United States Environmental Protection Agency Air and Energy Engineering Research Laboratory Research Triangle Park, NC 27711 Research and Development EPA/600/SR-94/198 January 1995 &EPA Project Summary The RAETRAD Model of Radon Gas Generation, Transport, and Indoor Entry Kirk K. Nielson, Vern C. Rogers, Vern Rogers, and Rodger B. Holt The report describes the theoretical basis, implementation, and validation of the RAdon Emanation and TRAnsport into Dwellings (RAETRAD) model, a conceptual and mathematical approach for simulating radon (Z22Rn) gas gen- eration and transport from soils and building foundations to the indoor en- vironment. It has been implemented in a computer code of the same name to provide a relatively simple, inexpensive means of estimating indoor radon en- try rates and concentrations. RAETRAD uses the complete, multiphase differ- ential equations to calculate radon generation, decay, and transport by both diffusion and advection (with pressure-driven air flow). The equa- tions are implemented in a steady-state, 2-dimensional finite-difference mode with elliptical-cylindrical geometry for maximum efficiency and modeling de- tail. For validation, the air flow part of RAETRAD was compared with a 2-di- mensional analytical calculation of air flow through a uniform field. Variations of less than 1% were observed between the analytical and numerical pressure fields. The radon generation, decay, and transport part of RAETRAD was vali- dated by similar comparisons with 1-di- mensional analytical calculations for open and concrete-covered soils. Most radon concentration profiles and sur- face radon fluxes for these compari- sons were also within 1%. RAETRAD calculations were also compared with empirical data from two 6 x 6 m research structures with floating-slab and slab-in-stem-wall con- struction. The comparisons included soil radon concentration profiles and indoor radon concentrations under dif- ferent air pressure and ventilation con- ditions. The RAETRAD values were consistently within less than 1 stan- dard deviation of the measured data. Indoor radon concentrations averaged within 11% of calculated values and had an average bias of only 3%. Com- parisons with measurements from other houses showed greater variations due to assumptions about house floor slab integrity and diffuslvity. This Project Summary was developed by EPA's Air and Energy Engineering Research Laboratory, Research Triangle Park, NC, to announce key findings of the research project that Is fully docu- mented in a separate report of the same title (see Project Report ordering infor- mation at back). Introduction Elevated indoor radon concentrations usually result from elevated radon gen- eration and mobility in soils combined with openings or pores in the building founda- tion. Although indoor radon levels are dif- ficult to predict, long-term average levels can be estimated by mathematical mod- els, which simulate the complex processes of radon generation, transport, and indoor entry using soil and house parameters. The RAETRAD model was developed to provide a new level of simplicity in detailed radon modeling. From user-specified house and soil proper- ties, RAETRAD computes detailed Printed on Recycled Paper ------- air-pressure and radon-concentration profiles in the floor slab, foundation, and surrounding soils, and the result- ing radon entry rate and indoor radon level. RAETRAD is designed to address ques- tions such as how strong and how close to the house can a radon source be for par- ticular soil and ground water conditions with- out excessively elevating indoor radon levels? This information is important for planning and regulating soil excavation, for replacement at radium-contaminated sites, and also in regulating building construction in areas with high-radium strata or with fill soils of higher or lower radium concentra- • tfon. The RAETRAD model represents slab-on-grade houses of different sizes and shapes on soils with any distribution of radon source strengths, physical proper- ties, water contents, and gas transport prop- erties. K was developed in part under the Florida Radon Research Program (FRRP), which has been cosponsored by the Florida Department of Community Affairs and the U.S. Environmental Protection Agency. It has been used in the FRRP to characterize the effects of foundation soil and fill proper- ties on indoor radon entry, to characterize the modes of radon entry, to characterize soil radon potentials for mapping of their geographic distributions, to develop simpli- fied lumped-parameter models, and to sup- port development of radon-protective building construction standards. Theoretical .Basis RAETRAD computes radon production from radium decay in floor slabs, founda- tion structures, and surrounding soils. It also computes the detailed radon interac- tions in the solid, liquid, and gas phases of the soils and concretes, and radon gas transport and indoor entry by both diffu- sion (concentration-driven) and advection (with pressure-driven air flow). The theo- retical equations used for defining radon generation and transport in the foundation and soil regions consider the effects of moisture and the simultaneous effects of diffusive and advective radon movement. Steady-state radon entry rates and in- door radon concentrations are computed in a two-step process that involves first solving the air-pressure and airflow distri- butions in the soil and foundation regions, and then solving the corresponding radon concentration profiles, considering the lo- calized radon generation rates, decay rates, and transport rates by diffusion and advection. The air pressure distributions under and near the house are solved with LaPlace's equation applied to discrete re- gions to represent specified floor, footing, and soil materials. The resulting localized airflow velocities are used in the corre- sponding radon calculations in computing simultaneous diffusive and advective ra- don transport. The equations are solved numerically in elliptical-cylindrical geom- etry to represent houses of different sizes and with varying rectangular aspect (length/width) ratios. Radon entry rates into a house are computed by integrating the total radon transport across the floor surface area. Indoor radon concentrations also are estimated from the computed en- try rates by dividing by the house volume and its air ventilation rate. Implementation The differential equations describing air flow and radon generation and transport are solved numerically by finite-difference techniques. The house floor slab, foot- ings, and soil layers are divided into nu- merous, user-defined mesh units for these analyses. Several analytical functions in RAETRAD enhance its computational effi- ciency and simplify its user interface. The numerical calculations of air flow and radon transport through floor cracks are acceler- ated by use of analytical functions to esti- mate the mesh-equivalent permeabilities and radon diffusion coefficients for the speci- fied cracks, rather than using finely-graded numerical meshes to represent them. Ana- lytical functions are also used to define soil radon diffusion coefficients and air permeabilities when measured values are unavailable. These use soil porosities, water contents, and textures to define the radon transport properties from empirical correlations with measured data. In addi- tion to modeling symmetric cracks in the floor slab, RAETRAD also accommodates asymmetric openings such as utility pen- etrations that do not match the elliptical symmetry computed for the equivalent rect- angular house shape. These are repre- sented by multiple numerical calculations that determine transverse leakage terms for the discrete-point floor openings. The numerical-analytical calculations are performed by computing all finite-difference coefficients for each model mesh unit and solving the equations simultaneously by a non-iterative matrix inversion technique. The resulting computer code is relatively small and efficient and operates in a Win- dows® environment on an IBM®-compatible personal computer. Typical execution times are on the order of 1-2 minutes or longer, depending on the complexity of the prob- lem being solved and the speed of the computer. A user interface provides que- ries for definition of an input file and se- lection of appropriate input parameters. House parameters include area, volume, shape, ventilation rate, indoor air pres- sure, foundation depth, floor slab open- ings, and concrete properties. Soil parameters include layer thicknesses and localized values of soil density, moisture, radium concentration, and radon emana- tion coefficient. Certain properties, such as radon diffusion coefficient and air per- meability, can be left unspecified for use of default values estimated within the com- puter code. Comparisons with Analytical Data The RAETRAD code was validated and benchmarked by several comparisons with analytical calculations and with empirical radon data. The analytical validations in- cluded comparison with a 2-dimensional air pressure field calculated for a simple uniform 15 x 31 ft (4.6 x 9.4 m) soil space with two different pressures applied at its top surface. Relative standard deviations of less than 1% were obtained between the RAETRAD calculations and the ana- lytical pressure field at the 1-, 2-, 4-, 8-, and 15-ft (0.3-, 0.6-, 1.2-, 2.4-, and 4.6-m) depths below the pressure boundary. Analytical validations with 1 -dimensional radon generation and diffusion from an open soil and a concrete-covered soil sug- gested the utility of defining a small (0.1-ft or 0.3-m) mesh unit at the top of the soil profile to minimize the effects of mesh spacing. In these comparisons, both soil radon profiles and surface radon fluxes agreed consistently within less than 1%. Additional 1-dimensional validations in- cluded a uniform soil with radon genera- tion, diffusion, and advective transport. In this case, the air flow velocities were forced by an external definition of a uniform pres- sure gradient, since RAETRAD is designed to compute drily realistic, 2-dimensional pressure profiles. Again, agreement was within less than 1% for all cases of air flowing into the soil profile. When air was drawn from the profile, a depletion of the profile was observed that caused a maxi- mum error of 4% for the case that was analyzed. This error was reduced by con- sidering a thicker soil profile and was ex- aggerated if a thin soil layer was considered. Comparisons with Empirical Data Comparisons of RAETRAD calculations with empirical radon measurements uti- lized two test-cell structures (6 x 6 m) constructed in South-Central Florida and monitored primarily by Southern Research ------- Institute (SRI). One of these structures (test cell 1) utilized floating-slab floor con- struction with concrete-block stem walls over a concrete footing. The other struc- ture had similar footings and stem walls, but its floor slab was poured to extend into a course of chair blocks at the top of the stem wall. Both cells had identical wood-frame superstructures, without win- dows, that were sealed with 2-3 cm of polyurethane foam to minimize air infiltra- tion. Soil densities, radium concentrations, radon emanation coefficients, and mois- tures were measured in this project from numerous cores collected around and un- der the test cells. SRI provided measured soil radon and air permeabilities, and in- door pressures, air ventilation, and radon concentrations. Field soil sampling at the test cell site extended only to 4-7 ft (1.2-2.1 m) depths for most cores; hence deeper soil regions were extrapolated from existing moisture and radium data. Calculated radon con- centration profiles were within 4.4% of the means of measured values under test cell 1, compared to a 34% root-mean-square uncertainty among the measured values. Calculated radon profiles were within 18% of the means of measured values under test cell 2, compared to a 42% root-mean-square uncertainty among the measured values. Measured soil air permeabilities differed from values calcu- lated from soil density, moisture, and tex- ture by 42% based on composite averages at four depths. Excluding a heterogeneous, low-permeability layer under part of the site, the agreement was improved to 24% relative standard deviation. Indoor radon in the test cells was ana- lyzed by RAETRAD to compare with mea- surements before and after drilling a center hole in each of their slabs. For the initial slab conditions, RAETRAD computed 97 pCi L'1 in test cell 1, only 2% above the mean of the measured values, 95 ± 44 pCi L'. The radon computed by RAETRAD for test cell 2 was 20 pCi L1, which was 10% below the mean of the measured values, 22 ± 7 pCi L1. With a 10-cm center hole in each slab, test ceil 1 was computed to have an indoor radon con- centration of 212 pCi L'1, which was 17% below the mean of the measured values, 255 ± 78 pCi L1. Test cell 2 with a'center hole had a computed radon concentration of 87 pCi L1, which was 18% above the mean of the measured values, 74 ± 33 pCi L1. Computed air pressure and radon concentration profiles under test cell 1 had relative standard deviations from measured values of 11 and 12%, respectively, which were smaller than the standard deviations among the replicate measurements. Com- puted air pressure and radon concentra- tion profiles under test cell 2 had relative standard deviations from measured val- ues of 25 and 20%, respectively, which also were smaller than the standard de- viations among the replicate measure- ments. Additional comparisons of RAETRAD calculations with radon measurements in the test cells were performed with test cell 2 at indoor pressures of -10 and -20 Pa instead of its pas- sive-condition pressure of -0.6 Pa. For the -10 Pa condition, test cell 2 was computed to have an indoor radon con- centration of 51.5 pCi L1, which was 3% higher than the measured 50 pCi L1 value. For the -20 Pa condition, an in- door radon concentration of 42.9 pCi L1 was computed by RAETRAD, 14% lower than the measured value of 50 pCi L''. Collectively, the six model comparisons with indoor radon measurements in the test cells had an average difference of 11%, with an average bias of -3%. Comparisons of RAETRAD calculations with indoor radon measurements in 50 FRRP demonstration houses exhibited much larger variations (geometric stan- dard deviations of 2.8) and a bias of a factor of 0.56 below the measured values. This was attributed to the much less de- tailed characterization of the houses, pri- marily with respect to the concrete slab integrity and diffusivity. Significant unob- served holes or cracks (>50 cm2) near utility penetrations or by walls, bathtubs, or other features could cause this much bias, as could a 3-fold higher radon diffu- sion coefficient than was used for the floor (0.001 cm2 s'1). Observations and mea- surements support either of these possi- bilities. Conclusions RAETRAD provides a relatively simple, 2-dimensional numerical-analytical simu- lation of steady-state radon generation and movement into rectangular-equivalent slab-on-grade houses. It combines detailed airflow and radon source, transport, and decay calculations to accurately assess the effects of soil moisture, radon source distribution, and other soil and house vari- ables of interest. Validations with special-case analytical calculations dem- onstrated accuracy to within approximately 1 %. Comparisons with empirical data from FRRP test-cell structures demonstrated accuracy that was well within the uncer- tainty of the empirical measurements. Ap- plication to other houses was limited by assumptions about their floor slab integ- rity and diffusivity. ------- KirkK. Me/son, Vern C. Rogers, Vern Rogers, and Rodger B. Holt are with Rogers and Associates Engineering Corp., Salt Lake City, UT 84110-0330. David C. Sanchez is the EPA Project Officer (see below). The complete report, entitled "The RAETRAD Model of Radon Gas Generation, Transport, andIndoor Entry," (OrderNo. PB95-1'42030; Cost: $27.00, subject to change) will be available only from National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone: 703-487-4650 The EPA Project Officer can be contacted at Air and Energy Engineering Research Laboratory U.S. Environmental Protection Agency Research Triangle Park, NC 27711 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati, OH 45268 Official Business Penally for Private Use $300 EPA/600/SR-94/198 BULK RATE POSTAGE & FEES PAID EPA PERMIT No. G-35 ------- |