EPA
600/
1985.1
                      INTEGRATED AIR CANCER PROJECT
                              INTERIM REPORT
                             September 25, 1985
                   U.S. Environmental Protection Agency
                   Research Triangle Park, N.C.  27711

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                                Table of  Contents
   I.  Executive Summary

  II.  Background and Rational

 III.  Goals of the Project
       A.
       B.
Long Range
Short Range
  IV.  Management

       A.  Approach
       B.  Management Plan
       C.  Budgeting
       D.  Peer Review and Advisory  Process

   V.  Technical Approach

       A.  Integrated Field  Study
       B.  Sampling
       C.  Source Apportionment
       D.  Bioassay Directed  Fractionation
       E.  Chemical/Analytical Measurements
       F.  Atmospheric Transformation
       G.  Human Exposure

  VI.  Project Status

       A.  RTP Measurements
       B.  RTP Measurements  - Resolving  Technical  Issues
       C.  Albuquerque Field  Measurements
       0.  Special Studies

 VII.  Technical Results

VIII.  Appendix

       A.  Potential  IACP Publications by Task
       B.  Technical  Protocols and Results by Task
       C.  Peer Review Participants  and  Comments

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I.   Executive Summary


         The  Integrated  Air Cancer  Project  (IACP)  is  planned  to  be  a closely


    coordinated interdisciplinary research  program to develop the scientific


    methods and data bases  for  identifying  the  major  sources  of  carcinogenic


    chemicals emitted into  the  air  and/or arising  from atmospheric  transforma-


    tion of chemicals emitted  into  the  air.   This  research  program  will  also


    be designed to  improve  the  methodology  and  data base  for  assessing  human


    exposure  and risk to airborne carcinogens.


         These objectives will  be achieved  in a stepwise  manner  by  conducting


    field studies in areas  of  increasing complexity.   Initially, airsheds


    with one  or two emission sources  will be  examined.  The first efforts
                                            *.

    will  focus on emissions from  wood combustion for  residential heating


    and from  mobile sources.


         Realization of  the Integrated  Air  Cancer  Project's goals requires  the


    combined  expertise of the  four  ORD  Laboratories located at RTP, NC.


    The project participants1  knowledge includes source description, characteri-


    zation and control;  source  measurement  and  analysis of  pollutants;  atmos-


    pheric transformation;  ambient  pollutant  measurement  and  analysis;  receptor


    and dispersion  modeling; exposure assessment;  and quantification of the


    mutagenic/carcinogenic  activity of  pollutants.  All of  these activities


    must include well  defined  QA/QC procedures  and  documentation.   And  finally,


    there must be a smoothly functioning interlab/intralab  management structure,


         In the final analysis, the results of  this project will identify the


    principal airborne carcinogens  and  their  sources  and  will  assess


    the human cancer risk they  pose.  Through the  combined  mechanisms of


    detailed  chemical/physical/biological analysis  of ambient air pollution

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 samples,  dispersion  models,  receptor models, atmospheric transformation
 models, and detailed knowledge  of  sources and  their emissions, it will be
 possible  to trace  these  airborne carcinogens back to their source.
 Effectiveness  of control  strategies for  reducing the emission of these
 airborne  carcinogens or  their precursors will  then make realistic cost
 benefit analyses possible.
      The  long  range  goals of this  project will require many years to attain.
 Approaching the  long term goals through  field  tests of relatively isolated -
 single source  categories, in a  stepwise  fashion, will yield the methodology
 to  understand  the  more typical  complex multiple source category environment
 experienced by the general population.
     Current data indicates that residential wood combustion and
 motor vehicles contribute substantially  to the mutagenic activity found
 in  ambient  air samples.  Therefore, Phase 1 (FY'85/'86), the first field
 test  series described in this document,  was aimed at developing and
•testing methodology  quantifying mutagenic and chemical  carcinogens emitted
 from  residential wood-fired  combustion systems and motor vehicles.  These
 areas of  investigation are outlined in Figure  1.   Two residential  communities
 were  selected to initiate Phase 1 of the IACP.  Albuquerque, NM was one
 site  selected due  to evidence from previous studies which showed the
 wintertime  particulate loadings were heavily impacted by wood smoke and
 vehicle emissions.    Raleigh, NC was selected as the second site in order to
 make  optimum use of  EPA personnel  located at the RTP, NC facility for
 methods development and evaluation studies.  The methods development
 studies were conducted to resolve specific sampling analysis uncertainties
 so  that standardized methods would be  available for subsequent field studies.

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Special  studies at RTP were conducted to provide data on wood stove

emissions under control conditions and to assess the role of atmospheric

transformation in altering mutagenicity of emitted chemicals.

     A summary of the interim accomplishments are listed below:
     1.' State of the art sampling and analysis procedures have been
         developed and implemented.  They are being evaluated and
         standardized for use in FY'86/'87 studies.
     2.  Sampling procedures for human exposure have been developed
         and evaluated in a pilot study.
     3.  Ambient, residential and source samples were taken simultaneously
         with equipment and procedures developed to provide comparable
         samples for chemical, physical and biological characterization.
     4.  Wintertime sample sets were collected for chemical  and
         bioassay analysis at two urban residential  sites impacted by
         wood burning emissions.
         A mutagenic activity data base on the semi-volatile and particulate
         organic samples has been generated a.s part  of these studies.
         These data will be incorporated into a source apportionment model
         which for the first time will  merge biological  and chemical/physical
         information.
     6.  Field and laboratory studies have both shown that greater mutagenicity
         was associated with the semi-volatile and volatile components than
         is associated with the particulate matter.
         Initial  receptor model  calculations from Albuquerque show that
         residential  wood combustion and mobile sources account for
         approximately 90% of the fine particle mass.  This result supports
         the earlier assumption  that these sources contribute significantly
         to the mutagenic potential  of the ambient air.

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II.   Background  and  Rationale
          Major  scientific  questions  regarding the relationship between air pollution
     and human cancer  remain unanswered.   Human cancer caused by^air pollution
     is  difficult  to elucidate  by traditional techniques of epidemiology.  The
     length  of time  (decades) that may pass  between an exposure to a carcinogen
     and diagnosis of  cancer precludes any meaningful prospective study of
     human populations and  their quantitative dosage of carcinogens.
     Retrospective studies  are  also difficult to perform since one does not
     know when the observed cancer was initiated.  Because most non-occupational
     cancers are not specific and could have multiple causations, the process
     of  associating  an observed cancer with a given putative agent has not met
     with great  success.   In 1977 and again  in 1982, international meetings
     were held in  Stockholm, Sweden to address the relationship between air
     pollution and cancer risk.  These meetings both concluded that air pollution
     arising from combustion products of  fossil fuels, probably acting together
     with cigarette  smoke,  have been  responsible for lOfc of all  cancers for
     the United  States.  Doll and Peto, in a recent review of causes of
     cancer  in the U.S., also suggest that 2% of cancer deaths could be attributed
     to  pollution.   Karen and Schneiderman recently reported that past
     analyses  of this  problem have overestimated the contribution of smoking
     and underestimated the multicausal nature of cancer.  They estimate that
     at  least  11% and  more  likely 21% of  lung cancer is related to air pollution.
          Regardless of which of these estimates proves to be the most accurate,
     there is  certainly reason  to believe  that the carcinogenic potential  of
     air pollution may be a serious public health problem.  EPA needs to
     undertake a major research program directed specifically at clarifying
     the risk  and  sources of carcinogens  in the air.  As part of this program
                                         5

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a methodology must be developed that will  allow an estimate  of the  future
cancer risk associated with human exposures to  present  day dosages  of
airborne carcinogens which can be related  to identifiable  sources.
     The Environmental Protection Agency has the responsibility and authority
to regulate the emission of carcinogens  into the air  (e.g.,  Section 112,
Clean Air Act), however, the identification of  which  carcinogens and
emission sources are of greatest potential  human risk is  not well  known and
remains a high-priority research effort.  In the past,  research on  hazardous
air pollutants has been conducted on individual  primary pollutants.
These substances have been selected for  study based upon  such available
data as national production volumes, volatility, estimated emissions,  and
known health effects data (including data  on suspected  carcinogenicity).
The compounds selected may, or may not,  actually be the principal carcinogens
to which people are exposed.  The Integrated Air Cancer Project adopts a
different approach:  it focuses on identifying  those  species actually
present in the air which are most likely to be  carcinogenic  and attempts
to describe how they came to be present  in the  environment.   The accomplishment
of this research requires the IACP to bring together  the  multi-disciplinary
talents of chemists, engineers and"health  scientists  to conduct a series
of coordinated field studies of emission sources, atmospheric transport
and transformation, and toxicological studies to address  the complex
issues involved.

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Objectives of the Project
A.  The major long-range goals of this research program are:
    I.  To Identify the principal  airborne carcinogens.
             The relative importance and contribution to the  total  airborne
        carcinogens of the volatile, semi-volatile and participate  organic
        compounds is not known.  This research will  develop the methodologies
        and data necessary to eventually provide such an evaluation.
        Within each of these fractions the specific  chemicals or
        chemical classes which contain mutagenic and carcinogenic compounds
        need to be identified and their concentration in air  quantitated.
        It is possible that these compounds could be transformation
        products produced after reactions of simple  hydrocarbons or
        complex polynuclear aromatic hydrocarbons with acidic and oxidizing
        gases in the atmosphere.  Therefore an integrated approach  is
        needed to address these goals.  Not only do  the emission sources
        need to be characterized, but transformation products from  these
        emissions need to be identified.
    2.  To determine which emission sources are the  major contributors of
        carcinogens to ambient aTr"!
             To control the emission of hazardous air pollutants, the sources of the
        hazardous compounds themselves or their precursors have to  be identified.
        Field studies with simultaneous emission characterizations  and ambient
        monitoring, followed by source apportionment calculations,  will  be
        conducted to determine which emission sources are the major contributors
        of carcinogens to the ambient air.  Characterization  of emissions
        "and ambient samples will be by both chemical and biological (mutagenicity
        and carcinogenicity) testing.

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    3.  Improve the estimate of comparative human cancer  risk from specific
        air pollution emission sources

             In order to improve the estimate of relative human cancer  risk  from

        specific air pollution emission sources, a comparative methodology is

        being developed to evaluate and utilize  short-term mutagenesis  and

        animal  carcinogenesis data  on emission sources.   In addition, better

        total human exposure estimates will  be developed  for these complex

        emission products and individual  carcinogens  including transformation

        products.

8.  The major short range goals of  this reasearch program are:

    1.  Phase 0, FY'84 Objectives:

        Design and planning of the  FY'85/'86 Integrated Air Cancer Project.

            a)   Preparation of background documentation.

            b)   Preparation of project research  plan  including work plan,
                protocols, and quality assurance plan.

            c}   Establishment of scientific  peer review and advisory
                group to review the concept  plans, project plans,  QA
                plan, and progress  of the project.

    2.  Phase I, FY'85 Objectives:

        Field and laboratory evaluation and  selection of  methodology.

            a)   Select data management tools.

            b)   Design and test community survey.

            c)   Evaluate and select sampling methodologies.

            d)   Evaluate and select fractionation and analysis methodologies.

            e)   Use air chemistry simulations  to assess the chemical
                distributions and hazardousness  of the air pollution anticipated
                in the background air at the likely field site.

            f)   Improve and validate sampling, analytical  and bioassay  method-
                ologies.

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            g)   Select appropriate  source  apportionment methodologies  for
                identifying  sources and  impacts  of  carcinogenic  species.

    3.   Phase II,  FY'86/'87  Objectives:

        a.   To  conduct an integrated field study of a  simplified air shed  in order
            to:

            1)   Identify and quantify classes of compounds  in  the ambient
                air resulting from  residential wood combustion and motor
                vehicles.

            2)   Quantify the relative contributions of emission  sources,
                specifically residential wood combustion  and motor vehicles,
                to the mutagenic  activity, organic  and fine particulate mass
                of ambient airborne pollutants.

            3)   Apply exposure assessment  methodologies for selected
                potential carcinogens, including aldehydes.

            4)   Develop a data base to compare the  human  cancer  risk of
                air impacted by residential  wood burning  to other combustion
                sources previously  evaluated (e.g., residential  oil burning,
                motor vehicles, etc.).

        b.   Develop methods  (sampling and  analysis) to extend  to other
            airsheds heavily impacted by wood stoves.

        c.   Conduct simulations of  the field site air  chemistry  in order to
            assess the resultant  changes in mutagenic  response and to
            characterize the chemical  changes which may occur  to the source
            emission materials.

        d.   To  complete development of scientifically  sound protocols,
            procedures and instruments for implementation by the
            states and regions of future woodsmoke  studies development
            for future IACP  studies.

        e.   Complete the analysis of samples from the  FY'85 study.
    To meet these objectives  established  methods  will  be  used at an

appropriate field site to obtain the data necessary  for objective  (a).

Research will  continue at RTF to meet objectives  (b-e).

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IV.   Management

     A.   Management  Afpnach

          The organization  and  management  of  this  project  is designed to ensure

     that the expertise  of  each of  the  four participating  laboratories  (HERL,

     AEERL,  ASRL,  and  EHSL)  is  applied  in  the most effective manner to  meet the

     project's scientific objectives.   Specific management objectives are:

         1.   Provide leadership and  direction for  the  project planning  and
             implementation which are closely coordinated  between the four
             laboratories.

         2.   Ensure  technical  input  from all  four  laboratories  in all aspects of
             the  project.

         3.   Provide a mechanism for efficient interdisciplinary decision making.

          In order to  accomplish these  objectives, a management plan was prepared

     which described the matrix management organization operating through a steering

     committee and technical  teams.  The membership and responsibilities

     of  the  steering committee  and  team leaders is described below in the

     management plan.  This plan was presented to  the  four laboratory directors

     for their discussion,  modification and approval.  This was a critical

     step in the  process of meeting  the above objectives since  several

     of  the  laboratory director's normal responsibilities  were  being delegated

     to  the  steering committee.

     B.   Management  Plan

          The Integrated Air  Cancer  Project is an  integrated interlaboratory project

     involving the expertise  of all  four research  laboratories  in the Research

     Triangle Park,  NC.  The  management plan  which has been developed,  reviewed,

     and agreed.upon by  the laboratory  directors utilizes  a steering committee and

     technical  teams with representatives  from each laboratory  as listed in

     Table 1.
                                         10

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          TABLE 1.   IACP STEERING COMMITTEE AND TEAM MEMBERS
      FY'85
             FY'86
Steering Committee:

   Joel 1 en Lewtas, HERL (Chairman)
   Tom Clark/Jack Puzak, EMSL
   Gene Tucker, AEERL
   Basil Dimitriades, ASRL

Study Design/Data Management/Interpretation Team:

   Larry Cupitt, ASRL (Team Leader)
   Dave Mage, EMSL
   Larry Claxton, HERL
   Bruce Tichenor, AEERL

Sampli ng Team:

   Charles Rodes, EMSL (Team Leader)
   Ralph Baumgargner, ASRL
   Bruce Harris, AEERL
   Judy Mumford, HERL

Analysis Team:

   Jim Dorsey,  AEERL (Team Leader)
   Nancy Wilson/Don Scott, EMSL
   Leon King, HERL
   John Sigsby, ASRL

Quali ty Assuranee:

   Jack Puzak,  EMSL
   Ralph Bauragardner, ASRL
   Gary Johnson, AEERL
Joel 1 en Lewtas, HERL (Chairman)
Jack Puzak, EMSL
Jim Dorsey, AEERL
Robert Stevens, ASRL
Larry Cupitt, ASRL (Team Leader)
Dave Mage, EMSL
Larry Claxton, HERL
Bob McCrillis, AEERL
Charles Rodes, EMSL (Team Leader)
Ralph Baumgargner, ASRL
Bruce Harris, AEERL
Judy Mumford, HERL
Ray Merrill , AEERL (Team Leader)
Don Scott, EMSL
Randy Watts, HERL
John Sigsby, ASRL
William Mitchell, EMSL
Ralph Baumgardner, ASRL
Gary Johnson, AEERL
                                  11

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     Because of the project's special nature, it was recommended that the Laboratory

Directors delegate responsibilities for project planning and implementation

to their representatives in the steering committee.

The responsibilities of the steering committee are listed below:

    1.  Provide overall scientific and technical  review and approval of
        project plans.

    2.  Ensure overall planning, coordination, and timely delivery of high
        quality Project outputs.

    3.  Ensure that project information is relayed to the Research Committee
        and Program Office (OAQPS).

    4.  Resolve any problems between the research teams or laboratories.

    5.  Ensure that RTP laboratory directors are kept informed on a semi-annual
        basis of the progress of the project, its resource requirements
        (especially for support from in-house personnel, which will vary as
        the project progresses).  Any management or technical  problems that
        cannot be satisfactorily resolved by the Steering Committee will be
        discussed with the laboratory directors as the need arises.

    6.  Assigning project tasks to the appropriate laboratories based upon
        factors including identified expertise and each respective laboratory's
        mission.

    7.  Distribute the'Project's extramural  resources (from the IACP portion
        of HAP funds) among the major tasks  in the project.  This will
        ensure that the steering commitee has sufficient authority over the
        project to see that its responsibilities can be implemented.  The
        Agency's current planning process has allocated funds  into a series
        of PPA's which have been identified  with the IACP.  These resources
        are not necessarily distributed among the laboratories by PPA propor-
        tionally to the work to be accomplished.   The ORD Steering Committee
        for the Air Cancer Project has agreed to consider the  extramural
        resources as one pool  of money for the project and distribute it
        according to the laboratories'  needs in the final approved project-
        plan.

The responsibilities of the research team leaders are to:

    1.  Plan and coordinate the work in their respective areas, ensuring
        best effort at meeting overall  project schedules prepared by the
        steering committee.

    2.  Submit detailed plans  for review and approval to the steering
        committee.  Present progress reports to the steering committee.
                                    12

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    3.  Ensure that expertise from all  four laboratories is used objectively
        in planning and implementation of tasks.
    4.  Work with other research teams to ensure  coordination of technical
        details.
C.  Budgeting an Inter-laboratory Project
    1.  Budgeting Resources
         Although this project was jointly planned by all  four laboratories as one
    integrated project with one set of objectives, the current budgeting
    process did not accomodate funding the project with one PPA (Planned
    Program Accomplishment).  Therefore, each laboratory submitted to their
    respective headquarter's office a proposed PPA and budget for the project.
    The Research Committee considered the four combined PPAs in funding the
    project.  The FY'85 resources were the following:
                  Lab        S&E        MY         R&D
EMSL
ASRL
AEERL
HERL
220
-0-
294.3
138.9
4.4.
-0-
5.0
2.8
980
94
349.3
337.5
                  Total       653.2     12.2       1760.8
D.   Peer. Review and Advisory Process
      The peer review and advisory panel  (Table  2)  selected  in February 1984
    consisted of experts from each of the disciplines  represented  in the
    project who were also experienced in  interdisciplinary environmental
    studies.   The peer reviewers  were sent copies of the IACP Concept Plan*
    and Study Design and invited  to participate  in  a 4-day workshop in April
    1984 on Genotoxic Air Pollutants  held at Quail  Roost Conference Center.
    Many of the technical  issues  addressed in the project plans were also
    addressed at this workshop.   Each peer reviewer also provided  individual
    written comments to the Steering  Committee (See Appendix B 1).

                                    13 '

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    The Peer Review Panel's comments and suggestions were used to revise the
design, scheduling and emphasis of the project prior to preparation of
the task protocols (work plans).  The peer reviewers were very strongly
encouraged and endorsed the project concept and approach.  They cautioned
the Steering Committee to proceed at a slower pace than had been projected
in order to develop the methods that would be needed for the project's
success.  They advised the project to strive for scientific quality rather
than quantity.
     During the first week in October 1984, after preparation of all  of the
task protocols and an initial budgeting of the resources, the peer review
panel was reconvened to review the technical approach in more detail.
The first two days of the meeting were used for technical presentations
and discussions with each scientist and engineer involved with the project.
The last several  days were used by the peer reviewers to prepare a report
to the Steering Committee and Laboratory Directors with their recommendations,
Their recommendations were presented in an open meeting to all project
participants, Laboratory Directors and other interested parties (such as
representatives from OAQPS and the ORD Headquarters Research Committee
staff).  The advisors recommended some limitations in the scope of the
project,-maximum use of EPA personnel, deletion of woodsmoke control-
related research, and changes in the objectives, approaches, and the
scope of specific tasks (See Appendix C 2).
                                14

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                       TABLE  2.   PEER  REVIEW  PANEL
Dr. Roy Albert
NYU Medical Center
550 First Avenue
New York, NY  10016

Dr. Ingird Alfheim      •  •
Central Institute for  Industrial Research
P.O. Box 350 Blinden
0314 Oslo 3, Norway

Dr. Bruce Appel
California Dept. of Health Services
Air and Industrial Hygiene Laboratory
2151 Berkeley Way
Berkeley, CA  94704

Dr. Joan Daisey
Institute of Environmental Medicine
NYU Medical Center
550 First Avenue
New York, NY   10016

Dr. Glen Gordon
Chemistry Department
University of Maryland
College Park, MD  20742

Dr. Charles Lochmuller
Department of Chemistry
Paul M. Gross Chemical Laboratory
Duke University
Durham, NC 27706

Dr. Goran Lofroth
Department of Radiobiology
Wallenberg Laboratory
University of Stockholm
S-10691 Stockholm, Sweden

Dr. James Pitts, Jr.
Statewide Air Pollution Research Center
University of California
Riverside, CA  92521

Dr. Dennis Schuetzle
Analytical  Science Department S-3061
P.O. Box 2053
Ford Motor Company
Dearborn, HI  43121
                                    15

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V-   Technical  Approach
    A.   Integrated  Field Study
             The Phase 1 integrated  field  studies'  goal  was  to develop  procedures
        to identify and quantify the airborne  emissions  from mobile  sources and
        residential  wood combustion.  Limited  residential  air measurements and
        woodstove appliance emission measurements  were  planned as  part  of
        the Raleigh study.
             Correlation between sources and ambient measurements, both inside
        and outside, are important considerations  for the  success  of the  IACP.
        Therefore,  to the greatest extent  possible, identical sampling  and
        analytical  schemes  were planned  for ambient and  source studies  to
        obtain samples for  bioassay, chemical  characterization and source
        signature studies.   Throughout the entire  field  study appropriate
        QA/QC procedures were  followed.
    B.   Sampling
             The sampling portion of this  study was planned  to include  the development
        of the detailed protocols which would  allow materials of known  integrity and
        sufficient  quantity to be collected.   These sampling protocols  were;
        structured  to facilitate the subsequent bioassay directed  fractionation
        and chemical  analyses  necessary to identify the  relationships between
        source, ambient and microenvironments.  Studies  were conducted
        to characterize, validate, and evaluate samplers to  collect  samples
        for chemical  and biological  characterization.   The sampling  protocols
        were to take into consideration techniques  necessary to collect
        particulate  material as well  as volatile,  semi-volatile, and  condensable
        organic material.  Combustion gases and other key  indicators  were
                                        16

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    to be measured as  part  of the sampling  activities.   Typical  activities
    for sources were to include sampling  with  extractive sampling equipment
    and appropriate participate filtration  and vapor  phase organic collection.
    Ambient sampling planned  to include size separation  of particulates,
    collection of respirafale  and inhalable  particulates  and other
    organic material.   Microenvironment sampling  procedures were to
    include volatile and semi-volatile sampling at  low concentration
    levels.
C.  Source Apportionment
         Source apportionment is a  combination of mathematical and analytical
    procedures which are used to determine  the contribution of specific
    emission sources to ambient concentrations of air pollution.  Several
    methods  have been  used  to apportion the contributions of  source emissions
    to ambient air quality.   These  include  emission inventory methods,
    source dispersion  models  and receptor models.   The receptor-model
    approach to source apportionment  was  thought  to be effective for this
    type of project, where  the number of  particulate  sources  are small
    and known.  In addition,  emissions from mobile  sources and wood
    burning  contain unique  elemental  tracers which  improve the accuracy
    of the source apportionment calculations.   The  key assumptions, based
    on the current state of the art of receptor modeling were:   (1)
    source signatures  would be unique, (2)  ratios of  elemental species
    emitted  from a source would remain unchanged  during  transport from
    source to receptor, (3) the measurements of composition would be
    precise  enough to  distinguish among sources,  (4)  ambient  concentrations
    would be high enough to be measured reliably, and (5) statistical
    receptor modeling  would require more  than  40  samples (day) and 40
                                    17

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    samples (night) and substantial  variability of source emission rates
    during the two sampling periods.
D.  Bioassay Directed Fractionation/Characterization
         This approach has been successfully used  to identify potential carcinogens
    in complex mixtures including synthetic  fuels, diesel  emissions,  and
    kerosene soot.  Basically, the complex mixtures are  fractionated  and
    each fraction is bioassayed.  The Ames Salmonella  typhimurium plate
    incorporation assay or the j>. typhimurium forward  mutation assay  have
    been the most widely used bioassays.   Mutagenically  active fractions
    are further fractionated, bioassayed,  and characterized  until  the
    major class or specific compounds responsible  for  the mutagenicity
    are identified.
       •   For Phase 1 this approach would  initially be aimed at identifying
    mutagens.  It was not expected to identify tumor promoters or
    chemicals with other toxic (non-mutagenic) activity.   The compounds
    and fractions identified as mutagenic  using this approach would be
    further evaluated for mutagenicity in  mammalian cells and carcinogem'city
    in rodents.
E.  Chemical/Analytical Measurements
    1.  Organic Compounds
             Chemical  analysis provides identification of those chemical
        species originating from wood combustion and mobile  sources and
        their -atmospheric transformation products  that are carcinogenic
        or potentially carcinogenic.   Analytical measurements were therefore
        planned to address three aspects.   First,  establish  profiles  of
      .  the organic compounds present, including volatile, semi-volatile,
        and non-volatile or particle-associated compounds.  Second, the
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    methods must provide identification of the  compounds  that  may
    pose a significant hazard  to  human health.   Third,  those compounds
    that have been identified  as  markers,  established carcinogens, or
    potent tnutagens must be quantified.
         Reliable or existing  methods  were considered initially  and
    modified and the necessary modifications  were  planned over the course
    of the project.  Initial  screening of  samples  would  involve  gas
    chromatography with flame  ionization or photoionization detection
    (GC/FID or GC/PID) for volatile  organic compounds and gas
    chromatography/mass spectometery (GC/MS)  and high performance
    liquid chromatography (HPLC)  with  ultraviolet, mass  spectrometry,
    or fluorescence detection  for semi-volatile and  particle-associated
    compounds.  The screening  approach was based primarily on  the
    mutagenicity of the fractions with chemical/analytical screening
    as a complementary procedure.
2.   Inorganic Compounds
         In order to apply current receptor models to determine  the
    fraction of ambient aerosols  that  orginate  from  wood  burning,
    extensive inorganic chemical  and physical analysis of ambient
    particles and source emissions is  necessary.   These measurements
    planned included:
    a.  The elemental composition of particulates  (principally of the
        elements potassium, chlorine,  lead, and bromine).  Carbon-14
        dating measurements were  also  included  to  apportion air
        particulate carbon into "new carbon"  such  as wood burning
        and "old carbon" such  as  gasoline, oil  and coal  etc.
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        b.   Determination of the amount of elemental  and  volatilizable
            carbon present in fine particles.   The  ratio  of elemental
            carbon to volatilizable carbon is  important in  resolving  the
            source of carbon.
        c.   Sulfate and nitrate concentrations  in fine particles.   These
            measurements were planned  to provide data for the  chemical mass
            balance receptor model  calculations.
        d.   The measurement of particle mass.
F.   Atmospheric Transformation
         A  growing number of laboratory and  field studies have suggested that
    there are unidentified compounds  present in ambient air which cause
    mutagenic responses in short-term  bioassay  tests, both  in  the vapor
    and aerosol  phases.  Recent studies in ASRL/HERL  have demonstrated
    that exposure of many organic  source emissions  to photochemical reaction
    conditions increases the mutagenicity of the emissions.
         The transformation studies carried  out as  part of  the Integrated Air
    Cancer  Project were planned to  utilize a large  reaction and atmospheric
    simulation chamber  (the Mobile  Aerosol  Reaction Chamber, or MARC) to
    produce  irradiation products of air mixtures like those found in
    typical  U.S.  'environments  and  in the IACP field study.   Operated  in
    a  dynamic mode, the MARC produces  consistent conditions which
    will  permits  direct exposure of bioassay test systems and  provides
    large quantities of the transformation products for chemical sampling
    and analysis.   Runs with differing  residence times or reaction conditions
    produce  differing product  distributions  for aid in identifying the
    potentially  hazardous  materials and in understanding  the processes
    which form the  target  chemicals.
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         The MARC was  designed  to begin with an examination of the simpler
    systems and an identification of  the  products which cause the bioassay
    responses.   More complex mixtures would then be examined as understanding
    of the processes increased,  culminating in simulations of the actual
    field conditions found  in the  IACP field studies.
G.   Meteorology (Task  9  and Task 10}
         A meteorological  understanding of the transport and diffusion of
    woodsmoke is essential  to interperting the ambient samples.  Such
    understanding is essential  to any extrapolation of the data to other
    locations and/or other  times through  dispersion modeling.  Meteorlogical
    measurements are planned to  determine the relative impact of nearby
    sources on the ambient  samples  and to determine how woodsmoke diffuses
    under stagnant conditions influenced  only by local drainage flows.
H.   Human Exposure Assessment
         Human exposure  to  airborne carcinogens is continuous throughout
    one's life.   However,  in order  to interpret measured exposure data so
    that the sources of  the carcinogens can be identified, it is necessary
    to analyze methodically the total exposure to carcinogens as the
    summed effect over multiple discrete  exposure intervals which can be
    aggregated into classes represented by common sources.  For example, a
    single collection  of airborne  particles over a 24-hour period may
    capture a specific carcinogen in  a significant quantity, but there
    would be no information as  to whether the exposure occurred in the
    subject's residence, in traffic while commuting, at work in an occupational
    setting, or outside  in the  ambient air.  It would help to measure the
    portions of the sample collected  in each of these categories independently
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to ascribe the probable source to one or  the  other  microenvironments.
There are two general  ways in which this  evaluation can  be  achieved.
In the first approach  the subject collects  a  discrete  sample  in  each
microenvironment passed through in the course of  a  day.   In the
second approach, samples are collected continously  in  each  microenvironment
and the subject's activities are monitored  to ascribe  to them an
exposure associated with each microenvironment.   The second approach
is the one selected as most applicable for  evaluation  of human carcinogen
exposure assessment in the integrated field studies  described above.
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VI.  Project Status
         The FY'85 program of the IACP focused  on three  main  areas  of  research:
     field measurements and methods development/evaluation work conducted  in
     the RTP area, field measurements in Albuquerque,  NM,  and special  efforts
     to enhance our understanding and preparations for Phase  2.
          The RTP field program included sample collection at fixed sites
     to characterize the mutagenicity and organic chemical composition of  the
     ambient aerosol, to permit receptor analysis of the origins of the'
     aerosol, and to characterize the air mass  for hazardous  and criteria
     pollutants and meteorological  parameters.   The fixed  site monitoring  was
     combined with measurements at various homes to describe  the nature and
     magnitude of the source emissions from the use of wood stoves.  Measurements
     inside and outside the homes were also made to assess the exposure levels
     of the residents.  The RTP effort included a series of tasks which
     were intended to resolve various technical issues related to the  sampling
     and analysis methods to be used in Phase 2 of the project.
          The Albuquerque field program, like the fixed  site  monitoring at
     RTP, included sample collection at two sites for bioassay characterization,
     for receptor analysis, and for characterizing ubiquitous gaseous
     pollutants and meteorological  factors.  One site was heavily impacted by
     residential woodburning and the other by vehicular  emissions.
          The special studies included laboratory determinations of the factors"
     influencing the emissions from wood stoves and smog-chamber simulations
     of the transformations of the wood smoke.   The special study area also
     covers a few tasks which were designed to  prepare for the FY'86/'87 time
     period.
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     The status of each of these areas  is  briefly discussed  beliOw.
A.   RTP Measurements
         Measurements in the  RTP area  were made  regularly  at two  fixed  sites
    (one in a RWC impacted neighborhood and  one  at a  background location),
    and for short periods of  time at one roadway site and  at 5 residences.
    The status of the effort  is  described  below.
    1.  Bioassay and Organic  Characterization  (Task 1 and  Task 3)
             The purpose of the  analytical  portion of the  field measurements was
        to prepare and analyze samples  for both  bioassay/organic  signature
        evaluation and source apportionment.   The Fiscal Year 1985  studies
        concentrated on residential , mobile  and  woodstove  ambient emissions as
        the primary sources of impact  for  the  airsheds and exposure routes to be
        studied.
             The signature sample preparation  involved collection/concentration of
        volatile, semi-volatile  and  particulate  organic materials from  ambient,
        residential  sites, and source  locations.   Gaseous  analysis  procedures
        involved cartridge collection  of aldehydes and canister collection
        of light hydrocarbons and halocarbons.
             Analytical  techniques used for  source signature involved direct
        analysis of the gaseous  organic compounds, extractable organic  material
        (EQM), and polycyclic aromatic  compounds  (PAC).  Bioassay (Ames) analyses
        were also performed on filter  and  sorbent extracts.   Additional sp'ecialized
        analyses to develop techniques  for bioassay directed fractionation and
        identification of mutagenic compounds  were planned and are  described in
        the special  projects  portion later in  this report.
             Samples submitted for volatile  organic analysis included:  16 impinger
        and 61 cartridge samples for aldehyde  analysis and 38 gas phase samples for
                                   24

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light hydrocarbons and halocarbons.   Samples  submitted  for  other organic

analyses included: 56 sets of filters for  source  apportionment, 20  sets

of filters and sorbent for residential  signature  analysis,  and  12 sets of

filters and sorbent for source emissions signature  analysis.  Additional

samples (approximately 130 filters  and  6 sorbents)  were submitted for

analysis to support research and methods development tasks.

     Analysis of samples from the field study is  underway.

Results of the signature analysis using volatile  organic compounds  are
                                                    *
essentially complete and show differences  between roadway and woodstove

impacted samples.  The volatile analysis for  aldehydes  developed under

part of the field effort provide comparable data  to, and are more sensitive

than the conventional impinger techniques.  Halocarbon  analysis did not

appear to yield data useful to source apportionment or  signature analysis

due to the very low levels of these compounds observed.

     Results from the filter and sorbent analyses are still being completed.

Residential samples and the comparable prime  site samples have  been

analyzed for EOM.  Initial results  indicate a low mass  loading  on filters

[approximately 1 to 4 ug/actual standard cubic meters (ASCM)] and

a much larger loading on the sorbents (10 to  30 ug/ASCM).  Mutagenesis

analyses are currently being performed on this set of samples to

determine  if the relative response of the samples follows the

mass loading or  if there is a difference in the activity between

the condensable  and semi-volatile material.

     Completion  of the EOM and bioassay analyses are planned  for  late

FY'85 and  early  FY'86.  All EOM analyses on source apportionment, ambient

signature  and source signature samples will be completed in the near


future.   Directed research tasks to identify and quantify the

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     mutagens using a combination of bioassay  directed  fractionation,
     chemical analysis and mutagenesis  bioassay will  continue  into
     FY'86.   Compilation and interpretation  of the  results  from  all
     facets  of the project will  result  in a  series  of peer  reviewed
     journal  articles in FY'86 and FY'87.
 2.  Modeling Data
          In an effort to identify species responsible  for  the ambient mutagenicity
     and to  relate them to their original  source types, measurements were made
     in Raleigh using the following samplers:  a dichotomous  sampler  (elemental
     and mass data for 0-2.5 urn and 2.5-10.0 urn), a carbon  sampler  (0-2.5 urn),
     and a nitric acid/nitrate sampler  (0-2.5  urn).   Twelve  hour, day and
     night,  samples were taken over a period from January 15 to  March 26, 1985.
     The dichotomous filter samples which were collected are being analyzed
     for elemental content by X-ray fluorescence at the RTF labs.  As of September
     1, mass analysis, nitric acid/nitrate analysis and elemental analysis of
     fine particles were completed. . Analysis  for volatilizable  carbon
     have been initiated.  Once the data  are formatted, a receptor   •
     modeling exercise will be performed  to  apportion the Raleigh
     aerosol.  Also, bioassay results from the samples  collected over
     the same time periods will  be added  to  the source-apportionment
     data base.
3.   Chemical  and Meterological  Support  Measurements (Albuquerque, Ralefgh and Task 9}
          Ancillary measurements including carbon monoxide  (CO), nitric oxide
     (NO), nitrogen dioxide (f^), ozone  (03), sulfur dioxide  (SOj), nephelo-
     meter Bscat, wind speed and direction,  precipitation,  solar radiation, and
     relative humidity were made to help  relate the RTF wood smoke measurements
     to other pollutant sources in the  vicinity, transport  and transformation,
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        and  measurements  from  other  studies.   The  pollutants  and meteorology were
        measured  with continuous  monitors  housed  in mobile  vans located at  the
        primary and background sites,  producing hourly averages from  1/9/85 to
        4/17/85,   Over 30,000  data points  were collected  by the on-site mini-
        computer  and final  validation  is  still in  progress.
    4.   Source Measurements (Task 22)
             The  objective  of  the field  source sampling task  was to sample
        different woodstoves  for  condensable  particulate  and  semi-volatile  organic
        material.  Duplicate  tests using  the  Woodstove Dilution Sampling  System
        were completed on four woodstoves  in  North Raleigh.   Samples  have been
        delivered to the  analytic group  for chemical  and  biological characterization.
        Additional  samples  are being acquired as  needed for specialized resarch
        tasks.
    5.   Exposure  Measurements  (Task  .13 and Questionnaire)
             In order to  address  exposure  to  wood  smoke near the main Raleigh
        site, selected measurements  were made inside  and  outside of five  resi-
        dences.  Particulate  samples integrated from.7 p.m.  to 7 a.m.  were  col-
        lected on Teflon  and-Pallflex  filters for  chemistry and bioassay, along
        with XAD-2 for semi-volatiles, DNPH tubes  for aldehydes, and  Tenax  and
        evacuated cannisters  for  volatiles.   Particle mass  data shows that
        the particle concentrations  are  much  lower indoors  than outdoors.
        The chemistry and bioassay analyses are in progress.   The  exposure*
        sampling  component  of the program  is  expected to  be expanded  in
        FY'86 to  include  a  much larger number of  homes selected by a
        statistically valid survey questionnaire.
B.  RTP Measurements - Resolving  Technical Issues
         A number of experiments  were  undertaken  at RTP to  resolve various
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technical issues which arose during the peer review.  The status of each
is discussed below.
1.  Extraction (Task 20}
         The primary objective of the extraction task was to optimize
    the recovery of mutagenic material from filter and sorbent material  used for
    IACP sampling activities.  One hundred seventeen (117) filters
    and six (6) XAD-2 sorbent modules from the primary sampling site were
    used for the task.  Composite filter particulate samples were
    extracted using combinations of organic solvents and extraction
    techniques.  Mass recovery and mutagenic activity data from the
    filter samples were obtained and these data are being used to
    compare various combinations of extractions.   All  laboratory work has
    been completed on the filter samples.   The same approach is planned  for
    for the XAD-2 sorbent samples.
         Future efforts involve application of statistical  analysis (ANOVA)
    to identify significant differences between the techniques evaluated.
    Completion of statistical  analysis will  allow additional  laboratory
    testing of the effect of the optimum solvent  on mutagenic activity
    ("inertness"  study).   A standard operating procedure and a journal
    publication are planned as the final  products of this task.
2.  Sample Integrity (Task 8)
         The purpose of this task was  the  investigation  of the effects" of sample
    storage over  time, both on the collection media (filters or sorbent  resin)
    and as extracts.  Eight samples (4 XAD-2 sorbent,  4  filters)  were generated
    as samples  for extraction.   Eight  extracts (4 XAD-2, 4 Filter)  were
    generated  and  stored  as extracts.   Organic and bioassay aliquot samples
    were stored in the appropriate solvents.
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3.
     Organic and bioassay analysts of the samples and the stored
extracts will be conducted over a period of 8 months.  Results from each
analysis period are compared to the other periods using an optimum design
statistical  approach.   The first three periods have been completed.
Chemical and bioassay analysis is complete on these samples.
     Data thus far from the Sample Integrity Task indicates little or no
chemical change in the samples over the storage period.  Some possible shift
between semi-volatile and condensable material was noted in the chemical
analysis.  These trends will be evaluated at the completion of
the task.
     The last sample set is to be evaluated shortly.  Following
completion of chemical and bioassay analyses the results will be reviewed
for trends and recommendations on sample storage for the FY'86 study.  An
SOP is planned as output from this task.
XAD-2 Clean-Up (Task 7)
     The objective here was to design and implement a more cost-effective
cleaning procedure that would produce clean XAD-2 sorbent resin
which met or exceeded existing QA requirements.  A developmental large scale
extraction apparatus was evaluated which allows approximately 2
kg of resin to be prepared per batch.  Twenty kilograms of resin
material were cleaned using this apparatus.  The sorbent resin
material prepared using this technique was evaluated against a
smaller scale clean up apparatus used to prepare resin for source
sampling.  Resin prepared in the new apparatus was found to be cleaner
in all cases than the smaller scale unit.  As a result all resin needs
were met.
                                29

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         The current activity for Task 7 involves  scaling  up  the  clean-up
    procedure using solvent elution instead of Soxhlet extraction.   The  new
    apparatus being evaluated will  allow cleaning  of at least 4 kg  of resin
    per batch and holds the possibility to generate resin  with a  lower
    background at a much lower cost than the extraction technique.   Upon
    completion of the final  -scale up evaluation, an SOP will  be
    generated which describes the selected technique for providing  clean
    sorbent resin for semi-volatile organic sampling.
4.  Fractionation (Task 19)
         The objective of this task is to  develop  a procedure to  divide
    complex organic mixtures extracted from IACP samples into fractions
    which simplify the mixture, concentrate the mutagenic  activity,
    and allow identification of chemical compounds or  compound
    classes responsible for  the activity.   The development of the
    fractionation scheme by  HPLC is in its early stages.   Compounds
    have been identified for use as standards  to mark  the  division
    between chemical  classes as they elute from the HPLC.   Blank  and
    control  samples have been assayed  in both  chemical  and mutagenic  assays.
    Efforts will  continue using source samples to  refine the  separation
    between chemical  classes to meet the objectives  of  the task.
         The limiting factor for fractionation and the  subsequent chemical
    and bioassay  testing is  the mass available from the  samples taken to
    date.   Individual  source samples are planned for the development  stage
    of .the  fractionation task,  followed by application  of  the  developed
    procedure to  source and  residential samples.   A refinement of
    the initial fractionation approach  has  been chosen  which  combines
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    the best of existing  approaches  used  previously in  bioassay  related
    projects and in chemical  analysis  related  projects.   The  efforts
    on this task will  continue in FY'86.
5.  Evaluation and Development of New  Bioassay Techniques (Task  15)
         This task, Evaluation of Microbial  Bioassay Techniques, is  the
    development and evaluation of rapid  and  automated microscale bioassay
    techniques, is proceeding on schedule.   While  one method, the Mutascreen
    system, has been shown to be inadequate, two other  usable methods  1} the
    micro-forward mutation assay and 2}  the  micro-reverse mutation assay
    have been implemented.  Bioassay results obtained to  date are
    reported as part of each  task in this section  and/or  in  Appendix  B.
    Support of other tasks is proceeding  with  the  receipt of  samples;
    however, due to late arrival  of  samples  bioassay studies  will  proceed
    into. Fiscal Year 1986.
6.  Organic- Signature/Apportionment  Analysis (Task 14)
         The objective of this work  is to define compounds,  groups of compounds,
    or other significant analytical  features that  will  be characteristic of
    an individual type of source and to  optimize this analysis.   The  focus
    in FY'86/'87 is on 2 specific sources:   woodsmoke and automotive  sources.
         More than 200 compounds have  been identified in  the  gas phase.
    Thirty-eight samples have been analyzed  including those  collected  from
    the concurrent residential study.   This  hydrocarbon data  has been "analyzed
    and initially verified.  Some additional nonhydrocarbon  compounds
    seen by GC/MS are still being verified.   Analysis of  the  semi-volatile
    fraction and all data obtained on  this task is in progress and will
    proceed into FY'86 .  Research to  determine the optimum  procedures for
                                31

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    profiling the organic extractables from the participate fraction has
    been initiated.
         Prel iminary results suggest that organic signature analyses
    of gas phase samples may differentiate between the background,
    roadway, and primary Raleigh sites.  Twenty-nine compounds
    gave initial indications of being site specific.
         Normal phase chromatography of the particulate related organic
    compounds proved to be inadequate.  Reverse phase HPLC with fluorescence
    detection and excitation at two different wavelengths show significant
    pattern differences in the different types of source samples studied.
         Future efforts will  include verification of the non-hydrocarbon
    components seen in the gas phase by GC/MS.  The semi-volatile
    fractions will  be analyzed when they become available.  This will
    include efforts to determine the distribution of the material  by
    molecular weight and/or boiling point.  In addition data from all
    analyses will  be merged by sample period for further data reduction
    and interpretation.  The particulate organic fraction will  also
    be further characterized and expanded to include the recently
    acquired electrochemical  detector.  A preliminary data assessment
    will- be made to identify the most promising components for full
    scale evaluation in future studies.   Some organic particulate
    extract samples will'be divided and  portions will be supplied  to
    N8S for cooperative analytical  studies.
7.   Comparison  by  Particle Size (Task 3)
         In order  to demonstrate differences in chemistry and mutagenic
    response as a  function of particle size, samples were to be collected  in
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    the FINE (0-2.5  urn),  COARSE  (2.5-10  urn),  and  TOTAL  (0-10  urn)  size
    ranges.   To collect enough mass  to  permit chemistry and bioassay
    on each  sample,  a higher flow rate  (20 CFM)  version of the
    dichotomous sampler was  built and field tested  at the Raleigh
    site for mass collection using quartz  filters.   The development
    of the samplers  proved  successful  but  took longer than expected,
    resulting in no  Pall flex samples being collected for bioassay.
    A continuation effort is planned in  December  1985 to complete
    this task at an  RTP site impacted by wood smoke.
8.   Development of a 2.5 urn  Sampler  for  the Hi-vol  (Task 5)
        A long range research and development effort was initiated  to
    provide  a 40 CFM hi-vol  adaptable sampling head for 0-2.5 urn.
    This flow rate should provide enough mass for bioassay-directed
    fractionation for wood  smoke or  pollutant classes to be  selected
    in the future.  A contract task  with the University of Minnesota
    has produced a prototype which has  worked well  in preliminary
    tests.  Delivery of three field  prototypes is expected by November
    1985 for field testing  at a  local RTP  site impacted by wood
   • smoke.
9.   Comparison of Face Velocity (Task 4)
         The effect of face velocity through Pall flex filters collection
    of organics was investigated using  specially designed sampling
    heads to provide velocities  of 15,  46, 80, and  120  cm/sec.
    Samples  were collected for five 12-hour periods on  Pall flex
    filters.  The chemical  analyses are almost completed and  data
                                33

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      analysis should be undertaken shortly.   The  study will  be  repeated
      in the Raleigh area in December 1985 with  the addition  of  XAD-2
      cartridges.
10.   Source Sampling Methods (Tasks 16 and Task  22}
           A Prototype dilution source sampler was designed specifically
      for wood stove emissions.  The unit  was  tested at several  homes
      near the main Raleigh site in conjunction  with the residential
      study, collecting 12-hour integrated Pallflex and XAD-2 samples
      from 7 p.m. to 7 a.m.  The analytical  results are expected  to  be
      available shortly.  The dilution system  worked very well and
      several  additional systems will  be built for the  FY'86  field study
      after only minor modifications.
 11.   Stove Operating Profiles (Tasks  18 and Task  24)
           This effort addressed cost-effective  wood stove operation monitoring
      methods  to permit large scale characterization of the stove operating
      profiles in a neighborhood.  Continuous  stove temperature monitors were
      installed in six homes in the vicinity of  the Raleigh site  and their
      profiles recorded for 10 weeks.   The data  are still being reduced because
      of the manual  data recorders.   Activity  in FY'86  will concentrate on
      automated data recording systems.
 12.   Micrometeorology (Task 10)
           The micrometeorology in  the vicinity  of the  main Raleigh  site" was
      monitored to assess the parameters most  likely to cause high ground level
      concentrations of woodsmoke-and  affect its transport.   Low  wind speed
      monitors and vertical  temperature gradient sensors were operated from
      February through April  at three  locations  near the main site.  Results

                                 34

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        to date indicate  that  much  more  sensitive  wind  speed monitors  are
        needed to study nighttime wood  smoke  transport  and  ultra-low wind
        speed monitors have been evaluated.   A variety  of new more  sensitive
        monitors are being procured for  the  FY'86  field study.
   13.  Source Impact Study (Task 10)
             The impact of single wood  stoves on the  smoke  concentrations  monitored
        at the Raleigh site were to be  investigated  using tracer gases.   Logistical
        problems delayed  awarding a cooperative agreement with  Washington  State
        University until  after the  Raleigh site was  shut down.   Some preliminary
        laboratory testing of  the tracers  has begun  and numerical modeling performed,
        Field work is planned  to commence  with the FY'86 study.
C.  Albuquerque Field Measurements
     The objective of the Albuquerque Field  Study  was to apportion  the
impact of residential wood combustion and  mobile sources upon the mass
loading and mutagenic activity of the ambient fine aerosol.  To accomplish
these objectives, measurements were made of the fine particle mass  (from
a dichotomous sampler), volatilizable and  elemental  carbon  (from a  modified
Sierra dichotomous sampler), nitric acid/nitrate (from  a denuder-difference
sampler), fine particle sample for  bioassay (from  a  hi-vol  with an  Anderson
impactor), ^C/^C (from a hi-vol with  an  Sierra impactor), CO, S02> NOX and
light scattering (integrating  nephelometer).   Measurements  of  nitric acid
and nitrates were made to assist in determing the  sources of nitrate and
their potential contribution to any nitrogenous organics that may be present
in ambient samples collected during the study.  Samples were collected
from December 28, 1984 to February  20,  1985 at a residential  site impacted
                                    35

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by wood smoke and at a roadway site.  Aerosol  samples were collected over
twelve hour periods from 7 a.m. to 7 p.m. and  from 7 p.m.  to 7 a.m.   As
of September 1, analysis for fine particle mass and elemental  composition
was completed for both Albuquerque sites.  Volatilizable and elemental
carbon analysis was completed for the residential  wood burning site.  An
interim receptor modeling exercise was completed for the available data.
Bioassay of collected filters and Hc/12c measurements are planned for
the near future.  Volatilizable and elemental  carbon data  for the roadway
site will  also be completed.   Compilation of the continuous gas monitor data
is also expected soon.  Once the data are available, a receptor modeling
exercise will  be undertaken incorporating the  bioassay results.
D.  Special  Studies
     The status of several  special  areas of investigation  is described
below.   These efforts are intended to augment  the  field work by providing
understanding of the processes involved.
    1.   Laboratory Source Studies (Task 24)
         The objective of this effort was to determine the impact of six
    operational  parameters  upon the mass and chemical  composition of wood
    smoke  emissions.  Statistical  considerations forced a  revision of the
    original  plans and investigation of two parameters was deleted from the
    effort.   A test matrix  of 10 burns, designed to examine the impact  of.
    burnrate,  wood species, wood moisture content,  and wood loading  upon  the
    source emissions was completed  in June. Measurements  were made  using a
    Modified Method 5 (MM5) approach.   Analysis of  the total  weight  of  material
    collected  in the probe  and filter,  CO, C02, and 03 versus  burnrate, wood
    load,  and  wood moisture content have been  completed.   Analysis of the PAH
                                    36

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content and correlations with wood species are anticipated to be available
soon.
2.  Transformation Studies {Task 25)
     The investigation of the transformation of wood smoke emissions was
undertaken with three major goals: (1) to assess whether or not transformation
would occur with resultant changes in chemical composition and mutagenicity;
(2) to examine the atmospheric stability of potential signature compounds;
and (3) to evaluate the relative mutagenicity of the particulate and
gaseous products.  The goals were successfully met by a series of irradiations
which evaluated the chemical and mutagenic changes caused by transformations
under the conditions found in both remote, isolated air sheds and in
urban areas.  The nature and extent of chemical and mutagenic changes
were characterized for both the gas-phase and aerosol-bound species, and
reaction profiles of several potential tracer compounds were obtained.
A publication of the results demonstrating an overwhelming contribution by
the gaseous irradiation products to the total mutagenic burden is planned
as a journal article.  A draft copy of the proposed journal article is
attached to the Transformation Studies protocol in the Appendix B.
3.   FY'86/'87 Preparations (Questionnaire, Site Selection and Data Management)
     Two survey questionnaires have been developed for use in the planned
field program.   Preparation of the OMB clearance package for the questionnaire
is underway.  A  Site Selection Workshop was conducted which narrowed
the  potential locations for the  FY'86/'87 field effort to three cities:
Boise,  ID;  Reno, NV; or Albuquerque,  NM.  Visits to each city are planned
in September to  examine potential sampling sites in each area.  A data
handling and sample tracking system was implemented for the FY'85 program.
                                 37

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Problems have been identified and remedial  actions  are underway.   Imple-
mentation of a computerized data entry and  tracking system  is  planned.
                                38

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VII.  Technical  Results

          Listed below is summary of the major  technical  results  obtained  to

      date.
           1.   State of the art sampling and  analysis  procedures  have  been
               developed and implemented.   They are being  evaluated  and
               standardized for use in FY'86/'87 studies.


           2.   Sampling procedures for human  exposure  have been developed
               and evaluated in a pilot study.


           3.   Ambient, residential  and source  samples were taken simultaneously
               with equipment and procedures  developed to  provide comparable
               samples for chemical, physical and biological  characterization.


           4.   Wintertime sample sets were  collected for chemical  and
               bioassay analysis at two urban residential  sites impacted by
               wood burning emissions.


           5.   A mutagenic activity data base on the semi^volatile and particulate
               organic samples has been generated as part  of these studies.
               These data will be incorporated  into a  source  apportionment model
               which for the first time will  merge biological  and chemical/physical
               information.


           6.   Field and laboratory studies have both  shown that  greater mutagenicity
               was associated with the semi-volatile and volatile components than
               is associated with the particulate matter.


           7.   Initial receptor model calculations from Albuquerque  show that
               that residential wood combustion and mobile sources account for
               approximately 90% of the fine  particle  mass.   This result supports
               the earlier assumption that  these sources contribute  significantly
               to the mutagenic potential of  the ambient air.


          A more detailed description of results can be found  in  Appendix  B

      under each task.
                                          39

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UNITED STATES ENVIRONMENTAL PROTECTION AGENCY
            HEALTH EFFECTS RESEARCH LABORATORY
                 RESEARCH TRIANGLE PARK
                  NORTH CAROLINA 27711
     INTEGRATED AIR CANCER PROJECT

            "Mini Symposium"
                Agenda
            March 14, 1986
               Room 3906
Welcome Donald Ehreth
0/erview Obeli en Lewtas
Source Sampling and Analysis Ray Merrill
Residential and fear Source Ross Highsmith
Sampling and Analysis
Ambient Sampling and Analysis Ross Highsmith
Source Apportionment Chuck Lewis
Transformation " Larry Cupitt
Synopsis Larry Cupitt
Future Plans Jo ell en Lewtas
Panel Discussion Everyone
Lunch
Poster Session.
Adjorn
9:30
9:35
9:45
10:00
10:15
10:30
10:45
11:00
11:15
11:30
12:30
2:00
4:00
a.m.
a.m.
a.m.
a.m.
a.m.
a.m.
a.m.
a.m.
a.m.
a.m.
p.m.
p.m.
p .m.

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m

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                      INTEGRATED AIR CANCER PROJECT
                      "Mini Symposium" Participants
Steering Committee

     Joel 1 en Lewtas, KERL
     Chairman
     MD-68
     FTS 629-3849
     919-541-3849

Team Leaders

     Larry Cupitt, ASRL
     Study Design/Data Management/
     Interpretation Team
     MD-84
     FTS 629-2878
     919-541-2878

     Ray Merrill, AEERL
     Analysis Team
     MO-62
     FTS 629-2558
     919 541-2558
Robert Stevens, ASRL
MD-47
FTS 629-3156
919-541-3156
Charles Rodes, EMSL
Sampling Team
MD-56
FTS 629-3079
919 541-3079
Other Participants

     Barbara Andon, EHRT
     Project Coordinator
     MD-69
     FTS 629-7532
     919 541-7532

     Ross Highsmith,  EMSL
     MD-56
     FTS 629-7828
     919 541-7828
Chuck Lewis, ASRL
MD-47
FTS 629-3154
919 541-3154

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 The Integrated Air Cancer Project
        Project Participants
U.S. Environmental  Protection Agency
 Research Triangle Park, NC   27711

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STEERING COMMITTEE
     Joel lien Lewtas, HERL (Chairman)
     MD-68
     FTS 629-3849
     919-541-3849

     Jack Puzak, EMSL
     MD-75
     FTS 629-2106
     919-541-2106

     Robert Stevens, ASRL
     MD-47
     FTS 629-3156
     919-541-3156

     Jim Dorsey, AEERL
     MD-62
     FTS 629-2509
     919-541-2509
TEAM LEADERS
     Larry Cupitt,  ASRL (Study  Design/Data  Management/Interpretation)
     MD-84
     FTS 629-2878
     919-541-2878

     Ray Merrill, AEERL (Analysis)
     MD-62
     FTS 629-2558
     919 541-2558

     Charles  Rodes,  EMSL (Sampling)
     MD-56
     FTS 629-3079
     919-541-3079
 PROJECT COORDINATOR
     Barbara  Andon, EHRT
     MD-69
     FTS  629-7532
     919  541-7532

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RESEARCHERS
     Bill  Barnard,  EMSL
     MD-77B
     FTS 629-2205
     919-541-2205

     Ralph Baumgardner,  ASRL
     MO-47
     FTS 629-4625
     919-541-4625

     Rudy  Boksleiter,  EMSL
     MD-77
     FTS 629-4746
     919-541-4746

     Bob Burton,  EMSL
     MD-76
     FTS 629-3078
     919-541-3078

     Larry Claxton, HERL
     MD-68
     FTS 629-2329
     919 541-2329

     Howard Crist, EMSL
     MD-77B
     FTS 629-2723
     919-541-2723

     Ron Drago, EMSL
     MD-76
     FTS 629-3078
     919-541-3078

     Bert  Eskridge, ASRL
     MD-80
     FTS 629-4551
     919 541-4451

     Peter Finkelstein, ASRL
     MD-80
     FTS 629-4551
     919-541-4551

     Bruce Harris, AEERL
     MD-62
     FTS 629-7807
    919-541-7807
 Tom  Hart!age,  EMSL
 MD-76
 FTS  629-3008
 919-541-3008

 Ross High smith,  EMSL
 MD-56
 FTS  629-7828
 919  541-7828

 Leon King, HERL
 MD-68
 FTS  629-3932
 919-541-3932

 Tom  Lawless, EMSL
 MD-56
 FTS  629-2291
 919-541-2991

 Bob  Lewis, EMSL
 MD-44
 FTS  629-3065
 919  541-3065

 Chuck Lewis, ASRL
 MD-47
 FTS  629-3154
 919  541-3154

 Tom  Lumpkin, EMSL
 MD-76
 FTS  629-3611
 919  541-3611

 David Mage, EMSL
 MD-56
 FTS  629-3184
 919  541-3184

 Bob McCrillis, AEERL
 MD-65
 FTS 629-2733
919 629-2733

 Judy Mumford,  HERL
MD-68
 FTS 629-3095
919 541-3095

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 Don Scott,  EMSL
 MD-78A
 FTS 629-7948
 919 541-7948

 John Sigsby, ASRL
 MD-46
 FTS 629-3037
 919-541-3037

 Si 1 vestre Tejada, ASRL
 MD-59
 FTS 629-2323
 919 541-2323

 Randy Watts, HERL
 MD-68
 FTS 629-2491
 919 541-2491

 Nancy Wilson, EMSL
 MD-44
 FTS 629-4723
 919 541-4723

Roy Zweidinger,  ASRL
MD-59
FTS 629-2323
919 541-2323

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U.S. Enrlronmental Protection
Library, Room 2404
-401 M Street, S.W.
Washington, DO   t0480

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