soluble phosphorus was a consistently larger fraction of the total soluble
phosphorus than was soluble reactive phosphorus.  Available soluble phos-1
phorus averaged 80 percent of the total soluble, while soluble reactive
phosphorus averaged 69 percent of the total soluble, as may be determined
from Tables 18-21.  Thus, a significant fraction of the nonreactive soluble
phosphorus of wastewater became available during the limited periods of
incubation of the bioassay studies.

   .  Another view of the biological availability of the soluble wastewater
phosphorus as it compared between plants and samples is shown in Figure 27.
In Figure 27 biologically available soluble phosphorus is plotted against
total soluble phosphorus for the four plants studied intensively.  The
degree of association between the two measures of phosphorus, the apparent
similarity of availability of soluble phosphorus between the different
treatment plants, and the lack of a non-zero intercept in the regression
equation which relates the two quantities, serve to support the conclusion
that the biological availability of soluble wastewater phosphorus is
unaltered during treatment by common treatment methods, including chemical
precipitation for phosphorus removal.  That is, phosphorus removal as it
occurs during.wastewater treatment does not selectively remove either
available or  non-available soluble phosphorus.  Consequently, efforts to
.manage'the discharge of biologically available soluble phosphorus in waste-
water effluents must focus on removal of the total soluble fraction to
maximize removal of available soluble phosphorus.
                                     87

-------
TABLE 23.  SUMMARY STATISTICAL PARAMETERS AND CORRELATION
           COEFFICIENTS FOR CHEMICALLY AND BIOLOGICALLY
	ASSAYED PHOSPHORUS IN 22 WASTEWATER SAMPLES*
Chemically
Assayed Phosphorus
Biologically Available Phosphorus
    BASP       BAPP       TBAP
    Correlation  Coefficients
TP
TPP
NaOH-P
TSP
SRP
NaOH + SRP
0.885
0.488
0.477
0.952
0.951
0.913
0.705
0.959
0.795 '
0.469
0.393
0.598
0.968
0.700
0.643
0.958
0.935
0.962

  rcrit, 0.05 = °'423' rerit, 0.01  = °'537
                           88

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      The relationship  between  biologically  available  soluble  phosphorus and
 soluble  reactive  phosphrous  in the wastewater  samples  is  illustrated  in
 Figure 28,  for  an analysis similar to  the previous  involving  total  soluble
 phosphorus.   Though  the  intercept of the regression was not shown  statisti-
 cally to be  different  from zero (p~0.09), the  regression  suggests  that
 generally more  soluble phosphorus was  available  than  that fraction  measured
 as  soluble  reactive  phosphorus.  However, the  regression  coefficient
 relating BASP to  SRP was essentially unity  which indicates the soluble phos-
 phorus in wastewater which is  measured as reactive  by  the analytical  test
 described earlier, is  totally  available for organism growth.

 Available Particulate  Phosphorus

      As  shown in  Table 23, biologically available particulate phosphorus
 correlated most closely  (r = 0.959, a  < 0.01)  with  the total  particulate
 fraction of  the wastewater samples.  The particulate phosphorus which could
 be  extracted with NaOH also correlated with available  particulate  phosphorus,
 but the  correlation  was weaker (r = 0.795,  a < 0.01) than that involving
 total particulate phosphorus.   The relationship  between BAPP  and TPP  is
 illustrated  in  Figure  29, which shows  BAPP  as  a  function  of TPP.  The linear
 relationship shown by  the data in Figure 29 suggest that  the  availability of
 particulate  phosphorus is affected only to  a minor extent during wastewater •
 treatment, a similar result to that given earlier for  soluble phosphorus.
 That  is,  the fraction  of the total particulate phosphorus of wastewater
 which can become  available to  support  algal growth remains relatively
 constant during treatment, including those  phases designed to remove  phos-
 phorus.   Thus,  neither available nor non-available particulate phosphorus in
 wastewater is removed  selectively during treatment; rather, each fraction is
 removed  in approximately the same proportion as  contained in the raw waste-
 water which  enters the treatment plant.  Thus, as was stated earlier  con-
 cerning  efforts to control the discharge of biologically  available  soluble
 phosphorus,  control  of available particulate phosphorus in wastewater
 effluents should  concentrate on the total particulate phosphorus fraction.

      A comparison of the data  in Figures 27 and  29 indicates a significantly
 lower proportion  of  available  particulate phosphorus as compared to available
 soluble  phosphorus,  relative to the total particulate and soluble fractions.
 The regression  coefficients which relate the biologically available soluble
 and particulate phosphorus to  the total amount of each fraction al9ng with
 their standard errors were 0.82 +_ 0.06 mg BASP/mg TSP and 0.55 +_ 0'.04 mg
 BAPP/mg TPP.  A similar comparison, calculated from the average value of the
 phosphorus fractions for all  bioassay  determinations as given in Tables 18-21
yields 0.81 mg BASP/mg TSP and 0.56 mg  BAPP/mg TPP.   These data indicate
 that  equal quantities of soluble and particulate phosphorus in a given waste-
water would  support more algal  growth  from  the phosphorus contained in the
 soluble fraction than from the particulate  fraction.  Thus, in terms of
 phosphorus removal and its relationship to objectives for water quality
management, emphasis should be placed on minimizing the total  soluble phos-
 phorus concentration of wastewater effluents.

     Much has been written about relationship  between the availability of
 particulate phosphorus to aquatic organisms and the extractability of

                                     90

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           92

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inorganic phosphorus from aquatic particulates by a JD...3 N solution of NaOH
(Armstrong et. al., 1971; Wildung et. al. .1977; Cowen and Lee, 1976; Sagher,
'1975, 1976; Logan et. al., 1979).  As indicated in Table 23 and illustrated
in Figure 30 the relationship between BAPP and the phosphorus extracted from
wastewater particulates by 0.1 N NaOH, according to the method described
earlier, was too variable to have much predictive value, though the relation-
ship had significance in a statistical sense (p < 0.01).  It should be
pointed out that the NaOH extractable particulate phosphorus measurements
determined during this investigation are not strictly comparable to the
methods used by others, such as Cowen and Lee (1976) and Sagher (1976), for
comparison of chemical and biological assay results, since the previous
workers measured only the reactive inorganic phosphorus content of the
extractant solution.  During the present work, the total phosphorus content
of the base extracts was measured and, thus, would include not only reactive
inorganic phosphorus, but also a portion of the organic phosphorus of the
particles under investigation.  Consequently, if only the inorganic fraction
of NaOH extractable particulate phosphorus were biologically available, then
NaOH-P reported here should systematically overestimate BAPP.  However, such
was not the case.  As seen in Figure 30, BAPP actually was greater than
NaOH-P in 11 of the 22 samples.  Furthermore, if the total particulate
phosphorus which was extracted by NaOH showed a weak relationship witht
biologically available particulate phosphorus, due to confounded error from
inclusion of base-extractable particulate organic phosphorus, then any
relationship between available particulate phosphorus and total particulate
phosphorus should be no less confounded.  Again, such was not the case and,
as reviewed earlier, total and biologically available particulate phosphorus
concentrations were strongly correlated among the wastewater samples.  Thus,
it appears that NaOH extractable particulate phosphorus is an analytical
method which has limited utility for predicting phosphorus availability when
applied to wastewater samples. ,

Available Total Phosphorus  .

     The total amount of biologically available phosphorus in the wastewater
samples was estimated by summation of the available particulate and
available soluble fractions on each sample.  The relationships between this
"total biologically available phosphorus" fraction (TBAP) and chemically
assayed fractions are given in Table 23 in terms of correlation coef-
ficients.  As could be anticipated from the foregoing results and
discussion, the total biologically available phosphorus in the wastewater
samples correlated most strongly (r = 0.968, a < 0.01) with the total phos-
phorus.  However, a nearly identical degree of correlation (r = 0.962,
a < 0.01) was noted between BAP and the sum of soluble reactive and NaOH
extractable phosphorus.

     The relationship between TBAP and the chemically assayed forms of
phosphorus are illustrated in Figures 31 and 32, where TBAP is given as a  ,'
function of the chemically measured forms.  Regression equations also are
given to facilitate a comparison between the two estimators of TBAP.

     Averaged over all samples of wastewater subjected to bioassay, TBAP
                                    93

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                                96

-------
 amounted  to  72  percent  of  the  total  phosphorus  in  the  samples,  as may  be
 calculated from data  given in  Table  23.   That percentage  is  identical  to  the
 regression coefficient  shown in Figure  31. for TBAP as  a function of  total
 phosphorus concentration.   The equality of the  two values  reflects the nearly
 uniform proportion of available phosphorus to the  total phosphorus in  waste-
 water  samples taken from various  locations within  the  treatment plants and
 the  relatively  narrow range of values for that  proportion  among treatment
 plants.

     The  sum of soluble reactive  plus NaOH extractable phosphorus generally
 underestimates  TBAP.  Using values for  all  the  wastewater  bioassays, given
 in Tables 18-21,  the  TBAP  averaged 112  percent  of  the mean sum  of soluble
 reactive  and NaOH extractable  phosphorus.   The  regression  coefficient  in the
 equation  which  relates  BAP to  the sum of reactive  and extractable phosphorus
 was  0.93, less  than would  be expected based on  the value of  the ratio  of the
 mean concentration of the  phosphorus fractions.  However,  examination  of
 Figure 32 suggests that the regression  coefficient is strongly  biased  by two
 data points  which represent relatively  low availability.   If the points are
 treated as outliers,  possibly  as a result of the large dilution factors
 required  for bioassay on such  concentrated  samples, then the recalculated
 regression coefficient equals  1.16 and  the  non-zeros intercept  becomes
 insignificant,  leaving a direct relationship between TBAP and (NaOH-P) +
 (SRP):

                   TBAP =  1.16 [(NaOH-P^)  +  (SRP)]  + 0.05

                                r = 0.951,

 which more closely reflects the relative  amounts of the biologically and
 chemically defined fractions.  Thus, as an estimator of available phosphorus,
 the  sum of the  soluble reactive and NaOH  extractable particulate phosphorus
 appears useful  only to obtain  an approximate minimum value for  total
 biologically available phosphorus, while  a clearly more conservative estimate
 would be  based  on the total phosphorus concentration.

     A final  point needs to be put forth  regarding interpretation and
 applicability of the  bioassay  data on available phosphorus as presented
 above.  It must be recognized  that the bioassays used to estimate the avail-
 ability of particulate and  soluble phosphorus" in the wastewater samples were
 of relatively short duration,  due to the  time constraints imposed on the
 investigation.  Further, the kinetics of  conversion of non-available to
 available phosphorus were  not examined directly.   Consequently,  reaction
 orders for the conversion were unknown and the extent of approach of the
 conversion to ultimate availability at the time of bioassay  termination could
 not be determined.  Such considerations should be addressed  in  future
 research.   However, the criteria for termination of an algal  assay:  plateaus
 in biomass increase and accumulation of phosphorus by the assay culture,
 permitted the availability estimates to. approach ultimate availability to
 the extent that changes in the  assay culture were detectable  over a  period
of a few days.   The point, then,  becomes one of recognizing that the
estimates  of phosphorus bioavailability and the regression coefficients
which relate them to chemically defined phosphorus fractions, as presented
                                     97

-------
in the preceeding, may be less accurate than estimates which are based on
truly long-term incubations.

SUMMARY

     Algal bioassays were conducted on 22 samples of wastewater., taken from
various locations in each of four wastewater treatment plants, to determine
the availability of both soluble and particulate phosphorus, to aquatic
organisms; ari*d, to determine the extent of relationship, if any, between
analytically-defined chemical fractions and bioassay-defined available phos-
phorus.  A comparison of available phosphorus fractions at the different
sampling points in each wastewater plant indicated that, at the wastewater
plants selected for study, the methods of treatment had no major effect on
the biologically available fraction of either soluble or particulate phos-
phorus relative to the total phosphorus content of those fractions,
including phosphorus removal processes.  Biologically available phosphorus
averaged 72 percent of the total phosphorus, the available particulate
fraction averaged 55 percent of the total parti cul ate phosphorus., and the
available soluble fraction averaged 82 percent of the total soluble phos-
phorus concentration in the wastewater samples.  Due to its greater
availability, soluble phosphorus should be the target fraction for phosphorus
removal efforts.  Biologically available phosphorus correlated best with the
chemically assayed fractions of phosphorus given above.  Additional, highly
significant correlations were observed between biologically available
phosphorus and soluble reactive phosphorus, and between total available
phosphorus and the sum of soluble reactive phosphorus and NaOH extractable
phosphorus; however, the latter chemically-assayed fractions consistently
underestimated biologically available phosphorus.
                                     98

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                                 SECTION 8

                               COST ANALYSIS

      The proper evaluation of a given phosphorus effluent standard requires
 the _costs incurred as well as the benefits obtained.  This section will
 examine operation and maintenance costs associated with phosphorus removal
 for the four treatment plants studied.  Also, for each of these plants
 various alternatives will  be generated for achieving a phosphorus effluent
 of 0.5 mg/L.  The incremental costs for each of these alternatives will  be
 discussed.

 GATES-CHILI-OGDEN

 Introduction

      Pa G|tes-Chili-Ogden (GCO)  wastewater treatment.plant is  a  20 tngd
      lO** m-Yday)  activated sludge plant located near Rochester, NY.   It  is
 operated by the Division of Pure  Waters of Monroe County.   A description  of
 the GCO wastewater plant and the  field data collected at  GCO have been
 presented previously (Section 6).   A summary of the  phosphorus  data and a
 line schematic  diagram of  the processes employed are shown  in Figure  33.

      Since the  middle  of 1978,  phosphorus  removal  has  been  practiced  at GCO
 by  means  of alum  precipitation.   Liquid alum is  added  between the aeration
 basin  and the final  sedimentation  basins.   As can  be seen from the  summary
 diagram (Figure 33), this  approach  can  result in "low phosphrpus effluent
 concentrations.   The average  effluent  concentration  was 0.75 mg/L  for  the
 sampling  period.   GCO  has  a  phosphorus  effluent  standard of  1.0 mg/L.

 fy.   I??-1!q!id *1ur used  at  GCO is a  48 Percent alum solution and purchased
 from Allied  Chemical.   During the sampling  period, a dosage of 70.1 mq/L
 was  used, which is equivalent to an Al+3 concentration of 3.0 mg/L.

 Operation and Maintenance  Costs

     Total operation and maintenance costs for GCO are presented in Table
 
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              TABLE 24.  GCO-TOTAL PLANT O&M COSTS



Before P-Removal
(Nov. 77-Apr. 78)
i
Labor
Power
Chemical
Miscellaneous
Total O&M
$/Year $71000 Gallons'

266,176
281,723
58,382
13,680
619,961

0.055
0.057
0.012
0.003
0.127


After P-Removal
(Nov. 78-Apr. 79)
$/Year $71000 Gallons'

288,563
304,971
189,195
11,040
793,679

0.059
0.064
0.039
0.002
0.165

         TABLE 25.   GCO O&M COSTS FOR PHOSPHORUS REMOVAL
                       (BASE PERIOD:  NOV.  78 -  APR.  79)


Labor
Power
Chemical
, Total

$/Year
728
101
119,408
120,237

$/l 000 Gallons
.<.001
<.001
0.025
0.026
'$/1000  gallons  is  equivalent  to  $/3.785  nT
                               101

-------
category.  This can be used as an approximate means to account for inflation
in comparing the two periods.

     Table 25 presents a summary of operation and maintenance costs
associated with phosphorus removal at GCO.  Each item will  now be explained.
Labor costs associated with phosphorus are not very significant at GCO.
When phosphorus removal was started, no additional personnel  were hired.
It is estimated that only two man-hours per week are allocated to the
specific phosphorus removal practice.  Using a rate of $7.00 per hour (from
plant records) only $728 per year is spent.

     Power costs were computed by determining the electricity required for
operating the one-half horsepower (373 watts) motor for the alum feed pump.
It was assumed that the pump is run continuously.  An average rate of
$0.031 per kilowatt hour is used for electrical costs which is the rate
charged the GCO plant by Niagara Mohawk Power Co.

     Finally, chemical costs were derived from actual costs incurred for
liquid alum over the six month period, extrapolated to one year.  The cost
of the liquid alum was $0.059 per pound.

     In examining the associated phosphorus removal costs it is evident that
the item most sensitive to phosphorus removal is the chemical costs.  Power
and labor costs associated with phosphorus removal are not significant.
Costs associated with the additional sludge generated from phosphorus
removal are discussed in a later section.

Analysis of Performance

     At the time of the sampling period at GCO, the alum was being added at
a dosage of 70 mg/L.  This corresponds to an Al+3 concentration of 3 mg/L.
Based on the field data, an aluminum to phosphorus molar ratio can be
calculated.  Metal ion to phosphorus ratios, on both a total  and soluble
phosphorus basis, are listed for all four plants monitored in Table 26.
Precipitation cation: soluble P dosage ratios are used in this report for  .
calculation of sludge production associated with phosphorus removal.  Ratios
relative to total phosphorus are used in evaluating metal ion dosages and
subsequent phosphorus removal.

     Since at GCO the alum was added after the aeration basin, some of the
4 mg/L soluble phosphorus present in the raw waste was incorporated by
biological synthesis into the mixed liquor biomass.  Assuming a BOD:N:P
ratio of 100:5:1 (uptake), approximately 1 mg/L of soluble P was removed by
biological uptake.  This left 3 mg/L of soluble P which could react with the
aluminum.  Accordingly, the phosphorus removal process at GCO was being
operated at a dosage such that the A1:P ratio  (soluble P basis) was 1.2.
On the other hand, evaluation of the A1:P ratio on a total P basis yielded a
value of 0.6, since the average primary effluent of total phosphorus was
5.5 mg/L.  The typical pH of the secondary effluent was 7.4.

     In addition to using the proper chemical and the proper dosage
effective phosphorus removal requires adequate capacity in the solids

                                    102

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Total P
Soluble P
           TABLE 26.  PRECIPITATION CATION TO PHOSPHORUS RATIOS
          	FOR THE PLANTS MONITORED	
                                    GCO  ~~
        Primary Effluent
            5.5 mg/L
            3.0 mg/L.
A1:P (Molar)
    0.6
    1.2 ,
                                    Ely
Total P
Soluble P
        Primary Effluent
              3.8
              1.4
A1:P (Molar)
    0.8
    2.0
                             Big Sister Creek
Total P ,
Soluble P
Secondary Sedimentation Effluent
              2.3
              2.1
Fe:P (Molar)
    2.1
    2.3
                                 Van Lare
Total P
Soluble P
        Primary Influent
              3.8
              1.1
A1:P (Molar)
    1.2
   3.8
                                    103  .

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separation process  in order to ensure a good removal of the precipitated
phosphorus solids.  A plot of phosphorus concentration versus overflow rates
is shown in Figure  34, for the sampling period at GCO.  As the process was
operating at Tow overflow rates, there is no trend in the total particulate
phosphorus concentration as a function of overflow rates.  Figure 34 shows
that for the period in which the sampling occurred, there was more than
adequate clarification capacity.  This is generally the case at GCO for most,
of the year.

     Thus, the GCO  plant was able to achieve good phosphorus effluent con-
centrations (average of 0.75 mg/L total P) by using moderate alum dosages
with a conservative clarification capacity during our sampling period.  GCO
has in fact been easily meeting the average 1.0 mg/L effluent standard,
based on monthly plant reports.

Alternatives to Meet a 0.5 mg/L Limit

     Based on our field data, it is assumed that if a 0.5 mg/L effluent P
standard were imposed at GCO, it could be met by increasing the alum dosage
to a molar ratio of 1.5 (A1:P, on a soluble P basis).  This would result in
an increase in the alum dosage from 3 to 4 mg/L Al+3.  This assumes that
sufficient clarification capacity would still be available.  This assumption
is critical to this alternative as most of the phosphorus remaining is most
likely in a colloidal form, and the additional alum added would riot be
precipitating phosphorus, but rather coagulating the particulate forms.
However, it should be pointed out that at the present time, two tertiary
sedimentation basins exist at GCO which are not used.  These were built for
the initial phosphorus removal practice of tertiary lime precipitation which
was abandoned at GCO in favor of alum precipitation in the secondary process
due to economic considerations.  Thus, additional clarification capacity
would be available at no additional capital  cost.  It might also be necessary
to add a polymer along with the alum for more effective particulate removal.

     The incremental costs of going to 0.5 mg/L will  be analyzed in terms of
additional costs for chemicals and sludge processing.  It is assumed that
any additional power and labor costs directly associated with the actual
phosphorus removal are negligible.

     The additional chemical  and sludge costs are shown in Table 27.   The
following assumptions were made in constructing Table 27.   The alum dosage
would be increased from 3 to 4 mg/L Al+3;  the unit cost of alum is $0.059
per pound; the flows for chemical  usage are the average six month flow of
13.3 mgd (5xl04 m3/day).   The polymer dosage (if necessary) would be 1  mg/L
at a unit cost of $1.32 per pound ($2.91/Kg).   This is for the same polymer
used by Monroe County Pure Waters at the Frank Van Lare plant.  The quanti-
ties of total  sludge generated at the plant are based on actual  plant
operations data corresponding to our sampling period.  The unit cost of
sludge processing (thickening, dewatering,  and incineration) was $71.37 per
ton of dry solids processed.   This figure was from actual  plant records for
the same time period.  The flow used to compute actual  sludge .costs was that
which has the average flow during the sampling period (9.5 mgd)  (3.6x104
m3/day).  The amount of sludge generated from phosphorus removal  was

                                    104

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         TABLE 27.  SLUDGE AND CHEMICAL COSTS AT GCO (SUMMER 1979)	

                   Chemical Costs  P'STudge2   Total Sludge P Sludge Cost
                   $71000 Gallons lbs/106 gals lbs/106 gals $/1000 Gallons
Present Conditions
0.75 mg P/L
0.5 mg P/L
(alum alone)
0.5 mg P/L
(alum with polymer)
0.025
0.030'
0.040
120
140
140
1387
1527
1527
0.004
0.005
0.005

               TABLE 28.  SUMMARY OF INCREMENTAL COST AT GCO
                          FOR ACHIEVING A 0.5 mg P/L RESIDUAL

Category
Sludge Processing
Chemical
I/Year
2080
24,364
$/1000 Gallons
0.001
0.005
(alum alone)

Chemical
(alum & polymer)
79,039
0.016
        gallons is equivalent to $/3.785 m
OK                                  "3
 lbs/10  gallons is equivalent to 0.12 g/m
                                    106

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calculated by stoichiometric relationships between aluminum ion and soluble
phosphorus and hydroxide as described by Vesilind (1979).

     Finally, the costs of sludge processing attributed to phosphorus
removal were computed by multiplying the amount of P sludge by the unit cost
of sludge processing.  This technique is somewhat liberal in that the alum
sludge generated from phosphorus removal is more difficult to thicken and
dewater than the mixture of primary or secondary sludge.  However, it-should
be noted that it is only a small percentage of the total amount of sludge
generated at GCO.

     The incremental costs for achieveing a 0.5 mg/L standard are summarized
in Table 28.  Several points should be noticed.  First of all, the incre-
mental sludge costs is not very significant in terms of the overall O&M
costs.  However, additional examination of the GCO plant would have to be
made in order to determine if adequate thickening, pumping, and dewatering
facilities exist for processing the additional sludge.  Such a complete type
of analysis was beyond the scope of this study.

     The additional alum cost would result in a 20 percent increase in
chemical costs.  If polymer were needed, the increase would be 66 percent.
These represent .significant increases.

     For GCO the phosphorus data indicate that an 0.5 mg/L P effluent limi-
tation could be met without tertiary filtration.  However, we have computed
the costs if GCO were required to add filtration.  For a 20 mgd (7.5x104 m3/
day) plant, such as GCO, the capital costs for filtration are estimated to
be $2.84xl06 (2nd Quarter, 1979) (EPA, 1978a), while the annual O&M costs
would be $290,000 (August, 1979) (Weston, 1977).

ELY

Introduction

     A description of the Ely, Minnesota wastewater treatment plant and the
field data collected there have been presented previously (Section 6).  A
summary of the phosphorus data and a line schematic diagram of the processes
employed are shown in Figure 35.

     The U.S. Environmental Protection Agency (EPA) in cooperation with the
City of Ely, funded construction of an advanced wastewater treatment
facility to demonstrate that a reduction in phosphorus from a point source
could improve the trophic status of Shagawa Lake.  Prior to the construction
of the tertiary plant, the Ely waste treatment facility consisted of a
conventional secondary treatment operation.  The tertiary plant began
operation in the spring of 1973.  It was designed and constructed as a
research facility with very high phosphorus removal efficiency (to limit the
phosphorus content of the effluent to 0.05 mg/L or less (EPA, 1978b)).

     Originally during the demonstration, phosphorus removal was practiced
by lime precipitation in the tertiary solids contact tanks.  After the
demonstration was finished the plant switched.to Fed3 precipitation of

                                   107

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 phosphorus from the trickling filter effluent.  Beginning in June, 1979 the
 plant switched to liquid alum and polymer addition to the trickling filter
 effluent followed by secondary settling and tertiary filtration.  This was
 the phosphorus removal practice used during the field sampling of this
 project.

      The liquid alum used for phosphorus removal was a 48 percent alum
 solution.   During the field sampling the dosage varied between 50 and 60
 mg/L.   The polymer added to the trickling filter effluent was Betz 1160, a
 cationic polymer.   It was added at a concentration of 0.3 mg/L.

 Operation  and Maintenance Costs

      Total  operation and maintenance costs for Ely are presented in Table 29.
 These  costs are based on the three month period of actual  plant  records  from
 June through August of 1979, extrapolated to one year.   Prior to June,
 phosphorus  removal  was practiced by Fed 3 addition;  therefore, the months of
 January through May were not used.   Fuel  costs were  not available for this
 three  month period;  hence,  1978 figures  were used for that portion of the
 power  costs.

     Table  29 shows  the amount of money  spent at Ely for wastewater treatment
 ($0.916/1000 gallons)  ($0.24/m3)  and that most of this  cost  is associated
 with labor  ($0.680/1000 gallons)  ($0.18/m3).   This  is primarily due to the
 fact that the City  of Ely has  a  contract  from the  EPA to run  this plant
 which  was built as  a research  facility.   At  the present time, a  consulting
 engineering company  is  operating  the plant for the City of Ely.   Thus, the
 O&M  costs are distorted by  labor  and overhead costs  which  are not typical
 for  a  treatment plant  of this  size  (approximately  1  mgd, 3.785x103
     Table 30 presents a summary of operation and maintenance costs
associated with phosphorus removal at Ely.  Labor costs associated with
phosphorus removal are computed by allocating 40 hours of manpower, per week.
This assumption is based on the judgment of the plant supervisor at Ely.
Using a rate of $6.00 per hour and 52 weeks per year, the labor costs
associated with phosphorus removal are thus $12,480 per year.  Power costs
were computed by actual horsepower requirements for tertiary wastewater
pumping (15 HP) (11.2 kilowatts), polymer and alum pumping (0.5 HP each)
(373 watts) and an air scour were operated for 20 minutes each day.  A rate
of $0.06 per kilowatt hour is used for calculating the electrical cost,
based on actual service charges at the Ely plant.  Chemical costs are based
on the 3 month costs for the liquid alum and polymer, and extrapolated to
one year.

     Sludge production associated with phosphorus removal is shown in Table
31.  The chemical  dosages are based on average dosages used during the field
sampling at Ely.  Total sludge production is based on actual  plant data
during the sampling period.   The sludge associated with phosphorus removal
was calculated by the stoichiometric relationship between the aluminum ion
and soluble phosphorus and hydroxide ion as described by Vesilind (1979).
Additional parti cul ate phosphorus sludge removed by filtration is also
included.
                                   109

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                  TABLE 29.   ELY -  TOTAL PLANT O&M COSTS
                       (TIME PERIOD BASIS:  SUMMER 1979)
                                  $/Year
                                  $/1000 Gallons
Labor
Power
Chemical
Miscellaneous
        223,200
          33,421
          24,648
          19,525
              0.680
              0.102
              0.075
              0.059
Total O&M
         300,794
                                                              1  0.916
       TABLE 30.  ASSOCIATED O&M COSTS FOR PHOSPHORUS REMOVAL -  ELY

Labor
Power
Chemi cal
Total
$/Year
12,480
6,325
16,501
35,296
$/100Q Gallons
0.038
, 0.019
' 0.050
0.1.07
               TABLE 31.  ELY SLUDGE PRODUCTION AND CHEMICAL
                            DOSAGES FOR P REMOVAL	
   Chemicals
 Ibs Alum/106 gals
                      P Sludge      Total  Sludge
Ibs ;Polymer/10b gals  lbs/106 gals  lbs/106 gals
       487
        2.84
82.45
3415
 1
  $/1000 gallons  is equivalent to $/3.785 nT
 2lbs/106 gallons  is equivalent to 0.12 g/m
                                     110

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      The unit cost of solids processing could not be determined for Ely due
 to lack of sufficient plant data, in, that separate solids and liquid treat-
 ment portions of the total cost were not maintained by the plant operators
 However, it can be seen that only a small percentage of the total  sludge
 generated is associated with phosphorus removal.

 Analysis of Performance

      The Ely wastewater treatment plant has a phosphorus effluent  standard
 of 0.4 mg/L.  During the time of the field sampling, liquid alum was added
 to the trickling filter.effluent at an average dosage of 58 mg/L which is
 equivalent to an aluminum ion concentration of 2.5 mg/L Al+3.   This resulted
 in an A1:P ratio of 0.8 on a total  P basis.   The average soluble phosphorus
 concentration coming into the trickling filter was 1.4 mg/L.   This results
 in a:Al:P molar ratio of 2.0 (soluble  basis) not accounting for the soluble
 phosphorus which was removed by biological  uptake in the trickling filter.
 If this were taken into account, assuming 1  mg/L soluble phosphorus taken
 up for every 100 mg/L BOD removed,  the soluble phosphorus concentration  at
 the point of liquid alum addition would be  0.5 mg/L and the A1:P would be
 5.5.   By either basis,  a  sufficiently  high  dose of liquid alum is  applied
 to the trickling filter effluent.   Examination of Figure 35 verifies  that
 almost all  of the phosphorus in the  secondary sedimentation effluent  is  in  a
 particulate form,  therefore the dosage used  is precipitating the phosphorus.
 The pH of the secondary effluent during the  sampling period was  typically
 / • O •

      At Ely,  a  trickling  filter plant,  it is  clear that the 0.4  mg/L effluent
 standard  can  not be met with chemical  addition alone.   While the phosphorus
 was successfully insolubilized  by the  alum addition,  it was not  effecitvely
 removed in  secondary sedimentation.  This may  be  due  to the nature  of  the
 settling  of the  solids  which slough  off trickling .filters as opposed to the
 zone  settling phenomenon  associated  with activated  sludge biomass which may
 better  capture  the  particulate  phosphrous.  At any  rate,  the concentration
 of  suspended  solids  in  the  secondary clarifier effluent was 58 mg/L.

      Figure 36 shows  the  results of  a jar test  conducted on the  trickling
 filter  effluent.   It  can  be  seen that the plant dosage  used, indicated by
 the arrow,  does  result  in a  low  soluble phosphorus concentration.  The
 phosphorus  is in a non-sett!eable particulate  form and  the jar tests data
 show  additional  alum  is required, approximately 3 times more to coagulate
 the particulate  phosphorus.  Note that the data for an alum dosage  of zero
 are for a control and do not match the initial data as  settling had occurred
 in  the jar test  beakers.  Although the Ely plant uses a cationic polymer
 dosage of 0.3 mg/L, no jar tests were conducted with the polymer.  If the pH
were adjusted to 6.0, a more optimal pH for phosphorus precipitation with
aluminum, it would produce little difference in the results.  This  is shown
 in Figure 37.  For these tests, alum was added to the samples and then the
pH was adjusted to 6.0.  These results indicate that additional alum is
required for coagulation to achieve  solid separation.

     A plot of the total phosphorus  concentration in the secondary  effluent
versus overflow rate is shown in Figure 38.   The secondary sedimentation

                                  111

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   2.6




   2.4



   2.2



   2.0




    1.8


i
 e  1.6
CO

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0.2
    250
                            1  ELY
                                     Secondary  Effluent
                  300
350
400
450
500
                 OVERFLOW RATE  (gal / day-f t2)

                 (I aal/ft2-dav = 0.041  m3/m -day]
                                                 day)
    Figure 38. Phosphorus concentration of secondary effluent  versus

              •overflow rate of secondary sedimentation basin  -  Ely
                              114

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  /   5 ""I/ f/i9n?d I°r ^ overfl°w rate of 765 gallons per day per square foot
  (31.4 m3/mZ/day) at a flow of 1.5 mgd (5.7x103 m3/day).  It can be seen that
  even at the low overflow rates observed during the field sampling, the phos-
  phorus did not settle out well, as most of the phosphorus is particulate
  (see Figure 35).  Therefore filtration is needed to approach the 0.4 mg/L
  standard at Ely.                                                      3
 *  4.     f1Itrat1on unit at Ely is a dual media filter -consisting of two
 feet (61 cm) of anthracite on top of one foot (30.5 cm) of sand.  It is
 backwashed for 20 minutes each day.  The data shown in Figure 39 indicate
 that the filter removes about 65 percent of the particulate phosphorus
 Improvement in particulate phosphorus removal might be achieved by using a
 Tl 1 T,Q K* ell Q •                                 '
 BIG SISTER CREEK (ANGOLA, NEW YORK)

 Introduction

      The Big Sister Creek wastewater treatment plant located near Angola,  NY
 is a 3.1 mgd (1.1x10^ m3/day) tertiary plant.   A description of the Big
 bister Creek wastewater plant and field data collected there have been
 presented previously (Section 6).  A summary of the phosphorus  data and a
 line schematic diagram of the processes employed are shown in Figure 40.

      Phosphorus removal  has  been  practiced at  Big Sister Creek  since May, "
 19/7.   It is removed during  tertiary treatment by the addition  of FeClq and
 a  polymer to 70 percent of the secondary effluent.   The  secondary treatment
 processes activated sludge  operated in an extended aeration mode.   Tertiary
 processes include  solids-contact  clarifiers and filtration through  a gravity
 sand filter.   The  plant has  a phosphorus effluent standard of 1.0 mg/L.

      The FeCl3  added for phosphorus  removal  was added at a concentration of
 25 mg/L,  which  is  equivalent to 8.7  mg/L of Fe+3,  during the sampling period
 at Big  Sister  Creek.   It must be  noted,  however,  that this dosage varied
 widely  throughout  the year.   During  a  three month  period of December 1977
 through  February 1979 no Fed 3 was needed  for  phosphorus  removal  as  effluent
 standards  could be met without the addition  of chemicals.   The  plant serves
 a resort  area and  thus, flows  are  higher  during  the  summer.   In  addition to
 FeCl3,  Hercules 847  (an  anionic polymer) was also used at  a  dosage of 0 6
 mg/L.

 Operation  and Maintenance Costs

     Total operation and maintenance costs for  Big Sister  Creek are  presented
 in Table 32.  These costs are taken from actual plant records from 1978
 Table 33 presents a summary of 'operation and maintenance costs associated
with phosphorus removal at Big Sister Creek.  Labor costs associated with
 phosphorus were based on the allocation of manpower by the plant supervisor
The total man-hours at Big Sister Creek during 1978 was 14,298 hours   Of
 * jS,fniS5? man-hours were allocated to operation of the filter (12 percent)
and 1835 hours were allocated to the solids contact clarifier (13 percent)
Power costs were assigned by actual horsepower data for each process. Fifty -

                                    115

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BIG SISTER CREEK
JULY 30 - AUGUST 10, 1979
3P
i •
TP
TP
0.5ma/L Tpp
T TPIITPP TPP
                                                     Fe Treated
                                                       Sed. Eff.
      Grit      , Extended
      Chamber   Aeration
                                      FeCI3 Polymer
                                                Solids
                                               j:ontc
 Final
'Eff.
Figure 40.  Summary of phosphorus  data and line schematic - Big Sister Creek
                                     117

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        TABLE  32.   BIG SISTER  CREEK - TOTAL  PLANT O&M COSTS  (1978)

Labor
Power
Chemical
Miscellaneous*
Total O&M
$/Year
258,384
99,301
16,983
45,994
420,662
$/1000 Gallons1
0.228
0.088
0.015
0..041
0,,372
'Includes such things as  telephone service  and water

              TABLE 33.   ASSOCIATED O&M COSTS FOR PHOSPHORUS
                         REMOVAL -  BIG SISTER CREEK
                               $/Year
                                            $/100()  Gallons
Labor
Power
Chemical
Total
91,133
4,834 '
12,501
108,468
0,081
0.004
0.011
0.096

             TABLE 34.  BIG SISTER CREEK SLUDGE PRODUCTION AND
                        CHEMICAL DOSAGES FOR P REMOVAL 	
Chemicals2 - lbs/106 gals    P Sludge2     Total  Sludge      P Sludge Cost
FeCU          Polymer       lbs/106 gals  lbs/106 gals      $/1000 Gallons
   149V
3.29
116
990
0.013
1                           '3                          '
 $/1000 gallons is equivalent to $/3.785 m
2lbs/106 gallons is equivalent'to 0.12 g/m3
3given for total plant flow; is equal to 212.8 lbs/10 g for treated flow
4given for total plant flow; is equal to 4.7 lbs/106g for treated flow

                                     118

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two percent of the power costs were due to the solids contact clarifier and
associated equipment, while 48 percent were due to the filter.  Chemical
costs were computed based on the dosages and flow (2.58 mgd, 9.8xl03 m3/day)
during the sampling period extrapolated to a nine month period, as chemical
addition for phosphorus removal is not necessary year round at Big Sister
Creek.  This estimate is on the high side as smaller dosages can be used
during much of the year due to seasonal variation in wastewater composition.

     Sludge production associated with phosphorus removal is shown in Table
34.  The chemical and polymer quantities are based on quantities used during
the field study and are based on a total flow (2.58 mgd, 9.8xl03 m3/day).
The sludge associated with phosphorus removal was calculated based on
stoichiometry (Vesilind, 1979).  The total quantity of sludge produced is,
from plant records, for the sampling period.  The costs associated with
phosphorus sludge processing is based on a unit cost of $223 per ton of dry
solids processed.  Again, this unit cost would be on the liberal side as the
iron-phosphorus sludge would be more difficult to process than the mixture of
primary, secondary, and chemical sludges on which the $223 figure is based.

Analysis of Performance

     At the time of the sampling period at Big Sister Creek, the FeCls was
being added at a dosage of 8.7 mg/L Fe+3.  The polymer was added at a dosage
of 0.6 mg/L.  Based on the field data an iron to phosphorus ratio can be
calculated.  On a total P basis, the ratio was 2.1.   Soluble phosphorus in
the secondary effluent averaged 2.1 mg/L.  This results in an Fe:P molar
ratio of 2.3 (soluble basis).  Jar test results for the secondary effluent
are shown in Figure 41.  Both the field data (Figure 40) and jar test data
indicate that the Fe dosage is adequate in both insolubilizing the phosphorus
and removing it by sedimentation.  In fact, the data show that a total phos-
phorus of less than 0.5 mg/L can be achieved.  The pH of the secondary
effluent during the sampling period was typically 7..4.

     A large fraction of the particulate phosphorus  was removed during the
extended aeration process with subsequent settling.   The secondary sedimen-
tation basin is conservatively designed with an overflow rate of 500 gallons
per day per square foot (20.5 m3/mVday).  This partially accounts for the
high degree of particulate .phosphorus removal.   In examining Figure 41,
which shows total and particulate phosphorus concentration .of secondary and
solids'contact effluents versus overflow rate,  it can be seen that the 0.5
mg/L phosphorus effluent limitation can be met without filtration.  Also
from Figure 42, it appears that an overflow rate of  550 gpd/ft2 (22.6 m3/m2/
day) and less produced similar results.  These data  demonstrated the good
efficiency of Fe in insolubilizing the phosphorus.  Both the secondary and
solids contact units were designed at overflow rate  of 500 gpd/ft2 (20.5
m3/m2/day) at a design flow of 22 mgd (8.3xl03 m3/day).   It should be pointed
out that because of the many variables associated with actual  performance,
it would take significantly more data to show the effect of overflow rate on
effluent quality.

     A plot of filter performance at Big Sister Creek is shown in Figure 43.
The filter used at Big Sister Creek consisted of 12  inches (30.5 cm) of high
                                    119

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grade silica with a uniformity coefficient of 1.3 - 1.5 and an effective size
of 0.55 - 0.65 mm.  Figure 42 clearly shows that the filter was a polishing
operation at the wastewater plant.  Most of the phosphorus going to the
filter is soluble, less than 0.2 mg/L is particulate.  The major purpose it
serves now is as a protective measure against solids blowout of the solids
contact units during periods of excessive flow.

Alternatives to Meet a 0.5 mg/L Limit

     Based on the results of the jar tests and field data, if a 0.5 mg/L
effluent standard were imposed at Big Sister Creek, it could be met by
treating all the flow, rather than the present 70 percent, at the same
dosages of FeCla and polymer.  This would result in an increase in chemical
costs of $5357 per year and in the generation of 50 extra pounds (23 Kg) of
sludge per million gallons treated which would result in an incremental
sludge handling cost of $3959 per year.  These costs are based on a flow of
2.58 mgd (9.8xl03 m3/day) for 9 months of the year.  It is assumed that no
additional power or labor costs would occur.

FRANK VAN LARE

Introduction

     The Frank Van Lare wastewater treatment plant is located in Rochester,
NY.  It has an average daily flow of approximately 100 mgd (3.78x105 m3/day).
A description of the Van Lare plant and the field data collected there have
been presented previously (Section 6).  A summary of the phosphorus data and
a line schematic drawing of the processes employed are shown in Figure 44.
The Van Lare plant (along with GCO) is operated by the Division of Pure
Waters of Monroe County.

     The Van Lare plant was upgraded several years ago from a primary to a
secondary treatment facility.  As part of  this upgrading, phosphorus removal
was included.  The original method of phosphorus removal at Van Lare after
upgrading involved lime addition to the primary settling tanks with pro-
vision for recovery of lime.  This method was used only for a brief time at
Van Lare and then abandoned due to excessive sludge production.

     Beginning in 1979, phosphorus removal was again practiced at Van Lare
with liquid alum and a polymer being added to a portion of the flow in the
primary sedimentation basins.  Due to the industrial input to the wastewater
at Van Lare, the waste is generally nutrient deficient and hence an effluent
concentration approaching 1 mg/L can be produced by means of conventional
secondary treatment.  In order to meet a level of 1 mg/L the operators began
treating increasing increments of the raw wastewater in the primary tanks,
until the present portion which is 20 percent of the flow was found to be
sufficient.

     Thus, at present 20 percent of the incoming flow is treated in one of
the primary settling basins on the east side (referred to in Figure 44 as
the Chemical Side) of the plant and then mixed with the other 80 percent of
the flow after secondary settling.  In other words, the 20 percent treated

                                    123

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FRANK VAN LARE
JULY 16- 27, 1979
TP
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CHEMICAL SIDE
PRIMARY TREATMENT

,
Img/L
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 Raw
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     .Primary _^eration_
     Sed.
                                                 CHEMICAL SIDE
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  £
                                                BIOLOGICAL SIDE
                                                BIOLOGICAL SIDE
                TP
                  TPP
                                                      TP
                                                         TPP
                                                                  Img/L
                                                                 0.5ma/L
Figure  44. Sunmary of phosphorus  data and line schematic - Frank Van  Lare

                                   124

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with liquid alum and polymer does not undergo biological treatment, in this
case the activated sludge process.

     The liquid alum used at Van Lare is a 48 percent alum solution purchased
from Allied Chemical.  During the sampling period, a dosage of 85 mg/L was
used which is equivalent to 3.2 mg/L of Al+3.  The polymer used was
Carborundum WT 3000, which was used at a dosage of 0.4 mg/L.

Operation and Maintenance Costs

     Total operation and maintenance costs for Van Lare are presented in
Table 35.  Note that two periods are shown — one corresponding to a time
when phosphorus removal was not being practiced and one when phosphorus
removal was practiced.  Each of these is based on five months of actual plant
records extrapolated to a one year period.  These costs are reported in
dollars of their respective periods and are therefore not indexed.  Based on
the Consumer Price Index for all urban consumers (CIP-U) (Department of Labor,
1979), the rate of increase was 11.8.percent fo'n August"1978 to August 1979
(unadjusted) for all items in the CPI expenditure category.  This can be used
as an approximate means to account for inflation in comparing the two periods.
The extremely high power costs listed in Table 35 are mostly due to sludge
incineration which is supplemented with oil.

     Table 36 presents a summary of operation and maintenance costs associ-
ated with phosphorus removal at Van Lare.  Labor costs associated with
phosphorus removal are not very significant.  As is the case at the GCO plant
when phosphorus removal was started, no additional  personnel were hired.  It
is estimated that only two man-hours per week are allocated to phosphorus
removal.  Specifically, using a rate of $7.00 per hour (from plant records)
only $728 per year is spent.

     The power costs directly associated with phosphorus removal are also
insignificant.  They were computed by converting electrical requirements for
pumping the alum and polymer to the primary sedimentation, basins.  Both are
pumped by 1/2 HP (373 watts) motors and it is assumed that both are operated
continuously.  An average rate of $0.029 per killowatt hour was used, which
was obtained from actual  plant records.   Although both Van Lare and GCO are
in the same area (Rochester), Van Lare being a larger consumer of electricity
is charged a lower rate by the power company.

     Finally, chemical costs were derived from actual costs incurred for  -
liquid alum and the polymer over the five months period extrapolated to one
year.  The total includes $233,141 for alum and $27,532 for polymer.  As was
the case with GCO, the chemical costs are the most significant item in terms
of phosphorus removal costs.

     Table 37 shows cost associated with the additional sludge generated from
phosphorus removal.  The alum and polymer quantities are based on actual .
dosages used during the field study.  The sludge associated with phosphorus
removal was calculated based on the stbichiometric relationship of Al+3 to
soluble phosphorus (Vesilind, 1979).  It also includes the addition of
suspended solids removed in primary sedimentation due to alum.  The total

                                    125

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                TABLE 35.   VAN LARE - TOTAL PLANT O&M COSTS

Before Phosphorus Removal After Phosphorus Removal
(Feb-June 1978) (Feb-June 1979)
$/Year
Labor 613,113
Power 2,090,599
Chemical 334,035
Miscellaneous 68,737
Total O&M 3,106,484
$/1000 Gallons1 $/Year
0.021 756,226
0.071 2,934,250
0.011 819,655
0.002 7,560
0.105 4,517,691
$/1000 Gallons
0.020
0.079
0.022,
0.002
0.123

TABLE 36. ASSOCIATED
O&M COSTS FOR PHOSPHORUS REMOVAL
- VAN LARE


Labor
Power
Chemical
Total
$/Year
728
190
260,674
261,592
$/100.0 Gallons
0.0001
0:0001
0.007
0.007

TABLE 37.
VAN LARE SLUDGE PRODUCTION AND
CHEMICAL DOSAGES FOR P REMOVAL
(BASE PERIOD: SUMMER, 1979)


2
Chemicals - Polymer
Alum lbs/106 gals
141.7 0.684
P Sludge2 Total Sludge
Ibs/I06gals lbs/106 gals
252 1529
P Sludge Cost
$/1000 Gallons
0,004

1/I/I000 gallons is equivalent "to $/3.785 m3
2lbs/106 gallons is equivalent to 0.12 g/m3
                                    126

-------
 quantity of sludge  produced  is  from plant records  for  the  sampling.period.
 The costs associated  with  phosphorus sludge  processing is  based  on a  unit
 cost of $158 per ton  of dry  solids,  taken from plant records  during the
 sampling period.  Again this unit  cost  would be on the liberal side as the
 alum sludge would be  more  difficult to  process than the mixture  of primary
 and secondary and alum  sludge on which  the $158 figure is  based.

 Analysis of Performance

      The Van Lare wastewater treatment  plant which discharges directly into
 Lake Ontario has  an effluent standard of  1.0 mg/L.  The wastewater which
 enters  the plant  is generally low  in total phosphorus  averaging  3.8 mg/L
 during  the field  sampling.   This is  mainly due to the phosphorus  ban on
 detergents in New York  State and a large  industrial input  which  is low in
 phosphorus.   Becuase  of this, a low effluent phosphorus level can be  achieved
 through conventional  primary sedimentation and the activated  sludge process,-
 without the addition  of chemicals.

      The data indicate  that  through  the biological  side of the plant, the
 average effluent  phosphorus  concentration was  1.5  mg/L.  The alum primary
 effluent had a phosphorus  concentration of 1.3 mg/L.   This would result in a
 plant effluent of 1.5 mg/L total phosphorus,  which .clearly would not  be
 acceptable.   It should  be  pointed  out,  however,  that these data were  col-
 lected  for a two  week period (rather than a  one month  average) and that
 during  the sampling period several  of the biological side,  primary and one of
 the secondary sedimentation  basins were not  in operation.  The alum effluent
 had a particulate phosphorus concentration of  1.1  mg/L  and the biological
 effluent had a particulate concentration  of  1.1  mg/L which would result in
 a  plant particulate phosphorus  concentration  of 1.1.   Therefore, most of the
 plant phosphorus  effluent was particulate, and the  fact that the clarifiers
 were!overloaded might be somewhat  responsible.

      The biological effluent consisted  of 30 mg/L  8005  and 53 mg/L SS while
 the alum effluent consisted  of  151 mg/L BODs and 53 mg/L SS. • Thus, the
 plant effluent, which would  be  54  mg/L  BODs and  53 mg/L SS would also not
 meet the secondary  treatment standards, based  on the two weeks of field data.

      A  plot  of phosphorus concentrations  versus  overflow rates for the
 primary sedimentation basin  in  which  the  alum  and  polymer  were added  is
 shown in Figure 45.   The basin  had a  design of 1000 gallons per day per
 square  foot  (40.7 m3/nr/day).   The points  on the far right occurred during
 a  storm.   No distinct trends  can be  identified by  the  data.

      Alum was  added to  the primary tank at a concentration of 3.7 mg/L Al+3.
 The soluble  phosphorus  concentration  in the influent was 1.1 mg/L and the
 total phosphorus  was  3.8 mg/L.  As summarized  in Table  26  the resulting
 A1:P  molar ratios on  a  soluble  P and  total P basis are  3.8 and 1.2,  re-
 spectively.   Jar  tests  conducted on  the raw wastewater  are shown in Figure
•46  (unadjusted  pH)  and  Figure 47 (pH  adjusted  to 6).  Note that the data for
 an  alum dosage  of zero  are for  controls and do  not match the initial  data as
 settling had occurred in the jar test beakers.  Also for Figure 47, alum was
 added to the samples  and then the pH was  adjusted  to 6.0.   The jar test

                                   127

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results confirm the plant performance data for P removal, indicating that
the alum dosage being used is not effective in reducing the total P below
1 mg/L.  This is because the alum is being added to raw wastewater; conse-
quently, alum is being used to coagulate the solids of the raw wastewater as
well as for P removal.  No jar test experiments were performed using the
polymer employed at the Van Lare plant.  However, comparison of plant phos-
phorus data with jar test results indicate that a considerable fraction of
the remaining phosphorus after treatment is particulate.  This particulate
P might be removed by increasing the alum dosage, lowering the pH, and/or
optimizing the polymer dosage.

Alternatives to Meet a 0.5 mg/L Limit

     Suggesting a feasible alternative approach for the Van Lare plant to
meet a 0.5 mg/L effluent standard would be very difficult on the meager
information available in this study.  Because of the complex and unusual
treatment approach currently being used and because of the final settling
problems observed during the monitoring period, any phosphorus removal
alternative suggestion would be highly speculative.  Furthermore, any new
approach would probably require significant alteration of the current
operation and, quite likely, require additional capital expenditure.

     It might be possible for the Van Lare plant to practice phosphorus
removal in the same manner as the GCO plant.  This approach would require
biological treatment of the entire flow, with phosphorus removal being
achieved by addition of liquid alum to the mixed liquor effluent from the
aeration basins.  The field data (Section 6) indicated an average value of
0.3 mg/L soluble phosphorus in the effluent from the biological side of the
plant.  Therefore, an alum dosage of 16 mg/L would be necessary for an Al:P
molar ratio of 2:1.  A polymer addition to the final clarifiers at a dosage
of approximately 0.5 mg/L might also be necessary to ensure effective solids
removal.  Assuming costs of $0.056 per pound ($0.12/Kg) for alum and $1.32
per pound ($2.90/Kg) for polymer, the chemical costs would be $0.013/1000
gallons of $435,159 per year, based on an average daily flow of 102 mgd
(3.86x105 m3/day).

     Based on the stoichiometric relationship between Al+3 and phosphorus,
33 Ibs of aluminum phosphate sludge would be generated from phosphorus
removal resulting in a cost of $0.003/1000 gallons treated for $96,592 per
year (based on a unit cost of $158.22 per ton of dry solids process).

     The capital expenses for adding the above phosphorus removal approach
to secondary treatment at Van Lare are impossible to estimate at this time.
Based on the field data it would appear that the final  settling facilities
at the plant are already overloaded.  Any costs for upgrading the secondary
sedimentation facilities could not be totally attributed to phosphorus
removal.  In order to assess the true investment necessary at the Van Lare
plant to meet a 0.5 mg/L effluent phosphorus standard,  a major study would
have to be made to determine all the ramifications - such as available
land, effect on pumping, sludge processing, etc. - which might result.
                                    131

-------
                                REFERENCES
 1.


 2.



 3.



 4.



 5.
APHA, Standard Methods.  1975.
Association, Washington, D.C.
14th Edition, American Public Health
Armstrong, D.E., M.A. Anderson, J.R. Perry, and D. Flatness,.  1977.
Availability of Pollutants Associated with Access to the Great Lakes.
Unpublished, EPA Progress Report.  University of Wisconsin, Madison.

Armstrong, D.E., R.F. Harris, and J.K. Syers.  1971.  Plant available
phosphorus status of lakes.  Final Report.  Water Resources Center,
University of Wisconsin, Madison.  25 pp.

Chamberlain, W. and J. Shapiro.  1969.  On the Biological  Significance
of Phosphate Analysis; Comparison of Standard and New Methods with a
Bioassay.  Limnol.  Oceanogr., 14, 921-927.

Cowen, W.F. and G.F. Lee.  1976.  Phosphorus Availability in Particulate
Materials Transported by Urban Runoff.  Jour. Water Pollution Control
Fed., 48(3), 580-91.
 6.  DePinto, J.V.  1978a.  Phosphorus Availability of Aquatic Sediment
     Material: A Review.  Environmental Engineering Technical Report.
     Clarkson College of Technology, Potsdam, N.Y.  24 pp.

 7.  DePinto, J.V.  1978b.  Annual Progress Report of EPA Grant No. R-804937.
     November 1, 1976 - October 31, 1977.

 8.  Dorich, R.A. and D.W. Nelson.  1978.  Algal Availability of Soluble
     and Sediment Phosphorus in Drainage Waterof the Black Creek Watershed.
     Unpublished report from Purdue Univ. Agricultural Experiment Station.
     20 pp.

 9.  Fitzgerald, G.P.  1970.  Aerobic Lake Muds for the Removal  of
     Phosphorus from Lake Waters.  Limnol. Oceanogr., 15, 550-55.

10.  Goltermann, H.L., C.C. Bakels and J. Jakobs-Mogelin.  1969.
     Availability of Mud Phosphates for the Growth of Algal.   Verh. Internat.
     Vevin. Limnol., 17, 467-479.

11.  Great Lakes Basin Commission.  1979.  Personal Communication.

12.  Gregor, D.J. and M.G. Johnson.  1979.  Nonpoint Source Phosphorus
     Inputs to the Great Lakes.  Presented at the llth Annual Cornell
     University Waste Management Conference.  Rochester, NY.
                                    132

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13.  IJC.  1978.  Great Lakes Water Quality Agreement of 1978.

14.  IJC.  1978.  Great Lakes Water Quality, 1977, Appendix C.   Remedial
     Programs Subcommittee International Joint Commissions.  Great Lakes
     Water Quality Board, 6th Annual Report.

15.  IJC.  1979.  Inventory of Major Municipal and Industrial  Point Source
     Dischargers in the Great Lakes Basin.  Great Lakes Water Quality Board
    -Remedial Programs Subcommittee.

16.  Logan, T.O., F.H. Verhoff, and J.V. DePinto.  1979.  Biological
     Availability of Total Phosphorus.   Technical Report Series.   Lake Erie
     Wastewater Management Study.  U.S. Army Engineer District, Buffalo,
     N.Y.  62 pp.

17.  McKosky, P.M.  1978.  Laboratory Study of the Kinetics of Phytoplankton
     Decomposition and Subsequent Phosphorus Regeneration.   M.S.  Thesis.
     Clarkson College of Technology,  Potsdam, N.Y.   99 pp.

18.  New York State Department of Environmental  Conservation.   1979.
     Descriptive Data of Sewage Treatment Plants in  New York State.

19..  Ontario Ministry of the Environment.  1977.  Water and Wastewater
     Treatment Works in Ontario.

20.  Peters, R.H.  1977.  Availability  of Atmospheric Orthophosphate.
     J. Fish. Res. Board Can., 34, 918-924.

21.  Sagher, A., R.F. Harris, and D.E.  Armstrong.  1975.  Availability of
     sediment phosphrous to microorganisms.   Technical  Report WISWRC-75-01.
     Water Resources Center, University of Wisconsin, Madison.

22.  Sagher, A.   1976.  Availability of soil runoff  phosphorus  to algae.
     Ph.D. Dissertation.  University of Wisconsin, Madison.  176  p.

23.  Scheiner, D.  1976.  Determination of Ammonia and Kjeldahl Nitrogen
     by Indophenol Method.  Water Research 10:37.

24.  USEPA.  1976.  Methods for Chemical Analysis of Water and  Wastes.
     U.S.E.P.A.  Office of Technology Transfer, Cincinnati,  Ohio.

25.  U.S. Environmental  Protection Agency.  1978a.  Construction  Costs for
     Municipal Wastewater Treatment Plants:  1973-1977.   EPA 430/9-77-013,
     MCD-37.

26.  U.S. Environmental  Protection Agency.  1978b.  Energy Consumption of
     Advanced Wastewater Treatment at Ely, Minnesota.  EPA600/6-78-001.
                                     v
27.  U.S. Department of Labor.  1979.  CPI Detailed  Report, August.
     Bureau of Labor Statistics.
                                    133

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28.  Vallentyne, J.R. and N.A. Thomas.  1978.  Point tributary, diffuse
     tributary, runoff.  Fifth Year Review of Canada-United States Great
     Lakes Water Quality Agreement Report of Task Group III.

29.  Vesilind, P.A.  1979.  Treatment and Disposal of Wastewater Sludges.
     2nd Edition, Ann Arbor Science Publishers, Inc.

30.  Weston Environmental Consultants-Designers.  1977.  Wastewater
     Treatment Processes and Systems, Performance and Cost.

31.  Wildung, R.E., R.L. Schmidt, and R.C. Routson.  1977.   Phosphorus
     status of eutrophic lake sediments as related to changes in
     limnological conditions - phosphorus mineral components.  Jour.  Env.
     Qua!. 6(1):100-104.

32.  Williams, J.D.H., J.K. Syers, S.S. Shukla, R.F. Harris,  and D.E.
     Armstrong.  1971.  Levels of inorganic and total phosphorus in lake
     sediments as related to other sediment parameters.  Envir. Sci.
     Techno!. 5:113-1120.
                                    134

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r-.i  UfSP
Clarkson
                                     APPENDIX A

                          QUESTIONNAIRE AND  SURVEY WORK'SHEET
      Dear Sir:

           At the present time, our Environmental Engineering .group is working
      in cooperation with the United States Environmental Protection Agency on a
      project entitled, "Analysis of Phosphorus Removal in Great, Lakes Basin
      Municipal Treatment Plants".   This project involves an analysis of the
      costs and benefits pertaining to the establishment of regulations regarding
      the removal of phosphorus from municipal wastewater in the Great Lakes
      Basin in order to generate useful information for deciding upon final
      effluent regulations.

           As part of this prqject, a survey is being conducted of municipal
      treatment plants larger than one MGD in the lower Great Lakes Basin in
      order to evaluate their treatment approach and plant operation; and to
      .document their.costs.  Your answers to the enclosed questionnaire and any
      further information you could supply would help us greatly in regard to our
      survey.

           We greatly appreciate your attention to this questionnaire, and please
      call me  (315-268-6515) if you have any questions concerning this question-
      naire or our project.            '                           ,    ,

                                        Sincerely,
                                        Michael Switzenbaum
                                        Assistant Professor
                                        Department of Civil.. and
                                        Environmental Engineering

      Enclosures

      CLARKSON COLLEGE, POTSDAM, NEW YORK, 13676
                                       135

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                          APPENDIX A (continued)
QUESTIONNAIRE
1.  What is the location of your..wastewater/treatment plant? 'Please give
    complete mailing address, name of plant and stream receiving discharge.

2.  What type of plant is it?  (Examples: conventional activated sludge,
    extended aeration,'contact stabilization, trickling filter,  primary
    treatment, etc.)

3.  What is the average daily flow and design flow at your plant?

4.  What method of phosphorus removal is being practiced at your plant?
    Please be specific as to type of chemical used and point at  which
    chemical is applied and any additional unit processes used in
    conjunction with phosphorus removal.  (Example: Alum added to effluent
    from trickling filter between filter and secondary clarifier followed
    by filtration.

5.  What are the average concentrations of phosphorus (both soluble and
    particulate) in the influent and. effluent of your plant?  What is the
    frequency of analysis (daily, weekly, etc.) and what is ;the  sampling
    basis (grab, or composite)?

6.  If the removal of phosphorus involves the use of chemicals,  please
    indicate quantities used (indicate dosage).

7.  Additional information.
                 PLEASE RETURN IN SELF-ADDRESSED STAMPED
                 ENVELOPE BY JULY 15, 1979.
                                   136

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                         -APPENDIX A (continued)
               WASTEWATER TREATMENT PLANT WORK SHEET
Plant Reference Numer ________  Source  of Information
  1.  Treatment plant name and address
  2.  Location
        a)  Lake Basin:
        b)  Regulatory region:
        c)  County:
        d)  City:
        e)  Discharge site:
  3.  Type of plant
  4.  Phosphorus treatment approach
        a)  Chemical(s)  used:
        b)  How much:
        c)  Where  in  process:
  5.  Flow data
        a)  Average daily flow
        b)  Design flow
  6.   Influent and Effluent  quality
        a)   Influent:   Total  P
        b)   Effluent:   Total  P
        c)   Basis:
Soluble P
Soluble P
  7.   Annual  phosphorus  load  (metric tons/year)
                                  137

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                                APPENDIX  B



                     WASTEWATER PLANT PERFORMANCE  DATA





           HASTEWATER PLANT  PERFORMANCE.  MONTHLY AVERAGES,  1979*

Wastewater
Treatment
Plant




Monthly
Average
Influent
Flow
(M6D)
Gates-Chili -Ogden
January 14.1
February
March
Apri 1
Frank Van
February
March
Apri 1
May
June
Big Sister
January
February
March
April
May
June
Ely
January
February
March
April
May
June
12.
16.
15.
Lare
92.
124.
117.
93.
88.
5
5
5

1
9
2
1
0
BOD
(mg02/L)
108
112
80
89

148.0
134.5
144.9
195.9
187.1
SS
(mg/L)
133
120
89
91

114.8
109.1
108.7
133.7
134.5
TP
(rug P/L)
4.7
4.6
3.9
3.6

2.64
3.01
2.13
2.94
2.86
Effluent
BOD
(mg02/L)
7
6
10
5

24.
32.
33.
33.
27.





9
0
2
1
4
SS
. (mg/L)
13
13
13
10

22.
42.
26.
30.
25.





1
1
7
7
5
TP
(mg P/L)
0.
0.
0.
0.

0.
0.
0.
1.
0.
80
70
96
90

98
99
75
04
82
Creek
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                                   TECHNICAL REPORT DATA
                            (Please read Instructions on the reverse before completing)
1. REPORT NO.
  EPA-6QO/2-Sn-117
                             2.
                                                           3. RECIPIENT'S ACCESSION-NO.
4. TITLE AND SUBTITLE
  Phosphorus Removal  in  Lower Great Lakes  Municipal
  Treatment Plants
                    5. REPORT JDATF
                      August  1980 (Issuing Date)
                    6. PERFORMING ORGANIZATION CODE
7-AUTHOR(S)Joseph V. DePinto, James  K.  Edzwald, Michael S.
  Switzenbaum and Thomas C. Young
                                                           8. PERFORMING ORGANIZATION REPORT NO.
9. P
                              i ADDRESS
  EBFORMING ORGANIZATION &LAME AND ADDI
  uarkson uoYiege of Technology
  .-Department of Civil and Environmental  Engineering
  Potsdam, New York  13676
                     10. PROGRAM ELEMENT NO.
                      PE  I35B1C  Task C/17
                     11. CONTRACT/GRANT NO.
                          R-806817
12. SPONSORING AGENCY NAME AND ADDRESS
  Municipal Environmental Research Laboratory -Cin., OH
  Office of Research  and Development
  U.S. Environmental  Protection Agency
  Cincinnati, Ohio  45268
                     13. T,*P.E O
 JIOD COVERED
                     14. SPONSORING AGENCY CODE
                        EPA/600/14
15. SUPPLEMENTARY NOTES
  E. F. Barth, Project Officer
(513) 684-7641
16. ABSTRACT
            This  report discusses a  survey of phosphorus treatment approaches and
  accomplishments for all lower Great  Lakes basin plants with  flows greater than
  1 mgd; field  operation monitoring  studies to evaluate the  performance of four
  municipal treatment plants practicing  phosphorus removal,  including a determination
  of the bioavailability of the wastewater phosphorus; and ,an  analysis of costs at
  each of four  plants monitored,  including incremental costs to  achieve a Oi5 mg/1
  standard.

       Of the 229 plants in this  survey,  52 percent are achieving an effluent total
  phosphorus concentration of 1.0 mg/1,  while only 8.3 percent (19 plants) are meeting
  a 0.5 mg/1 standard.  If all plants  in the Lake Erie basin not currently achieving
  a 1.0 mg/1 standard were to do  so, the municipal load would  be reduced by 2165 MT/yr.
  A standard of 0.5 mg/1 met in the  Lake Erie basin would reduce the current load
  by 3264 MT/yr.   Similar standards  achieved in the Lake Ontario basin would reduce
  municipal loads by 1450 and 2085 MT/yr., respectively.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                              b.lDENTIFIERS/OPEN ENDED TERMS
                                  c.  COSATI Field/Group
  Wastewater
  Activated sludge process
  Chemical removal
        Bioavailable phosphorus,
        Chemical  precipitation,
        Phosphorus removal,
        Filtration
                                                                              13B
13. DISTRIBUTION STATEMENT
   Release  to  Public
        19. SEqURITYjCLASjS (This Report)
                                                                         21. NO. OF PAGES
         JnciassTMed
161
                                              2O. SECURITY CLASS (This page)
                                               Unclassified
                                                                         22. PRICE
EPA Form 2220-1 (9-73)
     147
                                                          • U.S. GOVERNMENT PRINTING OFFICE:  1980 — 657-165/0128

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