United States Environmental Protection Agency National Exposure Research Laboratory Research Triangle Park, NC 5711 Research and Development EPA/600/SR-98/020 July 1998 Project Summary Monitoring and Assessment of In-Situ Biocontainment of Petroleum Contaminated Ground-Water Plumes R. Ryan Dupont, Darwin L. Sorensen, Marian Kemblowski, Mark Bertleson, Dietrick McGinnis, Idris Kamil, and Yang Ma Abstract This two-year field research project was conducted to assess the potential for natural attenuation of gasoline-con- taminated ground-water plumes at two underground storage tank (LIST) sites in northern Utah. An evaluation of rapid site-assessment techniques for plume delineation and subsurface site charac- terization was carried out using cone penetrometer and ambient temperature headspace (ATM) analysis techniques. An approach was developed for the col- lection and evaluation of soil and ground-water monitoring data for de- termining the efficacy of in-situ biocontainment and to identify "stabi- lized" fuel-impacted ground-water plumes. A decision framework was de- veloped to guide the user in data collec- tion, data reduction, data interpretation, and decision making efforts to evaluate the nature and potential extent of intrin- sic plume bioattenuation taking place under a given set of site conditions. Data collected from the two field sites are pre- sented and evaluated in detail, the rate and extent of the natural attenuation of ground-water plumes are quantified, and recommendations regarding source re- moval action are made for these two field sites. The information in this document has been funded wholly or in part by the United States Environmental Protection Agency under CR 818835-01 to the Utah Water Research Laboratory, Utah State University. It has been subjected to the Agency's peer and administrative re- view, and it has been approved for pub- lication as an EPA document. Mention of trade names or commercial products does not constitute endorsement or rec- ommendation for use. This Project Summary was developed by the National Exposure Research Laboratory's Characterization Research Division, Las Vegas, NV, to announce key findings of the research project that is fully documented in a separate report of the same title (see Project Report or- dering information at back). Introduction Ground-water quality impacts resulting from leaking underground petroleum stor- age tanks are a significant environmental concern due to the sheer number of such tanks and the extent of possible environ- mental contamination when they leak. Many of these tanks are being removed and re- placed or upgraded to eliminate the source of possible petroleum contamination to un- derlying aquifers. However, there remains a large number of sites with ground-water contamination above existing water quality limits (300,000 confirmed releases as of June 1995, with an additional 100,000 re- leases expected by 2000 (e.g., personal communication, Hal White, U.S. EPA, OUST, 1995). While contamination from pe- troleum storage tank releases can have a significant impact on public health and the environment, active remediation of these contaminated sites can be difficult and ex- pensive. Expectations of having to apply ------- active remediation at all sites has generally not allowed the focusing of resources on those sites representing the greatest threat to public health and the environment. When gasoline is released into the sub- surface, it distributes among the soil, gas, and aqueous phases that make up this en- vironment. As it moves through the unsat- urated zone, it leaves behind vapors con- taining volatile gasoline components and residual liquid hydrocarbons retained within the soil matrix. A large fraction of gasoline is water soluble and migrates to underlying aquifer with infiltrating water. Plumes of ground-water hydrocarbon contamination spread within the soil environment by ground-water advection and diffusion. Many gasoline components are biodegradable, and a primary mechanism for their trans- formation in the subsurface is via biodeg- radation. Biotransformation takes place under a variety of soil pH and oxidation re- duction potential (redox) conditions, and in- volves various terminal electron acceptors (oxygen, nitrate, manganese, iron, sulfate, carbon dioxide, carbon). If biodegradation of a contaminant proceeds at a rate greater than or equal to the rate of advance of the contaminant front, the plume will be effec- tively contained, and can eventually be com- pletely remediated if the source of contami- nation is removed. The only costs associated with site clean- up under these intrinsic biocontainment conditions are related to the costs for source removal and for the necessary, on-going monitoring of contaminant distribution and movement overthe lifetime of the dissolved contaminant plume. Without reliable con- tainment information, contamination may continue to spread, worsening existing con- ditions, posing increased public health risk, and increasing final clean-up costs. To ob- tain intrinsic degradation process rates for contaminants at fuel release sites, chemi- cal/biological parameters indicative of in-situ biodegradation processes taking place in these environments must be well under- stood and documented. Once this is accom- plished, routine measurements of these parameters, or a subset of these param- eters, would allow identification of condi- tions under which in-situ biodegradation could be relied upon to provide natural at- tenuation of a contaminant plume. The goal of this project was to identify and validate field monitoring techniques, and data reduction and reporting methods that can be utilized to rapidly and conclu- sively demonstrate the existence of intrin- sic biodegradation reactions at leaking LIST sites. With this demonstration of the natu- ral containment of a hydrocarbon plume, ra- tional decisions can be made regarding the need to actively remediate it to ensure the protection of public health and the environ- ment. Based on an evaluation of field and laboratory water quality determinations, soil core measurements, and companion mod- eling results, recommendations have been made regarding the selection of process variables, monitoring procedures, and data reduction and reporting methods that should be implemented at hydrocarbon contami- nated sites to document intrinsic bioreme- diation of ground-water plumes. Procedure The research was conducted in four phases. The first was a site assessment/ characterization phase in which contami- nant distribution and site hydraulic charac- teristics were determined using rapid field characterization methods. The second phase involved process monitoring, in which field techniques were used to monitor ground-water and soil gas characteristics that reflect in-situ biodegradation reactions taking place throughout the field sites. The third phase was the reduction of field data to yield estimates of total dissolved plume contaminant mass, center of mass, mass center trajectory, contaminant degradation rates, and estimated source lifetime. The final phase involved the use of a three-di- mensional analytical model to provide in- situ biodegradation process verification and long-term predictions of fate of the plume as attenuated by natural biodegradation reactions. Two field sites with known contamination from gasoline storage tanks were selected for this study: the Hill AFB site and the Layton, Utah site. Both sites were "aged" with initially "constant" source terms where it was reasonable to hypothesize that natu- ral biodegradation reactions, and subse- quent plume containment, had developed and were quantifiable. Single and multi-level ground-water monitoring probes were placed within and around the area of the contaminant plume at both sites. These wells included upgradient "background" wells, and wells within the area of contami- nation, allowing the definition of the bound- aries of the plumes with some certainty. A gradient of chemical and biological condi- tions was observed throughout each plume so that transformation/degradation rates, mass transfer rates, etc., could be esti- mated. Plume characterization was carried out using cone penetrometry and 5/8-in di- ameter piezometer ground-water sampling wells to rapidly and inexpensively collect soil textural information and ground-water data from sampling locations throughout each plume. During long-term monitoring, site characterization information was collected using all of the ground-water sampling points. The following data were collected throughout the site during the initial site characterization phase and six times dur- ing the process monitoring phase of the project: in ground water-pH, O2, Fe2+, Mn2+, NO3-, SO42', CI-; in soil gas—O2, CO2; and in both soil gas and ground water- aromatic hydrocarbons and total petroleum hydrocar- bons (TPH). Field data were reduced to generate es- timates of total dissolved mass of contami- nant using the Thiessen area method (Chow et al., 1988) to assign a specific plume area to each ground-water monitor- ing point. Total dissolved plume mass was estimated for each sampling event, while the center of the total dissolved plume mass was estimated by taking the first moment about a defined axis of the masses repre- sented at each sampling location within the contaminant plumes. The movement of the plume centroid over time was described based on the changes in its absolute posi- tion, and contaminant plume velocities were calculated between each sampling interval. Contaminant degradation rates were esti- mated based on the change in total dis- solved plume mass between each sampling interval. Aquifer assimilation capacity was estimated based on the change in terminal electron acceptor concentration and mass inside versus outside of the plume. Finally, an analytical, three-dimensional ground-water fate-and-transport model, which accounts for advection, dispersion, contaminant sorption and contaminant deg- radation, was applied to both field sites to validate intrinsic biodegradation reactions observed at these sites. Hydraulic proper- ties were selected based on measured field data and information regarding the nature of soil below each site. A source configura- tion was established for each site. Model input variables for measured source con- centrations, contaminant properties, and time since the release were varied to as- sess the sensitivity of the model to these parameters and to determine those combi- nations of parameters producing the best model fit of centerline contaminant concen- trations for a tester data set. The effects of source removal on the lifetime of the plume and the maximum plume travel distance were assessed using the site-specific, field- data calibrated model. Results and Discussion Site Assessment/Monitoring Techniques Cone Petrometer Testing (CPT) Methods The application of cone penetrometer testing (CPT) for soil textural data collec- ------- tion coupled to piezometer well placement is appropriate for initial site investigation activities at sites where no prior data regard- ing ground-water plume characterization are available. These techniques can also be effectively applied at sites where exist- ing data are limited in scope and detail, as was exemplified from the results obtained from CRT and ground-water probe data collected at the Hill AFB site. The Hill AFB site was the location of a former 18,000-gallon LIST that was exca- vated in 1989. At the time of excavation, holes were observed in the tank and petro- leum odors were detected in the tank pit. Five conventional ground-water monitoring wells were installed at the site and soil gas. Soil boring and limited ground-water moni- toring data collected from the site from 1989 to 1991 led to the conceptual site model suggesting a plume migrating to the south- west. Soon after site investigation activities began, it became apparent that the initial conceptual model of contaminant distribu- tion and plume migration at the Hill AFB site was significantly flawed. Ground probe samples that were collected near the source of contamination within the plume bound- aries showed hydrocarbon levels at back- ground concentrations. CRT analysis and ground-water piezometer sampling were moved into the north and northwest regions of the site in an attempt to locate the con- taminant plume. Field hydrocarbon screen- ing data collected from these piezometers were successful in identifying the true north- westerly direction of the hydrocarbon plume as indicated by the ground-water concen- tration data shown in Figure 1. CRT mea- surements collected in this study also pro- vided insight into ground-water flow condi- tions existing below the Hill site. Figure 2 clearly indicates a distribution of high and low permeability deposits that correspond to what appears to be an old stream bed resulting in channeling of the regional west- erly flow to the northwest direction beneath the Hill site. It is not known how widespread the find- ings for the Hill AFB site are in terms of the development of a less than complete pic- ture of actual plume distribution and trans- port using limited, conventional site investi- gation data. It was found, however, that the use of CRT methods facilitated the rapid collection of soil textural information and the placement and sampling of ground-water probes that allowed a much more compre- hensive picture of both structural and chemi- cal features of the subsurface than was possible using soil core sampling and labo- ratory analysis procedures routinely applied at LIST sites. This added information is com- bined with the complete elimination of soil • Single Level Piezometers * Multilevel Piezometers Q Monitoring Wells -20 0 20 40 60 80 100 120 140 160 180 North Coordinates (ft) Figure 1. Initial ground-water plume hydrocarbon data developed from field screening headspace analyses conducted at the Hill AFB site, July 1992. 180 160- 140- 120- 100- • Single Level Piezometers * Multilevel Piezometers O Monitoring Wells -20 -20 20 40 60 80 100 120 140 160 180 North Coordinates (ft) Figure 2. Textural map for soils at the ground-water table generated from CRT data collected at the Hill AFB site in July 1992. ------- cuttings and large volumes of contaminated ground water that are often costly and regulatorily challenging to manage, making the screening techniques used in this study ideal for application at many sites. The im- portance of additional insights into local ground-water flow conditions that can be provided by these CRT techniques is also unquestionable, especially when consider- ing an intrinsic remediation management option at a site. Ambient Temperature Headspace (ATM) Results Two data sets (July and December 1992) were collected from each field site to evalu- ate the representativeness of ATM field screening techniques compared to results generated from standard laboratory-gener- ated purge-and-trap hydrocarbon measure- ments. This comparison between field- and laboratory-generated results was based on total hydrocarbon determinations using se- rial dilutions of a gasoline-saturated water standard in the field and hexane-equivalent concentrations for laboratory results. The ratio of field- and laboratory-deter- mined ground-water hydrocarbon concen- trations was quite variable, ranging from a low of 0.0 to a high of 446. This ratio was generally consistent for a given sampling location between the two sampling times; however, some ratios varied by one to two orders of magnitude. The average ratio of field- to laboratory-determined ground-wa- ter hydrocarbon concentrations was greater than 1 for both sampling events at both sites, and ranged from 4.9 to 32.1. This result suggests that the field ATM procedures used in this study provided a conservative esti- mate of contaminant concentration from most sampling locations by a factor of 5 to 30. A statistically significant relationship was found between laboratory and field data for both sites. A background field concentration of 279 |ig/L was found when laboratory re- sults indicated azeroTPH concentration at the Hill AFB site, while at the Layton site, a ground-water concentration of 3,680 |ig/L was indicated from ATM readings before laboratory purge-and-trap methods de- tected TPH contamination. The slope of the field versus laboratory hydrocarbon concen- tration relationship was less than one for the Hill AFB site, indicating that when true ground-water concentrations (as defined by laboratory purge-and-trap results) exceed 842|ig/L, field ATM values under-predict ac- tual ground-water TPH concentrations. The slope of the Layton relationship was greater than one, however, indicating that unlike the Hill AFB data, field ATH measurements con- sistently over-predicted laboratory purge- and-trap ground-water concentrations by nearly a factor of two. These findings suggest that there is a general relationship between laboratory and field ATH determined hydrocarbon concen- trations, but this relationship is very much site-specific. The utility of these field ATH measurements appears then to be in the initial site assessment phase where rapid, semi-quantitative results are used for de- tailed plume delineation efforts. Field ATH measurements can be used to effectively guide initial ground-water quality investiga- tions and to optimize ground-water moni- toring probe and monitoring well placement for long-term site monitoring. Once this ini- tial screening is completed, however, labo- ratory analyses are necessary to provide accurate ground-water quality data for fur- ther site fate-and-transport and intrinsic re- mediation evaluation. Hill AFB Site Intrinsic Remediation Results Site Background Data This site is located in the west area of Hill AFB south of the city of Ogden, Utah. The site is immediately north of Building 1141 that was used by the Air Force for small vehicle maintenance. Generally, the regional shallow and deep ground-water flow direc- tion through the fluvial and lacustrine de- posits underlying the base is from the moun- tains on the east toward the Great Salt Lake on the west. Hydraulic conductivity of the shallow soils at the Building 1141 site, as determined by slug tests performed on se- lected wells by Engineering Science, were found to range between 1.0x10-5 and 7.7 x 10-5 cm/s. In December 1989, an 18,000-gallon bare steel gasoline UST was excavated and no free-phase hydrocarbons were observed at this time, although observations of odors and holes in the UST indicated that a re- lease may have occurred. Two soil samples and a ground-water sample were collected and analyzed for benzene, toluene, ethylbenzene, xylenes (BTEX), and total petroleum hydrocarbons (TPH). Data from this sampling event indicated that residual and dissolved BTEX and TPH contaminants were present in the soil and shallow ground water. Field investigative activities con- ducted in October and November 1990 in- cluded a soil-gas survey, soil borings, instal- lation of ground-water monitoring wells, col- lection of soil and ground-water samples for laboratory analyses, slug tests, and a site survey. From these analyses, limited re- sidual-phase and dissolved hydrocarbons were documented in the soil and the upper portion of the shallow aquifer immediately downgradient and adjacent to the former UST. In March 1991, levels of dissolved con- taminants in the ground water were similar to those documented in November 1990. No free-phase product was observed, indicat- ing that the bulkofthe released product was bound in capillary pore spaces of the shal- low soils. In July and August 1992, CPTdata were collected at 44 locations throughout the Hill AFB site to augment the existing five- well monitoring network. CPT data success- fully identified a subsurface stream chan- nel (Figure 2) at the ground-water table, producing a significant northerly flow com- ponent to the regional, westerly ground- water flow. Seven sampling events were used at the Hill AFB site to describe the distribution and movement of contaminants and electron acceptors occurring at the site between April 1992 and January 1994. These data were used to determine steady-state plume con- ditions and to estimate total mass and mass centervaluesforvariousanalyt.es at the site overtime. Intrinsic Remediation Assessment Determination of Steady-State Plume Conditions Based on centerline concentration data observed at the Hill AFB site overtime, the concentration profile for BTEX and TPH constituents remained at pseudo-steady- state after December 1992. To further evalu- ate plume stability conditions, total dissolved plume mass was estimated overtime. To determine dissolved plume mass, Thiessen areas were generated for each sampling event using a fixed outer plume boundary and individual areas determined based on the actual sampling locations used in a given sampling event. Specific com- pound mass data shown in Figure 3 sug- gest that steady-state conditions existed for some of the compounds (benzene, toluene, naphthalene) during a portion of the study period, while a continuously declining mass was seen for ethylbenzene and p-xylene during the entire study period. All of the spe- cific compounds of interest did show a sig- nificant decline at the end of the study, how- ever. Dissolved plume TPH mass confirmed the non-steady-state conditions existing at the Hill AFB site, as its mass was found to exponentially decay over time. Center of mass analyses showed migration of the mass center downgradient from its location in August 1992, although the total downgradient distance traveled was small, ranging from a maximum of 106 ft for TPH, to a low of only 17 ft for naphthalene. This ------- o Benzene o Toluene A Ethylbenzene * p-Xylene + Naphthalene Figure 3. Time course of total dissolved plume mass estimates for BTEX and naphthalene con- taminants at the Hill AFB site over the course of the study. decreasing contaminant mass and center of mass moving downgradient suggest that the source was finite, and despite plume mi- gration, the reductions in contaminant mass indicated assimilation was taking place. Estimation of Parent Compound Degradation Rate Because the mass of contaminants in the dissolved plume at the Hill site were found to be decreasing over time, the plume ap- peared to originate from a pulse source. With a pulse source, contaminant degrada- tion rates can be estimated by linear regres- sion of total dissolved contaminant mass data versus time. The results of these re- gressions are shown in Table 1. Estimation of Source Mass/ Lifetime The projected lifetimes of the BTEX ground-water plumes using this mass ver- sus time regression approach were quite short, being less than 2 weeks from the last sampling event. This was due to the low mass of contaminant remaining in the plume as of January 1994. The naphthalene and TPH plumes could persist for a much longer time but were estimated to last only slightly longer than 2 years at the current rate of degradation. The TPH plume mass center was projected to move the farthest of the compounds analyzed in the study, a total of 156 ft downgradient from its position in January 1994. This puts the mass center approximately 50 ft downgradient of the existing monitoring network, still within the boundaries of Hill AFB, and without impact to a downgradient receptor. Predicting Long-Term Behavior Consideration of a source removal sce- nario for this site is not relevant as data in- dicate that the initial contaminant mass has been depleted from the original source area through intrinsic processes of contaminant dissolution, dispersion, and degradation. The long-term behavior of the plume is modeled using the degradation rates of the contaminants within the "detached" dis- solved plume and the rate at which the con- taminants are migrating within the aquifer. The results of this analysis are shown in Table! Decision Making Regarding Intrinsic Remediation Impacted Receptors The long-term behavior of the contami- nant plumes existing at the Hill AFB site pro- jected from contaminant degradation and transport data suggests that the maximum extent of any plume of interest will only be 50 ft downgradient of the existing ground- water monitoring network. This limited ex- tent of potential contaminant migration en- sures that no downgradient receptors will be impacted by contamination at the Hill AFB site over the projected lifetime of the ground-water plumes that exists there. Potential Aquifer Assimilative Capacity When the mass of electron acceptor mov- ing onto a site equals or exceeds the sto- ichiometric equivalent of dissolved contami- nant in the plume, then it can be assumed that the availability of the electron acceptor will not limit future contaminant degradation and plume attenuation. The electron accep- tor concentrations quantified throughout the contaminated portion of the Hill AFB site were used along with the electron acceptor concentrations measured in background ground water to estimate the potential as- similative capacity existing within the aqui- fer. The hydrocarbon (HC) assimilative ca- pacities related to dissolved oxygen (0.66 mg HC/L), nitrate (5.4 mg HC/L) and sul- fate (10.7 mg HC/L) utilization were based on the lowest observed concentration in the background well. For iron (0.06 mg HC/L) and manganese (0.02 mg HC/L), their as- similative capacities were estimated based on the smallest increase in the soluble con- centrations of these solid phase electron acceptors observed within the center of the plume during the study. Sulfate was the most significant electron acceptor, accounting for more than 60 per- cent of the potential assimilative capacity at the site. The potential assimilative capac- ity projected for the site was more than 90 times greater than that required to assimi- late the TPH remaining there. This result provides additional evidence that an intrin- sic remediation management option for the Hill site would be protective of public health and the environment. Layton Utah Site Intrinsic Remediation Results Site Background Data The Elaine Jensen R.V. facility, Layton, UT, was used as a recreational vehicle (RV) sales and service facility during the study and consisted of a service shop, an RV sales building, and associated sales and display Table 1. Contaminant center of mass velocities and degradation rates based on ground-water data collected at the Hill AFB site from March 1992 to January 1994 Benzene Distance Traveled (ft) Contaminant Velocity (ft/d) Contaminant Velocity (ft/yr) Zero Order Degradation Rate (g/d) Zero Order Degradation Rate (g/yr) First Order Degradation Rate (1/d) First Order Degradation Rate (1/yr) Remaining Mass in 1/94 (g) Time to Degrade Remaining Mass - Zero Order (d) Time to Degrade 99.9% Mass - First Order (d) Travel Distance in Degradation Time (ft) 25.7 0.05 18 =0.10 =36.9 0.41 =4.1 =0.20 Toluene 53.3 0.1 37.4 =0.099 =28.5 0.66 =6.7 =0.67 Ethyl- benzene 42.9 0.08 30.1 0.063 23.4 0.53 8.4 0.67 P- Xylene 55.6 0.11 39 0.058 22.3 0.8 13.8 1.5 Naphthalene 17.2 0.03 12.1 =0.026 =9.5 0.13 =266 Q ~O TPH 106 0.2 74.2 0.009 3.285 28.8 768 156 ------- lots. The majority of the site is covered by asphalt, and several underground utilities are present. The ground surface slopes gently toward the southwest and toward U.S. Interstate Highway 15 which borders the site directly to the west. The property was in agricultural production until approxi- mately 1958, at which time it was leased to Sinclair Oil for retail gasoline sales from a newly constructed gasoline station building (the present service shop). The fuel stor- age and dispensing system consisted at that time of four USTs (2,000 gallons each) with suction pumps located to the west of the tanks. The property was subsequently uti- lized for camper sales between 1968 and 1974, followed by use for retail gasoline sales until 1984. The site was upgraded in 1974 with three additional 6,000-, 8,000-, and 10,000-gallon USTs equipped with pressurized dispenser systems. The tanks were removed in 1984, and the property was subsequently used forthe recreational vehicle sales and service facility that occu- pied the site during the study. The area sur- rounding the site is characterized as mixed residential and agricultural use. Soils encountered at the site are prima- rily sands in the southern portion of the site and silts and clays in the northern half of the site. Ground water is encountered at approximately 8 to 10 ft below grade. The direction of shallow ground-water flow is predominantly southwest, although westerly and northwesterly flows were observed at the site during the study. Hydraulic conduc- tivity values of the shallow aquifer at the Layton site, determined by slug tests per- formed during this study, indicated values ranging from 0.78 to 3.1 ft/d, with an aver- age of 1.5 ft/day. A soil-gas survey was performed in 1990 at a depth of approximately 4 ft below ground surface using a portable organic vapor monitor (OVM) equipped with a pho- toionization detector (PID). A total of 36 lo- cations were surveyed for volatile organic vapors. The highest vapor concentrations (250 to 1,975 ppmv) were found in the two tank excavations and in the dispenser is- land area between the former tanks. An outer area of lower vapor concentrations (0 to 250 ppmv) extended to the west and southwest. Overall, an area of elevated vapor concentrations of approximately 18,400 ft2 was identified. In January 1991, soil borings were collected and three ground-water monitoring wells were in- stalled and screened across the water table from 7 to 17 ft below ground surface. In July and August 1992, CRT data were collected at 27 locations to augment the existing monitoring network. This detailed site investigation effort provided analysis of soil textural features from the surface to a depth of 22 ft. This CRT information sug- gested a finer grained material than was in- dicated from soil boring data, and identified a clay to silty clay lens 2 to 6 ft thick cover- ing most of the site 12to 14 ft below ground surface. Seven sampling events were conducted at the Layton site to describe the distribu- tion and movement of contaminants and electron acceptors taking place there be- tween April 1992 and January 1994. These data were used to determine steady-state plume conditions and to estimate total mass and mass center values for these various analytes, and to model contaminant trans- port and degradation occurring there over time. Intrinsic Remediation Assessment Determination of Steady-State Plume Conditions A westerly centerline transect was used to make a determination regarding steady- state plume conditions. Figure 4 shows plume centerline data for combined BTEX concentrations at the Layton site from July 1992 to February 1995. A pseudo-steady- state was found to occur for both BTEX components and TPH. Both BTEX and TPH concentrations increased and decreased along the plume centerline transect over time, but no consistent pattern downgradient of the source was evident. Thiessen areas generated for each sam- pling event using a fixed outer plume bound- ary forthe Layton site are shown in Figure 5. Based on the Thiessen areas associated with each monitoring point at each sampling time, estimates of the total dissolved plume mass and center of mass of BTEX, naph- thalene, and TPH were made. Despite a decline in dissolved contami- nant mass observed at the Layton site be- tween July 1992 and September 1993, fur- ther sampling in January 1994 and Febru- ary 1995 indicated that the dissolved mass of the contaminants has remained essen- tially constant over the two and one-half year project period (Figure 6). The mobility of the center of mass of all of BTEX, naph- thalene and TPH was limited, with a maxi- mum of only a 10-ft movement of TPH mass over the two and one-half year field study. The pseudo-steady-state contaminant mass levels and limited center of mass movement downgradient suggest that a continuous source exists at the Layton site which reflects a plume stabilized by con- tinuing intrinsic attenuation mechanisms. 20 40 60 80 100 120 Distance Downgradient of CPT-19 Figure 4. Combined BTEX plume centerline con- centration data collected at the Layton, UT, site from July 1992 to February 1995. CPT-17 CPT-09 s jCPT-Hx --X^ ^ A SCPT-15 - . ,.MW-03_^—-\ CPT-08 [ CPT-13 MLP.06 CPT-07 >/CP\.14 * VMLP-OSC - CPT-19 0 MW-04 Figure 5. Outer plume boundary used for Layton site plume total mass and mass center calcula- tions. Thiessen areas forthe July 1993 sampling event are shown. 12000 3 10000 200 400 600 800 Time (days) Figure 6. Time course of total dissolved plume mass estimates for BTEX and naphthalene con- taminants at the Layton site during the study, July 1992 through February 1995. ------- Estimation of Contaminant Degradation Rate Using the intrinsic remediation protocol developed in this study, the estimation of contaminant degradation rates with a steady-state plume mass is carried out ei- ther from an analysis of plume centerline concentration data or through the calibra- tion of a fate-and-transport model using field data. Plume centerline concentration data A steady-state, time-averaged concentra- tion profile was used to estimate first order degradation rates, the results of which are summarized in Table 2. Naphthalene had the slowest degradation rate, while benzene was found to be the most degradable of the compounds investigated. These degrada- tion rates do not explicitly account for re- ductions in concentration due to dispersion and dilution (i.e., non-degradative) pro- cesses taking place within the Layton aqui- fer. The more preferred approach to esti- mate contaminant degradation involves the use of a ground-water fate-and-transport model that is calibrated to field-generated data. Ground-Water Model Calibration An analytical solution for the advection- dispersion equation with degradation (as- suming a continuous source with one-di- mensional ground-water flow) was applied, along with site-specific physical/chemical input parameters, to model the fate and transport of contaminants under actual field conditions. Aquifer pore water velocities were calculated based on measured values of hydraulic gradient (0.01 ft/ft) and hydrau- lic conductivity (1.5 ft/d) and estimated val- ues of total aquifer porosity (0.38) using Darcy's Law. An average pore water veloc- ity of approximately 0.037 ft/d resulted. Transverse dispersivity was assumed to be 1/20th of the longitudinal dispersivity while vertical dispersivity was assumed to be negligible (0.001 m). Based on current prac- tice, a longitudinal dispersivity of 0.1 times the plume length was used, resulting in lon- gitudinal and transverse dispersivity values of 14 and 0.7 ft, respectively. Contaminant retardation factors were estimated from compound-specific organic carbon normal- ized soil/water partition coefficients (Kocs). The soil organic carbon content, bulk den- sity, and porosity values assumed for the Layton aquiferwere 0.3%, 1.15 g/cm3, and 0.38, respectively. The analytical solution used in this intrin- sic remediation protocol assumes a con- stant plane source perpendicular to the di- rection of ground-water flow. The Layton site vertical source dimension was set equal to Table 2. Contaminant degradation rates estimated from time-averaged centerline concentrations measured at the Layton site from July 1992 to February 1995 Compound Benzene Toluene Ethylbenzene p-Xylene Naphthalene First Order Rate (1/d) 0.00087 0.00044 0.00026 0.00024 0.00014 95 Percent Confidence Interval (1/d) 0.00057 0.00010 0.00010 0.00013 0.00008 r2 0.8204 0.9742 0.9263 0.8737 0.8243 p Value 0.0129 0.0003 0.0021 0.0063 0.0123 10 ft, the approximate maximum thickness of the contaminated ground-water column observed in monitoring wells. The lateral source dimension was based on an inspec- tion of contaminant concentration profiles perpendicularto ground-water flow nearthe source area, approximately 100 ft. From the site history, a range of simula- tion times from 10 to 25 years was used for model calibration. Contaminant degradation rate and simulation time were varied to evaluate the sensitivity of model output to these parameters, and to determine those combinations of parameters producing the best model fit. From model calibration, a source simulation lifetime of 25 years re- sulted in the best overall model fit. Benzene results are shown in Figure 7, while Table 3 summarizes model-calibrated degradation rates for all contaminants of interest. Estimation of Source Mass/ Lifetime When a continuous source is identified at a site, the estimation of source mass and source lifetime is based on the total mass of contaminant existing both above and below the ground-water table. This mass is generally estimated based on soil core con- centration data collected from within the source area. The estimated source area mass at the Layton site appeared to be greatly underpredicted by soil core results based on the dissolved plume masses mea- sured in February 1995. Source area mass was then estimated based on typical re- sidual hydrocarbon saturation within a smear zone at and below the ground-water table for a given soil texture. It was assumed that approximately 10 percent of the sub- surface porosity could be expected to be occupied by product material in the clay to silty clay soils below the Layton site, result- ing in an estimated 241,000 Ib of TPH re- maining in the source area. Because of the large mass of contami- nant remaining within the source area, with- out source removal, site management re- quirements could be in excess of 100 years based on an ethylbenzene maximum con- taminant level (MCL) of 700 |ig/L and a source area ethylbenzene ground-water concentration of» 1,900 ug/L measured in February 1995. With source removal, the time to reach the ethylbenzene MCL is re- duced to slightly more than 10 years, with benzene becoming the contaminant taking the longest to assimilate, requiring approxi- mately 20 years before reaching its MCL. Source removal greatly reduces the length of time for assimilation of the mass of all contaminants at the Layton site, strongly suggesting the need for source removal so that the duration of site management be- comes acceptable. Predicting Long-Term Behavior The time to reach the MCL following source depletion can be predicted for each component using the calibrated fate-and- transport model described in this report by the superposition of a continuous source plume, with a source concentration equal to the negative of the original source con- centration, -Co, on top of the steady-state plume concentration profile, at a point in time corresponding to the time of source removal. A benzene plume of greater than the MCL of 5 ug/L is projected to persist for 18 years, while all other contaminants of concern are projected to reach their MCL values everywhere within the plume in less than 7.5 years following source removal. Decision Making Regarding Intrinsic Remediation Impacted Receptors The projected long-term behavior of the contaminant plumes existing at the Layton site suggests that they have stabilized and are not expected to migrate from the site as long as existing site hydraulic conditions persist. This limited extent of potential con- taminant migration ensures that no Potential Aquifer Assimilative Capacity The aquifer assimilative capacities re- lated to dissolved oxygen (0.76 mg HC/L), nitrate (19.6 mg HC/L), sulfate (30 mg HC/ L), iron (0.06 mg HC/L), and manganese ------- Ground-Water Contaminant Concentration (^ig/L) 7,000< 6,000- 5,000- 4,000- 3,000- 2,000- 1,000- 0 - I '1 Simulation Parameters: ' Degradation rate = 0.00086/c •i R = 2.7, t = 25 yr \ * » Field Measured Data ^ - Predicted Data \ v_ *""^*«fc 0 20 40 60 80 100 120 140 160 180 200 Downgradient Distance from Source Area ( Figure 7. Results of benzene plume centerline calibration at the Layton site using data collected in March 1993. (0.03 mg HC/L) amounted to approximately 50.5 mg HC/L. With a maximum TPH con- centration of nearly 100 mg/L and a maxi- mum BTEX concentration of nearly 25 mg/ L observed during the study, this potential assimilative capacity is marginal. This re- sult provides additional evidence that some form of source removal to reduce contami- nant mass flux into the impacted ground water is the preferred approach for the Layton site. Without additional contaminant source removal, intrinsic remediation ap- pears marginally protective of public health and the environment. CONCLUSIONS AND RECOMMENDATIONS The research was conducted in four phases: 1) site assessment and character- ization; 2) process monitoring; 3) field data reduction; and 4) three-dimensional analyti- cal modeling. Based on the results of the study, the following conclusions can be made. 1. Conventional site assessment tech- niques using a small number of large diameter ground-water monitoring wells and limited soil core and shal- low soil gas survey data can be se- verely limited in their ability to provide a detailed understanding of subsur- face soil conditions at a site. CRT techniques can be used to improve delineation of subsurface conditions that may greatly impact local ground- water flow and contaminant transport. Coupled with placement of small di- ameter ground-water monitoring probes and field ATM measurements, CRT measurements enabled the col- lection of cost-effective data for accu- rate plume delineation on nearly a real-time basis in this study. 2. The field ATM method used in this study appears more sensitive in situ- ations with free product or high levels of residual saturation, than at those sites where weathered fuel contami- nation exists. Field ATM measure- ments can be used to effectively guide initial ground-water quality investiga- tions and to optimize ground-water monitoring probe and monitoring well placement for long-term site monitor- ing. However, field screening data should not be used as a substitute for laboratory determined, long-term ground-water monitoring data. 3. Centerline concentration profile and dissolved contaminant mass analyses indicated that a significant decline in all contaminant mass levels took place at the Hill AFB site over the course of the study. Center of mass calculations suggested that the plume was re- sponding to a pulse source with con- taminant attenuation. Dissolved plume mass changes over time were used to estimate zero and first order deg- radation rates for BTEX, naphthalene, and TPH contaminants. The lifetime of the BTEX compounds within the Hill AFB plume were short. Approximately 270 days was pre- dicted for 99.9 percent naphthalene removal. More than 2 years was esti- mated for the same removal efficiency of TPH components under existing site conditions. The decision to apply intrinsic remediation at the Hill AFB site is warranted based on: a) the con- taminant degradation rates and plume attenuation observed; b)the absence of an impacted downgradient recep- tor; and c) the potential aquifer assimi- lative capacity that is more than 90 times greaterthan that required forthe assimilation of the TPH and BTEX re- maining in the dissolved plume. A long-term monitoring scheme for both compliance and process monitoring purposes can be carried out using the existing monitoring network. Annual monitoring until 1997 should provide adequate data to validate complete plume assimilation to permit site clo- sure. Centerline concentration profile, dis- solved contaminant mass and center of mass analyses for the Layton site indicated that the plume appeared to be at steady-state through February 1995. Results suggest that the Layton plume was acting as a continuous source which was stabilized by on-go- ing intrinsic attenuation mechanisms. Changes in contaminant plume centerline concentrations with dis- tance from the source area and a con- taminant fate-and-transport model de- scribed in this study were also used to estimate contaminant degradation rates using measured March 1993 field data. Comparison of results from the centerline concentration and model calibration methods for degra- dation rate estimates suggest that the Table 3. Contaminant degradation rates estimated from model calibration of the Layton site data collected March 1993 Compound Calibrated Degradation Rate(1/d) Retardation Factor, R Benzene Toluene Ethylbenzene p-Xylene Naphthalene 0.00086 0.00062 0.00020 0.00037 0.00012 2.7 4.4 7.2 7.5 12.8 ------- simpler degradation rate approach can be used to provide representa- tive contaminant degradation rates when a plume has reached steady- state conditions. 6. The soil core data available from the Layton site were limited, and residual product volume estimates based on gasoline residual saturation values re- ported in the literature for silty clay soils were used to estimate the mass remaining in the Layton site source area. From these residual mass esti- mates, the lifetime of the total mass of BTEX and naphthalene at the Layton site, based on reaching their MCL values in the plume, ranged from approximately 30 years for toluene to over 1 00 years for ethylbenzene. With 100 percent source removal, the re- quired site management timeframe, based on the ethylbenzene MCL, was reduced to approximately 8 to 14 years. Under these site conditions, however, benzene becomes the con- taminant with the greatest duration of concern, requiring approximately 18 to 22 years to reach its MCL value of 5 7. The decision to apply only an intrin- sic remediation plume management approach at the Layton site should be made with caution. Despite apparent plume stabilization and the absence of an impacted downgradient recep- tor, the low contaminant degradation rates (approximately one order of magnitude lower than at the Hill AFB site), large residual masses of con- taminant within the source area and marginal potential aquifer assimilative capacity observed at the site will re- quire long-term monitoring and site management (>30 years). Active source removal and residual mass remediation are warranted at the Layton site to accelerate the rate of contaminant removal from the site, and shorten the length of time re- quired for plume management. Based on the findings in this study, the following recommendations can be made: 1. The combined CPT/ATH procedures used for initial plume delineation proved to be rapid and cost-effective, leading to a significantly improved un- derstanding of subsurface conditions at both of the field sites. This approach should be refined and evaluated for general application for site assess- ment activities at UST sites. 2. The intrinsic remediation protocol de- veloped in this study provides a logi- cal, quantitative approach for evalu- ating the presence and rates of con- taminant assimilation within an aqui- fer system. The protocol provides im- provements over conventional plume containment assessment methods. Plume centerline concentration analy- sis is used, along with plume mass and center of mass determinations, to incorporate the aerial aspects of plume containment that have not nor- mally been included in other field evaluations of intrinsic remediation processes. Its application should be evaluated for routine use at UST sites. 3. The modeling approach used to de- scribe intrinsic remediation processes occurring at the two UST field sites al- lowed the quantitative assessment of contaminant migration and degrada- tion using actual field data. The model was easy to implement in a spread- sheet environment and appeared to provide a quantitative description of contaminant plume profiles that were observed at the two distinctly differ- ent field sites evaluated in this study. The model provided independent veri- fication of plume steady-state condi- tions, and allowed the rapid assess- ment of the impact of various source removal options on the duration of contaminant plumes produced from hydrocarbon releases at these sites. Its application should be evaluated for routine use at UST sites. REFERENCES Chow, V.T, D.R. Maidment, and L.W. Mays. Applied Hydrology. New York: McGraw Hill Book Co., 1988. ------- R.Ryan Dupont, Darwin L. Sorensen, Marian Kemblowski, MarkBertleson, Dietrick McGinnis, Idris Kamil and Yang Ma are with Utah Water Research Laboratory, Utah State University, Logan, UT 84322-8200 Charlita Rosa/ ;'s the EPA Project Officer (see below). The complete report, entitled "Monitoring and Assessment of In-Situ Biocontainment of Petroleum Contaminated Ground-Water Plumes," (Order No. PB98-145329; Cost: $47.00, subject to change) will be available only from: National Technical Information Service 5285 Port Royal Road Springfield, VA22161 Telephone: 703-605-6000 The EPA Project Officer can be contacted at: Characterization Research Division National Risk Management Research Laboratory U.S. Environmental Protection Agency Las Vegas, NV 89193-3478 United States Environmental Protection Agency Center for Environmental Research Information Cincinnati, OH 45268 Official Business Penalty for Private Use $300 EPA/600/SR-98/020 BULK RATE POSTAGE & FEES PAID EPA PERMIT No. G-35 10 ------- |