United States
                      Environmental Protection
                      Agency
 Atmospheric Research and Exposure
 Assessment Laboratory
 Research Triangle Park NC 27711
                      Research and Development
 EPA/600/S3-91/005 May 1991
1&EPA       Project Summary
                      Snow/Rain Collector  Sampler
                      Richard G. Purcell and Rick B. Brown
                        This report describes a new instru-
                      ment for collecting chemically accurate
                      precipitation (liquid and frozen) samples
                      and measuring precipitation rate and
                      quantity. The design goals include the
                      ability to operate  in a wide range of
                      weather  conditions at remote and un-
                      attended monitoring sites for at least
                      seven days, be easily operated by non-
                      technical personnel, provide for con-
                      venient sample and data transport, ex-
                      clude dryfall, and operate from  a lim-
                      ited power source. The design features
                      and fabrication of each subassambly
                      are discussed. The results of field tests
                      are provided, with particular emphasis
                      on chemical  measurements. Finally,
                      recommendations for future improve-
                      ments based on these test results are
                      provided.
                        This Project Summary was developed
                      by EPA's Atmospheric Research and
                      Exposure Assessment Laboratory, Re-
                      search Triangle Park, NC, to announce
                      key findings of the research project
                      that is fully documented In a separate
                      report of the same  title  (see Project
                      Report ordering information at back).

                      Introduction
                       The study of precipitation chemistry im-
                      plies the ability to collect chemically accu-
                      rate precipitation samples.  In general,
                      precipitation chemistry varies from  loca-
                      tion to location so geographically disbursed
                      collection is necessary. Geographical dis-
                      persion implies a collection device that
                      will operate continuously and unattended.
                      Such a device must be able to determine
                      when precipitation is occurring and, during
 non-precipitating  periods,  prevent con-
 tamination of collecting  surfaces. Addi-
 tionally, both liquid and frozen precipita-
 tion will be of interest so the instrument
 must have the ability to sense, collect and
 melt frozen  precipitation for convenient
 storage.

 Instrument Description

 Overview
  The precipitation gauge and collector is
 a computer controlled electro-mechanical
 device  for collecting chemically accurate
 precipitation samples and measuring pre-
 cipitation quantity and rate. It is designed
 to operate unattended for periods of up to
 one week from a 12 volt DC power source.
 The device includes a start of event sensor
 that detects the onset of precipitation, a
 collector funnel that/is automatically un-
 covered during precipitation, a liquid mea-
 surement apparatus referred to as  the
 accumulator, removable bottles for storage
 and transfer of precipitation samples, a
 mechanism for transferring liquid from the
 accumulator to the storage bottles,  and a
 controller to supervise the actions  of the
 instrument and collect data. The end of a
 precipitation event is determined when the
 accumulator has not become full within a
 predetermined time period. The controller
 records the time of start and end of pre-
 cipitation events and the time of  every
filling of the accumulator, ft also records
 status events such as door open, heater
 use, sample bottle number, and instrument
 exception information such as low power
voltage  and failure of the instrument to
behave, as expected. The majority of the
                                                                         Printed on Recycled Paper

-------
instrument workings are contained within
an insulated 28 x 13 x 13 enclosure. Pro-
vision has been made to heat the start of
event sensor, collector, and interior of the
enclosure irr-order to collect frozen pre-
cipitation.

Sub Assemblies

Accumulator
  The accumulator is a removable subas-
sembly that is designed to detect  a .01
inch increment of precipitation and to
transfer that increment into storage bottles.
It consists of a collection tube of a known
volume,  a lower  normally  closed  pinch
valve that  traps liquid in the collection
tube, an  upper normally open pinch valve
that allows precipitation to enter the col-
lection tube and optical sensors that detect _
the presence of liquid. The controller op-
erates the accumulator by monitoring the
liquid detectors during a precipitation event.
When it observes that both detectors see
liquid at  the top of the collection tube it
forces a sample  needle  and vacuum
needle through a storage bottle septum
by means of the injector assembly, opens
the lower pinch valve and turns on the
vacuum  pump to suck the increment of
precipitation into the storage bottle.  The
controller determines that a precipitation
event has ended when no liquid has col-
lected in the accumulator for a program-
mable interval of time.

Carrousel Assembly
  The carrousel is a removable subas-
sembly provided to hold the storage bottles
and to position them under the injector.
The carrousel is  designed to allow the
storage bottles to be installed and removed
as  a unit. The rack of bottles  may be
transferred without need to keep track of
the  bottles  on an individual basis.  The
carrousel assembly consists of a turntable
that accepts a rack of eight 500 ml bottles,
a  motor to drive  the -turntable,  a  motor
heater and a connector. Locator pins and
a  locator pin detector switch enable the
controller to determine the position of the
turntable.

Collector
  The collector consists of an eight inch
diameter aluminum  funnel coated  with
Halar to prevent sample  contamination.
To preserve cleanliness the collector is
covered between precipitation periods. The
bottom of the funnel  is connected  to the
accumulator. The controller servos the
heaters at 3°C during precipitation events
when ambient  temperatures are below
freezing.

Cover Assembly
  The cover assembly is provided to pre-
vent contamination from entering the col-
lector during non-precipitating periods. The
start of event sensor is mounted on  the
top of the cover. A mercury bead tilt sen-
sor is mounted  to a cover mounting arm.
The controller uses that sensor to deter-
mine that the cover has moved when an
open or close command  is given and to
detect when the cover  is approaching its
destination in order to  turn off the  cover
motor. The cover is entirely coated with
Halar for cleanliness.

Injector
  The injector is a remoyable_subassern-
bly that is designed to transfer liquid from
the accumulator to the  storage bottles. It
consists of a solenoid that forces a dual
needle assembly through a septum  in the
cap of the storage  bottles, a heater to
prevent liquid from freezing in the needles
and switch that enables the controller to
detect when  the needles  are retracted.
The septa are cut from  a special high tear
strength  silicons  elastomer to withstand
up to 64 penetrations. One of the needles
is plumbed to  a  vacuum  pump  and the
other to the bottom of the accumulator.
The controller transfers liquid from the ac-
cumulator to the storage bottles by plung-
ing the needles through the septum and
applying suction to the bottle by turning
on the vacuum  pump for a predetermined
time period. As a safety feature the con-
troller will not  automatically operate the
needles when the enclosure door is open.

Start-of-Event Sensor
   The start of event sensor (SOES) func-
tions by detecting the lowered resistance
of a printed circuit board grid pattern when
the  grid becomes wet. AC excitation of
the  grid  prevents long term degradation
due to electrolysis. A heater and control
electronics within the SOES housing keep
the temperature of the  grid above 3°C in
order to detect frozen precipitation. A short
chimney reduces the chance that frozen
precipitation will bounce out of the  SOES
before it melts.  The capability to force the
SOES heater on is provided so that the
grid may  be dried at the end of a precipi-
tation event.

Materials
   Chemistry and material compatibility
questions made material selection one of
 the  most  important  aspects  of the
 sampler's design. Fortunately, the choices
 were considerably simplified by selecting
 from a list  of materials  already deemed
 acceptable for handling NADP samples.
    All wetted surfaces were fabricated from
 materials included on this NADP  list with
 one  exception.  The collector funnel and
 cover were coated with  Halar  ECTFE, a
 copolymer of ethylene and chlorotrifluoro-
 ethylene. It gives an  inert, stable surface
 that  should avoid the potential problems
 of pinholes and porosity sometimes seen
 with  Teflon  coatings. Both  silicone and
 pvc tubing were tested in the accumula-
 tor. The  former was selected  based on
 less  variation in its inside  diameter and
 less  tendency to take a set in the pinch
 valves.
--•- The materials were assessed ,in two
 ways:  1) laboratory  testing of samples,
 and  2) chemical performance tests of the
 completed instrument.

 Results and Discussion
   The field tests were conducted in two
 modes. In the first procedure, 500 ml of a
 fairly clean water standard  was prepared
 and stored in a polyethylene sample bottle.
 At the start of the sampling week 200  ml
 was  poured  into  the collector and pro-
 cessed by the instrument into sample bottle
 #8. At the end of the  week, the procedure
 was  repeated and the liquid was passed
 into  sample bottle #7. The standard and
 two blanks, along with whatever precipita-
 tion that was collected in the other sample
 bottles, were sent to the  laboratory for
 analysis. We were looking for differences
 in species  concentrations  between the
 standard and the blanks. The   second
 procedure involved using a not so clean
 water standard, in this case tap water. We
 were looking for the loss of species.

 Conclusions
    The instrument described herein per-
 formed satisfactorily during  field testing. It
 demonstrated the ability to  operate in a
 cold winter mountain environment while
 powered by four automobile batteries. The
 removable carrousel of sample bottles
 proved to be easy to replace and transport.
 It is doubtful that the instrument can  be
 reproduced  in  quantity  for  $2,500. That
 figure will probably cover the  cost of  in-
 strument components and  assembly, but
 not test,  product support, and profit.
                                                                              U.S. GOVERNMENT PRINTING OFFICE: 1991/548-028/20216

-------

-------
  Richard G. Purcellis with the Atmospheric Sciences Center, Desert Research Institute,
    Reno, NV 89506. Rick B. Brown is with the Energy and Environmental Engineering
    Center, Desert Research Institute, Reno, NV 89506.
  Steven M. Bromberg is the EPA Project Officer (see below).
  TTje complete report, entitled "Snow/Rain Collector Sampler," (Order No. PB91 -
    167601/AS; Cost: $15.00, subject to change) will be available only from:
         National Technical Information Service  ,
         5285 Port Royal Road
         Springfield, VA 22161
         Telephone: 703-487-4650
  The EPA Project Officer can be contacted at:
         Atmospheric Research and Exposure Assessment Laboratory
         U.S. Environmental Protection Agency
         Research Triangle Park, NC 27711
 United States
 Environmental Protection
 Agency
Center for Environmental
Research Information
Cincinnati, OH 45268
      BULK RATE
POSTAGE & FEES PAID
         EPA
   PERMIT No. G-35
Official Business
Penalty for Private Use $300
EPA/600/S3-91/005

-------