vvEPA
                             United States
                             Environmental Protection
                             Agency
                               Environmental Research
                               Laboratory
                               Athens GA 30613-7799
                             Research and Development
                               EPA/600/M-89/009  Aug. 1990
ENVIRONMENTAL
RESEARCH  BRIEF
    Pathway Analysis of Chemical Hydrolysis for 14 RCRA Chemicals

               Heinz P. Kollig, J. Jackson Ellington, Eric J. Weber, and N. Lee Wolfe
The probable pathways of transformation by chemical
hydrolysis in an aqueous environment were postulated for
14 chemicals. Acid, base, and neutral half-lives at pH  7
are given  for the chemicals and their products.  A
structural formula is provided for each chemical.

Introduction

Assessment of potential risk posed to humans by man-
made  chemicals  in  the environment  requires the
prediction  of environmental concentrations  of those
chemicals under various scenarios. Whether mathematical
models or  other assessment techniques are employed,
knowledge  of equilibrium and kinetic  constants (fate
constants)  is required to predict the  transport and
transformation of these chemicals.

Under  section 301 of the Resource Conservation and
Recovery Act (RCRA), EPA's Office of solid Waste (OSW)
has identified wastes that may pose a substantial hazard
to human health and the environment. RCRA requires that
EPA develop and promulgate criteria for identifying and
listing hazardous wastes, taking into account, among other
factors, persistence and degradability in the environment.
                In 1986, OSW proposed additions to the list of chemicals
                regulated under the Toxicity Characteristic  section of
                RCRA. A land disposal decision model developed at the
                Environmental Research Laboratory in  Athens, Georgia
                (ERL-Athens) was applied to  determine  maximum
                permissible  leachate concentrations resulting from the
                Toxicity  Characteristic Leachate  procedure for the
                additional chemicals. ERL-Athens had provided hydrolysis
                rates and sorption data for these chemicals. Response to
                the  Federal Register proposals for regulated  concen-
                trations prompted  OSW to  (1) change some transport
                functions in the model and  (2) remove from the list 15
                chemicals that hydrolyze in order to evaluate these
                chemicals in more depth.

                OSW requested that ERL-Athens postulate the probable
                pathways of transformation in an aqueous environment by
                chemical hydrolysis for the 15 chemicals. The' chemicals
                were acrylonitrile, carbon tetrachloride, chlordane, 6/s(2-
                chloroethyl)ether, chloroform, 1,2-dichloroethane, hepta-
                chlor,  lindane, methoxychlor, methylene chloride,  1,1,1-
                trichloroethane, 1,1,2-trichloroethane, 1,1,1,2-tetrachloro-
                ethane, 1,1,2,2-tetrachloroethane, and  toxaphene. Toxa-
                phene was not addressed in the pathway analysis,

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however,  because it  is  a  mixture of more  than 600
polychlorinated terpenes.

Pathway Analysis

A team of scientists met to discuss the hydrolysis rates
and probable pathways of transformation.  The  methods
used to  arrive at the  reaction  products  were  based
primarily  on  the team's experience  with  similar
compounds, their knowledge of the hydrolysis theory, and
their understanding of  structure  activity relationships. The
final stable products were identified as containing either no
hydrolyzable  functional  group  (NHFG)  or  non-labile
functional  group  (NLFG). Although the molecule with  a
non-labile functional  group contains  one  or  more
heteroatoms, they  are  so unreactive towards hydrolysis
that they will not hydrolyze. (Over the pH range  of 5 to  9
and at 15SC, half-lives will be greater than 50 years if they
react at alt.)

Literature searches were conducted afterwards to find
needed  fate  data for the intermediate  products of
hydrolysis. If the literature failed to provide the required
data, they were determined in the laboratory  if possible. All
half-lives were calculated at pH 7. The values were arrived
at by  adding the  acid and/or base portion  of the rate
constant  at  pH 7 to  the neutral  rate constant and
calculating the half-life according  to: t1'2  =  (In 2)/rate
constant.

Acrylonitrile (Rgure 1) hydrolyzes through the intermediate
product acrylamide to  acrylic acid, a compound that has
no  hydrolyzable functional  group. Ammonia  is  formed
along with acrylic acid.
  107-13-1
  acrytonitrite; Ref. 1
  kA - 3.7E2 M-'Y-i
  ka - 5.3E3
  t"2 - 1.2E3 Y
 79-06-1
 acrylamkte; Ref. 1
 kA - 31.5 M-1Y-1
 kM - 1.8E-2Y-1
 t"2 - 38 Y
 79-10-7
 acrylic acid
    NHFG
CH2=CHCN
CH2=CHCONHa
 CH2=CHCOOH
 Figure 1.    Acrylonitrile, hydrolysis pathway.
                                Carbon tetrachloride (Figure  2)  hydrolyzes to inorganic
                                products, carbon dioxide and hydrogen chloride,  with no
                                detectable intermediates.

                                Chlordane (Figure 3) hydrolyzes to the final stable product,
                                2,4,5,6,7,8,8-heptachloro-3a,4,7,7a-tetrahydro-4,7-
                                methano-1H-indene. Hydrogen chloride  is formed in  the
                                process. No other products have been observed. (Only the
                                c/s-isomer, CAS #5103-74-2, undergoes  hydrolysis due to
                                the 1 -exo, 2-exo orientation of the chlorine.)
                                 56-23-5
                                 carbon tetrachloride; Ref. 3
                                 kN = 1.7E-2Y-1
                                 t1'2 = 41 Y
                         ecu
                                 124-38-9
                                 carbon dioxide
                                     C02
                                    NHFG
                          7647-01-0
                          hydrogen chloride
                               4HCI
                               NHFG
                                 Figure 2.    Carbon tetrachloride, hydrolysis pathway.
57-74-9
chlordane; Ref. 4
kB = 38 M-'Y-1
ti«  = 1.8E5Y
5103-65-1
2,4,5,6,7,8,8-heptachloro-3a,4,7,7a-
tetrahydro-4,7-methano-iH-indene
          NLFG
                                                            Figure 3.    Chlordane, hydrolysis pathway.
                                bis(2-Chloroethyl)ether (Figure 4) hydrolyzes through the
                                intermediate product, 2-(2-chloroethoxy)ethanol, to the final
                                stable  products, 6/s(2-hydroxyethyl)ether  and  para-
                                dioxane.  The  2-(2-chloroethoxy)ethanol will  build  to  a
                                significant steady state concentration. Hydrogen chloride is
                                formed in the process.

                                Chloroform (Figure  5)  hydrolyzes to  inorganic  products,
                                carbon dioxide and hydrogen chloride.

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 111-44-4
 CICH2CH2OCH2CH2CI
 b/s(2-chloroethyl)ether; Ref 2
 kN  = 0.23 Y-1
 ti/2 = 3.0 Y
 628-89-7
 CICH2CH2OCH2CH2OH
 2-(2-chloroethoxy)ethanol; Ref. 2
 kN = 0.28 Y-1
 ti/2  = 2.5 Y
                    0
    123-91-1
    p-dioxane; Ref. 11
    NHFG
 111-46-6
 HOCH2CH2OCH2CH2OH
 fa/s(2-hydroxyethyl)ether; Ref. 11
     NHFG
                                  75-01-4
                                  vinylchloride; Ref. 6
                                  CH2 = CHCI
                                  kB<3.5M-iY-i
                                  kN<7.0E-2Y-i
                                  t1/2>10 Y
 74-86-2
 acetylene
 CH^CH
  NHFG
                                                       107-06-2  CICH2CH2CI
                                                       1,2-dichloroethane; Ref. 3
                                                       kB =5.5E-6 M-1Y-1
                                                       kN = 9.6E-3 Y-1
                                                       tl/2 =
                                107-07-3
                                2-chloroethanol; Ref. 2
                                CICH2-CH2OH
                                kN = 3.9E-2 Y-i
75-07-0
acetaldehyde
CH3-CHO
 NHFG
107-21-1
ethylene glycol
HOCH2-CH2OH
 NHFG
                                  Figure  6.    1,2-Dichloroethane, hydrolysis pathway.
 Figure  4.    ft/s(2-Chloroethyl)ether, hydrolysis pathway.
 67-66-3
 chloroform; Ref. 5
 kB = 2.1E3 M-1Y-1
 kN = 2.3E-5 Y-1
 ti/2 = 3.QE3 Y
CHCI3
 124-38-9
 carbon dioxide
     C02
     NHFG
 7647-01-0
 hydrogen chloride
       3HCI
       NHFG
76-44-8
heptachlor; Ref. 9
kN = 56Y-1
t1'2  = 1.2E-2Y
                                                             24009-05-0
                                                             1 -hydroxychlordene
                                                                  NLFG
                                                                                   Cl
Figure 7.    Heptachlor, hydrolysis pathway.
 Figure 5.    Chloroform, hydrolysis pathway.
1,2-Dichloroethane  (Figure 6)  hydrolyzes  to  the fairly
stable product vinyl chloride and to the final stable product
ethylene  glycol  through  the  intermediate product 2-
chloroethanol. Vinyl chloride may  further  hydrolyze to
acetylene at alkaline  pHs or to acetaldehyde  at near
neutral  pH. Ethylene  glycol  is the main product at near
neutral pH, and the reaction shifts to give vinyl chloride as
the pH increases.  Hydrogen chloride is formed in the
process.

Heptachlor (Figure 7)  hydrolyzes to  1-hydroxychlordene,
which has an estimated half-life of longer than 8 million
years at pH 7. Hydrogen chloride is formed in the process.
                                 Lindane (Figure 8) hydrolyzes through the  intermediate
                                 product,  1,3,4,5,6-pentachlorocyclohexene, to  the final
                                 stable products, 1,2,3-trichlorobenzene and 1,2,4-trichloro-
                                 benzene. Hydrogen chloride is formed in the process.

                                 Methoxychlor  (Figure  9)  hydrolyzes to the  final  stable
                                 product,  2,2-bis(p-methoxyphenyl)-1,1 -dichloroethylene
                                 under alkaline conditions, and to the final  stable product
                                 anisil  through the  intermediate  product anisoin  under
                                 acidic  or  near neutral conditions. Hydrogen  chloride  is
                                 formed in  the process. Anisoin oxidizes to anisil. A rate of
                                 oxidation was not available.

                                 Methylene  chloride  (Figure  10) hydrolyzes with  no
                                 detectable intermediates to  the final  stable products,
                                 formaldehyde and hydrogen chloride.

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58-89-9
lindano; Ref. 4             ci
ka « 1.74E6M-1Y-1
kN-1.05Y-i             cl
It/2 = 0.5 Y
                                ci
                             O
                                      ci
                                I
                               ci
319-94-8
1,3,4,5,6-pentachlorocyclohexene; Ref. 2
kB - 6.5E5 M-»Y-1
kN - 0.26 Y-i
lira . 2.1 Y
                                CJ
                                       ci
                                        i
                                 ci
                                              CJ
                                        I
                                       CI
87-61-6
1,2,3-trtohtorobenzene
                          120-82-1
                          1,2,4-trichlorobenzene
                                ci
                                i
            Llndane, hydrolysis pathway.
   1,1,1-Trichloroethane (Figure 11)  hydrolyzes to the two
   final stable  products, acetic acid and  1,1-dichloroethene.
   Hydrogen chloride  is formed in the process. The ratio  of
   acetic acid to 1,1-dichloroethene is dependent on pH and
   temperature. Production  of  1,1-dichloroethene  increases
   directly with pH and temperature.

   1,1,2-Trichloroethane (Figure 12) hydrolyzes to  the  final
   stable  product  hydroxyacetaldehyde  through  the
   intermediate product chloroacetaldehyde and to the  final
   stable  product 1,1-dichloroethene. Hydrogen chloride  is
   formed the process.

   1,1,1,2-Tetrachloroethane (Figure 13) hydrolyzes to the
   final product, 1,1,2-trichloroethylene. Hydrogen chloride is
   formed in the process.

   1,1,2,2-Tetrachloroethane (Figure 14) hydrolyzes to the
   final product, 1,1,2-trichloroethylene. Hydrogen chloride is
   formed in the process.
 72-43-5
 meUioxychtor; Ref. 7
 ks - 1.2E4 M-1Y-1
 (CN » 0.69 Y-'
 ti/2 . 1.0 Y
                         CH3O -'
                                        -CH  -
                                         CGI,
-OCH3
 2132-70-9
 2,2-bis(p-melhoxyphenyl)-
 1,1-dicriloroethylene; Ref. 7
                                    119-52-8
                                    anisoin; Ref. 7
                                        CH3-0-
 CH3-0-
                       - O - CH3
                                                                    - O - CH3
                                                   1226-42-2
                                                   anisil; Ref. 7
             NLFG
                                     CH3-0-
                                                                    - O - CH3
                                                    NHFG
 Figure  9.    Methoxychlor, hydrolysis pathway.

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75-09-2
methylene chloride; Ref. 8
kN = 1.01E-3Y-1
ti/2 = 686 Y
 50-00-0
 formaldehyde
   CH2 = O
    NHFG
                          CH2CI2
                           7647-01 -0
                           hydrogen chloride
                           2HCI
                                 NHFG
630-20-6
1,1,1,2-tetrachloroethane; Ref. 3
kB = 1.1E4M-1Y-1
kN = 1.4E-2Y-1
ti/2  = 47 Y
79-01-6
1,1,2-trichloroethylene; Ref. 3
   NLFG
CCI3CH2CI
CCI2 = CHCI
Figure 10.  Methylene chloride, hydrolysis pathway.
71-55-6
1,1,1-trichloroethane; Ref. 3
kN = 0.65 Y-1
t1/2  = 1.1 Y
64-19-7
acetic acid
CH3-COOH
  NHFG
                                  CCI3CH3
                           75-35-4
                           1,1-dichloroethene
                           CCI2 = CH2
                             NLFG
Figure 11.   1,1,1-Trichloroethane, hydrolysis pathway.
                                                           Figure 13.   1,1,1,2-Tetrachloroethane,  hydrolysis  path-
                                                                        way.
                                                            79-34-5
                                                            1,1,2,2-tetrachloroethane; Ref. 3
                                                            kB  = 1.7E7 M-IY-I
                                                            kN  = 5.1E-3Y-1
                                                            ti/2 = o.41 Y
79-01-6
1,1,2-trichloroethylene; Ref. 3
   NLFG
                                CI2CHCHCI2
CCI2 = CHCI
                                                           Figure 14.   1,1,2,2-Tetrachloroethane,  hydrolysis  path-
                                                                        way.
                             CI2CHCH2CI
79-00-5
1,1,2-trichloroethane; Ref. 3
kB = 5.0E4 M-1Y-1
kN = 2.7E-5 Y-1
ti«  = 1.4E2 Y
107-20-0
chloroacetaldehyde; Ref. 10
CICH2CHO
kB = 2.6E4 M-IY-I
kN = 7E-3 Y-i
ti/2 = 72 Y
 141-46-8
 hydroxyacetaldehyde
 OHCH2CHO
   NHFG
Figure 12.   1,1,2-Trichloroethane, hydrolysis pathway.
                            75-35-4
                            1,1 -dichloroethene
                            CCI2 = CH2
                               NLFG
References
  1. Ellington,  J.  J., F. E. Stancil, and W.  D. Payne.
    1986. Measurement of hydrolysis rate constants for
    evaluation of  hazardous waste  land   disposal.
    Volume I.  U.S. Environmental Protection Agency,
    Athens, GA. EPA/600/3-86/043.
  2. Ellington,  J. J., F. E.  Stancil, W. D. Payne, and  C.
    D. Trusty. 1988.  Measurement of hydrolysis rate
    constants for evaluation of hazardous waste  land
    disposal.  Volume  III.  Data on  70  chemicals.  U.S.
    Environmental Protection  Agency,  Athens,  GA.
    EPA/600/3-88/028.
  3. Jeffers, P. M., L.  Ward, L. Woytowitch.  and N.  L.
    Wolfe. 1989. Homogeneous  hydrolysis  rate
    constants  for selected  chlorinated  methanes,
    ethanes,  ethenes and  propanes. Environ.  Sci.
    Technol.  23(8):965-969.
  4. Ellington,  J. J., F. E.  Stancil, W. D. Payne, and  C.
    D. Trusty. 1987.  Measurement of hydrolysis rate
    constants for evaluation of hazardous waste  land
    disposal.  Volume  II.  Data on  54  chemicals.  U.S.
    Environmental Protection  Agency,  Athens,  GA.
    EPA/600/3-87/019.

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5. Fells, I. and E. A. Moelwyn-Hughes. 1959. The kinetics
   of  the  hydrolysis of the  chlorinated methanes. J.
   Chem. Soc., Part 1. No. 72:398-409.
6. Hill, J., H. P. Kollig,  D. F. Paris,  N.  L Wolfe, R. G.
   Zepp. 1976.  Dynamic  behavior of vinyl  chloride in
   aquatic ecosystems.  U.S. Environmental  Protection
   Agency, Athens, GA. EPA/600/3-76/001.
7. Wolfe, N. L, R. G. Zepp, D. F. Paris, G. L. Baughman,
   R.  C. Hollis. 1977. Methoxychlor and DDT degradation
   in water;  Rates and products. Environ. Sci. Technol.,
   11:1077-1081.
8. Fells, I. and E. A. Moelwyn-Hughes. 1958. The kinetics
   of  the hydrolysis of  methylene dichloride.  J. Chem.
   Soc., Part 2, No. 268:1326-1333.
 9. Chapman, R. A. and C. M. Cole.  1982. Observations
    on  the  influence  of water  and soil  pH  on  the
    persistence  of insecticides. J.  Environ. Sci.  Health
    B17(5):487-504.
10. Osterman-Golkar, S.  1984. Reaction kinetics in water
    of chloroethylene  oxide, chloroacetaldehyde,  and
    chloroacetone. Hereditas, 101:65-68.
11. Payne, W. D. and T. W. Collette. 1989. Identification of
    bis(2-chloroethyl)ether hydrolysis  products by direct
    aqueous injection GC/FT-IR. HRC 12:693-696.

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United States
Environmental Protection
Agency
Center for Environmental Research
Information
Cincinnati OH 45268
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EPA/600/M-89/009

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