United States
                   Environmental Protection
                   Agency
National Exposure
Research Laboratory
Research Triangle Park NC 27711
                   Research and Development
EPA/600/SR-96/049  May 1996
4>EPA       Project Summary

                   Analysis  of Acid  Precipitation
                   Samples Collected  by  State
                   Agengies—Sampling  Period
                   January  1993-December 1993
                   Lloyd S. Shepard
                    This report presents analytical data
                   from the 29 acid precipitation collec-
                   tion sites in the State-Operated Net-
                   work  that were operational in 1993.
                   Samples are collected weekly in plas-
                   tic  bag  liners and shipped  in 500 mL
                   polyethylene  bottles  to  Global
                   Geochemistry Corporation (the central
                   laboratory for the network). This report
                   contains maps showing the  location of
                   each site, plots of analytical data, tables
                   of  all field and  analytical data,  plots
                   comparing field and laboratory pH and
                   conductivity, and information on data
                   quality.  Samples are  analyzed for pH,
                   strong acid, conductivity, fluoride, chlo-
                   ride, nitrite, phosphate, bromide, nitrate,
                   sulfate, ammonium, sodium,  potassium,
                   calcium, and magnesium. The central
                   laboratory renders technical  assistance
                   to the collection sites on problems con-
                   cerning  pH and conductivity. Each of
                   the ten participating state agencies re-
                   ceives  analytical reports for  the
                   samples analyzed the previous month.
                   Analyte  concentration data  are put on
                   tape for later  inclusion in  a national
                   acid deposition data base.
                    This Project Summary was developed
                   by  EPA's National Exposure Research
                   Laboratory, Research Triangle Park, NC,
                   to  announce key findings  of the re-
                   search project that is fully documented
                   in a separate report of the same title
                   (see Project Report ordering informa-
                   tion at back).

                   Introduction
                    The main report presents analytical data
                   from the 29 acid precipitation collection
                   sites in  the State-Operated Network for
the  year 1993. Samples are  collected
weekly in plastic bags inserted in buckets
and shipped in 500 mL polyethylene bottles
to Global Geochemistry Corporation (the
central laboratory for the network). Global
Geochemistry analyzes the samples and
monthly sends a report of the  analytical
results to each site. Global Geochemistry
also summarizes these results on mag-
netic tape for inclusion in a national acid
deposition data  base.  Individuals  con-
cerned with the collection  and interpreta-
tion of acid precipitation sample results
will find this report of interest.

Overview of Network Operation
and Sample Analysis
  The  central laboratory analyzes weekly
acid precipitation samples for pH, strong
acid, conductivity, fluoride, chloride, bro-
mide, nitrate, nitrite, sulfate, phosphate,
ammonium, sodium, potassium, calcium,
and magnesium.  The methods indicated
in Table I are used for these analytes.
  The  State-Operated Network collects
weekly samples using a wet/dry bucket
collector. Samples are collected in a plas-
tic bag inserted in the  bucket; an aliquot
of  the  collected  sample is  sent to  the
central laboratory in a 500 mL polyethyl-
ene bottle at ambient temperature (except
for one site that ships samples in a cooler).
The locations  of the network  sites  are
shown  in Figure 1.
  The  central laboratory  provides plastic
bucket liners, 500 mL sample bottles, field
data sheets,  pH and  conductivity solu-
tions, and other supplies incidental to col-
lecting  and shipping  a  collected rain
sample. The central laboratory also pro-

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Table 1. Method Used for Selected Analytes

Analyte                   Analytical Method
                                   Methodology
pH
Conductivity
Acidity

Cl, P04, S04
N03, F, Br, N02
NH4
A/a, K, Ca, Mg
EPA Method 150.1
EPA Method 120.1
Gran Titration

EPA Method 300. 0

EPA Method 350.1
EPA Methods 273. 1,
258.1,215.1,242.1
pH Electrode
Conductivity
Titration

Ion Chromatograph

Colorimetric
Atomic absorption
for Ca, Mg, Flame
Emission for A/a, K
vides technical assistance whenever it is
requested by a field site.  This assistance
consists mostly of field pH and conductiv-
ity measurement procedures  and equip-
ment.
  Monthly, the central laboratory sends a
report to each state agency describing the
analytical  results for all samples analyzed
from that agency's sites for the last month.
The  central laboratory  also  summarizes
the analytical  results for  all the  sites on
magnetic tape.

Report Contents
  The report contains a table showing the
latitude and longitude of each of the sites.
It also contains plots of analytical data for
each  site during the time period, tables of
all field and analytical data, a comparison
of analyte concentrations  at all sites  (fre-
quency  of occurrence), precipitation
weighted data for each site, plots compar-
ing field and laboratory pH and conductiv-
ity, and quality control tables and plots.

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  Lloyd S. Shepardis with Global Geochemistry Corporation, Canoga ParkCA 91303.
  Berne I. Bennett is the EPA Project Officer (see  below).
  The complete report, entitled "Analysis of Acid Precipitation Samples Collected by
    State Agengies—Sampling Period January 1993-December 1993," (Order No.
    PB96-175245; Cost: $44.00, subject to change) will be available only from
         National Technical Information Service
         5285 Port Royal Road
         Springfield,  VA22161
         Telephone:  703-487-4650
  The EPA Project Officer can be contacted at
         National Exposure Research Laboratory
         U.S. Environmental Protection Agency
         Research Triangle Park, NC 27711
United States
Environmental Protection Agency
National Risk Management
Research Laboratory (G-72)
Cincinnati, OH 45268
     BULK RATE
POSTAGE & FEES PAID
         EPA
   PERMIT No. G-35
Official Business
Penalty for Private Use
$300
EPA/600/SR-96/049

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