vvEPA
          United States
          Environmental Protection
          Agency
            Waste Management Division
            Region 1 -(HER-CAN6)
            Boston, MA 02203-2211
EPA/SO -t^B-92-DD 1
May 1992
           Research Library for Solid Waste
Compendium of
Materials on Municipal
Solid Waste
          Defining Degradability
  Printed on Recycled Paper

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                     DEFINING DEGRADABILITY
                       TABLE OF CONTENTS:
Introduction 	 ......... 	
Standard General and Specialized Reference Sources .... 4
Solid Waste Reference Sources  ... 	 ... 5
Federal Sources  	 	 5
State Legislative Definitions  	 ... 7
Professional and Other Sources 	 8
EPA, Environmental Fact Sheet: The Facts
on Degradable Plastics 	
EPA, Report to Congress: Methods to Manage^and Control
Plastic Wastes, "Types of Degradable Plastics and
Degradation Processes," February, 1991  	  12
Degrabable .Plastic Ring Carriers, Title I  of Public
Law 100-556  [S.1986]; October 28, 1988	1'
                                                          20
International Sources	

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Introduction:

The term 'degradable' and its 'photodegradable'  and
'biodegradable' variants are widely used with varying degrees of
appropriateness, depending upon the source and the purpose.
Defining degradability is much more than a mere  academic
exercise.  The definition rendered or accepted has an impact on
the processes chosen to produce many consumer goods.   It has an
impact on advertising, marketing, industrial design or redesign,
and the management of wastes, as well as on choices that are made
by the ultimate end user of these products: the  consumer.
Consider that some 5,700 "green" consumer products, many bearing
claims of "degradability" or "biodegradability," were marketed in
1989 alone.  ("Why Biodegradable Claims May Not Mean Much," by
John F. Wasik, San Francisco Chronicle, Sept. 24, 1990).

Society will ultimately require some standard for evaluating
claims of degradability.  Thus, generic and open-ended
definitions will compete in the future, as they have in the past,
with those bearing a higher degree of specificity.  This
Compendium offers examples of definitions for the_term .
"degradable" and, in doing so, provides a brief history of
definitions which began in the 1970s.

In the 1970s, the very same debate that now exists concerning the
degradability of consumer goods Was taking place.  The issues at
that time were plastics and waste nuclear materials.  At least  in
the case of plastics, many of the same solutions were proposed,
researched,  and discussed, principally in a dialogue.among
packaging industries  and in  a second dialogue between some
industries and  some government agencies.  "It is  almost
inconceivable," wrote John H. Abrahams, Jr. of the Glass
Container Manufacturers Association, "that you can instill  in a
product  that costs only a few pennies to create,  the Intelligence
to perform 100  percent and then, at a given point, to
automatically disappear and  destroy itself."  (Utilization of
Packaging Wastes, in  Reuse and Recycle of Wastes:  Proceedings,
3rd New  England Regional Conference, University  of Rhode Island,
1970).

"Degradable  plastics can now be  produced," countered  an  unsigned
editor in  the periodical, Chemical Week,  "but until manufacturers
are convinced there  is  a market  for them, progress toward
commercialization will  continue  to be very  slow." ("Degradables
Are Still  Debatables,"  Chemical  Week,  December  12, 1973).

Twenty years later/ we  are  still searching for  effective waste
management options  for many substances within the municipal waste
 stream.   This Compendium is an attempt to make  people aware of
 the various definitions that are either currently in use or have,
 at one time, been accepted to define the term "degradable."

 Standard reference sources,  academic sources, and specialized
 solid waste reference sources are included,  as  are Federal

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nmervtaa.  ciy     Compena3.um **
        forces ana purposes.
                                     z-

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DEFINITIONS
  3

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Standard General and Specialized Reference Sources

     biodegradability:  The characteristic of a substance that
     can be broken down by microorganisms. (McGraw-Hill
     Dictionary of Scientific and Technical Terms, 4th ed^,
     1989).

     biodegradability:  The susceptibility of an organic material
     to decomposition as a result of attack by microorganisms.
     The term is applied especially to detergents and
     insecticides, which vary widely in this respect.  For
     ecological reasons, a high degree of biodegradation is
     desirable to minimize the adverse environmental effect of
     such materials.  Sewage is highly biodegradable, and present
     methods of treatment are based on this property.  Phosphate
     compounds and'chlorinated hydrocarbons such as DDT* are not
     biodegradable, and it is largely for this reason that their
     use is restricted.  Biodegradable plastic containers have
     been developed to ameliorate the solid waste problem.
     (Glossary of Chemical Terms by Clifford A. Hampel and G.  G.
     Hawley, Van Nostrand Reinhold, 1976.)

     biodegradability:  The susceptibility of a substance to
     decompose by microorganisms, specifically the rate at which
     detergents and pesticides and other compounds may be
     chemically broken down by bacteria and/or other natural
     environmental factors.  Branched chain alkylbenzene
     sulfonates are much more resistant to such decomposition
     than are linear alkylbenzene sulfonates in which the long
     straight alkyl chain is readily attacked by bacteria.  If
     the branching is at the end of a long alkyl chain
     (isoalkyls), the molecules are about as biodegradable as the
     normal alkyls.  The alcohol sulfate anionic detergents and
     most of the nonionic detergents are biodegradable.  Among
     pesticides the organo-phosphorous types while highly toxic
     are more biodegradable than DDT and its derivatives.  Tests
     on a number of compounds gave results as follows: Easily
     biddegraded: n-propanol, ethanol, benzoic acid,
     benzaldehyde, ethyl acetate.  Less easily biodegraded:
     ethylene glycol, isopropanol, o-cresol, diethylene glycol,
     pyridine, triethanolamine.  Resistant to biodegradation:
     aniline, methanol, monoethanolamine,. methyl ethyl ketone,
     acetone.  Additives that accelerate biodegradation of
     polyethylene, polystyrene and other plastics are available.
     (Hawley's Condensed Chemical Dictionary, Revised llth ed.,
     Van Nostrand Reinhold, 1987).
  DDT is the acronym for dichlorodiphenyltrichloroethane,

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     biodegradable:  Susceptible to being degraded by natural
     action, usually microbial, that usually leaves no harmful
     residue in the environment.  (international Dictionary of
     Medicine, Wiley, 1986.)


solid waste Reference Sources

     biodegradable:  Waste material which is capable of being
     broken down by bacteria into basic elements.  Most organic
     waste, such as food remains and paper, is biodegradable.
     (Handbook of Solid Waste Management, ed. by David G. Wilson,
     Van Nostrand Reinhold, 1977).

     biodegradable:  Any biodegradable substance is capable of
     being broken down by microorganisms such that its
     objectionable qualities, as waste, are eliminated.  Thus for
     example pesticidal properties of pesticides, taste and odor
     of chlorophenols, etc. would be lost.  A compound that
     undergoes only slight degradation in a reasonable period of
     time is not biodegradable.   (Solid Waste Management Study
     Report, Vol. 2, by Raytheon Service Co. for Department of
     Public Works, 'Commonwealth of Massachusetts, 1972).
Federal Sources

     biodegradation:  Degradation that occurs through the action
     of microorganisms such as bacteria, yeast, fungi, and algae.
     Debate continues regarding the most appropriate definitions
     for  [these] degradation processes as well as regarding the
     operational or performance standards for such processes.
     The  absence of accepted definitions has been cited as a
     factor impeding the development of degradable plastics.  The
     American Society for Testing and Materials (ASTM) has
     organized a committee to define terms for plastics
     degradation and to develop standards for testing and
     measuring "degradability. "   (Methods To Manage and Control
     Plastic Wastes: Report to Congress, EPA/53 O-SW-89-051,
     1990) .

     biodegradation of organic compounds:  Biodegradation, as a
     theoretical concept, refers to the process by which an
     organic compound is converted to carbon dioxide, water, and
     other inorganic constituents by the action of living
     organisms.  In practice, several qualifying terms are used
     to modify this concept.  .  .  The main consideration in
     biodegradability is whether or not an organism exists that
     can  break down, metabolize, or oxidize the parent compound,
     either on first exposure to  it or after a suitable
     acclimation period.  .  . In real world situations, the extent
     of degradation within  a fixed time limit  is a very important
     consideration in any working definition of biodegradability.
      (Biodegradation and Treatability of Specific Pollutants by

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Edwin F. Earth and Robert L. Bunch, Wastewater Research
Division, ORD, EPA.  EPA-600/9-79-i034,  October, 1979).

biodegradability:  Strictly speaking, biodegradable
materials are those whose chemical structures make them
susceptible to assimilation by microorganisms such as molds,
fungi, and bacteria when buried in the ground or otherwise
contacted with the organisms under conditions conducive to
their growth.  Some non-biodegradable plastics are
erroneously believed to be biodegradable because they often
contain biodegradable additives that will support the growth
of microorganisms without causing the plastic itself to
become assimilated.  The term 'biodegradable' is often used
indiscriminately to refer to various types of environmental
degradation, including photodegradation.  Because a
polymeric material is degraded by sunlight and oxygen does
not necessarily mean that the material will also be
assimilated by microorganisms.  The term 'biodegradable'
should be reserved for that type of degradability that is
brought about by living organisms, usually, microorganisms.
(An Investigation of the Bioaegradability of Packaging
Plastics, EPA-R2-72-046, 1972.)

biodegradation:  If the chemical compound was susceptible to
natural degradation, cessation of human use would result in
the disappearance of the newly recognized toxicant from
ecosystems.  By contrast, if the compound was
nonbipdegradable, its harmful effects would continue for
months, years, or decades, because of the absence of an
effective means to rapidly eliminate the offending chemical
from natural ecosystems.  (Degradation Mechanisms:
Controlling the Bioacoumulation of Hazardous Materials by
Charles J. Rogers and Robert E. Landreth, Solid and
Hazardous Waste Research Laboratory, ORD, EPA.  EPA-670/2-
75-005, January, 1975).

degradable:  The term 'degradable' means the ability of a
material to be reduced to environmentally benign subunits
within  the shortest period  of time consistent with the
material's intended use but in no event greater than a
period  of 5 years.   (A Bill To Encourage the Development and
Use of  Recyclable Consumer  Plastics... 101st Congress,  1st
Session, House of Representatives.)

photodegradation and biodegradation:  See Attachments:
 (Environmental Fact Sheet:  The Facts On Degradable Plastics
from  EPA's Report To Congress On Methods To Manage and
Control Plastic Wastes, by  OSWER,  EPA/530-SW-90-017D,
February, 1990.)

photodegradation,  biodegradation,  and other  degradation
processes:   See Attachments:  (Report To Congress: Methods  To
Manage  and  Control Plastic  Wastes, by OSWER, EPA/53O-SW-89-
051,  February, 1990.) pp. 5-76 to  5-80.

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State Legislative Definitions

     biodegradable:  A material has the proven capability to
     decompose in the most common environment where the material
     is disposed within one year through natural biological
     processes into nontoxic carbonaceous soil, water, or carbon
     dioxide. (Deering's California Codes Annotated, 1990 Cal AB
     3994, Section 17508.5).

     biodegradable material:  Material which is capable of being
     broken down by bacteria into basic elements. (Vermont
     Statutes Annotated, 1989 Supplement, 10 VSA, 1521.)

     biodegradable:  Degradable through a process by which fungi
     or bacteria secrete enzymes to convert a complex molecular
     structure to simple gasses and organic compounds.  (Michie's
     South Dakota Codified Laws, Chapter 34A-7, Litter Disposal
     and Control, 1989).

     biodegradation:  As used in this section,  'biodegradation'
     means the conversion of all constituents of: (1) A plastic;
     or  (2) A hybrid material containing plastic as a major
     component, into miscellaneous component parts by the
     microbial action of fungi and bacteria upon natural
     materials such as  cornstarch.   (Michie's Burns Indxana
     Statutes Annotated, Title 4, Article 13.4  State Procurement,
     Chapter 4 Specifications: 4-13, 4-4-6, Degradable  plastic
     products.)

     biodegradation:  When used  in connection with  recycling,
     means the conversion of all constituents  of a  plastic or
     hybrid material containing plastic  as a_major  component to
     carbon dioxide, inorganic salts, microbial cellular
     components and miscellaneous by-products  characteristically
     formed from the breakdown of natural materials such  as corn
     starch.   (Illinois Revised  Statutes, Chapter 111  1/2,
     Environmental Protection Act, 111.  Rev. Stat., ch.  Ill 1/2,
     par 1003.68,  1988).

     biodegradable or photodegradable material: Means material
     which  is capable of being broken down by  bacteria or light.
      (Michie's Delaware Code Annotated,  Title  7 Conservation,
     Part VII, Chapter  60,  Subchapter III, Beverage Containers).

     degradable:   Degradable means capable of  being broken down
     by biodegradation, photodegradation, or chemical degradation
      into component  parts  within 360 days under exposure to the
     elements.   (Michigan  Compiled Laws,  1989,  Chapter 299,
     Labeling of Plastic Products,  299.481,  1989).

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     degradable:   Degradable means capable of decomposing by
     biodegradation,  photodegradation,  or chemical process into
     harmless component parts after exposure to natural elements
     for not more than three hundred sixty-five days.   (Code of
     Iowa 1989, Title XVII,  Chapter 455B, Division IV  Solid Waste
     Disposal, Part 1.)


Professional and other Sources

     biodegradation:   Biodegradation is a process wherein micro-
     organisms secrete enzymes to chemically break down material
     that they then eat.  This can be in the presence  of oxygen
     (e.g. composting) or in the absence of oxygen (e.g. in a
     landfill).  In either case, there must be moisture present
     and other conditions.must be met.    (Degradable Plastics: .
     Myth or Miracle? by Keep America Beautiful, Inc., Focus:
     Facts On Municipal Solid Waste, No. 2, March, 1990.)

     biodegradable:  Any substance that decomposes quickly
     through the action of microorganisms.  (Ha2ardous Materials,
     Hazardous Waste:  Local Management Options, International
     City Managers Assn., 1987.)

     biodegradable materials:  Waste material which is capable of
     being broken down by microorganisms into simple,  stable_
     compounds such as carbon dioxide and water.  Most organic
     wastes, such as food remains and paper, are biodegradable.
     (Garbage Solutions: A Public Official's Guide to Recycling
     and Alternative Solid Waste Management Technologies, by
     National Resource Recovery Association and the U.S.
     Conference of Mayors, 1989).

     biodegradation:  There is no agreed scientific definition of
     biodegradation—nor any standard laboratory test for
     biodegradability of solids.   ("Biodegradation in Landfills,"
     Health  & Environment Digest, by the Freshwater Foundation,
     Vol. 3,  #9, November, 1989).

     biodegradable:  An organic compound that can be degraded or
     converted to simpler compounds by microorganisms in the
     natural environment.   (Recycling In the Marketplace, by
     Camp, Dresser & McKee, Inc.,  1985).

     biodegradable:   Few people would regard a compound that
     undergoes only  slight degradation as biodegradable.  An
     intermediate position is occupied by the concept of
     'activity'  loss.  This means  that if the specific activity
     that renders the compound  objectionable is  lost through
     microbial degradation, the compound would be considered
     biodegradable.   (Determination of Biodegradability Using
     Warburg Respirometric Techniques, by J. V.  Hunter  and  H.
     Heukelekian in  Purdue University Proceedings of the  19th
     Industrial  Wastes Conference,  1964, part  2.)

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ENVIRONMENTAL FACT SHEET: THE FACTS ON DEGRADABLE PLASTICS
                      February, 1990
        FROM: U.S. ENVIRONMENTAL PROTECTION AGENCY
                   Office of Solid Waste
                     Washington, D.C.

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            Untied States
            Environmental Protecs ion
 Solid Waste and
 Emergency Response
 (OS-305)
EPJVS30-SW-90O17D
February 1990
            Office ol Sofid Waste
            Environmental
            Fact  Sheet
            THE FACTS ON DEGRADABLE
            PLASTICS

            FROM ERA'S REPORT TO CONGRESS ON
            METHODS TO MANAGE AND CONTROL
            PLASTIC WASTES
      Discorded plastic products and packaging make up a
   growing proportion of municipal solid waste. By the year 2000,
   the amount of plastic we throw away will increase by 50 percent
  ""Current volume estimates Jor plastic waste range from 14 to 21
   percent qfthe waste stream. By weight plastics contribute seven
   ^percent, and less than one percent qf plastic waste is currently
   recycled. Additionally, some plastic items end up as litter thai
   poses ecological risk to the marine environment  and aesthetic
   and economic loss. These facts have led to the exploration qf
   degradable plastics as one possible solution.
Degradabfe Plastics Defined
Degradable plastics are engineered to be less resistant to degradation
than "normal" plastic. The following are currently the most prominent
technologies being Investigated for consumer products and packaging:

     Photodegradation adds a sun-sensltlve component that
     triggers physical disintegration when exposed to sunlight

     Biodegradation adds a natural polymer such as corn starch or
     vegetable oil that degrades into smaller pieces of plastic when
     exposed to the appropriate environment.
                             \
o

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Do Degradables Fit Into Solid Waste Solutions?

      Reduction oj Waste:
      but the amount of waste produced is the same.
                Plastic rwyders fear that degradable plastics ; will

                  ^^^^
      how de^adable plastic bags work, however, they may prove
      useful in collecting and composting yard waste.



      ^degradation begins.













  Som'e^Oa^rS 7:30 p.m.ESTT. Monday «bn^mby. Ask the
  Hotline for informatioii on ordering the full report.
                                              Original Printing on Roeyctod Paper
                                      \\

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REPORT TO CONGRESS: METHODS TO MANAGE AND CONTROL PLASTIC WASTES
                         February, 1990


           FROM: U.S. ENVIRONMENTAL PROTECTION AGENCY
  Office of Solid Waste/Office of  Marine  & Estuarine  Protection
                        Washington, D.C.

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  Degradable products are not included in the integrated waste management system EPA
  prepared for MpoUcy, proposals in its 'Agenda for Action,' and thus do not have a defined
  role in current EPA pobc.es.  Further, degradable plastic products introduce a new range of
  environmental issues and their influence on current waste management concerns remains largely
  undefined.  These uncertainties are described in the sections below.


     5.5.1  Scope of the Analysis

  This section summarizes available information about the current and potential development of
  degradable plastics aod examines possible approaches to increasing the use of such materials
  All types of degradable plastics intended for use in plastic product markets are considered here
  Issues covered include types of degradation processes and the environmental implications of this
  waste management technique.


     5.5.2  Types  of Degradable Plastics aod Degradation Processes

  Six methods of enhancing or achieving degradation of plastic have been defined in the literature
  and are described bekw. The most important technologies, based on available data and
  apparent market potential, are pfaotodegradation, biodegradation, and biodeterioration.

    Photodegradation - Degradation caused through the action of sunlight .on the polymer

    Biodegradation - Degradation that occurs through the action of microorganismraucb as
    bacteria, yeast, fungi, and algae                                                       -

    Biodeterioration - Degradation that occurs through the action of-macrooreaiusms such AS
    beetles, slugs, etc,

    Autooxidation - Degradation caused by chemical reactions with oxygen

    Hydrolysis - Degradation that occurs when water cleaves the backbone of a porymer,
    resulting in a decrease in molecular weight and  a loss of physical properties

    Solubilization - Dissolution of polymers that occurs when a water-soluble link is included  in
    the polymer [Note:  soluble polymers remain in  polymeric form and do not actually
    "degrade." They are included here because they are sometimes mentioned in the literature
    on degradable plastics,]

Debate continues regarding the most appropriate definitions for these degradation processes as
well as regarding  the operation a! or performance standards for such processes. The absence of
accepted definitions has been cited .as a factor impeding the  development of degradable plastics
(U.S. GAO, 1988).  The American Society for Testing and Materials (ASTM) has organized  a
committee to define terms for plastics degradation and to develop standards for testing and
measuring 'degradability."

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        pane

                                     to
   Photo- arxf biodegradation are discussed in detail below, but a general comment about the
   processes can be made here.  Fir* the rate of degradation of plastic mS L the
   environment is a function of both the characteristics of the plastic product and the
   r^rTL?0^0115 fa ^ il b pUced- ^ »dditi°D of characteristics that increase
   photodegradabOity, for example, is an effective waste management step only if the product is
   expo ed  to sunlight  Thus, degradable plastics must be matched with an eventual

           °r Wlh ^                                                               to be
     the subsecuons below, more information is provided about the mechanisms involved for the
         JJ.h^T ?rOCeSSeS ^ ^ C0fflmercial »«^t>« that are being purged
  summary of  he degradation processes that have been introduced by manufacturers
  not nec«sanly commercially exploited) for plastic polymers is showi


     5.5.2.1   Photodejradstlon
 Sunlight is the dominant source of the ultraviolet radiation that will produce -photodeeradation
 bd^r bghtm« generaUy.will not produce photodegradation both be^use^dow^f^em'
 out most uluralet radiauon from sunlight and because other indoor light lounaita^
 Dh±CCerHCbK,Ultrr°Iet^diati0n'  ^^ P»»«^««»«tk)n is primarily an^door process
 photodegradable plasnc products used primarily indoors can therefore be given "controlled
                     productt are dtarded outdoors - K utter for
 To enhance the photodegradation properties of a plastic, manufacturers have modified or
 developed new polymen that contain photosensitive substances in the polymer chain.
                       ""       ^          t 8re Photo$ensjtive •«> ««se degradation of
                    THE.PLA.STJC POLYMER - Photodegradation may be accomplished by
incorporating a photosensitive link in the polymer chain.  The principal method used thus far
has been the incorporation of carbon monoxide molecules, also referred to as carbonyl groups,


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   into the Polymers.  If carbonyl groups absorb sufficient ultraviolet radiation they under™ *
   "rr^^^^
  The rate of photodegradation depends oo the number of carbonyl groups added

           to .Bow subsequent biodegradation of tower-weight chemical molecules  For Stance
             molecute n,ay have molecular weights of 20.000 or higher  WotS
  reduces this .eight, but for bWegradation of the polymer to occur « significant

                   ™ ^-"""^ » WO"*"'* »° <*>«*• »M « Sceo
                                                                                  been

              have developed potentially biodegradable products either by 'modifying the
              """    «lected *dditiv«-  1° the latter case, the plaitic polyTer  eft
                             additive Temaim intact altbou|h * may no
PLT1C fOLVMER - Most P3astic
                  ^ "
 commodity

«-
                                                             « «*
     ,  h        v             hOWCver' includin« se'e«ed polyesters and polyurethanes.
These  biodegradable resms were developed for low.volume specialty uses fbrwtieh
biodegradabOtty u desirable, such ai some agricultural applications (e.g., seedling pots for
automata reforestation machines).  Some of these end products for bJodegrad

                                         thdr
As of a 1957 symposium on degradable plastics sponsored by SPI, biodegradable resins
appropriate for use in packaging had not been developed (Johnson, 1987).  One type of "
aliphatic Polyester, polyester poly(3 hydroxyburyrate-3 hydroxyvalerate), or PHBV ha been
developed by Id Americas in England. It is biodegradable ind reputed to have ctaraSeA tics
                                           \

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.       The degradation
•ddition of the starch.  Starch
10% relative to the xt^
to 60% of product volume.
manufacturer. St. Lawrence S^rch, hai
by microorganisms and the autooddant
      help degrade the
           field
                                              P°plil!Li0n °f
                                              BOt been enhanced
                                                    « » «»«. U, « 5 to
                                                         S! fa tm°unts U
                                       hu              • One polymer
                                       bu7l.tbe«arcb «dditive  is consumed
                                            A?* ^ to f°m P6"8*1*



                                                                       '
Other Degradation Processes

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   Degrabable Plastic Ring Carriers
Title I of Public Law 100-556  [8.1986]

           October 28,  1988
                \V

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1
              PUBLIC LAW 100-556 [S. 1986); October 28,1988


            DEGRADABLE PLASTIC RING CARRIERS; SAN
                     FRANCISCO BAY NATIONAL
                         WILDLIFE REFUGE

                  For Legislative History of Act, see p. 3632.

      A* Act »• r*4«> pUstk ring tmrrimt 4*virai fc* Jigradrtli, mnt If »Mi«r fuffttt.
                                                                                               : \
        Be it enacted by the Senate and House of Representatives of the
      United States of America in Congress assembled,


        TITLE I—DEGRADABLE PLASTIC RING

                            CARRIERS

      SEC. 101. FINDINGS.
        The Congress finds that—
            (1)  plastic ring carrier  devices  have been found in large
          quantities in the marine environment;
            (2) Ash and wildlife  have been known to have become entan-
          gled in plastic ring carriers;
            (3)  nondegradable plastic  ring  carrier devices can remain
          intact, in the marine environment for decades, posing a threat to
          fish and wildlife; and
            (4)  16 States have enacted laws requiring that plastic ring
          carrier devices be made from degradable material in order to
          reduce litter and to protect fish and wildlife.

      SEC. 102. DEFINITIONS.
        As used in this title—
            (1) the term "regulated item" means any plastic ring carrier
          device that contains at least one hole greater than PA inches in
          diameter which is made, used, or designed  for the purpose of
          packaging, transporting, or carrying  multipackaged  cans or
          bottles, and which is  of a  size, shape,  design, or  type capable,
          when discarded, of becoming entangled with fish or wildlife; and
            (2}the term.^naturally degradable material" means a mate-
          rial .which, when discarded, will be reduced to environmentally
          benign  subunits-under  the action of normal-environmental
          forces,-such as, among others, biological decomposition, photo-'
          degradation, «r hydrolysis*?

      SEC. 103. REGULATION.
        Not later than 24 months  after the date  of the enactment of this
      title 
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  ^
  it
  Hi
   v'i
i% •*..
                  P.L. 100-556
                                              LAWS OF 100th CONG.—2nd SESS.
                                                                                      Oct. 28
                  Public
                  information,
                 Fish and fishing
                 16USC666dd
                 note
                 16USC66bdd
                 note
 of the item and the physical integrity required for such use. Such
 regulation shall allow a reasonable time for affected parties to com2
 into compliance, including the use of existing inventories.


                    R3AN>RANCISCO BAY
         NATIONAL WILDLIFE REFUGE

 SEC 2^. ENLARGEMENT OF REFUGE.

  Secti?\2 ?fthe Act entitled "An Act to pro/de for the establish-
 ?ent ?^dS>an Francisco Bay National Wjldfift Refuge", approved
 June 30,1$U <16 U.S.C. 668dd note), is arn^ded to read ksYiUoS
   'SEC. 2.  TVre shall be included  with/i the boundaries of the
 refuge the following:                 7
      "(1) Thosklands. marshes, tidal/flats, salt ponds, submerged
    lands,  and open waters  in the s/uth San Francisco Bay area
    generally depi&ied on the map/entitled  'Boundary Map Pro-
    pos,d San Francisco Bay National Wildlife Refuge*, dated July
    1971, and which comprise approximately twenty-one thousand
    six hundred and si*ty-two acres within four distinct units to be
    known as Fremont \fiveythousand five hundred  and twenty
    acres),  Mowry  SloughVs/ven thousand one hundred and sev-
    enty-five acresl, AlvisoYthree thousand and eighty acres), and
    Greco Island (five thods^snd eight hundred and eighty seven
    acres).  Said boundar^ ma)s  shall be on file and available for
    public  inspection it/the  offices of the  United States Fish and
    W ildlife Service, Department V the Interior.
      "(2) Up to 20,000 acres in theVicinity of the areas  described in
    paragraph (1). sfrid similar to th\ areas described in paragraph
    (1). which theJBecretary determined are necessary to protect fish
    and wildlife resources.".

SRC. 202. TOTAL/REA OF REFUGE.
  Subsection/a) of section 3  of such Act is\amended in the second
sen^nJ?e  b>/strik»ng  "twenty-three thousan\acres" and  inserting
"43,000 acnes .                            x

SEC. 20.1. AUTHORIZATION OF APPROPRIATIONS.
         5 of such Act is amended—
      

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    INTERNATIONAL SOURCES
    
    See Attached letters to the Research Library for Solid Waste, EPA
    Region 1 from:
    
    Asociacion Tecnica Para La Gestion De Residuous Solidos, Spain.
    
    General Secretariat, The International Solid Wastes and Public
    Cleansing Association, Copenhagen Office, Denmark.
    
    Polish Association of Sanitary Engineers and Technicians, Poland.
    
    The Swedish Association of Solid Waste Management, Sweden.
    
    Istituto Di Ingegneria Sanitaria, Politecnico Di Milano, Italy.
    
    
    [NOTE: ATTACHMENTS FOLLOW]
    

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                              ASOOACION TECNIC'A PARA LA GESTION
                              DE RESIDUOS SOLIDOS
    MIEMBRO NACIONAI DE ISWA
     MIEMBRO DE: CLEAN WORLD
             AGHTM
             ISWM
             APWA
                            RESEARCH LIBRARY FOR SOLID WASTE
                            U.S. ENVIRONMENTAL PROTECTION AGENCY
                            Region 1
                            HEE-CAN 6
                            J&hn F. Kennedy Federal Building
                            Boston, MA 02203 USA           -J
            \
     fi
     I
     ' X.
                                         11th. JTuly 1990
                   Dear Mr.  Friedman,
      I make reference to your  letter of the 23rd. May
    
    
      For me the term "biodegradable" means  something •
    that  can be destroyed bioligically  .
    
      Yours sincerely,
                                        A T t G R U S
                                         SECRETARY GENERAL
                                      6»pr«MnU.n» Cfkanol en fe 1SWA
                   P.S.  Please note our new address
    

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                  page
                   THE INTERNATIONAL SOLID WASTES AND PUBLIC  CLEANSING ASSOCIATION.
    
                                                             Gentr»t Secretariat
    
                                                             Jeanne Mailer
                                                             fctpenoerhuset
                                                             V. F«tim»8sgi8« 29
                                                             DK1606 Copenhagen V
                                                             Denmark
                                                             Ittepnone +4S33156S65
                                                             !•*•)*«. *4S33937171
                                                       15 June,  1990
                                                                JM/SM
     Fred T. Friedman
     Research Librarian
     United States Environmental  Protection Agency
     J.F. Kennedy Federal  Building
     Boston, Massachusetts 02203-2211
    
     Dear Mr. Friedman:
    
     We  have  asked  three  of  our engineers to  provide  us with a
     term for "biodegradable"  and  the following  is  their  exact
     definition.
    
     CHARACTERIZATION OF BIODEGRADABLE ORGANIC MATTER:
     Organic matter may  serve as  an energy and carbon source in a
     fciologijeal -system.    In environmental  engineering microbial
     ibiodegradstion is of special Interest.
    
     A  main 'Characteristic for  biodegradable organic  matter is
     the rol-e -of  biodegradation  relative  to the length of time
     biodegradation Is  considered,  ie.  residence time,  tr,  In a
     system.
               Biomass (relative)
    
                                                     theoretical limit
                                                     for non-biodeg-
                                                     radable organic
                                                     matter
                                                     tioe
     If change in  the  biomass IB  approximately  zero  during the
     residence  tine  in  question,   the  organic  matter  may  be
     regarded as  non-biodegradable.
    Pietaena      Woe Presioent
    
    HaioenDuU    JohnH Stunner
    Frans Has-aa- 3  CWic* oJ Resea.tr> ant! Development
    N' -6601 EE Soi  US Enwonmenial Proieciioo Agency
    Tne Ne?*-.2->35  401 MS«ee: Sw
    fasiPiesrfleni
    
    Jean Deleche
    Tranement HiSusif*!
    ees Resia js Urba.ns
    13t. OOJWvwO Ma ussmann
    Treasjte'
    RobenG Ferjuson
    439 Uni««rsit> Avenue
    Toronic. Ona-io V 66 1VE
    Washington Sub-Secretariat
    
    WitiiamS. Forester
    SWA
    Suite 401
    

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                     THE INTERNATIONAL SOLID WASTES AND PUBLIC  CLEANSING  ASSOCIATION.
                                                                          Je»nne Mallet
                                                                          Inoenoerhusei
                                                                          V F»rim»9sg»0e 29
                                                                          DK-1606 Copenhagen V
                                                                          •telephone *«533 166565
                                                                          ltle)a« *453393717t
                                                                        Page 2
    It   Is   important  that   the   same   organic  natter  may  be
    considered biodegradable  if (tr)  Increases.
    
    Yours sincerely,
    for  Jeanne M011er
    General "Secretary
                         U
     Susan McCarty
    Pies-oem
    
    Ha-oe-Dj--
    Fire, na'aiaa- 3
    NL 569! EE SOT
    1r»e Netnenznos
              O«ice o' Resea-cr. »no Deveiop-ne-n
              US Emmonme-.u1 Pioftoion Agency
              401 M Swet: Sw
              Vrtsr>ingior> D C. 20460
              USA
                                      R»si Presocii
                                      Jet-.
    ties Besifl js Urt>a>ns
    13*. bojieva'0 Majssmann
    F-76366RifisCeoe«08
    Fiance
                     Treasufe1
                     fiooen G v. '
                     Mei'OS" •»' '
                     439 u-' ••••
                             •A»«nue
    W.II.ZT.S Fo-esie-
    ISWA
    Sune 101
    1301 Pennsylvania Avenue. N\v
    Vkashmjion. D.C. 20004
    USA
    

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    /I
    ,'£
                                TTTUTET-
                 65-246 Zieloni G6ra, ul. Podg6rnB 50; skr. poczt. 47. Telefony: centrals 48-31 (fa.czy wszystkie n-ry
                 wewn.). Rektor 707-35; Prorektor d/s Nauki 703-82; Prorektor d/J Nauczania i Wychowania 722-06;
                 Dyrektor Adm. 39-44. Telex 043-22-15. Konto bank. NBP It O.M. Zielona G6ra nr 87026-521-189-31.
              PDiJiK
    
              Was? */»Ar
           Subject:  term:
           11 bi o a e grad£.bl ef'
                                     */»* .....
                                                        Zielona G6r».
                                   Research Library for Solid Waste
                                   U.S.  Environmental Protection Agency
                                   Region 1
                                   HES-CAN6
                                   John  P. Kennedy Federal Building
    
                                   Boston, £>A 02203, USA
                                   Attn.:  l-!r Pred 5f. Priedroan,
                                           Research Librarian
           Dear ir.r Priednian:
    
          Authorized by the Secretary General of the  Polish Association  of
           Sanitary " Engineers and Technicians iur Eysaard Parusz-ewski, 3. would
           £nsv.-er your letter of 23 i«ay 1990.
           You asked about the definition of the term ""biodegradable',.
           ans\ver  cannot be a unique  one, and should  be xather ..^Lescrisiive
           in some fe\v words only. I  looked through different BotcrcEst-.?end
           the results:
    
           I/ Oxford Advanced Learner's Dictionary  of Current English, by A.S.
              Hornby. Oxford University Press 1974.
              Biodegradable: (of substance)  that can be  broken down toy .bacteria.
           2/ Glossary on Solid V/aste,  by P.K.Patrick.  WHO Regional Office  for
              Europe, Copenhagen 1980.
              Biodegradable: Capable  of being broken  dorm physically and/or
              chemically by the action  of microorganisms.
           3/ Handbook of Industrial  »Vaste Disposal,  by ?...A.Conway, and li.D.
              ROES,  VaT; 3?c strand Eeinhold Kevj York  1980.
              Sorie techniques of . experimental determination of biodegradability
              v.lth references (3-1, 3-2,  3-3 P«143j are described in the  book.
    
           4/  Conpost Engineering, by Roger f.Haug. ^nn Arbor Science  Publisher
              Ann .r.rbor I960, pp.248.
              Haug introduced the  degradability coefficients, but he does no't
               give a definition for  "biodegradable" substances.
           5/  Jroastawy Ochrony Srodov;isl:a  (pundanentals of Environment1 Protect-
               ion - in i-olich), by B.Giovriak, il.S.Kempa,  and '1.,/innicki.  PWiv
    

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       Science Publishers Warsaw 1985,  pp. 45 and 59:                  _:
       Biodegradable substances: organic matter which  can be degraded by
       the action of microorganisms under natural, aerobic conditions in a
       quantity of 50j£ of the input during 48 hours.
       Remarks: Natural conditions means2 in soil, in  water, in wastewater|
       The contrary of biodegradable is: refractory or resistive.
    
    6/ Gospodarka odpadami miejskizai (Management of Uunicipal Refuse - in
       Polish), by Edward S. Kempa. AHKADY Publishing House, \Varsaw 1983,
       pp.88-89.
       For biodegradable substances I used the contractual term "FOS" -
       fermentable organic substance, which is a part  of YDS. In our stu-
       dies on the composition of municipal refuse from various Polish
       towns and cities, the FOS varied from 0.38 to 0.50 (with a weightec
       aver. 0.43-0.45) of YDS. In the analytical procedure it is assxir,ed,|
       that TOG makes O.47 FOS. The analytical procedure is described in:
       Er.Yi'AG-ISV/A fsdit. 2. Grabnerj: Methoden zur Untersuchung von .Kbfa
       stoffen (in"*German). Duebendorf 1977. Procedure K-3028.
    
    Could you please let me know whether you are satisfied with ssy informs
    tions. Should you have further questions, please do not hesitate to g(
    in contact with me.
                                           Yours sincerely,
                                       Dr.  Edward  S. Kempa,
                                        Professor  in Environmental
                                              Engineering.
    _cc._;  Kr Ryszard Paruszewski
    "Secretary General
          c/o Polskie Zrzeszenie Inzyniero\v
              i Technikow Sanitamych
    
              Czackiego 3/5
              00-950 Warszawa
    

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                 SVENSKA  RENHALLNINGSVERKS-FORENINGEN
            United  States Environmental
            Protection Affencrg	
          X^Att. Fred T. Friedman _^
            Region  i
            J.F.Kennedy Federal Bulldnlng
            Boston
            Massachusetts
            USA
                                          KHCHIVEL
                                                  1 S  90
            Malmoe, Sweden  1990-08-03
            Dear collegue,
    
            By request 1 will send you following definition of the term
            "biodegradable".
    
            Biological material which is possible to break down in a unaffected
            process.
    Please Jet a
            Best regards
    
            Yours^sincerely
                                   .are: totally wrong In our Interpreting
    Svenska
    Cstergat
    21122KWLM6
                          Na: 040-104045
                          Int. «46-4 0-104 045
                                       O40-97 10 64
    4724169-0
    
    BAntiarTo/B
    
    «5-9877
    Organtuientnumm*':
    
    SS6260-SSS3
    

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                            JJ1
                  VIA f«ATEJ.lJ GOKL1NI, I • 20JJ1 MILANO (ITALIAJ
                  TEL. t02»4S20J54-432054» . TELEX: 5JJ467 POLIMI- 1
     ILDIRETTORE
     MILANO
               "the 39   of October 1990
               . UP.
             NS. UF.
                   VIII.32
    •Mr. Fred FRIEDMAN - (Research Librarian)1
     Reserch Library for Solid Waste
     U. S. Environmental Protection Agency
     Region 1
     HEE - CAN 6
     John F. .Kennedy Federal Building
    [Boston, MA 02203 U.S.A.                 _J
                  Dear  Mr.  Friedman,
      with reference to  Year  letter of the 23   of Kay 1990, I have at present
      the opportunity  to supply you with a definition of the tens "biodegrada-
      ble".
    
                 Hoping  that  such definition will be useful to You for Your
      project, I send  my best wishes and regards.
                                                             ours sincerely
                                                                   onomo)
    own? . i.ooo . a.ee -
    

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                Biodegradability  is  a  general  term  usually  indicating  the
    aptitude of a substance to undergo a degradation process operated  by  living
    organisms,  that  is, a  degradation resulting  from  bacterial animal  and
    vegetable metabolism.
                He could practically define "biodegradable " as the aptitude  of
    a soluble organic compound to undergo a microbiological degradation,  mostly
    due  to bacteria. However, from a quantitative point of view, this is not  a
    specific  definition, as it doesen't reveal anything  about  the  reaction's
    npe«d and the destination of tKe reaction product*.
                The  "complete  biodegradability"  o  "mineralisation"  is  the
    transformation   (conversion)  of  complex  organic  compounds  into  final
    inorganic products such as COa,'HaO and mineral aalts, through the metabolic
    processes related to the growth of microorganisms.
                The    "functional    biodegradability"   is    the    microbial
    transformation (conversion) of a substance into intermediate products, whose
    characteristics differ from those of the original products.
                The intermediate products are generally less toxic (this process
    could be defined as "detoxification"), or in some rare cases, more toxic.
                On  the contrary, the term of "bior«moval" is intended  to mean
    the  removal  of  a substance from a solution, a suspension  or  an  aerosol
    state,   resulting  from  a  combined  or  "borrowed"  action  of  physical,
    chemical  or  biological  .feature (e.g.  the  bioflocculation  supported  or
    activated by microorganisms).
                The  quantitative  measure  is equivalent to the  time  of half
    conversion, ^t»0; t 1/2), which is needed in order to obtain the falling  off
    x>f  Suilf  x>f  the original product. On the base of  this  parameter  it   was
             :to adraw «ome biodegradability scales as the following one:
                        for  the  quantification of biodegradability
               Denomination
    t 1/2 (year)
                Biodegradable
    
                Moderately biodegradable
    
                Persistent
    
                Permanent
     0,01
    
     0,1
    
     > a
    
     > i
    0,1
    
    0,8
    

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