United States
                             Environmental Protection
                             Agency
       Hazardous Waste Engineering
       Research Laboratory
       Cincinnati OH 45268
                             Research and Development
       EPA/600/M-86/025 Jan. 1987
                             ENVIRONMENTAL
                             RESEARCH   BRIEF
           Microbial Degradation of 2,4,5-T and Chlorinated Dioxins
                                          A. M. Chakrabarty
This report from the  University of Illinois  College  of
Medicine at Chicago covers three years of research under
a Cooperative Agreement.

A pure culture of Pseudomonas cepacia strain AC1100,
isolated from a chemostat enrichment culture experiment,
is capable of growing on 2,4,5-T as its sole source of carbon
and energy. Metabolic pathway studies indicate the activity
of both constitutive and inducible enzymes. In laboratory
experiments,  soil contaminated with  2,4,5-T could be
detoxified by AC1100 treatment, with the liter  of AC11 00
rapidly falling to nearly undetectable levels after the 2,4,5-
T was substantially degraded.

Extensive homology observed between plasmids points to
the  role of  plasmid genes in the evolution and spread of
degradative characters against toxic chemical compounds.
A 1.3 kilobase pair DNA repeated sequence was found
in strain AC1100. The specificity of this sequence  to
AC1100 suggests that this unique  sequence may  be a
useful genetic probe of strain AC1100 and other novel
Pseudomonas strains which are under consideration for
deliberate release to aquatic and terrestrial environments.

Introduction

This research brief describes the effort conducted under
a cooperative agreement between the U.S. Environmental
Protection  Agency and the Department of Microbiology
of the University of Illinois College of Medicine at Chicago.
The research relates to the development and continued
biochemical and genetic studies of a specific bacterial
strain, Pseudomonas cepacia AC1100. These microorga-
nisms can  utilize a recalcitrant compound such as 2,4,5-
trichlorophenoxyacetic acid (2,4,5-T) as  a sole source  of
carbon and energy,  and can dechlorinate a  variety  of
chlorophenols. Additionally, such a strain is shown to be
highly effective in removing large quantities of 2,4,5-T from
contaminated soil, thereby allowing the growth of plants
that  are normally  sensitive to  the presence of  small
quantities of 2,4,5-T. This work attempted to elucidate the
organisms' metabolic pathways of degradation and gene
recombination involved in the evolution of the strain.

The Role of Plasmids

Plasmids are known to play a major role in the biodeg-
radation of  a variety of complex organic compounds.
However, only a few plasmids, such as pAC25, pWR1,
and pAC31 are known  to allow complete dechlorination
of the  compounds. The evolution of  a chlorobenzoate
degradative plasmid such as pAC25 specifying a number
of new enzymes having maximal activity  towards the
chlorinated substrates, raises the interesting question as
to how new degradative functions evolve in nature.

Several lines of evidence suggest that plasmids interact
with  one another to greatly extend the substrate range
of plasmid-specified enzymes. Growth  in a chemostat of
3-chlorobenzoate-degrading Pseudomonas  species  B13
with 4-chloro- or 3,5-dichlorobenzoate allows emergence
of strains capable  of degrading  these  compounds only
when other Pseudomonas strains  harboring  the TOL
plasmid are  introduced into the chemostat. This project
demonstrated that  under such conditions, a part of the
TOL plasmid undergoes transpostion on the chromosome
to provide the broad substrate specific benzoate oxygenase
function necessary for the conversion of chlorinated
benzoates to the corresponding chlorocatechols.

Since growth with 3,5-dichlorobenzoate needs the
participation of additional enzymes capable of dechlori-
nating the chlorolactone and chloromaleyl acetic acid, a
segment of TOL containing the replication/incompatibility

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genes and a segment of the chlorobenzoate plasmid pAC27
are recombined. This recombination  gives  rise to a
separate plasmid, which then  undergoes mutational
divergence to generate new enzymatic  activities for the
dechlorination of the chlorinated  intermediates. Thus,
plasmids appear to play a vital role in nature as carriers
of duplicated  genes for  their  ultimate  mutational
divergence to generate new degradative functions.

Gene Regulation

Other useful information emerging from  the  studies of
degradative plasmids  relates to the extent of clustering
of degradative genes on such plasmids. A physical map
of the chlorobenzoate degradative plasmid  pAC27 was
constructed to demonstrate that the degradative genes are
clustered within a single  EcoFM fragment of the plasmid.
The  cloned chlorobenzoate degradative genes, when
transferred to Escherichia  coif, are not expressed. The
specificity of plasmid promoter sequences in Pseudomonas
may help explain why, in spite of the transmissible nature
of such  plasmids, pseudomonads are  the  predominant
scavengers in nature.

Based on the premise that plasmids evolve by recruitment
of genes from other plasmids or from the chromosome,
and  that new  genetic functions are acquired through
mutational  divergence of  genes  specifying  analogous
biological functions, laboratory culture conditions were
developed which have yielded a strain of Pseudomonas
cepacia (strain AC1100) that can utilize 2,4,5/T as a sole
source of carbon and energy. Also, the AC1100 resting
cell  suspensions were found to be capable of oxidizing
and dachlorinating a number of chlorophenols. Dehaloge-
nation studies  revealed that different halogen atoms on
analogous molecules  can lead to different efficiencies of
dehalogenation. These results suggest that halogen atoms
are  removed in decreasing order FI>CI>Br>l, consistent
with the general literature information on dehalogenation
 of halogenated aromatic molecules. The implication is that
 other halogenated compounds can be considered similarly
 biodegradable.

The regulation of the dehalogenating functions of AC1100
 has been partially elucidated.  The enzyme(s)  for  the
conversion of 2,4,5-T to 2,4,5-TCP are constitutive,  but
the  enzymes  needed for  2,4,5-TCP degradation  are
 inducible. Also, 2,4,5-TCP  (or some metabolite), but not
 pentachlorophenol (PCP), can serve as an  inducer.

 Development of Strain AC 1100

 Pseudomonas  cepacia AC1100 was  developed  in  the
 laboratory using a chemostat. When the chemostat was
 switched over to 2,4,5-T as the sole source  of carbon and
 energy, it was acting as  a continuous enrichment culture
 and breeding ground for bacteria with the ability to rapidly
 metabolize 2,4,5-T and derive carbon and energy from it.
 Thus,  as the  genetic  information necessary for  the
 complete degradation of 2,4,5-T was evolving, growth on
 2,4,5-T alone  was the only selective pressure  present.
 There was no selective pressure on this organism to evolve
 an  effective means of regulating the 2,4,5-T degradative
 pathway in the presence  of alternate carbon  sources.
 Therefore, the  manner by which the 2,4,5-T degradative
pathway is regulated is thought to reflect the "evolutionary
youth" of this organism.

Homologies

Plasmid pJP4, like other 2,4-D-degradative plasmids such
as  pJP1, pJP2,  etc., was originally  isolated  from
Alcaligenes sp., whereas both pAC25 and pWR1  were
originally isolated from Pseudomonas sp. The question that
arises  is  whether the difference in expression is due to
(1) an  inherent variation in the structural and regulatory
genes on the 2 plasmids or (2) to a mismatch of the signal
sequences present on plasmid pJP4 with the transcription-
translation machinery of the new host, i.e., Pseudomonas
sp. The  second  explanation  seems plausible, since
Pseudomonas plasmids are known to be expressed poorly
in other hosts, particularly the enteric bacteria. However,
the presence of unique structural features present in the
plasmid pJP4.aD.pea;;?.Jojrjdica.tejhajt a^variatipnjnjhe
continuity of the structural and regulatory genes pertinent
to 3-chlorobenzoic acid degradation is the major difference
between pAC25 and pJP4.

Physical  maps of pJP4 and pAC27 were constructed with
extensive homology observed between the chlorobenzoate
degradative plasmid pAC27 and the 2,4-D degradative
plasmid pJP4 concerning the chlorocatechol-degradative
genes and that between the same regions of pJP4 and
the resident  plasmids of the 2,4,5-T-degrading strain of
P. cepacia AC1100. This points to the role of plasmid genes
in  the evolution  and spread of degradative characters
against toxic chemical compounds. Although this pheno-
menon is well-known in the evolution and dissimilation
of antibiotic-resistance genes, no clear evidence for the
occurrence of a similar trait in soil bacteria was available
 until now.

The structural studies performed in this work point to the
 important role of direct and inverted repeats in the genetic
 rearrangements necessary for rapid transition from growth
 on one  substrate to that of a different substrate. The
 amplification  of  the structural genes in  absence  of a
 putative regulatory element is analogous to that observed
 in case  of  antibiotic  resistance to allow the host
 microorganisms to withstand  high and  toxic  concentra-
 tions  of such antibiotics. Many toxic chemicals, resemble
 antibiotics in terms of their inherent toxicity, both towards
 animals as well as  microorganisms, and it is little wonder
 that microorganisms employ essentially identical tools, i.e.,
 deletion, fusion, insertion, and other modes of genetic
 rearrangements, to help evolve new degradative functions.
 Continued studies of  such processes  are expected  to
 provide  unique insights regarding the mode of evolution
 of new biological functions in bacteria.

 A DNA Repeated Sequence

 In an effort to identify and localize AC1100  genes
 associated with 2,4,5-T degradation, transposon insertion
 mutagenesis was  used  to generate mutants blocked in
 the 2,4,5-T degradative pathway. A 1.3 kilobase pair DNA
 repeated sequence was found in the 2,4,5-T-degrading
 Pseudomonas cepacia strain AC1100. One  copy of this
 sequence RSnoo-l was located  near the chromosomal
 transposon 5 insertion site of a 2,4,5-T-negative mutant

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designated PT-88.  Thus,  RSnoo-l appears to be closely
associated with at  least one 2,4,5-T gene and may have
played a  role in  gene rearrangement. As judged by
Southern hybridization analysis, the repeated sequence
was not homologous to DNAs from several other P. cepacia
DNAs and was absent in strains of P. aeruginosa, P. putida,
P. mendocina, and other pesudomonads isolated from soil
samples. The specificity of RSnoo-l to AC1100 suggests
that this unique sequence may be a useful genetic probe
of strain AC1100 and other novel Pseudomonas strains
which are under consideration for  deliberate  release to
aquatic and terrestrial environments.
7.   Tomasek, P., B. Frantz, D. K. Chatterjee, and A.  M.
    Chakrabarty. 1986. "Genetic and Molecular Basis
    of  the  Microbial  Degradation  of  Herbicides and
    Pesticides," In: Biotechnology for Solving Agricul-
    tural Problems, Augustine, P. C., H. D. Danforth, and
    M.  R.  Bakst, eds., Marinus Nijhoff  Publishers,
    Dordrecht, pp. 355-368.
 Detox/cation of Contaminated Soil

 In laboratory experiments, soil previously contaminated
 with as much as 5,OOO /ug of  2,4,5-T/g :of soil could be
 detoxified by AC1100 treatment, allowing the growth of
 plants sensitive to less than 10 /ug 2,4,5-T/g of soil. Soil
 contaminated with  as  much as 20,000 /ug of 2,4,5-T/g
 of soil showed greater than 90% degradation after six
 weekly AC1100 treatments.  After 2,4,5-T has  been
 substantially degraded in contaminated soil, the titer of
 AC1100 rapidly falls to nearly undetectable levels.
 Publications

 The following publications describe research supported by
 Cooperative  Agreement, CR809666, between the U.S.
 Environmental  Protection Agency and  the  University of
 Illinois College of Medicine at Chicago:
  1.   Chakrabarty, A. M., 1985. Genetically manipulated
      microorganisms and their products in the oil service
      industries. Trends in Biotechnology, 3:32-38.

  2.   Frantz, B., and A. M.  Chakrabarty. 1986. "Degrad-
      ative Plasmids in Pseudomonas." In: The Bacteria,
      Sokatch, J. R., and  L.  N. Ornston, eds.. Vol. 10, Ch.
      9, Academic Press,  New York, pp. 295-323.
 .^i. „ ^?.;'i* s-:*n' i? ir-rW-."! :?«siV}  Vi **%!--;  -£~%i ?r- •=;.?, i •- ^ -"-*>•.; *.^. -5*:^;;.
  3.   Ghosal, D., I.-S.  You, D. K. Chatterjee,  and A. M.
      Chakrabarty. 1985.  Genes specifying degradation of
      3-chlorobenzoic acid in  plasmids pAC27 and pJP4,
      Proc. Natl. Acad. Sci. USA. 82:1638-1642.

  4.   Ghosal, D., I.-S.  You, D. K. Chatterjee,  and A. M.
      Chakrabarty. 1985. Microbial  degradation of halo-
      genated compounds. Science,  222:135-142.

  5.   Ghosal, D., I.-S.  You, D. K. Chatterjee,  and A. M.
      Chakrabarty. 1985. "Plasmids  in the Degradation of
      Chlorinated Aromatic Compounds." In: Plasmids in
      Bacteria, Helinski,  D. R. et al, eds. Plenum Press,
      New York. pp. 667-686.

  6.   Tomasek,  P., B.  Frantz, and A. M. Chakrabarty:  a
      forthcoming paper  on repeated  sequences of DNA
      discovered in Pseudomonas cepacia strain AC1100.

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