United States
Environmental Protection
Agency
Risk Reduction
Engineering Laboratory
Cincinnati, OH 45268
Research and Development
EPA/600/SR-93/102    July 1993
Project  Summary
Thermal  Degradation
Characteristics  of
Environmentally Sensitive
Pesticide  Products
Debra A. Tirey, Barry Dellinger, Wayne A. Rubey, and Philip H. Taylor
  The thermal decomposition proper-
ties of the active ingredient of 16 pesti-
cides have been theoretically examined.
The parameter used to rank their sta-
bility was the temperature required for
99% destruction at a gas phase resi-
dence time  of 2.0 sec  under oxygen-
starved conditions (T99(2)). Experimen-
tal  studies  on five pesticide-related
materials were also conducted  under
controlled laboratory testing.
  Experimental studies of the high-tem-
perature oxidation and pyrolysis of four
key pesticide  materials including the
identification and quantification of prod-
ucts of incomplete combustion  (PICs)
were conducted.  The  four pesticides
were Aldicarb* and  Phorate (both in-
secticides) and Atrazine and Alachlor
(both  herbicides). These compounds
are the  active  ingredients of Thimet,
Temik, Aatrex-Nine-O, and Lasso II, re-
spectively. A fifth material, a polyethyl-
ene blend bag which  is  used  as an
Atrazine container, was also examined.
  The examination of  the incineration
ranking  among the 16 subject pesti-
cides indicated that they should be con-
sidered thermally fragile. However, each
pesticide in the controlled laboratory
testing decomposed to yield a  large
number of reaction intermediates. More
intermediates  were  consistently pro-
duced under pyrolytic  conditions. Al-
though most of the intermediates were
decomposed by 700°C,  some persisted
at the  maximum  testing temperature,
1000°C. It appears that these materials
tested  may be amenable to properly
* Mention of trade names or commercial products does
 not constitute endorsement or recommendation for
 use.
controlled, high-temperature incinera-
tion.
  We also concluded that open burn-
ing of spent pesticide bags may not
significantly reduce their effect on the
environment and that the analytical pro-
tocols associated with the monitoring
of decomposition  products from pesti-
cide materials should be further devel-
oped.
   This Project Summary was developed
by EPA's Risk Reduction Engineering
Laboratory, Cincinnati, OH, to announce
key findings of the SITE program dem-
onstration that is fully documented in a
separate report (see ordering informa-
tion at back).

Introduction
   Pesticides, insecticides, herbicides, and
fungicides are  applied  worldwide to con-
trol rodents, insects, weeds,  and fungi
thought to  be  a direct threat to  human
health or to livestock and crops raised for
human consumption. A renewed concern
over the effect of  applying these  chemi-
cals at  an  ever expanding rate, both to
the environment and to people, has, how-
ever, recently been raised.
   Many  studies conducted  to address
these concerns have evaluated the per-
sistence and toxicology of pesticide mate-
rials in  plant and  animal tissues  and  in
soils. These studies indicate that most
pesticides  themselves are fragile com-
pounds that are readily transformed in the
environment to other metabolites that may
or may  not be  more toxic or more persis-
tent than the parent material.
   What happens,  however, when pesti-
cides are thermally decomposed, as  in
the case of open  burning of spent bag
                                                  Printed on Recycled Paper

-------
materials  containing trace quantities of
pesticides—a common practice for many
farmers? Or, what occurs when a pesti-
cide has been  determined through  "per-
sistence and toxicological" studies to no
longer be suitable for widespread use and
is suddenly banned? The method of choice
to  dispose of these materials is, in many
instances,  incineration. How  will these
materials react  upon thermal decomposi-
tion? A review of the open literature sug-
gests that only limited information is avail-
able.
   In this study, the thermal decomposition
properties of the active ingredient of 16
pesticides have  been theoretically exam-
ined, and experimental studies on 5 pesti-
cide-related materials were conducted. The
theoretical  stability evaluations were pre-
pared with the use of available laboratory
data or with data on structurally similar
compounds in conjunction  with chemical
reaction kinetic  theory (Table 1). The pa-
rameter used to rank their stability  was
the temperature  required for 99% destruc-
tion at a gas phase residence time of 2.0
sec  under  oxygen-starved  conditions,
T99(2). Table 1 also indicates the  thermal
stability  ranking  and the thermal  stability
class  ranking of each of the pesticides
within the hierarchy of the 330 individual
compounds and 7 classes currently clas-
sified  ( a ranking of 1  being most stable).
Data  sheets on each pesticide are  pre-
sented in the full report.
Table 1. Pesticide Thermal Stability Data
Experimental Procedures
  An  experimental study of the thermal
degradation characteristics  of  Aldicarb,
Phorate, Atrazine,  and Alachlor was un-
dertaken. This included a successful atom
balance for carbon, nitrogen, sulfur, phos-
phorus, and chlorine.

Instrumentation
  All experiments were performed on the
Thermal Decomposition Analytical System
(TDAS). The TDAS  is a closed,  in-line,
quartz flow reactor system capable of ac-
cepting a  solid,  liquid, or gas  phase
sample, of exposing the volatilized sample
to a highly controlled thermal environment,
and then of analyzing the effluents result-
ing from this exposure.
  Gas-phase samples are swept with car-
rier gas of helium through heated transfer
lines into a quartz flow reactor where con-
trolled high-temperature exposure occurs.
Mean  residence times of 0.5 to 6.0 sec
may be achieved. Thermal decomposition
data may be taken over the temperature
range 200° to  1050°C.
  The effluent resulting from thermal ex-
posure is swept by carrier gas to a Hewlett
Packard 5890 gas  chromatograph  (GC)
where it is cryogenically focused  on the
head  of a capillary column located inside
the GC oven. Later, the oven temperature
is raised at a specified rate and the sepa-
rated  compounds eluting from the column
can then be sent to either the ion source
of an  HP 5970B mass selective detector
Pesticide
Compound
DCPA
Alachlor*
Acephate
Pronamide
Carbonfuran
Triallate
Fonofos
Ethoprop
Chlorprifos
Atrazine*
Terbufos
Cyanazine
Azinphos methyl
Phorate*
Methomyl
Aldicarbr
Oxygen-Starved
Condition,
Tu(2)rC)
750
620
595
570
560
550
530
530
510
510
510
500
460
400
200
200
Stability
Ranking
105-114
185-189
207
220
226-228
231-234
237-241
237-241
249-251
249-251
249-251
253-258
266-269
276-277
318-320
318-320
                                                                   Stability
                                                                 Class Division'
' Ranking of 1 indicates most stable.
f Derived from experimental data obtained from this study.
(MSD),  or to a flame ionization  detector
(FID) located within the GC assembly.
  Data  acquisition and analysis  for the
TDAS was done with the  aid of an HP
59970 ChemStation and the accompany-
ing system software that includes an on-
line National Institute of Health/U.S.  Envi-
ronmental Protection Agency (NIH-EPA)
mass spectral library. It was also neces-
sary to develop an interface between the
GC and the MSD. This interface, the in-
sertion-split, was designed  as a  compro-
mise between the typically used "direct-to-
source interface" and the "open-split  inter-
face" and incorporated the meritorious as-
pects of each. The direct-to-source  inter-
face promotes  heightened  sensitivity for
the mass spectrometer because effluents
from the column are deposited  directly
into the source. However, having the GC
column outlet placed directly in the source
of the mass  spectrometer  (typically held
at 10-6 or 10-7 torr) creates a huge  pres-
sure drop across the column that literally
pulls volatile  compounds through the lat-
ter portion of the column without allowing
for  any  separation that  may be  attained
by  interaction with the liquid stationary
phase. For these experiments, it was  para-
mount that such compounds as CO2, CH4,
and the light C2 gases be separated,  since
these were predicted to be  major PICs.
  The open-split interface provides for the
use  of  much larger column bores and
larger sample sizes but protects the source
of the mass spectrometer from undue wear
since much  of  the column  effluent  is di-
verted before it enters the source. One of
the chief drawbacks  of this type of  inter-
face is the loss of sensitivity relative to the
direct-to-source interface. Since one of the
goals of this study was to perform a  mass
balance of the data, isolating and analyz-
ing as many of the products as  possible
was imperative. The insertion-split  inter-
face provided the  best  answer to these
two dilemmas.
  Essentially the insertion-split interface
is a small-bore transfer tube placed within
a capillary column; the tube is surrounded
by  carrier gas that  is  constantly being
swept away. A drawing of this interface as
it is installed  in the TDAS is presented in
Figure 1. A  piece of narrow-bore, fused,
silica tubing  (uncoated but deactivated) is
positioned in the source of the mass spec-
trometer in much the same way that the
capillary column would be positioned if it
were direct-to-source, with  a fixed length
left on the oven side of the connection nut
(can be a variable length,  10 to 20 cm).
The end of  this tubing  remaining in the
oven is  then  placed inside  the outlet end
of the GC capillary  column. Obviously,

-------
    Direct
    to MS
i;
kXXXXXXXXXXXX X X^
I
£5^55555^5555^555555111^
•< 	 0.10mm
s
He IN
XXXXXXXXXXT
t
0.32 mm < 	
Capillary
Column

IX X X X ,
1

^ He OUT

/
/
                                        Press-fit
                                        Connector
                                          CXI—Drt
                            60 m DB-5
                             from
                             Reactor
                             to
                             Splitter
Figure 1.  Close-up schematic of the insertion-split interface as it is configured in the TDAS.
attention must be  paid to the inner  and
outer dimensions of the  two tubes.  The
film thickness of the capillary column  is
also important relative to gas chromato-
graph-mass spectrometer (GC-MS) opera-
tion. The ends of the transfer tubing  and
the capillary  column  that  overlap  are
housed within a stainless-steel piece  of
tubing fitted with inlet and outlet gas flows;
this allows a gaseous carrier to be purg-
ing the area surrounding the junction at all
times. Finally, the entire stainless-steel
miniaturized housing is firmly mounted in-
side the GC oven so as to remain station-
ary even while the GC oven fan is  run-
ning.
   Because there is  a  finite annular  gap
between the outer wall of the transfer tub-
ing and  the inner wall  of  the capillary
column and because this junction is  kept
pressurized by the addition of flowing he-
lium carrier surrounding the two overlap-
ping tubes, the outlet to the capillary col-
umn now experiences approximately at-
mospheric pressure. Thus, lightweight
materials are not "pulled" through the col-
umn without being separated as with the
direct-to-source interface. Also,  because
the transfer tubing is placed inside the
capillary column, transfer of sample from
column to mass spectrometer (MS) is al-
most continuous; there is no axial or open
gap in the flowpath of the column effluent
as  would be  experienced  by the  open-
split interface. This fact  helps to maintain
relatively good sensitivity for this interface
despite the fact that there  is some split-
ting of the sample at the column overlap
junction.
  Before invoking  the insertion-split inter-
face for this program, considerable devel-
opmental  work went into testing the lin-
earity of splitting for lightweight as well as
for  heavy materials (i.e., whether heavy
materials would be preferentially split rela-
tive to lightweight compounds because of
the axial position they would tend to oc-
cupy while traveling through the capillary
column). The insertion-split  interface de-
sign used a bluff-body mixing principle at
the annular split location as a contingency
for this concern. Test results indicated that,
indeed, the bluff-body design performed
as expected; splitting of test samples con-
taining a  wide-molecular range of com-
pounds was consistently the same for light,
intermediate, and heavy compounds. (The
compounds used were octane,  octadec-
ane, and octacosane in cyclohexane). We
also found that for a given volumetric col-
umn flow, linear velocity, and head pres-
sure, the insertion-split interface response
was always a fixed fraction (approximately
40% to 50%) of that experienced with  the
direct-to-source interface.  This  number
depends on the  length and diameter of
the transfer tubing positioned in the source
of the mass spectrometer.

Sample Introduction
   Standards of each of four  pesticides
were received from the National Reposi-
tory located at  Research Triangle Park,
NC. The  purity  of each was certified as
greater than 98%  (i.e., Aldicarb  99.8%,
Phorate  98.2%,  Atrazine  99.4%,  and
Alachlor 99.6%). Aldicarb, Atrazine, and
Alachlor were solids at room temperature,
whereas  Phorate was a viscous liquid.
The Atrazine 90 DF  bag  was  clean—no
pesticide material had been  placed in  it.
   Target test conditions for the four pesti-
cide active  ingredients were (1) 1%  mol/
mol of pesticide in carrier gas, (2) a gas
phase residence time (tr) = 2.0 sec, and
(3) two reaction atmospheres: pyrolysis at
a fuel/oxygen equivalence ratio (phi) of 10
and oxidation at phi = 0.5  (100% excess
oxygen).  The Atrazine bag  material was
run only under oxidative conditions.
   Sample delivery for the three solid pes-
ticide active ingredients (Aldicarb, Atra-
zine, and Alachlor) in this set of experi-
ments involved dissolving the solid mate-
rial in a suitable solvent and depositing an
aliquot of  the solution  into a  quartz
pyroprobe  tube. Once the  solvent  had
evaporated, the  tube was placed in  the
platinum  coil  of a  CDS  Model  120
pyroprobe assembly (Chemical Data Sys-
tem, Inc.) that was then  placed into the
insertion  region  of the TDAS. With  the
use of temperature programming  of both
the  insertion  region itself and/or  the
pyroprobe heating coil, each pesticide was
volatilized into  flowing carrier  gas  at  a

-------
specific, reproducible rate. Separate ther-
mal  gravimetric analysis (TGA)  experi-
ments were performed in flowing air and
nitrogen to aid in determining the first ap-
proximation of  these  temperature proto-
cols.
  Approximately 40 quartz tubes  were
loaded with sample from the same stock
standard solution, and solvent was allowed
to evaporate. The tubes were then  kept
covered at room temperature in a labora-
tory hood until just before their use. Load-
ing the quartz tubes in  this manner  pro-
vided the  best  reproducibility with regard
to sample size.
  Sample delivery for the only  liquid ac-
tive ingredient, Phorate, was more straight-
forward than that for the three solids. The
pure liquid (0.5 p.L) was injected into an
insertion region  held isothermally at 100°C
by using a 0.5 \iL  full-scale liquid syringe
fitted with  a 6-in. needle.
  For the polyethylene bag, approximately
2  mg of bag material was placed  in a
quartz pyroprobe tube (loaded with a  plug
of quartz wool to keep the  piece of poly-
meric material from falling out). The  tube
was then placed in the platinum coil of the
CDS pyroprobe assembly and put into the
insertion region of  the TDAS. As with the
solid pesticides, temperature programming
of both the insertion region itself and the
pyroprobe heating  coil volatilized the
sample into flowing carrier.  A separate
TGA experiment was performed in flowing
air to aid in determining the first approxi-
mation of this temperature protocol.
  The profiles  generated  using these
sample introduction techniques delivered
the maximum possible part per  million
(mol/mol) concentration of pesticide in the
carrier gas while also delivering a suitable
sample size to the analytical system down-
stream of the reactor for adequate  con-
version to products. The concentration  of
active  ingredients  ranged from 0.1%  to
0.5% mol/mol  in  the carrier, with the
sample sizes ranging from 77 to 500 jig.
Table 2 presents a summary of the pesti-
cide concentrations in carrier gas  used in
this study, the insertion region protocols
that  delivered these values, and  the ac-
companying oxygen  concentrations re-
quired for phi = 0.5.
  Degradation of each of the three pesti-
cides was conducted under both oxygen-
deficient (fuel/oxygen equivalence ratio of
10) and oxygen-rich (fuel/oxygen  equiva-
lence ratio of 0.4 to 0.5) conditions. Ap-
proximately 0.5% oxygen in helium (mol/
mol) was  available for combustion in the
oxygen-deficient conditions (as determined
by actual  measurement of  the reaction
gas), whereas a 10% mix of oxygen in a
balance of 51% helium/39% nitrogen was
used  for  the oxygen-rich  experiments
(these were the values obtained by mix-
ing compressed air and helium at a one-
to-one ratio vol/vol). Gas mixtures were
prepared  by  using a gas mixing device
developed inhouse. Residence time at tem-
peratures  for all exposures regardless of
atmosphere was held constant at 2.0 sec;
the reactor temperature varied over the
range 200° to 1000°C. Experiments were
conducted at 1.23 atm. Sample was intro-
duced by using the protocols described in
preceding paragraphs.
  The effluent resulting from a single re-
actor exposure (unreacted parent material
and all PICs) was directed to a 60 m, DB-
5, 0.32-mm i.d. column  (J&W  Scientific,
Inc.) held  at -60°C with the use of  liquid
nitrogen  as coolant. Individual  reaction
products were separated by programming
the GC oven from  -60° to 290°C at  10°C/
min with a 15-min hold  at -60°C and a 25-
min hold at 290°C. Detection was accom-
plished with the aid of an HP 5970B quad-
rupole mass spectrometer. The mass spec-
trometer was operated in full-scan  mode
with an electron energy of 70 eV and an
electron multiplier setting of 1700. To opti-
mize detection of products, during the first
20 minutes of the GC program, the  mass
range scanned was 10 to 200 amu; from
 Table 2.  Volatilization Parameters and Concentration of O2in the Carrier Used to Achieve Target Test Conditions

                                                                               Pyrolysis
                                                                Oxidation
Compound
Aldicarb/s*
Phorate/1
Atrazine/s

Alachlor/s

Atrazine DF
bags
Insertion
Region Program
Isothermal
@20CPC
Isothermal
@10CPC
Isothermal
@275°C

Isothermal
@300°C

Isothermal
@250°C
Pyroprobe
Program
No Program
Not used
Ambient to
275°C@
2CfC/ms
hold 20s
Ambient to
30CPC@
2CPC/ms
hold 20s
Ambient to
50(fC@
20PC/ms
Cone.
(mol/mol)
4000
5000
3000

4000

Not
applicable s
% 02* in
Carrier
0.5(0.5)
0.5(0.5)
0.5(0.5)

0.5(0.5)

0.5
p/j/*
10(10)
10(10)
10(10)

10(10)

Not
applicable
%02in
Carrier
10(9)
10(7)
10(10)

10(8)

10
phi
0.5(0.5)
0.5(0.5)
0.5(0.5)

0.5(0.5)

Not
applicable
 * Concenration of oxygen mol/mol in carrier required for complete combustion based upon the stoichiometric equation for the pesticide listed as: actual
 (theoretical).

 * Phi value for the oxidative experiments listed as: actual (theoretical).

 ' "s" indicates solid phase sample. "1" indicates liquid phase sample.

 s No attempt was made to calculate a "concentration" or "phi" value for the polymer.

                                                             4

-------
20 to 80 min, the mass range scanned
was 10 to 500 amu. This allowed for maxi-
mum detection of light gasses during the
first part of the GC program. Quantitation
and identification  of products was deter-
mined with the aid of an HP ChemStation
data system and an on-line NIH-NBS mass
spectral library as well as through manual
interpretation.
  Analytical standards for observed prod-
ucts were  run wherever possible to obtain
quantitative response factors. Where ob-
taining a product was  either impossible,
extremely difficult, or untimely (i.e., a 6-wk
or 2-mo waiting period), analytical  stan-
dards were run for compounds in the same
class or closely related in structure to the
compound of interest. These response fac-
tors were  then used to estimate the re-
sponse factors for the actual products seen
in thermal decomposition  experiments.
Response factors were typically obtained
from 4 or 5 point calibration  curves with
some replicate points  being  performed
where possible.
  Standards were injected into the TDAS
using the  same timetable,  valve  switch-
ing, split ratio, and GC program as  were
the pesticides. Thus, response factors gen-
erated from the  curves could be  used
directly to perform absolute quantification
of the area responses  reported in  each
data run by using the following equation:
        Ng of compound detected =
            Area counts of
       compound/response factor
The "ng detected" values were then con-
verted with the use of molecular formulas
and molecular weights to yield mass and/
or moles of carbon, nitrogen, sulfur, phos-
phorus, and chlorine. In this  way, a bal-
ance  of the atoms  at  each temperature
could be evaluated.  The compiled list of
analytical  standards  run  for this program
and  the response factors determined in
both reaction  atmospheres are given in
Appendix 2 of the full report.

Results
  The chromatograms generated in this
study were very  complex, especially at
intermediate destruction temperatures. For
example,  the  thermal  decomposition of
Alachlor under oxygen deficient conditions
yielded greater than 80 different PICs over
the temperature range of 275° to 1000°C.
A typical example chromatogram obtained
from the Alachlor experiments is presented
in Figure 2.
  Although the excess oxygen chromato-
grams were generally less complex than
were the pyrolysis ones,  a relatively large
number of products  were  nevertheless
detected in these experiments as well.
The  number of byproducts observed for
each of the pesticides is summarized in
Table 3.
  The  metabolite studies found in the lit-
erature reported that these four pesticides
were  not  persistent in  the  environment
and that they were readily transformed to
other compounds. Their thermal stability
as determined under the conditions of this
study was analogous to this  behavior. All
four  compounds themselves were labile,
disappearing  by  600°C under  both pyro-
lytic and oxidative conditions. The relative
stabilities can  be conveniently  ranked by
the temperature required for 99% destruc-
tion for a 2.0  sec residence time (T99(2))
(see Table 4). The  relative stabilities un-
der both sets  of conditions  in  this study
were:  Alachlor > Atrazine >  Phorate >
Aldicarb. Aldicarb and Phorate exhibited
degradation at the lowest reactor tempera-
ture  possible  on  the  TDAS, 200°C.  Be-
cause  no Aldicarb  was detected in the
quantitative transport  run  at 200°C,  this
temperature was assigned  as its T99(2)
value.  In the case of  Phorate, the T (2)
value is the temperature at which  no Phor-
ate was detected in  replicate runs. A more
in-depth explanation of the problems as-
sociated  with  running Phorate  are  dis-
cussed in the full report.
  Interestingly, none of the pesticides dis-
played a large dependence upon reaction
atmosphere  From  this  observation,  one
can  infer that  the decomposition mecha-
nisms  may be dominated by unimolecular
pathways. A more pictorial representation
of this can be  seen  in  the thermal decom-
position composite  curves generated for
the pesticides Alachlor and Atrazine in
Figure 3.
  The specific products detected in the
decomposition studies of  Aldicarb,  Atra-
zine, and Alachlor in the form of weight %
yield  (relative  to  parent) for each atmo-
sphere can be found in  Tables 5 through
10 of the full report. Many of the  products
detected in these  experiments  may be
environmentally significant.
  Because of the viscosity of Phorate, the
small volume  available for sampling (i.e.,
only 50 (iL in  a  1.5-mL vial volume) and
the short "shelf-life" of Phorate once ex-
posed to the  atmosphere, the reproduc-
ibility of injection was  not good. Replicate
and  triplicate  injections at each reaction
condition resulted in relative standard de-
viations of as much as ± 36%. For this
reason, only  qualitative  analysis of the
Phorate decomposition products are listed
in Tables 11  and 12 of the final report.
There, all areas of  peaks not  identifiable
by their mass  spectra are summed under
the heading "Unidentified."
  In the full report, the results obtained
from the Atrazine bag oxidation  experi-
ments  are similarly  presented (i.e.,  as
qualitative analysis of the decomposition
products). The act of volatilizing the poly-
mer in  the  insertion  region  necessarily
makes "weight % yield (relative to parent)"
type data meaningless. As with Phorate,
areas of peaks we were unable to identify
are summed under the heading "Unidenti-
fied." The products seen  from this series
of experiments were the  same ones ob-
served  in previous studies conducted in
this laboratory in  which polyethylene and
polyethylene/polypropylene blends were
thermally decomposed.
  Mass balance for the pesticide experi-
ments  was  achieved  with  a fairly good
degree  of success. Although some tem-
perature data points were clearly outliers,
most data points were within ± 30% of the
100% recovery mark. A listing of the atom
balances for C, N, S,  or Cl where appro-
priate are presented in Appendix 3 of the
full report. Because of the high degree of
uncertainty associated with the Phorate
data, no atom  balances were  attempted.

Conclusions
  The experimental results of this study
are very complex. Some simple  conclu-
sions are, however, readily apparent.
  1. Based on the stability of the  parent
     pesticides  and   their  thermal
     byproducts, these materials may  be
     amenable to properly controlled, high-
     temperature incineration. The number
     yields and stability of the  byproducts
     suggest, however, that open burning
     of  spent  bag materials  containing
     pesticide  residues  may not sig-
     nificantly reduce  their effect on the
     environment.
  2. When  compared with a previously
     generated ranking of hazardous waste
     incinerability, the 16 subject pesticides
     (with the possible exception of DC PA)
     should be considered thermally fragile
     (i.e., T(2)<600°C).
  S.With trie  exception  of Alachlor,
     reaction atmosphere had almost  no
     effect  on  pesticide stability. This
     suggests that the primary mechanisms
     of  decomposition are unimolecular
     (e.g., simple bond  rupture  or more
     complex  concerted  intramolecular
     reactions).
  4. Each pesticide decomposes to yield
     a   large   number   of  reaction
     intermediates. More  intermediates
     were consistently produced  under
     pyrolytic   conditions.  Most  inter-
     mediates  were decomposed  by
     700°C;  however, some persisted at

-------
6. OE5 _
5. OE5 —
4. OE5 -
| 3. OE5 J
2.0E5 _
1.0E5 ~
0





[
\uL
TICofData:ALAPY10.D
Data File: Data:ALAPY10.D
~u File Type: GC / MS Data File
Ltri^f
CsHp Name Info: 650C Alachlor 2S Tube 15 PestScc.A
~ ., Misc Into:
^2"4 Operator: JEB 1/22/9 1
CO?
Date: 22 Jan 91 4:20 pm
Instrument: MS 5970
Inlet: GC
Sequence Index: 0
Als Bottle Run: 0
Replicate Run: 1


Hd/H*
HCN yvt I
L™^ 	 /^^v^ U^_ 	 ^u^JsUUN

Aromatic
Hydrocarbons
and Heterocycles
I

ikliLU~~^
\ — \ — \ 	 \ — \ — j- 	 r1 • i i i | i i i i i i i i i | i i i | i i • i i
0 10 20 30 40 50 60
Time (min)
Figure 2.  Example chromatogram generated for Alachlor pyrolysis, phi= 10, 4000 ppm, 2 sec residence time, 1.23 atm.
    the maximum  temperature in this
    study,  1000°C.  The  most  stable
    organic intermediates were primarily
    nitrogen-containing compounds (i.e.,
    nitriles and cyanides).
  5. Relatively good mass balances were
    obtained for three of the pesticides;

Table 3. Number of Decomposition Byproducts
        Observed
Pesticide
phi = 10   phi = 0.4 to 0.5
Aldicarb
Phorate
Atrazine
Alachlor
39 (23)'
31 (19)
63 (50)
86 (59)
22 (17)
25 (17)
47 (36)
29 (23)
  ( )  indicates the number identified by the
  mass spectra, remainder listed as unidenti-
  fied.
    this suggests a reasonably complete
    set of product identifications.
  6. Polyethylene  bag  oxidation  inter-
    mediates did  not appear to be  as
    environmentally significant as  the
    pesticide intermediates.

Recommendations
  Because of the numerous byproducts
and complex chemistry  observed as the
results of the thermal degradation of pes-
ticides, we make  the followings recom-
mendations:
  1. Additional laboratory testing of other
    pesticide products  suspected  to  be
    environmentally sensitive  should  be
    performed. Results  of these studies
    can   be  used to evaluate  the
    environmental effect  of pesticide
                                                                           burning  and  to  guide larger scale
                                                                           evaluation programs.
                                                                         2. The analytical protocols  associated
                                                                           with the monitoring of decomposition
                                                                           products from  pesticide  materials
                                                                           should be further developed. Many of
                                                                           the byproducts  observed  in  our
Table 4. Pesticide Stability
TK(2) CC)
Pesticide
Aldicarb
Phorate
Atrazine
Alachlor
phi = 10
<400
510
620
phi = 0.4 to 0.5
200°C
<275
475
525

-------
            102
            101
            100
           10-1
           10-2
Alachlor Oxidation


Alachlor Pyrolysis


Atrazine Oxidation


Atrazine Pyrolysis
               200
  300
400                500

     Temperature (°C)
600
700
Figure 3.  Weight % remaining curves for parent materials, Alachlor and A trazine, generated under oxidative (phi = 0.5) and pyrolytic (phi= 10.0) conditions,
         2.0 sec residence time, 4000 and 3000 ppm respectively, and 1.23 aim.
    laboratory evaluations  are polar and
    may   be   water   soluble   thus
    complicating their analysis. Standard-
    ized analytical techniques  are  not
    available for many compounds that
    may be environmentally significant.
  3. Thermal decomposition chemistry and
    kinetics of pesticides should be  the
    subject of further research so that the
    open  burning  and   incineration
    behavior of pesticides  may be better
                understood.  Organic nitrogen and
                sulfur combustion  chemistry are
                largely unexplored  fields of apparent
                environmental significance.
              4. Close coordination between laboratory
                researchers and field test researchers
                should be attempted to ensure that
                the products identified in the laboratory
                are targeted for measurement in the
                field.
                                     5.lexicological  evaluation  of  the
                                       observed byproducts should be done
                                       to aid  in  determining the environ-
                                       mental risk associated  with  open
                                       burning and incineration of pesticides.
                                     The full  report was  submitted in fulfill-
                                   ment  of  Cooperative Agreement  CR-
                                   813938-01-0 by the University of Dayton
                                   Research Institute under the sponsorship
                                   of  the U.S.  Environmental  Protection
                                   Agency.
                                                                        •ffV.S. GOVERNMENT HUNTING OFFICE: IM3 - 7SO-07I/MM35

-------
D. A. Tirey, B. Dellinger, W. A. Rubey, and P. H. Taylor are with the University
  of Dayton Research Institute, Dayton, OH 45469-0132.
D.A. Oberackerand P.C.L Lin  are the EPA Project Officers (see below).
The complete report, entitled "The Thermal Degradation Characteristics of
    Environmentally Sensitive Pesticide Products," (Order No. PB93-201127;
    Cost: $19.50, subject to change) will be available only from:
      National Technical Information Service
      5285 Port Royal Road
      Springfield, VA22161
      Telephone: 703-487-4650
The EPA Project Officer can be contacted at:
      Risk Reduction Engineering Laboratory
      U.S. Environmental Protection Agency
      Cincinnati, Ohio 45268
  United States
  Environmental Protection Agency
  Center for Environmental Research Information
  Cincinnati, OH 45268

  Official Business
  Penalty for Private Use
  $300

  EPA/600/SR-93/102
     BULK RATE
POSTAGE & FEES PAID
         EPA
   PERMIT No. G-35

-------